Direct observation of electro-optic modulation in a single split-ring resonator Dmitry Yu. Shchegolkov1, Matthew T. Reiten1, John F. O’Hara2, and Abul K. Azad1* 1 2 Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA School of Electrical and Computer Engineering, Oklahoma State University, Stillwater, OK 74078, USA Supplementary Materials: Theory of polarization rotation with zinc-blende type crystals. For observation of the electro-optic nonlinearity we used [1,1,0] cut ZnTe, the crystal which has zinc-blende lattice type and one of the strongest quadratic (Pockels type) nonlinearities [1]. U2 Eo [0,0,1] U1 β Erf οΉ α [-1,1,0] Fig. 1. Axes assignment in a [1,1,0] plane of a zinc-blende crystal. Erf – direction of applied quasi-static field, Eo – direction of electric field in linearly polarized optical beam. U1 and U2 – axes along crystal's eigen polarizations. Applying electric field to ZnTe crystal induces birefringence, so that in [1,1,0] cut crystal the two normal polarizations, which are linear in this case, can be characterized by an angle οΉ between the crystal axis [-1,1,0] and the direction of the electric field in one of them, U1, the other one, U2, being orthogonal (Fig. 1). The angle depends on the direction of the applied in-plane quasi1 static electric field πΈππ , which we will characterize by an angle α with the same axis [-1,1,0]. We will be doing sampling of the induced birefringence with a linearly polarized laser beam which electric field Eo has an angle β with [-1,1,0] crystal direction. The dependence of normal polarizations on the direction of applied quasi-static electric field Erf is as following [2]: sinα πππ 2οΉ = √1+3cos2 . (1) α The relative phase shift between two polarizations after passing through the crystal is π€= π0 π π (π1 − π2 ) = ππ π0 π03 π41 πΈππ √1 + 3πππ 2 πΌ, (2) where d is the crystal thickness, π0 is the refractive index, π41 is the electro-optic coefficient, π0 is the probe beam's wavelength in vacuum. In the coordinate system associated with normal polarizations (U1, U2) the incident field amplitude can be written as π¬π = πΈ0 β (πππ (π½ − οΉ), π ππ(π½ − οΉ)). After passing through the crystal it will turn into π¬1 = πΈ0 β (πππ (π½ − οΉ)π ππ€⁄2 , π ππ(π½ − οΉ)π −ππ€⁄2 ). The main linear in Γ effect here is appearance of an orthogonal polarization, 90 degrees out of phase to the wave of initial polarization. In order to transform it into effective polarization rotation, a quarter wave plate oriented in accordance with Eo direction is used, so that after a quarter wave plate the orthogonal polarization oscillates in phase with the main component and this is used for further detection. The amplitude of the orthogonal polarization is |π¬1⊥ | = πΈ0 π€ |π ππ2(π½ − οΉ)|⁄2. After Wollaston prism oriented to separate the wave of initial polarization into two beams of equal power we get those beams amplitudes as following: 2 πΈ0 β ( 1 √2 ± π€ 2√2 |π ππ2(π½ − οΉ)|). Using two balanced square-law detectors, that results in voltage difference signal πΌ = ππΈ02 π€|π ππ2(π½ − οΉ)|, where constant π characterizes detector sensitivity and is determined by its internal properties. For β=90β° we get ππ πΌ = ρπΈ02 π€|π ππ2οΉ| = 2 π π03 π41 πΈππ πΈ02 πππ πΌ, 0 (3) where formulas (1) and (2) were used. The maximum signal corresponds to πΌ = 0. In our experiment we had [1,1,0] ZnTe crystal sample cut at 45 degrees to its axes and β=135β°, that results in πΌ = ππΈ02 π€|πππ 2οΉ| = ππ π0 π03 π41 πΈππ πΈ02 π πππΌ. (4) Provided that the RF field in the SRR gap in our experiment had an angle α=45β°, that gives 2√2 times lower EO signal compared to the previous case (3) and α=0. References: [1] B. Clough, D. H. Hurley, P. Han, J. Liao, R. Huang, and X.-C. Zhang, Sens. Imaging 10, 55 (2009). [2] S. Casalbuoni, H. Schlarb, B. Schmidt, P. Schmuser, B. Steffen, and A. Winter, TESLA Report (2005-01) 3