1 EXPERIMENTAL STUDY OF THE LASER-ACTIVE ELEMENT CHARACTERISTICS FOR HIGH-POWER NUCLEAR REACTOR-PUMPED LASER SYSTEM E.D.Poletaev, A.F.Gamaly, P.P. Dyachenko, V.N.Smolsky, M.Yu.Zaitsev, V.R.Agafonov, Yu.A. Dyuzhov, A.V.Gulevich, B.V.Kachanov, O.F.Kukharchuk Institute for Physics and Power Engineering, 1,Bondarenko Sq., Obninsk 249020,Russia Abstract. The results of experimental studying characteristics of the laser-active element with the Ar-Xe mixture on the 1.73 m transition of Xe atoms for the high-power pulsed reactorpumped laser system are presented . The experiments have been carried out on the BARS-6 two-core pulsed reactor using a special-purpose setup that is also described. INTRODUCTION One of the promising directions in a nuclear energy utilization is the development of the nuclear pumped lasers. At present time , a pilot model of highpower laser system based on optical quantum nuclear-power amplifier (OKUYAN) is under construction at the Institute of Physics and Power Engineering [1]. The main components of the laser module for this system are the laser-active elements (LAELs) with Ar-Xe mixture. The Ar-Xe mixture is used as a working medium for LAEL because of its detail studying under conditions of nuclear pumping [2-5]. Applying this mixture, nuclear-pumped lasers have been realized on the various transitions of Xe atoms in the microwave range with rather high output parameters - specific energy is up to 1 J/l, and efficiency of nuclear-to-laser energy conversion is up to 3.5 %. This paper is devoted to an experimental study of laser characteristics for the accepted variant of the Ar-Xe LAEL which will be applied in laser module of OKUYAN. EXPERIMENTAL SETUP Proc. Intern. Conf. ICENES’98, 1998 - 1998 Institute for Physics and Power Engineering, Technical Physics Laboratory http://www-tpl.ippe.obninsk.ru E-mail: kuh@ippe.obninsk.ru 2 The experiments have been carried out on the BARS-6 two-core pulsed reactor using a special-purpose setup for studies of nuclear-pumped lasers. Schematic layout of experimental setup is shown in Fig. 1. The laser-active element placed into the cylindrical polyethylene neutron moderator, was arranged near reactor cores at a distance of 68 cm. The LAEL is a thin walled stainless steel tube with outer diameter 49 mm and length 2500 mm with an internal 5 m -thick metal uranium-235 coating. The windows with a dielectric antireflection coating for the 1.73 m quartz optical wavelength were mounted on both ends of the LAEL. 1 2 5 6 4 3 7 9 8 6 6 6 6 16 12 13 14 15 He-Ne 6 11 10 10 Fig.1. Schematic layout of the experimental setup. 1 - nuclear reactor cores, 2 - neutron moderator, 3 - LAEL, 4, 5 - cavity mirrors, 6 - deflecting mirrors, 7, 10,11 - beamsplitters, 8 - lens, 9 - calorimeter, 12, 13, 14 - photoreceivers, 15 - alignment laser, 16 - shielding wall A vacuum pump, a filling system, a circulation line including the silicagel, titanium and sodium traps, and a bellows pump for continuos purification of Ar-Xe medium, were attached to the LAEL. The purification control was carried out by measuring intensity of radiation for bands of both the impurity molecules (N 2 , OH, Proc. Intern. Conf. ICENES’98, 1998 - 1998 Institute for Physics and Power Engineering, Technical Physics Laboratory http://www-tpl.ippe.obninsk.ru E-mail: kuh@ippe.obninsk.ru 3 etc.) and the heteronuclear ion of Ar+Xe under excitation by -particles. For this purpose a cell with -source (Pu-238) was included to a circulation line . The excited spectrum was measured by the MDR-6 monochromator . The optical scheme of experiment has two channels formed by beamsplitter (7) which is a mirror with a dielectric coating on 1.73 m having a reflection coefficient equal to 96 %. Therefore , the most part of laser beam entered a thermocouple calorimeter to detect the laser pulse energy. Another part of laser beam was directed by the plate aluminum mirrors to a measuring system including a set of various photoreceivers for registration of the laser pulse time shape. The alignment of optical system was carried out using a He-Ne laser. The copper and tungsten activation indicators placed into neutron moderator near surface of the LAEL were used to measure the thermal neutron fluence distribution along the LAEL. The time dependence of thermal neutron pumping pulse in moderator was measured by vacuum fission chamber with 235 U. In this experiment, the pressure jump in the LAEL was measured during the pumping pulse using the DMI-2 transducer in order to determinate the energy deposition of fission fragments into the gas. RESULTS AND DISCUSSION Measurement of the LAEL laser characteristics have been carried out in a free oscillation mode. Results of such experiments allow to obtain both optimal ratio and total pressure of laser mixture, and also so important parameters of active medium as an unsaturated gain, a saturation intensity and an efficiency of the nuclear-to-inversion energy conversion. A typical time-dependent laser oscillation on the 1.73 m transition is shown in Fig.2 together with a thermal neutron pumping pulse. The total laser output energy measured by calorimeter was about 1 J at optimal conditions. These data were used to normalize a laser output signal from Ge-photodiode recording a laser pulse shape. The thermal neutron signal from the 235 U vacuum chamber was normalized to the neutron fluence measured by activation method. Study of laser output energy as a function of Proc. Intern. Conf. ICENES’98, 1998 - 1998 Institute for Physics and Power Engineering, Technical Physics Laboratory http://www-tpl.ippe.obninsk.ru E-mail: kuh@ippe.obninsk.ru 4 ratio and total pressure of Ar-Xe mixture has shown that optimal parameters of medium is close to those of other studies [2-4]. 300 Laser power , kW 250 8 200 150 2 4 100 1 0 0 200 Pumping power , W / cm 3 12 50 400 600 0 800 Time , s Fig.2. Laser (1) and pumping (2) pulses. In Fig. 3, the results of measuring a jump of pressure in the laser active medium at P0=0.5 atm are compared with computed data obtained as a result of gasdynamic simulation. It is shown that side by side with common increase of pressure in laser volume, a sound wave is brought about by non-uniformity in the energy deposition into the gas along the LAEL. In time dependence of pressure, a slight increasing of the average pressure is observed right up to 50 ms. One of the reasons of such effect can be an action of the delayed reactor neutrons, and also neutrons reflected from the reactor box walls and the experimental equipment. Experiment and calculation have shown that contribution of these neutrons can make up around 20 % of the total energy deposited into the gas. The result of modeling used above assumption is shown in Fig. 3 by the smooth solid line with diamond symbols. Proc. Intern. Conf. ICENES’98, 1998 - 1998 Institute for Physics and Power Engineering, Technical Physics Laboratory http://www-tpl.ippe.obninsk.ru E-mail: kuh@ippe.obninsk.ru 5 P/P0 0.8 0.6 0.4 - Experiment 0.2 - Calculation - Model 0.0 0.00 0.02 0.04 0.06 0.08 0.10 t, s Fig. 3. Comparison of experimental relative pressure jump with results of gasdynamic calculation and modeling. Energy deposition , mJ /cm 3 40 30 20 10 0 0.0 0.2 0.4 0.6 0.8 1.0 Pressure , atm Fig. 4. Specific energy deposition into the gas vs. pressure. Proc. Intern. Conf. ICENES’98, 1998 - 1998 Institute for Physics and Power Engineering, Technical Physics Laboratory http://www-tpl.ippe.obninsk.ru E-mail: kuh@ippe.obninsk.ru 6 The specific energy deposition into the medium of the LAEL volume as a function of total medium pressure obtained by treatment of the pressure jump experimental data, is shown in Fig. 4. These results turn out to be less on 12 % than those obtained by the direct neutron-physical simulation [6,7]. Such a difference lies within the accuracy of both measurement and simulation. Three-dimensional distribution of fission fragment energy deposition in the LAEL at time of the neutron pulse maximum is presented in Fig. 5. It is shown that for our experimental geometry the rate of energy deposition into the gas is changed very strongly both along length and radius of the LAEL. Fig.5. Three-dimensional distribution of energy deposition rate at time of the neutron pulse maximum. Measurement of the laser energy dependence as a function of the output mirror transmittance have been carried out for the ratio Ar:Xe = 200:1 at the total mixture pressure of 0.5 atm, and the distance between reactor cores of 70 cm. Analysis of this dependence in the frame of the laser radiation transfer equation has allowed to evaluate Proc. Intern. Conf. ICENES’98, 1998 - 1998 Institute for Physics and Power Engineering, Technical Physics Laboratory http://www-tpl.ippe.obninsk.ru E-mail: kuh@ippe.obninsk.ru 7 the stored inversion energy that appeared equal to 1.4 J . Therefore , the efficiency of the nuclear -to-inversion energy is estimated equal to about 1 %. 12 Output power , kW 10 8 6 4 2 0 0 20 40 60 80 100 Transmittance , % Fig.6. The output laser power as a function of the output mirror transmittance. Measurement of the medium unsaturated gain have been performed using a method of calibrated losses within resonator. The gain value was found to be equal to 2.6 .10-2 cm-1 at the pumping power of 220 W/cm3. The gain coefficient obtained has been applied to calculate the saturation intensity parameter using the Rigrod’s equation [8] to approximate experimental data on the output laser power as a function of output mirror transmittance (Fig.6). As a result, the value of the saturation intensity has been determined equal to ~ 215 W/cm2 at the pumping power of 220 W/cm3. Using these data, we can estimate a value of power efficiency that appears equal to 2.5 % which is in agreement with result of [3]. CONCLUSION Thus, the results of studying the laser characteristics for the Ar-Xe LAEL carried out on the BARS-6 reactor facilities, have shown some good scope for applying this cell Proc. Intern. Conf. ICENES’98, 1998 - 1998 Institute for Physics and Power Engineering, Technical Physics Laboratory http://www-tpl.ippe.obninsk.ru E-mail: kuh@ippe.obninsk.ru 8 in the laser module of a demonstrative model of the high-power laser system. Also, it should be noted that most of experimental and calculated results are in a good agreement. REFERENCES 1. Dyachenko P.P. "Nuclear-laser power engineering as a perspective direction in nuclear energy utilization". Proc. of the ICENES’96 Conference , June 24-28, 1996, IPPE, Obninsk, Russia, p. 296. 2. Alford W.J., Hays G.N. "Measured laser parameters for reactor-pumped He/Ar/Xe lasers". J. Appl. Phys. ,vol.65, 1989, p. 3760. 3. Hebner G.A. and Hays G.N. "Fission-fragment excited xenon/ rare gas mixture .1. Laser parameters of the 1.73 m xenon transition". J. Appl. Phys. ,vol.73, 1993, p.3614. 4. Magda E.P. et.al. "Measurement of gain coefficient on the xenon 5d[3/2]1 -6p[5/2]2 transition under excitation of active medium by fission fragments". Proc. of the NPL’94 Conference, Arzamas-16, Russia, vol. 1, 1995, p.265. 5. Kononov V.N. et.al. "Nuclear pumped lasing experiments on fast burst reactor BARS-6". Proc. of the ICENES’96 Conference , 1996, IPPE, Obninsk, Russia, p.336. 6. Gulevich A.V., Kachanov B.V., and Kukharchuk O.F. "Models and codes for reactor-laser system dynamics computation". Preprint IPPE-2454, Obninsk, Russia,1995. 7. Pashin E.A. and Polevoy V.B. "LOCMMO_T - the code for simulation of nonstationary neutron flux functionals with local estimation methods". Preprint IPPE-2388, Obninsk, Russia,1994. 8. Rigrod W.W. "Homogeneously broadened CW lasers with uniform distributed loss". IEEE J. Quant. Electron. 1978, QE-14, p.377. Proc. Intern. Conf. ICENES’98, 1998 - 1998 Institute for Physics and Power Engineering, Technical Physics Laboratory http://www-tpl.ippe.obninsk.ru E-mail: kuh@ippe.obninsk.ru