Supplementary material of “Controllable plasmonic antennas with ultra narrow bandwidth based on silver nano-flags” Xiao-Yang Zhang,1,4 Tong Zhang,1,4, a) A. Hu,2 Yuan-Jun Song,1 and W. W. Duley3 1 School of Electronic Science and Engineering, Southeast University, and Key Laboratory of Micro-Inertial Instrument and Advanced Navigation Technology, Ministry of Education, Nanjing, 210096, People’s Republic of China 2 Department of Mechanical and Mechatronics Engineering, University of Waterloo, 200 University Avenue West, Waterloo, ON, N2L 3G1, Canada 3 Department of Physics and Astronomy, University of Waterloo, 200 University Avenue West, Waterloo, ON, N2L 3G1, Canada 4 Suzhou Key Laboratory of Metal Nano-Optoelectronic Technology, Suzhou Research Institute of Southeast University, Suzhou, 215123, People’s Republic of China Corresponding author: a) E-mail: tzhang@seu.edu.cn 1 Three-dimensional finite element method was used to simulate the optical properties of the silver nanostructures accurately. For short silver nano-flags, short nanowire (L = 300 nm) and the nanoplates, the numerical model is illustrated in Figure S1. The nanostructures were placed in the center of a rectangle with side widths of several micrometers. As the size of the short nano-flags is only 300 nm, they can be used as nano-antennas to trap and enhance the intensity of light with certain wavelengths significantly in nanoscale. To investigate the polarization-dependent spectral signature of the short nano-flag under the excitation of polarized incident light with controllable incident angle, the top boundary condition was set to be the input light source with rectangular wave (transverse magnetic (TM) 01 mode). To realize a certain incident polarization direction in the simulation, we kept the original polarization angle of the incident light unchanged and rotated the nanostructure according to the center of the input boundary along z axis. Scattering boundary condition1 was used at the other outer boundaries. We found that the light excitation processes can be efficiently simulated when TM 01 mode was used as the source boundary. The validity of our numerical model are confirmed as the simulation results shown in Fig 1 (b) and (c) are well matched with the experimental and theoretical results reported by other researchers.2-5 2 Figure S1. Illustration of the simulation cell and boundary conditions of the short nano-flag seen from the views of x-y plane (a) and y-z plane (b), respectively. The light source boundary was labeled in red color. The dashed lines illustrate the positions of light the source boundary and the integrated nanoplate, respectively. For long silver nano-flags and long nanowires (L = 2 µm), the numerical model is illustrated in Figure S2. The nanostructures were placed in a rectangle with side width of ~ 2µm and a length of ~ 5µm. To simulate the end excitation strategy of the long nano-flag and long nanowires as shown in the inset of Figure 2 (b), we set a light boundary as illustrated in Figure S2 (a) and (b). A square with a side width of 300 nm labeled in red show the position of the input light source with rectangular wave (transverse magnetic 01 mode). The end excitation strategy was used because such long nano-flags can 3 be used as resonators or switches controlled from the far-end.2 From Figure S2 (b) one can see the distance between the plane of the light source boundary and the nano-flag is 300 nm in z direction. Scattering boundary condition was used at the other area of the outer boundary of the rectangle. Non-uniform meshes are adopted to reduce the memory requirement and ensure high accuracy. Finer meshes with a maximum element size of ~1 nm – 2 nm, and an element growth rate of ~1.05 – 1.1 were used in the sub-domains such as the end of the nanowire and the tip of the nanoplate shown in Figures S2 (c) and (d). Meshes with a maximum element size of 8 nm – 15 nm, and an element growth rate of ~1.1 – 1.15 were used in the other domains of the nanostructures, such as the junction of the nanowire and the nanoplate shown in Figure S2 (e). 4 Figure S2. Illustration of the simulation cell and boundary conditions of the long nano-flag seen from the views of x-y plane (a) and y-z plane (b), respectively. The light source boundary was labeled in red color. The dashed lines illustrate the positions of light the source boundary and the integrated nanoplate, respectively. (c) - (e) show the details of the mesh grids of the nano-flag at the end of the nanowire, the tip of the nanoplate, and the junction of the nanowire and the nanoplate from the view of x-y plane, respectively. References 1 2 COMSOL Multiphysics 3.5 User’s Guide. Stockholm: COMSOL, 2008. M. W. Knight, N. K. Grady, R. Bardhan, F. Hao, P. Nordlander, and N. J. Halas. 5 Nanoparticle-Mediated Coupling of Light into a Nanowire, Nano lett. 7, 2346 (2007). 3 H. Ditlbacher, A. Hohenau, D. Wagner, U. Kreibig, M. Rogers, F. Hofer, F. R. Aussenegg, and J. R. Krenn, Phys. Rev. Lett. 95, 257403 (2005). 4 X. -Y Zhang, A. M. Hu, T. Zhang, W. Lei, X. -J. Xue, Y. H. Zhou, and W. W. Duley, ACS Nano 5, 9082 (2011). 5 I. Pastoriza-Santos, and L. M. Liz-Marzán, Colloidal silver nanoplates. State of the art and future challenges, J. Mater. Chem. 18, 1724 (2008) 6