Michael Downer http://www.ph.utexas.edu/dept/research/downer/ updated 2-19-07 Personal Born Married Citizenship July 19, 1954, Rockville Centre, New York Jane Castledine, August 22, 1993 U.S.A. Education Ph.D. M.A. B.A. Harvard University Oxford University, Brasenose College University of Rochester 1983 1978 1976 Applied Physics N. Bloembergen, supervisor Physics Physics Career Positions Professor of Physics Associate Professor of Physics Assistant Professor of Physics Postdoctoral Member Technical Staff University of Texas at Austin University of Texas at Austin University of Texas at Austin AT&T Bell Labs, Holmdel, NJ 1997 - present 1991 - 97 1985 - 91 1983 - 85 C. V. Shank, supervisor Honors/Awards College of Natural Sciences Distinguished Professor 1 Farrington Daniels Award (American Assoc. Physicists in Medicine) 2 Fellow, Optical Society of America President’s Associates Teaching Excellence Award, UT-Austin Teaching Excellence Award, College of Natural Sciences, UT-Austin Outstanding Graduate Teaching Award, UT-Austin 3 Fellow, American Physical Society Jack S. Josey Professorship, U T-Austin Research Fellow, Center for Ultrafast Optical Science, U. Michigan cited in Who's Who in Science and Engineering, and Who's Who among U.S. College Teachers NSF Presidential Young Investigator Award ONR Young Investigator Award IBM Faculty Development Award Trull Centennial Professorship, UT-Austin General George C. Marshall Scholar, Oxford University 145 invited talks at other institutions, professional meetings, etc 2006-present 2005 2003 2002 2001 2000 1999 1998 - 2000 1996 1993 ff. 1988-1993 1988-1991 1987-1989 1985 - 86 1976-78 1983-present $312,500 $150,000 $ 60,000 see attached list 1 for one of the two “best papers published in Medical Physics during 2004” (publication #87 on attached list). for “pioneering contributions to nonlinear and ultrafast laser spectroscopy of solid surfaces and plasmas” 3 for “fundamental contributions to nonlinear and ultrafast laser spectroscopy of solids and surfaces near the melting threshold and of gases and underdense plasmas near the thresholds of ionization and wakefield generation” 2 Professional Activities General Chair, Quantum Electronics & Laser Science (QELS ‘05) Program Chair, Quantum Electronics & Laser Science (QELS ‘03) Topical Editor, Journal of the Optical Society of America B *Member, Joint Council for Quantum Electronics (JCQE) Organized NSF Workshop on Micro/Macroscopic Semiconductor Interface Characterization Conference organizing committees: Conference on Lasers & ElectroOptics (CLEO 2000, 1997, 1991); Advanced Accelerator Concepts Symposium, Working Group Leader (2006, 2004, 2000, 1996) 2005 2003 2000- 2003 2000- 2003 1998 1991-present *12-member advisory board to promote cooperation among U.S. scientific organization that hold conferences in the field of quantum electronics & laser science, to organize and operate the 2 largest such conferences (IQEC and QELS), and to represent and advise their sponsoring organizations. Inventions M. C. Downer and P. T. Wilson, “System and Method for Frequency Domain Interferometric Second Harmonic Spectroscopy,” U.S. Patent 6,411,388 (granted 6-25-02). M. C. Downer, J. I. Dadap, J. K. Lowell, “Characterization of an external silicon interface using optical second harmonic generation,” U.S. Patent No. 5,557,409 (granted 9-17-96). C. W. Siders, E. Gaul, M. C. Downer, “Laser Beam Pointing Stabilizer,” marketed as INLINE TM by Technology Transfer Corportation, Longwood, FL under consulting agreement with inventors. Ph.D. Student Supervision (currently supervising 9 Ph.D. candidates) Bonggu Shim Ph. D. 2006: Coherently-controlled harmonic generation from exploding noble-gas clusters. Nicholas Matlis Ph.D. 2006: Snapshots of laser wakefields using frequency domain holography. Currently postdoctoral fellow, Lawrence Berkeley National Laboratory (supervisor: W. Leemans) Jinhee Kwon Ph.D. 2006: Second-harmonic and reflectance-anisotropy spectroscopy of vicinal Si(001) interfaces. Currently postdoctoral fellow, Rutgers Univ., NJ (supervisor: Ives Chabal) Ramon Carriles Ph.D. 2005: Nonlinear optical characterization of silicon/high-K dielectric interfaces. Currently postdoctoral fellow, Colorado School of Mines, Golden, CO (supervisor: Jeff Squier) Kui Wu Ph.D. 2004: Electric-field-induced second-harmonic microscopy, Currently staff scientist, Wuhan Telecommunications, China. Jiang Yingying Ph.D. 2002: Linear and nonlinear optical spectroscopies of SiGe interfaces and Si nanocrystals. Postdoctoral fellow, Vanderbilt U. (2003-04); Currently Instructor of Physics, Peking U. Daeyoung Lim Ph.D. 2001: Nonlinear optical spectroscopy of silicon-boron and other silicon-adsorbate systems. Postdoc LANL (2001-03); staff scientist at IBM T. J. Watson Research Center, NY (2003-05); currently Professor of Physics & Applied Physics, Kyunghee University, Korea. Erhard W. Gaul Ph. D. 2000: Production and characterization of a fully-ionized helium plasma channel for high intensity laser pulse propagation. Laser scientist, Gesellschaft für Schwerionforschung (GSI), Darmstadt, Germany (2001-04); Currently chief laser scientist, Texas Petawatt project. Philip T. Wilson* Ph. D. 2000: Frequency domain interferometric second harmonic spectroscopy. NRC post-doc at NIST, Gaithersburg, MD; currently research scientist at Milliken Chemical Co., Georgia. Mikal K. Grimes Ph. D. 1998: Vacuum heating and expansion of solid surfaces by intense femtosecond laser irradiation. Currently Senior MTS, Trilogy, Inc., Austin, TX. Yun-Shik Lee Ph. D. 1997: Optical fourth harmonic generation at crystalline surfaces. Postdoc, U. Michigan; currently Assoc. Prof. Physics, Oregon State U. Xiaofeng Hu Ph. D. 1997: Femtosecond linear and nonlinear spectroscopy of silicon, germanium and silicongermanium alloys. Senior Member of Technical Staff, Ball Semiconductor, Inc., Dallas, TX (1997-2000); currently senior MTS at Applied Materials, Inc, Santa Clara, CA. Craig W. Siders Ph. D. 1996: An experimental demonstration of the laser wakefield “photon accelerator”: longitudinal interferometric diagnostics for plasma-based acceleration. Director’s postdoctoral fellow, Los Alamos National Laboratory (1996-98); Research Faculty Scientist, UC-San Diego (1998-2000); Asst Prof. of Optics, CREOL, U. Central Florida, Orlando, FL. (2001-05); currently senior staff scientist, National Ignition Facility, Lawrence Livermore Natl. Laboratory Jerry Dadap Ph.D. 1995: Optical second harmonic electro- and thermo-reflectance spectroscopy of Si(001)/SiO2, H-Si(001), and Si(001)-(2x1) interfaces by femtosecond laser pulses. Postdoctoral fellow, Physics Dept., Columbia U. (1996-2000); Senior MTS, Tellium, Inc., NJ (2001-04); Currently Research Scientist, Brookhaven Natl. Laboratory and Columbia University. Hyeyoung Ahn Ph.D. 1994: Femtosecond dynamics of condensed matter under planetary interior conditions. Research Scientist, Nippon Telegraph & Telecommunication (NTT, 1994-96); Research Fellow, Japan Atomic Energy Research Institute (JAERI, 1996-2000); Research Scientist, Dept. Physics, National Tsing-Hua U., Taiwan. (2001-05); Currently Prof. of Photonics, Natl, Chiao Tung U., Hsinchu, Taiwan Charlie Wang Ph.D. 1993: Hydro- and electro-dynamics of solid targets under intense femtosecond laser excitation. Postdoctoral fellow and Senior Research Scientist, Columbia U. (1993-98). Currently Senior Development Engineer, Coherent Laser Group, Coherent, Inc., Santa Clara, CA. Heung Ro Choo Ph.D. 1992: Rapid scan femtosecond ellipsometry and its application to optical surface diagnostics and ultrafast carrier dynamics in semiconductors . Senior Researcher, Electronics & Telecommunications Research Institute (ETRI), Daejon, Korea (1993-2000). Gary W. Burdick Ph.D. 1991: Third order contributions to spin-forbidden rare earth optical transition intensities. Currently Professor of Physics, Andrews University, Michigan. William M. Wood Ph.D. 1991: Femtosecond study of plasma generation and dynamics by blueshifting of high intensity laser pulses. Currently Member of Technical Staff, Los Alamos National Laboratory. David H. Reitze** Ph.D. 1990: Femtosecond dynamics of phase transitions in carbon and silicon. Currently Professor of Physics, U. of Florida (Gainesville). Glenn B. Focht Ph.D. 1990: Frequency shifting of femtosecond laser pulses. Deceased. * winner National Research Council postdoctoral fellowship ** winner of 1991 UT Outstanding Dissertation Award. M.S. Student Supervision (currently supervising 2 M. S. candidates) M. S. 2005: Diagnostics for the laser wakefield accelerator M. S. 2004: Guiding a high energy laser beam through a plasma channel. M. S. 2003: Time-resolved reflectance-difference spectroscopy of semiconductor interfaces. M. S. 2002: Optical Parametric Amplifier for Nonlinear Optical Spectroscopy. M. S. 2001: Propagation of high intensity light through gas-filled hollow-core capillaries. M. S. 2000: Laser-scanning confocal electric-field-induced second harmonic generation spectroscopy. Ralf Büngener M. S. 1998: Si/Ge epitaxial growth surface monitoring by second harmonic generation. Stefan Düsterer M. S. 1998: Second harmonic generation from ferromagnets. Roland W. Kempf M. S. 1998: Second, third and fourth harmonic generation at crystalline Si(110) and Si(111) surfaces. Christian Fauser M. S. 1997: Lensing characteristics of a standing acoustic wave in a piezoelectric tube Mark H. Anderson M. S. 1997: Fourth harmonic generation from gallium arsenide. Christoph Trump M. S. 1996: Femtosecond interferometric study of phase transitions in silicon; Matthias Goldammer M. S. 1996: Low repetition rate pointing stabilizer for amplified laser systems; Alexander Frey M. S. 1994: Repetition rate synchronization of a colliding-pulse mode-locked laser with an external oscillator Nelson Turner III M. S. 1994: Dual beam detection of frequency shifted ultrafast laser pulses. Sebastian Jung Alexander Debus Florian Pollinger Carsten Winterfeldt Thomas Pfeiffer Jesse Canterbury Undergraduate Student Supervision in Research James Miller Brian Mattern Claudia Treml Joshua Migliazzo Hilary Lovett Mohammed Islam Afaque Ahmed Kin Foo Chan Michael Barber David Jenkins Summer 2004. Performed optical second-harmonic experiments on silicon/high K dielectric interfaces. Supported by NSF REU program. Co-author of publication #94. Summer 2003. Performed optical second-harmonic experiments on silicon nanocrystals. Supported by NSF REU program. Co-author of publication #90. 10/99-5/00. Built a Frequency-Resolved Optical Gating (FROG) device for characterizing femtosecond laser pulses. Pursued graduate work at U. Würzburg, Germany. 9/97-6/99. Developed commercial laser beam pointing stabilizer device (supported by Texas Advanced Technology Program). Earned graduate degree at Ecole Polytechnique. Summers 1997, 1998. Developed interferometric system for characterizing femtosecond pulses; developed femtosecond laser micromachining technique. Pursued graduate environmental engineering program. 1/96-8/96. Assisted with nonlinear optical experiments (supported by R. A. Welch Foundation). Earned Ph.D. in physics at U. California-Berkeley. 1/93- 9/95. Developed and maintained data acquisition system for in-situ optical second harmonic measurements (supported by Welch Foundation). Earned M.B.A. at McMaster U. 9/95-1/96. Performed optical second harmonic experiments on MOS structures. Earned Ph.D. in Biomedical Engineering, UT-Austin. Summer 1994. Assisted with in-situ optical second harmonic experiments (supported by NSF) Summer 1990. Helped construct a Ti:S femtosecond laser (supported by NSF Research Experiences for Undergraduates Program). Earned Ph.D. in physics at U. Maryland. Postdoctoral Supervision Y. Q. An A. Rundquist L. Mantese Z. Xu S. P. LeBlanc D. M. Riffe W. C. Banyai T. R. Zhang 2004-present 1998-2000 1998- 2000 1996-1997 1995-1999 1991-1994 1989-1991 1986-1988 Ph.D. U. Colorado Ph.D. U. Michigan Ph.D. NCSU Ph.D. U. Rochester Ph.D. Rice U Ph.D. Cornell U. Ph.D. U. Arizona Ph.D. U. Texas currently Assoc. Prof. of Physics, Hamline U., Minnesota currently MTS, Agilent, Inc, Santa Clara, CA currently MTS, Applied Materials, Inc, Santa Clara, CA current senior research scientist, 3M Corporation, Austin, TX currently Prof. of Physics, Utah State U., Logan, UT currently senior research scientist, Stanford University, CA currently MTS, Compact Software, Inc., Paterson, NJ CAREER RESEARCH HIGHLIGHTS (reference numbers from publication list) • Two-photon laser spectroscopy of rare earth ions [publications 1, 4, 5, 6, 15, 18 & two book chapters; 430 citations as of 3/06] In Ph.D. work during the 1980s, Downer pioneered the field of experimental two-photon spectroscopy of 4f4f transitions in lanthanide-doped crystals [1,4-6], an important class of solid-state laser media. Building on earlier theoretical work by B. R. Judd and B. G. Wybourne, he advanced a new class of 3rd and higher order “Wybourne-Downer mechanisms” [4,5,15,18] which accounted quantitatively for widespread anomalies in both two-photon and linear spectroscopy of lanthanides, which has provided a widely-cited foundation for both experimental and theoretical work in this field since the mid-1980s. • High-intensity laser-solid interactions: melting, hydrodynamic surface expansion, electron & x-ray emission, vacuum heating, ballistic hot electron transport [publications 9,12,17,19, 20, 22, 25, 26, 28, 31, 32, 34, 37, 62, 99, 100 & one book chapter; 540 citations as of 3/06] Downer led several key experiments which defined the ultrafast heating and melting physics of solid target surfaces [9-12,19,20,22,26,28,31,32,34,37]. He made the first femtosecond (fs) “movie” of the melting and plasma expansion of fs-irradiated silicon [9]. He demonstrated ultrafast melting of elemental carbon for the first time [19,22,26], then provided the first quantitative measurements of the temperature-dependent optical properties of the elusive liquid state of carbon [26,31], exploiting the well-defined surface of the transient sample during the first half-picosecond following excitation. These measurements stimulated new molecular dynamics simulations of the liquid state, and have astro- and geo-physical implications. Using innovative techniques based on ultrafast thin film interference [12] and ultrafast thermionic electron emission [32,37], Downer first demonstrated the significant role of Auger processes [12] and temperature-dependent electronphonon coupling [37] in governing heat transfer from carrier to lattice systems under ultrafast melting conditions, thus defining important differences from both lower and higher intensity regimes. Downer's group first experimentally identified "vacuum heating" [62] predicted by Brunel in 1987, in which light is absorbed by drawing electrons into vacuum and returning them to the target with the quiver velocity. In current work, Downer's group re-visits "fs imaging" [9] with relativistically intense pump pulses, to measure nonlocal radiative and hot electron transport in solid density plasmas [99]. These experiments provide input for codes used to analyze fast ignition of laser fusion, proton and ion beam generation, and astrophysics. • High-intensity laser interactions with gases & underdense plasmas: ionization blue-shifts, laser wakefield characterization, plasma channels, laser-cluster interactions [publications 16, 24, 27, 29, 30, 36, 39-42, 45-47, 51, 54, 59, 60, 66, 71, 72, 74, 86-89, 102-104; 750 citations as of 3/06] During the early 1990s, when unique features of intense-field atomic ionization were first coming to light, Downer performed the first fs-time-resolved experiments on ionizing gases using ionization-induced spectral blue-shifting [16,24,27,29,30,42,51,72,88]. In addition to fs-time-resolution, these experiments accessed higher gas densities than electron and ion detection experiments, thus probing high-intensity collisional physics for the first time. This widely cited work continues to impact research into propagation of intense short pulses through dense gases, as in the fast ignitor project. In the mid-1990s, Downer’s group pioneered fs-time-resolved experiments diagnosing laser wakefields [45,46,47,54,71,102] both in the lowdensity resonantly-driven regime using frequency-domain interferometry [45,46], and in the high-density forward Raman instability-driven regime, using collective Thomson scattering [47,60]. Recently his group has obtained the first holographic snapshots of laser wakefields [102] using frequency-domain holography, a single-shot extension of frequency-domain interferometry developed by Downer’s group [71]. To extend high-intensity interaction lengths to ≥1 cm, Downer's group improved on a plasma fiber technique developed by H. M. Milchberg, demonstrating distortion-free guiding of laser pulses with 0.2 x 1018 W/cm 2 peak intensity through 1.5 cm-long fully-ionized He plasma channels [74], and performing the first pump-probe experiments in such a channel [88]. His group developed the theory of Raman-seeded wakefield acceleration [89], a path to controlled, high-repetition rate production of MeV electron beams for medical applications [86,87], and developed a two-color terawatt laser system [104] for experiments. Recently he has demonstrated enhanced harmonic generation in exploding noble-gas clusters using a pump-probe scheme [103]. • Nonlinear optical spectroscopy of surface & interfaces [publications 33, 35, 43, 44, 48-50, 52, 53, 55-58, 61, 63, 65, 67-70, 73, 75, 76, 78-80, 82-85, 90-98, 101; 490 citations as of 3/06] Downer pioneered the application of widely tunable fs sources to even-order nonlinear spectroscopy of semiconductor surfaces [35,43,44,50,52,53,55-58,63-65,67-70,73,75,76,78-80], simultaneously advancing spectroscopic fundamentals [50,68,70,76,78,79], applications to semiconductor manufacturing [35,44,53,56], and spectroscopic techniques [55,58,65]. His contributions include: first quantitative characterization of angstrom-scale roughness at a buried interface (Si/SiO 2) based on optical second harmonic generation (SHG) [35, U.S. Patent 6,411,388]; first SHG spectroscopy of a metal-oxide-semiconductor (MOS) structure [44,83], leading to the most complete theoretical description of electric-field-induced SHG, or EFISH [48,49,61]; first quantitative, real-time, in-situ SHG-based measurements of kinetics of chemical vapor deposition growth of silicon and germanium films [43,50,53,56,57,63,69]; the first demonstration of 4th harmonic spectroscopy from crystalline surfaces below melting threshold [55,58,67]; first SHG spectroscopy of silicon nano-interfaces [75,80] including development of a novel two-beam SHG method for enhancing quadrupolar nano-interface response [90,91,97]; invention of frequency-domain interferometric second-harmonic (FDISH) spectroscopy [65,82,95, U.S. Patent 6,411,388]; first quantitative comparison of SHG and reflectance-anisotropy spectroscopy (RAS) on common (vicinal Si) surfaces [85,93,96]; first SHG spectroscopy of Si/high-K dielectric interfaces [94,101]. Named Physical Effect M. Tanaka and T. Kushida, “Interference between Judd-Ofelt and Wybourne-Downer mechanisms in the 5D0 - 7F J transitions of Sm2+ in solids, “ Journal of Chemical Physics 53, 588 (1996). The “Wybourne-Downer mechanisms” cited in the title of this recent paper were first introduced by me and UT graduate student Gary Burdick in two J. Chem. Phys. paper in 1988,89 (see #23, 27 on publication list). Recent Newsbrief Articles “Two-Beam Second-Harmonic Generation”, by L. Sun, S. Cattaneo, P. Figliozzi, Y. Jiang, Y. Q. An, W. L. Mochán, B. S. Mendoza, M. Kauranen, and M. C. DOWNER, in Optics & Photonics News, p. 34 (Dec. 2005). Special year-end issue devoted to “Optics Highlights of 2005”. “Ultrafast radial transport in micro-size laser-produced plasmas,” in Petawatters No. 8 (2005) – Newsletter of the Institute for Laser Energetics (ILE), Osaka, Japan. “New Light from Silicon Nano-Interfaces,” in Texas Materials Institute Bulletin, Winter 2005. “Stardust to Semiconductors,” in Focus on Science, Summer 2000. Billy Goodman, “Star in a Bottle,” Air & Space, February/March 1998. J. Glanz, “Meeting takes pulse of laser accelerators,” Science 271, 26 (1996). C. Joshi and P. Corkum, “Interactions of ultra-intense laser light with matter,” Physics Today 48, 36 (1995). N. Bloembergen, “First light on fluid carbon,” Nature 356, 110 (1992). New & Views article about publication #26. SUMMARY OF CURRENT RESEARCH (reference numbers from publication list) 1) High-intensity laser-plasma interactions a) Laser wakefield acceleration (primary financial support: Dept. of Energy) Diagnostics: We measure transverse and longitudinal structure of laser-generated wakefields in a single laser shot [102], using the technique of frequency domain holography [71]. We resolve wave front curvature seen previously only in simulations, and reconstruct and display wake morphology from raw data within seconds, providing real-time feedback for experimental optimization between laser shots. Such snapshots open a direct window into intense laser-plasma physics. Plasma “bubbles” and fast-ignitor tracks should be similarly observable. (1 Ph. D. student) Raman Seeding: Conventional laser wakefield accelerators operate at low laser repetition rate (≤ 10 Hz), whereas most applications demand kilohertz repetition rates to achieve µA average current. Using particlein-cell simulations, we developed the concept of “seeding” the forward Raman scattering instability by supplementing the main driving pulse with a weak (1%) co-propagating pulse shifted by the plasma frequency ωp [89]. Analogous to injection seeding of Raman amplifier, the seed suppresses noise and reduces driving pulse energy, enabling higher repetition rate. Simulated electron yield is promising for medical applications [86, 87]. A two-color terawatt chirped-pulse laser system has been developed [104] to implement experimental demonstration of Raman-seeded laser-wakefield acceleration. (2 Ph. D. students} Channeling: Distortion-free propagation of TW pulses through 1.5 cm long low Z plasma channels [74], and frequency-domain interferometric pump-probe experiments [88] have been demonstrated. Low Z channels are now being generated in a differentially-pumped cell, enabling efficient coupling of 5 TW pulses and generation of channeled laser wakefields. (1 Ph. D. student) b) Laser-solid interactions (primary financial support: NSF FOCUS Center) Harmonic generation in exploding clusters: Several years ago we predicted that harmonic generation from clustered plasma would become phase-matched at a critical cluster size and density [66]. We recently performed pump-probe experiments that confirm the predicted enhancement in third-harmonic generation [103], while revealing new subtleties caused by competition among time-varying phase-matching, resonant enhancement of the nonlinear cluster susceptibility χ(3) and linear absorption during cluster expansion. The enhancement mechanism is being scaled to generation of high-harmonics into the soft x-ray regime. (1 Ph. D. student) Nonlocal energy transport in solid density plasmas: Using fs microscopy [9] and x-ray imaging, we observe subpicosecond transport of thermal energy radially outward from micrometer-sized spot of low-Z and high-Z solid targets following relativistically intense fs excitation [99]. In this excitation regime, thermal plasma electrons reach ≥ 1 keV temperature, and much deposited energy channels into superthermal (tens of keV) electrons. Thus radiation and hot electrons become dominant carriers of energy out of the initially photoexcited volume. Results are being used to test particle-in-cell simulations of hot electron transport in self-generated mega-gauss magnetic fields, and theoretical models of radiative transport. The physics of this transport is relevant to fast ignition of laser fusion, generation of ultrashort x-rays and relativistic proton and ion beams, and to astrophysics. (1 Ph. D. student) 2) Optical second-harmomic spectroscopy of semiconductor nano-interfaces (financial support: NSF-DMR, Robert Welch Foundation) SHG spectroscopy of interfaces of embedded Si nano-crystals: Si nano-crystals embedded in glass behave in a most un-silicon-like manner: they glow brightly, a feature giving birth to Si light-emitting devices, maybe lasers. Unusualy bonding structures at the nanocrystal-glass interfaces are believed responsible, but effective experimental probes have eluded the surface scientist. We demonstrated that optical secondharmonic generation (SHG), a noninvasive spectroscopic probe of planar interfaces, is sensitive to these nano-interfaces [75, 80, 90, 97]. We invented a novel two-beam SHG configuration that generates a robust SH beam that is sensitive to chemical modification of the nano-interfaces [90,91,97]. Current experiments use tunable pulses, and pump-probe techniques, to measure the spectrum and lifetime of nano-interface states to elucidate their poorly understood electronic structure. (2 Ph. D. students, 1 postdoc) SHG and RAS of step-edges at vicinal Si surfaces: Step-edges at vicinal Si interfaces provide templates for growth of nano-wires, unique chemistry to control step-flow epitaxial growth, and unique electrical properties to control local fields, channel mobility and breakdown in opto-electronic devices. They also provide a unique context for directly comparing the two most important optical surface spectroscopies: secondharmonic generation (SHG) and reflectance-anisotropy spectroscopy (RAS) for the first time. We have made a direct experimental comparison of RAS and spectroscopic SHG of native-oxidized [85,93] and clean, reconstructed [96] Si(001) and discovered a common microscopic origin of RAS and SHG by analyzing both spectra with a simplified bond hyperpolarizability model (1 Ph. D. student). Current Research Grants M.C. Downer M. C. Downer M.C. Downer M. C. Downer M. C. Downer Department of Energy1 National Science Foundation2 Robert A. Welch Foundation3 National Science Foundation4 Sematech5 1/15/05 - 1/14/08 8/1/01-7/31/07 6/1/04 - 5/31/07 9/1/02 - 8/31/06 9/1/04 – 8/31/05 $650,000 $700,000 $150,000 $365,000 $100,000 1 "Laser wakefield acceleration: channeling, seeding and diagnostics" 2 ”Frontiers in Optical Coherent & Ultrafast Science (FOCUS)” (PH Bucksbaum, director) nonlinear optical probes of Column IV interface chemistry" 4 “Nonlinear spectroscopy of planar and nanocrystalline silicon interfaces: experiments for ab initio theory” 5 "Optical characterization of silicon high-K dielectric interfaces” 3 "Femtosecond TEACHING HIGHLIGHTS 1) Interactive teaching. Introduced "Concept Quiz" procedure, an interactive teaching method which encourages dialog between lecturer and students, and among students, in a large lower division classroom setting such as PHY 316, PHY 303L, or PHY 302L. This procedure was subsequently adopted by several other faculty (Chiu, Moore, Kleinman), was computerized as part of the Painter Hall lecture room remodeling, and has become a standard departmental procedure for large introductory lecture courses. In Fall & Spring 2002 and Spring 2004 semesters I introduced Concept Quizzes for the first time into Upper Division Course PHY 352K: Classical Electrodynamics. I composed and field-tested approximately 40 new concept quizzes, and found them to be an effective, well-received teaching tool at the advanced undergraduate physics major level. 2) New graduate course. Proposed, designed, and six times taught the graduate Advanced Course PHY 395K: "Nonlinear Optics and Lasers" on behalf of the Atomic & Molecular Physics group. Enrollment has exceeded 20 on every offering, and 30 on some. I will teaching this course for the seventh time in Fall 2006. 3) Laboratory course improvements. Introduced a substantial expository writing and public speaking into undergraduate (PHY 474) and graduate (PHY 380N) laboratory courses. Initiated 4 new experiments - high Tc superconductors, holography, diode laser spectroscopy, and an optical fiber experiment - in the advanced undergraduate laboratory PHY 474. 4) Undergraduates in research. Supervised and financially supported the work of 10 undergraduate students in my research program over the last 8 years. These included James Miller and Brian Mattern in the past 2 years, both of whom co-authored publications [Papers 90, 94 on publication list], made presentations on their work at the UT College of Natural Sciences (CNS) undergraduate research symposium, and have gone on to graduate scientific work. During most semesters when PHY 380N has been offered, supervised the semester-long research projects of 1 or 2 PHY 380N students working in my laboratory. 5) CIR-KITS. Initiated and developed a flexible inventory of low-cost “CIr-Kits” (take-home electrical circuit kits) with accompanying homework assignments for use in introductory Electricity & Magnetism courses. The contents of the kits fit in a small sandwich bag, and can be worked on in a student’s apartment, at the library, in the hallway, at the coaching tables, or in the cafeteria. I used Cir-Kits with 50 to 85 students in 6 different semesters in PHY 316 and PHY 302L classes starting in fall 97. With the help of a Dean’s Fellowship for Curriculum Development (spring 99), I expanded and streamlined the Cir-Kits with the aim of developing a standard Departmental procedure which could ultimately be used in the Physics Department’s 302L, 303L, 309L, 316, and 317L introductory E&M courses. Student Advising Faculty Advisor and co-founder of Texas Optics Society, a new UT student chapter of the Optical Society of America (OSA) and the International Society for Optical Engineering (SPIE). This organization sponsors faculty and student seminars and social events involving UT optics researchers in the Colleges of Natural Science and Engineering. Web site: http://www.engr.utexas.edu/texasoptics/ UT Physics Department Service Member, Undergraduate Committee, 2002-present Member, faculty recruitment committee; played central role in recruitment of T. Ditmire (2000) & G. Shvets (2003). Chairman, Budget Council Advisory Committee (BCAC), 1993-94; Member, BCAC, 1991-94, 1995-98 GRACL (GRaduate Academic CurricuLum committee), 1990-91 page 1 citation count from ISI Web of Science Refereeed Journal Publications key to roles: updated 1/3/08 group leader and P. I. = A primary junior researcher = B essential collaborator = C peripheral collaborator = D role citations # 67 1 M. Dagenais, M. DOWNER, R. Neumann, and N. Bloembergen, “Two-photon absorption as a new test of the Judd-Ofelt theory.” Physical Review Letters 46, 561-565 (1981). C 51 2 A. Bogdan, M. DOWNER, and N. Bloembergen, “Quantitative characteristics of pressure-induced degenerate frequency resonance in four wave mixing.” Optics Letters 6, 348-350 (1981). C 54 3 A. Bogdan, M. DOWNER, and N. Bloembergen, “Quantitative characteristics of pressure- induced four wave mixing signals observed with cw laser beams.” Physical Review A 24, 623-626 (1981). C 53 4 M.C. DOWNER, A. Bivas, and N. Bloembergen, “Selection rule violation, anisotropy, and anomalous intensity of two-photon absorption lines in Gd3+: LaF3.” Optics Communications 41, 335-339 (1982). B 110 5 M.C. DOWNER and A. Bivas, “Third and fourth order analysis of the intensities and polarization dependence of two-photon absorption lines of Gd3+ in LaF3 and aqueous solution.” Physical Review B 28, 3677-3696 (1983). B 82 6 M.C. DOWNER, C.D. Cordero-Montalvo, and H. Crosswhite, “Study of new 4f7 levels of Eu2+ in CaF2 and SrF2 using two-photon absorption spectroscopy.” Physical Review B 28, 4931-4943 (1983). B 191 7 W.H. Knox, M.C. DOWNER, R.L. Fork, and C.V. Shank, “Amplified femtosecond optical pulses and continuum generation at 5 KHz repetition rate.” Optics Letters 9, 552-554 (1984). C 91 8 M.C. DOWNER, R.L. Fork, and C.V. Shank, “Femtosecond imaging of melting and evaporation at a photoexcited silicon surface.” Journal of the Optical Society of America B 2, 595-599 (1985). B 204 9 W.H. Knox, R.L. Fork, M.C. DOWNER, D.A.B. Miller, D.S. Chemla, C.V. Shank, A.C. Gossard, and W. Wiegmann, “Femtosecond dynamics of resonantly generated excitons in room temperature GaAs quantum wells.” Physical Review Letters 54, 1306-1309 (1985). C 180 10 W.H. Knox, R.L. Fork, M.C. DOWNER, R.H. Stolen, C.V. Shank, and J. Valdmanis, “Optical pulse compression to 8 femtoseconds at a 5 KHz repetition rate.” Applied Physics Letters 46, 1120-1121 (1985). C 77 11 M.C. DOWNER and C.V. Shank, “Ultrafast heating of silicon-on-sapphire by femtosecond optical pulses.” Physical Review Letters 56, 761-764 (1986). B 16 12 G. Focht and M.C. DOWNER, “Generation of synchronized ultraviolet and red femtosecond pulses by intracavity frequency doubling.” IEEE Journal of Quantum Electronics 24, 431-434 (1988). A 6 13 T.R. Zhang, G. Focht, P.E. Williams, and M.C. DOWNER, “Theory of intracavity frequency doubling in passively mode-locked femtosecond lasers.” IEEE Journal of Quantum Electronics 24, 1877-1883 (1988). A 52 14 M. C. DOWNER, G. W. Burdick, and D. K. Sardar, “A new contribution to spin-forbidden rare earth optical transition intensities: Gd3+ and Eu3+.” Journal of Chemical Physics 89, 1787-1797 (1988). A 49 15 W.M. Wood, G. Focht, and M.C. DOWNER, “Tight focusing and blue shifting of millijoule femtosecond pulses from a conical axicon amplifier.” Optics Letters 13, 984-986 (1988). A 31 16 O.R. Wood II, W.T. Silfvast, H.W.K. Tom, W.H. Knox, R.L. Fork, C.H. Brito-Cruz, M.C. DOWNER, and P.J. Maloney, “Effect of laser pulse duration on XUV emission from femtosecond and picosecond laser-produced Ta plasmas.” Applied Physics Letters 53, 654-656 (1988). C 33 17 G.W. Burdick, M.C. DOWNER, and D.K. Sardar, “A new contribution to spin-forbidden rare earth optical transition intensities: analysis of all trivalent lanthanides.” Journal of Chemical Physics 91, 1511- 1520 (1989). A page 2 Refereeed Journal Publications updated 1/3/08 27 18 D.H. Reitze, X. Wang, H. Ahn, and M.C. DOWNER, “Femtosecond laser melting of graphite.” Physical Review. B 40, 11986-11989 (1989). A 40 19 D.H. Reitze, T.R. Zhang, W.M. Wood, and M.C. DOWNER, “Two-photon spectroscopy of silicon using femtosecond pulses at above gap frequencies.” Journal of the Optical Society of America B 7, 84-89 (1990). A 43 20 T.R. Zhang, H.R. Choo, and M.C. DOWNER, “Phase and group velocity matching for second harmonic generation of femtosecond pulses.” Applied Optics 29, 3926-3933 (1990). A 32 21 K. Seibert, G.C. Cho, W. Kütt, H. Kurz, M.C. DOWNER, D.H. Reitze, J. Dadap, and A.M. Malvezzi, “Femtosecond carrier dynamics in graphite.” PhysIcal Review B 42, 2842-2851 (1990). 22 G.W. Burdick and M. C. DOWNER, ‘The role of linear crystal field terms in hypersensitive Eu3+ optical transition intensities.’ Eur. J. Solid State Inorganic Chem. 28, 217-220 (1990). 23 M. C. DOWNER, W.M. Wood, and J.I. Trisnadi, “Comment on 'Energy Conservation in the Picosecond and Subpicosecond Photoelectric Effect'.” Physical Review Letters 65, 2832 (1990). A 37 24 J.I. Dadap, D.H. Reitze, G.B. Focht, and M.C. DOWNER, “Autocorrelation measurement of ultraviolet femtosecond pulsewidths by two-photon absorption in diamond.” Optics Letters 16, 499-502 (1991). A 77 25 D. H. Reitze, H. Ahn, and M. C. DOWNER, “Optical properties of liquid carbon measured by femtosecond spectroscopy. “ Physical Review B 45, 2677-2693 (1992). A 118 26 W. M. Wood, C. W. Siders, and M. C. DOWNER, “Measurement of femtosecond ionization dynamics of atmospheric density gases by spectral blueshifting.” Physical Review Letters 67, 3523-3526 (1991). A 40 27 X. Y. Wang and M. C. DOWNER, "Femtosecond time-resolved reflectivity of hydrodynamically expanding metal surfaces." Optics Letters 17, 1450-1452 (1992). A 37 28 B. I. Penetrante, N. M. Bardsley, W. M. Wood, C. W. Siders, and M. C. DOWNER, "Ionization-induced frequency shifts in intense femtosecond laser pulses." Journal of the Optical Society of America B 9, 20322040 (1992). A 42 29 W. M. Wood, C. W. Siders, and M. C. DOWNER, "Femtosecond growth dynamics of an underdense ionization front measured by spectral blueshifting." IEEE Transactions on Plasma Science 21, 20-33 (1993). A 4 30 M. C. DOWNER, H. Ahn, D. H. Reitze, and X. Y. Wang, "Dielectric function and electrical resistivity of liquid carbon determined by femtosecond spectroscopy." International Journal of Thermophysics 14, 361-370 (1993). A 28 31 D. M. Riffe, X. Y. Wang, M. C. DOWNER, D. L. Fisher, T. Tajima, J. L. Erskine, and R. M. More, "Femtosecond thermionic emission from metals in the space-charge-limited regime." Journal of the Optical Society of America B 10, 1424-1435 (1993). 32 H. R. Choo, X. F. Hu, M. C. DOWNER, and V. P. Kesan, "Femtosecond ellipsometric study of nonequilibrium carrier dynamics in Ge and epitaxial Si1-xGex." Applied Physics Letters 63, 1507-1509 (1993). A 21 33 T. Dallas, M. Holtz, H. Ahn, and M. C. DOWNER, "Structural phase of femtosecond laser melted graphite." Physical Review B 49, 796-801 (1994). C 51 34 J. I. Dadap, B. Doris, Q. Deng, M. C. DOWNER, J. K. Lowell, and A. C. Diebold, "Randomly-oriented angstrom-scale microroughness at the Si(100)/SiO2 interface probed by optical second harmonic generation." Applied Physics Letters 64, 2139-2141 (1994). A 16 35 E. V. Vanin, A. V. Kim, A. M. Sergeev, and M. C. DOWNER, "Excitation of ultrashort bursts of harmonics of the radiation during ionization of a gas by an intense light pulse." Pis'ma Zh. Eksp. Teor. Fiz. 58, 964-969 (1993) [JETP Letters 58, 900-906 (1994)]. 36 X. Y. Wang, D. M. Riffe, Y. S. Lee, and M. C. DOWNER, "Time-resolved electron temperature measurement in a highly excited gold target using femtosecond thermionic emission," Physical Review B 50, 8016-8019 (1994). A 37 C. W. Siders, E. Gaul, M. C. DOWNER, A. Babine, A. Stepanov, "Self-starting femtosecond pulse generation from a Ti: sapphire laser synchronously pumped by a pointing-stabilized mode-locked Nd: YAG laser," Review of Scientific Instruments 65, 3140-3144 (1994). A 6 19 16 90 14 A A A A page 3 Refereeed Journal Publications updated 1/3/08 4 38 D. L. Fisher, T. Tajima, M. C. DOWNER, and C. W. Siders, “Envelope evolution of a laser pulse in an active medium,” Physical Review E 51, 4860-4868 (1995). D 18 39 K. Nakajima, T. Kawakubo, H. Nakanishi, A. Ogata, Y. Kato, Y. Kitagawa, R. Kodama, K. Mima, H. Shiraga, K. Suzuki, T. Zhang, Y. Sakawa, T. Shoji, Y. Nishida, N. Yugami, M. C. DOWNER, D. Fisher, B. Newberger, and T. Tajima) “A proof-of-principle experiment of laser wakefield acceleration,” Physica Scripta T52, 61-64 (1994). C 225 40 K. Nakajima, D. L. Fisher, T. Kawakubo, H. Nakanishi, A. Ogata, Y. Kato, Y. Kitagawa, R. Kodama, K. Mima, H. Shiraga, K. Suzuki, K. Yamakawa, T. Zhang, Y. Sakawa, T. Shoji, Y. Nishida, N. Yugami, M. C. DOWNER, T. Tajima, “Observation of ultrahigh gradient electron acceleration by a self-modulated intense short laser pulse.” Physical Review Letters 74, 4428-4431 (1995). C 35 41 C. W. Siders, N. C. Turner III, M. C. DOWNER, A. Babine, A. Stepanov, and A. Sergeev, “Blueshifted third harmonic generation during ultrafast barrier suppression ionization of subatmospheric density noble gases.” Journal of the Optical Society of America B 13, 330-335 (1996). A 24 42 J. I. Dadap, X. F. Hu, N. M. Russell, J. G. Ekerdt, M. C. DOWNER, and J. K. Lowell, “Analysis of second harmonic generation by unamplified, high repetition rate ultrashort laser pulses at Si(001) interfaces.” IEEE Journal of Special Topics in Quantum Electronics 1, 1145-1155 (1995). A 67 43 J. I. Dadap, X. F. Hu, M. Anderson, M. C. DOWNER, J. K. Lowell, and O. A. Aktsipetrov, “Optical second harmonic spectroscopy of a Si(001) metal-oxide-semiconductor structure,” Physical Review B 53, R76077609 (1996). A 15 44 C.W. Siders, S. P. Le Blanc, T. Tajima, M. C. DOWNER, A. Babine, A. Stepanov, and A. M. Sergeev, “Plasmabased accelerator diagnostics based upon longitudinal interferometry with ultrashort optical pulses,” IEEE Transactions on Plasma Science 24, 301-315 (1996). A 83 45 C.W. Siders, S. P. Le Blanc, T. Tajima, M. C. DOWNER, A. Babine, A. Stepanov, and A. M. Sergeev, “Laser Wakefield excitation and measurement by femtosecond longitudinal interferometry,” Physical Review Letters 76, 3570-3573 (1996). A 57 46 S. P. Le Blanc, M. C. DOWNER, R. Wagner, S.Y. Chen, A. Maksimchuk, G. Mourou, and D. Umstadter, “Characterization of a self-modulated laser wakefield by time-resolved Thomson scattering,” Physical Review Letters 77, 5381-5384 (1996). A 13 47 O. Aktsipetrov, A. Fedyanin, and M. C. DOWNER, ‘DC-electric-field-induced second harmonic generation studies of surfaces and buried interfaces of Column IV semiconductors,” Laser Physics 6, 1142-1151 (1996). C 13 48 O. Aktsipetrov, A. Fedyanin, V. Melnikov, J I. Dadap, X. F. Hu, M. Anderson, M. C. DOWNER, J. K. Lowell, “Optical second harmonic electroreflectance spectroscopy of the Si(001)-SiO2 interface in Si-SiO2-Cr MOS structures: separation of the surface and bulk nonlinear contributions,” Thin Solid Films 294, 231-234 (1997). C 51 49 J. I. Dadap, N. M. Russell, X. F. Hu, O. A. Aktsipetrov, J. G. Ekerdt, and M. C. DOWNER, “Second harmonic spectroscopy of a Si(001) surface during calibrated variations in temperature and hydrogen coverage,” Physical Review B 56, 13367-13379 (1997). A 7 50 B. Rau, C. W. Siders, S. P. Le Blanc, D. L. Fisher, M. C. DOWNER, T. Tajima, “Spectroscopy of short, intense laser pulses due to gas ionization effects,” Journal of the Optical Society of America B 14, 643-649 (1997). C 30 51 J. I. Dadap, P. T. Wilson, M. ter Beek, M. H. Anderson, and M. C. DOWNER, “Femtosecond carrier-induced screening of dc-electric field-induced second harmonic generation at the Si(001)/SiO2 interface,” Optics Letters 22, 901-903 (1997). 52 Z. Xu, X. F. Hu, D. Lim, J. G. Ekerdt, and M. C. DOWNER, “Second harmonic spectroscopy of Si(001) surfaces: sensitivity to surface hydrogen and doping, and applications to kinetic measurements,” Journal of Vacuum Science and Technology B 15, 1059-1064 (1997). A 18 A page 4 Refereeed Journal Publications updated 1/3/08 11 53 C. W. Siders, A. J. Taylor, and M. C. DOWNER, “Multi-pulse interferometric frequency resolved optical gating: real-time phase-sensitive imaging of ultrafast dynamics,” Optics Letters 22, 624-626 (1997). C 9 54 Y. S. Lee, M. H. Anderson, and M. C. DOWNER, “Fourth harmonic generation at a crystalline GaAs(001) surface,” Optics Letters 22, 973-975 (1997). A 27 55 X. F. Hu, Z. Xu, D. Lim, M. C. DOWNER, P. S. Parkinson, B. Gong, G. Hess, J. G. Ekerdt, “In situ optical second harmonic generation monitoring of disilane adsorption & hydrogen desorption during Si(001) epitaxial growth,” Applied Physics Letters 71, 1376-1378 (1997). A 12 56 G. Hess, P. Parkinson, B. Gong, Z. Xu, D. Lim, M. C. DOWNER, S. John, S. Banerjee, J. G. Ekerdt, and S. K. Jo, “Evolution of subsurface hydrogen from boron-doped Si(100),” Applied Physics Letters 71, 2184-2186 (1997). C 9 57 Y. S. Lee and M. C. DOWNER, “Reflected fourth harmonic radiation from a centrosymmetric crystal,” Optics Letters 23, 918-920 (1998). A 2 58 C. M. Fauser, E. Gaul, S. P. Le Blanc, and M. C. DOWNER, “Optical guiding characteristics of a standing acoustic wave in a piezoelectric cylinder,” Applied Physics Letters 73, 2902-2904 (1998). A 2 59 J. Koga, S. Kato, Y. Kishimoto, S. P. Le Blanc, and M. C. DOWNER, “Optical field ionization effects on the generation of wakefields with short pulse lasers,” Nuclear Instruments and Methods in Physics Research A 410, 499-504 (1998). A 27 60 O. A. Aktsipetrov, A. A. Fedyanin, A. V. Milnikov, E. D. Mishina, A. N. Rubtsov, M. H. Anderson, P. T. Wilson, M. ter Beek, X. F. Hu, J. I. Dadap, and M. C. Downer, “DC-electric-field-induced and low-frequency electromodulation second-harmonic generation spectroscopy of the Si(001)-SiO2 interface,” Physical Review B 60, 8924-8938 (1999). 61 M. K. Grimes, A. R. Rundquist, Y.-S. Lee, and M. C. DOWNER, “Experimental identification of vacuum heating at femtosecond-laser-irradiated metal surfaces,” Physical Review Letters 82, 4010-4013 (1999). C 12 62 P. S. Parkinson, D. Lim, R. Büngener, M. C. DOWNER, and J. G. Ekerdt, “Second harmonic spectroscopy of Ge/Si(001) and Si1-xGex(001)/Si(001),” Applied Physics B 68, 641-648 (1999). A 8 63 R. Kempf, P. T. Wilson, M. C. DOWNER, E. Mishina, O. A. Aktsipetrov, “Third and fourth harmonic generation from Si-SiO2 interfaces and in Si-SiO2-Cr MOS structures,” Applied Physics B 68, 325-332 (1999). A 30 64 P. T. Wilson, Y. Jiang, O. Aktsipetrov, E. Mishina, M. C. DOWNER, “Frequency domain interferometric second harmonic spectroscopy,” Optics Letters 24, 496-498 (1999). A 24 65 T. Tajima, Y. Kishimoto, and M. C. DOWNER, “Optical properties of clustered plasma,” Physics of Plasmas 6, 3759-3764 (1999). C 2 66 Y. –S. Lee and M. C. DOWNER, “Reflected optical fourth harmonic generation at crystalline surfaces,” Thin Solid Films 364, 80-85 (2000). A 14 67 V. I. Gavrilenko. R. Q. Wu, M. C. DOWNER, J. G. Ekerdt, D. Lim, P. Parkinson, “Optical second harmonic spectra of silicon ad-atom surfaces: theory and experiment,” Thin Solid Films 364, 1-5 (2000). C 5 68 L. Mantese, K. Selinidis, P.T. Wilson, D. Lim, Y.Y. Jiang, J. G. Ekerdt, M. C. DOWNER, “In-situ control and monitoring of doped and compositionally-graded SiGe films using spectroscopic ellipsometry and second harmonic generation,” Applied Surface Science 154-155, 229-237 (2000). A 28 69 D. Lim, M. C. DOWNER, J. G. Ekerdt, N. Arzate, B. S. Mendoza, V. Gavrilenko, and R. Wu, "Optical second harmonic spectroscopy of boron-reconstructed Si(001)," Physical Review Letters 84, 3406-3409 (2000). A 9 70 S. P. Le Blanc, E. W. Gaul and M. C. DOWNER, “Single-shot ultrafast phase measurement by frequency domain holography,” Optics Letters 25, 764-766 (2000). A 33 A page 5 Refereeed Journal Publications updated 1/3/08 9 71 N. Andreev, M. V. Chegotov, M. C. DOWNER, E. W. Gaul, N. M. Matlis, A. A. Pogosova, and A. R. Rundquist, "Propagation of intense laser pulses through inhomogeneous ionizing gas profiles," IEEE Transactions on Plasma Science 28, 1090-1097 (2000). C 8 72 D. Lim, M. C. DOWNER, J. G. Ekerdt, “Second-harmonic spectroscopy of bulk boron-doped Si(001),” Applied Physics Letters 77, 181-183 (2000). A 40 73 E. W. Gaul, S. P. LeBlanc, A. R. Rundquist, R. Zgadzaj, H. Langhoff and M. C. DOWNER, “Production and characterization of a fully-ionized He plasma channel,” Applied Physics Letters 77, 4112 (2000). A 18 74 Y. Jiang, P. T. Wilson, M. C. DOWNER, C. W. White and S. P. Withrow, “Second-harmonic generation from silicon nanocrystals embedded in SiO2,” Applied Physics Letters 78, 766-768 (2001). A 13 75 V. I. Gavrilenko, R. Q. Wu, M. C. DOWNER, J. G. Ekerdt, D. Lim, P. Parkinson, “Optical second harmonic spectra of Si(001) with H and Ge ad-atoms: first principles theory and experiment,” Physical Review B 63, 165325-165332 (2001). C 76 F. Breitling, R. S. Weigel, M. C. DOWNER, T. Tajima, “Laser pointing stability control by neural network in submicroradian regime,” Review of Scientific Instruments 72, 1339-1342 (2001). D 29 77 M. C. DOWNER, B. S. Mendoza and V. I. Gavrilenko, “Optical second harmonic spectroscopy of semiconductor surfaces: advances in microscopic understanding,” Surface and Interface Analysis 31, 966986 (2001). A 2 78 M. C. DOWNER, Y. Jiang, D. Lim, L. Mantese, P. T. Wilson, B. S. Mendoza, and V. I. Gavrilenko, “Optical second harmonic spectroscopy of silicon surfaces, interfaces and nanocrystals,” physica status solidi (a) 188, 1371-1381 (2001). A 5 79 Y. Jiang, L. Sun, and M. C. Downer, “Second-harmonic spectroscopy of two-dimensional Si nanocrystal layers embedded in SiO2 films,” Appl. Phys. Lett. 81, 3034-3036 (2002). A 80 M. C. Downer, "A New Low for Nonlinear Optics," Science 298, 373-375 (2002). A 6 81 P. T. Wilson, Y. Jiang, R. Carriles, and M. C. DOWNER, "Optical second-harmonic amplitude and phase spectroscopy by use of broadbandwidth femtosecond pulses," J. Opt. Soc. Am. B 20, 2548-2561 (2003). A 1 82 E. Mishina, N. Tanimura, S. Nakabayashi, O. A. Aksipetrov and M. C. DOWNER, "Photomodulated secondharmonic generation at silicon-silicon oxide interfaces: from modelling to application," Jpn. J. Appl. Phys. 42, 6731-6736 (2003). C 83 K. Wu, J. D. Canterbury, P. T. Wilson and M. C. DOWNER, "Electric-field-induced second-harmonic microscopy," phys. stat. sol. (c) 0, 3081-3085 (2003). A 84 Jinhee Kwon and M. C. DOWNER, "Reflectance-difference and second-harmonic generation: a meeting of two spectroscopies," phys. stat. sol. (c) 0, 3055-3060 (2003). A 8 85 C. Chiu, M. Fomytskyi, F. Raischel, F. Grigsby, M. C. DOWNER and T. Tajima, "Laser accelerators for radiation medicine: a feasibility study," Med. Phys. 31, 2042-2052 (2004). C 10 86 K. K. Kainz, K. R. Hogstrom, J. A. Antolak, P. R. Almond, C. D. Bloch, C. Chiu, M. Fomytskyi, F. Raischel, M. C. DOWNER and T. Tajima, "Dose properties of a laser accelerated electron beam and prospects for clinical application," Med. Phys.31, 2053-2067 (2004). C 2 87 R. Zgadzaj, E. W. Gaul, N. H. Matlis, M. C. DOWNER, and G. Shvets," Femtosecond pump-probe study of preformed plasma channels," J. Opt. Soc. Am. B 21, 1559-1567 (2004). A 2 88 M. Fomytskyi, C. Chiu, F. Grigsby and M. C. DOWNER, "Controlled plasma wave generation and particle acceleration through seeding of the forward Raman instability," Physics of Plasmas 12, 023103 (2004). A page 6 Refereeed Journal Publications updated 1/3/08 12 89 P. Figliozzi, L. Sun, Y. Jiang, N. Matlis, B. Mattern, M. C. DOWNER, S. P. WIthrow, C. W. White, W. L. Mochán and B. S. Mendoza, “Single-beam and enhanced two-beam second-harmonic generation from silicon nanocrystals by use of spatially inhomogeneous femtosecond pulses,” Phys. Rev. Lett. 94, 047401 (2005). A 3 90 L. Sun, P. Figliozzi, Y. Q. An, M. C. DOWNER, W. L. Mochán and B. S. Mendoza, “Nonresonant quadrupolar second-harmonic generation in isotropic materials using two orthogonally polarized laser beams,” Optics Letters 30, 2287-2289 (2005). A 1 91 Jinhee Kwon, M. C. DOWNER and B. S. Mendoza, "Second-harmonic and reflectance-anisotropy spectroscopy of vicinal Si(001)/SiO2 interfaces: experiment and simplified microscopic model," Phys. Rev. B 73, 195330 (2006). A 1 92 R. Carriles, J. Kwon, J. C. Miller, Y. Q. An, M. C. DOWER, J. Price and A. C. Diebold, “Second-harmonic characterization of Si/Hf1-xSixO2 interfaces,” Appl. Phys. Lett. 88, 161120 (2006). A 1 93 R. Carriles, Y. Q. An and M. C. DOWNER, “Frequency-domain measurement of second harmonic phase,” phys. stat. sol. (b) 242, 3001-3006 (2005). A 94 J. Kwon and M. C. DOWNER, “Simplified bond model of spectroscopic SHG and RAS of oxidized and reconstructed vicinal Si(001),” phys. stat. sol. (c) 2, 3973-3977 (2005). A 95 L. Sun, P. Figliozzi, Y. Jiang, M. C. DOWNER, W. L. Mochán, B. S. Mendoza, “Second-harmonic spectroscopy of nano-interfaces,” phys. stat. sol. (c) 2, 4067-4071 (2005). A 96 D. Stoker, M.l C. DOWNER, M. F. Becker, J. W. Keto , “Optical third harmonic surface microscopy using ultrashort laser pulses,” phys. stat. sol. (c) 2, 3978-3982 (2005). D 97 B. T. Bowes, H. Langhoff, M. C. DOWNER, M. Wilcox, B. Hou, J. Nees and G. Mourou, “Femtosecond microscopy of radial transport in a micron-scale Al plasma excited at relativistic intensity,” Optics Letters 31, 116-118 (2006). A 98 J. A. Nees, B. Hou, N. M. Naumova, B. T. Bowes, A. Mordovanakis, E. Power, M. C. DOWNER, and G. Mourou, ”Distinctive physical effects and applications approaching the relativistic labmda-cubed regime,” J. Special Topics in Quantum Electronics 12, 223-232 (2006). C 99 R. Carriles, J. Kwon, Y. Q. An, L. Sun, S. K. Stanley, J. G. Ekerdt, M. C. DOWNER, J. Price, T. Boescke, and A. C. Diebold, “Optical characterization of process-dependent charging in hafnium oxide structures,” J. Vac. Sci. Technol. B 24, 2160-2168 (2006). A 7 100 N. H. Matlis, S. Reed, S. S. Bulanov, V. Chvykov, G. Kalintchenko, T. Matsuoka, P. Rousseau, V. Yanovsky, A. Maksimchuk, S. Kalmykov, G. Shvets and M. C. DOWNER, “Snapshots of laser wakefields,” Nature Physics 2, 749-753 (2006). A 2 101 B. Shim, G. Hays, R. Zgadzaj, T. Ditmire and M. C. DOWNER, “Enhanced harmonic generation from expanding clusters,” Physical Review Letters 98, 123902 (2007). A 102 T. Pfeifer and M. C. Downer, “Direct experimental observation of periodic intensity modulation along a straight hollow core optical waveguide,” J. Opt. Soc. Am. B 24, 1025-1029 (2007). A 103 K. Wu, R. Carriles and M. C. DOWNER, "Phase-sensitive electric-field-induced second-harmonic microscopy of metal-semiconductor junctions," J. Opt. Soc. Am. B. 24, 2736-2740 (2007). A 104 F. Grigsby, D. Peng and M. C. DOWNER, “Chirped-pulse Raman amplification for two-color high-intensity laser experiments,” submitted to J. Opt. Soc. Am. B (2007). A 105 Y. Q. An, R. Carriles and M. C. DOWNER, "Absolute phase and amplitude of second-order nonlinear optical susceptibility components at Si(001) interfaces," Physical Review B 75, 241307(R) (2007). A 106 Jinhee Kwon, R. Ehlert and M. C. DOWNER, "Optical second-harmonic and reflectance-anisotropy spectroscopy of molecular adsorption on Si(001) step-edges," in preparation (2007). A 2 page 7 Refereeed Journal Publications updated 1/3/08 107 A. Maksimchuk, S. Reed, S. S. Bulanov, V. Chvykov, G. Kalintchenko, T. Matsuoka, N. H. Matlis, S. Kalmykov, G. Shvets, M. C. DOWNER, C. R. Vane, J. R. Beene, D. Stracener, and D. R. Schultz, “Studies of laser wakeifeld structures and electron acceleration in underdense plasmas,” Physics of Plasmas, in press (2008). C Book Chapters 53 *1 M. C. DOWNER, ‘The puzzle of two-photon rare earth spectra in solids.” in Laser Spectroscopy of Solids II, ed. W.M. Yen (Springer-Verlag 1988), chapter 2, pp.29-75. A 2 2 G. W. Burdick and M. C. DOWNER, "One-photon rare earth optical transitions: recent theoretical developments." In Solid State Luminescence - Physics, Materials, and Devices, A. H. Kitai, ed., (Chapman and Hall, 1992), chapter 1, pp 97-126. A 2 3 M. C. DOWNER, H. Ahn, D. H. Reitze, D. M. Riffe, and X. Y. Wang, "Properties of condensed matter under planetary interior conditions measured by femtosecond spectroscopy." In Laser Interactions with Atoms, Solids and Plasmas, R. M. More, ed. (Plenum Publishing Corp., New York, 1994) pp. 249-271. A * cited both by book title "Laser Spectroscopy of Solids" (42) and series title "Topics in Applied Physics" (11) 3268 TOTAL CITATIONS (based on Science Citation Index via ISI Web of Science)