Bombardment of aluminum-27 by alpha particles produces phosphorous-30 and one other particle. Write the nuclear equation and identify the other particle. 27 13 Al + a He 2 4 30 15 P + 1 0 n Plutonium-239 can be produced by bombarding uranium-238 with alpha particles. How many neutrons will be produced as a by product of each reaction. Write the nuclear equation for this reaction. 238 92 U + 4 2 He 239 94 Pu + 1 ?0n 4 Unstable Isotopes and + or Excited nucleus Kelter, Carr, Scott, Chemistry A World of Choices 1999, page 439 Stable nucleus Energy Particles Radiation Unstable Nucleus Zumdahl, Zumdahl, DeCoste, World of Chemistry 2002, page 620 Fissionable U-235 Fission Process Nucleus Neutron Zumdahl, Zumdahl, DeCoste, World of Chemistry 2002, page 620 Two neutrons from fission Stages of Fission First stage: 1 fission Kelter, Carr, Scott, Chemistry A World of Choices 1999, page 454 Second stage: 2 fissions Third stage: 4 fissions Nuclear Power Plants map: Nuclear Energy Institute Energy Sources in the United States 100 91 Percent 80 71 70 60 50 40 40 20 58 50 21 9 26 20 5 10 3 21 26 16 10 0 1850 Wood 1900 Coal Zumdahl, Zumdahl, DeCoste, World of Chemistry 2002, page 307 1940 1980 Petroleum / natural gas 1990 2005 Hydro and nuclear Energy Sources in the United States 100 91 Percent 80 60 50 40 20 19 19 9 7 3 3 0 2005 1850 Coal Petroleum Nuclear Hydroelectric natural gas Renewable (biomass, geothermal, solar, wind) Source: US Energy Information Administration (2005 Electricity Generation) Coal Burning Power Plant Copyright © 2007 Pearson Benjamin Cummings. All rights reserved. Nuclear Power Plant Zumdahl, Zumdahl, DeCoste, World of Chemistry 2002, page 621 Reactor Core Hot coolant Control rods of neutron-absorbing substance Uranium in fuel cylinders Incoming coolant Zumdahl, Zumdahl, DeCoste, World of Chemistry 2002, page 622 Nuclear Power Plant Production of heat Copyright © 2006 Pearson Benjamin Cummings. All rights reserved. Production of electricity Chant of the Radioactive Workers We're not afraid of the alpha ray. A sheet of paper will keep it away! A beta ray needs much more care, Place sheets of metal here and there. And as for the powerful gamma ray (Pay careful heed to what we say) Unless you wish to spend weeks in bed Take cover behind thick slabs of lead! Fast neutrons pass through everything. Wax slabs remove their nasty sting. These slow them down, and even a moron Knows they can be absorbed by boron. Remember, remember all that we've said, Because it's no use remembering when you're dead. Inside a nuclear power plant. Shaft Surface deposits Nuclear Waste Disposal Aquifier River Interbed rock layer Host rock formation Repository Waste package Interbed rock layer Aquifier Bedrock Zumdahl, Zumdahl, DeCoste, World of Chemistry 2002, page 626 Waste form Half-Life 20 g 10 g 5g Start after 1 half-life Dorin, Demmin, Gabel, Chemistry The Study of Matter 3rd Edition, page 757 after 2 half-lives 2.5 g after 3 half-lives b emissions 131 53 I 89.9% 7.3% Half-Life 0.500 mg 1.00 mg 131 53 I 0.750 mg Xe 0.875 mg 0.500 mg 131 53 0.00 days I 0.250 mg 8.02 days 131 I 53 Dorin, Demmin, Gabel, Chemistry The Study of Matter 3rd Edition, page 757 131 Xe 54 0.125 mg 24.06 days 16.04 days + Xe* g emissions 131 54 131 54 131 54 b -1 0 + g Xe Half-life of Radiation Radioisotope remaining (%) Initial amount of radioisotope 100 After 1 half-life After 2 half-lives 50 After 3 half-lives t1/2 25 t1/2 12.5 t1/2 0 1 2 3 Number of half-lives 4 Half-Life Plot Amount of Iodine-131 (g) 20 Half-life of iodine-131 is 8 days 15 1 half-life 10 2 half-lives 5 3 half-lives 4 half-lives etc… 0 0 8 16 24 Time (days) Timberlake, Chemistry 7th Edition, page 104 32 40 48 56 Half-Life of Isotopes Half-Life and Radiation of Some Naturally Occurring Radioisotopes Isotope Half-Live Radiation emitted Carbon-14 5.73 x 103 years b Potassium-40 1.25 x 109 years b, g Radon-222 3.8 days a Radium-226 1.6 x 103 years a, g Thorium-230 7.54 x 104 years a, g Thorium-234 24.1 days b, g Uranium-235 7.0 x 108 years a, g Uranium-238 4.46 x 109 years a Half-life (t½) / 1 Calcium Ratio of Remaining Potassium-40 Atoms to Original Potassium-40 Atoms Argon 1/ 4 1/ 8 1/ 16 – Time required for half the atoms of a radioactive nuclide to decay. – Shorter half-life = less stable. 1/1 Potassium 2 Newly formed rock 1/2 1/4 1/8 1/16 0 0 1 half-life 1.3 2 half-lives 2.6 3 half-lives 3.9 Time (billions of years) 4 half-lives 5.2 Half-life (t½) Potassium Argon Calcium Ratio of Remaining Potassium-40 Atoms to Original Potassium-40 Atoms – Time required for half the atoms of a radioactive nuclide to decay. – Shorter half-life = less stable. 1/1 Newly formed rock 1/2 1/4 1/8 1/16 0 0 1 half-life 1.3 2 half-lives 2.6 3 half-lives 3.9 Time (billions of years) 4 half-lives 5.2 How Much Remains? After one half-life, 1 2 of the original atoms remain. After two half-lives, ½ x ½ = 1/(22) = 1 4 of the original atoms remain. After three half-life, ½ x ½ x ½ = 1/(23) = 1 8 of the original atoms remain. After four half-life, ½ x ½ x ½ x ½ = 1/(24) = 1 16 of the original atoms remain. After five half-life, ½ x ½ x ½ x ½ x ½ = 1/(25) = 1 32 of the original atoms remain. After six half-life, ½ x ½ x ½ x ½ x ½ x ½ = 1/(26) = 1 64 of the original atoms remain. 1 2 Surviving “parent” isotopes Beginning 1 half-life Accumulating “daughter” isotopes 1 4 1 8 2 half-lives 3 half-lives 1 16 4 half-lives 1 32 5 half-lives 1 64 6 half-lives 1 128 7 half-lives 1. A small piece of fossil is burned in a special furnace. 2. The burning creates carbon dioxide gas comprised of carbon-12 isotopes and carbon-14 isotopes. Nitrogen Stable C-12 isotope Decaying C-14 isotope 3. As the carbon14 decays into nitrogen-14, it emits an electron. 4. A radiation counter records the number of electrons emitted. Note: Not to scale. SOURCE: Collaboration for NDT Education MATT PERRY / Union-Tribune Electron The iodine-131 nuclide has a half-life of 8 days. If you originally have a 625-g sample, after 2 months you will have approximately? a. b. c. d. e. 40 g 20 g 10 g 5g less than 1 g N = No(1/2)n N = amount remaining No = original amount n = # of half-lives N = (625 g)(1/2)7.5 N = 3.45 g Data Table: Half-life Decay ~ Amount 625 g 312 g 156 g 78 g 39 g 20 g 10 g 5g 2.5 g 1.25 g Time 0d 8d 16 d 24 d 32 d 40 d 48 d 56 d 64 d 72 d # Half-Life 0 1 2 3 4 5 6 7 8 9 Assume 30 days = 1 month 60 days = 7.5 half-lives 8 days Given that the half-life of carbon-14 is 5730 years, consider a sample of fossilized wood that, when alive, would have contained 24 g of carbon-14. It now contains 1.5 g of carbon-14. How old is the sample? Data Table: Half-life Decay ln N = - k t No t1/2 = 5730 y = ln 2 0.693 k Amount Time 24 g 12 g 6g 3g 1.5 g 0y 5,730 y 11,460 y 17,190 y 22,920 y # Half-Life 0 1 2 3 4 0.693 k k = 1.209 x 10-4 ln 1.5 g = - (1.209x10-4) t 24 g t = 22,933 years Half-Life Practice Calculations • The half-life of carbon-14 is 5730 years. If a sample originally contained 3.36 g of C-14, how much is present after 22,920 years? 0.21 g C-14 • Gold-191 has a half-life of 12.4 hours. After one day and 13.2 hours, 10.6 g of gold-19 remains in a sample. How much gold-191 was originally present in the sample? 84.8 g Au-191 There are 3.29 g of iodine-126 remaining in a sample originally containing 26.3 g of iodine-126. The half-life of iodine-126 is 13 days. How old is the sample? 39 days old • • A sample that originally contained 2.5 g of rubidium-87 now contains 1.25 g. The half-life of rubidium-87 is 6 x 1010 years. How old is the sample? Is this possible? Why or why not? 6 x 1010 years (60,000,000,000 billions years old) What is the age of Earth??? Demo: Try to cut a string in half seven times (if it begins your arm’s length). The half-life of carbon-14 is 5730 years. If a sample originally contained 3.36 g of C-14, how much is present after 22,920 years? Data Table: Half-life Decay t1/2 = 5730 years n = Amount 22,920 years 5,730 years 3.36 g 0y 1.68 g 5,730 y 0.84 g 11,460 y 0.42 g 17,190 y 0.21 g 22,920 y n = 4 half-lives (# of half-lives)(half-life) = age of sample (4 half-lives)(5730 years) = age of sample 22,920 years Time # Half-Life 0 1 2 3 4 Uranium Radioactive Decay 238 234 230 Mass number 226 222 a 4.5 x 109 y 24 d 1.2 m 2.5 x 105 y 8.0 x 104 y 1600 y 3.8 d 3.0 m 27 m 160 ms 5.0 d 138 d stable Th-234 b a U-238 Pa-234 b U-234 a Th-230 Ra-226 a Rn-222 a 218 Po-218 a 214 Pb-214 b 210 Pb-210 206 Pb-206 b 81 82 Bi-214 b Po-214 a Bi-210 b Po-210 a 83 84 85 86 87 Atomic number 88 89 90 91 92 140 Nuclear Stability 130 120 110 100 Decay will occur in such a way as to return a nucleus to the band (line) of stability. Neutrons (N) 90 80 70 60 50 40 30 20 10 0 10 20 30 40 50 Protons (Z) 60 70 80 90 Copyright © 2007 Pearson Benjamin Cummings. All rights reserved. 160 150 Band of Stability 140 130 120 Number of neutrons 110 n= p 100 90 80 70 60 50 40 Stable nuclides Naturally occurring radioactive nuclides Other known nuclides 30 20 10 0 10 20 30 40 50 60 70 80 Number of protons 90 100 110 140 a decay 209 83 Bi N 1.52 Z 130 120 184 74 W N 1.49 Z 110 100 Neutrons (N) 90 b decay 80 107 47 Ag 70 N 1.28 Z 60 50 N 1 Z 56 26 Fe 40 N 1.15 Z 30 positron emission and/or electron capture 20 20 10 Ne N 1.0 Z 10 0 10 20 30 40 50 Protons (Z) 60 70 80 90 140 a decay 209 83 Bi 130 N 1.52 Z 120 184 74 W 110 N 1.49 Z Nuclear Stability 100 90 Decay will occur in such a way as to return a nucleus to the band (line) of stability. Neutrons (N) b decay 80 107 47 Ag 70 N 1.28 Z 60 50 N 1 Z 56 26 Fe 40 N 1.15 Z 30 positron emission and/or electron capture 20 20 10 Ne 10 N 1.0 Z 0 10 20 30 40 50 Protons (Z) 60 70 80 90 Half-Lives of Some Isotopes of Carbon Nuclide Half-Life Carbon-9 Carbon-10 Carbon-11 Carbon-12 Carbon-13 Carbon-14 Carbon-15 Carbon-16 0.127 s 19.3 s 10.3 m Stable Stable 5715 y 2.45 s 0.75 s Enlargement of part of band of stability around Neon 23 10 23 10 Ne moves into band of 22 10 stability by beta decay. 23 10 Ne 19 10 0 -1b by positron emission. Electron capture would also move 199 F into the band of stability. 10b Ne 23 11Na 21 10 Ne Ne moves into band of stability 19 10 Ne Ne 19 9 F 20 10 Ne 19 9F 19 10 Umland and Bellama, General Chemistry 2nd Edition, page 773 Ne 23 11 Na Number of protons Effects of Radioactive Emissions on Proton and Neutrons Loss of 4 He 2 Loss of 0 e -1 Loss of 0 e or 1 electron capture Number of protons Nuclear Decay “absorption”, “bombardment” vs. “production”, “emission” 223 88 4 2 a 2+ 87 37 4 2 Ra 14 7 + a 2+ 17 8 N 0 -1 b Rb 219 86 + O + 87 38 + Alpha 4 2 a 1 1 Sr Beta 2+ 0 -1 b neutron 1 0 n 2 1 Rn H H 2 1 + H 14 6 + 3 1 2 1 4 2 H 4 2 H 0 -1 b C Positron 0 +1 + He + He 17 7 N Gamma b 0 0 proton 1 1 H 1+ g 1 0 n Units Used in Measurement of Radioactivity Units Measurements Curie (C) radioactive decay Becquerel (Bq) radioactive decay Roentgens (R) exposure to ionizing radiation Rad (rad) energy absorption caused by ionizing radiation Rem (rem) biological effect of the absorbed dose in humans Effects of Instantaneous Whole-Body Radiation Doses on People Dose, Sv (rem) Effect Alexander Litvinenko >10 (1000) Death within 24 h from destruction of the neurological system. 7.5 (750) Death within 4-30 d from gastrointestinal bleeding. 1.5 – 7.5 (150 – 750) Intensive hospital care required for survival. At the higher end of range, death through infection resulting from destruction of white-blood cell-forming organs usually takes place 4 – 8 weeks after accident. Those surviving this period usually recover. < 0.5 (50) Only proven effect is decrease in white blood cell count. The intensity of radiation is proportional to 1/d2, where d is the distance from the source. Alpha, Beta, Positron Emission Examples of Nuclear Decay Processes b- emission (beta) a emission (alpha) 238 92 U 42 He 234 90 Th 42 He 226 88 Ra 42 He 222 86 230 90 226 88 Th Ra Rn 27 12 Mg -01e 14 8 O 01e 14 7 Cl 32 17 Cl 01e 32 16 Ca 14 8 O 01e 14 7 27 13 S -01e 35 17 K -01e 40 20 35 16 40 19 b emission (positron) Al N S N Although beta emission involves electrons, those electrons come from the nucleus. Within the nucleus, a neutron decays into a proton and an electron. The electron is emitted, leaving behind a proton to replace the neutron, thus transforming the element. (A neutrino is also produced and emitted in the process.) Herron, Frank, Sarquis, Sarquis, Schrader, Kulka, Chemistry, Heath Publishing,1996, page 275 Nuclear Reactions First recognized natural transmutation of an element (Rutherford and Soddy, 1902) 226 88 Ra α 4 2 222 86 Rn First artificial transmutation of an element (Rutherford, 1919) 14 7 N a 4 2 O ? 17 8 1 1 p Discovery of the neutron (Chadwick, 1932) 9 4 Be a 4 2 12 6 C ?n 1 0 Discovery of nuclear fission (Otto Hahn and Fritz Strassman, 1939) 235 92 U n Bailar, Chemistry, pg 361 1 0 Ba 141 56 92 36 Kr 3 n 1 0 Preparation of Transuranium Elements Atomic Number Name Year Symbol Discovered 93 Neptunium Np 94 Plutonium Pu 1940 1940 Reaction 1 U n 92 0 238 2 U H 92 1 238 Np 93 238 Americium Am 1944 239 96 Curium Cm 1945 239 97 Berkelium Bk 1949 241 Cf Ralph A. Burns, Fundamentals of Chemistry 1999, page 553 1950 0 Pu e 94 -1 238 0 Am e 95 -1 240 4 Pu He 94 2 4 Am He 95 2 4 Cm He 96 2 242 Californium 1 Np 2 n 93 0 238 1 Pu n 94 0 95 98 0 Np e 93 -1 239 1 Cm n 96 0 242 1 Bk 2 n 97 0 243 1 Cf n 98 0 245 Preparation of Transuranium Elements Atomic Number Name Year Symbol Discovered 93 Neptunium Np 94 Plutonium Pu 1940 1940 Reaction 1 U n 92 0 238 2 U H 92 1 238 Np 93 238 Americium Am 1944 239 96 Curium Cm 1945 239 97 Berkelium Bk 1949 241 Cf Ralph A. Burns, Fundamentals of Chemistry 1999, page 553 1950 0 Pu e 94 -1 238 0 Am e 95 -1 240 4 Pu He 94 2 4 Am He 95 2 4 Cm He 96 2 242 Californium 1 Np 2 n 93 0 238 1 Pu n 94 0 95 98 0 Np e 93 -1 239 1 Cm n 96 0 242 1 Bk 2 n 97 0 243 1 Cf n 98 0 245 Additional Transuranium Elements 99 100 101 102 103 104 105 106 107 108 109 110 111 112 114 116 118 Einsteinium Fermium Mendelevium Nobelium Lawrencium Rutherfordium Dubnium Seaborgium Bohrium Hassium Meitnerium Darmstadtium Unununium Ununbium Es Fm Md Nb Lr Rf Db Sg Bh Hs Mt Ds Uun Uub Uuq 1952 1952 1955 1958 1961 1964 1970 1974 1981 1984 1988 1994 1994 1996 1999 2002 2006 (Russia) (Russia)