Tailoring Spin Dynamic Properties of Sputtered NiFe Thin Films with Different Seed Layers Deepika Jhajhria*, Nilamani Behera, D K Pandya, Sujeet Chaudhary Thin Film Laboratory, Indian Institute of Technology Delhi, New Delhi 110016 Corresponding author’s e-mail: deepika.jhajhria@gmail.com, Tel.: +91-7503733805; Fax: +91-11-26581114 * 1400 Resonance Field (Oe) Abstract We studied the tailoring of magnetization dynamics in 10 nm thick NiFe thin film with different seed layers (Ta, Cu, Ru). Damping can be effectively tuned by choice of seed layer, while the static magnetic properties remain relatively constant. Smallest FMR line width was obtained for Ta seed layer implying it is suitable for NiFe based spin current devices. 1200 NiFe 1000 Ta/NiFe Cu/NiFe 800 Ru/NiFe 600 400 200 (a) 0 2 3 4 5 6 7 8 9 10 11 Introduction The magnetization dynamics of soft magnetic thin films have been a subject of recent interest for its applications in high frequency and spin current based devices and it is often desirable to tailor the damping behavior of magnetic relaxation. In this regard we used different seed layers (Ta, Cu, Ru) for tuning the magnetization relaxation and Gilbert damping in NiFe thin films. Experimental NiFe films were deposited on seeded Si (100) substrate in presence of magnetic field of 600 Oe at room temperature by dc magnetron sputtering. The thickness of NiFe film was kept at 10nm and that of seed layer at 5nm. Ferromagnetic resonance (FMR) signal was recorded in 3 - 10 GHz range using a vector network analyzer (VNA) and employing a coplanar waveguide. Static magnetic measurements were done using MOKE (Magneto-Optic Kerr Effect) experimental setup. Structural and surface morphology studies have been carried out using X-ray diffraction (XRD) and Atomic force microscopy (AFM) respectively. 28 26 24 22 20 18 16 14 12 10 8 6 4 NiFe Damping Constant () Keywords: Magnetization dynamics, seed layer, damping, FMR line width, spin current. FMR linewidth (Oe) Frequency(GHz) Ta/NiFe Cu/NiFe Ru/NiFe (b) 2 3 4 5 6 7 8 9 Frequency (GHz) 10 11 0.007 0.006 0.005 0.004 0.003 (c) 0.002 NiFe Ta/NiFe Cu/NiFe Ru/NiFe Seed Layers Fig. 1: (a) Frequency dependence of resonance fields, (b) FMR line width ΔH as a function of frequency, (c) Damping constant for different seed layers As seen from Fig. 1c the damping constant α was least at 0.0028 for sample with Ta seed layer and highest at 0.007 for Ru seed layer. However, α (~0.0045) is comparable for single layered NiFe thin film and the one with Cu seed layer. Correlation of interface roughness and microstructure with the damping constant will be presented at the conference. Conclusions Magnetic relaxation in NiFe thin films can be tuned in wide range using different seed layers via different interfacial effects and microstructure. Ta seed layer results in lowest line width and may benefit various spin current based magnetic devices. References Results Fitting of frequency dependence of resonance field H res data (Fig. 1a) using Kittel equation showed that effective magnetization does not change much with different seed layers. The intrinsic Gilbert damping constant α was determined from the FMR line width ΔH (Fig. 1b) using the relation of H 2 H 0 3 [1] Sangita S. Kalarickal, Pavol Krivosik, Mingzhong Wu, Carl E. Patton, Michael L. Schneider, Pavel Kabos, T. J. Silva, and John P. Nibarger, “Ferromagnetic resonance linewidth in metallic thin films: Comparison of measurement Methods”, J. Appl. Phys,. 99, 093909 (2006). [2] Lichuan Jin, Huaiwu Zhang, Xiaoli Tang, Feiming Bai, and Zhiyong Zhong, “Effects of ruthenium seed layer on the microstructure and spin dynamics of thin permalloy films”, J. Appl. Phys., 113, 053902 (2013).