Supplementary information for: Permeability changes in experimentally fractured granite during and after frictional sliding Wataru Tanikawa a,* Osamu Tadai b Hideki Mukoyoshi b,c a Kochi Institute for Core Sample Research, Japan Agency for Marine-Earth Science and Technology, 200, Monobe-otsu, Nankoku, Kochi 783-8502, Japan b Marine Works Japan Ltd., 200, Monobe-otsu, Nankoku, Kochi 783-8502, Japan c Faculty of Education and Integrated Arts and Sciences, Waseda University, 1-6-1, Nishiwaseda, Shinjuku, Tokyo 169-8050, Japan *Corresponding author Address: Kochi Institute for Core Sample Research, Japan Agency for Marine-Earth Science and Technology, Nankoku 783-8502, Japan Tel: +81-88-878-2203; fax: +81-88-878-2192 E-mail: tanikawa@jamstec.go.jp Supplementary Information item 1: Mineral composition of Aji granite The mineral composition of Aji granite used in our friction tests is listed in Table S1. Supplementary Information item 2: Calculation of temperature and gas viscosity at slip plane during friction tests We used numerical modeling to calculate the temperature distribution in specimens during frictional sliding. We assumed an axisymmetric two-dimensional problem (Fig. S1a) and used a computer program based on the finite-element method developed by Kuroda (2001). In our modeling the half-specimen on one side of the slip plane was represented by 600 elements, each 0.5 × 0.5 mm (Fig. S1b). The time step we used was such that temperature changes were less than 1 K for each time step. Temperature on the top of the specimen (boundary A, Fig. S1b) was fixed to room temperature in our modeling. Heat transfer to the surrounding atmosphere from the rock specimen (boundary B, Fig. S1b) followed Newton’s law of cooling, which states that the rate of heat loss from the rock specimen is proportional to the difference between the surface temperature and the surrounding temperature (room temperature in our model). This relationship is qs = α(T – Ts), (S1) where qs is the heat flux per unit are to the surroundings, α is the heat transfer coefficient, T is the temperature on the rock surface, and Ts is the surrounding temperature. We assumed a heat transfer coefficient of 10 W/m2 K. The heat flux per unit area of slip surface generated by friction at boundary C (Fig. S1b), qf, is described in terms of shear stress and slip velocity as qf = σf ×v/2, (S2) where σf and v are the shear stress and slip velocity, respectively. We assumed constant shear stress on the surface during sliding to simplify the model setting, even though the shear stress changes with slip in our friction test. We used 1.28 MPa of shear stress in our model based on the average friction coefficient of 0.64 in our friction tests. The thermal properties of Aji granite, listed in Table S2, were measured by using a commercial instrument (TPS1500, Hot Disk AB Ltd., Sweden) and used in the model calculation. Assuming that shear stress is constant across the entire slip surface, heat flux is greatest at the external edge of the specimen. As the rate of heating was not uniform across the slip surface, the temperature increased radially from the center of the slip surface and deviated markedly from the average temperature, especially for high-velocity friction tests (Figs. S1c and S1d). The lowest and highest temperature rise across the slip surface were observed in the internal and external edges of the specimen, respectively, at all velocities (Fig. S1d). The deviation of temperature at the slip surface increases with slip velocity, and the deviation is greater than 30 K for 97 mm/s of slip velocity. The deviation of temperature induces the deviation of gas viscosity due to the temperature dependence on the viscosity described in equation (3). According to equation (3) the deviation of viscosity reaches 6% for a friction test at 97 mm/s slip velocity, and gas viscosity is greatest at the external edge of the specimen. For lower slip rates (< 9.7 mm/s of slip velocity), though, the deviation is less than 1%. Supplementary Information item 3: Reproducibility of our results The experimental results for an additional series of friction tests using a different set of cylindrical specimens from the same Aji granite block are shown in Figs. S2 to S4. Sample sizes and experimental conditions for this series were almost the same as those for the experiment described in this paper, although the sequence of slip velocities was different (Fig. S3a). Normal stress was applied at 2 MPa with 1.5 m of slip displacement for a series of friction tests. We pre-rotated 53 m at 5 mm/s slip velocity and 2 MPa of normal stress before conducting friction tests. Normal stress dependence on the permeability of this specimen (Fig. S2a) was similar to that of the specimen discussed in the main text. Even though the data were fewer than those for the main test, transmissivity during sliding was proportional to the friction coefficient (Fig. S4b). The overall trends of slip velocity dependencies (Fig. S4a to S4c) and initial transmissivity dependencies (Fig. S4d to S4f) were similar to those presented in the main text. These additional data confirm the reproducibility of our results. Supplementary Information item 4: The thermomechanical properties of Aji granite were measured by a Thermomechanical Analyzer (TMA-60, Shimazu Corporation, Japan), and the calculated thermal property was used to estimate the thermal stress from the heating test. We applied 0.1 MPa of normal stress during the thermomechanical test. References Everl DD (2003) User’s Guide to RockJock: A Program for Determining Quantitative Mineralogy from Powder X-Ray Diffraction Data. USGS Open-File Report, 2003-78. Kuroda H (2001) Two-Dimensional Heat Flow Analysis Program Using Finite Element Method, 255 pp., CQ, Tokyo (in Japanese). Captions Supplementary Fig. S1. Model calculation of temperature and viscosity change during friction tests. (a) Illustration of the area used for modeling of the temperature distribution within specimens during friction tests. (b) Detail of the area modeled showing mesh geometry and boundaries used. (c) Snapshot of the modeled thermal distribution for an Aji granite specimen after 1.5 m slip displacement for an average slip rate of 97 mm/s (= 100 rpm). (d) Snapshot of temperature distribution of the slip surface after 1.5 m slip displacement at various slip rates. (e) Change of maximum temperature difference along slip surface during shearing at various slip rates. (f) Change of maximum deviation of gas viscosity on slip surface at various slip rates. Constant shear stress of 1.28 MPa and constant slip ratio were assumed during frictional sliding. Supplementary Fig. S2 (a) Permeability as a function of normal stress for an intact specimen and for simulated fault rocks before and after slip. Loading and unloading were applied to the same samples. (b) Gas flow rate, measured in the flow line before entry to the shearing apparatus, as a function of differential pore pressure (Pu2 – Pd2)/Pu. Inset graph is a magnified view at low flow rate. Supplementary Fig. S3. (a) Friction coefficient and (b) slip velocity as a function of cumulative slip displacement for a series of successive friction tests performed on the second pair of hollow granite specimens. (c) Average coefficient of friction during slip displacement of 1.5 m as a function of slip velocity. (d) Average friction coefficient during slip as a function of average fracture transmissivity during slip (T1) for different slip velocities. Supplementary Fig. S4. Relative fracture transmissivity (a)–(c) as a function of slip velocity and (d)–(e) as a function of initial transmissivity. T0, initial fracture transmissivity; T1, average fracture transmissivity during slip; T2, fracture transmissivity after slip; T3, fracture transmissivity approaching steady state 15 min after slip. Supplementary Fig. S5. Thermal expansion of Aji granite during heating. Supplementary Table S1. Mineral composition of Aji granite (%) determined using the RockJock program (Everl, 2003). Supplementary Table S2. Thermal and physical properties used for numerical modeling of the temperature distribution during friction tests.