Remediation of Land Affected by Radioactive Residues Proceedings of an International Conference on the Remediation of Land Affected by Radioactive Residues Organized by the International Atomic Energy Agency, Hosted by the Government of Kazakhstan and held in Astana, 18-22 May 2009 International Atomic Energy Agency REMEDIATION OF LAND AFFECTED BY RADIOACTIVE RESIDUES The following States are Members of the International Atomic Energy Agency: AFGHANISTAN ALBANIA ALGERIA ANGOLA ARGENTINA ARMENIA AUSTRALIA AUSTRIA AZERBAIJAN BAHRAIN BANGLADESH BELARUS BELGIUM BELIZE BENIN BOLIVIA BOSNIA AND HERZEGOVINA BOTSWANA BRAZIL BULGARIA BURKINA FASO BURUNDI CAMBODIA CAMEROON CANADA CENTRAL AFRICAN REPUBLIC CHAD CHILE CHINA COLOMBIA CONGO COSTA RICA CÔTE D’IVOIRE CROATIA CUBA CYPRUS CZECH REPUBLIC DEMOCRATIC REPUBLIC OF THE CONGO DENMARK DOMINICAN REPUBLIC ECUADOR EGYPT EL SALVADOR ERITREA ESTONIA ETHIOPIA FINLAND FRANCE GABON GEORGIA GERMANY GHANA GREECE GUATEMALA HAITI HOLY SEE HONDURAS HUNGARY ICELAND INDIA INDONESIA IRAN, ISLAMIC REPUBLIC OF IRAQ IRELAND ISRAEL ITALY JAMAICA JAPAN JORDAN KAZAKHSTAN KENYA KOREA, REPUBLIC OF KUWAIT KYRGYZSTAN LATVIA LEBANON LESOTHO LIBERIA LIBYAN ARAB JAMAHIRIYA LIECHTENSTEIN LITHUANIA LUXEMBOURG MADAGASCAR MALAWI MALAYSIA MALI MALTA MARSHALL ISLANDS MAURITANIA MAURITIUS MEXICO MONACO MONGOLIA MONTENEGRO MOROCCO MOZAMBIQUE MYANMAR NAMIBIA NEPAL NETHERLANDS NEW ZEALAND NICARAGUA NIGER NIGERIA NORWAY OMAN PAKISTAN PALAU PANAMA PARAGUAY PERU PHILIPPINES POLAND PORTUGAL QATAR REPUBLIC OF MOLDOVA ROMANIA RUSSIAN FEDERATION SAUDI ARABIA SENEGAL SERBIA SEYCHELLES SIERRA LEONE SINGAPORE SLOVAKIA SLOVENIA SOUTH AFRICA SPAIN SRI LANKA SUDAN SWEDEN SWITZERLAND SYRIAN ARAB REPUBLIC TAJIKISTAN THAILAND THE FORMER YUGOSLAV REPUBLIC OF MACEDONIA TUNISIA TURKEY UGANDA UKRAINE UNITED ARAB EMIRATES UNITED KINGDOM OF GREAT BRITAIN AND NORTHERN IRELAND UNITED REPUBLIC OF TANZANIA UNITED STATES OF AMERICA URUGUAY UZBEKISTAN VENEZUELA VIETNAM YEMEN ZAMBIA ZIMBABWE The IAEA’s Statute was approved on 23 October 1956 by the Conference on the Statute of the IAEA held at United Nations Headquarters, New York; it entered into force on 29 July 1957. The Headquarters of the IAEA are situated in Vienna. Its principal objective is “to accelerate and enlarge the contribution of atomic energy to peace, health and prosperity throughout the world” PROCEEDINGS SERIES REMEDIATION OF LAND AFFECTED BY RADIOACTIVE RESIDUES PROCEEDINGS OF AN INTERNATIONAL CONFERENCE ON THE REMEDIATION OF LAND AFFECTED BY RADIOACTIVE RESIDUES ORGANIZED BY THE INTERNATIONAL ATOMIC ENERGY AGENCY, HOSTED BY THE GOVERNMENT OF KAZAKHSTAN AND HELD IN ASTANA, 18-22 MAY 2009 INTERNATIONAL ATOMIC ENERGY AGENCY VIENNA, 2012 FOREWORD In past decades, when supplies of uranium were urgently needed for nuclear weapons production and for nuclear energy generation, the emphasis of the industry was on production, often at the expense of the environment from which the uranium ore was taken. The uranium mining activities of this era have left a legacy of tailings piles and polluted land and water courses in many countries of the world. The need to restore the affected areas is now recognized and remediation programmes are under way in many countries. Uranium was mined in some countries which had no other nuclear or radiation related practices and, as a result, there is little or no expertise to manage the remediation. Furthermore, these countries tend to have only modest resources and so, finding funds to remediate the uranium legacy sites is often difficult. These problems have been recognized by the international community and efforts to assist countries in resolving them have been made in recent years. With this background, the International Atomic Energy Agency decided to organize an international conference on the Remediation of Land Affected by Radioactive Material Residues with the purpose of reviewing global progress in remediating areas affected by radioactive materials – with special emphasis on areas affected by former uranium mining and milling activities. The conference was held in Astana, Kazakhstan from 11 to 22 May 2009. This was the second conference organized by the International Atomic Energy Agency on this subject. The first was held in 1999 in Arlington in the United States of America and was titled ‘Restoration of Environments with Radioactive Residues: The Arlington conference was focused mainly on the cleanup of nuclear weapons test sites and areas affected by nuclear accidents. In contrast, the Astana conference was concentrated on legacy sites from uranium mining and milling activities. The Astana conference was organized in eight sessions: From Arlington to Astana – Lessons Learned, International Cooperation and Support in Environmental Remediation, Complying with Safety Criteria, Innovative Technologies in Environmental Remediation, Life Cycle Planning and Stakeholder Issues, Case Studies (2 sessions), and Expediting and Enhancing Experience Exchange. This publication, which constitutes the record of the conference, includes the opening address, the invited papers, the summaries of the individual sessions and the conference president’s summary. The IAEA gratefully acknowledges the support and generous hospitality of the Government of Kazakhstan in hosting this conference. The IAEA officers responsible for this publication were R. Edge of the Division of Radiation, Transport and Waste Safety and H. Monken Fernandes of the Division of Nuclear Fuel Cycle and Waste Technology. EDITORIAL NOTE The Proceedings have been edited by the editorial staff of the IAEA to the extent considered necessary for the reader’s assistance. The views expressed remain, however, the responsibility of the named authors or participants. In addition, the views are not necessarily those of the governments of the nominating Member States or of the nominating organizations. Although great care has been taken to maintain the accuracy of information contained in this publication, neither the IAEA nor its Member States assume any responsibility for consequences which may arise from its use. The use of particular designations of countries or territories does not imply any judgement by the publisher, the IAEA, as to the legal status of such countries or territories, of their authorities and institutions or of the delimitation of their boundaries. The mention of names of specific companies or products (whether or not indicated as registered) does not imply any intention to infringe proprietary rights, nor should it be construed as an endorsement or recommendation on the part of the IAEA. The authors are responsible for having obtained the necessary permission for the IAEA to reproduce, translate or use material from sources already protected by copyrights. CONTENTS CONFERENCE SUMMARY .................................................................................................... 1 OPENING SESSION Opening Address ........................................................................................................................ 7 H. Forsstroem FROM ARLINGTON TO ASTANA – LESSONS LEARNED (Topical Session 1) Summary of the 1999 International Conference on the Restoration of Environments with Radioactive Residues .............................................................................................. 13 D.W. Reisenweaver Remediation of Contaminated Areas of Kazakhstan ............................................................... 17 A.M. Magauov International Policies and Strategies for the Remediation of Land Affected by Radioactive Residues ...................................................................................................... 21 A.J. González Assisting the Return to Normal Life in Chernobyl–Affected Regions: the International Chernobyl Research and Information Network (ICRIN) ............................................... 31 O. Leshchenko, L. Vinton, Z. Carr, D.H. Christie, V. Berkovskyy, E. Sherstyuk, A. Karankevich, E. Stanislavov SUMMARY OF SESSION 1 H. Forsstroem INTERNATIONAL COOPERATION AND SUPPORT IN ENVIRONMENTAL REMEDIATION (Topical Session 2) Remediation of Radioactively Contaminated Sites – Review of Projects Supported by the International Science and Technology Center (ISTC) .............................................. 41 V. Rudneva, W. Gudowski SUMMARY OF SESSION 2 S. Vorobiev COMPLYING WITH SAFETY CRITERIA (Topical Session 3) The Existing Regulatory Framework in Russia on Environmental Remediation .................... 51 N.K. Shandala, M.F. Kiselev, M.I. Balonov, M.K. Sneve US Policies for Cleanup at Radioactively contaminated sites ................................................. 57 S. Walker Principles of Uranium Stewardship: Guidance from the World Nuclear Association ............. 61 S. Saint-Pierre Adapting International Experience to Regulatory Supervision of Legacy Sites in the Central Asian Republics ................................................................................................. 67 M. Sneve, M. Kiselev, N. Shandala, T. Zhunussova, A. Kim, U. Mirsaidov, B. Tolongutov SUMMARY OF SESSION 3 A.J. González INNOVATIVE TECHNOLOGIES IN ENVIRONMENTAL REMEDIATION (Topical Session 4) Innovative Mathematical Modelling in Environmental Remediation ...................................... 79 G.T. Yeh, J.P. Gwo, M.D. Siegel, M. H. Li, Y.L. Fang, F. Zhang, W.S. Luo, S.B. Yabusaki Advances in the Application of Electrical Techniques for Site Remediation .......................... 85 D.F. Osborne Site Remediation in Practice .................................................................................................... 91 A. Várhegyi, G. Földing, Z. Berta , M. Csövári Monitored Natural Attentuation of Metals and Radionuclides in Soil and Groundwater ........ 97 M. Denham, K. Vangelas SUMMARY OF SESSION 4 V. Adams LIFE CYCLE PLANNING AND STAKEHOLDER ISSUES IN ENVIRONMENTAL RESTORATION (Topical Session 5) Balancing the Uranium Production Cycle: Central Asia as a Case Study ............................. 107 A.T. Jakubick, D.R. Metzler, P.Waggitt, R. Edge IAEA Preliminary Assessment of the Former French Nuclear Test Sites in Algeria ............ 119 D.W. Reisenweaver Social and Ethical Issues in Remediation .............................................................................. 127 D.H. Oughton A Guide for the Remediation of Radioactively Contaminated Sites: EURSSEM ................. 131 L.P.M. Van Velzen, L. Teunckens, M. Vasko, E. Hajkova, V. Daniska, K. Kristofova Improving Radioactive Waste and Source Management at the Vinča Institute ..................... 139 M. Recio, J. Kelly, M. Kinker SUMMARY OF SESSION 5 M. Paul CASE STUDIES (ENVIRONMENTAL REMEDIATION IN CENTRAL ASIAN COUNTRIES) (Topical Session 6) Environmental Effects of Possible Landslides in the Areas of Radioactive Waste Storage in Kyrgyzstan ................................................................................................... 147 I.A. Torgoev, Y.G. Aleshin, G.E. Ashirov The Radiological and Environmental Situation Near to the Decommissioned Uranium Mines in Uzbekistan ..................................................................................................... 153 E.A. Danilova, A.A. Kist, R.I. Radyuk, G.A. Radyuk, U.S. Salikhbaev, P. Stegnar, A. Vasidov, A.A. Zhuravlev Multiple Stressors – Environmental Impact at Sites Contaminated with Radionuclides and Metals ..................................................................................................................... 159 B. Salbu Industrial Environmental Monitoring — a Land Restoration Costs Tracking Tool .............. 165 M. Iskakov, M. Nurgaziyev, B. Eleyushov, P. Kayukov SUMMARY OF SESSION 6 A. Kim CASE STUDIES II (Topical Session 7) Challenges in Estimating Public Radiation Dose Resulting from Land Application of Waters of Elevated Natural Radioactivity .................................................................... 173 P. Lu, R. Akber, A. Bollhöfer Experience of the Constraints Affecting the Implementation of Decommissioning/Remediation Programmes at Uranium Mining Sites ...................... 179 M.R. Franklin Lessons Learned from the Remediation at Villa Aldama Uranium Extraction Plant ............ 185 R. Fabian Ortega Occupational Exposure During Remediation Work at a Uranium Tailings Pile ................... 191 M.L. Dinis, A. Fiúza Baseline Radiological Survey of the Uranium–Bearing Region of Poli (Northern Cameroon) .................................................................................................................... 195 S. Saïdou, F. Bochud, S. Baechler, K.N. Moïse, P. Froidevaux Romanian Experience in the Remediation of NORM Contaminated Sites – A Case Study ............................................................................................................................. 203 O. Velicu, A. Toma Radioecological Assessment and Remediation Planning of Uranium Milling Facilities at the Pridneprovsky Chemical Plant in Ukraine .............................................................. 211 T.V. Lavrova, O.V. Voitsekhovych, M.G. Buzinny Experience Gained in Transferring WISMUT Radiation Protection Know–How to International Projects in Uranium Mining Remediation............................................... 217 P. Schmidt, C. Kunze, J. Regner Justification of Remediation Strategies in the Long Term After the Chernobyl Accident .... 223 S. Fesenko, P. Jacob, A. Chupov, A. Ulanovsky, I. Bogdevich, N. Sanzharova, A. Panov, N. Isamov, V. Kashparov, Y. Zhuchenka Experiences in the Remediation of Contaminated Land ........................................................ 229 I. Adsley, R. Murley, L. Fellingham, K. Stevens Assessment of Current Doses from Uranium Tailings........................................................... 235 R. Avila, O. Voitsekhovych, I. Zinger, P. Keyser SUMMARY OF SESSION 7 B. Salbu EXPEDITING AND ENHANCING EXPERIENCE EXCHANGE (Topical Session 8) The ENVIRONET – Network on Environmental Management and Remediation ................ 247 H. Monken-Fernandes SUMMARY OF SESSION 8 D. Louvat SUMMARY AND CONCLUSIONS OF THE CONFERENCE .......................................... 253 Report of the Conference President CHAIRPERSONS OF SESSIONS ........................................................................................ 257 PRESIDENT OF THE CONFERENCE ................................................................................ 257 SECRETARIAT OF THE CONFERENCE ........................................................................... 257 PROGRAMME COMMITTEE ............................................................................................. 257 ORGANIZING COMMITTEE IN KAZAKHSTAN ............................................................ 258 AUTHOR INDEX .................................................................................................................. 259 LIST OF PARTICIPANTS .................................................................................................... 261 CONFERENCE SUMMARY This conference was concerned with the progress being made globally in the remediation of land areas affected by radioactive residues. This was the second conference organized by the International Atomic Energy Agency on this subject. The first was held in 1999 in Arlington in the United States of America and was titled Restoration of Environments with Radioactive Residues. The Arlington conference was focused mainly on the cleanup of nuclear weapons test sites and areas affected by nuclear accidents. In contrast, the Astana conference was concentrated on legacy sites from uranium mining and milling activities. Uranium mining legacy sites exist in many countries and result mainly from mining activities in the period 1950–1990 when uranium was being sought globally for nuclear weapons and for nuclear energy generation. Some of the countries affected are among the poorest of nations. The problems that these countries have in remediating their legacy sites stem mainly from the lack of available economic and human resources. The uranium mining site remediation issue has emerged strongly in recent years since the end of the Cold War. In response, the international organizations have begun to provide support to the countries concerned in addressing the problems, especially to the countries of Central Asia. It was mainly for this reason that the conference was held in Astana the capital city of Kazakhstan. The conference was designed to cover all relevant aspects related to environmental remediation including: Regulatory and Safety Regimes, Innovative and Mature Technologies, Life-Cycle Planning, Technical Experience Exchange, and Stakeholder Issues and International Cooperation and Support. A series of case study presentations was organized to provide the participants with an overview of environmental remediation activities in different parts of the world. A special session addressed environmental remediation in Central Asian Countries (Kazakhstan, Kyrgyzstan, Tajikistan and Uzbekistan) where many legacy sites were created without proper consideration of the associated environmental impacts. Unlike most other areas of radiation protection, there is not a global consensus on radiological principles and criteria for the remediation of areas affected by radioactive contamination. This was shown at the Arlington conference where a wide variation in the radiological criteria being used as the basis for decisions on the cleanup of contaminated areas was demonstrated. Most of the concern at Arlington was with artificial radionuclides. In the context of the present conference, it is relevant to consider if the criteria should be the same when the contamination is caused by naturally occurring radioactive material. Guidance on radiological criteria for remediation has been given by the international organizations but it is by no means universally accepted, especially by the persons living in the affected areas. Despite the fact that, in many situations, such as the areas affected by the Chernobyl release, the exposures to radiation are low, and below the levels of acceptability recommended by national and international organizations, the population living in these areas remain unconvinced. In some of the countries in which uranium has been mined, the regulatory infrastructure is weak and is not yet capable of ensuring that tailings remediation operations are conducted safely. Efforts are being made to correct this situation by the transfer of experience and expertise from industrialized countries. The progress of this work, which involves national and international organizations, was reported at the conference. It is clear that many of the environmental problems that have resulted from the mining and milling of uranium could have been avoided with proper planning during the uranium extraction phase. Nowadays, life cycle planning is being emphasised as a strategy for avoiding the generation of future legacy sites. Life cycle planning means considering the potential environmental and other impacts at all stages in the life of a facility, e.g. design, 1 CONFERENCE SUMMARY construction, operation, closure and decommissioning, and planning to avoid them. A session focussing on this strategy was an important element of the conference. A major aim of the conference organizers was to promote the transfer of remediation technology from countries which already have considerable experience in addressing the problem to countries which are relative newcomers to the subject. It was also intended to provide countries having similar problems with an opportunity to exchange information. Special sessions of case studies were included for this purpose. The aims of these information transfer sessions are similar to those of an IAEA networking initiative called ENVIRONET whose objectives are to provide coordinated support, to organize training and demonstration events, and to foster information exchange by establishing a forum for discussion in different areas. The final structure of ENVIRONET is still being developed but the programme was formally announced at the General Conference of the IAEA in October 2009. Remediation activities often affect local populations by requiring them to change their habits and lifestyles or even to be relocated. For these reasons, the concerned public must be part of the decision making process and formal arrangements must be established to enable this to happen. In recognition of the importance of this topic, often termed ‘stakeholder involvement’, it was specifically addressed in one of the conference sessions. The problems associated with the uranium mining legacy sites in the countries in Central Asia are well known and many international organizations are interested in providing assistance to the concerned countries. However, to date, the coordination between them has been less than optimal and this conference led to an agreement among the participating international organizations that a mechanism to facilitate coordination is desirable. The concerned organizations include the European Commission (EC), the International Science and Technology cleanup (ISTC), the European Bank for Research and Development (EBRD), the North Atlantic Treaty Organization (NATO), the Organization for Security and Cooperation in Europe (OSCE), the World Bank, the World Health Organization (WHO) and the IAEA. In this context, it was suggested that the mechanism used by the IAEA for coordinating international and bi-lateral cooperation in northern Russia (the Contact Expert Group (CEG)) could be used as a model for coordinating international cooperation in Central Asia. In summary, environmental contamination of land with radionuclides is a problem in many countries. The policies and regulatory strategies for managing the remediation of affected areas are not yet harmonized globally although there is considerable experience in the world on remediation technology. Some of the concerned countries have insufficient resources and expertise to properly manage the remediation required to render the affected areas fit for human use and occupancy. Efforts in the future should therefore be focused on unifying regulatory policies and strategies, promoting the transfer of knowledge and, where necessary, supporting countries in their efforts to remediate their lands. In the third session, the progress of the relevant international organizations in developing recommendations and guidance to ensure the safety of remediation were summarized and, in addition, the international operators’ organization, the World Nuclear Association, presented its safety code of practice for industry. The development of regulatory frameworks in Russia and in the United States of America (USA) were described as well as a Norwegian-led initiative to improve regulatory supervision in the countries of Central Asia. The discussion in this session led to a recognition of the need for coordination among regulatory authorities and it was suggested that an international forum for the regulatory supervision of legacy sites should be created. Different technologies for the remediation of sites were discussed in Session 4. It was shown that local conditions have to be well understood in order to design appropriate cover systems for uranium tailings piles. Bioremediation techniques are still at the stage of development but it was demonstrated that this is a particularly attractive solution for 2 CONFERENCE SUMMARY situations where the groundwater reservoir is deep and difficult to access. Natural Monitored Attenuation is an approach in which the attenuation of the migration of the contaminant by natural processes is utilised. In many cases, if a sufficiently good understanding of the location and movement of the contaminant plume can be obtained, no further remedial measures may be needed. This approach seems to be gaining support in the USA from the cost perspective; it is an alternative to treating large volumes of water for long periods of time. Electrical vitrification of contaminated soil to produce a solid matrix has been applied at various sites around the world. Its main advantage is that it creates a waste form that isolates the radionuclide or metal contaminants and prevents leaching by water. Because of this, it avoids the long term monitoring that other waste storage options require. Mathematical modelling is an essential tool for the design and performance assessment of remediation solutions. Most models use of the Kd approach but since this approach not really represent the processes taking place in the environment, it must be used with caution. Instead, it was recommended that reactive transport models should be used whenever the necessary data can be obtained. Along the same lines, the planning approach used by the US Department of Energy (DOE) to manage environmental remediation projects was presented. It was pointed out that the regulator must be involved in the overall management programme as well as the stakeholders. In relation to the session (Session 6) devoted to the Central Asian countries (Kazakhstan, Tajikistan, Uzbekistan and Kyrgyzstan) it was evident that the countries share common problems, such as, similar histories and geographical locations for the tailings sites, a lack of funds to deal with remediation, a lack of local expertise and equipment and, as a result, inadequately characterized sites. Furthermore, the radiological conditions of people living near to the sites may not be known. Each country has particular conditions that have caused the situation to worsen. In some areas, precipitation has caused an increase in erosion, landslides have caused significant changes in previously stable storage sites and residues have been used as building material in homes and public buildings such as schools. If solutions are not implemented in a timely manner, the possibility exists that contamination from one country could cross national borders and cause contaminated areas in surrounding countries. So far, only preliminary studies have been conducted at the Central Asian legacy sites. It was concluded that near term actions for all of these sites should involve: measurement and assessment studies in order to gain an understanding of the radiological situation at each site; the identification of alternative water supplies if ground water has been contaminated; the maintenance of institutional controls at the sites; routine monitoring to ensure controls are performing their intended functions; and finally, the enhancement of public awareness of the local situation. It was stressed that decisions on intervention at these sites must be the result of a comprehensive risk assessment, and decision making based solely on the perceived risk must be resisted. It was noted in one study that risk assessment studies should take account of all the risks present, not just those due to radionuclides. It is often the case that other pollutants are present together with radionuclides; they are typically heavy metals and chemicals. More case studies were discussed in Session 7. In some countries environmental remediation works cannot be easily implemented by local technical people and international assistance is essential. However, working in different juridical, social and political environments has proved to be difficult. As a result, local capacity building is of utmost importance and this is an essential role to be played by the relevant international organizations. Stakeholder involvement in the context of environmental remediation emerged as one of the most important themes discussed during the conference. Many presentations highlighted 3 CONFERENCE SUMMARY the importance of effective stakeholder involvement in reaching solutions which satisfy all parties. 4 OPENING SESSION OPENING ADDRESS H. Forsstroem International Atomic Energy Agency Vienna Your Excellency, Mr Minister, Mr Mayor, on behalf of all of us I would like to thank you very much for the warm welcome that we have received coming to Astana this week and for the excellent preparations for this international conference. Ladies and Gentlemen, dear Colleagues, we have come to Astana to discuss the challenges involved in the remediation of lands affected by radioactive residues, which is an international problem. In the past, many industries, such as the uranium mining industry, were often developed without deep consideration of environmental issues in the overall planning and implementation of their operations. Many of these industries operated in an environment that did not have appropriate or effective environmental laws and regulations. As a result, many contaminated sites have been created. Other nuclear activities, e.g. defence programmes and the Cold War legacy, as well as nuclear and radiological accidents, such as Chernobyl and Goiania, also created important legacy sites. Such sites can lead to undesired health effects for members of the public and harm to the environment. The objective of environmental remediation is to mitigate the radiation exposure from existing areas of contaminated land to reduce exposures now and in the future. The main goal is, if possible, to release the land for unrestricted use, which means total removal from regulatory control. However, there are situations in which the removal from regulatory control cannot be practically achieved. In these cases, once the cause of unacceptable risks to man and environment is removed, restrictions on access and use of the area must be established and long term stewardship schemes put in place. It is important to remember that remediation can be done not only by removing the contamination itself but also through other actions that prevent the contamination from influencing human and non-human biota. From the perspective of radiation safety, two main principles govern the decision making for any remediation programme. Firstly, justification, the implementation of the remediation programme shall produce more good than harm; and secondly optimization, working to ensure that the residual doses will be as low as reasonably achievable, social and economic factors taken into account. Therefore, when selecting an optimized remediation option, a wide variety of factors need to be considered. The need to address radiological liabilities has been increasingly recognized since the end of the Cold War. However, in many Member States, remediation programmes have made little progress beyond the assessment and/or planning stages. One reason for this is that the costs of remediating contaminated sites can be very high and. in many cases. these costs cannot easily be met, even by the State. Just to give you an example of the costs involved on environmental remediation projects, in the United States of America (USA) more than US $5 billion are spent per year on activities related to environmental remediation. In many cases, remediation might require that resources have to be diverted from other priority actions in order to improve the environmental conditions of a particular site or region. It is thus critical to develop remediation projects together with all interested parties and, in particular, with the local communities. Today, with increasing activity in uranium production, the challenge for the international community is to avoid that new legacy sites are created. This can be achieved through the development of sustainable good practices and stewardship principles throughout 7 OPENING ADDRESS the global uranium production industry. There is a need for active promotion of the concept of lifecycle planning at the early stages. This is valid for all projects – be they remediation of legacy sites, establishment of new developments, such as uranium mines, or re-development of legacy sites for renewed production of radioactive minerals. In this context, the development of a widespread safety culture and the building of relevant safety infrastructures and competences are key factors. The present situation in the Central Asian countries is an illustrative example. One of the reasons that this conference is taking place in Kazakhstan is to highlight the need to find a viable and effective architecture to address the remediation of the existing legacy sites, which have resulted from the inappropriate development of several uranium mining and milling operations. The mining enterprises that extracted uranium and rare earth elements for over 50 years in Central Asia have left behind very large amounts of industrial waste, including radioactive residues. Recent initiatives by the International Atomic Energy Agency concerning the former uranium mining and production activities in Central Asia include cooperation and communication with other international organizations. We expect that improved coordination among affected countries and international organizations will result in a regional initiative to tackle the health and environmental consequences of these legacies. Meanwhile, the IAEA provides comprehensive assistance at both national and regional levels with the aim of upgrading institutional capabilities. So far, the main focus of this assistance has been on upgrading regulatory control, and expanding environmental monitoring and laboratory analysis capabilities in full compliance with the International Safety Standards. In the future, the emphasis will shift to helping States to fully implement environmental remediation programmes. Another very important case of environmental remediation is concerned with the Chernobyl accident that took place in 1986. It resulted in a very large release of radionuclides to the environment. The Chernobyl Forum, which was an initiative grouping together the three affected countries and eight United Nations organizations, completed its tasks in 2005 and issued consensus reports on the health, environmental, social and economic consequences of the Chernobyl accident. The Forum also provided directions for future actions and, in particular, for the remediation of contaminated territories, the decommissioning of the Chernobyl NPP and the management of radioactive waste resulting from these operations. As a follow up, the IAEA is carrying out a regional programme of technical cooperation on the remediation of agricultural land and it is supporting the Ukraine in decommissioning planning and radioactive waste management. As we all know, there have been other activities that resulted in the contamination of extensive areas. The former nuclear weapons testing programmes radioactively contaminated large territories in many places. Here, in Kazakhstan, there are still 16 000 km2 where public use is restricted. The IAEA has provided an independent assessment of the radiological situation at some of these former test sites and is prepared to continue to support its Member States in assessing present and future radiological threats and in planning the remediation of these sites. The IAEA has thus been working worldwide to assist Member States with their efforts to come to grips with the important task of remediating radioactively contaminated sites. Numerous activities are ongoing, primarily national and regional Technical Cooperation projects. However, the IAEA is not alone in working to alleviate this situation. Other agencies and organizations have also been working on these same issues. In recent times, there has been a major effort directed at Central Asia to bring all the players together to work with the affected nations to better coordinate and complement the many aspects of the existing programmes. This will culminate in a series of meetings later this year with the objective of producing a Framework Document that will bring all the issues together in one place so that a 8 FORSSTROEM common approach can be taken to obtain the necessary funding for the remediation of these sites. Let us remember, however, that environmental remediation programmes are not only constrained by the lack of financial resources. Technical and non-technical factors including appropriate programme management, socio-economic issues and changing regulatory regimes have also contributed to the slow pace at which cleanup projects are being implemented. A lesson which has been learned is that strong involvement at government level is essential. From the regulatory perspective, legal instruments applicable to cleanup requirements for groundwater and soil are evolving. It is necessary to keep track of these changes as new regulations or improved international standards may affect the selection of cleanup strategies and techniques. Legal requirements will determine the standards and levels of compliance to be achieved. Such standards need to take into account updated scientific evidence. The policies and regulatory frameworks are essential to provide assurance to members of the public that they are being adequately protected. This will be discussed in Session 3 of the conference. Technologies must continuously evolve to bring solutions to existing problems in a cost-effective way and to achieve compliance with regulatory standards. Some of the most well established technologies can be ineffective in meeting modern regulatory standards. A close follow-up of the performance of innovative technologies is thus essential. But it should also be noted that remediation implementers are sometimes reluctant to promote innovative technologies on a commercial scale, partly owing to the risk that innovative technologies may fail to perform as predicted. Session 4 will provide some good illustrations of this. Every remediation project is composed of separate tasks which are prioritised to assist in planning and to optimise the use of resources. These tasks will vary significantly in size and scope. It may be, from time to time, efficient to catch the less costly ‘low hanging fruits‘ first in order to bring immediate relief to the most important problems, without affecting the long term objectives. It is important to ensure in the planning that ‘the best will not become the enemy of the good’. For these and other reasons, the involvement of different stakeholders in the decision making process has become more and more relevant. Stakeholders may include local communities, non-governmental organizations with national, regional or international outreach, regulatory authorities and other relevant authorities. Failing to obtain complete stakeholder involvement in environmental remediation programmes will usually result in unnecessary delays and higher costs in project implementation. Session 5 will touch upon these aspects. The scope of environmental remediation has increased dramatically lately. A series of study cases will be presented during Sessions 6 and 7 and in the Poster Session to give you an overview of various environmental remediation programmes in different countries, representing different regions of the world. It is not only uranium mining, weapons testing and nuclear scientific applications that have given us contaminated sites. Some radiological problems may have arisen as a consequence of non-nuclear activities, for example, as a result of the so called NORM industries. What is the role of the IAEA in all this? The key role of the IAEA is to assist Member States with the planning, development, implementation, maintenance and continuous improvement of programmes and activities. The IAEA provides support in the form of guidance documentation, technical advice and training. The guidance may be found in the IAEA documents including Safety Standards and Safety Reports, Technical Reports and Technical Documents. The technical advice and training is mainly provided through Technical Cooperation Programmes or bi-lateral assistance agreements. By taking full advantage of these opportunities, a Member State should be able to avoid creating new legacy 9 OPENING ADDRESS sites as well as achieving a significant decrease in the costs associated with extensive and long lasting environmental remediation programmes. The IAEA recognizes, however, that new mechanisms and means of experience exchange and information transfer must be put in place. For this reason the IAEA is establishing networks in different areas such as decommissioning, waste disposal and, specifically, related to the scope of this conference, environmental remediation (the ENVIRONET – will be presented during Session 8). This conference creates a good opportunity to discuss the relevant issues relating to the environmental remediation of radioactively contaminated sites. It follows on from the environmental remediation conference that took place 10 years ago in Arlington, USA and will allow you to discuss the achievements, the successes, the failures and the lessons learned, as well as the new challenges that have emerged since that time. The conference will also provide a forum for discussions on financing mechanisms and support for the international or multi-lateral organization of environmental remediation programmes; regulatory and safety issues; mature and innovative technologies; life-cycle planning and non-technical issues in environmental remediation; As a result, it is expected that the conference will encourage and assist the establishment of different partnerships; reveal synergies that can help in the full implementation of environmental remediation projects, and provide a forum for improved coordination among the international organizations that support environmental remediation programmes, especially in this region. Finally, the conference will allow the IAEA to collect ideas for its programme and for the assistance it gives to its Member States. I wish you all a fruitful and rewarding conference with good and intensive discussions both here and in the coffee breaks. 10 FROM ARLINGTON TO ASTANA – LESSONS LEARNED (TOPICAL SESSION 1) Chairperson H. FORSSTROEM IAEA SUMMARY OF THE 1999 INTERNATIONAL CONFERENCE ON THE RESTORATION OF ENVIRONMENTS WITH RADIOACTIVE RESIDUES D.W. REISENWEAVER Alion Science & Technology, Los Alamos, United States of America Abstract In November 2008, an international conference on the ‘Restoration of Environments with Radioactive Residues’ was held in Arlington, Virginia in the United States of America. This paper reviews the contents and outcomes of the Arlington conference and examines its relevance for the issues of today. 1. INTRODUCTION In November 1999, the International Atomic Energy Agency organized an international conference on the Restoration of Environments with Radioactive Residues in Arlington, Virginia in the United States of America (USA). The conference was co-sponsored by the US Department of Energy, the US Environmental Protection IAEA and the US Nuclear Regulatory Commission. This was the first IAEA conference to address the subject of environmental remediation. The format of the conference comprised five technical sessions, a panel discussion, a poster session and opening and closing sessions. Thirty-seven papers were presented orally in the technical sessions. The discussions that followed each paper together with the panel discussion were recorded and an edited version of them was included in the conference proceedings. Summaries of each of the five sessions were also included in the proceedings which were published by the IAEA [1]. In addition, over 120 contributed papers were published as a separate volume of the proceedings. 2. SESSION ONE – GLOBAL OVERVIEW The first session provided a global overview of the environments contaminated with radionuclides requiring restoration and identified the major areas where environmental contamination has occurred. Presentations addressed the radioactive residues in the USA, the Russian Federation, the European Union and China. Other presentations addressed areas contaminated with naturally occurring radioactive material, residues from accidents that have occurred in the former Soviet Union and the general approach that the IAEA was taking to establish policies on environmental restoration. The session clearly illustrated that radioactive residues exist at many sites around the world and result from events including accidents, nuclear weapons testing, decommissioning and inappropriate past practices. There are also many areas that are affected by elevated levels of naturally occurring radioactive materials. Three major issues were identified during the discussions: – The need for harmonized criteria for guiding restoration efforts; – The need for consistency in the treatment of natural versus man-made radioactive residues; – The need for good communications with the public on decisions related to restoration. 13 TOPICAL SESSION 1 SESSION TWO – RESTORATION PRINCIPLES AND CRITERIA 3. The papers in this session described current remediation approaches and cleanup criteria being used by different countries, i.e. USA, Germany, France and the Russian Federation. The three concerned governmental agencies in the USA have slightly different approaches and criteria and these were discussed. The recommendations of the International Commission on Radiological Protection (ICRP) relevant to cleanup were also presented. There was considerable discussion of the issues contained in this session. It was apparent that a unified view on the subject of radiological criteria and policies for aiding cleanup decisions did not exist. It was recognized that the concept of ‘intervention’ is generally not recognized in national regulations. Proposals were discussed on how to build a framework that can deal with the remediation of residual contamination situations associated with both man-made and naturally occurring origins. The following major conclusions were identified during the discussions: – The involvement of interested parties as part of the overall remediation process is of primary importance; – Establishing derived (and measurable) criteria is necessary for the management of contamination situations as well as the protection of the environment; – There is a serious potential for overestimating risks because of overly conservative and unrealistic modelling and this can prove to be very costly. SESSION THREE – CASE STUDIES 4. In the third session, various case studies involving remediation efforts were presented. The session was divided into five sub-sessions, each dealing with a particular type of remediation problem. Each type of problem has unique issues and requires different approaches to the remediation. The sub-sessions were concerned with: – – – – – Nuclear weapons test sites; Legacy of discharges; Legacy of accidents; Mining and milling activities; and Residues from the termination of practices. It was identified that choosing between alternative restoration options should be based on weighing the potential reduction achieved in worker and public doses against the associated cost of the strategy. Site characterization approaches must include both a historical review and a contaminant assessment. It was stressed that a good understanding of the site is important when planning the characterization activities. The importance of interested party involvement as part of the restoration activities was underlined and it was recognized that this involvement is critical for project success. Since most sites are affected by both chemical and radiological contamination, the harmonization of cleanup levels and goals for these different contaminants is an important issue. It was also recognized that consideration has to be given to the possible uses of the site and, if necessary, the maintenance of institutional controls to limit use or access. Policies in this area still needed development at the time of the conference. 14 REISENWEAVER 5. SESSION FOUR – CRITICAL ANALYSIS OF CASE STUDIES A critical review of the case studies presented during Session Three had been conducted by a small group of experts. The radiological protection approach, the criteria used for remediation, the application of various non-radiological factors and the involvement of interested parties were all considered during this analysis. It was determined that there were no uniform criteria in use for guiding restoration activities. The criteria being used ranged from 0.1 to 10 mSv/a. The cost/benefit justification for the lower levels was questionable and it was clear that the decisions on remediation were influenced by social, political and psychological factors, rather than by health or safety aspects. The importance of early planning and the involvement of interested parties in the decision making process was emphasized. The lack of public acceptance of even low levels of voluntary risk was a significant factor influencing the decision making process. It was recognized that the lack of disposal facilities for the high volumes of material that can be generated during the restoration process can be problematic. 6. SESSION FIVE – ROLE OF PUBLIC PARTICIPATION This session was concerned with public involvement during the restoration process, from the initial planning and decision making through to the final disposition of the site. This issue was discussed during the other sessions, but this session focused on two programmes that were developed to foster public participation in the process. The first was the Superfund programme in the United States and the second was the European Commission ETHROS programme involving territories that were contaminated due to the Chernobyl accident. It was determined that the public must be brought into the decision making process at an early stage to ensure the success of the project. The level of information needed will vary depending on the level of interest of the individuals, and this may range from information summaries to documentation of the detailed studies and data. It is important that involved members of the public get the feeling that their input is important. It should be recognized that individuals may have different concerns from those of the overall community and these concerns must be taken into account. 7. PANEL SESSION The panel session was designed to bring together a wide range of interested parties to discuss their concerns about the restoration process. The panelists included a radiation protection expert, an individual from the local government of an area affected by nuclear tests (the Marshall Islands), a representative from a local environmental group, a representative from a public interest group and an environmental expert. Not surprisingly, the concerns and the approach that should be taken to restore a site can vary depending on the perspective of the individual or group providing comment. The radiation protection expert thought there were three main issues concerning site restoration: standards and limits, risk limitation with respect to natural verses manmade radiation, and the role of the radiation protection community. The Marshall Island governmental representative was concerned with the people and his community; how the island would be restored, and how the people and community would be compensated. The environmental group representative was concerned with the local population being involved with the federal and local governments in a timely manner and in ensuring that all information is presented to allow an informed decision to be made. The environmental expert agreed that stakeholder involvement is important, but that it is not a substitute for governmental or official action. It was considered that for stakeholders, the process is often more important than the criteria. The 15 TOPICAL SESSION 1 public interest group representative considered that the intelligence of the general public is sometimes underestimated and that scientists sometimes tend to patronize the public. It was emphasized that respect must be shown to all interested parties. 8. SUMMARY The closing session summarized the overall conference. The basic concepts of restoration were agreed and the need for consistent criteria was identified. The problem within the United States of the divergent opinion of governmental agencies on radiological criteria was identified and a plea was made for convergence. There was also a recognition that the concept of intervention was not fully endorsed by everyone and that this issue needs to be addressed to help avoid confusion in the future. At the beginning of the conference it was thought that there was a need for education of the public but by the end of the week it was determined that this was not the problem, and that what is needed is early public involvement in the remediation planning phase. The following is a list of questions that was developed from the discussions on the major issues: – Have consistent criteria been established that provide guidelines for the remediation of contaminated sites? – Can a single criterion be applied to the remediation of all forms of contaminated site, be they nuclear test sites, areas resulting from accidents, the termination of practices, mining and milling activities or legacy discharges? – Should areas contaminated with man-made versus natural radioactive material have different criteria? – Is the public being properly involved during the decision making process? – How do we ensure that overly conservative and unrealistic modelling is not being used which could lead to the overestimation of risks? – Have we harmonized the cleanup levels and goals for sites that are contaminated with chemical and radioactive material? – How do we justify removing material from one site and moving it to another site verses stabilizing the material in place? I consider it to be appropriate to challenge this (Astana) conference to reflect on these questions and I ask “Have these questions, that were identified 10 years ago, been addressed in the intervening time?” REFERENCES [1] 16 INTERNATIONAL ATOMIC ENERGY AGENCY, Restoration of Environments with Radioactive Residues, Proceedings of an International Conference held in Arlington, USA, November 1999, IAEA, Vienna (2001). REMEDIATION OF CONTAMINATED AREAS OF KAZAKHSTAN A.M. MAGAUOV1 Ministry of Energy and Mineral Resources, Astana, Kazakhstan Abstract This paper provides a summary of the situation in Kazakhstan in relation to environmental contamination with radioactive materials. It identifies the sources of the contamination and describes the progress made towards the remediation of affected areas. 1. INTRODUCTION The main sources of radioactive contamination in Kazakhstan are: (a) (b) (c) (d) (e) Uranium mining enterprises; Mining enterprises of the non-uranium industry (rare metals, phosphoric and coal deposits); Oil fields; Former nuclear test sites; and Commercial and research reactors (BN–350 power reactor in Aktau (under decommissioning) and four research reactors). Radioactive waste management in Kazakhstan in the period 1999–2009 has been managed under both national and local budgets. The major programmes are: (1) (2) (3) Improving and maintaining uranium mining enterprises and remediating the consequences of past mining activities; Radiation safety; Scientific, technical and technological support. 2. REMEDIATION OF URANIUM MINING AND MILLING SITES From the 1950s until 1991, Kazakhstan provided 40% of the uranium production in the Soviet Union. Conventional uranium mining and milling continued until 1995/6 when it was discontinued. Numerous legacy sites were left behind in Northern, Central/South and Western Kazakhstan. After the development of a specific legislative framework for the purpose in the late 1990s, a governmental programme for the remediation of the legacy sites was started in 2001. The responsibility for remediation in Kazakhstan is with the State Enterprise ‘Uranlikvidrudnik’. By 2007 a substantial part of the most urgent remediation work had been completed. The remediation work is currently (2008–2010) being concentrated on the storage sites at Aktau (Western Kazakhstan) and Stepnogorsk (Northern Kazakhstan). The remediation 1 Presented by K. Kadyrzhanov, National Nuclear Centre, Kurchatov, Kazakhstan. 17 TOPICAL SESSION 1 activities are conducted under close radiological supervision with constant operational monitoring in order to ensure the protection of workers, the public and the environment. The programme for the maintenance of active uranium mining sites and for the remediation of the residues at the sites has been implemented in several steps: Step 1 (2001–2005) – 8 sites; Step 2 (2006–2010) – 6 sites; Step 3 is concerned with the remediation of buildings and facilities above ground and the monitoring of the ground surface in the vicinity of flooded shafts. The responsibility for uranium mining in Kazakhstan is with the National Atomic Company Kazatomprom which is also responsible for the management of the mining waste at the active mine sites. 3. BN–350 REACTOR DECOMMISSIONING When the BN–350 fast breeder reactor reached the end of its operating life in 1999, Kazakhstan assumed its international obligations related to the prevention of nuclear weapons proliferation. The Government of Kazakhstan resolved to decommission the reactor. According to the Government Resolution (Decree No.456, April 22, 1999), spent fuel must be transported to the ‘Baikal–1’ research reactor site complex of the National Nuclear Centre, located on the territory of the former Semipalatinsk Nuclear Test Site near to Kurchatov town, for long term storage. All of the spent fuel has been unloaded from the reactor and packed in sealed containers. Preparations are being made to transport the nuclear fuel but for the time being it is temporarily stored in the cooling ponds of the BN–350 reactor. Work has started on arrangements for packaging the fuel in special transport casks. It is envisaged that 60 metal concrete casks containing the spent nuclear fuel will be transported by rail and road to Baikal– 1 for long term storage. 4. RADIATION SOURCE MANAGEMENT Spent radiation sources represent a substantial proportion of the total of accumulated radioactive waste in Kazakhstan and a significant amount of work has been carried out to render these sources safe. The work follows two main directions: (a) (b) Solving the radiological problems associated with the accumulation of spent sealed sources; Developing technologies for the recycling and use of spent radiation sources in industry in Kazakhstan and the establishment of manufacturing facilities. Since 1995, the Baikal–1 complex has been used for the long term storage of all spent sealed sources in Kazakhstan and a special storage facility has been created there for that purpose. 18 MAGAUOV 5. REMEDIATION OF NUCLEAR TEST SITES All types of nuclear weapons tests were carried out on the territory of Kazakhstan in the period 1949 to 1989: they included air explosions, above ground explosions, underground explosions, high altitude explosions and tests in space. From 1996 to 2001, after the removal of the nuclear weapons infrastructure at the Semipalatinsk Test Site, 181 tunnels at the Degelen site and 13 unused boreholes and the facilities for 12 silo missile launchers at the Balapan site were destroyed. All of the operations were carried out under strict radiological supervision and with the approval of experts from the Ministry of Ecology and the Ministry of Emergency Situations. It is expected that up to 95% of the Semipalatinsk Test Site area can eventually be returned to normal economic use. 6. RADIATION SAFETY SUPPORT The radiological investigation of the territories of Kazakhstan is being carried out as part of a national programme. The basic tasks of the programme are: (a) (b) (c) (d) 7. Assessment of the radiological situation in Kazakhstan, including an assessment of the radiation doses to the population; The zoning of radioactively contaminated territories and of areas for monitoring; evaluation of the effectiveness of remediation and assessment of protection of the population from non-standard exposures, e.g. hot particles; Prevention of the dispersion of radioactive materials in the environment adjacent to the Irtysh Chemical and Metallurgical Plant; Support for the radiation and nuclear safety of the former Semipalatinsk Test Site, for example, its use for agricultural activities, the seismic condition of underground explosion locations and radioecology aspects. REGULATORY AND LEGAL FRAMEWORK The fundamental legislation governing the remediation of uranium mining and processing sites comprises the legal acts on Atomic Energy Use, Radiation Safety of the Population and Licensing. Relevant governmental decrees are: Decree on the Atomic Energy Committee of the Ministry of Energy and Mineral Resources of the Republic of Kazakhstan, Decree on the Licensing of Activities related to the Use of Atomic Energy, and Decree on the Final Disposal of Radioactive Waste in the Republic of Kazakhstan. The strategies and plans for remedial work have been established in compliance with the following regulations: Norms of Radiation Safety (NRB–99), Hygiene Standards to Ensure Radiation Protection (SP PORB–2003), Hygiene Standards for the Decommissioning, Remediation and Conversion of Production Units for the Mining and Processing of Radioactive Ores (SP LKP–98), and Hygiene Standards for the Handling of Radioactive Waste (SPORO–97). 8. INTERNATIONAL COOPERATION AND PERSPECTIVES The problem of radioactively contaminated areas is global and the Republic of Kazakhstan has experience which can help others with similar problems. International programmes can be of help in starting remediation programmes, for example, the programmes of the International Atomic Energy Agency, the North Atlantic Treaty Organization, the Institute for Scientific and Technological Cooperation, and the European Commission. In the case of Kazakhstan, the combining of national and international programmes has helped to 19 TOPICAL SESSION 1 strengthen the scientific and technical potential of the country in this field. 9. CONCLUSIONS A regulatory and legal framework exists in Kazakhstan which facilitates the control and regulation of radioactive waste management. The potential to create facilities for the long term storage and processing of radioactive waste exists at many locations in Kazakhstan. The remediation of the former uranium mining enterprises is almost complete. A monitoring system around the ground areas near to flooded mine shafts will have to be developed. In the context of supporting the non-proliferation regime, substantial work is being carried out which helps in the evaluation of the radiation situation in the territories of Kazakhstan. Countries can benefit from international cooperation in this field and this conference is a good example of such cooperation. 20 INTERNATIONAL POLICIES AND STRATEGIES FOR THE REMEDIATION OF LAND AFFECTED BY RADIOACTIVE RESIDUES A.J. GONZÁLEZ Argentine Nuclear Regulatory Authority, Buenos Aires, Argentina Abstract The paper addresses the international policies and strategies for the remediation of land affected by radioactive residues. The main aim of the paper is to describe the evolution and status of the international paradigms in this area while, at the same time, identifying some of the associated misunderstandings, mainly due to the terminology employed. The international radiation protection approaches for remediation are described. They derive from the recommendations of the International Commission on Radiological Protection. Prolonged exposure situations, which are typical in the case of contaminated land, are analyzed in some detail. Finally, the international safety standards on remediation, which are being established under the aegis of the International Atomic Energy Agency, are explored. The paper suggests that the time is ripe for a simple and clear international agreement on the levels of land contamination with radioactive material that may be considered unambiguously safe. 1. INTRODUCTION The so-termed remediation of territories experiencing ‘contamination’ with radioactive residues has been one of the more elusive issues to tackle and regulate for the radiation protection community. Radiation protection experts have generally been unable to respond to a simple and straightforward question from anxious members of general public: “Is it safe for me and my family to live here?”. Experts have tried to explain that, while the territory was in fact contaminated, remediation had to be optimized, and depending on many factors (generally incomprehensible for the common public) they might, or might not, be able to remain there. Moreover, sometimes, experts have implicitly advised members of the public that it was ultimately their decision whether to leave or to remain in contaminated land or whether it should be remediated. The meanings of the terms contamination and ‘remediation’, in the context of radioactive material on land surfaces, are sometimes not clear to nonspecialists and can create ambiguity in understanding. The paper’s main aim is to describe the evolution and status of the international paradigms and standards for the remediation of land affected by radioactive residues and also to discuss the misunderstandings caused by the terminology used. It also suggests further international actions to help countries to solve their problems in this area. The ideas in this paper are elaborated in greater depth elsewhere [1]. While many States have been challenged by the issue of remediating contaminated land, Kazakhstan has been particularly challenged because its territory suffered extensive contamination from the nuclear testing activities of the former Soviet Union. In May 1993, representatives of the Kazakhstan Government informed the International Atomic Energy Agency of their concern [2]. Subsequently, at the request of the Government of Kazakhstan, the IAEA undertook to carry out a study of the radiological situation at Semipalatinsk [3]. From 1949 to 1989, the former Soviet Union had conducted 456 nuclear explosions at the Semipalatinsk test site. Until 1963, the explosions were mainly carried out on the surface and in the atmosphere. After 1963, testing was conducted underground. The last nuclear explosion at the site was in 1989. Two Semipalatinsk areas, the so-called Ground Zero and Lake Balapan areas were found to be heavily contaminated. Since the IAEA assessment, little aid has been provided by the international community to help Kazakhstan remediate this vast area 21 TOPICAL SESSION 1 of territory. The IAEA had clearly qualified its assessment as ‘preliminary in nature’ and expressly indicated that “it does not constitute a comprehensive radiological survey of the site, which covers a very large surface area, but rather identifies the topics on which further study is needed in order to develop a full understanding of the radiological situation at the site” [3]. 2. MISUNDERSTANDINGS The term (radioactive) ‘contamination’ is widely misunderstood and its misinterpretation has had significant effects in radiation protection strategies. Surprisingly, the term derives from a historical religious background as a descriptor of impurity. Contamination originates from the Latin ‘contaminat-’, ‘contaminare’, or ‘make impure’. The obvious conclusion from this definition is that something that is ‘contaminated’ is automatically unacceptable, regardless of the quantification of such ‘contamination’. The original intention of radiation specialists was to denote the presence of radioactive materials, as expressed by the quantity (radio) ‘activity’, a denotation describing an amount or concentration of radionuclides in a given energy state at a given time. The intention was not of a connotation of impurity or dirtiness, nor even of the magnitude of the hazard involved. However, in the public mind, ‘contamination’ became a quasi-synonym of dangerously undesirable ‘radioactivity’. In sum, while the term is commonly used by experts to quantify the presence and distribution of radioactive material in a given environment, it has become widely misinterpreted as a measure of radiation-related dangerousness. Moreover, ‘contamination’ strictly refers to radioactive substances on surfaces, or within solids, liquids or gases (including those in the human body), where their presence is unintended or undesirable, or to the process giving rise to their presence in such places. Unfortunately the term is used more informally (even by experts) to refer to the amount of (radio)activity on a surface, and it is misinterpreted and misunderstood as a dangerous level of (radio)activity. The term (radioactive) ‘remediation’ became closely associated with the misinterpretations of ‘contamination’, as the former is a consequence of the latter. The term may be used in a variety of contexts and, as a result, it can be badly misunderstood. In common parlance, it means providing a remedy, namely a pharmaceutical product, cure or treatment, for a medical condition. Not surprisingly, members of the public became extremely anxious when informed that the place where they are living would be subject to remediation because of a radiation-related contamination! Environmental radiation protection specialists, however, use remediation to mean the removal or reduction of radioactive substances from environmental media such as soil, groundwater, sediment, or surface water. The ultimate purpose of ‘remediation’ is protecting human health and the environment against potential detrimental effects from radiation exposure, rather than eliminating contamination completely. The untranslatable and more informal English term ‘cleanup’ has been used as a synonym of remediation and this usage has added to the misunderstanding. The term implies making a place ‘clean’, and is taken to mean making it absolutely free from dirt or harmful substances. The confusion arises because a decision to reduce a given level of radioactive contamination may be taken simply because the radioactivity is measurable and not because it is ‘dirty’ or ‘harmful’. Moreover, the term ‘clean’ can also be tacitly equated to ‘morally pure’, which again has religious implications. This interpretation combined with the misinterpretations of the term ‘contamination’ described previously may have played an important role in the misunderstanding. Members of the public may be further confused because regulations for the remediation of contamination are not established in terms of quantities expressing radioactivity levels in the ‘contamination’ but rather in terms of radiation doses to be expected from the contamination. Increasing the confusion is the fact 22 GONZÁLEZ that these doses can be expressed as integrated doses (e.g. doses to be incurred over life-time) or as dose-rates (e.g. annual doses). It seems, therefore, that there is a strong connection between the misunderstandings of contamination and remediation and the quantities used to measure them. In simple terms, remediation should be expected if there is contamination and there will be contamination if, and only if, the levels of ‘radioactivity’ per unit area are above values considered to be unsafe. Despite the confusion described in this section of the paper, it is considered that the usage of the terms contamination and remediation etc. is so entrenched in radiation protection practice that changes at this stage into more precise language may produce more harm than good. 3. SCENARIOS Radioactive residues can originate from several causes, as follows: (a) (b) (c) (d) (e) Occasionally, they may have been generated by the accumulation of radionuclides from normal discharges of radioactive effluents into the environment from planned and properly authorized human activities (the so-called ‘practices’ in international jargon); They may also be radioactive remnants from the termination of a practice and the decommissioning of the installations used by it; Most commonly, radioactive residues are the result of unregulated human activities that have been carried out in the past, where the termination of the activity and the handling of the remaining residues would most probably not have been adequately considered when the activity was initiated; (A simple example of this is the ancient practice of mining and milling operations of ores containing natural radioactive substances.) Radioactive residues may also remain from past events that may have been unforeseeable at the time of occurrence, such as accidents releasing long-lived radioactive materials to the environment; Finally, the largest part of the radioactive residues in the human habitat is a legacy from past military operations that were both foreseeable and avoidable. It should be noted that the complexity of the situations that may arise from territorial contamination was not recognized early enough by the international community. The many assessments of the aftermath of the Chernobyl accident have shown the difficulties in dealing with this type of situation. However, it was not until the year 2002 that the IAEA issued a report in which governments and international organization documented the severity of the problem [4]. 4. THE ICRP RECOMMENDATIONS At the root of the international approach for the remediation of contaminated land is the discipline of radiation protection. Radiation protection is not a science but a paradigm, namely a model for keeping people safe from the potential detriment that radiation exposure may cause. The International Commission on Radiological Protection (ICRP) provides international recommendations on radiation protection. The ICRP recommendations that are still used in current standards appeared as Publication 60 [5] in 1990. Recently, in 2007, new recommendations were issued as ICRP Publication 103 [6]. Virtually all international standards and national regulations addressing radiological protection are based on the ICRP recommendations contained in ICRP Publication 60. The relevant international standards are the International Basic Safety Standards for Protection against Ionizing Radiation and for the 23 TOPICAL SESSION 1 Safety of Radiation Sources, or BSS [7]. Currently, a process is cleanup to revise the BSS taking into account the new recommendations contained in ICRP Publication 103. In the context of remediation, there is an important presentational difference between the ICRP Publications 60 and 103. The former is founded on a process-based approach using the concepts termed ‘practices’ and ‘interventions’ (a practice being defined as a human endeavour that can increase the overall exposure to radiation and an intervention being defined as human actions that decrease the overall exposure to radiation). Thus, remediation, in the language of ICRP Publication 60, is an archetypical intervention. Conversely, ICRP Publication 103 uses a situation-based approach to characterize the possible circumstances where radiation exposure may occur. It considers that the term ‘planned exposure situations’ better characterizes its previous intentions for defining practices and, similarly, that ‘emergency exposure situations’ and ‘existing exposure situations’ better characterize interventions. The new characterization is defined as follows: (a) (b) (c) Planned exposure situations are situations involving the deliberate introduction and operation of sources; Emergency exposure situations are situations that may occur during the operation of a planned situation, or from a malicious act, or from any other unexpected situation and require urgent action in order to avoid or reduce undesirable consequences; Existing exposure situations are exposure situations that already exist when a decision on control has to be taken, including prolonged exposure situations after emergencies. Thus, in ICRP 103 language, contaminated territories requiring remediation could be considered a case of existing exposure situations, which, however, could have originated from planned situations or from emergency situations or could be an existing situation proper. Three fundamental principles provide the basis of the ICRP paradigm. They are termed justification, optimization, and individual dose limitation, and are particularly relevant to situations of remediation and, importantly, they are based on solid ethical principles. Within the context of remediation, these fundamental principles can be formulated as justification of remediation, optimization of remedial actions and restriction of residual individual doses: Justification of remediation: Any remediation should be justified, namely: the alteration that remediation generates in the radiation exposure situation of the contaminated territory should do more good than harm. This means that by reducing the existing exposure through remediation, the individual or societal benefit must offset the detriment that the remediation may cause. Optimization of remedial actions: Remediation measures in a contaminated territory should be optimized, namely: the level of protection to be achieved by the remediation should be the best under the prevailing circumstances, maximizing the margin of benefit over harm. Optimization should result in that the likelihood of incurring exposures, the number of people exposed, and the magnitude of their individual doses, are all kept as low as reasonably achievable, taking into account economic and societal factors. Individual dose restrictions: In order to avoid severely inequitable outcomes of the optimization procedure, there should be restrictions on the doses or risks to individuals remaining in the contaminated territory. Restrictions are applied to the doses to a nominal individual (or reference person). Protection options resulting in doses greater in magnitude than such restrictions should be rejected at the planning stage. Importantly, these restrictions on doses are applied prospectively, as with optimization as a whole. If, following the implementation of an optimized protection strategy, it is subsequently shown that the value of the constraint or reference level is exceeded, the reasons should be investigated, but this fact alone should not necessarily prompt regulatory action. The ICRP has traditionally recommended an individual-related annual dose limit of 1mSv for planned exposures from 24 GONZÁLEZ regulated practices and has further recommended the use of source-related dose constraints and reference levels, which, in the context of remediation, can be described as follows: (i) a dose constraint is a prospective and source-related restriction on the individual dose from a specific contamination source, which provides a basic level of protection for the most highly exposed individuals from such a source, and serves as an upper bound on the dose in optimization of protection for that source; (ii) in contrast, if protection cannot be planned in advance for a situation, reference levels should be used in deciding on intervention with protective measures. Reference levels should represent the level of dose or risk above which it is judged to be inappropriate to plan to allow exposures to occur and below which optimization of protection should be implemented. The chosen value for a reference level will depend upon the prevailing circumstances of the exposure under consideration. The ICRP now recommends that reference levels, set in terms of individual dose, should be used in conjunction with the implementation of the optimization process for exposures in existing exposure situations. The objective is to implement optimized protection strategies, or a progressive range of such strategies, which will reduce individual doses to below the reference level. However, exposures below the reference level should not be ignored; these exposure circumstances should also be assessed to ascertain whether protection is optimized, or whether further protective measures are needed. An endpoint for the optimization process must not be fixed in advance and the optimized level of protection will depend on the situation. It is the responsibility of regulatory authorities to decide on the legal status of the reference level, which is implemented to control a given situation. Retrospectively, when protective actions have been implemented, reference levels may also be used as benchmarks for assessing the effectiveness of the protection strategies. The use of reference levels in existing situation is illustrated by Fig. 1, which shows the evolution of the distribution of individual doses with time as a result of the optimization process. FIG. 1. The use of a reference levels in existing exposure situations and the evolution of the distribution of individual doses with time as a result of the optimization process. 25 TOPICAL SESSION 1 According to the new ICRP recommendations, reference levels for existing exposure situations such as those candidates for remediation should be set typically in the 1 to 20 mSv band of projected dose. The individuals concerned should receive general information on the exposure situation and the means to reduce their doses. In situations where individual lifestyles are key drivers of the exposures, individual monitoring or assessment as well as education and training may be important requirements. Living in contaminated areas after a nuclear accident or a radiological event is a typical situation of that sort. The current recommended values for protection criteria are compared in the following table with those provided by the previous recommendations in ICRP Publication 60 [5] and the derivative ICRP Publication 82 [7]. The comparison shows that the current recommendations are essentially the same as the previous recommendations encompassing the previous values but are wider in their scope of application. Intervention Previous reference levels [7] Unlikely to be justifiable <≈10mSv/year May be justifiable >≈10mSv/year Almost always justifiable Towards 100 mSv/year Current reference level [6] Between 1 and 20 mSv/year according to the situation Remediation usually includes considerations of environmental protection. The traditional position of the ICRP on environmental protection has evolved over time. Usually, the traditional environmental concern of radiation protection has been limited to the transfer of radionuclides through the human habitat primarily in relation to planned exposure situations (because this transference directly affects the protection of human beings). In ICRP Publication 60, the ICRP considered that the standards of environmental control needed to protect the general public would ensure that other species are not put at risk. Under this approach, if remediation is not needed for humans it should not be needed for other species. While the ICRP continues to believe that this is likely to be the case, it also recognizes that interest in the protection of the environment has greatly increased in recent years in relation to all aspects of human activity. This has been accompanied by the development and application of various means of assessing and managing the many forms of human impact upon the environment. The growing need for advice and guidance on such matters in relation to radiological protection have, however, not arisen from any new or specific concerns about the effects of radiation on the environment. There seemed to be a lack of consistency at international level with respect to addressing such issues in relation to radioactivity. ICRP is also aware of the needs of some national authorities to demonstrate, directly and explicitly, that not only humans but the overall environment is being protected and, therefore, it decided to develop a clearer framework to assess the relationships between exposure and dose, and between dose and effect, and the consequences of such effects, for non-human species, on a common scientific basis. This issue was first discussed in ICRP Publication 91 [8], and it was concluded that it was necessary to draw upon the lessons learned from the development of the systematic framework for the protection of human beings. Another issue affecting international remediation policies is the necessary global agreement on situations that do not justify being remediated. The ICRP has long recognized that there may be exposure situations for which it will be obvious that remediation to reduce exposures is either not feasible or not warranted [9]. While many exposures from contaminated territories are controllable, a number of situations can be either uncontrollable or essentially unamenable to control (for example exposure undisturbed levels of natural radioactivity). Exposure situations that are uncontrollable or unamenable to control are generally subject to ‘exclusion’ from the scope of radiological protection measures. Other 26 GONZÁLEZ situations may be controllable but considered trivial by the authorities and not requiring control. Exposure situations for which control is not needed are subject to ‘exemption’. According to ICRP, the decision as to what components of existing exposure are either not amenable to control or do not need to be controlled, requires a judgment by the regulatory authority that will depend on the controllability of the source or exposure and also on the prevailing economic, societal and cultural circumstances. Moreover, it should be emphasised that non-technical factors have an enormous influence on remediation policies. For this reason, the ICRP has always cautioned that its recommendations are based on objective assessments of the health risks associated with exposure levels and on radiological protection attributes of various exposure situations. However, members of the public (and sometimes their political representatives) may have personal and distinct views on radiation risks, for instance between those attributable to artificial sources of exposure in relation to those due to natural sources. Social and political attributes, generally unrelated to radiological protection, usually influence the final decision on remediation. Therefore, while the ICRP reports should be seen as a provider of decisionaiding recommendations, mainly based on scientific considerations on radiological protection, the outcome of the ICRP advice is expected to serve just as an input to a final (usually wider) decision-making process, which may include other societal concerns and considerations and the participation of relevant stakeholders rather than of radiological protection specialists alone. The ICRP is issuing new recommendations on the application of the ICRP’s recommendations to the protection of individuals living in long term contaminated territories after a nuclear accident or a radiation emergency. The new recommendations recognize that nuclear accidents and radiation emergencies are managed according guidance covering short, medium and long term actions. The most recent guidance related to the management of the short and medium actions is provided by recently approved ICRP recommendations on the Application of the Commission’s Recommendations for the Protection of People in Emergency Exposure Situations. The post-accident rehabilitation situation covered by these recommendations corresponds to the long term actions that may be necessary to be implemented in the case of a nuclear accident or radiological event resulting in long lasting contamination of large inhabited territories. The transition from an emergency exposure situation to an existing exposure is characterised by a change in management, from strategies mainly driven by urgency, with potentially high levels of exposures and predominantly central decisions, to more decentralised strategies aimed at improving living conditions and reducing exposures to as low as reasonably achievable given the circumstances. These strategies must take into account the long term dimension of the situation with the direct involvement of the exposed individuals in their own protection. The ICRP recommends in its new report that this transition should be undertaken in a co-ordinated and fully transparent manner and agreed and understood by all the affected parties. The decision to allow people to live in contaminated territories marks the transition between emergency and the existing exposure situations and will be taken by the authorities. This will be the beginning of the post-accident rehabilitation phase and is where the new recommendations have their focus. 5. INTERNATIONAL STANDARDS The International Basic Safety Standards (BSS) [10] of 1996 are standards that govern general international requirements on radiation protection. The BSS, however, are basically mute about remediation of contaminated territories. They only include generic requirements for intervention in what, at the time, was termed ‘chronic’ exposure situations. The BSS presumed that States should determine the allocation of responsibilities among regulatory authorities, national and local intervening organizations and even registrants or licensees, for 27 TOPICAL SESSION 1 the management of interventions in chronic exposure situations. Under this proviso, the BSS require that generic or site specific remedial action plans for chronic exposure situations shall be prepared by intervening organizations, as appropriate. The plans shall specify remedial actions and action levels that are justified and optimized, taking into account: (a) the individual and collective radiation exposures; (b) the radiological and non-radiological risks; and (c) the financial and social costs, the benefits and the financial liability for the remedial actions. They also require that action levels for intervention through remedial action shall be specified in terms of appropriate quantities, such as the annual average ambient dose equivalent rate or a suitable average activity concentration of radionuclides that exist at the time remedial action is being considered. However the BSS failed to prescribe numerical action levels for remediation. The many assessments of the Chernobyl accident [11–17] clearly demonstrated that the BSS had to be complemented with specific guidance. In the year 2000, the IAEA issued guidance on the restoration of environments affected by residues from radiological accidents, with approaches to decision making [18]. Areas needing remediation from technologically enhanced natural radiation were also discussed in various fora (see, e.g. [19–22]. After the accident in Goiănia, Brazil, the IAEA started to publish a review of major radiological abnormal situations around the world, many of them requiring remediation [e.g. 3, 23,]. Last but not least, the IAEA started to tackle the controversial issue of decommissioning of nuclear installations and the remediation of sites [24, 25]. However, it was not until November 2003 [26] that the IAEA finally established safety requirements for the remediation of areas contaminated by past activities and accidents. The new requirements did not introduce any fundamental change in the remediation philosophy. The objectives of remediation were now formulated as: (i) to reduce the doses to individuals or groups of individuals being exposed; (ii) to avert doses to individuals or groups of individuals that are likely to arise in the future; and, (iii) to prevent or reduce environmental impacts from the radionuclides present in the contaminated area. Reductions in the doses to individuals and environmental impacts were to be achieved by means of interventions aimed at: (i) removing the existing sources of contamination; (ii) modifying the pathways of exposure; and/or, (iii) reducing the numbers of individuals or other receptors exposed to radiation from the source. In some cases the restricted use of human habitats may be the outcome of the optimization process for remediation [27]. The requirements established a generic reference level for aiding decisions on remediation as an existing annual effective dose of 10 mSv from all environmental sources, including the natural background radiation. The IAEA also analyzed the non-technical factors influencing decision making processes in environmental remediation [28]. It concluded that a range of non-technical factors will influence the choice of technologies to be employed in remediation and the strategy for their implementation, including: economy, employment and infrastructure; costs, funding, and financing; regulatory and institutional aspects; stakeholder perception and participation; project implementation related risks; co-contamination issues; future land use; and, stewardship issues. 6. OUTLOOK It is clear that substantive international recommendations, policies, strategies and, ultimately, standards are available for the remediation of land affected by radioactive residues. What is missing, however, is a simple, clear, unambiguous and unmistakable international agreement on what is safe and what is unsafe in relation to land contamination with radioactive materials. Fundamentally, an international safety regime is also missing – one that governs the standardization of protection in the remediation of contaminated territories and also the appraisal of compliance. Conveniently, an agreement on remediation 28 GONZÁLEZ could be expressed in terms of a derived practical quantity rather than in terms of the fundamental dosimetric radiation protection quantities. For instance, it could be expressed as activity per unit area rather than as a dose. Expediently, the agreement could ignore distinctions among radionuclides, even if it became over-conservative for some of them, and just include three basic numbers, for alpha-, beta- and gamma-emitters, with some caveats for hot particles. The time is ripe for such an agreement. People dwelling in the so-called ‘contaminated’ lands continue to ask an elementary question: “Is it safe for me and my family to live on this land?” And we, the radiation protection community ought to provide a clear and unambiguous answer. REFERENCES [1] [2] [3] [4] [5] [6] [7] [8] [9] [10] [11] [12] [13] [14] GONZALEZ, A.J., International Approaches to Remediation of Territorial Radioactive Contamination, Radioactivity in the Environment 14 (2009) 1-40. Strengthening Radiation and Nuclear Safety Infrastructures in Countries of the Former USSR, Proceedings of a Forum (IAEA/UNDP), IAEA Proceedings Series, Vienna (1993). INTERNATIONAL ATOMIC ENERGY AGENCY, Radiological Conditions at the Semipalatinsk Test Site, Kazakhstan: Preliminary Assessment and Recommendations for Further Study, Radiological Assessment Report Series, IAEA, Vienna (1999). http://wwwpub.iaea.org/MTCD/publications/PDF/Pub1063_web.pdf INTERNATIONAL ATOMIC ENERGY AGENCY, Radiation Legacy of the 20th Century: Environmental Restoration, IAEA–TECDOC–1280, IAEA, Vienna (2002). INTERNATIONAL COMMISSION ON RADIOLOGICAL PROTECTION, 1990 Recommendations of the International Commission on Radiological Protection, Publication 60, Annals ICRP 21 1–3, Elsevier, Amsterdam (1991). INTERNATIONAL COMMISSION ON RADIOLOGICAL PROTECTION, The 2007 Recommendations of the International Commission on Radiological Protection, Publication 103, Annals ICRP 37 2–4, Elsevier, Amsterdam (2007). INTERNATIONAL COMMISSION ON RADIOLOGICAL PROTECTION, Protection of the public in situations of prolonged radiation exposure, Publication 82, Annals ICRP 29 1/2, Elsevier, Amsterdam (1999). INTERNATIONAL COMMISSION ON RADIOLOGICAL PROTECTION, A framework for assessing the impact of ionising radiation on non-human species, Publication 91, Annals ICRP 33 3, Elsevier, Amsterdam (2003). INTERNATIONAL COMMISSION ON RADIOLOGICAL PROTECTION, Scope of Radiological Protection Control Measures, ICRP Publication 104, Annals ICRP 37 5, Elsevier, Amsterdam (2008). INTERNATIONAL ATOMIC ENERGY AGENCY, International Basic Safety Standards for Protection Against Ionizing Radiation and for the Safety of Radiation Sources, Safety Series No. 115, IAEA, Vienna (1996). INTERNATIONAL ATOMIC ENERGY AGENCY IAEA, Proceedings of the All-Union Conference on the Medical Aspects of the Chernobyl Accident, IAEA–TECDOC–516, IAEA, Vienna (1988). INTERNATIONAL ATOMIC ENERGY AGENCY, The International Chernobyl Project: Assessment of Radiological Consequences and Evaluation of Protective Measures, IAEA, Vienna (1991). INTERNATIONAL ATOMIC ENERGY AGENCY, Declaration of Participants of the First International Conference of the European Commission, Belarus, Russian Federation and Ukraine on the Radiological Consequences of the Chernobyl Accident, INFCIRC/511, IAEA, Vienna (1996). http://www.iaea.org/Publications/Documents/Infcircs/1996/inf511.shtml One Decade after Chernobyl: Summing up the Consequences of the Accident. Proceedings of an International Conference in Vienna, Austria, 8-12 April 1996; IAEA Proceedings Series, Vienna (1996). 29 TOPICAL SESSION 1 [15] INTERNATIONAL ATOMIC ENERGY AGENCY, Dosimetric and biomedical studies conducted in Cuba of children from areas of the former USSR affected by the radiological consequences of the Chernobyl Accident, IAEA–TECDOC–958, IAEA, Vienna (1997). [16] INTERNATIONAL ATOMIC ENERGY AGENCY, International Conference Chernobyl: Looking Back to Go Forward, Vienna, 6–7 September 2005, Organized by IAEA on behalf of the Chernobyl Forum (2006). http://www.iaea.org/NewsCenter/ Focus/Chernobyl/pdfs/05–28601_Chernobyl.pdf [17] INTERNATIONAL ATOMIC ENERGY AGENCY, Environmental Consequences of the Chernobyl Accident and their Remediation: Twenty Years of Experience, Report of the UN Chernobyl Forum Expert Group ‘Environment’, Radiological Assessment Series Reports, IAEA, Vienna (2006). [18] INTERNATIONAL ATOMIC ENERGY AGENCY, Restoration of Environments Affected by Residues from Radiological Accidents: Approaches to Decision Making, IAEA–TECDOC–1131, IAEA, Vienna (2000). [19] INTERNATIONAL ATOMIC ENERGY AGENCY, Technologically Enhanced Natural Radiation (TENR II), Proceedings of an International Symposium held in Rio de Janeiro, Brazil, 12–17 September 1999, IAEA–TECDOC–1271, IAEA, Vienna (2002). [20] INTERNATIONAL ATOMIC ENERGY AGENCY, Testing of Environmental Transfer Models Using Data from the Remediation of a Radium Extraction Site, (IAEA BIOMASS–7), IAEA, Vienna (2004). [21] INTERNATIONAL ATOMIC ENERGY AGENCY, The Long Term Stabilization of Uranium Mill Tailings, IAEA–TECDOC–1403, IAEA, Vienna (2004). [22] Environmental Contamination from Uranium Production Facilities and their Remediation, Proceedings of an International Workshop, Lisbon, February 2004, IAEA Proceedings Series, IAEA, Vienna (2005). [23] INTERNATIONAL ATOMIC ENERGY AGENCY, Dosimetric and medical aspects of the radiological accident in Goiania in 1987, IAEA-TECDOC-1009, IAEA, Vienna (1998). [24] Safe Decommissioning for Nuclear Activities, Proceedings of an International Conference in Berlin, Germany, 14–18 October 2002, IAEA Proceedings Series, IAEA, Vienna (2003). [25] INTERNATIONAL ATOMIC ENERGY AGENCY, Planning, Managing and Organizing the Decommissioning of Nuclear Facilities: Lessons Learned, IAEA–TECDOC–1394, IAEA, Vienna (2004). [26] INTERNATIONAL ATOMIC ENERGY AGENCY, Remediation of Areas Contaminated by Past Activities and Accidents Safety Requirements, Safety Standards Series No. WS–R–3, IAEA, Vienna (2003). [27] INTERNATIONAL ATOMIC ENERGY AGENCY, Remediation Process for Areas Affected by Past Activities and Accidents, Safety Standards Series No. WS–G-3.1, IAEA, Vienna (2007). [28] INTERNATIONAL ATOMIC ENERGY AGENCY, Non-Technical Factors Impacting on the Decision Making Processes in Environmental Remediation, IAEA–TECDOC–1279, IAEA, Vienna (2002). 30 ASSISTING THE RETURN TO NORMAL LIFE IN CHERNOBYL–AFFECTED REGIONS: THE INTERNATIONAL CHERNOBYL RESEARCH AND INFORMATION NETWORK (ICRIN) O. LESHCHENKO*, L. VINTON*, Z. CARR**, D.H. CHRISTIE**, V. BERKOVSKYY***, E. SHERSTYUK****, A. KARANKEVICH****, E. STANISLAVOV**** * United Nations Development Programme (UNDP) ** World Health Organization (WHO) *** International Atomic Energy Agency **** United Nations Children’s Fund (UNICEF) Abstract This article describes the International Chernobyl Research and Information Network (ICRIN) project, a programme designed to meet the priority information needs of communities in areas of Belarus, the Russian Federation and Ukraine which were affected by the 1986 nuclear accident. Its aim is to empower Chernobylaffected communities through targeted delivery of the most recent scientific information on the accident’s impacts, translated into practical advice, including recommendations on healthy lifestyles. Supported by a United Nations (UN) General Assembly resolution, the project is part of a broader effort by all UN agencies to help local communities return to normal life, under the UN Action Plan on Chernobyl to 2016. 1. INTRODUCTION On 26 April 1986 and over the following days, one of the Chernobyl reactors released around 14×1018 Bq of radioactivity into the environment, mainly in the form of iodine (131I), caesium (137Cs) and strontium (90Sr). Around 340 000 people were evacuated and millions have lived since then in territories classified as ‘contaminated’. Although in 1986 more than 200 000 km2 of Europe was contaminated with radionuclides (at a level greater than 37 kBq/ m2 of 137Cs), nowadays the radiation exposure has been reduced by a factor of several hundred through natural processes and countermeasures. Now, most of the contaminated land is safe for life and economic activities, but around 5 million people in Belarus, Russia and Ukraine still live in Chernobyl-affected areas. Although in most places the Chernobyl exposure is comparable with the exposure due to natural radiation, in about 700 settlements annual individual doses exceed the value of 1 mSv (in addition to the dose due to natural background radiation) and protective measures could be required. In recent years, a consensus has emerged among governments and United Nations (UN) agencies that a sustainable development approach is the way forward for the Chernobyl area. Local communities have not fully recovered from the enormous socio-economic impact of the accident, produced by population resettlement, psychological trauma, unemployment, broken social ties, anxiety and fear. Investment remains scarce, infrastructure is often lacking or neglected, and young people tend to leave the region to seek opportunities elsewhere. All these factors have been exacerbated by the upheaval that followed the break-up of the Soviet Union. 31 TOPICAL SESSION 1 2. UN CHERNOBYL FORUM Between 2003 and 2006, the UN Chernobyl Forum brought together the governments of Belarus, Russia and Ukraine, eight UN agencies and the World Bank, with the objective of conducting a rigorous scientific investigation into the long term health, environmental and socio-economic consequences of the accident. In a resolution A/RES/60/14 the UN General Assembly “notes with satisfaction assistance rendered by the International Atomic Energy Agency to Belarus, the Russian Federation and Ukraine on remediation of agricultural and urban environments, cost-effective agricultural countermeasures and the monitoring of human exposure in areas affected by the Chernobyl disaster” and “Notes the necessity of further measures to ensure the integration of the assessment by the Chernobyl Forum of the environmental, health and socioeconomic consequences of the Chernobyl nuclear accident into the International Chernobyl Research and Information Network process through dissemination of the findings of the Forum, including in the form of practical messages on healthy and productive lifestyles, to the populations affected by the accident in order to empower them to maximize social and economic recovery and sustainable development in all its aspects”. According to the findings and recommendations of the UN Chernobyl Forum [1, 2], lack of information is one of the biggest challenges for those residing on the Chernobylaffected territories. The solution to this situation is seen in improved information provision that will help dispel the misconceptions surrounding Chernobyl, promote healthy lifestyles and encourage the restoration of community self-reliance by showing local residents that they themselves hold the key to their own recovery, whether in health, environment, or employment creation. The Forum pinpointed the fact that many local people were traumatized not only by the accident but also by their rapid relocation. They remained anxious about their health, perceiving themselves as ‘victims’ rather than ‘survivors’. Fear and uncertainty about the long term effects of radiation were having a detrimental effect on the health of many citizens, translating into elevated anxiety levels, chronic stress, unexplained physical symptoms and subjective poor health. The Chernobyl Forum came to the conclusion that the lack of information about the long term effects of the accident was a major problem, and that knowledge and information were necessary in order to reassure the populations and to address psychological impacts and mental well-being. Other public health problems such as unhealthy lifestyles and socioeconomic deprivation also needed to be addressed. A concerted cross-sectoral approach was deemed to be necessary, in order to assist the inhabitants to live a normal life and to overcome the dominating stigma of the Chernobyl accident. 3. UN ACTION PLAN ON CHERNOBYL TO 2016 On 20 November 2007, the UN General Assembly voted a resolution demanding a new action plan for the third decade after the Chernobyl accident. The aim of this ‘Decade of Recovery and Sustainable Development’ is to ensure that, by 2016, the stigma in the area will be overcome and a full return to normal life will be achieved. The resolution underlines the need to disseminate the findings of the Chernobyl Forum, by providing accurate information on the impact of radiation in accessible language. The provision of information to affected populations should include the promotion of healthy lifestyles and support for community-based social and economic development, as well as the provision of evidence-based policy advice to national authorities. The UN Action Plan on Chernobyl to 2016 is a practical framework [3] that builds on recognized IAEA mandates and competencies. It seeks to maximize the effects of limited resources, while avoiding the 32 LESCHENKO ET AL. duplication of efforts. ICRIN is one of the major joint UN activities foreseen under the UN Action Plan on Chernobyl to 2016. 4. ICRIN: A FOUR–IAEA PROJECT BY UNDP, WHO, IAEA and UNICEF The International Chernobyl Research and Information Network (ICRIN) is a 2.5 million USD programme designed to meet the priority information needs of communities in Belarus, the Russian Federation and Ukraine. Funded by the UN Human Security Trust Fund, the project is operated by the United Nations Development Programme (UNDP), the World Health Organization (WHO), the United Nations Children’s Fund (UNICEF) and IAEA. This three-year programme, which began in 2009, aims to translate scientific information on the consequences of the accident into sound practical advice for residents of the affected territories. Activities planned under ICRIN include education and training for teachers, medical professionals, community leaders and the media; providing local residents with practical advice on health risks and healthy lifestyles; the creation of Internet-equipped information centres in rural areas; and small-scale community infrastructure projects aimed at improving living conditions and promoting self-reliance. ICRIN objectives – – – – Deliver information in non-technical language and linked to day-to-day life; Adapt scientific knowledge to public needs; Build the capacity of local stakeholders; Invest in information technologies at the local level. ICRIN main activities – Match current scientific knowledge to local information needs and introduce efficient methods of dissemination; – Set up a monitoring system with a focus on changes in human security levels, behavioural patterns and perceptions of the affected population; – Develop practical information materials and ‘user-friendly’ recommendations for residents of contaminated areas. ICRIN expected outcomes – Credible communication and communicators will help residents regain confidence and self-reliance; – Local stakeholders and general public will gain access to and become able to rely on up-to-date and scientifically accurate information; – The stigma still associated with the affected territory will be overcome; – Poverty reduction will be achieved; – Support will be available for innovative solutions accepted or proposed by the communities; – Healthy lifestyles will be promoted among all age groups; – Success will be achieved in turning a generation of victims into a generation of proud survivors. UNDP The UNDP approach is based on the recommendations of the 2002 United Nations report [4], which outlines the shift from humanitarian to development assistance. In line with 33 TOPICAL SESSION 1 this change in strategy and at the request of the UN Secretary-General, UNDP has assumed responsibility for the UN-wide coordination of Chernobyl issues since 2004. UNDP is also responsible for coordinating the UCRIN project. Before ICRIN began, UNDP conducted surveys in Belarus, Russia and Ukraine, aimed at identifying specific information needs and at assessing public perception of the issue of radioactive contamination. Information needs in the three countries turned out to be very consistent. The top three answers to the question "What worries you the most?" were the health effects of radioactivity and low standards of living/poverty, followed by radioactivity in the environment. Under the UN Action Plan, UNDP places particular emphasis on community development efforts. These include: – – – – Expanding community-development efforts in Belarus through integrated projects that include improving the income of small private farmers by helping them develop products that meet health and safety standards; supporting community decision-making; advocating healthy lifestyles; improving access to primary health-care services; and establishing school centres for radiological advice and training; Promoting the replication of the Bryansk local economic development centre in other Chernobyl-affected oblasts of the Russian Federation; Expanding the Chernobyl Recovery and Development Programme (CRDP) in Ukraine, to bring practical infrastructure improvements, job creation, and a message of self-reliance to affected communities; Supporting the creation of local economic development agencies in affected areas of Ukraine to stimulate small and medium-sized businesses and improving the business and investment climate in the region. UNDP’s presence in local communities will help ensure that the message of reassurance that emerged from the UN Chernobyl Forum will reach local residents. WHO According to the WHO report on the health consequences of the Chernobyl accident [5], an important aspect of the ICRIN project is the mitigation of one of the largest consequences of the Chernobyl accident – psychological impact – by shifting the stigma away from the inhabitants of the Chernobyl area. It is also vital to address the fears about radiation, which are mostly caused by information gaps, and the development issues, as well as the other public health problems which are not specific to the Chernobyl area but that remain common throughout many former Soviet Union states. In these States, the top five causes of death are, according to the WHO Global Health Risks report: high blood pressure, tobacco use, high blood glucose, physical inactivity, overweight and high cholesterol levels [6]. The situation is further aggravated by the lack of adequate resources in rural health care settings, which resulted from economic changes following the break-up of Soviet Union. In view of these facts, the WHO contribution to ICRIN is focused on the following areas: – 34 Assisting the national authorities of technical guidance, consultation and medical monitoring, particularly of educational and information activities, programmes; the three most affected countries with advice on health-care programmes and high-risk groups, through a series of such as workshops, seminars and training LESCHENKO ET AL. – – – Translating the health findings of the Chernobyl Forum into easy-to-understand messages and producing targeted education packages tailored for health workers, teachers and local decision-makers; Achieving a broad dissemination of these messages, in a format accessible to local residents; Shaping the Chernobyl research agenda and promoting priority research in the area of the health consequences of the Chernobyl accident – drawing on the recommendations of the Chernobyl Forum. IAEA The IAEA was the driving force behind the UN Chernobyl Forum. The International Chernobyl Research and Information Network (ICRIN) project is a part of the IAEA contribution to the UN Action Plan on Chernobyl to 2016. Within the framework of ICRIN project the IAEA and will continue efforts in: (a) (b) (c) Adaptation of the scientific information about environmental and radiological consequences of Chernobyl accident to meet public needs; Promotion of a safety culture and the delivery of information in non-technical language, linked to daily life; Development of public information materials and resources about Chernobylrelated issues. In addition to its role in the ICRIN project, under the UN Action Plan the IAEA will focus on: – – – – – Radiological support for the rehabilitation of areas affected by the Chernobyl accident and upgrading of national capabilities to control public exposure; Assistance in the remediation of affected areas using environmentally sound technologies; Assistance in improving safety at the Chernobyl nuclear plant, in the decommissioning of Units 1, 2, and 3, and in radioactive waste management; Support to Ukraine in fulfilling its Nuclear Safeguards Agreement obligations to report relevant nuclear material related to decommissioning and excavation at the Chernobyl site; Cooperation within the scope of the IAEA mandate with other organizations in the planning, design, and implementation of projects and activities related to the broader issue of mitigating the health, environmental, and socio-economic consequences of the accident. UNICEF UNICEF has been actively participating in ICRIN development and design from the beginning. The ICRIN Scientific Board is a welcome arena in which UNICEF is glad to provide child-related contributions, expertise in the area of psycho-social well-being, as well as ideas about support to vulnerable families and micro-nutrient supplementation. UNICEF’s main contribution to ICRIN is ‘Facts for Life Chernobyl’ [7], an empowerment tool that helps people, in particular children, young people and women, to enjoy healthy and productive lives. This publication provides people living in affected areas with practical information on how to cope with the environmental, social and health problems that they face. Using 16 key messages, it provides facts on proper nutrition, young child 35 TOPICAL SESSION 1 development and iodized salt consumption for the prevention of iodine deficiency disorders. The publication also addresses cancer prevention and provides information on health-care services. ‘Facts for Life Chernobyl’ was first launched in March 2008 in three languages in Ukraine, Russia and Belarus, using UNICEF regular resources. The ICRIN project will give a decisive boost to its dissemination, enabling media advocacy and training for health workers and teachers, in coordination with the other UN agencies. Outside the ICRIN project, UNICEF will also invest in the promotion of universal salt iodization. This includes enhancing national capacities for monitoring iodized salt quality, establishing an efficient system for the prevention of iodine deficiency diseases, and helping to investigate and disseminate information on iodine nutrition and the iodine deficiency status of children and women. 5. CONCLUSION: A SINGLE VOICE ON CHERNOBYL This article has shown that several UN agencies are active in Chernobyl recovery efforts. They are united under the principles of the UN Action Plan Chernobyl to 2016 and share the same resolve to support the territories affected by the accident in achieving a full return to normal life. The ICRIN project, with its emphasis on providing affected communities with the information they need to live normal, healthy lives, offers the four UN agencies involved an opportunity to demonstrate the benefits of joint UN action on a common theme. A first indication of how well this effort is succeeding will be found in the SecretaryGeneral’s report on Chernobyl to the UN General Assembly, due in the course of 2010. REFERENCES [1] [2] [3] [4] [5] [6] [7] 36 INTERNATIONAL ATOMIC ENERGY AGENCY, Environmental Consequences of the Chernobyl Accident and their Remediation: Twenty Years of Experience, Report of the Chernobyl Forum Expert Group “Environment”, Radiological Assessment Reports Series 8, IAEA, Vienna (2006). http://www-pub.iaea.org/MTCD/publications/PDF/Pub1239_web.pdf INTERNATIONAL ATOMIC ENERGY AGENCY, Chernobyl’s Legacy: Health, Environmental and Socio-Economic Impacts and Recommendations to the Governments of Belarus, the Russian Federation and Ukraine, IAEA, Vienna (2006). http://www.iaea.org/Publications/Booklets/Chernobyl/chernobyl.pdf UNITED NATIONS (UN), Action plan on Chernobyl to 2016, UNDP (2008). http://chernobyl.undp.org/english/docs/action_plan_final_nov08.pdf UNITED NATIONS DEVELOPMENT PROGRAMME, Human consequences of the Chernobyl nuclear accident: a strategy for recovery, UNDP (2002). http://chernobyl.undp.org/english/docs/strategy_for_recovery.pdf WORLD HEALTH ORGANIZATION, Health effects of the Chernobyl accident and special health care programmes. Report of the UN Chernobyl Forum Expert Group ‘Health’. Eds: B. Bennett, M. Repacholi and Z. Carr, WHO, Geneva (2006). Available at: whqlibdoc.who.int/publications/2006/9241594179_eng.pdf WORLD HEALTH ORGANIZATION, Global Health Risks, WHO report, Geneva (2009). http://www.who.int/healthinfo/global_burden_disease/GlobalHealthRisks_report_full.pdf UNITED NATIONS CHILDRENS FUND, Facts for Life, Russian edition, (2008). www.unicef.org/ukraine/media_8495.html SUMMARY OF SESSION 1 H. Forsstroem IAEA, Vienna FROM ARLINGTON TO ASTANA – LESSONS LEARNED The first session was quite short and contained only four presentations. The topics covered were: a review of the 1999 Arlington conference, a review of international policies and strategies for remediation, a new UN initiative on Chernobyl and a summary of remediation activities in Kazakhstan. Ten years ago, the IAEA organized a conference entitled ‘Restoration of Environments with Radioactive Residues’ in Arlington, USA. This Astana conference is seen as a follow-up, however, there are a lot of differences between the two conferences. The Arlington conference focused on the cleanup of nuclear weapons test sites and areas affected by nuclear accidents while this conference is concentrating on uranium mining and milling sites. Also, at the time of the Arlington conference, there was quite a controversy surrounding the subject of radiological criteria for remediation and so it was an important topic at that conference. The concept of intervention had been introduced in international recommendations – and criteria had been developed to go with it. However, many countries continued to use criteria developed for normal operations for guiding remediation activities. In the USA, where the conference was being held, there was a separate ongoing controversy because of the different approaches to radiological protection being used by the regulatory agencies. An important element in the Arlington conference was the analysis of a number of test cases covering different remediation situations. The analysis showed that there was a wide variation in the radiological criteria being used as the basis for decisions on cleanup. The criteria values at the lower end of the range were judged to be due to the influence of social/political factors influencing decision making, that is, the low dose values that were being used were not cost effective. The analysis also raised the question of whether the same criterion should be used in all types of contamination situation, that is, whether a contamination situation is due to an accident or whether it is the result of a poorly controlled practice. Other questions raised were, should the same criteria be used for man-made and naturally occurring radiation, how should the public be involved in decision making, and should criteria for the cleanup of radioactive and chemical contamination be harmonized? These issues were addressed in Session 3 at this conference. The second presentation in Session 3 was a review on International Policies and Strategies for the Remediation of Land affected by Radioactive Residues. It set out the roles of the international organizations UNSCEAR, ICRP and IAEA as, respectively, providing the basic scientific knowledge, the radiological interpretation of that knowledge and the development of international standards. The presentation drew attention to the problems caused by the technical language used in this area, in particular, the term ‘contamination’ is often used in a misleading way; for example, in the context of Chernobyl affected areas, it is used to describe land which, on the basis of the associated risks, is fit for habitation. The presentation was concluded by noting that the international recommendations and standards have not yet provided a simple answer to the question “Is it safe for me and my family to live here?”. Chernobyl continues to cast a shadow over many countries and, in spite of the many studies and international reviews that show radiation doses to persons living in affected areas 37 SUMMARY OF SESSION 1 to be low, many people continue to be adversely affected in the aftermath of the accident. Unexplained physical conditions, anxiety, and mental problems are much more frequent in Chernobyl affected populations and it has been concluded that psychological and social effects now represent the main impact. A new United Nations action plan will seek to resolve the situation by promoting knowledge and understanding in those affected and to relieve their poverty. The third presentation described the plan, organized by UNDP, WHO, IAEA and UNICEF, which will seek to do this by ‘building a bridge between science and people’. The final presentation described the legacy of past nuclear activities in Kazakhstan; it included the numerous areas affected by the uranium mining and milling activities, several areas affected by nuclear weapons testing activities, the shut down fast breeder reactor at Aktau, and the many disused sealed sources used in military and civilian activities. – In the last ten years, Government remediation programmes for the uranium mining and milling sites have been effective and most sites have been cleaned up; – At the nuclear test sites, the underground testing wells and mines have been destroyed but more remains to be done before the sites can be fully opened to the public; – The spent fuel has been removed from the fast breeder reactor and a plan has been developed for transporting the packaged fuel for storage at Baikal on the Semipalatinsk Test Site; – Disused sealed sources have been collected from all over Kazakhstan and are also being stored at the Baikal waste storage site. Kazakhstan has had help in its remediation work through its cooperation with other countries and with the international organizations. 38 INTERNATIONAL COOPERATION AND SUPPORT IN ENVIRONMENTAL REMEDIATION (TOPICAL SESSION 2) Chairperson S. VOROBIEV Russian Federation REMEDIATION OF RADIOACTIVELY CONTAMINATED SITES – REVIEW OF PROJECTS SUPPORTED BY THE INTERNATIONAL SCIENCE AND TECHNOLOGY CENTER (ISTC) V. RUDNEVA, W. GUDOWSKI ISTC–International Science and Technology Center, Moscow, Russian Federation Abstract The International Science and Technology Center (ISTC) is an intergovernmental organization founded in Moscow fifteen years ago by the European Union, Sweden, Norway, Japan, the Russian Federation and the United States of America. The ISTC has focused its mission on the human dimension of non-proliferation and global safety and security through international cooperation on science and technology. The ISTC has developed a broad spectrum of tools for advancing science, improving human health, stimulating economic growth, mitigating environmental damage, and addressing other international global concerns. By January 2009, the Center and its Partners had provided US $815 million in grants, equipment, travel and training support for almost 2650 projects in diverse areas of civilian basic and applied research. These projects engaged over 71 000 scientists and engineers from 980 institutes, research centres and production facilities in collaborative work. This paper reviews the ISTC projects in the area of radioactive waste management and projects related to radioactively contaminated sites. INTRODUCTION The International Science and Technology Center (ISTC) is an intergovernmental organization founded by the European Union (EU), Sweden, Norway, Japan, the Russian Federation and the United States of America (USA) in 1992. Some time later, Canada and the Republic of Korea joined the ISTC. Presently, the ISTC ‘family’ consists of 39 members (27 from EU). The ISTC defines its goals as follows: – Addressing the human dimension of non-proliferation, including redirecting and engaging the intellectual potential of former weapons experts into challenging civilian projects; – Support of basic and applied research and technology development; – Contribution to the solution of national and international technical problems of global or regional dimensions; – Contribution to the transition to market-based economies; – Assistance in the integration of scientists from the Confederation of Independent States (CIS) into the international scientific community. The ISTC is a unique organization focused on the responsible use of sensitive knowledge and technology through international cooperative scientific and technical projects. Through these projects, based on scientific excellence, the ISTC has built up trust and confidence among scientific communities dealing with problems of global safety and security. The ISTC has developed a broad spectrum of tools for advancing science, improving human health, stimulating economic growth, mitigating environmental damage, and for addressing other global concerns. The ISTC Secretariat has its headquarters in Moscow with branch and information offices in six CIS countries. An internationally recruited staff manages, oversees and monitors more than 680 active projects under the Science Project Programme, provides training and business support to CIS project managers, and implements the Center programmes that support the integration of scientists into the international community. 41 TOPICAL SESSION 2 The Science Project Programme is the most comprehensive activity conducted by the ISTC. Through this programme, the ISTC solicits scientific project proposals from institutes throughout the CIS and provides funding and logistic support to project teams. Ultimately, the Science Project Programme together with other supplementary ISTC programmes supports and enforces the transition to sustainable, innovation driven science and technology. By January 2009, the Center and its Partners had provided US $815 million in grants, equipment, travel and training support for almost 2650 projects in diverse areas of civilian basic and applied research. These projects have engaged more than 71 000 scientists and engineers from almost 980 institutes, research centres and production facilities, involving many of the best scientists from Russia and other CIS countries, including many foreign collaborators. Statistically, ISTC projects cover fourteen technology areas. The main areas are Biotechnology and Life Sciences, Ecology, Physics, Fission Reactors, Materials, Instrumentation, Space and Aircraft and Surface Transportation, and Non-Nuclear Energy (Fig. 1). Other 18.7% Biotechnology and Life Sciences 13.0% Space, Aircraft and Surface 3.6% Chemistry 6.3% Physics 12.8% Environmental 16.2% ` Fission Reactors 10.4% Non-Nuclear Energy 2.6% Materials 8.2% Instrumentation 4.6% Information and Communication 3.5% FIG. 1. Technology areas supported by ISTC projects. In 1997, the ISTC launched the Partner Programme as a tool to provide long term cooperation between research and technology development communities in the Russian Federation/CIS and private organizations, research institutes and other entities in ISTC member states. Through this programme, the Partners have funded and conducted science and technology projects using a very flexible and transparent ISTC framework which has minimized the risks of failure and also administrative and overhead costs [1]. By January 2009, the Partner organizations had committed nearly US $245 million to scientific research through 692 ISTC projects. The ISTC currently has more than 300 partners. Among active ISTC partners are such organizations as European Organization for Nuclear Research (CERN), Commissariat à l’Énergie Atomique (CEA), Areva, Airbus, Danone, Defense Advanced Research Projects IAEA (DARPA), Bayer, Boeing, General Atomic, Cambridge Research Centre and others. OVERVIEW OF ISTC PROJECTS RELATED TO RADIOACTIVE WASTE MANAGEMENT One of the most complicated ecological problems in the Russian Federation, Kazakhstan and some other CIS countries is the management of radioactive waste 42 RUDNEVA, GUDOWSKI accumulated as a result of past activities in the production and testing of nuclear weapons, use of nuclear energy for peaceful purposes, and as a result of reductions in nuclear arms. The radioactive waste situation in the Russian Federation required immediate actions to achieve improvement. The safe management of radioactive waste is a challenge which is not limited to the Russian Federation alone; it concerns all states engaged in nuclear activities. A number of countries and international organizations have started cooperative projects with the Russian Federation in the handling of accumulated radioactive waste and spent fuel. In order to promote and to coordinate these efforts, a special Contact Expert Group (CEG) for international radioactive waste projects in the Russian Federation was established under the auspices of the International Atomic Energy Agency in 1996. The ISTC has worked in close cooperation with CEG and ISTC projects are included in the database of IAEA projects. New proposals are discussed at workshops of CEG, and priorities for new projects are identified. The results of ongoing projects are presented at international conferences, seminars and workshops. The ISTC projects in the field of management of radioactive waste and spent nuclear fuel are classified as follows: 1. 2. Management of Radioactive Waste and Spent Nuclear Fuel: – Treatment of High-Level Waste (HLW); – Treatment of Low- and Intermediate Level Waste; – Storage and Disposal. Decommissioning of Nuclear Facilities: – Decommissioning of Nuclear Power Plants (NPPs); – Decommissioning of Nuclear Submarines; – Decontamination and Remediation of Nuclear Sites. The majority of ISTC projects in this field deal with the different techniques to be used for waste volume reduction. These include: HLW solidification technology, development of matrix compositions (glass, mineral-like and ceramic compositions) ensuring mechanical, chemical and radiation stability during long term storage and final disposal; technologies for incinerating the combustible part of waste, selection of geologically suitable sites, environmental monitoring, solidified radioactive waste condition monitoring, prediction of the environmental impact of radioactive waste storage facilities and burial sites throughout their entire operation, development of a computer-based data system for the evaluation of the radiation legacy of the former Soviet Union, and evaluation and development of decontamination and rehabilitation techniques. By January 2009, 140 projects had been funded by the ISTC Parties (about USUS $ 48.5 million in funds were provided). About 50 Russian and CIS institutions are involved as project leaders or participants. More than 75% of them are from the Russian Federation. The most active institutions submitting projects to the ISTC have been the following: Khlopin Radium Institute, St. Petersburg, All-Russian Scientific Research Institute of Non-Organic Materials named after A. Bochvar, Moscow, All-Russian Research and Design Institute of Production Engineering (VNIPIPT), Moscow, Russian Federal Nuclear Center – Zababakhin All-Russia Research Institute of Technical Physics (VNIITF), Snezhinsk, Russian Federal Nuclear Center-All Russian Scientific Research Institute of Experimental Physics (VNIIEF) Sarov, Institute for Physics and Power Engineering named after A.I. Leypunsky (IPPE), Obninsk, Nuclear Technology Safety Center, Almaty, Kazakhstan, Institute of Atomic Energy, Kurchatov, Kazakhstan, Kurchatov Research Center, Moscow, and the All-Russian Research Institute of Chemical Technology (VNIIKhT), Moscow. 43 TOPICAL SESSION 2 About 350 institutes, companies, and governmental organizations from the United States of America, the European Union, Norway, Japan and the Republic of Korea have participated in the projects related to radioactive waste management as collaborators. The unique role of the ISTC in the promotion of cooperation to resolve the most severe environmental problems is particularly visible in the ISTC Projects No. 245 (245, 245-2B, 245-2C) ‘Radiation Contamination Database’ and No. 2097 ‘Radio-Ecological Database’. These projects, led by the All-Russian Research Institute of Chemical Technology, Moscow, were financially supported by EU and Sweden. Project No. 245 had three phases and the main result of the work was a database containing all potential and existing dangerous radiation sources spread over the territories of CIS countries. The project led to the formation of the ‘RadLeg GeoInformational Center’ under MinAtom of the Russian Federation, where the database is maintained. This comprehensive computerized database permits the prioritization of territories according to potential dangers. The implementation of this project involved 26 institutions, 7 ministries, and 2 State Committees in the Russian Federation. Scientists from Kazakhstan, Ukraine, Kyrgyzstan, Uzbekistan, and Tajikistan were also involved in the expert-evaluation process. The Radio-Ecological Database was developed under Project No. 2097 and, this together with the modelling of the radionuclide migration processes, helped to start an assessment of the impact of the sources on the environment and population and the development of recommendations on countermeasures. OVERVIEW OF ISTC PROJECTS RELATED TO THE REMEDIATION OF NUCLEAR SITES Like many other countries, the Russian Federation faces the challenge of decontaminating and remediating its territories, conditioned by the ongoing process of nuclear power plant and nuclear site decommissioning. Recognizing the global scale of these problems, the ISTC has funded many projects in this field. Some of the projects related to remediation of contaminated soil are: No. 0016 ‘Development of electro kinetic and chemical methods for the rehabilitation of soil and ground water contaminated by radionuclides and heavy metals’, with the Federal State Unitary Enterprise Research and Development Institute of Power Engineering named after N.A.Dollezhal, Moscow, as the Lead Institute. The aim of this project was to develop a new technology for the decontamination of sites. Successful application of the technique was demonstrated in the laboratory and at a site affected by 137Cs decontamination. A state-of-theart complexant for the selective removal of contaminants from soil was developed together with a mobile installation for removing contaminants from soil. No. 1567 ‘Use of IPEC for Remediating Soils Contaminated from Nuclear and Industrial Activities’; with the All-Russian Scientific Research Institute of Non-Organic Materials named after A. Bochvar, Moscow, as the Lead Institute. The project was aimed at the development of technique for applying new polymeric stabilizers to protect soils against wind and water erosion and to restore the plant cover. The project’s results have shown that interpolyelectrolite complexes (IPEC)-based polymers are suitable for preventing radionuclide spread by wind/water erosion through combining the most contaminated finely dispersed soil fractions into larger aggregates which are more stable against erosion processes. Accidental events leading to a real contamination require a combination of efforts directed to soil stabilization to prevent the spread of radioactivity in the shortest possible time and with minimum personnel exposure. No. 2055 ‘Development and Demonstration of Technology for the Decontamination of Solid Surfaces and Soils by Subcritical Carbon Dioxide’ with the Khlopin Radium Institute, St Petersburg, as the Lead Institute. The main objective of the project was development of a decontamination technology for soils and other solids (protective clothes, individual 44 RUDNEVA, GUDOWSKI protection equipment) using subcritical CO2. The subcritical decontamination technology developed was tested on a large scale with the use of real contaminated samples, including soils. No. 3189 ‘The Development of Composition and Technology of Amendment Production for Rehabilitation of Soils Contaminated by Radionuclides and Assessment of Their Application Efficiency’, with the Scientific and Production Association Typhoon, Obninsk, Kaluga as the Lead Institute. This is an ongoing project; the project goal is to develop a technology for producing the most effective and ecologically safe additives and organo-mineral mixtures based on natural raw material and industrial waste and a method for forecasting their efficiency. The main applications of the project are the rehabilitation of soils contaminated by radionuclides in Belarus and Russia after the Chernobyl NPP accident. Recommendations on the production of additives for soil rehabilitation will be produced. No. B-247 ‘Rehabilitation of the Environmental Objects Contaminated with Radionuclides’ with the Joint Institute of Energy and Nuclear Research - Sosny, Minsk, Sosny, as the Lead Institute. The project is aimed at developing a decontamination method for soil and sewage water contaminated during the Chernobyl accident and as a result of other nuclear activities. Analytical and mathematical models were developed for the electro kinetic process of water and soil cleanup. A method of decontamination, with the use of special plants to accumulate radionuclides, was developed. Two Belarus patent applications were filed on the basis of the project results. No. B-852 ‘Development of Conversion Technology for the Isolation of Radionuclidefree Cellulose and Nitrolignin from the Straw of Agrocultures as a Method for Rehabilitation and De-activation of Territories’ with the Belarusian State University/Institute of Physical Chemical Problems, Minsk, as the Lead Institute. This approach was suggested for the rehabilitation of radionuclide-polluted lands based on the implementation of a specially developed technology for producing pulp and paper products and soil ameliorants. This approach not only minimizes the contamination levels of affected areas but also creates a potential market for materials produced in the affected areas. No. K-237 ‘Development of Methods for Remediation of Soils with Increased Contents of Heavy Metals, Radionuclides and Improvement of Soils for Ecologically Clean Agricultural Production Systems Taking into Account the Population Health Indicators’ with the Kazakh Research Institute of Fruit Growing and Viticulture, Almaty, Kazakhstan as the Lead Institute. The objective of this project was to develop methods for the remediation of polluted geosystems and for the improvement of soils for clean agricultural production and the prophylaxis of effects on the health of the population. A new amelioration scheme for technogenic-polluted soil was developed based on the principles of antagonism-synergism of elements and a change of regimes of nutrition and irrigation of crops. For medium- and heavily-polluted soils, the best ameliorates were colloid sulphur, boron with aluminum and boron with magnesium on a bio-humus background. Recommendations were made for the rehabilitation of public and environmental health in affected regions of south and southeast Kazakhstan. No. K-632 ‘Genetic Overall Examination of the Ecological Situation at the Toxic Waste Storage Koshkar-Ata and the Development of Rehabilitation Actions’ with the National Nuclear Centre of the Republic of Kazakhstan/Institute of Nuclear Physics, Almaty, Kazakhstan as the Lead Institute. The purpose of the project was to investigate the current ecological situation in the territories adjacent to the Koshkar-Ata tailings pond and to develop rehabilitation measures, taking into consideration local soil/climatic peculiarities. A primary outcome of the project was the development of proposals for stage-by-stage rehabilitation of the land. Two control sites within the project are now also part of a special governmental programme on the full-scale rehabilitation of the tailings pond. The ISTC project was central in raising awareness among state and local authorities of the need to address rehabilitation 45 TOPICAL SESSION 2 problems at Koshkar-Ata. In 2007, the Government of the Republic of Kazakhstan allocated US $1 million from the state budget for the first stage of rehabilitation and restoration at the tailings pool Koshkar-Ata. CONCLUSIONS The ISTC has played a very important role in stimulating and supporting projects focused on environmental remediation in the Russian Federation, Kazakhstan and other CIS countries. Research teams have concentrated their attention and scientific efforts on technologies suitable for environmental remediation and protection. For specific technical information on the projects, the project recipient institutes may be contacted [2]. REFERENCES [1] [2] 46 The ISTC Annual reports – ISTC, Moscow (1996-2007). ISTC website: www.istcinfo.ru. SUMMARY OF SESSION 2 S. Vorobiev Russian Federation INTERNATIONAL COOPERATION AND SUPPORT IN ENVIRONMENTAL REMEDIATION From the presentations in Session 2, it is clear that a wide range of international organizations are well-positioned to undertake work in the remediation of lands affected by radioactive contamination in Central Asia: – The Organization for Security and Co-operation in Europe (OSCE) with a mandate for facilitating broader environmental rights and security and heightened regional profiles; – The European Commission, previously through its TACIS programme and now through its Instrument for Nuclear Safety and Cooperation (INSC); – The European Bank for Reconstruction and Development (EBRD) through its range of funds dedicated to radioactive damage prevention and remediation; – The International Scientific Technology Center (ISTC) with its wide network of scientists, radioactive contamination database and research and development expertise; – The North Atlantic Treaty Organization (NATO) through its active measurement and assessment projects in this area; – The International Atomic Energy Agency as an ideal forum for cooperation with tools for establishing safety standards, knowledge transfer, technical and regulatory capacity-building; – The World Health Organization (WHO) whose mandate includes radiation health matters; and – The United Nations Development Programme (UNDP) whose regional office in Central Asia has already initiated cooperation between regional actors. Several issues permeated the presentations of the representatives of all of these organizations and of the ensuing discussion: (a) The need for better coordination between international organizations (although all organizations expressed their eagerness to engage with one another and provide expertise); (b) The importance of ownership and commitment by the national host government in its approach to radioactive waste management; (c) The necessity of regional, trans-boundary approaches guided by ‘master-plans’, or ‘road-maps’; (d) The integration of regulatory aspects into international radiological assistance projects; (e) The need to consider the problem of environmental remediation from a multi-faceted perspective, including not only direct health effects, but also lasting economic, social, and psychological consequences; (f) The best ways of measuring success. Are concrete, scientific measurements and indicators the only method or should broader criteria of social contentment also play a role? (g) The urgency of finally moving from talk, surveys and assessments to concrete actions; (h) The ability of the aforementioned organizations to bring together interested stakeholders. 47 SUMMARY OF SESSION 2 Considering the discussions of the panel of speakers, these points should form the basis for any new approach for assessing the effectiveness of aid being rendered to countries, for improving the quality and relevance of the aid and for strengthening the coordination of the organizations involved in radioactive waste remediation. One possible scenario for cooperation, which could guide the international approach to remediation in Central Asia, is the Contact Expert Group (CEG), a model for coordination developed by the IAEA and used with much success in relation to the environmental problems in North-West Russia. A CEG for Central Asia would bring together all interested states, international organizations, donor organizations, non-governmental organizations, and independent experts for working-level meetings and annual plenary sessions. The purpose of the CEG would be to: (1) Stimulate cooperation, coordination, and co-funding of remediation activities; (2) Share information on past, ongoing, and planned activities in order to maximize effectiveness and avoid redundancy; (3) Exchange information on best practices and experiences to avoid repeating historical mistakes; (4) Provide a stable platform with permanent membership for the elaboration of joint projects; (5) Outline what specifically needs to be funded and what regional solutions are available. A high-level political conference designed to generate awareness, political will and technical expertise in order to increase funding to support land remediation projects in Central Asia is planned. It was suggested that this conference would provide a good forum for discussing the idea of a Central Asian CEG model in the context of land remediation. 48 COMPLYING WITH SAFETY CRITERIA (TOPICAL SESSION 3) Chairperson A.J. GONZÁLEZ Argentina THE EXISTING REGULATORY FRAMEWORK IN RUSSIA ON ENVIRONMENTAL REMEDIATION N.K. SHANDALA*, M.F. KISELEV**, M.I. BALONOV***, M.K. SNEVE**** * Burnasyan Federal Medical Biophysical Centre, Moscow, Russian Federation ** Federal Medical-Biological IAEA of Russia, Moscow, Russian Federation *** Institute of Radiation Hygiene, St-Petersburg, Russian Federation **** Norwegian Radiation Protection Authority, Oslo, Norway Abstract The paper addresses the public radiation exposures and medical consequences resulting from the territories of the Russian Federation contaminated with residual radioactive materials due to nuclear weapons tests and large-scale accidents. A comparison is made between the current Russian system of environmental remediation regulation and the new international approaches of ICRP Publication 103. 1. INTRODUCTION The nature and extent of radioactive contamination of territories in the Russian Federation is currently assessed in relation to the regulations established on the basis of the Russian legislation in the fields of sanitary and epidemiological supervision of the public, radiation safety and protection of the environment. The same regulations are used to define harm to human health and the environment. According to current Russian legislation, the Federal Medical-Biological IAEA (FMBA of Russia) is responsible for medical and sanitary support as well as for state sanitary epidemiological supervision. It covers organizations in some industrial branches at which there are especially hazardous work conditions and the population of some Russian territories according to a list approved by the Government. This list includes all radiation hazardous facilities in Russia (more than 400 facilities). One of the FMBA’s principle functions is the state regulatory supervision of safety in nuclear energy exploitation. 2. PROBLEMS IN THE NUCLEAR INDUSTRY AND LAND AFFECTED BY RADIOACTIVE MATERIAL RESIDUES IN RUSSIA Routine discharges from nuclear facilities do not contribute significantly to the exposure of the general public. In contrast, some historical radioactive releases which occurred in emergency situations (Techa River, 1949, Kyshtim, 1957, Chernobyl, 1986) resulted in radiation doses to population groups that significantly exceeded safe levels (see Table 1). Exposures of this magnitude can lead to adverse health effects such as radiation sickness and a long-term increase in the incidence of cancer in the residents of the affected areas (Table 2). The research institutions of the FMBA study the consequences of the contamination of Techa River, Southern Urals, due to both unauthorized radioactive discharges from the PA Mayak in the late 1940s and the accident at Mayak in 1957. These institutions are: the Southern Urals Institute of Biophysics and Urals Research Centre of Radiation Medicine. 51 TOPICAL SESSION 3 TABLE 1. RADIATION DOSES FROM MAN-MADE RADIONUCLIDE RELEASES (AFTER UNSCEAR [1]) Source Time period Significant nuclides Mean dose (mSv) Global fallout 1950-2020 137 1.1 Techa River 1949-2020 90 50-2000 Chernobyl 1986-2056 131 Cs, 90Sr, 131I, 14C, 3H Sr, 89Sr, 137Cs, other I, 134Cs, 137Cs, 90Sr Effective - up to 500; Thyroid - up to 104 (mGy) TABLE 2. OBSERVED HEALTH EFFECTS FROM ENVIRONMENTAL EXPOSURES (AFTER UNSCEAR [1]) Source Number of persons exposed Global fallout Few billions Techa River 28 thousand Chernobyl Few millions Observed health effect None observable against a very large background of cancer incidence 100-1000 cases of chronic radiation sickness; leukemia and solid cancer 2000 thyroid cancers in children by 2000; more are expected Following some nuclear accidents, various radiobiological effects in non-human species, e.g. plants and animals, have also been observed. Thus, managing the mitigation of effects applies to the environment generally, as well as to humans. In addition to the above mentioned challenges in the Russian nuclear industry, some additional problems affecting the land areas of Russia are to be considered: the inadequacy of the containment provided by some shallow radioactive waste storage facilities (and the absence of any reserve of storage facilities at some NPPs) and the consequences of military activities within the areas of nuclear submarine bases. (This latter activity has resulted in large amounts of the spent nuclear fuel and radioactive waste being accumulated at the sites of temporary storage in the Russian Northwest and Far East.) Radioactive contamination due to the presence of uranium tailing dumps is also a very important environmental issue for Russia. The residents of some Russian settlements are subjected to significant radiation exposure due to high concentrations of 222Rn in dwellings. For example, an unsatisfactory situation in this respect exists at two areas under FMBA responsibility. These are: Oktyabrsky village in Chita region (Eastern Siberia, the Chinese border) and Lermontov city in the Stavropol Territory. Oktyabrsky village is situated in the neighbourhood of the largest Russian uranium complex facility. Radiation dose rates in the area of this village are typical for uranium containing areas. Levels exceeding the 222Rn limit (200 Bq/m3) have been found in 39% of dwellings. The FMBA submitted the findings of its examinations to Rosatom (the State Atomic Energy Corporation) and, at the end of 2007, the decision was made to re-settle the residents of this village. A similar problem in Lermontov city, which has about 1000 dwellings with high radon levels, is not yet solved. Thus, in the foreseeable future, the Russian nuclear industry will have to solve many resource-intensive environmental problems. For this purpose, the special Federal Target Programme ‘Nuclear and Radiation Safety for 2008 and for the period till 2015’ is currently in force in Russia. The FMBA is taking part in some activities within this Programme. 52 SHANDALA et al. 3. CURRENT REGULATION OF ENVIRONMENTAL REMEDIATION IN RUSSIA National radiation protection standards of many states, including Russia, are based on documents of the International Commission on Radiological Protection (ICRP) and of the International Atomic Energy Agency: – – – ICRP: Recommendations on Radiological Protection (Publication 103, 2008 [2]); IAEA: Basic Safety Standards, 1996 [3] (now under revision); Russia: Radiation Safety Standards (NRB-99), 1999; (to be reviewed). NRB-99 contains guidance (intervention criteria) with respect to previously radioactively contaminated areas. Optimized protective and remedial measures are recommended at annual doses within the range 1 - 20 mSv; at a dose > 20 mSv, residence within the territory is forbidden. Quite good compliance with the recommendations of ICRP Publication 103 is evident; nevertheless, the existing application of the lower boundary (1 mSv/year) for large-scale situations (Chernobyl, Kyshtym, Techa) seems to be inappropriate. This can be explained by the Chernobyl Law adopted on the rise of democracy at the early 1990s and by the incorrect use of the public dose limit in the case of emergency and existing exposure situations. 4. REGULATORY TRENDS IN ENVIRONMENTAL REMEDIATION IN RUSSIA According to ICRP Publication 103 [2], environmental contamination can be considered as an existing exposure situation, i.e. the exposure situation already exists when a decision has to be made on radiation protection. This kind of exposure situation includes prolonged exposure due to excess radiation background, after radiation accidents and following previous radiation substance handling (including nuclear weapon manufacturing and tests, etc.). In many respects, the Chernobyl accident resulted in the generation of such exposure situations. The previous ICRP publication on this subject, Publication 82 (1999) [4], and the IAEA documents (WS-R-3 [5], WS-G-3.1 [6]) recommended the following principal provisions with respect to remediation situations: – Dose limits cannot be used; – Criteria for the human protection – justification and optimization of intervention; – General criterion of non-intervention – non-exceedance of an annual effective dose to the public (due to all environmental sources (including background)) of 10 mSv. Intervention should be implemented above this level. ICRP Publication 103 [2] and a draft special ICRP Publication on remediation (2009) reject the previously mentioned ‘intervention’ concept and introduce the ‘reference dose or risk level’. The reference level is a level above which radiation exposure is not allowed, and so optimized protective measures are to be taken. The regulatory body should establish the reference level for the specific or typical situation. In the case of existing exposure situations, the reference level of annual effective dose is suggested to be in the range from 1 mSv to 20 mSv. Higher levels are proposed to be applied for larger-scale situations. In addition to the review of the Russian NRB-99, some special criteria for environmental remediation are to be developed. The special environmental programmes and Government directives serve as the legal basis for carrying out such developments: – The Federal Law on ‘The Special Environmental Remediation Programmes of Some Parts of the Territory under Radioactive Contamination’, 2001; 53 TOPICAL SESSION 3 – The Federal Law on ‘The Transfer of Lands from One Category to Another‘, 2004; – The Government Directive on ‘Use of Lands under Radioactive or Chemical Contamination, Performance of Reclamation Operations there, and Establishment of Security Areas’, 2004. According to these laws, remedial measures must be anticipated at the stage of the remediation design development. The programme of site remediation must be developed for normal living activities of the population and land use. Information on the radiation situation must be provided in relation to the public living close to the facility in the affected zone. International cooperation can play a significant role in regulatory aspects of environmental remediation because of the similarity of the problems existing in the states which have researched and developed nuclear technologies. The large-scale international collaborative project with participation of the Norwegian Radiation Protection Authority and the FMBAederal Medical Biological IAEA is an example of the application of up-to-date regulations to environmental remediation in Russia. This project deals with radiation safety regulation in Northwest Russia, in particular, at the Kola Peninsula, where two ex-navy bases are located. At these bases, spent nuclear fuel and radioactive waste from nuclear submarines is are stored. In the course of such cooperation, the FMBA’s specialists together with their Norwegian colleagues have developed many regulatory documents based on the findings of scientific research. These documents include the remediation criteria and regulations relevant to the site of spent nuclear fuel and radioactive waste temporary storage, taking into account up-to-date ICRP approaches. 5. CONCLUSIONS – Nuclear weapons tests, large-scale radiological accidents, discharges of effluents from nuclear facilities and poor storage of solid radioactive waste have led to the appearance of man-made radionuclides in the biosphere as a whole and to excess radioactive contamination of some areas of Russia. Defense activities have been the largest contributor to this areal contamination. – Levels of radiation exposure of environmental media, typical for the routine operation of the nuclear energy using facilities, are hundreds and thousands of times less than those, which can affect the biota. However, radiation effects in environmental media have been found in limited areas within territories most contaminated after the accidents at Chernobyl accident in 1986 and at PA Mayak in 1957. – In many respects, the ICRP and IAEA have developed the international radiation protection system for the existing (prolonged) public exposure situations under the influence of the Chernobyl experience. – The current Russian radiation protection system is not well enough arranged in its documentation and differs from the international one, in particular, in the application of the dose limit for planned exposure situations (1 mSv/year) for situations of emergency and existing exposure. REFERENCES [1] [2] 54 UNITED NATIONS SCIENTIFIC COMMITTEE ON THE EFFECTS OF ATOMIC RADIATIONS, UNSCEAR 2000 Report to the General Assembly, with scientific annexes (2000). INTERNATIONAL COMMISSION ON RADIOLOGICAL PROTECTION, Recommendations of the ICRP, Publication 103, Ann. ICRP 37 2-4 (2008). SHANDALA et al. [3] [4] [5] [6] INTERNATIONAL ATOMIC ENERGY AGENCY, International Basic Safety Standards for Protection Against Ionizing Radiation and for the Safety of Radiation Sources, Safety Series 115, IAEA, Vienna (1996). INTERNATIONAL COMMISSION ON RADIOLOGICAL PROTECTION, Protection of the Public in Situations of Prolonged Radiation Exposure, Publication No. 82, Pergamon Press, Oxford, New York (2000). INTERNATIONAL ATOMIC ENERGY AGENCY, Remediation of Areas Contaminated by Past Activities and Accidents, Safety Standards Series, WS-R-3, IAEA, Vienna (2003). INTERNATIONAL ATOMIC ENERGY AGENCY, Remediation Process for Areas Affected by Past Activities and Accidents, Safety Standards Series, WS-G-3.1, IAEA, Vienna (2007). 55 US POLICIES FOR CLEANUP AT RADIOACTIVELY CONTAMINATED SITES S. WALKER US Environmental Protection IAEA, Washington, D.C., United States of America Abstract The United States Environmental Protection IAEA (EPA) Office of Superfund Remediation and Technology Innovation is responsible for implementing the long term (non-emergency) portion of a key law regulating cleanup: the Comprehensive Environmental Response, Compensation and Liability Act, CERCLA, nicknamed ‘Superfund.’ This paper provides a brief overview of the approach used by EPA to conduct Superfund cleanups at contaminated sites, including those that are contaminated with radionuclides, to ensure protection of human health and the environment. The theme emphasized throughout the paper is that within the Superfund remediation framework, radioactive contamination is dealt with in a manner consistent with chemical contamination, except to account for the technical differences between radionuclides and chemicals. This consistency is important since at every radioactively contaminated site being addressed under Superfund’s primary programme for long term cleanup, (the National Priorities List), chemical contamination is also present. 1. INTRODUCTION The United States (US) Environmental Protection IAEA (EPA) Office of Superfund Remediation and Technology Innovation (OSRTI) is responsible for implementing the longterm (non-emergency) portion of a key law regulating cleanup: the Comprehensive Environmental Response, Compensation and Liability Act, CERCLA, commonly known as ‘Superfund.’ The purpose of the Superfund programme is to protect human health and the environment over the long term from releases or potential releases of hazardous substances from abandoned or uncontrolled hazardous waste sites. The focus of this paper is on Superfund, including how radiation is addressed by the Superfund programme. This paper provides a brief overview of the approach used by EPA to conduct Superfund cleanups at contaminated sites, including those that are contaminated with radionuclides, to ensure protection of human health and the environment. The paper addresses how it is determined if a site poses a risk to human health and the framework used to determine cleanup levels. The theme emphasized throughout the paper is that within the Superfund remediation framework, radioactive contamination is dealt with in a manner consistent with chemical contamination, except to account for the technical differences between radionuclides and chemicals. This consistency is important since at every radioactively contaminated site being addressed under Superfund’s primary programme for long term cleanup, (the National Priorities List (NPL)), chemical contamination is also present. While every Superfund site is unique, and thus cleanups must be tailored to the specific needs of each site, there are two requirements that must be met at each site. Firstly, CERCLA requires that all remedial actions at Superfund sites must be protective of human health and the environment. Therefore, cleanup actions are developed with a strong preference for remedies that are highly reliable, provide long term protection and provide treatment of the principal threat by permanently and significantly reducing the volume, toxicity, or mobility of the contamination. In addition, EPA believes that site cleanups should protect ground water that is a current or potential source of drinking water to drinking water standards whenever practicable. Secondly, CERCLA specifically requires Superfund actions to attain the standards and requirements found in other State and Federal environmental laws and 57 TOPICAL SESSION 3 regulations unless there is a specific basis for waiving that standard or requirement. This mandate is known as compliance with ‘applicable or relevant and appropriate requirements’ or ARARs. 2. REMEDY SELECTION A comprehensive regulation known as the National Oil and Hazardous Substances Pollution Contingency Plan or NCP contains the guidelines and procedures for implementing the Superfund programme. The NCP sets forth nine criteria for selecting Superfund remedial actions. These evaluation criteria are the standards by which all remedial alternatives are assessed and are the basis of the remedy selection process. The criteria can be separated into three levels: threshold, balancing, and modifying. The first two (of the nine) criteria are known as ‘threshold’ criteria. They are a reiteration of the CERCLA mandate that remedies must (1) at a minimum assure protection of human health and the environment and (2) comply with (or waive) ARARs. They are the minimum requirements that each alternative must meet in order to be eligible for selection as a remedy. After the threshold criteria are applied, EPA considers the other evaluation criteria. Five of the criteria are known as the ‘balancing’ criteria. These criteria involve assessing tradeoffs between alternatives so that the best option will be chosen, given site-specific data and conditions. The criteria balance long term effectiveness and permanence, reduction of toxicity, mobility, or volume, short term effectiveness, implementability and cost. The final two criteria are called ‘modifying’ criteria: new information or comments from the State or the community may modify the preferred remedial action alternative or cause another alternative to be considered. 3. RISK-BASED CLEANUP LEVELS Cleanup levels for radioactive contamination at CERCLA sites are generally expressed in terms of risk levels, rather than dose (millirem or millisieverts), as a unit of measure. CERCLA guidance recommends the use of slope factors based on the risk coefficients contained in Federal Guidance Report 13, which is based on International Commission on Radiological Protection (ICRP) publications 60 and 72. Compliance with ARARs is often the determining factor in establishing cleanup levels at CERCLA sites. However, where ARARs are not available or are not sufficiently protective, EPA generally sets site-specific remediation levels for: 1) carcinogens at a level that represents an upper-bound lifetime cancer risk to an individual of between 10 -4 to 10-6; and for 2) non-carcinogens such that the cumulative risks from exposure will not result in adverse effects to human populations (including sensitive sub -populations) that may be exposed during a lifetime or part of a lifetime, incorporating an adequate margin of safety. The specified cleanup levels account for exposures from all potential pathways, and through all media (e.g. soil, ground water, surface water, sediment, air, structures, and biota). The 10 -4 to 10-6 cancer risk range can be interpreted to mean that a highly exposed individual may have a one in 10 000 to one in 1 000 000 increased chance of developing cancer because of exposure to a site-related carcinogen. Once a decision has been made to take an action, EPA prefers cleanups that achieve the more protective end of the range (i.e. 10-6). EPA uses 10 -6 as a point of departure and establishes Preliminary Remediation Goals (PRGs) at 1 × 10-6. To assess the potential for cumulative non-carcinogenic effects posed by multiple contaminants, EPA has developed a hazard index (HI). The HI is derived by adding the non-cancer risks for site contaminants with the same target organ or mechanism of 58 WALKER toxicity. When the HI exceeds 1.0, there may be concern for adverse health effects due to exposure to multiple contaminants. Radioisotopes of uranium are generally the only radionuclides for which EPA will evaluate the HI. 3.1. Preliminary remediation goals (PRGs) PRGs are used for site ‘screening’ and as initial cleanup goals, if applicable. The PRG's role in site screening is to help identify areas, contaminants, and conditions that do not require further federal attention at a particular site. PRGs not based on ARARs are risk-based concentrations, derived from standardized equations combining exposure information assumptions with EPA toxicity data. PRGs based on cancer risk are established at 1 × 10-6. PRGs are modified, as needed, based on site-specific information. 3.2. Superfund risk and dose soil and water models EPA has developed a PRG for radionuclides electronic calculator, known as the Rad PRG calculator. This electronic calculator presents risk-based standardized exposure parameters and equations that should be used for calculating radionuclide PRGs for residential, commercial/industrial, and agricultural land-use exposures, tap water and fish ingestion exposures. The calculator also presents PRGs to protect groundwater which are determined by calculating the concentration of radioactively contaminated soil that does not result in leaching from soil to groundwater that would exceed MCLs or risk-based concentrations. The Rad PRG calculator may be found at: http://epaprgs.ornl.gov/radionuclides/. To address ARARs that are expressed in terms of millirem per year, an approach similar to that taken for calculation of PRGs is used to calculate soil ‘compliance concentrations’ based upon various methods of dose calculation in another EPA tool, the ‘Dose Compliance Concentrations’, or DCC calculator. The DCC calculator equations are identical to those in the Rad PRG calculator, except that the target dose rate (ARAR based) is substituted for the target cancer risk (1 × 10-6), the period of exposure is one year to indicate year of peak dose, and a dose conversion factor (DCF) is used in place of the slope factor. The DCC calculator may be found at: http://epa-dccs.ornl.gov/. 3.3. Superfund decommissioning models EPA has recently completed two risk assessment tools that are particularly relevant to decommissioning activities conducted under CERCLA authority. EPA developed the Preliminary Remediation Goals for Radionuclides in Buildings (BPRG) electronic calculator to help standardize the evaluation and cleanup of radioactively contaminated buildings at which risk is being assessed for occupancy. BPRGs are radionuclide concentrations in dust, air and building materials that correspond to a specified level of human cancer risk. The BPRG calculator may be found at: http://epa-bprg.ornl.gov/. EPA developed the Preliminary Remediation Goals for Radionuclides in Outside Surface (SPRG) calculator to address hard outside surfaces such as building slabs, outside building walls, sidewalks and roads. SPRGs are radionuclide concentrations in dust and hard outside surface materials that correspond to a specified level of human cancer risk. The SPRG calculator may be found at: http://epa-sprg.ornl.gov/. 3.4. Superfund ecological risk model EPA is also developing the ‘Radionuclide Ecological Benchmark’ calculator. This calculator provides biota concentration guides (BCGs), also known as ecological screening 59 TOPICAL SESSION 3 benchmarks, for use in ecological risk assessments at CERCLA sites. The calculator develops ecological benchmarks for ionizing radiation based on cell death only. 4. COMPLIANCE WITH ENVIRONMENTAL LAWS Compliance with (or waiver of) ARARs is a cornerstone of CERCLA. Because the diverse characteristics of Superfund sites preclude the development of prescribed ARARs, it is necessary to identify ARARs on a site-by-site basis. Some of the radiation standards most frequently used as ARARs at Superfund sites are the soil cleanup and indoor radon standards developed to address contamination at sites that are subject to the Uranium Mill Tailings Radiation Control Act of 1978 (UMTRCA). When used as an ARAR at Superfund sites, the soil cleanup level for radium-226 and radium-228 combined, or thorium-230 and thorium-232 combined, is 5 picoCuries per gram (pCi/g) [0.185 Becquerels per gram (Bq/g)] above background, while the indoor radon level is 0.02 working levels inclusive of background. For a list of ‘Likely Federal Radiation Applicable or Relevant and Appropriate Requirements (ARARs)’, see Attachment A of EPA's guidance ‘Establishment of Cleanup Levels for CERCLA sites with Radioactive Contamination’ at: http://www.epa.gov/superfund/health/contaminants/radiation/pdfs/radguide.pdf One extremely important category of ARARs that should be noted are Maximum Contaminant Levels (MCLs) that are established under the United States law for drinking water standards, called the Safe Drinking Water Act. EPA believes contaminated ground water should be restored to beneficial use, whenever practicable. This means that sites where the contaminated ground water is a potential or current source of drinking water should be remediated to concentrations corresponding to drinking water standards (e.g. concentrations corresponding to MCLs or more stringent State drinking water standards). The Superfund programme requires MCLs be met within the aquifer, not at the tap. The current MCLs for radionuclides are set at 4 mrem/y [0.04 mSv/y] to the whole body or an organ for the sum of the doses from beta and photon emitters, 15 picoCuries per litre (pCi/L) [0.555 Bq/L] for gross alpha, and 5 pCi/L [0.185 Bq/L] combined for radium-228 and radium-226, and 30 micrograms per litre of uranium. EPA has published concentration tables for each radionuclide that correspond to the 4 mrem/y MCL which may be found at: http://www.epa.gov/safewater/radionuclides/pdfs/guide_radionuclides_tablebetaphotonemitters.pdf. 5. SUMMARY The CERCLA framework for addressing hazardous sites ensures that risks from radioactive contamination will be addressed in a manner consistent with risks from nonradioactive contamination, except to account for technical differences posed by radionuclides. For more information and copies of EPA guidance documents for addressing radioactively contaminated CERCLA sites, see the EPA’s Superfund Radiation webpage. For more information and copies of EPA guidance documents for developing cleanup levels for long term CERCLA sites, see EPA’s Remedy Decisions webpage. These webpages may be found at: http://www.epa.gov/superfund/health/contaminants/radiation/index.htm http://www.epa.gov/superfund/policy/remedy/sfremedy/index.htm Both of these webpages contain numerous Office of Solid Waste and Emergency Response (OSWER) Directives, which are EPA’s official guidance for the Superfund programme and other material that is useful for cleaning up CERCLA sites. 60 PRINCIPLES OF URANIUM STEWARDSHIP: GUIDANCE FROM THE WORLD NUCLEAR ASSOCIATION S. SAINT-PIERRE World Nuclear Association, London, United Kingdom Abstract The World Nuclear Association (WNA) has established ‘Principles of Uranium Stewardship’ whose purpose is to ensure that uranium and its by-products are managed so as to combine safety, environmental responsibility, sound economics and social acceptability. The principles are equally relevant for operators, contractors, and regulators newly engaged in uranium mining and processing. This paper outlines the background to the principles and the essential features of the WNA principles document. 1. INTRODUCTION The worldwide community of professionals engaged in uranium mining and processing recognizes that managing health and safety, waste and the environment is of paramount importance. This recognition – and the acceptance of commensurate responsibility – is fundamental to the vision of the World Nuclear Association (WNA), its values and measures of success. Responsible management of uranium mining and processing projects should be applied at all stages of planning and activities – from exploration through to development, construction and operations, and on to decommissioning. Today, the WNA is acting to ensure that all parties directly involved in uranium mining and processing – including operators, contractors, and regulators – strive to achieve the highest levels of excellence in these fields of management. The WNA is doing this by sustaining a strong safety culture based on a commitment to a framework of common, internationally shared principles. These international principles build on – and are complementary to – the World Nuclear Association’s ‘Charter of Ethics’ and its ‘Principles of Uranium Stewardship’. The WNA Charter of Ethics is founded on the belief “... that sustainability must be the guiding principle of global development – requiring worldwide policies that meet the needs and aspirations of the present generation without compromising the opportunity of future generations to fulfil their needs and aspirations". The Waste Management and Decommissioning Working Groups (WM and DWG) of the WNA each currently consists of over forty radiation protection experts from various sectors of the nuclear industry and from around the world. This policy document was developed by a subgroup which consists of relevant uranium mining experts. The WNA Principles of Uranium Stewardship focus on the commodity on which nuclear energy is based. The principles embody best practice and ethical conduct for the entire global nuclear industry. The WNA programme of Uranium Stewardship is based on a commitment to ensure that uranium and its by-products are managed so as to combine safety, environmental responsibility, sound economics and social acceptability. The WNA document sets out principles for the management of radiation, health and safety, waste and the environment and is applicable to sites throughout the world. In national and regional settings, where activities of the nuclear fuel cycle have reached advanced stages of development, these principles already serve to underpin Codes of Practice that govern uranium mining and processing. In any given setting, a Code of Practice is needed to guide practical implementation of these principles according to the regional, national or site61 TOPICAL SESSION 3 specific context. The WNA has published these principles in the belief that they hold special relevance for emerging uranium producing countries that do not yet have fully developed regulations for the control of radiation, health and safety, waste and the environment associated with uranium mining and processing. Moreover, experience shows that close cooperation among these three parties is a key to the successful management of radiation, health and safety, waste and the environment. While the independence of regulators is clearly essential to their function, the very existence of these regulatory agencies derives from governmental recognition that uranium mining can provide socially beneficial results. Thus, the ultimate purpose of such regulators is to enable mining and processing in compliance with acceptably high standards. Of course, each principle affirmed in the WNA document will not apply to the same extent for each party. For example, general responsibility for installations and sites lies fundamentally with operators, who must accept overall responsibility for the performance of contractors. Ultimately, the precise allocation of responsibilities must be set at national and local levels. Once national regulations are fully developed, they can be expected to embody the principles enunciated in WNA’s document. During any transition period during which regulatory rules and regimes are not yet fully formed, the principles should still be applied. The WNA document holds the status of a policy and ethical declaration by the full WNA membership, which encompasses most of the wide range of enterprises that comprise the global nuclear industry – from uranium miners, to equipment suppliers, service providers, and generators of electricity. In the category of uranium miners, the WNA membership includes all major uranium mining and processing companies as well as many midsize and junior companies. The principles affirmed here are supported by key relevant international organizations, including the International Atomic Energy Agency. Indeed, these principles have been affirmed as an outgrowth of an IAEA cooperation project aimed at encouraging expanded exchanges between professionals from governments and industry. These principles are also supported by the global mining community through relevant international and national associations that cover uranium mining and processing. 2. PRINCIPLES Principle 1: Adherence to sustainable development Conduct all aspects of uranium mining and processing with full adherence to the principles of sustainable development as set forth by the International Council on Mining and Metals (ICMM). Apply these principles with emphasis on excellence in professional skills, transparency in operations, accountability of management, and an overarching recognition of the congruency of good business and sound environmental practices. Discussion: In establishing its ‘sustainable development’ principles, the ICMM adopted the landmark definition of that term advanced by the United Nations’s Brundtland Commission in 1983: “Development that meets the needs of the present without compromising the ability of future generations to meet their own needs”. To this the ICMM added: “In the mining and metals sector... investments should be financially profitable, technically appropriate, environmentally sound and socially responsible”. In emphasizing the practical necessity of financial profitability, the ICMM underscored that economic profitability and sustainable development, far from being at odds, 62 SAINT-PIERRE must be consistent and reinforcing goals. This congruency of purpose is reflected in the ICMM commitment to “seek continual improvement in performance and contribution to sustainable development so as to enhance shareholder values”. Principle 2: Health, safety and environmental protection In all management practices, ensure adequate protection of employees, contractors, communities, the general public, and the environment, as follows: Mining safety – Ensure safe, well maintained site conditions for the protection of employees and the public from all conventional mining hazards, including those related to airborne contaminants, ground stability and structure, geological and hydrogeological conditions, storage and handling of explosives, mine flooding, mobile and stationary equipment, ingress and egress, and fire. Radiation safety – Comply with the principles of Justification, Optimization and Limitation, as follows: Justification: Authorize the introduction of any new practice involving radiation exposure, or the introduction of a new source of radiation exposure within a practice, only if the practice can be justified as producing sufficient benefit to the exposed individuals or to society to offset any potential radiation harm. Optimization and Limitation: Optimize radiation exposure to as low as reasonably achievable, taking into account all socioeconomic factors. Ensure compliance with the occupational and public dose limits laid down by the appropriate national and international regulatory and advisory bodies. In so doing, classify, according to risk, site personnel and work areas that are subject to radiation exposure. Plan and carefully monitor employee and contractor doses, radioactive discharges and emissions as well as resulting environmental concentrations and exposure rates. Estimate potential radiological impacts on the public and the environment. Personal protective equipment – Ensure that employees and visitors are provided personal protective equipment (PPE) appropriate for the hazard being controlled and compliant with relevant standards or specifications to control exposure to safe levels. Ensure that relevant personnel remain properly trained in the use and maintenance of this equipment. Ventilation – Ensure that workplaces are adequately ventilated and that airborne contaminants are minimized in workplaces. Pay particular attention to controlling radon and related radiation exposures in uranium mines and processing facilities. Water quality – Develop and implement site specific water management practices that meet defined water quality objectives for surface and ground waters (focusing particular attention on potable water supplies). Subject water quality objectives to periodic review to ensure that people and the environment remain protected. Environmental protection – Overall, avoid the pollution of water, soil and air. Optimize the use of natural resources and energy and minimize any impact from the site and its activities on people and the environment. In so doing, include considerations of sustainability, biodiversity and ecology in guarding against environmental impact. Principle 3: Compliance Support the establishment of a suitable legal framework and relevant infrastructure for the management and control of radiation, occupational and public health and safety, waste and the environment. Ensure that all activities are authorized by relevant authorities and conducted in full compliance with applicable conventions, laws, regulations and requirements, 63 TOPICAL SESSION 3 including, in particular, the Safety Standards of the IAEA. In recognition that effective interaction of operators (including contractors) and the appropriate regulatory authorities is essential to safety, ensure that operators and contractors are licensed, having met the requirement of relevant authorities. Principle 4: Social responsibility At all stages of uranium mining and processing, properly inform – and seek, gain and maintain support from – all potentially affected stakeholders, including employees, contractors, host communities, and the general public. Establish an open dialogue with affected stakeholders, carefully consider their views, and provide feedback as to how their concerns are addressed. Principle 5: Management of hazardous materials Manage and dispose of all hazardous materials (radioactive or non-radioactive) – including products, residues, waste and contaminated materials – in a manner that is safe, secure and compliant with laws and regulations. Act systematically to establish and implement controls to minimize risks from such waste and contaminated materials. Take actions to maintain and treat sources of hazardous materials on-site wherever it is practicable to do so. Control and minimize any releases into the environment, using carefully planned strategies that involve pollution control technologies, robust environmental monitoring, and predictive modelling to ensure that people and the environment remain well protected. Rely, where possible, on proven, best available, industry scale technologies. Focus particular attention on managing ore stockpiles and such potentially significant sources of contamination as waste rock, tailings, and contaminated water or soils. With tailings, concentrate special effort on the design and construction of impoundments and dams and on the application of a recognized tailings management system for operations, monitoring, maintenance and closure planning. Use risk analysis and controls to account for the current and long term stability of waste repositories and containments. As an integral aspect of mining and processing, characterize the ore and waste rock. Consider the geochemistry and assess the risk of acid rock drainage (ARD); where ARD could occur, develop an ARD management plan which accounts for ARD producing ore, rejects materials and gangue, and provides for appropriate scheduling of mining, stockpile segregation, processing and contaminant containment. Use effective containment designs to ensure against long term liability from ARD producing rock. Use all opportunities to reduce the creation of hazardous waste and contaminated materials. To the extent practicable, recover, recycle and reuse such waste and materials, regarding waste disposal as a last resort option. At each site, control the release or removal of waste and contaminated materials; use a ‘chain of custody’ approach, where needed. Safely manage all off-site streams for hazardous materials and contaminated waste. Principle 6: Quality management system Employ a recognized quality management system – including the quality assurance steps of ‘Plan, Do, Check and Act’ (PDCA) – in administering the management of all activities pertinent to managing radiation, health and safety, waste and the environment. Planning – At all development and operational stages, plan the management of radiation, health and safety, waste and the environment. With the constant goal of avoiding risk and optimizing the use of natural resources and energy, update such plans regularly, and particularly in response to any significant change in activities or site conditions. Include, as a 64 SAINT-PIERRE central element in such plans, steps for the control of emergencies and unplanned events. Ensure that plans are well documented and communicated. Environmental impact assessment – In developing uranium mining or processing projects, prepare formal Environmental Impact Assessments (EIAs) that deal with all questions and concerns related to radiation, occupational and public health and safety, waste and the environment, as well as the socio-economic impact. Submit the EIA as part of the public review process so as to provide response opportunities for stakeholders, especially the workforce and host communities. During the life of a project, prepare further EIAs if and as warranted by new circumstances. Risk management – Apply risk assessment and management procedures. Identify, characterize and assess all risks that can impact on health, safety and environmental protection. Mitigate risks with controls using engineering, administration and other protective measures. Apply a hierarchy of risks and controls. Monitor risks and take timely action to offset the emergence of new risks. Regularly review performance to improve procedures, further reduce risk, detect weaknesses and trigger corrective measures. Documentation – Document and report relevant data and maintain records in compliance with regulatory requirements. Place special emphasis on data required by the quality assurance management system. Principle 7: Accidents and emergencies Identify, characterize and assess the potential for incidents and accidents, and apply controls to minimize the likelihood of their occurrence. Develop, implement and periodically test emergency preparedness and response plans. Ensure the availability of mechanisms for reporting and investigating all incidents and accidents so as to identify the ‘root cause’ and facilitate corrective actions. Principle 8: Transport of hazardous materials Package and transport all hazardous materials (radioactive and non-radioactive), including products, residues, waste, and contaminated materials, safely, securely, and in compliance with laws and regulations. For radioactive materials, adhere to IAEA Regulations for the Safe Transport of Radioactive Material, relevant IAEA Safety Guides, applicable international conventions, and local legislation. Principle 9: Systematic approach to training In each area of risk, provide systematic training to all site personnel (employees and contractors) to ensure competence and qualification; include in such training the handling of non-routine responsibilities. Extend such training, where appropriate, to visitors and relevant persons in communities potentially affected by these risks. Regularly review and update this training. Principle 10: Security of sealed radioactive sources and nuclear substances Ensure the security of sealed radioactive sources and nuclear substances, using the ‘chain of custody’ approach where practicable. Comply with applicable laws, international conventions and treaties, and agreements entered into with stakeholders on the safety and security of such sources and substances. 65 TOPICAL SESSION 3 Principle 11: Decommissioning and site closure In designing any installation, plan for future site decommissioning, remediation, closure and land reuse as an integral and necessary part of original project development. In such design and in facility operations, seek to maximize the use of remedial actions concurrent with production. Ensure that the long term plan includes socio-economic considerations, including the welfare of workers and host communities, and clear provisions for the accumulation of resources adequate to implement the plan. Periodically review and update the plan in the light of new circumstances and in consultation with affected stakeholders. In connection with the cessation of operations, establish a decommissioning organization to implement the plan and safely restore the site for reuse to the fullest extent practicable. Engage in no activities – or acts of omission – that could result in the abandonment of a site without plans and resources for full and effective decommissioning or that would pose a burden or threat to future generations. 66 ADAPTING INTERNATIONAL EXPERIENCE TO REGULATORY SUPERVISION OF LEGACY SITES IN THE CENTRAL ASIAN REPUBLICS M. SNEVE*, M. KISELEV**, N. SHANDALA***, T. ZHUNUSSOVA*, A. KIM****, U. MIRSAIDOV*****, B. TOLONGUTOV****** * Department for Emergency Preparedness and Environmental Radioactivity Norwegian Radiation Protection Authority, Osteras, Norway ** Federal Medical-Biological IAEA, Moscow, Russian Federation *** Burnasyan Federal Medical Biophysical Centre, Moscow, Russian Federation **** Kazakhstan Atomic Energy Committee, Astana, Kazakhstan ***** Tajikistan Nuclear and Radiation Safety IAEA, Dushanbe, Tajikistan ****** State IAEA for Environment Protection and Forestry of the Kyrgyz Republic Abstract This paper outlines progress being made within the regulatory cooperation programme between the Norwegian Radiation Protection Authority and its sister organizations in the Russian Federation. Experience is drawn from work at nuclear technology legacy sites, such as the Sites of Temporary Storage at Andreeva and Gremikha, and also on the remediation of uranium mining and milling facilities. The planned application of this experience to the enhancement of regulatory supervision in Kazakhstan, Tajikistan and the Kyrgyz Republic is described. Preliminary observations are made concerning how this work might feed into the development of international guidance. 1. INTRODUCTION In the last decade, the global community has addressed the environmental legacy from the earlier development of nuclear technologies. In this the general objectives have been to develop a responsible approach to environmental and human health protection and to help ensure that future developments do not create new problematic legacies. Radiation protection and nuclear safety are a significant part of legacy management, and strong independent regulatory supervision is, in turn, crucial to the delivery of safety and confidence in the whole process. At the same time, a wide range of other issues contribute to decisions on how the legacies should be managed. For example, radiation and radioactive material are not the only health protection issues at sites affected by radioactive residues; there are many other pernicious pollutants and physical safety factors to consider. Yet more broadly, decisions on legacy site management have often to be made in the recognition that there are limited financial and other resources. In addition, account has to be taken of many other social and cultural factors which operate on many different temporal and spatial scales. The overall system of norms and standards and the related regulatory process need to be strong and clear enough to provide a proper basis for environmental as well as health and safety management and flexible enough to allow an effective interface with the wider management issues so that balanced and proportionate decisions can be made. 67 TOPICAL SESSION 3 2. EXPERIENCE OF REGULATORY SUPPORT IN THE RUSSIAN FEDERATION The Norwegian Radiation Protection Authority (NRPA) is the radiation and nuclear safety regulatory authority in Norway. It falls naturally to NRPA to assist the Norwegian Ministry of Foreign Affairs in implementing the Norwegian Plan of Action on Improving Nuclear and Radiation Safety in Northwest Russia. The initial Plan of Action focused on the safety of nuclear technology development and application and therefore included consideration of nuclear power plants. A significant component of the Plan of Action is for NRPA to provide support to its sister authorities in the Russian Federation. The situation is complex because of the technical and political history. However, over the years, a considerable degree of confidence and mutual trust has been built up among all the relevant organizations, allowing for real progress to be made in meeting protection objectives. This forms a strong basis for continued cooperation to mitigate radiation risks and the prevention of the development of new legacies. The Norwegian government has recognised the effectiveness of the programme and the Plan of Action was updated in 2008 and extended until at least 2012 with renewed focus on managing the nuclear legacy from the Cold War period and other operations carried out at the time of the Soviet Union. 2.1 Who is involved? The two key regulatory authorities for civil protection in Russia are the Federal Environmental, Industrial and Nuclear Supervision Service of Russia (Rostechnadzor) and the Federal Medical-Biological IAEA (FMBA). Rostechnadzor focuses on nuclear and radiation safety and the FMBA focuses on radiological protection. Both are supported by technical support organizations, notably the Science and Engineering Centre for Nuclear and Radiation Safety (SEC-NRS) and the Burnasyan Federal Medical Biophysical Centre (FMBC). Many of the legacy issues originated from the military programme. It is therefore vital that the military authority is involved. In fact, the the Directorate of State Supervision over Nuclear and Radiation Safety of the Ministry of Defence of the Russian Federation (DSS NRS) has agreed to take part in the cooperation programme. Regulators and operators must rigorously and transparently retain their separate responsibilities and integrities. At the same time, an effective dialogue is necessary between them. Thus, the programme allows for and encourages FMBA, Rostechnadzor and DSS NRS to regularly hold information exchange meetings with other Russian authorities, notably Rosatom. Experts from other national authorities and technical support organizations participate through the review of project proposals and the provision of technical output. They include the Institut de Radioprotection et de Sûreté Nucléaire, the Swedish Radiation Safety Authority, the US Environmental Protection IAEA and the Environment IAEA of England and Wales. International contacts are maintained with the Nordic Liaison Committee for Atomic Energy, the European Union, the World Health Organization and the International Atomic Energy Agency. 2.2 What are the objectives? The objectives are: 1. 2. 68 Efficient and effective regulatory supervision of nuclear legacy projects in order to protect western and Russian investment in nuclear legacy management. Integrated coverage of nuclear and radiation safety, comprising: – Worker and public safety; – Environmental and human health protection and monitoring; SNEVE et al. – – – 3. 4. Normal and accident conditions; Emergency preparedness and response; Addressing high risk issues arising from nuclear legacies, but, at the same time; – Addressing longer term management, site remediation and waste storage and disposal, so as not to prejudice safety in the future, thereby avoiding the creation of new legacies. Long term development of an enhanced safety culture. The development of a close working relationship with Russian authorities so that future challenges can be addressed effectively. 2.3. What has been achieved? The projects have helped provide the regulatory authorities with the tools they need to carry out their responsibilities. They have resulted in: (a) Updated Federal norms and regulations and regulatory guidance which take account of international requirements and recommendations, as well as other relevant national good practice; (b) The development of effective and efficient regulatory procedures for licensing and compliance monitoring. The work began with the review and comparison of environmental impact assessment in Russia, Norway and other European countries. Based on the developed understanding of the system and situation, the industrial projects in which NRPA cooperation has supported regulatory development and supervision have included: (1) Decommissioning of the Lepse spent fuel storage vessel; (2) Decommissioning of radio-thermal generators (RTG); (3) Rehabilitation of the Sites of Temporary Storage (STS) at Andreeva and Gremikha; and (4) Development of waste acceptance criteria for storage of radioactive waste at Sayda Bay. The work has proceeded as far as the promulgation of official regulatory norms and standards. Progress is reported in technical NRPA reports [1-3] which include English translations of relevant regulatory guidance. The integrated coverage of radiological risks, from optimization of especially hazardous operations to standard setting for radioactive waste management has been especially worthwhile and effective at the Sites of Temporary Storage. The programme of work is also widely promulgated to a broader audience in conference papers (e.g. [4, 5]), but also in a less technical context in NRPA information bulletins, e.g. on a joint exercise for emergency preparedness [6] and on RTG decommissioning safety in the IAEA Bulletin [7]. Finally, it should not be forgotten that the work is fundamentally based on science, and the programme has also resulted in the publication of peer reviewed journal articles, such as one on the basis for remediation criteria [8]. 2.4. How has it been achieved? The NRPA policy has been to start by addressing real regulatory problems that need to be solved in order for legacy management projects to proceed under relevant and effective 69 TOPICAL SESSION 3 supervision. Hard work, patience, tenacity and perseverance from all concerned has been necessary but the most important factor is effective communication, particularly through listening to the real needs of Russian colleagues and then responding robustly noting the limits on resources and other practical factors. 3. RELEVANCE AND APPLICATION IN THE CENTRAL ASIAN REPUBLICS The details of situations for legacy management are different in each country, not only because of technical and geographical differences, but also because national regulatory frameworks are different, social and cultural attitudes are different and political choices on resource management can constrain options in different ways. However, the strategy approach adopted in the cooperation between the Russian authorities and the NRPA is planned to be followed with the authorities in Kazakhstan, Tajikistan and Kyrgyzstan, with broadly the same objectives. 4. NEXT STEPS The next steps in cooperation with the Russian authorities involve enhancement of regulatory compliance monitoring as major industrial projects are implemented, for example under the Strategic Master Plan V2. It is also hoped to extend the work completed at SevRAO and other facilities in NW Russia to other sites. This is already happening, for example, concerning the application of regulatory documents developed for the Lepse to the decommissioning [9] of other floating nuclear objects, and the application of hygienic standards for Very Low Level Waste Management at Sites of Temporary Storage to other sites. The initial phases of the work in Central Asia concern support in the development and application of national radioactive waste management strategies and preliminary threat assessments to determine regulatory priorities. The work will, as in Russia, be based on practical problems at real sites. Little if any of this work could be done were it not for the goodwill and positive attitude to cooperation among the project participants. However, support from international and other national organizations has also been important. The proposed establishment of a new working group for coordinating activities in the Regulatory Supervision of Legacy Sites, under the auspices of the IAEA, is therefore much welcomed. The key to success will be to make international guidance as clear and precise as possible without prejudicing the regionally or locally optimum solution. REFERENCES [1] [2] [3] [4] 70 NORWEGIAN RADIATION PROTECTION AUTHORITY (NRPA), Upgrading the Regulatory Framework of the Russian Federation for the Safe Decommissioning and Disposal of Radioisotope Thermoelectric Generators. Stralevernrapport 2007:5, Osteras (2007). NORWEGIAN RADIATION PROTECTION AUTHORITY (NRPA), Radiological Regulatory Improvements Related to the Remediation of the Nuclear Legacy Sites in Northwest Russia. Stralevernrapport 2007:11, Osteras (2007). NORWEGIAN RADIATION PROTECTION AUTHORITY (NRPA), Regulatory Improvements Related to the Radiation and Environmental Protection during Remediation of the Nuclear legacy Sites in North West Russia. Report of work completed by NRPA and FMBA of Russia in 2007. Stralevernrapport 2008:7, Osteras (2008). KISELEV, M., SHANDALA, N., GNEUSHEVA, G., et al., Radiation protection of workers from uranium mines and of the public living nearby uranium mining and milling facilities. In: SNEVE et al. [5] [6] [7] [8] [9] Proceedings 12th International Radiation Protection Association Conference, Buenos Aires (2008). SNEVE, M.K., KISELEV, M., KOCHETKO, O., et al., Practical Application of the International Safety Regime in NW Russia: Experience from the Norwegian Plan of Action. In: Proceedings 12th International Radiation Protection Association Conference, Buenos Aires (2008). NORWEGIAN RADIATION PROTECTION AUTHORITY (NRPA), Emergency Preparedness and Response Exercise for medical teams in Andreeva Bay. NRPA Bulletin 17:2006, Osteras (2006). SNEVE, M.K., Remote Chance. IAEA Bulletin 28/1. Vienna (2008). SHANDALA, N.K, SNEVE, M.K., TITOV, A.V., et al., Radiological criteria for remediation of sites for spent fuel and radioactive waste storage in the Russian Northwest. Journal of Radiological Protection 28 4 (2008). SNEVE, M.K., BERGMAN, C., MARKAROV, V., Licensing Procedures for a Dedicated Ship for Carrying Spent Nuclear Fuel and Radioactive Waste. Report from workshop held at GOSAOMNADZOR, Moscow, 2-3 July 2001. StrålevernRapport 2001:8. Østerås: Statens strålevern (Norwegian Radiation Protection Authority) (2001). http://www.nrpa.no/dav/e48eeab4ff.pdf 71 SUMMARY OF SESSION 3 A.J. González Argentina REGULATORY ASPECTS This session, which consisted of five oral presentations followed by a Panel Discussion, was mainly concerned with existing international and national safety standards for environmental remediation. In the first presentation, the ongoing process to update the International Basic Safety Standards (BSS) was described. Particular emphasis was given to the incorporation of the new standards on environmental remediation (i.e. IAEA Safety Standards No WS-R-3 of 2003) within the new BSS and the adaptation of the BSS to the new recommendations of the International Commission on Radiological Protection (ICRP) (Publication 103). In the new BSS, the remediation of land affected by radioactive residues will be considered as an ‘existing’ exposure situation, following the new ICRP classification of ‘planned’, ‘emergency’ and ‘existing’ exposure situations. However, it was pointed out in discussion that remediation may be considered at the planning stage of some operations such as mining; in this case, it would be treated as a ‘planned’ exposure situation. Moreover, it was also pointed out that although remediation is usually necessary after an emergency, such a need would normally materialize in the aftermath of the emergency and the situation therefore may be considered a ‘de facto’ existing exposure situation. The second presentation was concerned with the regulatory framework for environmental remediation in the Russian Federation. There are many situations requiring environmental remediation in Russia; they include areas affected by nuclear accidents, those due to poorly controlled practices and those that are a legacy of past military activities. At the present time, there are no comprehensive regulatory instruments for dealing with existing exposure situations in Russia but the revision of the relevant regulatory documents is cleanup and is taking account of the recent and ongoing international developments, including the recommendations in ICRP Publication103 and the requirements of the new BSS. The standards used by the United States Environmental Protection IAEA (USEPA) for environmental remediation were the subject of the third presentation. These are the CERCLA or ‘Superfund’ regulations and apply to abandoned sites at which activities such as uranium mining and milling, thorium gas mantle production and nuclear weapons production were previously carried out. The regulations are very detailed with specific numerical criteria for application to environmental materials, surfaces and aquatic media. The criteria are based on the associated risk of cancer – unlike those in international recommendations and standards that are used by other US Federal Agencies which are based on weighted radiation dose criteria. Because the criteria are different, ‘ad hoc’ agreements have been reached between the US agencies to cover situations where their jurisdictions overlap. In the fourth presentation, the new guidance from the World Nuclear Association on principles for the decommissioning and remediation of uranium mining and milling facilities was presented. The guidance stresses the need for proper planning at the design stage to anticipate all of the issues which will arise - including the provision of sufficient financial resources for decommissioning and the arrangements for the long term management of waste. In the fifth and final presentation, a plan to assist in the regulatory supervision of legacy sites in the Central Asian Republics proposed by the Norwegian Radiation Protection Authority (NRPA) was described. The extensive disused uranium mining and milling sites in 73 SUMMARY OF SESSION 3 these countries are in need of remediation. Based on the previous experience of the NRPA in Russia, the plan envisages assisting the countries by improving regulatory infrastructures and, in particular, providing training to the regulatory body in procedures and regulatory supervision. It was also suggested that IAEA might become involved, for example, by promoting forums of regulators to discuss common problems. In the Panel Discussion, some of the questions related to criteria for remediation that remained unanswered at the Arlington conference were addressed, namely: (1) Have consistent criteria been established that provide guidelines for the remediation of contaminated sites? (2) Can a single criterion be applied to the remediation of all forms of contaminated site, be they nuclear test sites, areas resulting from accidents, the termination of practices, mining and milling activities or legacy discharges? (3) Should areas contaminated with manmade versus natural radioactive material have different criteria? Can the same criteria be used for both? (4) Should the public being involved during the decision making process? (5) How can it be ensured that overly conservative and unrealistic modelling is not being used which could lead to an overestimation of the risks? (6) Have the cleanup levels and goals for sites that are contaminated with chemical and radioactive material been harmonized? (7) How can the removal of material from one site to another versus stabilizing the material in place be justified? The Panel, composed of the presenters of the papers in this session, responded to the questions arising from the Arlington conference, as follows: – In response to the question concerning the global unification of criteria for remediation, it was concluded that the international recommendations of ICRP and the intergovernmental safety standards issued by the IAEA provide a framework within which optimized criteria can be developed taking into account country and site specific features. The USEPA risk based approach differs from the radiation-dose based approach recommended by the international organizations and used in most countries. In the context of the subject of the conference, it was noted that the risk based approach has the merit of allowing radiation risks to be compared on the same basis as risks from chemical hazards. However, it was observed that there are some problems with the approach and these have been discussed by the ICRP. The aims of any approach used should be the same, namely protecting people adequately from the health hazards attributable to radiation exposure. However, it is noted that a comprehensive approach that takes account of both radiation and other hazards in a coherent and consistent manner is currently missing in international guidance. (a) It was recognized that decisions on remediating areas contaminated with artificial radionuclides are usually different from those for areas affected by naturally occurring radionuclides even though the ‘natural’ doses to exposed persons might be the same and, in some cases, many times higher than the ‘artificial’ doses. The international system does not differentiate between the health hazards of natural and those due to artificial radiation. A dichotomous approach for remediating artificially versus naturally contaminated land is therefore scientifically unjustifiable. Nevertheless, such separate approaches are used in practice, perhaps due to a perceived public reluctance to remediate areas in which enhanced radiation levels occur naturally; 74 SUMMARY OF SESSION 3 (b) The public should be involved in decisions on remediation - but when, and to what extent, may vary. In some countries, the public is more empowered than in others and in those countries it will insist on having its views heard at all stages of the remediation process. The time available did not allow the Panel to address all of the questions arising from the Arlington conference. 75 INNOVATIVE TECHNOLOGIES IN ENVIRONMENTAL REMEDIATION (TOPICAL SESSION 4) Chairperson V. ADAMS United States of America INNOVATIVE MATHEMATICAL MODELLING IN ENVIRONMENTAL REMEDIATION G.T. YEH*, J.P. GWO**, M.D. SIEGEL***, M. H. LI****, Y.L. FANG*****, F. ZHANG******, W.S. LUO******, S.B. YABUSAKI***** * ** *** **** ***** University of Central Florida, United States of America Nuclear Regulatory Commission, United States of America Sandia National Laboratories, United States of America National Central University, Taiwan, China Pacific Northwest National Laboratory, United States of America ****** Oak Ridge National Laboratory, United States of America Abstract Subsurface contamination problems of radionuclides, metals, and organic co-contaminants are ubiquitous. These contaminants may exist in the solute phase or may be bound to soil particles and interstitial portions of the geologic matrix. Innovative tools to reliably predict the migration and transformation of these radionuclides, metals, and co-contaminants in the subsurface environment enhance the ability of environmental scientists, engineers and decision makers to evaluate the efficacy of alternative remediation techniques and to analyze their impact prior to incurring expense in the field. A realistic mechanistically-based numerical model that considers feedback between fluid flow, thermal transport, and reactive transport could provide such a tool. This paper communicates the development and applications of a mechanistically coupled fluid-flow, thermal-transport, hydrologic-transport, and reactive biogeochemical model where both fast and slow reactions occur in porous and fractured media. Four example problems are employed to demonstrate how numerical experimentation can be used to evaluate the feasibility of different remediation approaches. 1. INTRODUCTION Groundwater has always played an important role in human history and groundwater contamination has been subject to intensive investigations since the mid-1980s. Contaminants in the water environment undergo changes in concentration resulting from physical, chemical, and/or biological processes, and a capability to understand and model these processes is at the core of water-quality management. Accurate tools for the reliable prediction of contaminant migration and transformation are necessary to support the task. Consideration of equilibrium chemistry, kinetic chemistry, and hydrologic transport and the interaction between fluid flow and reactive transport is necessary in order to reflect the complexity of the many systems. For example, solid phase reactions including precipitation and dissolution can potentially plug pores or open fractures reducing matrix diffusion and promote rapid flow through fractures. The development of mechanistically-based reactive chemical transport models has increased dramatically in the last two decades [1-8]. These numerical reactive transport models have had varied scopes. This paper describes the development and application of the latest versions of HYDROGEOCHEM [7], a mechanistically-based numerical model for the simulation of coupled fluid flow, thermal transport, and reactive chemical transport in variably saturated porous and fractured media. These latest versions are among the most versatile codes for dealing with biogeochemical processes under variably saturated flow conditions. 79 TOPICAL SESSION 4 2. MATHEMATICAL BASIS The reactive transport equation of any species can be derived based on the conservation law of material mass stating that the rate of mass change is due to biogeochemical reactions and hydrologic transport [7]. This statement would result in M partial/ordinary differential equations (PDEs) involving M species concentrations and N reaction rates. The number of unkowns is (M + N), which is more than the number of PDEs. Thus, N more equations are needed. We will asuume that the N reactions are made of NE equilibrium and NK kinetic reactions. For each of the NK kinetic reactions, its rate is explicitly formulated based on experimental evidence. For each of the NE equlibrium reactions, its rate is implicitely defined with an algebraic equation, for example, a mass action equation. The substitution of explicit rate equations for kinetic reactions into the system of PDEs results in (M + NE) unknowns in M PDEs. This coupled with NE algebraic equations of thermodynamic realationships forms a closed system of (M + NE) mixed differential-algebraic equations. Decoupling of the NE unknowns of equilibrium rates from the M unknowns of species concentrations can be made via the Gauss-Jordan reduction of reaction networks [2]. Performing matrix decomposition of the reaction matrix, we obtain two subsets of equations as described below: (1) M-NE transport equations for M-NE reaction extents (1) Ei L Eim Dij f j , i M N E in which Ei t jN K aC jM ij j where Ei is the i-th reaction extent [M/L3]; L is the hydrologic transport operator; Eim is the portion of Ei, which contains the linear combination of only mobile species; is the moisture content [L3/L3]; {NK} = {1,2,..,NK}; fj = fj(Ci:i{M}) is an explicit function of M Ci’s that represents the rate equation of the j-th reaction; Dij is an element of decomposed reaction matrix; {M-NE}{M} having (M-NE) members is a subset of {M} where {M} = {1,2,..M}; and aij is the element of a M x M matrix resulting from the matrix decomposition of a unit matrix and it represents the coefficient of the linear combination of Cj in Ei. (2) NE rate-equations for NE fast/equilibrium reactions Dik Rk Ei L Eim Dij f j , k N E , i M E t jN k (2) where Dik is an element of decomposed reaction matrix corresponding to an independent equilibrium reaction; Ei, the i-th reaction extent, is called an equilibrium variable since it corresponds to an independent equilibrium reaction; {NE} = {1, 2, .., NE}; and {ME}, having ME (=M-NE) members, is a subset of {M}. The (M - NE) PDEs in Equation (1) are coupled with NE non-linear algebraic equations, Fk Ci : i {M } 0, e. g. kE Ci ik / Ci iM iM ik 0, k N E (3) which implicitely define the rates of NE equilibrium reactions, to form a system of M equations for the unknowns of M species concentrations, Ci’s. In Equation (3), kE is the modified equilibrium constant of the k-th equilibrium reaction and ik and ik, respectively, 80 YEH et al. are the reaction stoichiometries of the i-th species in the k-th reaction associated with reactants and products, respectively. 3. EXAMPLE PROBLEMS Example 1: This problem considers the release and migration of uranium from a simplified uranium mill tailings pile. The mill tailings pile was located adjacent to a surface that slopes down to a river. The problem consisted of a reaction network of 35 aqueous complexation and 14 precipitation-dissolution reactions involving 56 species [6]. Diagonalization of the reaction network resulted in seven major chemical components: calcium, carbonate, uranium, phosphate, sulphate, proton, and ferrous [6]. Simulation results on the migration of uranium and other chemical species over 300 days were reported in Yeh et al. [7]. The same 56-species uranium tailing problem was applied to a proposed waste disposal site at Melton Branch Watershed. The parallel version of the code was employed and computations were distributed over a number of processors to speed-up the computations. Migrations of uranium, proton, carbon, and iron are given elsewhere [9]. Example 2: This problem simulated Monitored Natural Attenuation (MNA). In addition to the processes of the previous problem, adsorption-desorption processes were also included. The objectives were to conduct a parametric study of adsorption-desorption of uranium. Different sorption mechanisms, including fast (or reversible), slow, and irreversible sorption, were simulated. Three cases were studied: equilibrium sorption, kinetic-limited sorption with slow uptake, and rapid adsorption with slow desorption. For Case 1 – fast adsorption only, four equlibrium reactions were included. For Case 2 – mixed fast and slow adsorption, two more equlibrium reactions and one reversible kinetic reaction were included. For Case 3 – mixed reversible and irreversible reactions, the slow kinetic reaction was considered partially irreversible. Simulation results indicated that (1) a dissolved uranium plume moves faster when sorption processes are not included, (2) the amount of sorbed uranium on the fast site is higher than on the mixed site, (3) since less uranium is sorbed on to the mixed site, the intensity of the dissolved uranium plume is lower than at the fast site during the desorbing period, (4) the separation and alteration of the mass centre of the dissolved uranium plume is the effect of non-linear sorption/desorption reactions, (5) during the sorbing period, the irreversible site can provide almost the same sorption ability as the reversible site, (6) during the desorbing period, the irreversible site partially confines the migration of uranium, and (7) the complete removal of adsorbed uranium from the irreversible site requires more time to achieve than at the reversible site. Example 3: This example investigated laboratory experiments involving extremely high concentrations of uranium, technetium, aluminium, nitrate, and toxic metals [10]. The experiment was modeled with a reaction network of 92 equilibrium and 5 kinetic reactions involving 138 chemical species. The conceptual model involving 12 chemical components was proposed for the experiments: nitrate, Na, K, Al, Si, sulphate, Ca, Mg, Mn, U, Co, and Ni [10]. An equilibrium reaction model that considers 72 aqueous complexation reactions was first used to perform the speciation calculation for each data point to determine the concentrations of individual species given the pH and the total aqueous concentrations of nitrate, Na, K, Al, Si, sulphate, Ca, Mg, Mn, U, Co, Ni, and Cl. Based on the calculated aqueous species concentrations, the saturation index was calculated for each of the 26 minerals considered and a decision was made to include only five precipitation-dissolution reactions. Finally, soil buffering capacity was modeled with six ionization reactions of a polyprotic acid (H4X) and a polyprotic base (Y(OH)2). Simulation results indicated good agreements between experiments and theoretical predictions using the proposed reaction network. 81 TOPICAL SESSION 4 Example 4: This example modeled bioremediation field experiments conducted at a Uranium Mill Tailings Remedial Action (UMTRA) site using acetate amendment to stimulate microbially mediated immobilization of uranium in the unconfined aquifer. Experiments at the Rifle site showed that the growth of acetate-oxidizing Fe(III)-reducers dominated by Geobacter sp., was accompanied by significant uranium removal from groundwater. An important feature of these field experiments was the eventual onset of sulphate reduction, which was characterized by a decrease in aqueous sulphate, near complete consumption of acetate, and less efficient U(VI) removal from groundwater. A key observation from field experiments at the Rifle site was that longer-term, post-biostimulation U(VI) removal from groundwater was associated with longer periods of sulphate reduction. This led to the inclusion of abiotic chemistry for the bioreduced U(IV), Fe(II), and sulphide products of the principal terminal electron accepting processes (TEAPs), to address their potential roles in long term uranium immobilization. The conceptual model was developed to facilitate understanding of the principal processes and properties controlling uranium biogeochemistry. The model included four TEAPs involving two pools of bioavailable Fe(III) minerals (phyllosilicate, oxide), aqueous U(VI), and aqueous sulphate, two distinct functional microbial populations (iron, sulphate reducers), as well as aqueous and surface complexation and mineral precipitation and dissolution. The model assumes 1) co-metabolic uranium bioreduction via active iron reducers, 2) the onset of sulphate reduction is controlled by a bioavailable Fe(III) threshold, 3) iron, sulphate, and uranium TEAPs occur simultaneously during sulphate reduction, and 4) there is no abiotic U(VI) reduction. The conceptual model reflects findings from laboratory studies that during biostimulation, 90-99% of the Fe(III) initially reduced is in the phyllosilicate clays [11] and biogenic Fe(II) resulting from phyllosilicate iron reduction generally remains in the layer silicate structure. Simulated and measured breakthrough at several locations down-gradient of the injection gallery show good agreement. ACKNOWLEDGEMENTS The work is supported in part by the US Department of Energy under Grant DE-FG0204ER63916 with University of Central Florida. REFERENCES [1] [2] [3] [4] [5] 82 BACON, D.H., WHITE, M.D., MCGRAIL, B.P., Subsurface Transport Over Reactive Multiphases (STORM): A General, Coupled, Nonisothermal Multiphase Flow, Reactive Transport, and Porous Medium Alternation Simulator, Version 2, PNNL-13108, Pacific Northwest national Laboratory, Richland, WA 9935 (2000). FANG, Y., YEH, G.T., BURGOS, W.D., A Generic Paradigm to Model Reaction-Based Biogeochemical Processes in Batch Systems. Water Resources Research 33 4 (2003) 10831118. LICHTNER, P.C., Continuum formulation of multicomponent-multiphase reactive transport, In: Lichtner, P.C., Steefel, C.I. and Oelkers, E.H. (Eds), Review in Mineralogy. Chapter 1, In: Reactive Transport in Porous Media. Mineralogical Society of America, Washington, D. C. (1996). PRUESS, K., TOUGH2: A General Purpose Numerical Simulator for Multiphase Fluid and Heat Flow, Lawrence Berkeley Laboratory Report LBL-29400, Berkeley, CA (1991). STEEFEL, C.I., YABUSAKI, S.B., OS3D/GIMRT, Software for MulticomponentMultidimensional Reactive Transport: User’s Manual and Programmer’s Guide, PNL-11166, Pacific Northwest National Laboratory, Richland, WA 99352 (1996). YEH et al. [6] YEH, G.T., TRIPATHI, V.S., HYDROGEOCHEM: A Coupled Model of HYDROlogical Transport and GEOCHEMical Equilibrium of Multi component Systems, ORNL 6371, Oak Ridge National Laboratory, Oak Ridge, TN. 37831 (1990). [7] YEH, G.T., SUN, J.T., JARDINE, P.M. et al., HYDROGEOCHEM 5.0: A Three Dimensional Model of Coupled Fluid Flow, Thermal Transport, and HYDROGEOCHEMical Transport through Variably Saturated Conditions Version 5.0. ORNL/TM-2004/107, Oak Ridge National Laboratory, Oak Ridge, TN 37831 (2004). [8] ZYVOLOSKI, G.A., ROBINSON, B.A., DASH, Z.V., et al., Models and methods Summary for the FEHM Application. FEHM MMS SC-194. Los Alamos National Laboratory, Los Alamos, New Mexico (1994). [9] http://www.csm.ornl.gov/~g4p/chapman_1/isosurface.htm [10] ZHANG, F., LUO, W., PARKER, J.C. et al., Geochemical reactions affecting aqueous-solid partitioning metals during titration of uranium contaminated soil. Environmental Science and Technology 42 21 (2008) 8007-8013. [11] KOMLOS J., PEACOCK, A., KUKKADAPU, RK., Long term Dynamics of Uranium Reduction/Reoxidation under Low Sulphate Conditions. Geochimica Et Cosmochimica Acta 72 (2008) 3603-3615. 83 ADVANCES IN THE APPLICATION OF ELECTRICAL TECHNIQUES FOR SITE REMEDIATION D.F. OSBORNE Linkforce Pty Ltd, Mawson Lakes, Australia Abstract Electrical techniques in site remediation have advanced over the past 10-15 years as a result of the experience gained in their application to various types of waste and sites. The main advances have been in the equipment design and construction combined with improvement in the understanding of the vitrification process. An overview is given of the advances together with an account of an application to a particular remediation problem. 1. INTRODUCTION GeoMelt is a technique that has been in commercial use since 1989. It was invented by the Battelle Institute for the United States Department of Energy (DOE) for use in the ‘in situ’ treatment of radioactively contaminated sites. Until recently, the process was used exclusively in a mobile form with the equipment being assembled on site. Now, permanent treatment facilities have been established in which the contaminated soil is brought to the plant for treatment – this is the case at the Japanese Daiei Kankyo facility. The initial design was for fixed electrodes (initially six molybdenum electrodes) to be drilled into the area to be treated. Then electricity was applied to the fixed electrodes to promote the melting process. Over the years, the equipment has been modified with items such as the electrodes being changed - with graphite collars fixed over molybdenum inner rods. Nowadays, commercially available ‘off-the-shelf’ type graphite electrodes are used. The number of electrodes has been reduced to four, and sometimes only two electrodes are used for specific ‘in container’ type melts. The ‘off-gas’ capture hoods were initially made from a heat resistant fabric but after a fire they were replaced by hoods of fabricated stainless steel. These were effective but not easy to assemble. Later, a change to modular type panel hoods was made; this allows ease of assembly and reduces the requirements for lifting equipment on site to move the hoods between melts. Today the technology is used in different configurations (in situ, in container, staged and planar (starting the melts subsurface)) and the basic technology has become a very flexible and adaptable process capable of many different applications. Individual melts have been achieved in excess of 1000 tons in total. 2. PROCESS DESCRIPTION GeoMelt vitrification uses graphite electrodes to supply alternating current from a GeoMelt transformer through the electrodes and into the contaminated soil or waste being treated. Gases generated by the vitrification process are captured in a hood covering the treatment area and drawn through an ‘off-gas’ treatment system before being released to the atmosphere. The temperatures reached in the process can be as high as 2000º C. Organic materials in the soil are destroyed and heavy metals and radionuclides are incorporated into the vitrified product and immobilized. 85 TOPICAL SESSION 4 Substantial volume reduction is achieved, usually a minimum of 50% and, depending on the contents of the soil/waste mixture, the volume reduction can be as high as 75-80%. Soil is the normal medium to which the technique is applied, but when it is applied to materials containing high levels of asbestos or fly ash, little or no soil is required in the melting process. The off-gas treatment system used is varied depending on the waste being treated and the regulatory requirements applicable to the project. Usually, the configuration consists of a pre- or roughing filter, a thermal oxidiser (if required), a scrubber and mist eliminator, a heater and high efficiency particulate air (HEPA) and/or carbon filters. Specific additional requirements can be added if materials containing mercury and arsenic, for instance, are encountered. Electrodes In Situ Contaminated Soil Hood Melt Hood diagram in half for clarity of process In-Situ Process Configuration Treatment Cell Boundary Staged Soil and Wastes Staged in Cell Process Configuration In-Container Process Configuration FIG. 1. Diagrams of the GeoMelt process application. 86 OSBORNE 3. APPLICATIONS GeoMelt has been applied to many varying types of waste containing organic and heavy metal contaminants or combinations of radionuclides and mixed waste. Summary tables (Tables 1 and 2) show previously treated waste types and radionuclides. TABLE 1. SUMMARY OF SOME MATERIALS PREVIOUSLY TREATED Heavy metals Pb As Cd Cr Ni Ba Zn Hg Cu Al Fe Nd Rb Liquid organics PCBs Dioxins Furans TCE PCE Benzene Toluene Acetone Formaldehyde Methylene chloride Ethylene glycol MEK Carbon tetrachloride Solid organics Wood Rubber Asphalt PVC Polyethylene Neoprene Paper Cotton Polypropylene DDT,DDD,DDE TBT,RDX,HMX Hexachlorobenzene Ion exchange resins Solid debris Concrete Steel plates Structural steel Tires Drums Rocks Bricks Clay pipe Glass bottles Ash Tanks The materials in Table 1 have been treated either as part of an overall waste stream or individually, e.g. with items such as Hexachlorobenzene or ion exchange resins. TABLE 2. EXAMPLES OF RADIONUCLIDES TREATED Am-241 Ag-110m Cs-134 Cs-137 Co-57 Co-58 Co-60 Eu-152 Eu-154 Eu-155 Mn-54 Ni-59 Pu-238 Pu-239 Pu-240 Ru-106 Sr-90 Sb-125 Tc-99 U-234 U-237 U-238 Zn-65 Zr-95 87 TOPICAL SESSION 4 4. PROJECT EXAMPLE The rehabilitation of the Maralinga nuclear test site is representative of contaminated soil remediation at a large scale and in a remote location. The traditional in-situ technique was applied; this allowed the greatest sized batch to be achieved. Control Room & GeoMelt Transformer Offgas System HV Generators GeoMelt Hoods Completed Melt Maralinga Rehabilitation Project – remote South Australia FIG. 2. Layout of application at the Maralinga site (Taranaki burial pits). The Maralinga site is a former nuclear weapons test range in South Australia used by the British Government in the 1950s and 1960s for above-ground nuclear testing. Several hundred experiments involving conventional explosives resulted in plutonium (Pu), uranium (U), and beryllium (Be) being dispersed in the environment. At the Taranaki area of Maralinga, 12 minor tests were performed that involved the explosive dispersal of 22 kg of Pu, resulting in large amounts of contaminated debris and soil that were placed in burial pits. The Taranaki pits were typically excavated by blasting in the native limestone. Several years later, concrete caps were placed on tops of the pits. The Cleanup of the Taranaki burial pits was part of the Maralinga Rehabilitation Programme managed by the Commonwealth of Australia. In 1989, GeoMelt was identified as the preferred technology for remediating the burial pits in a cooperative British/Australian study by the Maralinga Technical Assessment Group. Confirmatory testing and radioactive demonstrations were performed before dedicated equipment was designed and manufactured for remediating the pits. The pits were believed to contain ~2 to 4 kg of Pu; a similar amount of U; various metals including lead (Pb), barium (Ba), and beryllium (Be); and large amounts of debris (e.g. massive steel plates, steel beams, lead bricks, barytes shielding bricks, cable, and organic-based materials). A mound of silica sand was placed over each pit, and the GeoMelt equipment was positioned for treatment. The sand provided a level and uncontaminated base for workers to prepare the system. Melting was initiated in the sand layer. The sand augmented the melt chemistry by providing more glass-forming ions, which improved the chemical and physical characteristics of the vitrified product. 88 OSBORNE This project was completed in 1999 and achieved its primary objective of converting the loose, friable, radioactive contamination in the pits into dense, hard, intrusion-resistant vitrified masses, eliminating the long term hazards of subsidence or human intrusion. The resulting vitrified monoliths of each pit were intrusively sampled and examined to characterize the vitrified product and confirm the completeness of treatment. Specific project results are as follows: – No partitioning or elevated concentrations of Pu were found in any of the monoliths; – There was no indication that Pu was present in the melted steel phase, when such a phase was present at the base of the vitrified monoliths; – Pu retention in the melts was >99.99%, which minimized the level of equipment contamination and the radiological hazard to workers. The hoods and off-gas piping did not require decontamination after any one melt; – Samples of vitrified product from two of the full-scale melts were subjected to the Product Consistency Test (PCT). The normalized release rates for the major oxides from the 28-day tests were substantially <1 g/m2.day, with most release rates <0.1 g/m2.day. Long term leach rate measurements (4.5 years) established that the normalized leach rates decline with time. The normalized leach rate for Pu decreased by over 1000 times during the leaching period, demonstrating that the vitrified product has outstanding leach resistance. Vitrified Block – note electrode’s embedded into the vitrified product. FIG. 3. Vitrified monolith of what was previously a burial pit. The costs associated with traditional methods of containing waste such as uranium mine tailings are initially less than those of the GeoMelt process, but the ongoing costs of maintenance, dewatering, monitoring and repair/replacement of the containment media are substantially more than a permanent solution such as vitrification. 89 TOPICAL SESSION 4 Cost Permanent Solutions Traditional Containment Methods Time Construction/Treatment Phase Ongoing Maintenance Phase FIG. 4. Comparison of costs of remediation solutions. 5. SUMMARY Advances made in the GeoMelt process of electric vitrification since its initial commercialization in 1989 have greatly increased its capability and flexibility. Projects such as that at Maralinga clearly show that the GeoMelt process of vitrification can be used for radioactively contaminated soil sites, such as mine tailings. 90 SITE REMEDIATION IN PRACTICE A. VÁRHEGYI, G. FÖLDING, Z. BERTA , M. CSÖVÁRI MECSEK-ÖKÓ Zrt, Pécs, Hungary Abstract This paper describes the remediation of a former uranium mining area in Hungary. The work was carried out using stringent quality controls and special attention was paid to the radiological survey during the cleanup works on the roads, on pipe lines and yards, on the mill site and places used earlier for heap leaching. Groundwater quality control and the related groundwater quality restoration were the most important aspects of the post remediation phase which was aimed at the long term protection of the nearby drinking water aquifer. The expenditure for the remediation was about 100 million US dollars. The estimated cost for long term monitoring and water treatment is about 4 million US dollars/year. 1. INTRODUCTION Uranium mining and processing were developed in the southern part of the country in the Mecsek Hills, near to the county town of Pecs. The uranium mining activity lasted from 1958 to 1997. Approximately 47 million tonnes of rock were mined from 5 shafts and 19 million tonnes of ore were processed using acid leaching. Approximately 7.2 million tonnes of low-grade ore were heap leached by an alkaline process. The uranium mining and processing was terminated in 1997 because of the high production cost. Remediation of the site started immediately after the termination of the production and was practically finished by 2008. The mine ore, after radiometric sorting, was divided into three grade-groups according to its uranium content: – Waste rock (U < 100 g/t), dumped into three major waste rock piles (WP1, WP2 and WP3) and 6 smaller piles; – Low grade ore (processed by alkaline heap leaching); – Upgraded ore (processed in the mill using sulphuric acid leaching). Elaboration of the remediation plan for the waste rock piles (WPs), heap leaching residues, mill tailings, etc. started with the estimation of the quantity and quality of waste, the composition of the seepage from the waste rock piles, the expected mine water composition and groundwater contamination in the immediate vicinity of the WPs. Based on preliminary site investigations and appropriate laboratory studies, field trials and feasibility studies, the general remediation plan was compiled. The overall plan comprised 10 sub-projects according to the type of work to be carried out. In the separate sub-projects, the main technical data and schedules regarding the planned work were determined together with the arrangements for quality assurance. The expenditure for the remediation was provided from the State budget. During the remediation operations, particular attention was paid to the protection of the groundwater quality. 2. CHARACTERIZATION OF WASTE Some important data for the characterization of solid waste are presented in Table 1. It can be seen that the uranium content and other radiological characteristics of the waste are much higher than those due to the naturally occurring radionuclides in the region; therefore the waste had to be remediated. First of all, it had to be covered with non-radioactive earth to 91 TOPICAL SESSION 4 isolate it from the possible direct contact with humans and to reduce further pollution of the environment. The composition of the liquid waste is summarized in Table 2. The waters can be divided into two main groups: – Waters with elevated uranium concentration (mine water, seepage from the waste rock piles); – Groundwater with elevated dissolved solids (TDS) in the vicinity of the tailings ponds (TPs). Remediation measures included water treatment for removing the uranium and quality restoration for groundwater in the vicinity of the tailings ponds. The groundwater restoration was a task of great importance because the water aquifer is situated almost in the immediate vicinity of the tailings ponds. TABLE 1. CHARACTERIZATION OF THE ORIGINAL SOLID WASTE Type of waste Volume (million tonne) Uranium content (g/t) Gamma-dose rate (mGy/h) 50 65 Radium concentration (Bq/g) ~0.6 ~1.2 Waste rocks Heap leaching residues Mill tailings Background in the region 19.2 7.2 20.3 68 ~4-10 ~12 ~5*10-2 3-8* ~0.1-0.2 ~0.5 ~1 * Depending on the tailings pond area selected. TABLE 2. COMPOSITION OF THE LIQUID WASTE Type of water U TDS pH Na Ca Mg SO4 Cl Ra (mg/L) (mg/L) (mg/L) (mg/L) (mg/L) (mg/L) (mg/L) (Bq/L) 8 1600 7.1 260 205 140 890 120 0.7 Mine water* (Shaft N1 2001) Contaminated 0.7 groundwater in the vicinity of WP (2001) Contaminated 0.02 groundwater in the vicinity of tailings pond (1998) 1250 7.3 160 320 160 390 60 0.02 14 700 7.2 740 490 1580 6680 1500 0.06 * Including collected seepage from waste rock piles. 3. SITE REMEDIATION AND MONITORING 3.1. Preliminary investigations To determine the appropriate remediation measures it was necessary to carry out preliminary investigations. It was considered that the determination of the water contamination (groundwater and run-off waters) on and around the sites had highest priority. For screening, e.g. on the tailings ponds site, a geophysical multi-electrode survey was used 92 VÁRHEGYI et al. (Fig. 1). This measurement provided valuable information on the electric conductivity of the soil, and consequently on the contamination of the groundwater with inorganic compounds originating from the tailings water. This method proved to be very useful for determining the extent of the contaminated area and the depth penetration of the inorganic contaminants from the tailings ponds. Low resistive zones around the tailings ponds were found not only in the shallow zones but also in deeper zones because of the penetration of highly contaminated tailings water into these zones. For the estimation of the amount of the contaminants in the groundwater, data from the material balance of the mill process was used. Taking into account the amount of the consumed acid (sulphuric acid for leaching, hydrochloric acid for the ion exchange process) and the amount of the neutralizing agents (lime, dolomite of the processed ore, etc.) and some other data, the loading of the tailings ponds with dissolved solids during the mill process was calculated. On the basis of these data, the concentration of the total dissolved solids in process water was estimated for the full period of the ore processing. The data are presented in Fig. 2. These data show that on average the total dissolved solids in water was about 20 g/L and in total about 700 thousand tonnes of dissolved compounds (mainly MgSO4, and NaCl) have been discharged into the tailings ponds. The dispersion of these dissolved solids around the tailings ponds was detected by means of the geoelectric survey. 3.2. Environmental monitoring The environmental monitoring consisted of radiological, hydrological, geochemical, geotechnical, and geophysical monitoring, as presented in Fig. 3. 93 TOPICAL SESSION 4 FIG. 1. Geophysical multi-electrode profiling of the tailings ponds site. TDS TDS in discharged tailings water 40 35 30 25 20 15 10 5 0 FIG. 2. TDS in process water discharged into the tailings ponds. Radiological monitoring was essential during the cleanup of different areas (yards, pipeline areas, roads, heap leaching sites, the mill site etc.) Yearin order to meet the cleanup standards. In practice, the excavation of the contaminated soil was carried out at the same time as gamma-dose rate monitoring and the measurement of the specific activity of the soil. The cleanup procedure was continued until the relevant standards were met. The radiological monitoring was important also for the estimation of the equivalent radiation dose to the population living in the vicinity of the remediated areas; this work was carried out using an automatic monitoring station placed in the village. Hydrological monitoring was essential for protecting the surface and ground water quality. The results were used for the cleanup of the contaminated sites, the planning of ground water restoration systems etc. The monitoring provided input data for the integrated water management of the former uranium mining and ore processing site, allowing the controlled discharge of all kinds of waters from the former uranium-mining site through one 94 TD TD VÁRHEGYI et al. common discharge basin. There were 612 sampling points in 2007 from which 1472 samples were collected and analyzed for radio-elements and other components. Environmental Monitoring System Soil Water Radiology Radiology (U, Ra, Th, dose) Hydrology (Chemical pollution:CH, acid, trace elements) Geotechnic (soil mechanics, erosion) (U, Ra) Hydrology Air Biosphere Radiology Radiology Radio activity of the aerosol, (Chemical pollution: fallout, Inorganic, CH, Radon progeny (radio-elements in vegetation) Human dosimetry, and (labour hygiene) Trace elements, Water level and volume) Geophysics (soil movement, geoelectric probing ) FIG. 3. Scheme of the environmental monitoring system. 3.3. Basic methods of radiological and hydrological monitoring – In situ measurements and investigations (ambient gamma dose rate, 222Rn, short-lived radioactive aerosols etc., pH, Eh, electrical conductivity, etc.); – Sampling and laboratory analyses of samples (soil, plant, aerosol, fall-out, specific activity, gamma-spectrometry, U, Ra concentrations in water, chemical composition, etc.); – Automatic monitoring stations (dose components, different water parameters). 4. WATER TREATMENT An inevitable part of the remediation is water treatment. This consists of the treatment of the mine water to remove the uranium (in the form of commercial concentrate) and the 95 TOPICAL SESSION 4 treatment of the extracted groundwater to reduce the total dissolved solids in the discharged water. The methods used are described in some earlier publications (1-3). REFERENCES [1] [2] [3] 96 INTERNATIONAL ATOMIC ENERGY AGENCY , Treatment of liquid effluents from uranium mines and mills during and after operation. Report of a co-ordinated research project 1996-2000, IAEA-TECDOC-1419, Vienna (2004). BÁNIK, J., et al., Water treatment issues at a former uranium mining site, In: Uranium Production and Raw Materials for the Nuclear Fuel Cycle - Supply and Demand, Economics, the Environment and Energy Security, Proceedings of an International Symposium held in Vienna, 20–24 June 2005, 277-285, International Atomic Energy Agency, Vienna (2006). FÖLDING, G., et al., Post-closure water management practice on the former uranium mining site in Hungary, Proceedings of the 10th IMWA Congress 2008, Ed. Nada Rapantova, Published by VSB –Technical University of Ostrava (2008). MONITORED NATURAL ATTENTUATION OF METALS AND RADIONUCLIDES IN SOIL AND GROUNDWATER M. DENHAM, K. VANGELAS Savannah River National Laboratory, Aiken, South Carolina, United States of America Abstract Natural attenuation processes, which include a variety of physical, chemical, or biological processes, can work to bring about the remediation of a contaminated site. Monitored natural attenuation (MNA) is a remediation approach which relies on these processes. The United States Environmental Protection IAEA has established a four-tier system for demonstrating that MNA is a viable solution for metal and radionuclide contaminated sites. To meet the criteria specified by this guidance requires a fundamental understanding of how geochemical conditions will change in the future. The United States Department of Energy has funded an applied research initiative led by the Savannah River National Laboratory aimed at increasing the understanding of the geochemical evolution of sites in the context of remediation. This paper describes the relevant regulatory framework and the use of geochemical gradients established by plumes as a framework for understanding waste site evolution. 1. INTRODUCTION Although it has been ten years since Monitored Natural Attenuation (MNA) first became recognized as a viable remedy for groundwater remediation, there are relatively few records of decisions involving MNA being implemented for sites with metal or radionuclide contaminants. In the past, remediation has primarily consisted of attempts to remove contaminants from the subsurface by excavation or ‘pump-and-treat’ systems. Increasingly these approaches have come to be seen as inefficient and ‘in situ’ immobilization of contaminants is now the favoured remedy at most sites. Whether explicitly stated or not, ‘in situ’ remedies must ultimately rely on natural attenuation processes to keep contaminants immobile; this is, in fact, the desired end-state of MNA. A common misconception is that invoking Monitored Natural Attenuation after active remediation is a means of abandoning the site without further obligation. To the contrary, the use of MNA in a remediation strategy requires a long term commitment to the site and can be a complicated process. Unlike organic contaminants that degrade, metals and radionuclides can persist in the subsurface indefinitely. The exceptions are radionuclides with short halflives. However, uranium isotopes, plutonium isotopes, 99Tc, 129I, and many of the actinides present at United States Department of Energy (USDOE) sites persist for thousands to millions of years. The continued presence of these in the subsurface following active ‘in situ’ remediation requires site owners to prove, to the satisfaction of regulators and stakeholders, that the contaminants will not be a threat to human health and the environment over long time periods. Three initiatives in the United States are directed toward facilitating the use of Monitored Natural Attenuation in the context of metal and radionuclide contamination. The United States Environmental Protection IAEA (USEPA) has issued two guidance documents describing the level of proof expected for demonstrating that MNA will be effective and the specific technical aspects that should be considered for selected metals [1, 2]. Forthcoming documents from the USEPA are: a volume pertaining to MNA for selected radionuclides and an official policy statement on the use of MNA for inorganic contaminants. The Interstate Technology and Regulatory Council (ITRC) has convened a team to provide a framework for site owners, regulators, and stakeholders to evaluate MNA as an option for metal and 97 TOPICAL SESSION 4 radionuclide contaminated sites. The third initiative, funded by the USDOE and led by the Savannah River National Laboratory (SRNL), is focused on developing approaches, tools, and guidance that will facilitate achieving the required monitored natural attenuation endpoint for metal and radionuclide contaminated sites. 2. REGULATORY HISTORY OF MONITORED NATURAL ATTENUATION IN THE UNITED STATES Natural attenuation strategies have been incorporated into environmental regulations and technical guidance since the early 1990s. The early guidance involved the attenuation of petroleum hydrocarbons; this was followed by guidance on chlorinated volatile organic contaminants (CVOCs), and, most recently, guidance on metals and radionuclides. From a technical perspective, the development of technical guidance has followed a logical progression from contaminants most amenable to destruction by robust and simple mechanisms to those that are not destroyed or for which destruction only occurs on the order of geologic timeframes. Many organizations have produced technical guidance related to the natural attenuation of petroleum hydrocarbons and CVOCs. In the United States, the policy document that all natural attenuation based guidance documents are based upon is the USEPA Office of Solid Waste and Emergency Response (OSWER) Directive No. 9200.4-17P, titled ‘Use of Monitored Natural Attenuation at Superfund, RCRA Corrective Action, and Underground Storage Tank Sites’ [3]. This document lays out the groundwork for all MNA remedies. It defines MNA as: “the reliance on natural attenuation processes (within the context of a carefully controlled and monitored site cleanup approach) to achieve site-specific remediation objectives within a time frame that is reasonable compared to that offered by other more active methods. The ‘natural attenuation processes’ that are at work in such a remediation approach include a variety of physical, chemical, or biological processes that, under favourable conditions, act without human intervention to reduce the mass, toxicity, mobility, volume, or concentration of contaminants in soils or groundwater. These ‘in situ’ processes include biodegradation, dispersion, dilution, sorption, volatilization, radioactive decay, and chemical or biological stabilization, transformation, or destruction of contaminants.” Regarding inorganics (metals and radionuclides), USEPA [3] states that: “natural attenuation of inorganic contaminants is most applicable to sites where immobilization or radioactive decay is demonstrated to be in effect and the process/mechanism is irreversible.” The Directive also provides guidance in terms of specific objectives that need to be considered for implementation of MNA. The USEPA has subsequently issued two volumes that provide guidance for the implementation of MNA for inorganic contaminated sites http://www.epa.gov/ada/pubs/reports.html): Volume 1 outlines the regulatory aspects of Metals/Radionuclides MNA and then describes a tiered approach for implementation and the use of modelling in the tiered screening process. After describing the chemical and microbiological controls over the fate of inorganic contaminants, Volume 1 reviews general site characterization requirements for Metals/Radionuclide MNA. 98 DENHAM, VANGELAS Volume 2 discusses the contaminant-specific factors affecting the MNA of Arsenic, Cadmium, Chromium, Copper, Lead, Mercury, Nickel, Nitrate, Perchlorate, Selenium, and Zinc. Chapters are devoted to each of these and contain sections on Occurrence and Distribution, Geochemistry and Attenuation Processes, Site Characterization, Long term Capacity, and the application of Tiered Analysis for the particular contaminant. A third volume on the MNA of radionuclides, including isotopes of Americium, Caesium, Iodine, Plutonium, Radium, Radon, Strontium, Technetium, Thorium, and Uranium, as well as Tritium, is in preparation. The first three tiers in the approach for evaluating a site for MNA are progressive layers of evidence that contaminants will not pose a future threat [1]. If the criteria of the first tier are not met, MNA is not a viable option and the site owner can avoid the more complicated and expensive analyses required in Tier 2. Likewise, the site owner would only advance to collecting the additional data required for Tier 3, if the criteria of Tier 2 are met. The fourth tier is the design of a long term monitoring system and a contingency plan in the event that MNA fails. The ITRC team on ‘Attenuation Processes of Metals and Radionuclides’ is currently developing a framework and flowchart, based on the USEPA four-tiered approach, to guide users through the process of evaluating MNA for metal and radionuclide contamination. 3. THE USDOE APPLIED SCIENCE INITIATIVE The USDOE applied science initiative is focused on improving understanding of the geochemical evolution of waste sites contaminated with metals and radionuclides and its use to increase the efficiency of remediation at these sites. It is fostering an approach to remediation that begins with the recognition that the desired end-state of ‘in situ’ remediation of metals and radionuclides is MNA. The approach encourages the idea that the characterization of a site and the selection of a remedy should be consistent with the geochemical evolution of the site. If a site meets all of the criteria up to and including Tier 3 of the USEPA approach for evaluating sites for MNA, then it has been sufficiently demonstrated that contaminants are unlikely to be significantly remobilized in the future. To achieve this requires a fundamental understanding of the future geochemical evolution of the site, since, with the exception of radioactive decay, all other mechanisms of attenuation and enhanced mobility are highly dependent on geochemical conditions within the aquifer. To predict attenuation in the future is complicated because the factors controlling attenuation evolve with time. A contaminant plume is a transient perturbation of natural subsurface conditions that can change the chemistry, mineralogy, and microbiology within the aquifer as the plume migrates. Over time, as the contamination source is depleted or contained, the plume will eventually migrate to an exposure point or dissipate and background uncontaminated groundwater will migrate through the zone traversed by the plume. The result of this sequence will be the long term evolution of the chemical, mineralogical, and microbiological conditions within the affected portion of the aquifer. As these overall biogeochemical conditions evolve, attenuation processes of any contaminant metals and radionuclides will change in rate and magnitude. Thus, the long term prediction of whether natural attenuation processes can limit contaminant concentrations to below regulatory standards at exposure points requires an understanding of the overall biogeochemical evolution of the waste site. One organizing principle to simplify the understanding of the overall biogeochemical evolution of waste sites is that the most dynamic changes in contaminant attenuation occur at biogeochemical gradients induced by the plume. Fig. 1 shows a cartoon of a plume emanating from an industrial source at the surface. When the contaminant plume is introduced to the 99 TOPICAL SESSION 4 subsurface, a biogeochemical gradient is created at the leading edge of the plume, at the interface of the contaminant plume and natural groundwater. Dilution of the plume, reaction with aquifer minerals, adsorption of plume constituents, desorption of natural constituents, and changes in microbiology can all occur at this gradient. In point of fact, different types of gradients move at different rates, though all are driven by the same hydrodynamic forces. For example, a leading gradient caused by dilution alone moves according to hydrodynamic forces and is unimpeded by chemical reactions. In contrast, a pH gradient is impeded by the buffering reactions associated with aquifer mineral dissolution and adsorption of free protons (H+) to mineral surfaces. Likewise, a leading redox gradient can be impeded by microbiological reactions and reaction with redox sensitive aquifer minerals. FIG. 1. Cartoon showing a leading gradient at the front of a contaminant plume. Trailing gradients form where natural up-flow groundwater meets the infiltrating plume or enters the zone affected by the plume. As long as plume infiltration is relatively constant, the trailing gradient is stationary. Once the plume flux from the vadose zone to the saturated zone is eliminated or substantially reduced, the trailing gradient migrates into and through the plume zone (Fig. 2). Trailing gradients are controlled by hydrodynamic forces, dilution, reaction with plume-altered minerals, and the influx or elimination of nutrients to sustain microbial growth. FIG. 2. Cartoon showing a trailing gradient at the back end of a contaminant plume. Examples of reactions with plume altered minerals are desorption of free protons from plume zone minerals or oxidation of reduced minerals created within the plume zone. One way in which consideration of biogeochemical gradients simplifies the long term prediction of natural attenuation is that, for sites with multiple contaminants, the contaminants can be grouped according to how their migration is controlled. Some contaminants will be controlled only by dilution, some predominantly by pH, and others predominantly by redox conditions. Large changes in contaminant mobility only occur across sharp gradients in these factors. Thus, the attenuation of contaminants is controlled by the migration rates of these gradients. The other way in which consideration of biogeochemical gradients simplifies long term prediction of natural attenuation is that it compartmentalizes characterization and modelling into zones of importance. This is because large changes in mobility only occur across controlling gradients. Characterization and modelling should be focused on the leading and 100 DENHAM, VANGELAS trailing gradients, which are most important in controlling overall contaminant mobility. Consider, for example, an acidic plume with contaminants that are predominantly controlled by adsorption, which in turn is controlled by pH. It is more important to characterize what is present and down flow of the leading pH gradient than what is between the leading and trailing gradient. Likewise, it is more important to understand and model the processes occurring in those parts of the aquifer in the vicinity of the gradients; less emphasis can be given to parts of the aquifer between these gradients. The use of geochemical gradients in the remediation of a waste unit at the Savannah River Site is discussed in reference [4]. At the waste unit site there is an acidic plume containing concentrations of uranium isotopes, 90Sr, and 129I that exceed regulatory limits. A remediation system that is consistent with the evolution of the waste site has replaced a costly ‘pump-and-treat’ system. The pH of groundwater passing through the gates of a hybrid funnel-and-gate system is neutralized, resulting in stronger adsorption of 90Sr and uranium. Essentially, an artificial pH gradient has been installed that accelerates the return of the groundwater to its natural pH of 6; this system will be active until the natural trailing pH gradient reaches the funnel-and-gate. At this point, additional treatment will not be required and the desired end-state of MNA will be achieved. An injectable amendment to immobilize 129I in a way that is consistent with the evolution towards higher pH has been developed by SRNL and field testing is currently cleanup. REFERENCES [1] [2] [3] [4] UNITED STATES ENVIRONMENTAL PROTECTION IAEA, Monitored Natural Attenuation of Inorganic Contaminants in Ground Water Volume 1 - Technical Basis for Assessment, EPA/600/R-07/139 (2007). UNITED STATES ENVIRONMENTAL PROTECTION IAEA, Monitored Natural Attenuation of Inorganic Contaminants in Ground Water Volume 2 - Assessment for Non-Radionuclides including Arsenic, Cadmium, Chromium, Copper, Lead, Nickel, Nitrate, Perchlorate, and Selenium, EPA/600/R-07/140 (2007). UNITED STATES ENVIRONMENTAL PROTECTION IAEA, Use of Monitored Natural Attenuation at Superfund, RCRA Corrective Action, and Underground Storage Tank Sites, Office of Solid Waste and Emergency Response (OSWER) Directive 9200.4-17P (1999). DENHAM, M., VANGELAS, K., Biogeochemical gradients as a framework for understanding waste site evolution, Remediation Journal 19 5-17 (2008). 101 SUMMARY OF SESSION 4 V. Adams United States of America INNOVATIVE TECHNOLOGIES IN ENVIRONMENTAL REMEDIATION This session contained seven presentations concerned with technologies for use in environmental remediation with emphasis on some innovative approaches. The first presentation provided an overview of the science and technology behind the application of cover systems in the remediation of contaminated sites. It was pointed out that no universal solution is available. Moreover, if remediation is not planned in the initial stages of an operation, the available options will decrease and costs will increase significantly. The involvement of stakeholders in the planning process is essential for a successful project. The main factor affecting the long term performance of dry covers is erosion and, because of that, it is critical to observe the potential interactions between vegetation, the cover material, the waste and the associated transport mechanisms (gas and water) in developing an appropriate cover design. This is an area where more guidance could usefully be provided by international organizations to Member States. The use of bioremediation as a technique to remediate contaminated groundwater was reviewed in the second presentation. The remediation of groundwater contaminated by metals and radionuclides involves the conversion of the contaminants into more complex states, sorption, precipitation, or valence state changes at multiple scales. For the successful application of bio-remediation, an integrated approach involving site characterization and monitoring (using hydro-geological, geochemical, geophysical and microbiological methods supported by mathematical modelling) is needed. It has been demonstrated that for the long term remediation of uranium contaminated sites, organic carbon should be supplied naturally to offset continuous influxes of dissolved oxygen. This technique may be the only viable solution for deep and widely dispersed plumes of heavy metals and radionuclides, which are otherwise inaccessible. It can be used for complex mixtures of contaminants provided that appropriate microorganisms are employed. In the third presentation, the technique of Monitored Natural Attenuation was described. The technique is gaining acceptance by regulatory bodies in the context of remediation of contaminated groundwater. It was highlighted that the approach must not be seen as a ‘do nothing option’. On the contrary, justification for the adoption of this strategy depends heavily on appropriate modelling of the fate and transport of pollutants in groundwater. It was pointed out that the forecasting and monitoring strategies need to be discussed with the relevant stakeholders to ensure that the predictions and their limitations are well understood. The strategy is gaining acceptance worldwide because the costs of treating water over long periods of time have been shown to be prohibitively high. The US Environmental Protection IAEA is making available guidance on the use of this approach. The fourth presentation described innovative mathematical modelling approaches applied to environmental remediation. The presenter emphasized that the use of mathematical models based on Kd approaches can lead to very conservative estimates and, instead, reactive geochemical transport modelling should be used wherever possible. Good interaction between proponents and regulators is a critical issue and mutual understanding about the overall simulation details must exist. Vitrification, as a means of immobilizing and isolating contaminated soil zones, has been used at various locations in the world. The fifth presentation described the improvements that have taken place in the technique over the last 10-15 years. These improvements have 103 SUMMARY OF SESSION 4 been achieved through its application to various problems and from an increased understanding of the melting process. It was argued that the technique avoids many of the problems of other remediation approaches by providing an almost ‘permanent’ solution that does not require active maintenance. Furthermore, the public is said to be convinced by the technique. The costs, while initially higher than other techniques, are said to become comparable or less over time because of the absence of the need for maintenance or storage. Mitigative approaches are now being applied to address the safety issues which were associated with use of the technique in the past, e.g. incidents involving steam explosions caused by groundwater heating. The final presentation described the remediation of an actual uranium mining site in Hungary. Restoration of rock piles, ponds and heap leaching sites was necessary. The steps needed to reduce radiation levels on the site, roads, pipelines and in groundwater to acceptable values were described. In all of the presentations, the importance of stakeholder involvement was emphasized. The confidence of stakeholders, including the affected public, must be obtained when applying the various techniques described in this session. 104 LIFE CYCLE PLANNING AND STAKEHOLDER ISSUES IN ENVIRONMENTAL RESTORATION (TOPICAL SESSION 5) Chairperson M. PAUL Germany BALANCING THE URANIUM PRODUCTION CYCLE: CENTRAL ASIA AS A CASE STUDY A.T. JAKUBICK*, D.R. METZLER*, P.WAGGITT*, R. EDGE** * ** Uranium Mining and Remediation Exchange Group (UMREG) IAEA, Vienna, Austria Abstract This paper examines the lessons learned from studies of the status of uranium mining and milling legacy sites in the countries of Central Asia. A review is given of the condition of the sites, of the potential risks associated with them and of the remediation needs. Drawing on experiences from around the world, guidance is given on how to avoid some of the problems of the legacy sites when entering into new uranium production programmes. 1. URANIUM PRODUCTION LEGACY SITES AND WHAT THEY TEACH US REGARDING MANAGEMENT OF THE URANIUM PRODUCTION CYCLE 1.1. Introduction During the Cold War era the global uranium production industry generated huge volumes of radioactive mining and processing waste and caused a degradation of land and surface and ground water resources on an unprecedented scale. The end of the Cold War coincided with a period of low uranium prices. As a consequence, several of the companies which generated these legacies went out of business, leaving the former production sites unremediated. In most cases this was because there were no regulations regarding remediation and long term safety and no requirements to deposit remediation funds. In response to the increase in environmental awareness of this problem, in the period from 1989 to the early 1990s, governments in several countries deployed large scale programmes for mitigating the liabilities caused by the uranium industry. The most well known of these programmes are: – The US Department of Energy’s Uranium Mill Tailings Remedial Action (UMTRA) Programme; – The Wismut Remediation Programme of the German Federal Ministry of Economics; – Programmes in Canada (e.g. the National Uranium Tailings Programme and decommissioning at Elliot Lake and elsewhere) and Australia (e.g. Rum Jungle); and – The European Commission’s multi-country Phare pilot projects for remediation of the uranium legacy sites in Central and Eastern European Countries. 1.2. Analysis of the unit remediation costs Taking the year 1992 (i.e. 3 years after end of the Cold War) as a baseline for comparison, an analysis of the above ‘old’ remediation programmes provides the remediation costs per unit of ‘yellow cake’ production, Table 1 [1, 2, 3]. 107 TOPICAL SESSION 5 TABLE 1. TOTAL PRODUCTION AND UNIT COSTS OF REMEDIATION PER URANIUM PRODUCTION (IN ORDER OF INCREASING CUMULATIVE PRODUCTION) Country Sweden Slovenia Spain Hungary Gabon Namibia Australia South Africa Germany (Wismut) Canada USA (UMTRA, Title I) USA (UMTRA, Title II) Cumulative production by end of Unit remediation costs 1992 (metric tonnes of U3O8) (US $ / kg U3O8) 200 89.0 379 80.5 3 777 11.0 19 970 3.7 21 446 1.2 53 074 0.9 54 225 1.3 143 305 0.5 232 000 22.6 257 702 0.3 56 000 32.4 254 000 1.0 Table 1 indicates that the unit cost of remediation (except for a few outliers) generally decreases with the volume of production. However, a more detailed look reveals that beyond production size, the unit remedial costs are affected by a series of other factors. In the case of large remediation programmes, the indicators are based on average remediation costs, which depend on the range of variation of the individual project costs. For instance, the costs for Uranium Mill Tailings Remedial Action (UMTRA) Project Title I sites in the United States are based on 22 tailings remediation projects (i.e. on a large number of projects dealing with the remediation of the tailings ponds only), the costs of which vary from US $2.6 to US $375 per kg of U3O8. The WISMUT Remediation Programme comprised the full scale of uranium mining and processing wastes remediation; it included remediation of underground mines, an open pit mine, waste rock dumps, tailings ponds, area remediation, decommissioning and demolition. The programme costs (approximately US $6.2 billion) also included compensation for damages caused during the period of production, social mitigation and corporate restructuring. The mines Rudnik Žirovski Vrh, RŽV (Slovenia) and Ramstad (Sweden) can be used as examples of small projects. At RŽV, approximately 380 te of uranium were produced from 1984 to 1990 and approximately US $ 36 million was spent on closeout and remediation (until 1992). Accordingly, the unit costs were approximately US $80 per kg of U3O8. These costs are at the upper end of the unit costs in Table 1. Although the project in Ramstad is comparable in terms of total production (200 te U) and remediation costs (approximately US $89 per kg of U3O8), the technical comparison is flawed because Ramstad was an open pit mine and RŽV, an underground mine. Thus, the ‘real’ unit costs of U production and remediation depend on the characteristics of the specific site and on the design selected and agreed upon (with regulator and stakeholders) for implementation. 2. ASSESSMENT OF PRIME LEGACY SITES OF URANIUM PRODUCTION IN CENTRAL ASIA Based on the results and observations during the International Atomic Energy Agency’s (IAEA) Technical Cooperation Regional Project on Monitoring and Assessment of the Uranium Production Legacy Sites in Central Asia, 2005 – 2008, a preliminary expert opinion is provided in Table II on the prime uranium legacy sites in the region. In spite of the IAEA 108 JAKUBICK et al. Regional Programme and numerous other international programmes, there is still a shortage of reliable and systematic measurements from the Central Asian legacy sites. For this reason, the characterization and comparison of the legacy sites and facilities cannot be based on ‘classical’ Environmental/Radiological Impact Assessments (EIA). The assessment in Table II goes beyond environmental and radiological aspects, taking into account ‘politically’ justified remediation criteria as well as cross-boundary and socio-economic impacts and possible economic benefits from re-treatment of legacy waste for recovery of valuable constituents (Au, Ag, Mo, V, rare earth element residues, etc.). Although qualitative in nature, the structure of Table II follows the principles of risk assessment: Risk = Likelihood x Consequences where Likelihood or Probability is (Frequency of impact) x ((Frequency of failure events) / (Lifetime of waste facility)) Frequency of Impact = How often the release of contaminants occurs and Consequences or Impact includes: Severity (how much contamination is released); Extent (how many people are affected, size of territory involved etc.); and, Duration (of damage, exposure after release and/or cumulative effect of continuous small releases) 109 TOPICAL SESSION 5 TABLE 2. ASSESSMENT OF PRIME URANIUM PRODUCTION LEGACY SITES IN CENTRAL ASIA Country: Kazakhstan, Kz Vulnerability and Potential impact likelihood of release Robust piles; direct Steady local accumulation of radiation and wind contaminants from seepage erosion prevented by and discharge in soil, remediation aquifer(s) and river sediments Seasonal release of Geomechanical damages to contamination into open pit mines ground water Contaminated water left in Sustainability of open pits remediation results Seasonal exposure of summer needs regular house residents using maintenance contaminated water for flooded open pit mines irrigation left unremediated Koshkar Ata: Stable TP Local accumulation of Tailings pond (TP) Contaminants release contamination in soil due to on the Caspian due to dusting from continuous dusting Sea, near Aktau the dry tailings surface No public exposure due to Hydrogeology of site long distance from Aktau prevents leakage from TP is an obstacle to TP development of town to a sea Scrap metal side resort scavenging prevented by a concrete cover in parts of TP Stepnogorsk TP TP in operation and Local accumulation of at Aksu: under operational contamination in soil due to 3 compartments monitoring continuous dusting, occasional filled to 95% with Contaminants release seepage and leakage through legacy tailings from the dry tailings base of TPs surface due to dusting Leakage from TP does not Responsibility for reach the deep ground water legacy tailings unclear No public impact Site and waste facilities Sites in N, E and S Kazakhstan: Mines, ore and mine waste piles* *(national remediation programme; completion in 2010) 110 Remedial measures needed Assess contamination release via water pathway Establish long term monitoring and maintenance programme Assess contamination release via air pathway International peer review prior to remedial works Assess contamination release via air pathway Enforce legal commitment to legacy remediation JAKUBICK et al. Site and waste facilities Mailuu Suu: Mine and mine waste, tailings piles Ak Tuz: Mine and mine waste, 4 tailings ponds Min Kush: Mine and mine waste TPs: Tuyuk Suu, Taldy Bulak Orlovka: TPs Country: Kyrgyzstan, Kg Vulnerability and Potential impact likelihood of release Tailings piles prone to Threat of damming up of river sliding on mountain and contamination of site slopes; Some relocated eliminated and/or confined Assessment of radiation Release probability exposure insufficient aggravated due to potential earthquakes Failure of some TPs Animal grazing at likely due to contaminated site questionable dam Potent. ‘tailings flow’ would stability and neglected damage and contaminate the maintenance downstream plains Water diversion canals Release would cause radiation not functional exposure of local population Release probability Potential contamination of the aggravated by seasonal transboundary Chu River surface water runoff Potential dispute with Kz from mountains and/or Potential for tailings reearthquakes treatment Potential acid mine Increased contamination due to drainage (AMD) may AMD would limit use of mine enhance contaminants water for irrigation release in mine water Potential ‘tailings flow’ after discharge dam failure at Tuyuk Suu Tuyuk Suu: would damage and Probability of contaminate the river valley overtopping and loss below Min Kush of containment likely Radiation exposure of due to a landslide, population at Min Kush seasonal surface runoff mainly due to use of from the mountains radioactive ash for insulation and earthquake of houses Taldy Bulak: Failure Potential tailings release at of crucial drainage Taldy Bulak would pipe under load of contaminate a small, tailings and seasonal uninhabited mountain valley mountain runoff without regular maintenance very likely Water diversion canals Potential tailings release would not functional damage and contaminate the Stability of TP transboundary Chu River Burdinskoye Potential dispute with Kz. questionable Potential for tailings retreatment Remedial measures needed Completion of remediation in agreement with radiation safety standards Enforce site security Perform EIA Remediate TPs Regular maintenance and monitoring Re-treatment to be made conditional on remediation Testing for AMD potential; EIA Feasibility study of Tuyuk Suu remediation options: (a) In situ remediation with regular maintenance (b) relocation of tailings Taldy Bulak: thorough maintenance programme EIA Feasibility study of remediating TP Burdinskoye Monitoring and maintenance Re-treatment to be made conditional on remediation 111 TOPICAL SESSION 5 Site and waste facilities Degmay (near Chkalovsk): Tailings pond (TP) Taboshar: Open pit mine Mine waste, Low grade U-ore pile Tailings 112 Country: Tajikistan, Tj Vulnerability and Potential impact likelihood of release Dry tailings surface Steady local accumulation of exposed to wind contaminants in soil due to erosion continuous dusting Leaky base of TP and Continuous leakage of steady release of contaminants in ground water; contaminants Extensive contamination of aquifer(s); Downstream distance to Syr Darya River 9 km Radiation exposure of local population due to use of contaminated ground water, scavenging of scrap metal and animal grazing on contaminated site Potential disputes with Uz due to contamination of transboundary Syr Darya River Continuous discharge Continuous exposure of from flooded open pit population by use of mine through contaminated discharge from dewatering tunnels on the open pit due to lack of outskirts of town alternatives Steady erosion of Steady accumulation of unprotected U-ore pile contamination of the local by wind and runoff creeks and flood plains on the water site due to release of Seasonal release of particulates from pile and highly contaminated discharge from tailings seepage through Potential AMD would damaged and fundamentally affect remedial inadequate tailings strategy covers Animal grazing on site Potential AMD in Partial use of contaminated tailings would enhance materials for construction contaminants release Remedial measures needed EIA; assessment of ground water contamination and impact on Syr Darya River Feasibility study of remediating TP Installation of an upto-date ground water monitoring system Treatment of water discharging from open pit Enforcement of site security Testing of tailings for AMD EIA Feasibility study for a complex remediation plan International peer review prior to remedial works JAKUBICK et al. Site and waste facilities Cherkasar 2: Mine and mine waste Yangiabad: Mine and mine waste Country: Uzbekistan, Uz Vulnerability and Potential impact likelihood of release Abandoned mine Contaminants discharge from works present a safety shaft into local river hazard Animal grazing on Open shaft allows contaminated site water discharge and Use of radioactive materials radon exhalation for construction in town Perimeter wall allows Economic depression of access to site former mining town Abandoned mine Contaminants discharge from presents a safety mine into local river hazard and allows Potential radiation exposure water and radon due to unsecured access to discharge mine and waste rock piles Uncovered mine waste piles exposed to wind and water erosion Remedial measures needed EIA; assess in-door radon levels; Feasibility study for remediation Improve site security Educate local population Monitor site EIA Feasibility study for remediation Improve site security Educate local population Monitor site The assessment in Table 2 shows that the 5 priority (most risky) legacy sites/facilities in Central Asia are the: – Degmay tailings pond, – Taboshar site, – Tailings ponds no. 2 and 4 at the Ak Tuz site, – Burdinskoye tailings pond, and – Tuyuk Suu tailings pond at the Minkush site. The remediation priorities of these sites/facilities are justified (in addition to the local radiological risk) at Degmay by the ongoing release of contaminants into the ground water and the closeness of the site to the Syr Darya River, at Taboshar by the extensive use of the contaminated water from the open pit mine by the population, by the high concentration of contaminants released from the low grade uranium ore pile and tailings into the creeks and by the central role the flooded open pit mine would play in any remediation strategy designed for the site. Security of the tailings piles at the Ak Tuz site primarily depends on the water diversion works, which are not functional; the dams at TP2 and TP4 are in a badly deteriorated state and the site is subject to a significant risk of seismic events and excessive water runoff from the mountains. A potential release of tailings in the form of a slurry wave would severely affect the agricultural plains downstream of the site and the transboundary Chu River. The same arguments apply at the Orlovka site and to a lesser degree at the Minkush site. Only localized impacts can be expected at the Cherkasar and Yangiabad sites. Nonetheless, these sites should also be the subject of a detailed environmental impact assessment and a monitoring and maintenance programme should be established. The major tailings impoundment at Navoi in Uzbekistan, containing large volumes of uranium legacy tailings, is in operation but is presently receiving non-radioactive ‘gold’ tailings. Although the ‘gold’ tailings discharge regime is adjusted to serve the remediation of the legacy tailings, the long term performance of this remediated site warrants an international peer review. The quantification of the specific risk factors for each site and the calculation of the health and environmental impacts is a task to be tackled in the preparatory phase of the respective remediation projects. From a pragmatic point of view, it should be sufficient to assume that a waste facility is safe if the risk = {[(failure × release) probability] × impact} is in compliance with the regulatory requirements of the respective country. To reduce risk 113 TOPICAL SESSION 5 levels to as low as reasonably achievable, it is a good policy to follow existing internationally recommended procedures and standards for the safe management or remediation of the waste facilities. The maintenance of safety at the legacy sites requires the establishment of long term legacy sites management programmes (for contaminated water treatment, site maintenance and monitoring, etc.) in each country. 3. OPTIMIZATION OF THE URANIUM PRODUCTION CYCLE One of the most important lessons learned from the completed remediation programmes/projects is that prevention is less costly than the creation of new legacy sites and that minimization of waste generation is the best uranium production strategy. Whenever a new uranium mine development is evaluated it is important to evaluate the costs of the whole uranium production cycle (UPC) which comprises all the activities involved, from exploration, feasibility studies, environmental impact studies, development of production facilities, mining and processing through to, decommissioning, remediation and post-remedial management of the sites (i.e. from cradle to grave). Environmental issues arising at all stages of the cycle are an integral part of the UPC. Consequently, responsible decisions must be based on cost/benefit calculations derived for the lifetime costs of the entire UPC. At major decision making points, this includes taking into account any requests of the legitimate stakeholders, in order to obtain a ‘social licence’ from the public in addition to all the necessary legal permissions and authorizations. 114 JAKUBICK et al. TABLE 3. OPTIMIZATION OF THE PRODUCTION/WASTE GENERATION IN THE URANIUM PRODUCTION CYCLE Stage No.: 1 2 Uranium production (Goal: Maximization of production and revenue) Exploration →Resources Pre-feasibility assessment Detailed exploration →Reserves Feasibility assessment Design of mining and processing options Planning of operations 3 Mining of ore 4 Ore processing → ‘yellow cake’(U3O8) 5 Closure planning Decommissioning and demolition 6 a) Remedial preparation: Design and planning; target levels according to clearance criteria and planned utilization; b) Remedial works and water treatment c) Regulatory clearance d) Assignment of long term institutional control of the legacy site Waste generation, discharges and spills (Goal: Minimization of waste, risk and expenses) Segregation of radioactive (e.g. ore samples, cores) and conventional waste and disposal EIA and reference environmental baseline For each option: Assessment of waste generation, discharges, risks and associated costs over the lifetime of the facility Contamination of land, water and waste Monitoring of operations and baseline Adjustments and continuous optimization Contamination of land, water and waste Monitoring of operations and baseline Continuous optimization and adjustments Segregation of generated radioactive/nonradioactive waste → orderly storage Monitoring of operations and baseline a) EIA of long term impacts for each option, including water treatment requirements b) Monitoring of works and baseline c) Reclaimed land utilization; provision of clean water d) Long term stewardship and maintenance (LTSM): legacy site management and supervision of confinement integrity The minimization of waste generation (and, thus, of the health, environmental and socio-economic risks) cuts across the whole uranium production cycle and solutions must emerge from actions at each stage of the cycle. Although corporate commitment is crucial, the involvement of the employees at each stage should be solicited and their proposals, if promising, implemented in the planning. It is assumed that production management is carried out at each stage as efficiently as possible, but the decision making should include both prevention and minimization criteria and be an integral part of corporate operations that link the production cycle throughout the corporate planning process. 3.1 The effect of a lifetime cost/benefit assessment on decision making: an example To be able to decide during the project preparation (the design, development and engineering stage) from among the options available for the development of a new mine/ processing site or remediation of a legacy site, it is essential to make the comparison on the basis of the lifetime costs. Sub-optimal design stage decisions are difficult to correct after implementation of the works and can result in cost differences of 10s to 100s millions of USD. For instance, using a probabilistic risk assessment for comparison of wet tailings remediation (such as implemented at Elliot Lake, Ontario, Canada) with dry tailings remediation (such as implemented by Wismut in Saxony and Thuringia, Germany) it was shown that the initial investment cost advantage of a wet remediation can be entirely reversed when the post- remedial phase is included in the assessment, as shown in Fig. 1 [4]. 115 TOPICAL SESSION 5 The case study is based on the situation of the Helmsdorf tailings pond in Germany. The Helmsdorf tailings pond contains approximately 50 million tonnes of tailings. It is an upstream, valley type of impoundment. In 1992, the main dam was 1800 m long and 59 m high and did not meet the safety standards for water retaining structures. In the case of a complete dam failure, 6 million m3 of pond water and 15 – 30 million m3 of tailings slurry would have been released containing, among other contaminants, 80 tonnes of uranium and 600 tones of arsenic. Approximately 1000 inhabitants would have been affected by the slurry wave directly, and approximately 6500 people would have been affected by the damming up of the Mulde river. An area of approximately 1000 hectares would have been damaged and contaminated. 100 95 80 65 Percentiles 60 “Wet” Tailings Remediation Remediation “Dry” Tailings Remediation 40 Comparison based on case of the Helmsdorf tailings pond, Wismut, Germany 20 0 0 250 Initial investment costs 500 750 1000 1250 2500 2750 Million Euro FIG. 1. Example of increase of cumulative probabilities of equivalent costs for maintenance, damages and mitigations over the lifetime of a tailings pond for wet and dry tailings remediation options in a low to moderately seismic zone (based on the Helmsdorf tailings pond, Wismut, Germany)[4]. After having worked out the risk-cost relationship for the entire lifetime of the Helmsdorf tailings pond (Wismut, Germany), a remediation leading to a dry landscape proved to be both safer and more economic than the ‘wet’ remediation option, which had lower initial investment costs. Both technical options were feasible except for the long term risk management. Because the regulator and the main stakeholder (the local community that would be impacted in case of a failure) requested a safety performance of 95%, the initial cost advantage of a wet remediation option was lost because in the range above the 65% safety level, the cost/benefit ratio of the dry remediation was considerably more favourable. This, however, does not mean that the wet remediation is, in all cases, worse. Unlike the Elliot Lake site, the Helmsdorf site has a history of seismic activities that made it imperative to design for a 95% safety performance. As demonstrated, fundamental decisions - irrespective of whether it concerns the development of a mine, processing plant, waste management or waste containment facility should only be made on the basis of full lifetime costs. 116 JAKUBICK et al. 4. REGULATORY CHALLENGES OF THE NEW URANIUM MINING PROJECTS IN CENTRAL ASIA The orderly management of the uranium production cycle requires that an appropriate legislative and regulatory framework, a responsible regulatory IAEA and national policies, programmes and plans are in place in this regard. In view of the lessons learned from the legacy sites, the rush to develop new uranium mines in Kazakhstan and Uzbekistan presents a considerable challenge for the existing legislative and regulatory systems. The regulators in these countries have to realize that it is not sufficient to rely on ‘end-of-the-pipe’ regulations. Instead, the regulatory policy should aim to ensure that uranium mining companies consider and manage potential environmental liabilities as part of their fundamental business practice and ensure that these activities are accounted for in both the project financing and plans submitted for approval. The costing of the projects must be based on the lifetime costs of the uranium production cycle. After closure of most of the conventional uranium mines in Central Asia in 1995, the new mining projects focused on in-situ-leach mining (ISL) for uranium. During the last decade, ISL mining has been continuously growing in the region because of the low capital expenditure required and because it can exploit low grade ore deposits. Besides economic advantages, compared to conventional mining, the ISL process generates little waste and has only a small impact on the surface. Current ISL plants use an ‘enclosed system’ for the recovery and ion exchange process steps thereby reducing the possibilities of radon release; furthermore, vacuum dryers are used (rather than higher temperature calciners) with little, if any, particulate emissions. Taking into account all these advantages, a further growth of ISL mining in Central Asia can be expected over the coming years. From a long term perspective, however, there is a need in Central Asia to give greater attention to the prevention of aquifer degradation and the protection of scarce ground water resources. ISL requires that mining operators have good control of the injection and recovery flows and therefore a good monitoring system for the well-field is essential. For this reason, cautious ISL operators install, in addition to monitoring wells in the aquifers below and above the mined unit, observation wells in the well field itself (trend wells) to obtain a better control of the dynamics in the mined unit. In addition, these wells can act as an ‘early warning’ system. Unfortunately, the transfer of the most modern ISL technologies to Kazakhstan and Uzbekistan has not been matched by the introduction of up-to-date ground water monitoring instruments and methods. Experience from Kazakhstan shows that, due to the convenient geology of the ISL aquifers, there is no immediate need to remediate the mined units afterwards; the acidic conditions in the units become neutralized relatively quickly. In this connection, it should be noted that the required environmental impact assessment and monitoring for ISL facilities places the same requirements as those applied to conventional mills (i.e. the aquifers are considered as receptors instead of being assessed as a mined medium). The remediation bond can accordingly be kept very low (sometimes less than USD 1 million per ISL field). Even in the case where the leached-out ISL field really does not require any remediation, the regulators would be well advised to request the installation of some monitoring wells in the abandoned mining fields to observe the rate of reinstatement of natural conditions in the aquifers. The natural buffering capacity of the mined aquifer can come to an end with the progress of ISL from mining unit to mining unit. The return of the aquifer to natural conditions or restoration to conditions consistent with the original designated use of the groundwater is essential for long term use. If needed, the restoration of the ‘mined out’ units is usually done in stages. This involves pumping of residual fluids from the well field and conventional treatment of the fluid; the radioactive constituents, primarily radium-226, are removed by standard methods, such as barium117 TOPICAL SESSION 5 sulphate precipitation, reverse osmosis, etc., and disposed of subsequently as a small volume of naturally occurring radioactive material (NORM) residue. In view of the ever increasing withdrawal of water for agricultural purposes in Central Asia, the economics of water resources management is bound to change drastically in the near future. From a macroeconomics point of view, when considering the revenues generated from U3O8 production by ISL it should be borne in mind that it takes, on average, approximately one litre of water to produce one calorie from food crops. To achieve the remediation of the numerous legacy sites and to master the present uranium ‘boom’ in a balanced way, it will require pragmatic policies, programmes and plans at the policy making level, a well established legislative framework and effective regulatory institutions in the Central Asian countries. The international community, and primarily the IAEA, should face up to this challenge and provide as much assistance in this matter as possible. 5. CONCLUSION: A NEW BUSINESS MODEL OF URANIUM PRODUCTION The amount of long term savings in a life-cycle based costing comes not only from adjusting production, there are important planning and accounting issues as well. The proposed changes have to respect that cash flow projections show the fair value of the mining project but must at the same time address the environmental and stakeholder issues affecting the mining corporation from the earliest stages of the mining project. International co-operation and co-ordination are essential to support these efforts and any State action aimed at regulating uranium production. National regulations need to be attuned to individual circumstances by implementation of suitable policies, programmes and plans at the level of governments. However, uncoordinated actions using diverging instruments will only confuse uranium producers and distort competition. What is needed is a strengthening of the leadership role of the international organizations, such as the IAEA, through their engagement with the industry, stakeholders and regulators in creating an environment which is protective of the public and the environment whilst simultaneously encouraging economic development of uranium mining and production. REFERENCES [1] [2] [3] [4] 118 HAGEN, M., JAKUBICK, A.T., LUSH, D., METZLER, D., Integrating Technical and NonTechnical Factors in Environmental Remediation: Conclusions and recommendations of the UMREG’02 Meeting Wismut GmbH (2003). BMWI, Study No. 90/95, Costs of decommissioning and remediation of uranium mining and milling projects in international comparison, Final report of the research project No. 37/93, Uranerzbergbau GmbH (UEB) (1995). WISMUT GMBH, Audit Report, Investment Programme for the Remediation Tasks of Abandonment of the Hungarian Uranium Industry (1999). ROBERDS, W., VOSS, C., JAKUBICK, A.T., et al., Multi-Attribute Decision Analysis of Remediation Options for a Uranium Mill Tailings Impoundment in Eastern Germany, American Nuclear Society, Proceedings of International Topical Meeting on Probabilistic Safety Assessment (PSA '96) - Moving Towards Risk Based Regulations, Park City, Utah (1996). IAEA PRELIMINARY ASSESSMENT OF THE FORMER FRENCH NUCLEAR TEST SITES IN ALGERIA D.W. REISENWEAVER Alion Science & Technology, Los Alamos, United States of America Abstract In 1999, the International Atomic Energy Agency received a request from the Government of Algeria to perform an assessment of the radiological conditions of the former sites used by the French government in the early 1960s for the testing of nuclear weapons. This paper describes the history and the nature of the test site and the tests that were performed, the methodology of the IAEA assessment and the results and conclusions drawn from the mission of international experts. 1. INTRODUCTION In 1999, the International Atomic Energy Agency received a request from the Government of Algeria to perform an assessment of the radiological conditions at the former sites used by the French government in the early 1960s for the testing of nuclear weapons. In response to this request, in late 1999, the IAEA sent an international team of experts to perform a radiological assessment. The expert team was composed of experts from France, New Zealand, Slovenia, the USA and the IAEA. The terms of reference for the expert mission were to: – Make a preliminary assessment of the existing radiological situation at the Reggane and In-Ekker test sites by performing radiation/radioactivity measurements at the sites and at selected inhabited locations; – Collect selected environmental and food samples for analysis; and – Based on the results of these measurements, perform a preliminary dose assessment and develop a plan for monitoring the test sites more comprehensively, if justified. The mission was able to achieve more than initially expected because of the detailed information provided by France related to the history and location of the tests. 2. TEST SITES Nuclear tests were performed at two test sites in Algeria, they were Reggane and InEkker. Both of these sites are located in the southern central part of the country and are shown in Fig. 1. 119 TOPICAL SESSION 5 FIG.1. Location of Algerian test sites. Reggane test sites The Reggane test sites were used for above ground nuclear weapons tests and are located approximately 50 km south of Reggane, a small oasis village and 150 km south of Adar, a city of approximately 50 000 inhabitants. The following table provides information concerning the four atmospheric tests performed at the Reggane site. TABLE 1. ATMOSPHERIC NUCLEAR TESTS CONDUCTED AT REGGANE Test Date Type Yield, W (kt) Gerboise Bleue Feb 1960 Tower, 100 m 40<W<80 Gerboise Blanche Apr 1960 Surface W<10 Gerboise Rouge Dec 1960 Tower, 50 m W<10 Gerboise Verte Apr 1961 Tower, 50 m W<10 The largest contribution to the radiation dose that can be measured at the present time is due to 137Cs; other fission or activation products contribute less than 5% to the dose rates. Fig. 2 shows the radiation dose rates and surface activity levels of 137Cs in the surface areas of the fallout zones. The Gerboise Blanche test was performed on the surface and a crater was produced that was later filled in. Consequently, a large amount of the residual activity remains in material buried under several metres of sand. 120 OUGHTON GERBOISE BLEUE GERBOISE VERTE GERBOISE ROUGE N N Z1 N Z2 Z5 0.15 km2 0.08 km2 0.15 km2 0.22 km2 0.56 km2 0.5 km 0.5 km 0.5 km GERBOISE BLANCHE N 0.002 km2 Z0 0.006 km2 0.015 km2 0.05 km 1 km2 0.5 km from 0.05 to 0.5 Gy/h (from 0.02 to 0.2 MBq/m2) from 0.5 to 1.5 Gy/h (from 0.2 to 0.6 MBq/m2) from 1.5 to 5 Gy/h (from 0.6 to 2 MBq/m2) from 5 to 15 Gy/h (from 2 to 6 MBq/m2) FIG. 2. Radiation dose rates and surface activities of 137Cs at Reggane (in 1999). In the area of the Gerboise Rouge test site, an additional series of tests was performed to measure the velocity shock wave in a pellet of plutonium. 35 experiments were performed, each using a plutonium pellet weighing about 20 g. These tests were performed in pits designed to limit dispersal. The majority of the plutonium remained in the pits after the tests, but low residual activity can still be detected near to the pits. The pits have been backfilled with sand. In-Ekker test site In-Ekker consists of two sites, Taourirt Tan Afella and Adar Tikertine. Underground nuclear weapons tests were performed in tunnels that were dug into the granite massif at Taourirt Tan Afella. This area was virtually uninhabited at the time of the tests. Thirteen tests were performed at this site; details are given in Table 2. All of these tests were performed in 121 TOPICAL SESSION 5 tunnels that were designed so that the radioactive products would be confined within the mountain at the ground zero point in rock that would become molten at the moment of firing. TABLE 2. UNDERGROUND NUCLEAR TESTS CONDUCTED AT TAOURIRT TAN AFELLA Test Date Yield, W (kt) Agate Nov 1961 W<10 Beryl May 1962 10<W<40 Emeraude Mar 1963 10<W<40 Amethyste Mar 1963 W<10 Rubis Oct 1963 10<W<40 Opale Feb 1964 W<10 Topaze Jun 1964 W<10 Turquoise Nov 1964 W<10 Saphir Feb 1965 W>80 Jade May 1965 W<10 Corindon Oct 1965 W<10 Tourmaline Dec 1965 10<W<40 Grenat Feb 1966 10<W<40 Nine of the tests (Agate, Emeraude, Opale, Topaze, Turquoise, Saphir, Corindon, Tourmaline and Grenat) were fully contained. Two tests (Rubis and Jade) were not fully contained and some radioiodines and gases were released from the tunnel openings. Two tests (Beryl and Amethyste) were only partially contained and significant releases of radioactive material occurred. All of the tests, except these last two, did not produce any significant radiological residues outside the tunnels. To contain the tests, a spiral shaped tunnel opened into the firing chamber as shown in Fig. 3. The spiral was designed to be closed off by the shock wave before the lava could reach the entrance to the tunnel. During the Beryl and Amethyste tests, this blocking of the main tunnel did not occur. During the Amethyste test, a small quantity of molten rock was deposited near the tunnel entrance. In 1965, the residual dose rate 1 metre above the lava surface was reported as exceeding 50 Gy/h. In 1999, the residual dose rates were just above 1 Gy/h. The Beryl test resulted in a much more significant release to the environment. Approximately 5–10% of the test product activity was released as lava, aerosols and gaseous products. Most of the residual contamination is fixed in the lava. The 1999 estimated dose rates in the area of contamination are shown in Fig. 4. These levels are not insignificant but the Beryl test site is located in an area that is very difficult to gain access to. Nevertheless, to prevent access, the area contaminated by the test was fenced off and appropriate warning signs were affixed to the fence. However, over time, this fence has become ineffective as shown in Fig. 5. 122 OUGHTON FIG. 3. Arrangement of tunnel used for weapons testing. FIG. 4. Radiation dose rates in 1999 in the area contaminated by the Beryl test. 123 TOPICAL SESSION 5 FIG. 5. Typical fence surrounding area where nuclear tests were performed. Five additional experiments were performed about 30 kilometres south-west of Taourirt Tan Afella, in the region of Adar Tikertine. The purpose of these experiments (called the Pollen experiments) was to simulate an accident involving plutonium and to measure its consequences, including the degree of contamination that might be produced in the vicinity of the tests. The method involved measuring the amounts of plutonium aerosols generated by pyrotechnic dispersal. The experiments involved 20 to 200 g of plutonium and were performed when the wind was blowing across the area planned for collection of the fallout. After each test, the most contaminated area was covered with asphalt to limit resuspension. Low levels of residual activity can still be detected near the ground zero point. 3. FIELD SAMPLING Some field sampling was performed during the mission. This sampling was not as comprehensive as would be required for a full scale radiological monitoring programme and only a limited number of samples were taken. All samples were analyzed at the IAEA laboratory in Seibersdorf, Austria. Soil, water and vegetation samples were taken. Soil samples were taken for evaluating the resuspensible fraction that might expose intermittent visitors and travelers as a consequence of high winds in the area. The water from three different wells in the area of InEkker was sampled by collecting water directly from the buckets used by travellers. Vegetation samples were taken from near the Beryl tunnel entrance where the largest release occurred. The plant types collected were known to be used by camels as food. The results of these samples are provided in the IAEA report of this mission [1]. 124 OUGHTON 4. CONCLUSIONS AND RECOMMENDATIONS The two areas that had the highest residual activity were: – The ground zero locations at the Gerboise Blanche and Gerboise Bleue atmospheric test sites located near Reggane; and – The vicinity of the tunnel where highly radioactive lava was ejected during the Beryl underground test. Two additional areas had residual activity but at a lower level: the vicinity of the tunnel for the Amethyste test and at the Adrar Tikertine site where the Pollen tests were performed. All of the other areas had little residual activity. A conclusion of the assessment was that environmental remediation is not required at any of the test areas in order to reduce doses below established safety standards, and that any possible exposures at Taourirt Tan Afella can be controlled through access restrictions. However, future decisions by the Algerian authorities to carry out further remediation or to further limit public access might be appropriate if economic conditions change in the area and a more permanent presence of people is indicated. 4.1. Specific conclusions Reggane Radiation doses to visitors to the remote desert tests sites area are estimated to be less than a few Sv/day. Residual steel fragments and fused sand, if removed from the site, do not present any significant radiological risk. However, if fused sand were ground to respirable dust without respiratory protection, this could present an inhalation hazard. Calculated radiation doses to residents of the town of Reggane from the airborne transport of dust from the test areas are predicted to be very low, much less than 1 Sv/y. Taourirt Tan Afella Nomadic camel and goat herders grazing their animals on the sparse vegetation in the area of the Beryl and Amethyste galleries might receive small doses, principally from external radiation, of less than about 50 Sv/y. Persons scavenging metals in the immediate vicinity of the lava from the Beryl tunnel might receive doses of up to about 0.5 mSv in 8 hours. Current external exposure dose rates are less than one-tenth of those existing in 1966. These dose rates are decreasing annually due to the decay of 137Cs (1999 maximum concentrations were 2 kBq/g). The alpha activity concentration in the lava is in the range 40 – 400 Bq/g, which is roughly similar to that of natural rock with 0.2 percent uranium content, and below that of a commercial uranium ore body. Adrar Tikertine The concentration of plutonium was determined in a small number of sand samples too few to be representative of the area. Nevertheless, the activity concentration of anthropogenic radionuclides in those samples measured was generally below laboratory detection limits. Thus, it is expected that the residual surface contamination from the plutonium dispersion experiments is unlikely to give rise to doses to nomadic herdsmen or their families exceeding 1 Sv/a. 125 TOPICAL SESSION 5 4.2. Recommendations The integrity of the fence constructed in the 1960s after the accident at Taourirt Tan Afella should be restored and maintained to avoid exposures arising from human and animal intrusion in the region around the Beryl tunnel entrance or through any removal of samples of lava from the site. The upper bound evaluation of the radiological conditions assessed in this preliminary study is considered robust, and further extended sampling for radiological assessment is not considered necessary. Corroboration of the predicted low inhalation doses arising from the Reggane site could be readily achievable through an appropriate air sampling programme, and it is recommended this be carried out. Similarly, corroboration of the findings of no dose impact to the local herdsmen and nomadic people in the In-Ekker area should be achieved by an appropriate environmental monitoring programme, in particular, water from wells adjacent to the Taourirt Tan Afella test site could be analyzed. Better descriptions of the lifestyles of the people that frequent these areas would add credibility to the findings of the assessment. REFERENCES [1] 126 INTERNATIONAL ATOMIC ENERGY AGENCY, Radiological Conditions at the Former French Nuclear Test Sites in Algeria: Preliminary Assessment and Recommendations, Radiological Assessment Reports Series, IAEA, Vienna (2005). SOCIAL AND ETHICAL ISSUES IN REMEDIATION D.H. OUGHTON Norwegian University of Life Sciences, Aas, Norway Abstract The contamination of environments with radionuclides can give rise to consequences additional to the health risks from exposure to radiation. As experience from Chernobyl has demonstrated, both accident and remediation measures can have serious social, ethical and economic consequences. This paper presents a review of some of these issues and presents a ‘check-list’ of the socio-ethical aspects of remediation measures. The paper also discusses remediation measures that are directed towards benefits other than dose reduction. 1. INTRODUCTION Remediation measures can do much to alleviate anxiety and restore the way of life in communities living in contaminated areas. However, remediation is rarely without sideeffects: the Chernobyl accident showed that remediation can be expensive, socially disruptive, or damaging to the environment [1–4]. On the other hand, remediation can have benefits that go beyond radiation dose reduction, such as restoring ecosystems, increasing public understanding and control, restoring consumer confidence in a product, or securing the livelihood and social structure of affected populations. While the primary objective of remediation is usually dose reduction, for an action to be justified, the benefits from dose reduction or averted dose should outweigh the costs of implementing the countermeasure [5]. It follows that a decision on how to reduce exposure to radiation will involve an ethical judgement: a choice is being made about which doses to reduce and at what cost. While the main criteria for remediation are usually based on technical or economic constraints, an extended evaluation can include social factors such as public perceptions of risk and dialogue with affected communities, as well as ethical aspects such as informed consent and the fair distribution of costs and benefits [1, 2, 6] This paper reviews the main social and ethical issues associated with remediation decisions. It includes a summary of the generic social and ethical aspects of remediation, and concludes with a presentation of some of the remediation measures that are not primarily intended to reduce radiation dose. 2. MULTI-DIMENSION ASPECTS OF REMEDIATION The multi-dimensional aspects of remediation were an important part of the STRATEGY 5th Framework EU project – Sustainable Restoration and Long term Management of Contaminated Rural, Urban and Industrial Ecosystems [www.strategyec.org.uk], and the follow-up EURANOS project (www.euranos.fzk.de), both of which included a number of remediation evaluation criteria, such as practicality and acceptability, socio-ethical aspects, environmental consequences and indirect side-effect costs [6, 7]. Stakeholder evaluation of countermeasures suggested that many options were as likely to be rejected on socio-ethical grounds as on technical and economic grounds [8]. Examples included a strong aversion to any measure that would bring about contamination of previously uncontaminated foods (e.g. mixing milk from different sources) or environments. Legal constraints also play an important role, particularly with respect to environmental legislation (e.g. habitat protection) and labour rights [1]. The summary of social and ethical factors below 127 TOPICAL SESSION 5 is taken from previously published work carried out under the STRATEGY and EURANOS projects [1, 6, 9]. The focus in this paper is on issues that are grounded in fundamental ethical values, and which are relevant to any risk assessment. Obviously, the list is not exhaustive and can provide only an illustration of some of the issues that might be considered, hence descriptions and examples are rather general. Self-help/disruptive: ‘Self-help’ adresses the extent to which the affected persons themselves can implement actions and their degree of control or choice over the situation. Voluntary actions that are carried out by the public or affected individuals themselves, or that increase personal understanding or control over the situation, are usually deemed positive as they respect the fundamental ethical values of autonomy, liberty and dignity. Concrete examples include the provision of counting equipment, dietary advice and certain agricultural procedures that could be carried out by the farmer. On the contrary, imposed measures that are highly disruptive, infringe upon liberty, or restrict normal practices can often be judged to be negative. Examples include relocation, bans on amenity use, or a radical change in farming practice. Welfare: Doses, costs and side-effects: The averted radiation dose and the calculated cost of remediation have direct consequences for the welfare of society and/or individuals, and are thus also important ethically relevant aspects. Remediation may have additional impacts on community or cultural values in a number of ways. Negative side-effects can include rural breakdown, loss of consumer faith in a product, and the stigma of being ‘contaminated communities’. Disruptions to existing social and cultural patterns – such as those requiring changes in employment or lifestyle – are generally taken as negative, and the community can benefit from protection against such factors. Creation of local employment opportunities can benefit communities. Free informed consent of workers: The issue of consent is strongly linked to the fundamental ethical value of autonomy. Employers have a duty to obtain the informed consent of any worker who may be exposed to chemical and or radiation risk. This is particularly important if lower paid workers are employed to carry out the measure, as it has been suggested that the necessary conditions for free-informed consent are often violated for these groups [10]. The increased risk may justify some form of compensation via higher wage premiums, but compensation itself can raise questions of whether or not this may coerce people into taking risks they would otherwise not have [10]. Experience from Chernobyl illustrates the problems of compensation in promoting the ‘victimization’ of affected populations [2-4]. Distribution of dose, costs and benefits: The way in which remediation impacts on the distribution of costs, risks and benefits, has significance due to the fundamental ethical values of equity, justice and fairness. Costs, benefits and risk may vary over both space and time, and between different members of a community. The radiation dose distribution is obviously a main consideration for radiation protection, and many remediation measures that reduce collective dose may change the distribution of dose, for example, from consumers to workers or populations around waste facilities. The question of who is paying the monetary and social costs of remediation and who will receive the benefits must also be addressed. Another question is whether the action has implications for vulnerable or already disadvantaged members of society (children, ethnic or cultural minorities)? Who is being affected? Who is paying? Liability and/or compensation for unforeseen health or property effects: Employers usually hold legal and ethical responsibilities over their employees, and contractors or industries may be held legally or financially liable for any damage they may cause to public or private property. The matter of who bears liability is relevant both from considerations of responsibility (moral and legal) and because of links to equity issues. Liability can become particularly important if outside contractors are paid to carry out remediation, both for the 128 OUGHTON contractors themselves – Will I be sued if the actions cause unforeseen damage? – and the workers/property owners who may risk injury – Will I be compensated if the remediation causes me damage? Change in public perception or use of an amenity: If remediation has an effect on the public’s use of a particular amenity (such as restricting access to a park), then this will have an influence on acceptability. As was seen in the Chernobyl case, people place a large value on places with strong community and personal ties, such as those having childhood memories. Such effects can have deeper relevance than whether or not people are able to use the amenity. Perceptions can include, for example, that something has changed from being ‘natural’ to ‘unnatural’ or ‘clean’ to ‘damaged’. Alternatively, remediation that brings into use a previously restricted amenity will be socially more robust. Uncertainty: Uncertainty in this context can be taken to refer to an evaluation of the risk (environmental, technical, social) associated with remediation, and relate to the question of what the possible consequences of the remediation might be and the probability that those outcomes can occur. What are the main uncertainties associated with the remediation strategy? What action might be taken to avoid or reduce these uncertainties, and are some inevitably indeterminate? What are the consequences of being wrong? Environmental risk from ecosystem changes, groundwater contamination, etc: Remediation actions that change or interfere with ecosystems (e.g. ploughing or changing catchment drainage) may produce negative environmental consequences. In addition to the obvious questions of uncertainty, environmental risk raises a variety of ethical issues including consequences for future generations, sustainability, cross-boundary pollution, and balancing harm to the environment/animals against benefit to humans. The ethical acceptability of remediation will clearly depend on the ecological status of the area and the degree to which the action diverges from usual practice. In most cases, environmental legislation must be considered. Any countermeasure involving the generation of waste and/or its treatment will have ethical relevance (and controversy) in itself. Treatment of waste ‘in situ’ can be positive as it av oids problems arising from ‘dilute and disperse’ or the ‘redistribution’ of exposures to persons living close to disposal sites. Such issues were seen as being very important in some European countries after the Chernobyl accident [8]. But ‘in situ’ treatment may also have negative side effects because it can complicate future waste removal. 3. NON DOSE-REDUCING REMEDIATION STRATEGIES For certain remediation measures, reduction in radiation dose need not be the only benefit, or even the main benefit. In the STRATEGY and EURANOS projects, a number of remediation measures were evaluated in which dose reduction was not the primary aim [7, 9]. These included measures such as: the provision of medical check-ups and dietary advice, the setting up of public information centres, the instigation of education programmes, compensation, the provision of counting equipment and the stimulation of stakeholder involvement in the decision-making process. Indeed, it is to be hoped that many of the procedures, specifically those directed towards communication and stakeholder involvement would be generic to any remediation process. Provision of counting equipment and independent monitoring are methods that have been successfully applied in Chernobyl affected communities. A study carried out Belarussian villages concluded that the approach not only resulted in reducing exposures with minimal social and psychological side effects, but was also more economically cost effective than the standard ‘top-down’ management procedures [11]. A recent stakeholder study following up on Norwegian farming communities most affected by Chernobyl fallout indicated that access 129 TOPICAL SESSION 5 to local food monitoring stations was particularly important [12]. Independent monitoring following waste disposal are commonly requested in community stakeholder processes. 4. CONCLUSION Any remediation strategy will be strengthened by an approach to remediation that integrates economic, ecological, and health measures; it is not sufficient to simply focus on the dose reduction aspects of radiation protection. This is supported by many multidisciplinary research projects on the long term management of radioactive contamination. The projects highlight the importance of including the affected populations with regard to self-help measures and involvement in decision-making processes. In addition to respecting people’s fundamental right to shape their own future, and thereby increasing trust and compliance, such approaches can lead to significant improvements in the effectiveness of remediation measures and in their acceptance by communities. REFERENCES [1] OUGHTON, D.H., et al., An ethical dimension to sustainable restoration and long term management of contaminated areas, J. Environ.Radioactivity 74 (2004) 171-183. [2] BAY, I., OUGHTON, D.H., Social and economic effects, In: Chernobyl, Catastrophe and Consequences (eds J. Smith and N.A. Beresford), Springer-Verlag, Berlin (2005)239-262. [3] INTERNATIONAL ATOMIC ENERGY AGENCY, Chernobyl’s Legacy: Health, Environmental and Socio-Economic Impacts, The Chernobyl Forum, IAEA, Vienna (2005). [4] UNITED NATIONS DEVELOPMENT PROGRAMME (UNDP), The Human Consequences of the Chernobyl Nuclear Accident - A Strategy for Recovery (2002). [5] INTERNATIONAL COMMISSION ON RADIOLOGICAL PROTECTION, Optimisation and decision making in radiological protection, Annals of the ICRP, Publication No. 55, Oxford, Pergamon Press (1989). [6] HOWARD, B.J., et al., Sustainable restoration and long term management of contaminated rural, urban and industrial ecosystems, Radioprotection - colloques 37 (C1) (2002) 1067–1072. [7] EUROPEAN COMMISSION, Generic handbook for assisting in the management of contaminated food production systems in Europe following a radiological emergency, Deliverable from the EURANOS Project, EURANOS(CAT1)-TN(06)-06 (2006). [8] NISBET, A.F., Management options for food production systems contaminated as a result of a nuclear accident, Radioprotection-Colloques, vol 37, C1 (2002) 115-120. [9] OUGHTON, D.H., BAY-LARSEN, I., VOIGHT, G., Social, Ethical, Environmental and Economic Aspects of Remediation, In: Radioactivity in the Environment, Volume 14 (2009) 428-451. [10] BULLARD, R.D., Dumping in Dixie: Race, Class and Environmental Quality. Westview Press, Boulder, CO (1990). [11] HERIARD DUBREUIL, G.F., et al., Chernobyl post-accident management: the ETHOS project, Health Physics 77 (1999) 361–372. [12] OUGHTON, D.H., et al., Long-term Rehabilitation of Contaminated Areas in Norway: Results of co-expertise meetings in Norway, Deliverable for the EURANOS project (CAT3)RT-08 (2008). 130 A GUIDE FOR THE REMEDIATION OF RADIOACTIVELY CONTAMINATED SITES: EURSSEM L.P.M. VAN VELZEN*, L. TEUNCKENS**, M. VASKO**, E. HAJKOVA***, V. DANISKA***, K. KRISTOFOVA*** * Nuclear Research and Consultancy Group, Arnhem, The Netherlands ** AF-Colenco AG, Baden, Switzerland *** Decom a.s., Trnava, Slovakia Abstract A first draft of EURSSEM (European Radiation Survey and Site Execution Manual) has been developed within the framework of the ‘Co-ordination Network on Decommissioning of Nuclear Installations’ project (2005-2008) funded by the European Community. The objective of EURSSEM is to provide a consensus approach and guidance to conduct all actions at radioactively contaminated and potentially radioactively contaminated sites and/or groundwater - up to their release for restricted or unrestricted (re)use. This approach and guidance is intended to be both scientifically rigorous and flexible enough to be applied to a diversity of site (surface) cleanup conditions. A brief description is given on the background and the need for a document such as EURSSEM, about key issues such as stakeholder involvement and archiving for future referencing, including the follow-up of the further development of EURSSEM. 1. INTRODUCTION The purpose of the Co-ordination Network on Decommissioning of Nuclear Installations (CND) was to organize and operate this Network with organizations from the European Union as well from candidate countries involved in decommissioning activities [1]. An important aim of the CND was to encourage a continuous improvement in capabilities and effectiveness that should lead to increased competitiveness. The CND was managed by a Steering Group that had the objective of driving the CND forward to increase and transfer knowledge and to exchange experience so that organizations could derive the maximum benefit from this EC funded project. One of the main topics/work packages in the CND was ‘Site Characterization, Remediation and Reuse’. The aim of this work package was to improve the exchange of knowledge between specialists and especially experts of the European Community in this field; it had the following objectives: – To promote common understanding of key issues in the fields of site characterization, remediation and reuse; – To identify good/best practices in characterization, remediation and reuse of sites based on practical experience and to disseminate good practice in areas that will benefit from a better characterization, remediation and reuse of sites; – To promote the exchange of information in these fields. 131 TOPICAL SESSION 5 The intention at the start of the project was that each of the three topics, e.g. site characterization, remediation and reuse could be dealt with separately. However, although a number of commercial firms had interests in these topics, and especially in the results and experiences of competitors, the same firms were reluctant to share their own experiences with others. For this reason, it was very difficult to demonstrate that participating in the CND project and in this working group had a real added value. Therefore, the Steering Committee of the CND decided to change course in order to meet the project objectives. This change of course meant that the effort would be made by a motivated group of partners to develop the intended guidance documents. This effort resulted in this first draft of EURSSEM. 2. DEVELOPMENT OF THE FIRST DRAFT OF EURSSEM 2.1. Purpose and scope The purpose of EURSSEM is to provide a consistent guideline for the execution of an environmental remediation programme for radioactively or potentially radioactively contaminated land and/or ground water. The guidance and approaches should be both scientifically rigorous and flexible enough to be applied for a diversity of sites (surfaces) and ground waters. 2.2. Point of departure The following points of departure were defined for the development of EURSSEM: (a) EURSSEM should be written from an advisory or a consultancy point of view. This means that EURSSEM can contain all existing information and information on future developments in approaches etc. that deal with the development, implementation and execution of an environmental remediation programme applying the best options and practices for a particular site. Due to the fact that the guidance is generic and no national or international regulations/laws are taken into account, the regulatory body in the country where it is used should be consulted. Further, it is evident that the advice given will not necessarily correspond with the viewpoint of a site owner, a regulator or a public community; (b) Commercial interest. The authors do not have any commercial intentions considering: (i) The use and the distribution of EURSSEM by third parties. It is evident that the use of EURSSEM is the responsibility of the user; (ii) The inclusion of commercial information, e.g. company names, specific commercial products, process, etc. in EURSSEM; (c) EURSSEM is available for all companies, regulators, members of the public (all stakeholders) involved in or interested in environmental remediation programmes; (d) The level of information provided in EURSSEM should be acceptable for an interested member of the public as well as for specialists in the field; (e) EURSSEM should be free from any judgement about preferred strategies, approaches, procedures, equipment that can be applied in an environmental remediation programme. 132 VAN VELZEN et al. 2.3. Need for a document such as EURSSEM Over the last decades, organizations like the International Atomic Energy Agency [2], the United States Interstate Technology and Regulatory Council (US-ITRC) [3], the Construction Industry Research and Information Association (CIRIA) [4], United Kingdom governmental agencies (Safety and Environmental Guidance for the Remediation of Contaminated Land on UK Nuclear and Defence Sites (Safegrounds Learning Network) [5]), US governmental agencies (Multi-IAEA Radiation Survey and Site Investigation Manual (MARSSIM) [6]), and various other national institutes, etc. have performed a substantial amount of work to improve knowledge and understanding of ‘best practices’ in an environmental remediation programme. EURSSEM incorporates information provided in documents prepared by the above-mentioned organizations and the importance and the quality of the information and know-how presented in their documents is acknowledged. However, this existing information was, until now, not combined into one consistent document or guideline. Independent of their origin (e.g. IAEA, US-ITRC, etc.), the available documents and guidelines have a kind of common structure: they present global information on all aspects that have to be considered in the design, planning and execution of an environmental remediation programme, although the level of the treatment can vary and, for specific aspects, very detailed information may presented. In Fig. 1, as an example, an overview of topics/documents is presented that can be found on the website of the US-ITRC. However, these documents are not combined into one consistent guide. FIG. 1. Overview of the document topics at the US-ITRC website [2]. Relevant documents for performing an environmental remediation programme have been prepared over a period of 10 to 15 years. During this time period: (a) Knowledge has increased; both theoretical and practical experience has been obtained; (b) Viewpoints and insights into the relevant science have changed; (c) During the preparation of these documents, a large number of authors/scientists from many fields of science were involved; 133 TOPICAL SESSION 5 (d) The level of the published documents is not always the same; (e) The applied terms and definitions have not always been consistent. As a result, it will be difficult for some stakeholders involved in an environmental remediation programme to judge the true merits of the advice. Therefore, combining the available information into one consistent guideline will be a help for all stakeholders. 2.4. Literature study An extensive literature study has been performed using internet and references in leading documents. All literature was sorted according to the different aspects of an environmental remediation programme. After sorting, emphasis was put on how to combine and re-edit the collected information to create an approach that is as consistent as possible for all aspects. The next step was to combine and re-edit the selected literature. The last step in the process was to perform a second literature study to fill in the gaps of missing information/examples and/or expanding the level of detail. Although a lot of work has been performed by the authors/editors, they do not claim that the information on all aspects of an environmental remediation programme is equal in depth or detail. 3. FIRST DRAFT OF EURSSEM 3.1. Use of the manual Potential users of this manual are companies, government agencies and other parties that can be described as stakeholders involved in processes to remediate or restore radioactively contaminated sites for restricted or unrestricted (re)use. The manual is intended for a technical as well as a non-technical audience. 3.2. Structure of the manual EURSSEM begins with guidance on how to decide if EURSSEM guidance or part(s) of EURSSEM guidance are applicable. It is followed by the section ‘Development of a contaminated land strategy’ which provides a clear context and objectives, as well as information about effective external participation (stakeholder involvement) whether it is required by organizational policy or by regulations to meet stakeholder expectations or to improve decision-making. This section focuses in detail on the strategy to be applied, describing two major topics, i.e. stakeholder involvement in the process and the requirements/establishment of an ‘archive for future referencing’. These two topics are linked to all actions in the process. The document provides guidelines for the formulation of all necessary plans at a generic level, e.g. historical site assessment, risk assessment approaches, a health physics plan, a safety and security plan, an environmental protection plan, waste management and transport, record keeping, etc. The ‘archive for future referencing’ has not to be seen as a special part of the project file, but as an archive that will contain information that can be consulted in the short term and the long term future for answering questions concerned with former radioactive contaminants present at the site and/or in the groundwater. In the next section, the focus is on the radiological characterization of a site and on the processes involved in doing this, e.g. the design of field-based site characterization, determining the radioactive contaminants and their behaviour, sampling, sampling frequencies/locations/patterns, intrusive and non-intrusive methods, field and laboratory equipment, analysis of samples, data interpretation, reporting, common mistakes, etc. and 134 VAN VELZEN et al. how to decide if the data obtained meet the remediation or the release criteria to an acceptable degree of uncertainty. Remediation and post-remediation activities (restoration) guidelines are presented in the next section. These guidelines are focused on the design of a remediation plan that can be accomplished safely. Different planning approaches are described, but also, guidance is given on criteria for the evaluation of an approach or technique. Further, an extensive overview is given of available remediation techniques presented in literature, guidance on the selection of applicable remediation techniques as well as on implementing remediation and postremediation (restoration) actions. 135 TOPICAL SESSION 5 1. Decide whether EURSSEM guidance or part(s) of EURSSEM guidance applies Stakeholder involvement 2. Develop contaminated land strategy Context and objectives Stakeholder involvement Historical site assessment Preliminary risk assessment Formulate plans o Health physics, safety, security and environmental protection plan o Site characterisation o Remediation o Waste management plan o Stewardship o Record keeping o Quality assurance and quality control Assessment criteria for short term and long term land use Archive for future referencing Archive for future referencing 3. Characterisation of radioactively contaminated sites and/or groundwater Measurements of site and/or groundwater specific data on the levels and distribution of residual contamination and background Decide whether data obtained meet the remediation or release criteria within an acceptable degree of uncertainty 4. Environmental remediation Strategy for environmental remediation and objectives Develop a remediation plan that can be accomplished safely Selection of applicable remediation technologies Implementing remediation activities Disposal of waste Conducting post-remediation activities 5. Stewardship Decide if short term or long term stewardship has to be implemented Establish short term or long term management strategy for whole a site or part of a site and priorities for specific areas Establish most appropriate management option for each contaminated area FIG. 2. The five interrelated parts of EURSSEM. (For simplicity, in Fig. 2 the iterative issue has been omitted). The last section provides information and guidelines on ‘Reuse and Stewardship’. It is evident that not all radiological contaminated sites and/or groundwater can be cleaned and released for unrestricted use within an acceptable time scale. Sometimes, this is not needed, 136 VAN VELZEN et al. for example, for industrial areas. Therefore, guidance is given on decision making and the implementation of short term or long term stewardship. EURSSEM is presented in a modular format, with each module containing guidance on conducting specific aspects of, or activities related to the process. If followed in the related order, each module leads to the generation and the implementation of a complete plan. Where appropriate, examples and/or checklists are included that condense and summarize the major points in the process. The checklists may be used to verify that every suggested step is followed or to flag a condition in which specific documentation should be provided to explain why a step was not needed. A schematic overview of the content of the first draft of EURSSEM is presented in Fig. 2. 4. FUTURE WORK At this moment EURSSEM is available at http://www.eurssem.eu/. The authors/editors are looking forward to working with other specialists, companies and institutes to update this draft at regular time intervals. It is intended that the website will become a forum where specialists and non-specialists can exchange information. The website will also offer the opportunity to upload improvements and new information. These improvements and information will be reviewed and if they contain material with an added value, it will be incorporated into the next version of EURSSEM. In the future, EURSSEM will be extended by including an appendix containing abstracts of published articles dealing with cases or aspects of environmental remediation. 5. CONCLUSION By creating EURSSEM, a gap and a need is being filled so that the design, implementation and execution of environmental remediation programmes can be performed according to the latest approaches, techniques, etc. By making EURSSEM available to everyone via the internet and in combination with a forum, EURSSEM can contribute to a better understanding of environmental remediation programmes and to the harmonization of approaches. REFERENCES [1] [2] [3] [4] [5] [6] TEUNCKENS, L., Co-ordination Network on Decommissioning of Nuclear Installations; 3rd Annual Report (2008). http://www.iaea.org/ http://www.itrcweb.org/gd.asp http://www.ciria.org/index.html http://www.safegrounds.com/index.html http://www.marssim.com 137 IMPROVING RADIOACTIVE WASTE AND SOURCE MANAGEMENT AT THE VINČA INSTITUTE M. RECIO, J. KELLY, M. KINKER International Atomic Energy Agency, Vienna Abstract The Vinča Institute Decommissioning Project (VIND) represents the largest project in the history of the Technical Cooperation Programme of the International Atomic Energy Agency. Its scope is subdivided into three tasks: (1) spent fuel repatriation to the country of origin, (2) waste management, and (3) decommissioning of the RA research reactor and associated facilities. One major project involves the dismantling and decommissioning of old waste management facilities, along with processing of the waste and conditioning of the sealed sources stored in those facilities. This paper describes the progress made and problems encountered in implementing the waste management and decommissioning projects. 1. INTRODUCTION The Vinča Institute of Nuclear Sciences (referred to as the ‘Vinča Institute’) is located within 20 km of Belgrade, Serbia, which has a population of approximately 2 million people. The Vinča Institute was built in the mid-1950s to provide nuclear research services to the former government of Yugoslavia. Two research reactors were established: a research reactor for high power irradiation services for a variety of experiments (the RA reactor), and a zero power research reactor to provide criticality research data (RB reactor). 2. BACKGROUND The RA reactor, which is a 6.5 MWt, tank-type, heavy water moderated and cooled research reactor containing highly enriched uranium (HEU) and low enriched uranium (LEU) fuel of Russian origin, began operations in 1959 and was ‘temporarily’ shut down in 1984 but was never restarted. This was linked to the severe economic crisis in Serbia during the same period. In 2004, a programme was instituted by a decision of the Serbian Government to begin decommissioning activities at the RA reactor and associated nuclear facilities at the Vinča Institute. This decision resulted in the establishment of the Vinča Institute Nuclear Decommissioning (VIND) Programme to decommission the nuclear facilities at the Vinča Institute. The Programme has attracted support from a number of organizations, including the Serbian Ministry of Science and Technological Development, the United States Department of Energy, the European Commission (EC), the Slovenian Nuclear Safety Administration, the Czech Republic, private donors (e.g. the Nuclear Threat Initiative) and the International Atomic Energy Agency. For the IAEA, the project represents the largest project in the history of the IAEA’s Technical Cooperation Programme. The VIND Programme began in 2004 and will continue until at least 2011, and is forecast to cost as much as US $75 million dollars (US) to conduct and complete all planned activities. 3. VIND PROGRAMME The VIND Programme consists of three major tasks: (1) Spent fuel repatriation to the country of origin; 139 TOPICAL SESSION 5 (2) Decommissioning of the RA research reactor and associated facilities; and (3) Radioactive waste management. Task 1 (spent fuel repatriation project) is part of a United States, Russian Federation, and IAEA co-operation under the Russian Research Reactor Fuel Return programme. Nonirradiated (fresh) fuel was repatriated in 2002 and the repackaging of spent fuel will begin in August 2009. Preparations for the transport of the spent fuel are currently on schedule, and transport activities are scheduled to be completed by the end of 2010. Task 2 decommissioning activities are also on schedule; the draft decommissioning plan has been completed, 90% of the excess/abandoned materials have been removed, and physical dismantlement of related facilities (e.g. old waste hangars) is scheduled to begin in 2010. However, additional storage capacity is needed for the waste generated during the fuel repatriation and decommissioning. Task 3 focuses on improving radioactive waste management at the Vinča Institute. The Serbian government and international donors (USA, Nuclear Threat Initiative, UK, and Slovenia) are supporting the construction of new waste storage and processing facilities. The EC is contributing to this project by funding the procurement of equipment for the new facilities, including waste containers for the spent nuclear fuel repatriation project and other decommissioning projects. Currently, solid RAW from the entire former Yugoslavia is being stored in storage Hangars 1 and 2 - both of which are in a poor condition. The stored waste comprises several hundred drums of unconditioned and uncharacterized waste that includes yellow cake, metallic uranium, hundreds of high radiation dose-rate disused radioactive sources, and thousands of excess and disused sealed sources, many of which are of IAEA Hazard Category 1 and 2. Liquid transuranic waste is stored in four underground tanks. None of the waste inside Hanger 1 is properly characterized or packaged in accordance with international standards. In order to support the VIND radioactive waste management activities, three new facilities have been built and are expected to be operational in 2009: they comprise a new Waste Storage Facility (WSF), a Secure Storage Bunker, and a new Waste Processing Facility (WPF). In addition, a former isotope production facility is in the process of being upgraded for use as a Source Conditioning Facility (SCF). Progress on this project is dependent upon completion of construction of the new waste storage facility (WSF) and the associated waste processing facility (WPF). Significant progress has been made towards facility construction, and several of the major equipment items have been purchased. Each of these facilities is scheduled to be in start-up mode at the beginning of the waste management work; therefore, in addition to the requirements for facility licenses and Final Safety Analysis Reports (FSAR), Vinča will also need developed operational strategies, production schedules, safety and security strategies, and staff training. In 2008, the EC began its contribution to supporting specific waste management activities under Tasks 2 and 3 above, with a focus on resolving long term waste management issues. These comprise the decommissioning and dismantlement of the old waste storage facilities, along with the processing of the associated waste and the conditioning of the sealed sources stored in those facilities. The projects will be jointly managed and implemented by the Vinča Institute and the IAEA. 4. IAEA CONTRACTING APPROACH The Vinča Institute does not have sufficient staffing or experience to implement all of the projects under the VIND Programme within the objective timeframes. The Vinča Institute also lacks clear operational/safety and security strategies and schedules for implementing non140 RECIO et al. fuel projects. Therefore, additional staff with specific expertise will be needed to support the start-up and early operation of the new waste processing and storage facilities; the dismantling and/or decontamination and decommissioning of the old waste storage facilities; the training of Serbian technicians, and to ensure that all programme activities are being performed in a safe and professional manner consistent with the applicable procedures, regulations, international standards, and best practices. For this reason, it was decided that external contractors with expertise and experience in these areas would be hired. IAEA contracting therefore focused on augmenting Vinča capabilities in these areas. The projects were expected to begin in early 2009. In order to reach this objective, three primary areas of preparatory activities were identified to achieve the work and funding schedules: Consolidation and Coordination of Contracts and Inputs, EC Contribution Agreements and Financial Assistance Agreement, and Procurement. Initial contract specifications were developed from the original 2009–2011 VIND Programme Design. An expert panel met in October 2008 in order to develop detailed technical specifications and bidder evaluation criteria. The expert panel further consolidated the specifications and developed them into detailed technical specifications for 12 service contracts. These contracts were further revised to incorporate new guidance from the IAEA Office of Procurement Services, and, as a result, two service contracts were developed: (1) to provide radiation protection services for overall waste management work, and (2) to perform much of the site characterization, waste removal and dismantling and decommissioning of the old waste storage Hangers 1 and 2, source conditioning, and waste processing and storage in new waste facilities recently constructed at the Vinča Institute. The Request for Proposal (RFP) packages were sent to over 20 companies which had international experience in RAW and sealed source management. The outcome of the bidding process was disappointing. Only a single bid was received for the radiation safety service RFP within the specified timeframe. No bids were received for the waste management service RFP. A technical evaluation was performed on the single bid received in order to determine whether it met the technical requirements identified in the bidder requirements, and to provide recommendations for future submittals of this RFP. The expert panel concluded its evaluation of the bid with the determination that the single received bid was not of sufficient quality or detail to justify an award. The panel also recommended that the RFPs be revised to take account of the bidder’s recommendations. After discussions with other potential bidders, the expert panel identified a number of factors resulting in their failure to produce bids. These factors, which include available human and financial resources, international teaming arrangements, manpower qualification, etc., will need to be taken into consideration for future bidding processes. 5. CONCLUDING REMARKS Currently, the IAEA is working with EC and the Serbian Ministry to restructure the VIND projects, resulting in some activities being deleted, and most or all activities being postponed to late 2010 or early 2011. This is being driven by two factors: (1) the continuous delays in construction and commissioning of the waste management facilities and the source conditioning facility, and (2) the need to ensure adequate funding for spent fuel repatriation activities, all of which are critical to the new projects. As the IAEA begins the process of reevaluating the VIND Project contracts, it is likely that the waste management and decommissioning activities will need to be re-evaluated, with priority being given to ‘incremental decommissioning’ of the old waste storage Hangers 1 and 2, underground liquid waste tanks, spent fuel storage pool, reactor hot cells, and the RA reactor structure. Other VIND waste management and radiological infrastructure activities, including waste and source management activities, the Orphan Source Search and Recovery programme, a site141 TOPICAL SESSION 5 wide radiological assessment, and upgrades to the radiation protection and emergency response facilities, will be given a lower priority. 142 SUMMARY OF SESSION 5 M. Paul Germany LIFE CYCLE PLANNING AND STAKEHOLDER ISSUES This session consisted of eight presentations and dealt with two important topics in environmental remediation: life cycle planning and stakeholder issues. One general concern expressed in this session was that the upsurge in nuclear power plant building will lead to new demands for uranium and a ‘new wave’ of uranium exploration and extraction. It is vital that lessons should be learnt from the past and that new legacy sites should not be created. A working group that involves experts from different disciplines has been established in France. Its purpose is to provide an appraisal of the residual environmental situation after the completion of remediation works at a former uranium production centre. The participation of international organizations in the activities of this group adds value to its outcome and reassures the public of the credibility its findings and reports. Adaptations of this working methodology could be usefully considered in other countries in order to improve the process of stakeholder involvement in decision making on environmental remediation programmes. A negative aspect that was discussed during the presentation is that, in order to be effective, the work of this group has involved several meetings leading to an intense agenda. An approach to quantitatively assess the environmental impacts of any industrial activity throughout its entire life-cycle was described. This approach allows the identification of potential opportunities for improving operations so that there are reductions in material and energy consumption as well as reductions in discharges to the environment; it also integrates the idea of considering environmental remediation as part of the whole life cycle of the operation. In another presentation dealing with life cycle management, it was stressed that to ensure a low environmental impact and to minimize possible remediation costs arising after operations cease, new uranium mine developments should follow a ‘whole-of-life mining cycle approach’. Through this approach, the need for post-operation remediation can be minimized by effective planning at the design and operational stages. In developed uranium producing countries, the appropriate involvement of stakeholders, such as neighbouring communities, public representatives, independent scientists and non-governmental organizations (NGOs), is very much in the interest of the operators of uranium mines or implementers of remediation projects. Companies need to obtain the support of the public to receive - in addition to the regulatory licences and permits - a ‘social licence’ from the local community and district in which the project is being operated. Environmental remediation was addressed from the point of view of project management - based on the experiences of the US Department of Energy (DOE), although the experience presented is useful for all environmental remediation programme implementers and managers. In the past, insufficient project management at DOE led to inefficiency and a waste of money. Nowadays, the DOE uses well established protocols for environmental remediation project management. The work done is accurately measured and accounted for so as to avoid unnecessary expenditures. It was emphasized that the participation and integration of regulators in project management is essential to guarantee the success of the project implementation. Environmental remediation was also assessed from the ethical point of view. One key element is that the people involved in presenting the different issues related to environmental remediation must use credible and accurate information and numbers. If the wrong figures are 143 SUMMARY OF SESSION 5 used it can promote confusion and distrust; this can ultimately turn the process against the interests of the population that should be the beneficiaries of the environmental remediation project. This occurred after the Chernobyl accident where misinformation led to many undesirable decisions and unnecessary fear. It was suggested that ethical evaluation can aid in structuring decision making in environmental remediation. A scheme to guide the implementation of environmental remediation projects called EURSSEM was presented. This will be released for free use on the internet by the end of September 2009 and it is expected become an important tool to aid in the structuring of environmental remediation projects. An assessment, by a team of international experts of the radiological situation in the desert environment of Algeria, where nuclear weapons testing was conducted by the Government of France in the 1960s, was described. The tests were conducted above ground and in mountain caverns. Remediation of the affected areas was carried out after the testing period ended. The expert team was able to detect evidence of the testing but, when the habits of the sparse local population were taken into account, the assessed potential radiation doses were very small. A full report of the assessment is published in the IAEA’s Radiological Assessment Reports Series. The final presentation addressed the issues that can make it difficult when international organizations like the IAEA give assistance to countries. A case study concerned the decommissioning of the Vinca nuclear research institute facilities in Serbia. Constraints in the bidding process, problems with employing local manpower and the difficulties that companies face when taking jobs outside Western Europe were some of the issues that had to be faced. 144 CASE STUDIES (ENVIRONMENTAL REMEDIATION IN CENTRAL ASIAN COUNTRIES) (TOPICAL SESSION 6) Chairperson A. KIM Kazakhstan ENVIRONMENTAL EFFECTS OF POSSIBLE LANDSLIDES IN THE AREAS OF RADIOACTIVE WASTE STORAGE IN KYRGYZSTAN I.A. TORGOEV, Y.G. ALESHIN, G.E. ASHIROV Institute of Physics and Rock Mechanics of the National Academy of Sciences, Kyrgyzstan Abstract This paper describes the problems caused by the location of uranium mine and mill tailings in the mountainous regions of Kyrgyzstan which are subject to potentially disrupting natural events such as landslides and flooding. It describes the modelling analyses which have been carried out to provide an improved predictive capability of potential future events, On the basis of these analyses, strategies have been developed to avoid some of the worst consequences of the natural events. 1. LANDSLIDE GEOENVIRONMENTAL HAZARDS IN MAILUU-SUU A former large industrial mining complex was located in the Mailuu-Suu area of the north-eastern foothills of the Fergana depression (Fig. 1). Landslide activity in this unstable geological environment has been enhanced by the mining operations (uranium, coal, oil) and associated infrastructure developments in the area. Kazakhstan Uzbekistan China Fergana valley FIG. 1. Map of landslide susceptibility in Kyrgyzstan. Landslides occur most frequently (98%) in the mid-stream of the Mailuu-Suu River (Fig. 2), in a band of mid-mountain (900–1600 m) topography, on a propagation zone of Meso-Neozoic sediments strongly crushed in folds, which, due to their lithologic (presence of loess-like loams and clays) and stratigraphic (alternation of water-permeable and waterproof soils) features, are predisposed to slumping. Hence, the presence within the study area of both ancient and new folded and disjunctive structures of various kinds, high geodynamic regional activity conditioned by the meridional compression of Tien-Shan, and the wide propagation of old landslides have caused the active development of new landslides, of which 50% are confined to slopes of ancient origin. 147 TOPICAL SESSION 6 FIG. 2. Landslides and tailings in Mailuu-Suu valley. At the present time in this area, more than 200 new landslides of various scales, ages, and development stages have been registered. Based on the situation at the beginning of 2008, the whole area affected by landslides is estimated to be 6.37 km2, and the total volume of landslide masses moved during 1950–2005 is 260 000 000 m3. More than 30 landslides are in a ‘preparation stage’, before the main movement, and they pose a direct danger to the population and to building structures, roads etc. as well as to stored radioactive waste tailings. Due to a deficit of suitable and available areas, housing estates, roads and industrial structures, including radioactive waste tailings (tailing dumps and stockpiles), were placed along riverbeds, in floodplains and over-floodplain terraces of the Mailuu-Suu river and its tributaries, on mountain foothills and/or on the slopes themselves, as well as on weakly stable old landslide sites (Fig. 2). For these reasons, landslides represent a source of great risk for Mailuu-Suu town. The landslides, which are formed on the edges of the river valley and its tributaries (Fig. 2), are the most hazardous because their development, and, particularly their final stage, often has a synergetic character (domino effect). Landslide events in narrow river valleys can trigger a series of other hazardous phenomena by the following scenario: landslide rockslide-landslide blockage of riverbed or river valley - landslide dam upstream submergence - breach of this dam - downstream flood or mudflow. During the last 17 years in the Mailuu-Suu area, more than 10 landslide movement episodes involving the blockage of a river and its tributaries have been registered. The most destructive of them was a river blockage in the Tektonik landslide zone in June 1992, when, as a result of landslide mass movement, a dam of 15 m height and 800 m length was formed and simultaneously a smallsized mine tailing storage (No 17) was pushed into the river. A special hazard of such synergetic scenarios can be their effects on tailings and dumps of radioactive waste located along riverbeds of the Mailuu-Suu, Karagach and Kulmen-Sai (Fig. 2). In such cases, the propagation area of the radioactive materials stored in them may be substantially expanded owing to their transfer through the drainage network of the MailuuSuu river to the Syrdarya river basin. The environmental risks related to the destruction of tailings stores as a result of the direct fall of landslide masses have been assessed [1]. The risks associated with tailings store submergence after dam breach and mud-flow effects are significant, taking into account a series of previous incidents in the study area [2]. In April 1958, following the No 7 tailing 148 TORGOEV et al. dam destruction triggered by extremely heavy rainfall and increased seismic activity in the nearest zone (R < 100 km), the mass of radioactive tailings, with a volume of 400–600 thousand m3, burst from this tailings dam, was propagated as a mudflow with 250m3/s water discharge downstream into the Mailuu-Suu river, causing the destruction of some civil and industrial structures and the radioactive contamination of a river bed, a floodplain and the valley train of the river, including some areas in Uzbekistan. At the present time, the largest risk is at the site of the vast (V > 5-7 million m3) Koitash landslide (Fig. 2). In the case of a river valley blockage during the simultaneous unloading of this landslide, a dam of 15–25 m height may be formed, and the weakly stable tailings Nos 5 and 7 with a total volume about 800 thousand m3, may be enclosed within this submergence zone. The largest submergence risk is in the spring season and at the beginning of summer, when water discharge to the Mailuu-Suu river (at the crest segment) may reach 100 m3/s. The computation shows that, based on the most pessimistic scenario - absolute destruction of tailings Nos 3, 5, 7, 8, 18 (Fig. 2) through the direct or indirect influence of Tektonik and Koitash landslides - the total volume of radioactive tailings which may be dispersed on the flood-plain and on the debris cone of the river, may be approximately 1 million m3 (total activity is about 1014 Bq). In order to reduce the risk of uranium tailings landslide destruction at Mailuu-Suu, it is planned, during the next 2–3 years, to introduce a series of preventive measures and projects, including the southern flank unloading of the Tektonik landslide, the transportation of Nos 3 and 8 tailings to a safer zone, a bypass tunnel construction on a site of possible river blockage by the Koitash landslide, as well as the provision of monitoring and an early warning system for landslide hazards in the area of the uranium tailings. 2. GEOENVIRONMENTAL RISKS IN MIN-KUSH SETTLEMENT Within the last years, an emergency situation has arisen in the area of the Tuyuk-Syy uranium tailings store located directly in a river-bed (Fig. 3) linked to the Naryn river basin (Syrdarya). These tailings are at a height of more than 2000 m above sea level, and they occupy a 5 hectare zone, in which 640 000 m3 of Kavak uranium tailing waste, including 450 000 m3 of radioactive tailings, have been concentrated. FIG. 3. View of the tailings and landslide in valley of river Tuyuk-Suu. Based on the results of a comparative risk analysis of the Tuyk-Syy tailings, it is considered that, at the present time, the greatest risk is associated with the destruction of the supporting dam and the by-pass channel. This could happen if mudflows passed through it following a landslide event. Such a landslide began to develop during the moisture-abundant 149 TOPICAL SESSION 6 spring of 2004 on the right hand side of a narrow valley 120–150 m lower than the study tailing area (Fig 3). FIG. 4. Modelling results of a landslide blockage of the river in the lower part of the TuyukSu tailings. The development of this landslide movement, predicted to occur during Spring 2009, would be dominated by blockage of this narrow valley with a landslide dam, of height, according to calculations, of more than 30 m over the Tuyuk-Suu river bottom (Fig. 4). An under-pond lake would be created with a volume of more than 500 000 m3 which would lead to tailings submergence. The results of a stability assessment of the lower supporting radioactive waste dam showed that, due to water saturation of the tailings body, the stability factor is rather low even without taking into consideration the submergence and/or dynamic forces from possible earthquakes. In the case of the unexpected breaking of the dam due to landslides, an outburst flow (wave) with an initial water discharge up to 600 m3/s capturing and entraining radioactive tailings in its movement, could occur. In the final analysis, there is a high probability of, not only the destruction of the Min-Kush settlement housing located in the adjoining zone of the Tuyuk-Suu river outfall, but of the subsequent extensive contamination of Min-Kush, Kokomeren, Naryn riverbeds and flood-plains by radioactive waste. As preventive measures, landslide movement monitoring is being carried out and special arrangements have been planned for the controlled water discharge in the case of river blockage by landslide masses. The longer-term plan is to transfer the Tyuk-Suu tailings to the safer zone adjoining the Min-Kush settlement. 3. CONCLUSIONS The high probability of hydrodynamic accidents and environmental catastrophes of both regional and transboundary character in storage areas for radioactive and toxic mining waste in Mailuu-Suu, Min-Kush and other areas of Central Asia is mainly due to the fact by that these waste stores are located in the influence zones of hazardous geological processes (earthquakes, landslides, avalanches, mudflows), which are typical for the geodynamic active mountain areas of Tien-Shan. During the designing and building of these stores planners did not take into consideration the specificity of the mountain region with high geodynamic activity, the weak geomechanical stability of mountain slopes when influenced by anthropogenic activities, the 150 TORGOEV et al. propagation of hazardous natural processes and phenomena in mountain areas and the high environmental vulnerability of mountain zones to climate changes. The short-sighted engineering decisions made during the storage of radioactive and toxic waste in catchment areas in narrow river valleys and on slopes with landslide hazards have, after 40–50 years, led to the transformation of local landslide hazards into regional and transboundary health and environmental risks associated with radioactive contamination. REFERENCES [1] [2] TORGOEV, I.A., ALESHIN, Y.G., MELESHKO, A.V., et al., Hazard Mitigation for Landslide Dams in Mailuu-Suu Valley (Kyrgyzstan), Italian Journal of Engineering Geology and Environment, Special Issue on Security of Natural and Artificial Rockslides Dams, NATO ARW, Bishkek (Kyrgyzstan) (2004) 99–102. TORGOEV, I., ALESHIN, Y., KOVALENKO, D., et al., Risk assessment of emergency situation initiation in the uranium tailings of Kyrgyzstan, Uranium in the Environment, Springer Verlag (2006) 563–570. 151 THE RADIOLOGICAL AND ENVIRONMENTAL SITUATION NEAR TO THE DECOMMISSIONED URANIUM MINES IN UZBEKISTAN E.A. DANILOVA*, A.A. KIST*, R.I. RADYUK*, G.A. RADYUK*, U.S. SALIKHBAEV*, P. STEGNAR**, A. VASIDOV*, A.A. ZHURAVLEV* * Institute of Nuclear Physics, Tashkent, Uzbekistan ** Jozef Stefan Institute, Ljubljana, Slovenia Abstract Uzbekistan is an important producer of uranium. There are several operational as well as decommissioned uranium production enterprises in Uzbekistan which lack appropriate strategies for remediation, mainly due to the unavailability of the necessary information. Their remediation is complicated because many of the mining and tailing sites are located in mountainous areas and in the vicinity of rivers (which are potential drinking water supplies). Many of the tailings sites are endangered by possible mudflows. Radioactivity measurements have been carried out in the vicinity of several of the decommissioned mining and tailing sites, such as Yangiabad, Chorkesar and Krasnogorsk. Outdoor and indoor radon levels have been measured and the results obtained have been used for radiation dose assessment purposes. In addition, the concentrations of radionuclides have been determined in soil, water and foodstuff specimens collected near to the decommissioned mining and milling sites. The results obtained have been used for a preliminary radiological and environmental assessment as a basis for establishing an appropriate strategy for remediation. 1. INTRODUCTION Uzbekistan, along with other Central Asian Republics, is a significant producer of uranium. As a result of uranium mining in the past, there are dumps of tailings and rocks which contain radioactive and toxic elements. In many cases, the dumps are located in mountain areas near to rivers, which are sources of water for the population. Many of the dumps are endangered by periodic mudflows which may transfer materials into the rivers. All of these conditions create environmental and potential health problems, since the local population obtains its livelihood from agriculture in the neighbourhood of the tailings piles. For these reasons, there is a need to carry out radiological examinations in such territories with the purpose of estimating the risk to the public and, if necessary, developing strategies for health protection and environmental remediation. It is noted that this problem is very important for all countries of the Central Asian region because of the commonality of climate and hydrosphere and because of the exchange of foodstuffs between them. Some mines are close to the Uzbekistan border. For example, one of the largest decommissioned mines in Kyrgyzstan is only 8 km from the Uzbekistan border and the potential hazard to local populations in Kyrgyzstan is likely to be greater than to those in Uzbekistan. Fig. 1 shows the location of mines in Uzbekistan and their proximity to country borders. 2. ENVIRONMENTAL MONITORING Environmental monitoring missions have been carried out to measure gamma dose rates, indoor and outdoor concentrations of radon (Radon-222) in air, and to collect samples of water, soil and foodstuffs in the areas of the former uranium mines. Measurements were carried out in Yangiabad (Tashkent district), Krasnogorsk (Tashkent district) and Chorkesar (Namangan district in Fergana valley). 153 TOPICAL SESSION 6 FIG. 1. Uranium mines in Uzbekistan and mines close to the state border. The village of Yangiabad is situated 140 km from the capital of Uzbekistan, Tashkent. The territory of Yangiabad is about 77 hectares in area. In the village there is a municipal hospital, a kindergarten, a children’s day nursery, a school, private houses and other buildings. The buildings of the village were built in the 1950s using mainly imported materials; only some of the buildings were built using local raw materials (some of the building material may have been taken from the vicinity of the local mine). Close to the village is the mining and milling site. In the neighbouring area are radioactive waste deposits from mining covering an area of 50 km2. The total amount of radioactive waste is about 500 000 m3. The gamma radiation dose rates in the polluted areas are in the range 0.60 to 2.0 Sv/h. The village of Chorkesar is situated 20 km from the regional centre Pap of the Namangan district (Fergana valley). There are schools, a kindergarten, a hospital and other buildings. This village is very close to two decommissioned uranium mines, Chorkesar-1 and Chorkesar-2. Uranium was produced using mining and underground leaching techniques to depths of 280 m. The radioactive waste is stored in dumps covered with soil which, in places, has been washed away by rainfall. The total activity of the radionuclides in the waste dump is estimated to be 3х1013 Bq. The total volume of the tailings is estimated to be 480 000m3 deposited on an area of 206 000m2. There are three large tailing sites and one open cast site. They are separated from the local settlement by a 1m stone fence. However, the fence is damaged in several places and access to the territory of the mine is possible for the local population and cattle. Radiation dose rates here are in the range 3.0–4.5 Sv/h. Underground water flows from several of the mines. This water contains high concentrations of uranium, radium and radon and may be used by inhabitants and livestock. 154 DANILOVA et al. The village of Krasnogorsk (14 000 inhabitants) is situated at 40 km from Tashkent. There are three tailing sites near to the village. Radiation monitoring has been carried out in this area, doses to the local population have been estimated and the natural radiation background of the area has been measured. Measurements have been made of radon (by active and passive methods), gamma radiation (dose rate and gamma spectra), and environmental samples have been taken for analysis. 3. RADON MEASUREMENTS The elevated concentration of radon-222 is correlated with the content of uranium in rocks. Sources of radon can be soils, water, mining and mill tailings, ores, and building materials. The hazard to the health of the population is connected not only to the level of radiation dose received but also to the duration of the exposure and the age of the exposed population. The risk of development of a cancer from radon decreases with age, and for smokers this hazard is increased by about 10 times [1, 2]. The indoor levels of radon in air were measured in the 30 most frequently visited buildings (school, kindergartens, first-aid post, hospital, magistrates office, living houses, etc.) in Yangiabad, in 5 rooms in Krasnogorsk and in 18 similar premises in Chorkesar. The concentration of radon in Yangiabad was in the range 70–350 Bq/m3 (the average was 200 Bq/m3). Significantly elevated levels were found in buildings constructed from local materials (up to 770 Bq/m 3). The concentration of radon in Krasnogorsk was in the range 30-100 Bq/m3. In Chorkesar, the concentrations of radon were in the range 80–390 Bq/m3 (average 250 Bq/m3). High levels were found in two premises (670 and 1410 Bq/m3). According to national regulations, the average annual concentration of radon in the air of inhabited rooms should not exceed 80 Bq/m3 [3]. The effective annual exposure doses of the population were calculated. In Yangiabad, the effective dose was found 0.9–4.0 mSv/y (average 3 mSv/y) and for two rooms with high concentrations of radon it was 5.4 and 19.2 mSv/y. This means that in Yangiabad, the effective annual exposure dose does not exceed the permissible value, except for the occupants of the two rooms. In Krasnogorsk, the effective dose was 0.6–2.3 mSv/y. In Chorkesar, the effective dose was 2.0–6.5 mSv/y (average 4.5 mSv/y). In three rooms it was 8.7, 8.8 and 13.5 mSv/y. Gamma dose rates were also measured in the same premises. In Yanghiabad they were 0.2–0.4 Sv/h, in Krasnogorsk 0.15–0.27 Sv/h. and in Chorkesar 0.3–0.75 Sv/h. 4. RADIONUCLIDES IN WATER AND SOIL In the Chorkesar area there are leakages of water from mine drifts close to the village. Water samples (5 L) were taken from this area. To prevent sorption of elements on the walls of flasks, the samples were acidified using high purity nitric acid. Samples of soil (1 kg) were dried, milled, sieved and averaged by quartering. In water taken from the mine shaft, the following levels were found: Pb-214 - 5.2 Bq/kg, Bi-214 - 4.0 Bq/kg and Ra-226 – 2.7 Bq/kg. The concentration of radium-226 exceeds the permissible value (0.5 Bq/kg) by about 5 times [3]. The concentrations of radionuclides in soil taken from the area where there is leakage of water from shaft are given in Table 1. 155 TOPICAL SESSION 6 TABLE 1. RADIONUCLIDE CONTENTS OF SOIL (BQ/KG) Nuclide Tl-208 Pb-212 Bi-212 Pb-214 Bi-214 Ra-226 Concn. 349 1100 1200 4900 4600 62 800 Nuclide Th-234 U-235 Pa-234m Ra-223 Pb-210 Conc. 22 100 2700 73 600 3900 15 000 These data show that the soil is contaminated and that remediation or removal and burying of the soil is necessary. 5. FOODSTUFFS Some foodstuffs are produced in contaminated areas near to decommissioned mines (fruit, vegetables, meat, milk, etc.). To study this problem, the typical daily diet in Yangiabad and Chorkesar was determined. It was observed that the foodstuffs: milk, bread, flour, pancakes, pasta, carrots, fruits, tomatoes, beet, radish, onion, cabbage, meat, water, were bought in local shops and markets (bazaars). A model daily diet was prepared. The diet was analyzed using gamma spectrometry and neutron activation analysis. The daily radionuclide intake is given in the Table 2. TABLE 2. DAILY INTAKE OF RADIONUCLIDES WITH FOODSTUFFS (BQ) Nuclide 40 К 226 Ra 238 U Yangiabad 140 ± 17 < 1.0 < 2.0 Krasnogorsk 270 ± 17 < 1.0 <1.0 Chorkesar 133 ± 15 19 ±3 12 ± 8.04 In Chorkesar, the intake of radium-226 and uranium-238 with foodstuffs is significantly higher than in Yangiabad and Krasnogorsk. 6. CONCLUSION – The results obtained show that the decommissioned mines have a serious impact on the environment and possibly on the health of the local inhabitants; – The results show that the elaboration of a strategy for the remediation of the territories is needed as well as some additional studies; – It is also necessary to carry out a more complete estimation of the concentrations and of the behaviour of radionuclides and toxic elements in the environment of the decommissioned mines and to compare the data obtained with health statistics data; – It is necessary to carry out measurement and assessment studies over wider areas because of the long transport distances of the radioactive and toxic elements; – Additional useful information may be obtained by analyzing additional types of samples, including bottom sediments, airborne particles, human bio substrates (human hair); etc. – For a more complete estimation of the hazard it would be interesting to study experimentally the leaching of the radioactive and toxic elements from waste by the river water to obtain a better indication of the consequences of transport of the tailings into rivers by mudflows; 156 DANILOVA et al. – It is important to promote, possibly through international projects, the wider exchange of results obtained among Central Asian countries because of the similarity of conditions and the interconnection of transport media (e.g. rivers). REFERENCES [1] [2] [3] POLKA, J., Health Risks of Radon are given a New Look, NatureV.331 6152 (1988) 107. CASTRÉN, O., Strategies to Reduce Exposure to Indoor Radon, Radiation Protection Dosimetry 24 1–4 (1988) 487-490. SANITARY NORMS AND REGULATIONS IN RADIATION SAFETY, Uzbekistan, No 0193–2006, (2006) (in Russian). 157 MULTIPLE STRESSORS – ENVIRONMENTAL IMPACT AT SITES CONTAMINATED WITH RADIONUCLIDES AND METALS B. SALBU Norwegian University of Life Sciences, Aas, Norway Abstract Various nuclear events have contributed to the radioactive contamination of the environment. At most of the affected sites, however, the contamination includes not only radionuclides but also other contaminants, such as metals. Following nuclear events such as nuclear weapon tests, nuclear accidents with reactors, releases from nuclear installations and leaching from dumped nuclear waste, a major fraction of refractory radionuclides, such as the isotopes of uranium and plutonium, are associated with particles containing metals. Particles containing radionuclides and metals have also been identified at uranium mining and tailings sites, for instance, at sites in Central Asia. Here, the uranium isotopes and uranium daughter radionuclides are integrated in mineral structures with elevated levels of heavy metals. As radionuclides and metals can induce free radicals and affect the same biological endpoints, multiple stressor exposures may lead to additive, antagonistic or synergetic effects in exposed organisms, both in humans and biota. Therefore, the multiple stressor concept should be integrated into radioecology, as the observed effects may not be attributed to one stressor alone but to the action of mixtures. This paper presents some challenges related to the multiple stressor effects in radioecology and for the assessment of the environmental impacts associated with contaminated sites. 1. INTRODUCTION Radionuclides, artificially produced or naturally derived, rarely occur alone. Sources contributing to radioactive contamination often contain a mixture of radionuclides as well as metals. Processes affecting ecosystem behaviour, mobility, biological uptake, metabolism and the accumulation of radionuclides will also influence trace metals. Furthermore, radiation induced free radicals resulting in biological umbrella endpoints such as reproduction failure, immune system failure, genetic instability and mutation, morbidity, and mortality can also be induced by free radicals arising from metals exposure. In mixed contaminated areas, organisms are exposed to a cocktail of contaminants, i.e. multiple stressors [1]. One single stressor may induce multiple biological effects if multiple interactions occur or if interactions with different biological targets take place. In mixtures with several different stressors, multiple types of interactions and interactions with multiple target sites may occur. For contaminants having the same mode of interactions with the same target sites, effects can be concentration-additive (1+1=2), antagonistic (1+1 2) or synergistic (1+1 >2). If contaminants have different modes of interaction, and act at different target sites, they should act independently. As information on interaction mode and target sites for most contaminants is scarce, well-controlled mechanistic experiments, utilising advanced molecular and genetic tools are needed to identify early biological responses. To protect the environment from contaminants, authorities apply Environmental Quality Standards (EQSs) that are based on a one dimensional concept, assessing one component independently of others. So far, the system has been directed towards contaminants such as metals and organic compounds, while attempts are being made to derive EQSs also for radionuclides. Problems arise from extrapolating toxicity data: from acute to chronic effects, from laboratory to field conditions, from effect concentration to no-effect concentration and from isolated test-species to complex systems. According to the Organization for Economic Co-operation and Development (OECD), uncertainties in extrapolation can be covered by Safety Factors, being 100, 10, and 1 for acute, chronic and field data, respectively [2]. Taking the multiple stressor approach into account, including synergisms and antagonisms, the 159 TOPICAL SESSION 6 uncertainties could go far beyond those estimated for individual stressors. Therefore, there is an urgent need to improve the scientific bases for establishing EQSs for mixed contaminants and to assess the impact from mixtures. 2. SOURCES CONTRIBUTING TO MIXED RADIONUCLIDE AND METAL RELEASES Over the years, artificially produced and naturally occurring radionuclides have been released to the environment from a variety of sources related to nuclear weapons and the civil nuclear cycle; releases have occurred from nuclear weapons tests, accidents with vehicles carrying nuclear weapons, nuclear reactor accidents, such as fires or explosions, nuclear waste dumped at sea, effluents from the operation of nuclear installations as well as from uranium mining and tailings sites. Radionuclides are seldom released individually, but as mixtures, and the environmental impact from radioactive contamination can be attributed to mixtures rather than to individual radionuclides. Releases of radionuclides usually contain other environmental ‘stressors’, such as stable trace metals. To identify multiple stressor releases, the techniques of advanced particle analysis can be utilized, since a major fraction of released refractory radionuclides such as the isotopes of uranium is associated with particles. This has been clearly demonstrated within the International Atomic Energy Agency’s (IAEA) Co-ordinated Research Project (CRP) on the characterization of radioactive particles from different nuclear sources [3]. Radioactive particles in the environment are defined as localized aggregates of radioactive atoms that give rise to an inhomogeneous distribution of radionuclides significantly different from that of the matrix background [3, 4]. ‘Hot spots’ identified in the field reflect the presence of particles. Based on radioautography (P-imaging), environmental scanning electron microscopy (ESEMEDX) and synchrotron radiation X-ray microscopic techniques such as µ-XRF and µ-XRD, [3, 4], radioactive particles have been identified in the environment. Examples are: – Nuclear weapons tests, including peaceful nuclear detonations at Semipalatinsk, Kazakhstan; – Accidents associated with the detonation of nuclear weapons by conventional explosives (Palomares, Spain, and Thule, Greenland); – Reactor accidents such as Chernobyl; – Effluents from nuclear installations (Sellafield and Dounreay, United Kingdom; La Hague, France; Krasnoyarsk and Mayak, Russian Federation); – Leaching from radioactive waste dumped at sea; – The use of depleted uranium ammunition (Kosovo, Kuwait); – Uranium mining and tailings in Central Asia. These techniques have been utilized for the characterization of particles with respect to radionuclide and metal composition as well as crystalline structures. Radioactive particles from most of these sites contain a variety of radionuclides as well as different trace metals. Furthermore, the radionuclide and metals composition of the released particles depend on the source, while particle characteristics, such as particle size distribution, crystallographic structures, oxidation states and weathering rates, also depend on the associated release scenarios [5, 6]. 2.1. Case: mixed particles released during the Chernobyl accident Following the Chernobyl accident, radioactive particles varying in composition, size, shape, structure and colour were identified, ranging from compact small-sized crystalline 160 SALBU single particles to large amorphous aggregates [5, 7]. Fragments and large particles settled close to the site, while small-sized particles were transported to more than 2000 km from the site [5]. Based on synchrotron-radiation X-ray micro-techniques, it has been shown that inert fuel particles with a core of UO2 and with surface layers of U-C or U-Zr were released during the initial explosion. In contrast, more soluble fuel particles with a UO2 core and surface layers of oxidised uranium were released during the fire [5]. The particle weathering rate and soil to plant transfer was low for particles released during the explosion and high for particles released during the fire [6]. Using advanced techniques, a variety of fission products, as well as trace metals, were identified within individual U particles. Therefore, particle weathering results in the remobilization and ecosystem transfer, not only of radionuclides, but also of trace metals [5–7]. 2.2. Case: mixed particles associated with uranium mining sites During the Cold War, the Central Asian Republics (Kazkhstan, Kyrgyzstan, Tajikistan, Uzbekistan) were the major suppliers of uranium for the nuclear weapons and nuclear energy programmes of the former Soviet Union. Mining sites were established to extract uranium from different enriched resources such as hydrothermal and sedimentary deposits. At the mining sites, ore crushing took place, and, at some of the sites, the first steps in the chemical leaching procedure (acid leaching) were performed. The operation of uranium mining and milling enterprises produced a large volume of low-level radioactive waste in the form of crushed rock deposits, rock spoil heaps, hydro-metallurgical plant tailings dumps, and basins of mine waters. In recent years, detailed investigations of the radionuclide and metal contamination at selected sites in the Central Asian countries have been performed by the North Atlantic Treaty Organization (NATO) RESCA project and the Joint Project between Norway-Kazakhstan- Kyrgyzstan-Tajikistan. From the results of these projects, it has been demonstrated that elevated levels of a variety of metals can be observed at all investigated sites, although the levels of the metals vary according to ore deposits and geological characteristics. Using advanced techniques, metals and radionuclides can be identified within individual particles. In many places, the observed elevated levels of metals, such as arsenic, require restrictions/remediation action even without considering the radioactivity levels. Taking the multiple stressor concept into account, remedial measures at several sites may be needed. 3. MULTIPLE STRESSORS Some stressors, such as radiation and trace metals, induce free radicals in organisms due to the excitation and ionisation of water molecules in cells and Haber–Weiss and Fenton reactions. The free radicals produced are extremely reactive and will recombine and produce various reactive compounds in cells (e.g. HO2, H2O2, H2, O2) which may result in damage to membranes, tissues, enzymes, proteins and DNA/RNA. Following free radical induction, a number of biological endpoints can be influenced, such as superoxide dismutase (SOD), catalase, the glutathion cycle, and lipid peroxidation, enzyme inactivation and DNA strand breakage. Mixed exposures, in particular, long term chronic exposure to low concentrations of contaminants, may result in a variety of negative biological responses: free radical production and induced oxidative stress, causing important biomolecules such as chromosomes to change or degrade; effects on the immune system, altering susceptibilities to infectious diseases; effects on the neurological system, affecting developmental and differentiation processes. Traditional endpoints, like survival and growth, are not sufficiently sensitive to detect the various potential chronic effects. Mechanistic studies performed under well-controlled exposure conditions utilising modern advanced molecular and genetic tools to identify 161 TOPICAL SESSION 6 induced effects are needed for studying effects following low dose chronic exposures of multiple stressors [8]. 3.1. Case: Multiple stressor exposure experiments To illustrate the combined effects of radionuclide and metal mixtures (multiple stressor) exposures, experiments with Atlantic Salmon (Salmo salar) have been carried out. The experiments were designed to identify cellular effects in key organs in salmon after exposure ‘in vivo’ to low dose gamma radiation and subtoxic levels of aluminum (Al) and cadmium(Cd), alone or in combination, using a reporter cell line for the determination of stress signal activity (Bystander effects). Radiation doses as low as 4 mGy delivered over 5 hours, alone or in combination with Cd and/or Al, caused bystander signals to be produced in tissues harvested from ‘in vivo’ exposed salmon. The effects varied between different organs and were not consistently additive or synergistic for a given treatment. Tissue type also appears to be critical, with gill cells showing high degrees of synergism between radiation and metal exposure. Most data for Cd suggest also that lower toxicity is found when the metal is used in combination with radiation exposure [9, 10]. Compared to responses induced by the individual stressors, the combination of metals and low gamma doses resulted in responses that would not be predicted from the extrapolation of toxicity data for single stressors. 4. CONCLUSIONS When radionuclides are released to the environment, they are rarely released as single radionuclides but, rather, they are in mixtures containing other radionuclides and other stressors such as stable trace metals. As a result of historic events, mixtures of stressors have been released to the environment. In most radioactively contaminated areas, organisms are therefore exposed to a ‘cocktail’ of contaminants, i.e. multiple stressors. Despite this fact, impact assessments and regulations tend to be based on one dimensional concepts, assessing one component independently of the others; one stressor at a time. The scientific basis for protecting the environment from radiation associated with one single radionuclide still represents a challenge, as concepts associated with low dose chronic exposure and related effects are, to a certain extent, based on cancer in man. Thus, improvements in knowledge about dose–effect units, radiation effects, dose rate effects, internal–external radiation effects and dose–biological endpoint relationships for biota for one radionuclide and for radionuclide mixtures are still crucial topics in radioecology. It is internationally recognised that there are severe gaps in basic knowledge with respect to biological responses to multiple stressor exposures. The identification of biological responses to mixed exposure calls for early warning biomarkers, utilising modern molecular and genetic tools. Information on dose–response relationships (on/off mechanisms), sensitivity (detection limits, thresholds), and synergetic and antagonistic effects, as well as the role of protecting agents such as antioxidants, is therefore needed. The development of advanced techniques to characterize mixed exposures and to link mixed exposures to early responses in sensitive organisms, utilizing advanced biomarkers, should be encouraged in order to increase knowledge about biological impacts from multiple stressors in the future [11]. REFERENCES [1] 162 SALBU, B., ROSSELAND, B.O., OUGHTON, D.H., Multiple stressors - a challenge for the future, Journal of Environmental Monitoring 7 1–2 (2005). SALBU [2] ORGANIZATION FOR ECONOMIC COOPERATION AND DEVELOPMENT, (OECD). (http://puck.sourceoecd.org/vl=3238197/cl=45/nw=1/rpsv/periodical/p15_about.htm?jnlissn=16 07310x) [3] INTERNATIONAL ATOMIC ENERGY AGENCY, Radioactive Particles in the Environment: Sources, Particle Characterization and Analytical Techniques, IAEA-TECDOC-1663, IAEA, Vienna (2011). [4] SALBU, B., Fractionation of radionuclide species in the environment, Journal of Environmental Radioactivity 100 4 (2009) 283-289. [5] SALBU, B., KREKLING, T., LIND, O.C., et al., High energy X-ray microscopy for characterisation of fuel particles, Nuclear Instruments and Methods, Part A, 467 (21) (2001) 1249–1252. [6] KASHPAROV, V.A., OUGHTON, D.H., PROTSAK, V.P., Kinetics of fuel particle weathering and 90Sr mobility in the Chernobyl 30 km exclusion zone, Health Physics 76 (1999) 251–259. [7] SALBU, B., Speciation of Radionuclides, Encyclopaedia Analytical Chemistry 12993–13016 (2000). [8] MOTHERSILL, C., SEYMOUR, R.J., SEYMOUR, C.B., Bystander effects in repair-deficient cell lines, Radiation Research 161 (2004) 256–263. [9] MOTHERSILL, C., SALBU, B., HEIER, L. S., Multiple stressor effects of radiation and metals in salmon (Salmo salar), Journal of Environmental Radioactivity 96 1–3 (2007) 20–31. [10] SALBU, B., DENBEIGH, J., SMITH, R.W., Environmentally Relevant Mixed Exposures to Radiation and Heavy Metals Induce Measurable Stress Responses in Atlantic Salmon, Environ. Sci. Technol. 42 (2008) 3441–3446. [11] SALBU, B., Challenges in radioecology, J. Env. Radioactivity 100 12 (2009) 1086-1091. 163 INDUSTRIAL ENVIRONMENTAL MONITORING — A LAND RESTORATION COSTS TRACKING TOOL M. ISKAKOV, M. NURGAZIYEV, B. ELEYUSHOV, P. KAYUKOV National Atomic Company, (Kazatomprom), Almaty, Kazakhstan Abstract This paper describes a procedure in use in Kazakhstan for controlling the rehabilitation of sites damaged by undersurface operations. It sets out the legal requirements and a methodology for Production Environmental Control in which a procedure is established for monitoring and impact assessment and for optimizing remediation approaches, taking into account the environmental impact and the associated costs of different options. 1. INTRODUCTION In operations which involve activities in the subsurface zone, e.g. near-surface mining, the organization and implementation of the subsequent reclamation of the disturbed land has an important role. In this context, reclamation means the works necessary for restoration of the land which was lost as a result of the land disturbance caused by the subsurface operations. ‘Land disturbance’ is considered to have a broad meaning and includes the loss of economic value or the reduction in the potential utility of the area due to damage of the soil cover, the hydrological regime or other adverse changes. In accordance with national legislation in Kazakhstan, provisions for the restoration of land and other natural bodies disturbed as a result of subsurface operations are being made by establishing an abandonment fund and a remediation programme. 2. NATIONAL REGULATIONS In Kazakhstan, the utilization of natural resources and their environmental impacts is controlled by a number of regulations. The basic regulation, in this context, is the Environmental Code of the Republic of Kazakhstan dated January 9, 2007 No.212-Sh ZRK. This regulation sets out special environmental requirements for users of natural resources, among which are requirements concerning the reclamation of disturbed lands. Some of these requirements are given below: – Production techniques must be applied which are in compliance with sanitary and epidemiologic requirements and which prevent operations from causing harm to the health of people and damage to the environment by implementing the best available technologies; – Actions must be taken for the reclamation of disturbed lands and the restoration of land to its previous state. The requirements for land and subsurface resource protection and for the decommissioning of nuclear facilities are also described in other regulations of the Republic of Kazakhstan. According to the Law ‘On the resources and subsoil use’, the right to carry out works involving subsoil use can only be exercised after the establishment of a contract between the Government and the subsoil user. By filing for an application for subsoil use, a company already takes on a reclamation obligation and according to the contract terms and conditions, an abandonment fund has to be established by the subsoil user to remove the 165 TOPICAL SESSION 6 effects of subsoil use operations. The amount of the contributions to the fund and the procedure for implementation is stipulated by the contract. The abandonment fund money can be used upon authorization by the competent body (the regulator in the field of subsoil use). Thus, right from the start of the development of a subsurface activity, the applicant must begin to think about the reclamation of land and subsoil resources after the completion of activities at the site. 3. PRODUCTION ENVIRONMENTAL CONTROL In in-situ leaching operations, mining soil and vegetation cover undergo significant changes and, even at the outset of reclamation activities at in-situ leaching mining facilities, there is strong evidence of this impact. Due to the rapid development of the in-situ leaching technique in uranium deposit mining, proper solutions do not yet exist which take account of the new objectives for environmental protection. The use of modern techniques for uranium mining has provided an increase in production efficiency and a decrease in solid, liquid and gaseous waste. At the same time, in-situ leaching mining can produce significant impacts on the environment when environmental requirements are not met during mining operations and when preventive measures to avoid or mnimize environment pollution are not available. The application of Production Environmental Control at all stages of the land reclamation process for land areas damaged by uranium exploration and mining has proved to be very effective in achieving successful land reclamation programmes; this is one of the forms of control stipulated by the environmental law. TABLE 1. LIFE CYCLE OF LAND RECLAMATION ACTIONS Period prior to reclamation Design Stage Restoration Period Post-reclamation period Review of environment conditions. Obtain data on natural background concentrations of chemical and radioactive substances in the environment prior to deposit development. Mine designing and construction. Mine operation. Environmental monitoring to meet the objectives of the expected reclamation as contained in the Production Environmental Control programme. Reclamation Project - Environment Impact Assessment including Production Environmental Monitoring programmes. Land plots reclamation in accordance with design solutions Implementation of environmental measures Implementation of Production Environmental Control Radiation and sanitary control at abandoned facilities Implementation of Production Environmental Control Accounting and Reporting As can be seen from the life cycle chart in Table 1, there is a period prior to reclamation during which the environment monitoring of land areas where reclamation is to be carried out is required. Such an approach is required for the purpose of minimizing environment pollution and for saving funds during the budgeting of reclamation expenditures; it includes design and exploration surveys, soil and field surveys, laboratory analysis, and mapping. All such activities must be included in the Production Environmental Control Programme. As part of this, environmental and radiation monitoring data are to be collected and analyzed for the estimation of future reclamation costs. 166 ISKAKOV et al. Production Environmental Control in the life cycle period prior to reclamation means: – A mechanism to identify, study and assess obvious and hidden damage to the natural state of environmental components which might lead to its degradation or deterioration; – A tool for the control of the environmental impact of the operation and for preventing and eliminating violations of environmental standards and rules; – A method for providing information to the public about any environmental and population health risks associated with the operation; – An instrument for providing inputs to decision making on possible future activities of the enterprise (reconstruction, renewal, conversion, temporary closure, closing down of individual sites). The content and volume of the work performed is defined primarily by the tasks prescribed in the Production Environmental Control System. The list of such tasks may be rather long and specific. Among the typical tasks of Production Environmental Control to be implemented within the pre-reclamation period of in-situ leaching mining are the following: – System analysis and evaluation of environmental aspects, continuous radioecological monitoring of production technological processes (possibly based on an automated system of continuous environmental and radiation monitoring on the lands to be reclaimed); – Minimization of adverse environmental impacts; – Use of natural and energy resources; – Creation of an environmental monitoring database on the territory of the enterprise, the sanitary protection area and neighbouring populated areas; – Prevention of accidental environment pollution and development of planned corrective actions (in case it happens); – Record keeping – timely submission of reports on the results of Production Environmental Control to State authorities. Thus, the system of Production Environmental Control is represented at every stage of the land reclamation. The main elements can be presented as the following sequence of actions: – First – collection and handling of information at the source of contamination (monitoring); – Second stage – detection and elimination of deviations from the technological requirements relevant to the source (clear task distribution among the staff plays a determining role during this stage.); – Last – the basis of the whole interaction chain is taking management decisions aimed at the end effect – minimization of environmental pollution through compliance with ecological standards and requirements. This is directly connected to the modernization or reprofiling of production and the fulfillment of environmental actions. The planning of environmental and radiation monitoring at sites subject to rehabilitation should be done within the framework of the Programme for Production Environmental Control developed by an enterprise. It should be noted that environmental monitoring includes experimental (on a measurement basis) or indirect (on a calculation basis) evaluation of the conditions of the production process, the emissions (and radiation exposure) as a result of operations, and the state of the environment in accordance with the requirements set by the relevant legislation. Direct measurements can be done by staff or by outside accredited 167 TOPICAL SESSION 6 laboratories. Irrespective of the monitoring organizational structure, the enterprise conducting special environmental management is fully responsible for information quality. Uranium-mining enterprises that are a part of JSNAC Kazatomprom are obliged to develop a Programme for Production Environmental Control and to implement it based on the most effective approaches (direct and indirect) with regard to the monitoring of operational characteristics, emissions and the state of the environment. An important role in Production Environmental Control during land reclamation belongs to the Environmental Services of the enterprise whose functions are as follows: – Personnel training and education on the forms and methods for organizing monitoring at a facility; – Analysis of the reasons for non-compliance with the environmental requirements and norms for radiation security at a contaminated site; – Making decisions on the elimination of deviations and providing for compliance with environmental aspects of the technological process; – Formation of an environmental management system with clear allocation of responsibilities for compliance with environmental laws, environmental quality standards and radiation standards. On the basis of the foregoing discussion, the importance of the role of the Production Environmental Control and Management organization can be seen in the process of the development and exploitation of uranium deposits, in the minimization of environmental pollution as a result of such activities, and in the reduction of the financial costs associated with the rehabilitation of the environment after its exploitation. REFERENCES [1] [2] [3] [4] [5] [6] [7] 168 ENVIRONMENTAL CODE OF THE REPUBLIC OF KAZAKHSTAN, No. 212 – III LRK dated January 9, 2007 (2007). LAW OF THE REPUBLIC OF KAZAKHSTAN, dated January 27, 1996, No. 2828, ‘About subsoil and subsoil use’ (1996). LAND CODE OF THE REPUBLIC OF KAZAKHSTAN. LAW OF THE REPUBLIC OF KAZAKHSTAN, dated April 14, 1997 No. 93–I ‘On usage of nuclear energy’ (1997). JSNAC KAZATOMPROM, ST NAC 17.1-2008, Standard Programme for Production Environmental Control of in-situ leaching enterprises (2008). MINISTER FOR ENVIRONMENT OF THE REPUBLIC OF KAZAKHSTAN, Rules for Coordinating the programmes for Production Environmental Control and requirements on reporting the results of Production Environmental Control, dated April 24, 2007, No. 123-p. (2007). JSC VOLKOVGEOLOGY, Environmental impact assessment of uranium mining by in-situ leaching method at abandoned deposits – Northern Karamurun, Kanzhugan, Uvanas and Mynkuduk. Almaty (2002). SUMMARY OF SESSION 6 A. Kim Kazakhstan CASE STUDIES I: ENVIRONMENTAL REMEDIATION IN CENTRAL ASIAN COUNTRIES This session consisted of eight plenary presentations and was concerned with the status of sites that have been contaminated with radioactive residues in the Central Asian countries of Kazakhstan, Tajikistan, Uzbekistan and Kyrgyzstan. The four countries in Central Asia have common problems concerning residues due to uranium mining and milling activities conducted mainly during the Cold War years. In addition, the territory of Kazakhstan has been affected by nuclear weapons testing on several locations. It is recognized that environmental management took a back seat to operations while the uranium mining was most active and, as a result, there are large areas of territory affected by residues. The public is concerned in all of the countries about the potential impacts of the releases of radioactivity into the environment. The presentations showed there to be a general lack of data concerning the characterization of the sites and a lack of experience and funding to perform remediation activities; these are some of the reasons why these problems are still unresolved. Many areas have elevated radiation backgrounds caused by a variety of circumstances, for example, arising from the residues of the mining and processing of uranium ore but also from the mining and processing of other minerals, from oil and gas exploration, from nuclear weapons testing and due to naturally elevated concentrations of radionuclides in the soil. Some of these conditions have led to increases in the radon concentrations in the atmosphere in occupied areas and to groundwater which is used for drinking and agricultural purposes being contaminated with radionuclides and/or chemicals and metals. Each country has its own particular conditions. In some areas, precipitation has caused the erosion of tailing piles; in others, landslides have caused significant changes in previously stable storage sites. In some areas, residues have been used as building material in homes and public buildings such as schools. Because of the physical geography of some of the Central Asian countries, contaminants from one country can be transported by rapidly flowing rivers across national borders. Generally, although large land areas have been affected by uranium mining activities, the associated radiological conditions are not sufficiently serious to justify ‘intervention’ on the basis of international safety standards but, on the other hand, the radiation exposures can often be reduced by simple expedients. The radiological situation in these countries is currently being assessed - sometimes with the aid of the international organizations. However, insufficient attention is being given to the presence of chemicals and metals in the residues; in some cases these could represent the main hazard to humans. One presentation raised the issue of large airborne particles containing a mixture of radionuclides and metals - which have been detected at some sites, e.g. the Semipalatinsk Nuclear Test Site. However, the hazards presented by these particles are difficult to assess. 169 SUMMARY OF SESSION 6 The following short term actions, if implemented, would assist in mitigating some of the concerns at the uranium legacy sites: – Perform comprehensive environmental impact assessments for each site to include all potential contaminants (radiological and chemical); – Identify alternative water supplies if ground water has been contaminated; – Implement and maintain institutional controls at the sites; – Perform routine monitoring to ensure the controls are performing their intended functions; – Increase public awareness of the local situation and answer public concerns about safety issues. While these near term actions are being implemented, longer term actions can be identified and planning can be started to find permanent solutions. It was clear from the presentations that there are a number of international organizations providing support to the countries, but it was not clear if these support actions are fully coordinated. It is also recognized that there is not a technical network which allows an exchange of information among the countries and the coordination of activities. 170 CASE STUDIES II (TOPICAL SESSION 7) Chairperson B. SALBU Norway CHALLENGES IN ESTIMATING PUBLIC RADIATION DOSE RESULTING FROM LAND APPLICATION OF WATERS OF ELEVATED NATURAL RADIOACTIVITY P. LU*, R. AKBER**, A. BOLLHÖFER*** * EWL Sciences, Darwin, Australia ** Safe Radiation Pty Ltd, Calamvale, Australia *** Supervising Scientist Division, Department of the Environment, Darwin, Australia Abstract Ranger Uranium Mine is located in the northern wet/dry tropical region of Australia. The mine implements a comprehensive water management programme and land application of water from its retention pond 2 (RP2) is a part of that programme. The land application areas are located in common woodlands within the mine lease boundary – the combined area is about 336 ha. RP2 contains run-off from the waste rock and low grade ore stock piles and the water is therefore elevated in natural radionuclide activity concentration. When the water is applied to the land, the radionuclides are adsorbed within a few centimeters of the surface. A comprehensive project is cleanup to estimate the radiation dose likely to be received by the critical group during occupancy of these areas after rehabilitation. The distribution of radionuclides and the traditional use of the land are such that direct application of commonly used parameters in dose estimates through pathway analysis may not be adequate. This paper describes the site, identifies the special aspects of the distribution of radioactivity on the ground and their influence on radiation dose estimation through the different exposure pathways. 1. INTRODUCTION Ranger Uranium Mine is located in the Alligator Rivers uranium province in the northern tropical region of Australia. Mining at Ranger commenced in 1980 and is still continuing. The main uranium deposits at Ranger are hosted in altered schists and silicified carbonates. Acid leaching is used to extract Uranium. The total lease area of Ranger Uranium Mine is 7908 ha. It is located near the township of Jabiru. The lease area is surrounded by Kakadu National Park which is World Heritage listed both for its natural value and for its cultural significance due to ancient Aboriginal habitation of the area. The climate in the Alligator Rivers Region is monsoon-like with distinct wet and dry seasons. Almost all of the rain falls during November to March and the dry season lasts from about May to September. The mean average rainfall for the past 32 years at Jabiru Airport was 1579 mm and the mean annual evaporation (2628 mm) exceeds the rainfall [1]. The region is subject to severe weather events such as cyclones and floods. Seasonality adds to distinctive features in the physiography of the land. The seasonal and often unpredictable rainfall patterns pose water management challenges for Ranger Uranium Mine. Run-off water from areas of above background natural radioactivity is collected in retention ponds. Retention Pond 2 (RP2, Fig. 1) catches water mainly from the waste rock and low grade ore stock pile areas at Ranger and consequently, it exhibits elevated activity concentrations of naturally occurring radionuclides. The pond is about 12m deep and 24.86 ha in surface area. The water volume retained at any time in the 173 TOPICAL SESSION 7 pond varies – from nearly empty to its full capacity of 1 100 000m3. Some water from the pond is used to sustain mining and milling operations, but since 1985, large volumes have been disposed of through a technique of land application to common woodland within the mine lease. FIG. 1. Locations of land application areas (hatched) and retention pond 2 (RP2). 2. LAND APPLICATION Land application technology relies on the ability of soil and plant systems within the application area to retain radionuclides, metals and some major ions from the applied water volumes. As the land can be more appropriately monitored, managed and rehabilitated than water, an advantage of successful land application of effluent waters is the transfer of the constituents from a less manageable aqueous phase to a more containable solid phase. If immobilized by adsorption in the soil system, the radionuclides will not reach the aquatic ecosystems through run-off and sub-surface flow during subsequent wet seasons. 174 LU et al. TABLE 1. LAND APPLICATION AREAS AT RANGER URANIUM MINE Location Section Magela Original Extension Original Extension Original Extension RP1 Djalkmara Jabiru East Corridor Creek Size (ha) 33 20 46 8 18 20 52 141 Year commissioned 1985 1994 1995 2006 1997 1999 2006 2007 Water quality unpolished unpolished polished unpolished polished polished unpolished unpolished The area of land application at Ranger has gradually increased (Table 1). Overall, 336 ha of land is now set aside for this purpose. Raw RP2 water is applied to most land application areas. In some areas, polished (wetland filtered) RP2 water is applied; this has a lower concentration of radionuclides than the raw RP2 water. Water is applied through a grid of sprinklers with a 6 to10m radius. The application rate is controlled such that no runoff occurs. Total applied volumes have varied from year to year, ranging from 6.3 × 104 to 1.3 × 106 m3 between 1985 and 2008. No water was applied to the land in 1990 or 1999. When compared to natural waters, RP2 water contains elevated concentrations of 238U, 226Ra and 210 Pb with values around 12, 0.3 and 0.15 Bq.L-1 respectively. 3. DISTINCTIVE FEATURES OF NORM DISTRIBUTION IN LAND APPLICATION AREAS Soils from different land application areas have been investigated for their ability to retain RP2 water solutes [2, 3]. In particular, the original Magela land application area has been extensively investigated. The studies based on batch and column experiments showed that the soils have a strong adsorption capacity for radionuclides such that during land application they are likely to be retained within a few centimetres of the ground surface. Gamma spectrometry analyses of sections of soil cores from the land application area demonstrate this. The signal decreases rapidly with depth and, typically, below 10 cm it reduces to natural background levels. Water and a number of other, less reactive, chemical species infiltrate to the subsurface [2, 3]. Land application of RP2 water has therefore created areas of relatively high radioactivity in a surface zone (a few centimetres in depth) over 336 ha of common woodland. The spatial distribution of radioactivity is non-uniform; higher values occur closer to the sprinklers. The mine operators are committed to rehabilitate the land application areas such that future occupancy does not lead to radiation doses exceeding the regulatory limits. Special consideration is required for the traditional local life styles which are based on a strong relationship with the land, some food gathering and hunting activities. 4. IMPLICATIONS FOR DOSE ESTIMATES To determine above background radiation doses to members of the public that may enter the lease area after rehabilitation of the mine, Ranger Uranium Mine has developed a project to assess the radiological condition of the land application areas so that appropriate rehabilitation plans can be developed and remediation actions taken if required. Exposure pathways that must be considered are direct irradiation, inhalation of radon and its progeny, 175 TOPICAL SESSION 7 inhalation of resuspended long-lived radionuclides in dust, and direct ingestion of radionuclides in soils or through the consumption of bush foods collected from the land application areas. This project has identified that standard values of a number of different parameters that are commonly used in models for estimating radiation doses in areas in which mining and milling of radioactive ores is carried out may not be strictly applicable to the special case of land application – the discrepancies in some cases may be up to several orders of magnitude. The differences arise mainly due to the fact that adsorbed radionuclides are likely to be present at the mineral grain surface, rather than being distributed throughout the mineral matrix. The radionuclides are also retained within the surface zone of the soil. By contrast, naturally occurring radionuclides, are likely to be more or less evenly distributed in the bulk of the soil grains and throughout the deeper soil layers. In addition, the traditional use of bush foods is an important factor to be considered [4, 5]. Due to their significance for radiological assessments, the differences are identified in this paper: 1. In traditional life styles, the bare skin may be exposed to ground surfaces. For this reason external radiation dose measurements should take into account both the nonpenetrating Hp(0.07) and penetrating Hp(10) radiation; 2. With regards to the 222Rn source term, 226Ra presence near the surface of grains will lead to higher 222Rn emanation rates than expected from bulk soil 226Ra distribution. In addition, as the applied 226Ra is retained close to the soil surface, 222Rn is likely to diffuse more readily; 3. Atmospheric radon concentration is typically measured at a height of 1-2 metres, but the traditional Aboriginal life style may involve sitting and sleeping on the ground. Radon concentration above ground may vary as a function of height, wind speed and due to the presence or absence of perennial vegetation [6]; 4. Resuspension factors are commonly used to estimate the expected concentration of airborne radioactivity in dust relative to that on the surface of the ground (to a few centimetres depth). These factors have been developed for the wet-dry tropical areas in northern Australia [2, 7]. Corrections are required to determine the contribution of suspended dust in land application areas. This is because a strong gradient exists in the soil activity concentration as a function of depth and also, because of the larger surface area to volume ratios (as smaller particles tend to have higher adsorbed activity concentrations). Additionally, preliminary observations show differences in the dust loading values as a function of heights representative for a person lying down, sitting, a juvenile standing and an adult standing; 5. Conventionally determined concentration factors for edible fruit and forage may also not be valid for the land application areas. During the operational phase, foliage and fruit in the land application area may be sprayed directly by the water derived from the mine areas. Following rehabilitation, the uptake is likely to be through root system only. For larger fruit bearing trees, roots may be distributed underground to depths of greater than a few centimetres and may not be influenced by the applied radionuclides which are retained near the surface. Taking account of these issues, a comprehensive programme of direct measurements has been established. This programme is now cleanup and the results will become available in due course. 176 LU et al. REFERENCES [1] [2] [3] [4] [5] [6] [7] AUSTRALIAN BUREAU OF METEOROLOGY, Climate averages at Jabiru airport. AKBER, R.A. (Ed.), Proceedings of the Workshop on Land Application of Effluent Water from Uranium Mines in the Alligator Rivers Region. Jabiru, 11–13 September 1990, Supervising Scientist for the Alligator Rivers Region, AGPS, Canberra (1992). WILLETT, I.R., BOND, W.J., Fate of manganese and radionuclides applied in uranium mine waste water to highly weathered soils, In Proceedings of the First International conference on Contaminants and the Soil Environment, Geoderma 84 (1997) 195211. MARTIN, P., HANCOCK, G.J., JOHNSTON, A., MURRAY, A.S., Natural-series radionuclides in traditional north Australian Aboriginal foods. Journal of Environmental Radioactivity 40 (1998) 37–58. RYAN, B., MARTIN, P., ILES, M., Uranium-series radionuclides in native fruits and vegetables of northern Australia, Journal of Radioanalytical and Nuclear Chemistry, 264 2 (2005) 407–412. BOLLHÖFER, A., The geographical variability of airborne radon concentration at the rehabilitated Nabarlek mine site during the dry season 2005, Internal Report 527, Supervising Scientist, Darwin. Unpublished paper. BOLLHÖFER, A., HONEYBUN, R., ROSMAN, K., Atmospheric transport of radiogenic lead in the vicinity of Ranger uranium mine determined using lead isotope ratios in dust deposited on acacia leaves, Internal Report 451, August 2003, Supervising Scientist, Darwin, Unpublished paper. 177 EXPERIENCE OF THE CONSTRAINTS AFFECTING THE IMPLEMENTATION OF DECOMMISSIONING/REMEDIATION PROGRAMMES AT URANIUM MINING SITES M.R. FRANKLIN Institute of Radiation Protection and Dosimetry, Brazilian Nuclear Energy Commission, Rio de Janeiro, Brazil Abstract It is well known that the need for extensive remediation programmes derives from the lack of appropriate planning at the beginning of mining operations, i.e. remediation is not adequately taken into consideration in the overall mining development. As a consequence of this, the implementation of remediation work generally faces several constraints that prevent the adoption of the necessary cleanup procedures. These constraints can be of an economic, technical, regulatory or social nature. In Brazil, the remediation of the uranium mining site of Poços de Caldas constitutes a very significant challenge for the mine operator and regulatory organizations. Many research/technical projects have been carried out by different institutions but the integration of the results of these works into a coordinated framework has never been achieved. There is also a lack of synergism between the environmental and nuclear regulatory authorities, and the mine operator does not seem to have a clear plan of action to deal with the problem. As a result of this situation, the expertise existing in the country is not being properly utilised to facilitate the development of the necessary actions. Also, members of the public have not yet been properly involved in the decision making process and this will constitute a serious problem in the near future. This paper discusses potential actions to overcome these constraints based on international experience. 1. INTRODUCTION In Brazil, activities related to the exploration, production and processing of uranium ores are implemented by the state-owned company Indústrias Nucleares do Brasil (INB). Uranium is produced to supply the domestic demand, presently represented by two PWR-type nuclear reactors. As a result of the decision not to depend on the external supply of uranium, the exploration of the available and known low-grade ore bodies in Brazil has been undertaken. The first deposit to be exploited was the one located at the municipality of Poços de Caldas. This deposit was discovered in the 1970s. The ore grade was of about 0.1% uranium, which occurred as pitchblende, associated with pyrite (FeS2), fluorite (CaF2), and zirconium and molybdenum minerals. The Uranium Mining and Milling Facility of Poços de Caldas (UMMFPC) started operations in 1982. After 13 years of non-continuous operations, the mining activities were finally suspended. The total uranium production was 1242 tonnes of U3O8 [1]. At the present time, the UMMFPC is in the first phase of a decommissioning/remediation process and a general project for the mine closure is cleanup. Several scientific and technical projects have been developed by different organizations dealing with the closure and remediation of this installation. However, a well-defined plan of action has not yet been conceived. This paper discusses the reasons for this situation, i.e. why there are problems in implementing the UMMFPC remediation works. The Brazilian situation is used as the basis for this analysis but it is expected that some of the lessons learned may serve to aid the implementation of remediation programmes at other sites that share similar problems. 179 TOPICAL SESSION 7 DESCRIPTION OF THE MINE SITE – ACID MINE DRAINAGE PROBLEM 2. The uranium production centre of Poços de Caldas is located on the Poços de Caldas plateau, in the Southeast region of Brazil. This alkaline complex corresponds to a circular volcanic structure whose formation began in the upper Cretaceous period (87 ma (million years ago)) and evolved in successive steps until 60 ma. The uranium enrichment in the Poços de Caldas mine is related to hydrothermal events (primary mineralization) and to later weathering processes (secondary mineralization). The uranium in this mine was extracted by open pit operations. About 45×106 m3 of ores were processed which gave rise to approximately 12×106 m3 of waste rock, while the mill process generated a volume of approximately 2.4×106 m3 of tailings [2]. The main sources of pollutants to the environment are the tailings dam (TD), the waste rock piles (WRPs) and the open pit (OP). Pyrite oxidation was found to be the driving force in leaching metals and radionuclides into the environment. It has been estimated that acid drainage generation will last for 600 and 200 years from the waste rock piles and the tailings dam respectively [2]. The long timescale involved in the oxidation of sulphidic materials implies a need to adopt permanent remedial solutions. It was also estimated that the release of untreated effluent from the tailings dam and waste rock piles into the environment, without any treatment, would result in radiation doses as high as 8.0 mSv/y to members of the public. These values are higher than the primary dose limit for members of the public established by the Brazilian regulatory authority, i.e. 1.0 mSv/y [2, 3]. 3. REGULATORY CONSTRAINTS One of the first issues to constrain the implementation of remediation works in Brazil, especially at uranium mining sites, is concerned with the regulatory framework. Uranium mining operations are regulated both by the Federal Environmental IAEA (IBAMA) and by the Nuclear Regulatory Authority (CNEN). However, when the mine was developed, the environmental legislation, now available, was not in place. As such, the mining developer did not have to present an Environmental Impact Statement (EIS) prior the operation of the mining and milling facilities. The licensing process was mainly dictated by the Nuclear Regulatory Authority because uranium mining and milling facilities are considered to be nuclear installations in Brazil. From the point of view of the Nuclear Authority (CNEN), the decommissioning/environmental remediation of a mining facility is treated as ‘abandonment of the installation’. The requirements are rather generic in nature and the actions to be implemented regarding the post-operational phase of facilities were not prescribed. The requirements include the following actions to be implemented by the operator: – Backfilling of the open pit with mine debris and sealing of all wells, holes, galleries or any other excavation for research or ore removal, in the surface or sub-surface, to prevent the occurrence of accidents; – Actions to limit the potential risks to human health and safety; – Classification of areas in the mine to avoid the release of toxic substances to the environment; – Implementation of an abandonment and area restoration plan, to be approved by the Regulatory Authority. This plan should contain, to the extent possible, predictions of possible future uses of the area. 180 FRANKLIN These criteria are contained in the regulatory document CNEN–NE–1.13 (1989) (www.cnen.gov.br) which also contains the regulatory requirements to be applied in the licensing of uranium and thorium mining and milling facilities. Numerical standards however, are not provided but it seems to be implicit that the releases to the environment should not exceed those authorized for the operational phase of the installation. More specific requirements are available for the management of tailings dams (Standard CNEN–NE–1.10 (1980) (www.cnen.gov.br)). It is required that waste shall be stabilized physically and chemically in order to ensure that effluents leaving the system comply with the appropriate regulatory levels. Stabilization should begin immediately after the termination of waste disposal. The systems should be provided with means to seal or eliminate contaminated drainage sources in order to avoid, as much as possible, the collecting and treatment of the drainage. The system should also be protected against natural drainage by means of engineering works, such as dykes and embankments. It should also be controlled and marked in order to restrict intrusion by members of the public and to prevent non-authorized use of the waste. The stabilization, control and maintenance of the system in the long term should be documented and this record must be part of any commercial transaction involving the area. CNEN should also be informed promptly about any new landowner. After 1986, EISs began to be required for any operation in Brazil that could cause significant impacts in the environment. The EIS document should be presented to the IBAMA for approval. In addition, every project involving mineral extraction in the country should make available an ‘Area Restoration Plan’, based on the decree No 97623 of April 10, 1989 linked with the Brazilian Constitution (article 225, paragraph 2). The decree also establishes that, in the case of a new project, the plan must be presented during the environmental licensing of the project. Economic aspects of the environment restoration are also to be taken into account and the costs related to this activity must be part of the overall project cash flow. As the uranium mining and milling operations in Poços de Caldas began before the above dates, the Environmental IAEA (IBAMA), in July/2002, made use of a mechanism known as ‘Terms of Environmental Commitment (TEC)’. By signing this, the operator commits himself/herself to present a Degraded Area Restoration Plan (DARP), to be inserted in the Decommissioning Project of the installation. In the Terms of Reference (ToR) that have been elaborated to guide the operator in complying with the safety requirements established in the DARP, different elements related to the appropriate and definitive remediation of the tailings disposal area, open pit and waste rock dumps are clearly defined. The resulting situation is that, if the operator does not wish to declare the mine as abandoned, i.e. if it is intended to continue water treatment operations indefinitely, no constraint will be made by the Nuclear Regulatory Authority as long as the emissions level is below that leading to radiation doses to members of the public of 0.3 mSv/y. On the other hand, the Environmental IAEA requires the adoption of a remediation plan as soon as possible, but as long as radiological issues are involved and while the IBAMA does not have the necessary expertise to deal with them, a ‘grey area’ exists and this can only be solved by means of proper negotiations and mutual understanding between the relevant parties. It is important to mention that other stakeholders must also be involved in this process in an appropriate way. 4. MANAGERIAL CONSTRAINTS AND TECHNICAL ISSUES Unlike some other mining sites in the world (that are located in dry areas) the mining site of Poços de Caldas is located in an area characterized by high precipitation rates, i.e. 1800 mm/y, meaning that, if the water treatment is not functioning, undue emissions of radionuclides and heavy metals into the environment will occur. On the other hand, when the 181 TOPICAL SESSION 7 water is being treated, large amounts of material (sludge) – containing significant levels of radionuclides and heavy metals - have to be disposed of. Because of this, disposal areas at the mining site have to be made available. As the tailings dam is not capable of containing any more waste, the material resulting from water treatment is disposed of in the mine pit (an operation that was not predicted in the mining operation plan). Because of this, it seems to be clear that the starting point for any remediation plan for the site should be the abatement of acid drainage generation. Unfortunately, the mine operator, despite several studies already carried out at the site, has not understood and drawn the proper conclusions from the results of these studies. Instead of channeling resources to pursue solutions for the problem of acid drainage, efforts have been directed towards the implementation of ineffective solutions. For example, resources have been wasted in the revegetation of the waste-rock piles; in trying to decrease the amount of water infiltrating these systems, in applying – without appropriate understanding and calculations – a clay layer on the top of the waste rock piles; and in enhancing the disposal volume of the tailings dam. Another important managerial flaw is the lack of effort in trying to collect and organize the relevant information about the site. This includes, for example, descriptions of the mining operations, environmental monitoring data, publications related to the site, etc. This situation is aggravated by the fact that a large part of the work force has left the company or has been relocated to other productions centres or has been retired. As a result, the memory of the site will soon be lost to a very large extent. Finally, the full dismantling of the industrial area and site remediation do not constitute priorities for the company. Since these operations are resource consuming and no funding mechanism (e.g trust fund) has been created to support them, the company prefers to invest the available resources in the development of the mining and processing operations of the new production centre in Caetité in the northeast region of the country. The problem is that acid drainage has been estimated to last for at least 600 years and, in the long term, it will require a very significative amount of resources. In other words, procrastination of the implementation of effective solutions for the remediation of the site is not a wise managerial decision. Instead, the operator should seek appropriate support from experienced professionals in the pursuit of the design and implementation of an adequate remediation plan. 5. LEGAL CONSTRAINTS In December/2002 to attend to the requirements embodied in the Terms of Environmental Commitment (TEC), the operator started an international bidding process to contract specialized consulting services for the development of the necessary studies for the elaboration of the DARP. The type of bidding was based on the lowest price and was open to contractors from outside Brazil, as long as the technical requirements (based on the terms of reference) were fulfilled. This process was not concluded because of problems in complying with Brazilian legislation (mainly problems related to the exchange rate variation). At the end of 2004, another bidding process was opened, but reduced to a national outreach while allowing for the possibility of establishing partnerships between Brazilian and international companies. A consortium between a European consulting company and a Brazilian one won the bidding. However, the contract was cancelled in June of 2006 by INB due to technical problems. At the end of 2006, a third bidding attempt was opened by INB. Once again the process was not concluded. This time no proposal could comply with the requirements established in the bidding process. According to information obtained from INB (personal communication) it is foreseen that another bidding procces will be started in 2009. The main problems that the operator faces in the bidding process relate to the legal/bureaucratic constraints resulting from the legal status of the company, i.e. a state182 FRANKLIN owned company. This prevents flexibility and imposes serious constraints in the setting up of good contracts. Another factor that contributes to the inefficiency of the process is the lack of experienced companies in the country dealing with the remediation of radioactively contaminated/nuclear sites. While a considerable amount of research work has been carried out dealing with the decommissioning and remediation of the site [4 – 11] practical remediation experience is still lacking in the country. To make things worse, there is no contact (or synergism) among the different research projects and the results are not being assimilated by the regulatory authorities or the operator. 6. CONCLUSIONS The uranium production centre of Poços de Caldas is the first uranium production centre to be decommissioned and remediated in Brazil. Due to the lack of experience in developing uranium mining operations and also due to the lack of an appropriate regulatory framework, significant environmental liabilities have been generated. Eleven years after the termination of the mining and milling operations at the site, a well-defined site remediation plan has not yet been designed. As demonstrated in this paper, this situation results from three main issues: regulatory, managerial and legal constraints. Lack of financial resources certainly plays a role, but overcoming the first steps may contribute to reducing the costs associated with site remediation. It would also avoid the waste of financial resources in the implementation of inappropriate and/or ineffective solutions. Individual measures to improve the overall situation can be suggested. They would include: – Commitment of the upper hierarchies of the company and regulatory authorities to the implementation of a remediation programme; – Coordination of actions amongst the different regulatory authorities; – Integration of the results arising from the technical and scientific work; – Greater autonomy of the operator to conduct the bidding process – Involvement of all relevant stakeholders; – Allocation of appropriate financial, material and human resources The adoption of any one of the above elements in isolation would not be enough to improve the overall situation. Lessons learned from other countries that have had to face similar challenges reveal that it is essential to establish administrative arrangements that lead to the formation of a working group that can discuss and propose a road-map for the design and implementation of the remediation plan. This group should be made up of representatives of the operator (and its consultant company), the regulators (at the federal and state level), relevant technical and scientific institutions and other relevant stakeholders. REFERENCES [1] [2] [3] MAJDALANI, S.A.,TAVARES, A.M.,. Status of uranium in Brazil. In: Proceedings of a Technical Committee meeting on Assessment of uranium deposit types and resources – a world perspective, International Atomic Energy Agency, Vienna (2001) 119–127. FERNANDES, H.M., FRANKLIN, M.R., Assessment of acid rock drainage pollutants release in the uranium mining site of Poços de Caldas – Brazil. Journal of Environmental Radioactivity 54 (2001) 5–25. FERNANDES, H.M., FRANKLIN, M.R., VEIGA, L.H.S., Acid rock drainage and radiological environmental impacts. A study case of the Uranium mining and milling facilities at Poços de Caldas. Waste Management v.18 (1998) 169–181. 183 TOPICAL SESSION 7 [4] FERNANDES, H.M.; VEIGA, L.H.S., FRANKLIN, M.R., et al., Environmental impact assessment of uranium and milling facilities: a study case at the Poços de Caldas uranium mining and milling site, Brazil. Journal of Geochemical Exploration v.52 n.1–2 (1994) 161– 173. [5] FERNANDES, H.M., FRANKLIN, M.R., VEIGA, L.H.S., et al., Management of uranium mill tailings: geochemical processes and radiological risk assessment. Journal of Environmental Radioactivity v.30 n.1 (1996) 69–95. [6] WIIKMANN, L.O., Caracterização química e radiológica dos estéreis provenientes da mineração de urânio do planalto de Poços de Caldas. Universidade de São Paulo – USP. 98p. (in portuguese)(1998). [7] FERNANDES, H.M., FRANKLIN, M.R., Assessment of acid rock drainage pollutants release in the uranium mining site of Poços de Caldas – Brazil. Journal of Environmental Radioactivity v.54 (2001) 5–25. [8] RODRIGUES, J.A., 2001, Drenagem Ácida do Bota-Fora 4 (Mina de Urânio de Caldas – MG): Aspectos Hidroquímicos e Hidrogeológicos. Departamento de Geologia, Programa de PósGraduação em Evolução Crustal e Recursos Naturais, Universidade Federal de Ouro Preto UFOP, Ouro Preto – MG. 194p. (in portuguese) (2001). [9] FRANKLIN, M.R., FERNANDES, H., GENUCHTEN, M.T.V., et al., Application of Water Flow and Geochemical Models to Support the Remediation of Acid Rock Drainage from the Uranium Mining Site. In: Proceedings 11th International conference on Environmental Remediation and Radioactive Waste Management ICEM2007, Bruges, Belgium (2007). [10] CIPRIANI, M., Mitigação dos Impactos Sociais e Ambientais Decorrentes do Fechamento Definitivo de Minas de Urânio. Tese de Doutorado. Instituto de Geociências, Universidade Estadual de Campinas, 332p. (in portuguese) (2002). [11] FAGUNDES, J.R.T., Balanço hídrico do bota-fora BF4 da mina de Urânio Osamu Utsumi, como subsídio para projetos de remediação de drenagem ácida. Escola de Minas, Departamento de Engenharia Civil, Programa de Pós–Graduação em Engenharia Civil, Universidade Federal de Ouro Preto, Ouro Preto – MG. 147p. (2005) (in portuguese). 184 LESSONS LEARNED FROM THE REMEDIATION AT VILLA ALDAMA URANIUM EXTRACTION PLANT R. FABIAN ORTEGA Nuclear Safety and Safeguards National Commission, Mexico City, Mexico Abstract From 1969 to 1971, a uranium extraction plant operated in close proximity to Villa Aldama city in Chihuahua state, the plant ceased operations in 1971 leaving 30 000 tons of uranium tailings, 1735 tons of uranium ore and contaminated equipment and buildings. The whole facility and the radioactive material remained almost unattended for more than 20 years. During this time the tailings and ore contaminated the soil around them. At the same time, the city of Villa Aldama expanded and its houses began to approach the site boundary. Because of this and other factors, such as the potential contamination of groundwater, remediation actions were required by the Nuclear Safety and Safeguards National Commission. These actions were, basically, the decontamination of the site and the disposal of the radioactive waste generated in the process. This paper describes the remediation efforts that brought the facility to a safe status. 1. INTRODUCTION In 1967, the Mexican Mining Development Commission, which was a decentralized entity of the federal government, set up a project for the operation of a uranium and molybdenum ore processing facility in Chihuahua State in the north of the country. For this purpose, a small city called Villa Aldama (the name was later changed to Ciudad Aldama) was selected, because of favourable factors for the siting and operation of the facility – such as its relative proximity to the uranium mining sites (located 50 km north of the city) and the easy access to urban services such as electric power and water supplies and also the availability of a work force. Then, In June 1969, the plant was transferred to URAMEX (short for Mexican Uranium), which also was a federal entity (now extinct). The purpose of this transfer was that URAMEX would use the facility as an experimental plant focusing only on the extraction of uranium. The operation of the experimental uranium extraction plant started in 1969 and ended two years later due to its demonstrated low profitability. The plant ceased operations in 1971 but remained under the responsibility of URAMEX until 1985, the year in which URAMEX was liquidated. The facility was returned to the Mining Development Commission along with approximately 35 000 tons of uranium tailings generated during the two years of plant operation, and around 1735 tons of non-processed uranium ore. The tailings were deposited on a non-stabilized provisional impoundment located on the site – west of the main building in an area called zone 1 (see Fig. 1). The ore was deposited in an area to the east of the main building in zone 2. Zone 3 included the grinding section, the processing building, the machine room, the laboratory, and transit areas between buildings. (This layout and nomenclature were adopted for the remediation and dismantling activities). In September 1992, the Mining Development Commission was also liquidated and the facility and the radioactive material were transferred to the Mining Development Trust (FIFOMI). This transference also included rights, obligations and non-fulfilled commitments. 185 TOPICAL SESSION 7 FIG. 2. Villa Aldama Plant Layout. 2. NEED FOR REMEDIATION MEASURES The facility, the tailings and the ore were given little attention for more than 20 years until 1991, the year in which the Nuclear Safety and Safeguards National Commission (CNSNS) identified the need for remediation actions due to the following facts: (1) The growth of Ciudad Aldama. The plant and the onsite impoundment for the tailings were located only a few hundred metres from houses and other inhabited buildings. Projections suggested that the population of the city would continue growing at an increasing rate, raising the risk of direct exposure to radiation and the risk of intake of radioactive material by members of the public; (2) The original impoundment and the ore were located over a ground water body from which water is extracted to be used as a part of the city’s urban services. (Groundwater is approximately 20-30 metres beneath the surface at the site); (3) The original impoundment and the ore were located on the slope of a hill which is part of a rainwater basin; (4) The edges of the original impoundment were made of non-stabilized filling soil, and therefore the material was not properly immobilized and the integrity of the impoundment was not assured. 3. REMEDIAL ACTIONS In order to decide how to proceed for the remediation of the site, several meetings, involving the main entities were held in 1991. Those involved were: CNSNS as the regulatory body, FIFOMI as the owner of the site, Ciudad Aldama Government as the affected party (but also in a role of supporting party), and the Nuclear Research National Institute (ININ) as FIFOMI’s technical support organization. As a result of these meetings, it was decided to carry out the following actions (to be performed by the ININ): (1) The removal of the tailings from the site (zone 1) These activities were divided into two stages. 186 FABIAN ORTEGA The first stage started in July 1994. During the first stage 35 000 tons of uranium tailings and 1735 tons of uranium ore were removed from the site. The tailings were taken to the Peña Blanca uranium mining site, which is the place where the uranium mineral came from. It was necessary to construct a new impoundment at Peña Blanca for the disposal of the uranium tailings removed from the Villa Aldama facility. However, due to the long period that the tailings had remained at the Villa Aldama Site in an impoundment without impermeable layers, the soil beneath the tailings was contaminated by the uranium tailings. This soil did not meet the criteria established by the CNSNS, so it was determined that a second removal stage was necessary. The second stage started in 1996 and ended in 1997. During this period, an additional 30 000 tons of contaminated soil were taken to the Peña Blanca disposal site, making a total amount of 65 000 tons of waste disposed. (2) The removal of uranium ore (zone 2) The 1735 tons of uranium ore were also moved to the Peña Blanca site, and deposited in the amortizing zone of the impoundment facility. (3) The decontamination of the buildings and the equipment (zone 3) Mineral, tailings and other material with high concentrations of uranium, were removed from the process buildings. Walls, floors and process equipment were decontaminated using aggressive methods such as high pressure water (hydro-laser), mechanical brushing and the use of strong solvents (fuel oil and mixed acids). The decontamination of zone 3 spanned the time period December 1993 until March 1994. The goal of the decontamination of buildings and equipment was to take the contamination to levels below the criteria given by the CNSNS. However, some components could not be decontaminated as required by the authority and they had to be dismantled and removed. The destination for this radioactive material was a mine gallery called Las Margaritas at the Peña Blanca mining site. The amount that had to be moved was about 30 tons. After that, the mine gallery entrance was sealed with concrete. 4. CRITERIA APPLIED FOR CLEARANCE At the time that the remediation actions were required by the regulatory body (1991), the regulation involving soil and buildings clearance had not yet been established. The CNSNS had therefore to issue provisional specific clearance criteria for the release of soil, buildings and equipment. These criteria were issued specifically for application to the remediation activities at the Villa Aldama Uranium Extraction Plant, and were not to be used elsewhere. The criteria and requirements established by the CNSNS [1] were as follows: (1) The average concentration of Radium-226 in 100m2 of land shall not be above the background levels by more than: – 0.185 Bq/g (5 pCi/g) averaged over the first 0.15 m of the soil; – 0.555 Bq/g (15 pCi/g) averaged over 0.15 m thick layers of soil more than 0.15 m below the surface; (2) For occupied or habitable buildings: 187 TOPICAL SESSION 7 – The average annual concentrations of Radon-222 short lived decay products (including the background) shall not exceed 0.02WL; – The exposure rate shall be reduced to as low as reasonable achievable, but shall not be above the radioactive background by more than 20 µR/h; (3) In order to release the facility, equipment and any other components for unrestricted use, they shall comply with the following requirements: – No paint or any other cover shall be applied to contaminated surfaces of equipment or structures unless a reasonable effort has been made to reduce contamination below the applicable limits stated in Table I of the Regulatory Guide 1.86 of the US Atomic Energy Commission; this shall be determined by direct measurements, and appropriate records shall be generated; – Reasonable efforts for the removal of the residual contamination shall be carried out; – Contamination levels shall be determined on the internal surfaces of process piping, drain lines or ducts; this determination shall be carried out by direct measurements in appropriate accessible points representative of the contamination levels inside such pipes lines or ducts. 5. RESULTS OF THE REMEDIATION ACTIONS Despite the efforts applied in the removal of uranium ore, tailings and contaminated soil, the contamination in the land area of the facility (zone 2 and 3) still persisted, although at lesser concentrations than previously. The options considered to address this situation were: – To take even more contaminated soil to the disposal facility at Peña Blanca site; or – To cover the soil with a 0.15 m thick layer of alluvium, establishing restrictions for the use of the land. The involved parties CNSN, ININ, FIFOMI, and the Local Government, discarded the first option and agreed to proceed according to the second one. The results obtained from applying this option were quite good in terms of the resulting exposure rate [2].. However, in terms of contamination, a few persistent spots remained with concentrations of Radium-226 slightly above the given criteria. Therefore, the CNSNS established the following conditions [3] for the restricted use of the land and buildings on the site: – Agricultural activities and shepherding of cattle will not be allowed; – The construction of habitation buildings will not be allowed; – Drilling for water wells will not be allowed; – The minerals yard (zone 2) can be used only as a transit zone as long as the radiation levels remain slightly above the background levels; – For any activity carried out in the property, it shall be guaranteed that the personnel will not stay more than 40 hours a week, averaged on an annual basis. 188 FABIAN ORTEGA The above restrictions are still in force and the CNSNS periodically carries out visits to the site to verify that these conditions are met. At the present time, the local government of Ciudad Aldama is responsible for the former facility including the land and buildings. The main processing building of the plant is now used as a warehouse for several types of construction materials that will be used in public works; the yards of the property are now used as parking areas and a service station for local government vehicles (zone 2) and as a depository for plastic residues that will be recycled (zone 3). 6. LESSONS LEARNED The remediation actions at the former Villa Aldama Uranium Extraction plant prevented a potential risk situation for the population of Ciudad Aldama. However, remediation could have been avoided if a proper and timely decommissioning of the facility had been carried out. Because responsibilities for the site passed from one entity to another, there was a delay in concluding the decommissioning activities. This delay was enough to allow the migration of contaminants to the underlying soil with the resulting potential for groundwater contamination. The delay also allowed the expanding city of Ciudad Aldama to approach too close to the site. Additionally, the site selection process for the plant was performed in the late 1960s when no regulation or recommendations existed at national, or even at international level, and so more priority was granted in the siting process to having easy access to urban services, and less to issues with potential safety impacts such as projections of future activities and populations in the region or the proximity of the facility to groundwater. REFERENCES [1] [2] [3] COMISIÓN NACIONAL DE SEGURIDAD NUCLEAR Y SALVAGUARDIAS, Criterios Para garantizar la seguridad radiológica de la población y el medio ambiente, durante el desmantelamiento de la Planta de Villa Aldama, AOO.211/646/94, México D.F. (1994). FABIAN ORTEGA, R., Decommissioning of Villa Aldama Uranium Extraction Plant, in Proceedings of the International conference on Lessons Learned from the Decommissioning of Nuclear Facilities and the Safe Termination of Nuclear Activities, 11-15 December 2006, Athens, Greece, International Atomic Energy Agency, Contributed Paper IAEA-CN-146-026, IAEA, Vienna (2006). COMISIÓN NACIONAL DE SEGURIDAD NUCLEAR Y SALVAGUARDIAS, Liberación Condicional del predio de Villa Aldama, AOO.200/116/98, México D.F (1998). 189 OCCUPATIONAL EXPOSURE DURING REMEDIATION WORK AT A URANIUM TAILINGS PILE M.L. DINIS, A. FIÚZA Geo-Environment and Resources Research Centre, University of Porto, Portugal Abstract The aim of this study is to assess the occupational exposure at an abandoned uranium mining site due to work activities involving tailings pile remediation. A hypothetical scenario has been created in which the workers involved in the remediation activities are exposed to radiation through internal and external pathways. The results indicate that occupational radiation doses may reach a significant fraction of occupational radiation protection limits. For future tailing site remediation projects, which are planned in Portugal, individual dose levels should therefore be carefully measured, controlled and registered. Also, optimization techniques to reduce individual and collective doses in the remediation work activities should be implemented. 1. INTRODUCTION The exploitation of uranium ore in Portugal took place from 1913 to 2000. There were mining activities at 61 sites, mostly at small open pits, although there were also some underground mines. The great majority of the mining sites are located in the districts of Guarda and Viseu (central-east Portugal). In this region, the country’s most important mine, the Urgeiriça mine, is located. From 1913 to 1944, it was only mined for radium. After World War II, its purpose changed and in 1951 a chemical treatment plant for the production of lowgrade uranium concentrates was built. Later, the plant was modified for the production of high grade uranium concentrates. The ores from the Urgeiriça mine, as well as from other Portugese uranium mines, were processed in the uranium mill facility built near to Urgeiriça. Tailings from this facility include most of the radionuclides contained in the processed ores (those of the uranium decay chains), as well as some minor amounts of residual chemicals [1]. Since 1996, the Portuguese government has had to deal with the decommissioning of the mines, mills and other facilities and the rehabilitation of the mining sites. In particular, for the remediation of the Urgeiriça uranium site, a reclamation programme was instituted on July 20th, 2005. At this site, the rehabilitation of the Old Dam was considered to be a key element of the overall environmental remediation programme. The programme at the Urgeiriça site also included remediation of the industrial area, where the remains of the former milling and processing plants were located, as well as two former stockpile areas, one for ore and another for waste rock. Some of the waste arising from the industrial area had to be transferred to the tailings pile. After remediation, the tailings were to be fenced off to prohibit public access [1]. These works were planned for completion before the end of 2007. In fact, the tailings pile rehabilitation was concluded in April 2008. This paper focuses on the potential occupational exposure during the Old Dam remediation. The tailings at this site were a source of external radiation and also a significant source of radon gas and airborne dusts. During the remediation only external radiation doses were monitored. In fact, the workforce could have been exposed to radiation through three main exposure pathways: i) inhalation of radon decay products, ii) inhalation of dust-borne long-lived alpha emitters and iii) external radiation. This paper describes a preliminary assessment with limited data and focuses, in particular, on radon inhalation and external (gamma) radiation exposures. 191 TOPICAL SESSION 7 2. METHODS AND MATERIALS 2.1. Occupational exposure in remediation/rehabilitation activities Occupational exposure is defined by the International Commission on Radiological Protection (ICRP) as all exposures incurred at work as a result of situations that can reasonably be regarded as being the responsibility of the operating management [2]. The European Council Directive 96/29 EURATOM stipulates a limit on exposed workers of 100mSv in a consecutive 5 year period subject to a maximum effective dose of 50mSv in any single year. Below this dose limit, the principle of optimization requires that any radiation exposure should be kept as low as reasonably achievable (ALARA). When the annual dose limit is exceeded, the regulatory body can permit this exposure by considering the individual case and/or imposing work conditions and dose restrictions for the successive years. The exposure scenario adopted in this study considers both internal and external radiations exposures. The critical group is represented by an average adult worker, involved in the remediation of the tailings, assumed to be exposed during an 8-hour work day, 5 days per week, 48 weeks per year (assuming that he/she is away on vacation for 4 weeks per year), for 3 years. It was also assumed that all of the working time is spent outdoors. It is recognized that these assumptions are conservative and are likely to result in dose estimates at the upper end of the likely range. The relevant pathways considered for the workers exposure are radon inhalation and gamma radiation from the tailings. 2.2. Sampling A radon survey over a 13.3 ha area of the tailings pile was carried out during two field campaigns: in March 2001 (45 sampling points) and in August of 2002 (22 sampling points). The radon concentrations in the atmospheric air measured at 1 m above the soil ranged from 195 to 1205 Bq/m3, with an average value of 557 Bq/m3 [3]. To assess the external dose, in the absence of direct measurements of external radiation, the doses were estimated based on radionuclide concentrations in the soil determined for individual radionuclides by gamma-spectrometry (Table 1). TABLE 1. ESTIMATED RADIONUCLIDE CONCENTRATIONS IN SOIL AND DOSE COEFFICIENTS [4, 5] Radionuclide Average soil concentration (Csoil,i) (Bq/kg) ± Dose coefficients (DCext) (Sv/s)/(Bq/m2) U 483 ± 975 1.48 x 10-16 234 Th 6506 ± 14 262 8.32 x 10-18 226 Ra 3004 ± 5692 6.44 x 10-18 235 192 210 Pb 3046 ± 5541 2.48 x 10-18 137 Cs 9.9 ± 10.1 2.85 x 10-19 40 K 1738 ± 871 1.46 x 10-16 DINIS, FIÚZA 3. RESULTS 3.1. Effective dose assessment The effective dose received by a worker depends on many factors including the radon concentration, the exposure time, the exposure frequency and the characteristics of the radon decay products are given by equation (1): DRn CRn DCinh E f f eq (1) where DRn is the annual dose resulting from radon inhalation (mSv/year), CRn is the average radon concentration in air breathed at the tailings pile (Bq/m3), DCinh is the radon effective dose equivalent factor, (mSv/(Bq.h/m3), Ef is the outdoor exposure frequency (hour/year), feq is the equilibrium factor for radon decay products. The recommendations of the United Nations Scientific Committee on the Effects of Atomic Radiations (UNSCEAR) for the conversion of potential alpha energy exposure (Bq. h/m3) to effective dose equivalent (nSv) have been adopted [6]. A value of 9 nSv per Bq.h/m3 was adopted for the radon effective dose equivalent factor. This conversion factor incorporates an adult average breathing rate of 19.2 m3/d. An outdoor exposure frequency of 1920 hours per year and an equilibrium factor for radon decay products of 0.4 were assumed. For external exposure due to contaminated ground surfaces (Dext,i), the dose coefficients (Table I) were converted into the appropriate units by assuming a soil density of 1600 kg/m3 () and a soil depth contamination of 1 m (Ts) [5]. Dext ,i Csoil,i DC ext E f 3600 Ts (2) The dose estimates obtained from the assessment of exposure from external radiation and from intake of radon were combined for the assessment of the value of total effective dose for comparison with dose limits. 3.2. Summary results For the hypothetical exposure scenario, the effective dose for one year’s radon exposure at 557 Bq/m3 is 3.85 mSv while, for external exposure, the estimated gamma radiation dose is 4.5 mSv/year. The total effective dose is obtained by summing the doses resulting from internal and external exposure. The value for the total effective dose is 8.35 mSv/year. 4. CONCLUSIONS This assessment, because of limited data and the associated uncertainties, should be regarded as only indicative of the likely exposures received by workers. Nevertheless, it is clear that the workers involved in the Old Dam remediation could have been exposed to significant radiation doses via both internal and external pathways. In addition, radiation doses due to the inhalation of dust containing radionuclides, which were not considered in the assessment, may also contribute significantly. External exposure to gamma radiation (54%) 193 TOPICAL SESSION 7 and internal exposure due to the inhalation of radon (46%) were both found to contribute significantly to the total dose. The results show that occupational radiation doses for this assumed exposure scenario reach a significant fraction of the protection limits. If it is assumed that their exposure to work activities is for three years, the dose would be about 25% of the 100 mSv limit for the consecutive five years of exposure. These calculations were done assuming that no radiation protection precautions were applied during work activities. Further remediation actions are planned for other former uranium tailings sites in the vicinity of the Old Dam. This preliminary assessment indicates that, for these planned remediation projects, improved radiation protection procedures and surveillance of workers should be implemented. The individual worker dose levels, therefore, should be carefully measured, controlled and registered. Optimization techniques to reduce individual and collective doses should be established. Radiation exposure of the workers should be reduced by proper planning and use of protective equipment in order to keep doses as low as reasonably achievable (ALARA). Implementing some simple precautions, such as the wearing of appropriate work clothes and dust masks would contribute to this objective. Additionally, workers should be monitored and controlled periodically in order to assess the exposure being received. REFERENCES [1] [2] [3] [4] [5] [6] 194 EUROPEAN COMMISSION, Verifications Under the Terms of Article 35 of the Euratom Treaty, PT-06/07 (2006). INTERNATIONAL COMMISSION ON RADIOLOGICAL PROTECTION, The 2007 Recommendations of the International Commission on Radiological Protection, Publication 103, Annals ICRP 37(2–4), Elsevier, Amsterdam (2007). EXMIN, Estudo Director de Áreas de Minérios Radioactivos – 2.ª fase. Companhia de Indústria e Serviços Mineiros e Ambientais, SA (2003). FALCÃO, J.M., et al., MinUrar, Minas de Urânio e seus Resíduos: Efeitos na Saúde da População, Relatório científico I, Publ. INSA, INETI, ITN (2005). ECKERMAN K.F., RYMAN J.C., Federal guidance Report n.º12, Exposure-to-Dose Coefficients for General Application, Based on the 1987 Federal Radiation Protection Guidance, EPA-402-R-93-081 (1993). UNITED NATIONS SCIENTIFIC COMMITTEE ON THE EFFECTS OF ATOMIC RADIATION, Sources, Effects and Risk of Ionization Radiation. United States Scientific Committee on the Effects of Atomic Radiation, Report on General Assembly (2000). BASELINE RADIOLOGICAL SURVEY OF THE URANIUM–BEARING REGION OF POLI (NORTHERN CAMEROON) S. SAÏDOU***, F. BOCHUD*, S. BAECHLER*, K.N. MOÏSE**, P. FROIDEVAUX* * University Institute for Radiation Physics, Lausanne, Switzerland ** Centre for Atomic Molecular Physics and Quantum Optics, University of Douala, Douala, Cameroon *** Institute for Geological and Mining Research, Yaoundé, Cameroon Abstract This paper describes a baseline study of the uranium-bearing region of Poli where it is expected that the uranium deposit of Kitongo will be exploited in the near future. Soil, water and foodstuffs were sampled. The results show that activity concentrations of natural radionuclides in soil and water samples are low and comparable with global averages, but higher in foodstuffs (vegetables) (210Po and 210Pb). Further elaborated studies of this type should be undertaken by the company that develops the mine, prior to the beginning of operations. 1. INTRODUCTION Many reported studies reveal the impact of uranium mining and milling in the environment [1–9]. Prior to any uranium mining and milling, a baseline radiological study is necessary. Thus, measurements of naturally occurring radioactive materials (NORM) carried out within the framework of this study will be helpful to assess the environmental impact of the mining and milling of the Kitongo uranium deposit on the Poli region of Cameroon and later, to the site remediation after these processes are completed [9]. Since 1950, many geological studies for assessing the uranium potential of the Kitongo deposit have been carried out [10–12]. This deposit may be exploited in the near future by the Government of Cameroon [13]. To date, no radiological study in the area of this deposit has been undertaken. The main objective of the present work is to carry out the first part of a baseline study of the uranium-bearing region of Poli. This study has involved the sampling of soil, water and foodstuffs. Indoor radon concentrations were also measured in some dwellings as radon can contribute significantly to the radiation dose to the public. 2. MATERIALS AND METHODS 2.1. Sampling The uranium-bearing area zoned during uranium prospecting corresponds to a surface of 6710 km2 as illustrated in Fig. 1 [10–12]. In the present work, a surface of 144 km2 was sampled. The sampling plan comprises a square grid on which soil samples were collected at points separated by distances of 4 km. Each sampling point corresponds to a square surface area of 1 m2. At each point, a sample to 0-5 cm depth was taken giving an average sample whose dry mass is around 500 g. At Gata, a soil profile was sampled (0–5 cm, 5–10 cm, 10– 15 cm, 15–20 cm and 20–25 cm of depth) to study the vertical distribution of the radioactivity. In total, 20 soil samples were taken. In addition, 10 water samples and 10 195 TOPICAL SESSION 7 foodstuff samples were collected in the small town of Poli and its neighbourhood. The water samples were taken from rivers, wells and drinking fountains. All of the soil and foodstuff samples collected were dried, sieved (2 mm) and homogenized. FIG. 1: Strategy of sampling for the uranium-bearing region of Poli including the town of Poli and the Kitongo deposit. The points A, B, C and D circumscribe the area (6710 km2) over which a German institute undertook an airborne survey [10–12]. 2.2. Methods for radioactivity measurement The measurement procedure for uranium and thorium isotopes used in this study has been described in [14] and the procedure for 210Po determination is fully described in [15]. Uranium measurements were performed using thin films containing diphosphonate and sulphonate groups that have been shown to have the required selectivity for uranium [16]. For 226 Ra measurement, a thin film containing MnO2 in 100 ml of water sample was used [16]. After exposure, the thin films were dried at ambient temperatures and measured using αspectrometry. For 210Po measurements, a silver disc coated on one face with plastic rubber was put into weakly acidified water containing 50 mBq of the 209Po tracer. 210Po and 209Po were spontaneously deposited on to the disc. The silver disc, dried at ambient temperatures was measured using α-spectrometry. Gamma spectrometry measurements were performed using a Canberra p-type HPGe well detector (GCW4523) with a total active volume of 206 cm3, a relative photopeak 196 SAÏDOU et al. efficiency of 45%, and a resolution at 122 and 1332 keV of 1.24 and 1.93 keV, respectively. Treatment of the data was carried out using GENIE 2000 software. The spectrometer was calibrated using a liquid solution of 241Am, 109Cd, 57Co, 139Ce, 137Cs, 88Y and 60Co traceable to international standards and emitting γ-rays in the energy range 59-1836 keV. Coincidencesumming corrections for 88Y and 60Co were determined by Monte Carlo calculations [17]. The self-absorption correction factors were also calculated by Monte Carlo simulation [18]. 2.3. Measurements of radon in dwellings Indoor radon concentrations were measured in five dwellings in the uranium-bearing region of Poli by using electret detectors (E-perm) [19]. These detectors were exposed in dwellings (bedrooms, classrooms and offices) for a three month period. 3. RESULTS AND DISCUSSION 3.1. Radioactivity in soil The measurements in 20 soil samples are summarised in Fig. 2. The activities of 210Po and Pb are higher compared to other members of the 238U series. The results presented in Fig. 3 show an exponential decrease of the 210Po and 210Pb activity concentrations with sampling depth. The enrichment of soil surface (0–5 cm) in 210Po and 210Pb is explained by the deposition of radon progeny coming from the disintegration of radon in atmosphere after emanation. A similar result was observed for 210Po and 210Pb around closed uranium mines in Portugal [8]. 208Tl activity is lower than the equilibrium value due to the branching ratio (36%) of its mother product, 212Bi. 210 Activity (Bq/kg) 1000 100 10 FIG. 2. Box plot of the activity (Bq/kg) distribution of 40K and natural series 232 Th in 16 soil samples from the uranium-bearing region of Poli. 235 K40 Tl208 Bi212 Pb212 Ra224 Th228 Ac228 Th232 Po210 Pb210 Bi214 Pb214 Ra226 Th230 U234 Th234 U238 U235 1 U, 238 U and The average activities observed in the world are 420 Bq/kg for 40K, 38 Bq/kg for 238U and 45 Bq/kg for 232Th [20]. Activities of 40K measured in 20 soil samples, as illustrated in Fig. 2, show a median activity of 552±10 Bq/kg, a mean activity of 506±3 Bq/kg and a maximal value of 1124±27 Bq/kg (Mont Tchegui sampling point). Fig. 2 shows median activities of 25±2 Bq/kg for 238U, 23.3±6.3 Bq/kg for 226Ra and 30.5±1.7 Bq/kg for 232Th. Radioactivity levels in the region of Poli are comparable to global averages and, as might be 197 TOPICAL SESSION 7 expected, lower than reported results from measurements [8–9] undertaken in the environments of closed uranium mines. Sampling depth (cm) 5 Po-210 Pb-210 10 15 20 25 20 FIG. 3. Vertical distribution of point. 40 60 Activity (Bq/kg) 210 Po and 210 80 Pb in materials sampled at the Gata sampling Activity (Bq/kg) 100 10 1 0.1 0.01 U235 U238 U234 Th230 Ra226 Pb210 Po210 Th232 Th228 K40 FIG. 4. Box plot of the activity concentration (Bq/kg) distribution in foodstuffs frequently consumed in the region of Poli. 3.2. Radioactivity in foodstuffs From Fig. 4., it can be observed that activity concentrations of 40K are high compared to the values observed for the other radionuclides. This is not of great concern from the standpoint of radiation protection due to the homeostatic regulation of 40K in the human body. The activities of 210Po and 210Pb are higher in vegetables due to the deposition of radon progeny. The activities measured in beef are 5±0.5 Bq/kg for 210Po and 5±1 Bq/kg for 210Pb; this can also be explained by the deposition of radon progeny in pastureland as well as the ingestion of soil by cattle. 3.3. Radioactivity in water All measurements of 226Ra in water were under the limit of detection of α-spectrometry (10 mBq/L). Fig. 5 presents activities of 238U, 234U and 210Po respectively. All the reported results show that radioactivity in water of the region of Poli is low compared, for instance, with radioactivity around the closed uranium mine of Rayrock [7]. 198 SAÏDOU et al. 16 Activity (mBq/l) 14 12 10 8 6 4 2 0 U235 U238 U234 Ra226 Po210 . FIG. 5. Box plot of activity distribution in water (river, well and drinking fountain) of the uranium-bearing region of Poli. 226Ra is represented by its limit of detection in water. 3.4. Radon in dwellings Table 1 presents the results of 222Rn measurements in dwellings in the Poli region. The average indoor concentration (without values obtained for the office) is 120±21 Bq/m3. The value obtained for the office is 2000±100 Bq/m3 which is very high compared to the world average value of 40 Bq/m3 and this value was identified as being in need of further investigation. Many studies have been reported on measurements of radon in dwellings [4, 21–25]. The reported results reveal the large variation in the radon level in houses. It has been recognised that in most houses with high radon levels, the main source is not the building material but the convective radon influx from the soil. The radon level depends also on geological and meteorological factors, ventilation conditions and other factors [26]. TABLE 1. CONCENTRATION OF 222RN IN 5 DWELLINGS OF THE URANIUMBEARING REGION OF POLI Exposure area Inn Room Classroom Parlour Office 4. Concentration (Bq/M3) 11519 11318 10619 13718 2000100 CONCLUSION In this environmental baseline study of the uranium-bearing region of Poli, it has been found that soil, drinking water and food do not contain high levels of radioactivity, although the leaves of vegetables contain relatively higher levels of 210Pb and 210Po. Any changes in environmental radioactivity due to mining activities will be evident by comparison with the results of this study and further studies of this kind. Once uranium ore is brought from depth to the surface, 222Rn emanation and 210Pb and 210Po deposition might lead to an increase in the radiation dose to the population of the Poli area. Thus, no mining licence 199 TOPICAL SESSION 7 should be given by national authorities without the mining company being required to undertake an adequate monitoring programme. Well water may also be an interesting component in which to assess any damage from mining to the environment because of the very low levels of uranium and radium radioisotopes in water at the present time. REFERENCES [1] [2] [3] [4] [5] [6] [7] [8] [9] [10] [11] [12] [13] [14] [15] [16] [17] [18] [19] 200 VANDENHOVE, H., SWEECK, L., MALLANTS, D., et al., Assessment of radiation exposure in the uranium mining area of Mailuu Suu, Kyrgyzstan. J Environ Radioactivity 88 (2006) 118139. MARTIN, P., TIMS, S., RYAN, B., et al., A radon and meteorological measurement network for the Alligator Rivers Region, Australia. J of Environ Radioactivity 76 (2004) 35-49. MARTIN, P., TIMS, S., MC GILL, A., et al., Use of airborne -ray spectrometry for environmental assessment of the rehabilitated Nabarlek uranium mine, Australia. Environ Monit Assessm 115 (2006) 531-553. GORJANACZ, Z., VARHEGYI, A., KOVACS, T., et al., Population dose in the vicinity of closed Hungarian uranium mine, Rad Prot Dosim 118 (2006) 448-452. UZUNOV, I., DIMITROV, M., STEINHÄUSLER, F., Environmental radiation levels and occupational exposure due to uranium mining and milling operations in Bulgaria, Radiat Prot Dosim. 45 (1992) 141-143. VAUPOTIC, J., KOBAL, I., Release of radium from an abandoned uranium mine site: Zirovski Vrh Uranium mine, Slovenia. J of Radioanal Nucl Chem 1 (1999) 107-111. VESKA, E., EATON, R.S., Abandoned Rayrock uranium mill tailings in the Northwest Territories: environmental conditions and radiological impact, Health Phys. 60 (1991) 399-409. CARVALHO, F.P., MADRUGA, M.J., REIS, M.C., et al., Radioactivity in the environment around past radium and uranium mining sites of Portugal, J of Environ Radioactivity 96 (2007) 39-46. WINKELMANN, I., THOMAS, M., VOGL, K., Aerial measurements on uranium ore mining, milling and processing areas in Germany, J Environ Radioactivity 53 (1981) 301-311. GEHNES, P., THOSTE, V., Rapport sur la mission d’expertise du projet –Prospection d’uranium au Nord-Cameroun, 16 Oct-19 Déc 1980, rapport non diffusé, Hanovre (1981). OESTERLEN, M., Uranium exploration in North Cameroon, region of Poli. The Kitongo uranium exploration, Nov. 1982-Apr. 1983. Unpublished report, Hannover (1981). THOSTE, V., Uranium exploration in North Cameroon, region of Poli. Project definition, execution and results, Jan. 1982- Dec. 1984. Unpublished report, Hannover (1985). MEADON, H.M, Nuclear Energy Corporation, Geological review of the Kitongo uranium deposit, Poli area, Northern Cameroon (2006). SAÏDOU, BOCHUD, F., LAEDERMANN, J-P., et al., A comparison of alpha and gamma spectrometry for environmental radioactivity surveys, Appl Radiat and Isot 66 (2008) 215-222. SAÏDOU, BOCHUD, F., LAEDERMANN, J-P., et al., Calibration of an HPGe detector and selfattenuation correction for 210Pb: Verification by alpha spectrometry of 210Po in environmental samples, Nucl Instr and Meth A 578 (2007)_ 515-522. SURBECK, H., Alpha spectrometry sample preparation using selectively adsorbing thin films, Appl Radiat Isot 53 (2000) 97-100. DÉCOMBAZ, M., GOSTELY, J.J., LAEDERMANN, J-P., Coincidence-summing corrections for extended sources in gamma-ray spectrometry using Monte Carlo simulation, Nucl Instr and Meth A 312 (1992) 152-159. BOCHUD, F., BAILAT, C.J., BUCHILLIER, T., et al., Simple Monte Carlo method to calibrate well-type HPGe detectors, Nucl Instr and Meth A 569 (2006) 790-795. KOTRAPPA, P., BRUBAKER, T., DEMPSEY, J.C. et al., Electret ion chamber system for measurement of environmental radon and environmental gamma radiation, Radiat Prot Dosim 45 (1992) 107-110. SAÏDOU et al. [20] UNITED NATIONS SCIENTIFIC COMMITTEE ON THE EFFECTS OF ATOMIC RADIATION, Sources and effects of ionizing radiation, United Nations (2000). [21] COMMISSION FEDERALE DE LA PROTECTION CONTRE LES RADIATIONS ET DE SURVEILLANCE DE LA RADIOACTIVITE, Analyse des contributions à l’irradiation de la population Suisse en 2004 (2005). [22] MAGALHAES, M.H., AMARAL, E., SACHETT, I., et al., Radon-222 in Brazil: an outline of indoor and outdoor measurements. J of Environ Radioactivity 67 (2003) 131-143. [23] FAISCA, M.C., TEIXEIRA, M., BETTENCOURT, A. O., Indoor radon concentrations in Portugal: a national survey, Radiat Prot Dosim. 45 (1992) 465-467. [24] BINNS, D., FIGUEIREDO, N., MELO, V.P., et al., Radon-222 measurements in a uraniumprospecting area in Brazil, J of Environ Radioactivity 38 (1998) 249-254. [25] SOMLAI, J., GORJANACZ, Z., VARHEGYI, A., et al., Radon concentration in houses over a closed Hungarian uranium mine, Sci Total Environ. 367 (2006) 653-665. [26] INTERNATIONAL COMMISSION ON RADIOLOGICAL PROTECTION (ICRP), Protection against radon-222 at home and at work, Pergamon Press, Oxford (1993). 201 ROMANIAN EXPERIENCE IN THE REMEDIATION OF NORM CONTAMINATED SITES – A CASE STUDY O. VELICU*, A. TOMA** * ** National Commission for Nuclear Activities Control, Bucharest, Romania Nuclear Activities Autonomous Administration, Pitesti, Romania Abstract In January 2006, the National Commission for Nuclear Activities Control (CNCAN) received an official letter from the Mayor of a village claiming that an area of the local environment was radioactively contaminated due to some past liquid discharges from gas exploitation in the area. This paper describes the steps taken by CNCAN to investigate the situation and to resolve it by a programme of remediation which involved the polluter, the local community, the radiological assessment organization and local and national regulatory authorities. 1. INTRODUCTION In Romania, naturally occurring radioactive materials (NORM) have been produced as a result of various industries, such as uranium and non-uranium mining and milling facilities, chemical fertilizer production, oil and gas extraction and exploitation, etc. These industrial facilities are at different stages in their life cycles: some are still operating but many of them have ceased operations and are, at present, at an advanced stage of decommissioning. The nuclear field in Romania is governed by the Law No. 111/1996, on the safe deployment, regulation, licensing and control of nuclear activities. The general radiation protection requirements stipulated by this law are detailed by the Fundamental Norms on Radiological Safety, approved by the National Commission for Nuclear Activities Control (CNCAN) Presidential Order No. 14/2000. Chapter VII of these Norms is dedicated to situations of significantly increased exposure due to natural sources and Chapter X to radiation protection in the case of interventions. More detailed requirements on radiological safety during working activities involving NORM were issued in November 2008 as a result of the European Communities’ Phare project No. 017-519-03.03, ‘Development of CNCAN capabilities regarding the regulatory aspects of Naturally Occurring Radioactive Materials (NORM) and Technologically Enhanced Naturally Occurring Radioactive Materials (TENORM) related activities’. However, these regulations do not address past activities. There are no specific requirements for intervention in the case of chronic exposure to radiation or to environmental radioactive contamination. The principles and general requirements for environmental protection in Romania are established under the Romanian Government Urgent Ordinance no. 195/2005, approved with modifications and completions by the Law no. 265/2006. Specific requirements for the investigation and assessment of soil and sub-soil pollution, as well as for the remediation of affected areas are established by the Romanian Government Decisions no. 1408/2007 and 1403/2007, but they do not address radioactive contamination. In 2008, the Ministry of Environment and Sustainable Development initiated a process of developing similar Government Decisions for radioactively contaminated sites; a first meeting of the working group was held, in order to justify the need to develop such Decisions. 203 TOPICAL SESSION 7 2. CASE PRESENTATION 2.1. Identification of radioactively contaminated land In January 2006, CNCAN received an official letter from the Mayor of a village situated in the west of the country, claiming that an area of the local environment was radioactively contaminated due to some past liquid discharges from gas exploitation in the area. CNCAN investigated the area in February 2006, performing measurements and environmental sampling for laboratory analysis. Fig. 1 shows the investigated area, located to the north-easterly limit of the forest in the vicinity of the village and comprising a drainage channel (2 m wide, 475 m long) and a woodless area with a meandering water flow (4 m wide, 80 m long) linked to a drainage ditch (1 m wide, 155 m long). The drainage channel is almost covered with bushes and small trees. At the time of the investigation, both the drainage channel and ditch were partly covered with ice. FIG. 1. The contaminated site. The ambient gamma radiation dose rate values measured in the area are generally within the typical range of natural background, except for the drainage channel, where values two to three times higher than background were measured on the banks. The middle of the channel showed the highest values (up to 6 times higher than natural background). Four samples of water, soil and sediment were collected from the hotspots for subsequent gamma-spectrometric analyses. The water sample showed a 40K activity concentration equivalent to natural background levels. In the soil and sediment samples, radionuclides from the 238U and 232Th series were identified at concentrations one order of magnitude higher than the average concentrations in undisturbed soil of Romania. 204 VELICU, TOMA Consequently, CNCAN confirmed the presence of the radioactive contamination on the land but noted that it did not represent a significant radiological risk for the local population. However, it also noted that due to the fact that the neighbouring land has been sold and that houses are being built in the vicinity of the contaminated area, the presence of the enhanced NORM might become a real radiological risk in the near future. 2.2.1. Regulatory dispositions The polluter company was identified and, based on the provisions of the Fundamental Norms on Radiological Safety, it was asked: (a) To mark the perimeter of the contaminated area and to limit the access of the public inside the perimeter; (b) To assess the level of radioactive pollution of the contaminated area; and (c) To send the results to CNCAN, in order for it to establish the appropriate remediation actions. 2.2.2. Immediate actions Warning signs were posted in March 2006. The building of a fence around the contaminated area took more than 6 months, due to all of the authorizations and approvals necessary from different public authorities (local public administration, land administration, forest administration, gas transport company) but also because of the time taken to identify all the owners of the land (including one private person). 2.2.3. First assessment of the radioactive pollution of the contaminated area In order to assess the level of radioactive pollution of the contaminated area, the polluter company contracted the Pitesti Nuclear Research Branch, (Radiation Protection Laboratory), which is approved by CNCAN, to perform radioactivity measurements in environmental samples. It was led by a qualified radiation protection expert. The radiological investigation was performed in 2007, while both the drainage channel and the drainage ditch were flooded, and it consisted of: – Radiological mapping, performed by systematic measurements of the radiation count rate 10 cm above the ground at different steps along three mapping elements; – Measurement of the ambient equivalent dose rate 1 m above ground; – Field sampling and laboratory spectrometry analysis: 8 soil samples were collected from hot spots by core drilling down to 80 cm. In order to determine the depth migration profile of the radionuclides, the cores were divided into 5 segments representing different depths (0 – 20 cm, 20 – 35 cm, 35 – 50 cm, 50 – 65 cm, 65 – 80 cm). Five background soil samples were collected, including one depth profile; the others were taken from the 20 cm top layer of soil. Ten samples of vegetation were collected (one background), to assess the radionuclide transfer from soil to plants. Four surface water samples were collected from the contaminated area and one sample of well water from the Gas Separators Station. All samples were prepared following laboratory procedures and were analyzed by high resolution gamma spectrometry. The count rate values obtained by direct measurement were converted in units of ambient equivalent radiation dose rate and processed via a bi-variate interpolation method following grid generation by a linear kriging method. In Fig. 2, these values are presented as dose rate maps for each of the radiological mapping regions. 205 TOPICAL SESSION 7 Area were considered to be contaminated when the background ambient dose rate was exceeded by at least two times. On this basis it was concluded that the extent of the contamination was approximately 1500 m2. The ratios between 238U and 232Th progeny concentrations in soil samples from the area and in the background sample are generally higher than 1 in the 0–20 cm and 20–35 cm layers, with higher values in the first layer. Maximum values of the ratios are registered for 226 Ra in the first layer and they vary between 7 and 47. For each sample, excepting one, the radionuclide concentrations decrease to the average concentrations of the background depth profile within 20 to 35 cm. One soil core shows a greater depth migration of radionuclides, probably because it was collected from near the discharge point. FIG. 2. Radiological mapping of: (a) drainage channel, (b) woodless area, (c) drainage ditch. The radionuclide concentrations in the water samples from the area are similar to that of the background sample. The contaminant transfer factors from soil to vegetation are in good agreement with the ranges of values indicated in the literature for the radionuclides under consideration. Taking into account the extent and the depth of the contaminated soil layer, it is estimated that there is a maximum of 550 m3 of contaminated material. The assessment of the radiation doses to the public was done using the RESRAD 6 computer code, developed by Argonne National Laboratory in the United States of America. The source term was derived from the soil measurement results. A contaminated surface of 1500 m2 was assumed and, for conservative reasons, the recipient was placed directly above the contaminated area. A 35 cm thick layer of contaminated soil was assumed - without a covering layer. The following additional assumptions were made: density of soil 1.7 g/cm3, average wind velocity 1 m/s, annual precipitation rate 1000 L/m2 and the annual rate for soil irrigation 200 L/m2. The dose conversion factors were taken from The US Environmental Protection IAEA’s (EPA) Federal Guidance Reports Nos. 11 and 12. The consumption data 206 VELICU, TOMA for the public are the default values contained in the RESRAD code. On this basis, the additional dose to the population was calculated to be 25.4 mSv/y, of which 24.3 mSv/y is due to radon in homes built directly above the contaminated soil and inhabited for 24h/day. If the contaminated area is not used for building houses, the additional dose to population will be less than 1.1 mSv/y, representing about half of the dose received due to natural background radiation, but slightly exceeding the public dose limit of 1mSv/y. 2.2.4. Proposals for remedial actions The results of the study were presented to CNCAN in July 2007, together with the following proposals for further actions: (a) Removal of vegetation and drainage of water from the contaminated area; (b) Removal of a soil layer up to 35 cm thick in areas in which the radiation dose rate exceeds twice the natural background, under radiological supervision; (c) Final disposal of the removed material by one of the following methods: dispose of it in the National Low and Intermediate Level Radioactive Waste (LILW) Repository or in a sludge pile of the National Uranium Company; make a slurry of the soil and inject it into an oil extraction well or, dilute the contaminant concentration by mixing the contaminated soil with uncontaminated soil at the same location. In August 2008, during a meeting involving all stakeholders (the polluter company, the local environmental protection IAEA, the Mayor of the commune, CNCAN and the team responsible for the study), these proposals were discussed, with the following conclusions: (a) The removal of the vegetation and water from the contaminated land must be followed by another set of measurements, in order to check that there are no other hot spots; (b) The precise volume of the soil to be removed must be decided after this second study is completed; (c) The final disposal of the removed material in the National LILW Repository is not acceptable; (d) The National Uranium Company did not accept such material for disposal in its sludge piles; (e) The injection of the sludge into an extraction well is not feasible; (f) The dilution of the contaminated soil with uncontaminated soil was not agreed to by the Mayor of the commune, nor by CNCAN. 2.2.5. Second assessment of the radioactive pollution of the contaminated land In 2008, the same laboratory was contracted to perform new measurements and analyses in the same area, after the vegetation and water had been removed. All of the water and vegetal material removed was checked for radioactivity. It showed natural background values. The new study was performed in July 2008 using the same methods with slightly different approaches: – The radiological mapping was performed in smaller steps along the drainage channel; – The value of 300 nSv/h of ambient dose rate measured in contact was selected as a criterion for deciding if land is contaminated. With this, 8 hot spots were identified and marked on the field; – From each hot spot, soil samples were collected by core drilling down to 60 cm; the cores were scanned by in situ gamma-spectrometry and then divided into 4 segments of 15 cm each; 1 soil background sample was collected, representing one depth profile. 207 TOPICAL SESSION 7 Using the 300 nSv/h operational intervention level, the extent of the contamination was reduced to 560 m2. It was also calculated that removing the 35 cm top layer of soil from the hot spot areas would ensure the removal of 50% of the radioactive inventory. Taking into account the extent and the depth of the contaminated soil layer, a maximum of 200 m3 of contaminated material is estimated to be present. New calculations of the additional dose to the public resulted in similar values to those previously estimated, that is: 23 mSv/y, of which 21.8 mSv/y is due to radon in a house built on the contaminated land and inhabited for 24 h/d. If the area is not used for house building, then the dose would be 1.2 mSv/y. 3. REMEDIAL PROPOSALS These new results were presented to CNCAN in November 2008, together with the following proposals: (a) Removal of the 35 cm top layer of soil from the hot spot areas, under radiological supervision; (b) Intermediate storage of the removed material, in one of the polluter’s facilities, located near to the contaminated site; (c) Disposal of the contaminated soil in one of the future disposal facilities designed for hydrocarbon contaminated soil. CNCAN accepted these solutions, with the following conditions: (a) The removal of the contaminated soil will be approved only if the operations are assisted by radiologically qualified staff and performed under such conditions that the workers will not receive radiation doses higher than the public dose limit (1 mSv/y); (b) The intermediate storage of the contaminated soil will be approved only if the polluter company can demonstrate that it has the capacity to store it in a safe condition; (c) The site will be released from regulatory control only if, after the removal of the contaminated material, it can be demonstrated by measurements that the doses to the public will not exceed the legal dose limit (1 mSv/y); (d) If agreed by the environmental protection authorities, the disposal of the contaminated soil in one of the disposal facilities for hydrocarbon contaminated soil will be approved provided that the results of a radiological safety assessment of the disposal facility are acceptable. Due to weather constraints, the removal of the material cannot be carried out until March 2009. By the end of March, the polluter company must present to CNCAN its practical solutions for removing and storing the contaminated soil documented in such a manner as to demonstrate the observance of the previously stated conditions. 4. CONCLUSIONS From this example, several lessons can be learned. The remediation of a land area contaminated with radioactive material requires, first of all, an understanding of the physical processes taking place in the local environment. Unexpected delays must always be expected, starting with those involved in the search for persons owning the land and finishing with the problems caused by the different (technical) languages spoken by the authorities and companies involved in the process. The perception of the radiological risk by the public has also to be taken into consideration. Finally, it is a matter of finding the proper balance 208 VELICU, TOMA between the need for an intervention, public concern, regulatory requirements, the capabilities (and financial resources) of the polluter and the actual possibilities for effective remediation. REFERENCES [1] [2] [3] [4] [5] [6] [7] INTERNATIONAL ATOMIC ENERGY AGENCY, Radiation Protection and the Management of Radioactive Waste in the Oil and Gas Industry, Safety Reports Series No. 34, IAEA, Vienna (2003). INTERNATIONAL ATOMIC ENERGY AGENCY, Extent of Environmental Contamination by Naturally Occurring Radioactive Material (NORM) and Technological Options for Mitigation, Technical Reports Series No. 419, IAEA, Vienna (2003). INTERNATIONAL ATOMIC ENERGY AGENCY, Regulatory and Management Approaches for the Control of Environmental Residues Containing Naturally Occurring Radioactive Material (NORM) IAEA-TECDOC-1484, Vienna (2006). ARGONNE NATIONAL LABORATORY ENVIRONMENTAL ASSESSMENT DIVISION, An Assessment of the Disposal of Petroleum Industry NORM in Nonhazardous Landfills, DOE/BC/W-31-109-ENG-38-8 (1999). ARGONNE NATIONAL LABORATORY ENVIRONMENTAL ASSESSMENT DIVISION, Potential Radiological Doses Associated with the Disposal of Petroleum Industry NORM via Land spreading, DOE/BC/W-31-109-ENG-38-5 (1998). RAAN – SCN PITESTI, Nota tehnica nr. 5442/17.04.2007, Studiu de estimare a poluarii radioactive in zona Dumbravita, Timis (2007). RAAN – SCN PITESTI, Nota tehnica nr. 17012/07.10.2008, Studiu de estimare a poluarii radioactive in zona Dumbravita, Timis, etapa 1 (2008). 209 RADIOECOLOGICAL ASSESSMENT AND REMEDIATION PLANNING OF URANIUM MILLING FACILITIES AT THE PRIDNEPROVSKY CHEMICAL PLANT IN UKRAINE T.V. LAVROVA*, O.V. VOITSEKHOVYCH*, M.G. BUZINNY** * ** Ukrainian Hydrometeorological Institute, Kiev, Ukraine Marzeev Institute Hygiene and Medical Ecology, Kiev, Ukraine Abstract During the last 3 years, comprehensive radiological studies at the largest uranium production legacy site in the Ukraine, the Pridneprovsky Chemical Plant, have been carried out. The studies included gamma-dose mapping, radon-222 indoor and outdoor measurements, characterization of the dump sites and other hazardous facilities in this territory, as well as the preliminary dose assessment for people working at the industrial site. The paper describes the current status of remediation planning and the development of a new concept for the decontamination of the former uranium extraction facilities. 1. DESCRIPTION OF THE CURRENT STATUS OF THE LEGACY SITE Uranium mining was carried out intensively in Ukraine from the end of the 1940s to the beginning of the 1990s [1]. The former State Industrial Enterprise, the Pridneprovsky Chemical Plant (PChP), was one of the largest metallurgical facilities in the Former Soviet Union. Uranium ores were processed there from 1948 until 1991. During that time, uranium extraction was carried out on raw ore products delivered from Central Asia, Germany and the Czech Republic. In addition to imported ores, the PChP processed uranium-bearing sludge obtained from the smelting of iron ore from the uranium mines of Ukraine. In the early 1990s, due to disintegration of the former Soviet Union and consequently the uranium industry, the PChP was split into several separate enterprises and the processing of uranium was stopped. Nine tailings impoundments were created in an area containing about 42 million tonnes of uranium extraction residues with a total activity of 3.2 × 1015 Bq (86 000 Ci) [1]. Some of the highly contaminated equipment and metals used at the facilities were deposited at the storage sites within the area of the industrial zone of Dnieprodzerzhinsk, and other residues were disposed of about 14 km to the south east of the site. Each tailing impoundment has been inventoried based on information obtained from limited studies carried out during the past decade under a programme initiated by the Ministry of Fuel and Energy of Ukraine. However, the quality of the information available for each particular facility is not always reliable and more specific studies are required. 211 TOPICAL SESSION 7 FIG. 1. The PChP uranium production legacy site. 1-Tailing Zapadnoe, 2 – Tailing Centralny Yar, 3 - Tailing Yugo-Vostochnoe, 4 - Tailing D (Dnieprovskoe). The PChP territory is demarcated by a concrete fence. The area of the former PChP is divided by a railway into two large areas – the upper and lower parts. The main former uranium extraction facilities of PChP are situated in the upper part of the territory, and the largest tailings dump, Dnieprovskoe, is in the lower part, south of the Konoplyanka River – also referred to as the drainage canal (see Fig. 1). The upper part of the PChP territory, where the facilities are located, is much more contaminated with uranium-thorium series radionuclides than the lower part, due to the influence of the former uranium extraction facilities. No proper engineered barriers were provided for most of the tailings. After full capacity was reached, each tailing impoundment was usually covered with local soils, debris and other industrial waste. The distinctive feature of this site and its uranium residue tailings is that it is located within the populated area of Dnieprodzerzhinsk town (about 276 thousand citizens). The residential area is situated close to the industrial zone at a distance of 1–2 km from the nearest tailings (see Fig. 1). Therefore, the planning of the remediation of the former uranium production facilities is very sensitive to the opinions of the local population. 2. CURRENT ACTIVITIES IN AND AROUND THE PCHP TERRITORY In 2008, about 20 enterprises were still in operation in the PChP area. Most of the enterprises are not related to the former uranium processing activities. However, the workplaces of these enterprises are situated close to the highly contaminated tailings dumps and former buildings used for ore milling and extraction. The presence of contamination from these facilities may expose workers – externally due to gamma-radiation and internally due to radon–222 emanations and alpha-aerosol dispersion [2]. Some small enterprises make use of facilities which were not decontaminated in a proper way. The regulatory constraints for enterprises within this territory are still not well developed and require improvement. 212 LAVROVA et al. In addition to the enterprises already operating on this territory, there is significant interest in the further exploitation of the empty buildings on the site. For example, some workshops of the former hydrometallurgical plants that were used in the past for the extraction of the uranium concentrate have been sold to a new owner who intends to use these workshops for the processing of raw materials containing gold. It is clear that such ‘reprofiling’ of the former uranium facilities requires the complete decontamination of the facilities. Assessments have shown that there is an environmental impact at most sites where there are uranium tailings and waste. The impact is mainly due to releases of radionuclides from the uranium decay series (238U, 230Th, 226Ra, 210Pb and 210Po) to surface waters and to the groundwater table, as well as to radon emissions and dust dispersion into the air. Typical external gamma dose rates in the territory are generally rather low: 0.15 – 0.30 µSv/h. However, in some places, e.g. at the tailings surface, external gamma dose rates may reach 1 – 3 µSv/h and even 30 – 60 µSv/h. In such local ‘hotspots’ (e.g. the Central Yar tailings), 226Ra activity in soils at the surface of tailings reaches 0.1 – 0.2 kBq/g. The radon exhalation at such hot spots was measured to be 2 – 6 Bq/m2.s. Surveillance studies showed that the surface cover on such tailings is not sufficient to reduce the exhalation rates [2, 3]. Surface contamination on machinery, equipment, metal scrap etc. from the period of uranium production still exists and these items are kept in close proximity to the former uranium production workshops. Some of the most contaminated debris and metal were dumped together with uranium residues at the tailings sites. This material contains, among other nuclides, 226Ra and the long-lived radon daughter nuclides 210Pb and 210Po on the surfaces of contaminated equipment and scrap. Monitoring has shown that the activity concentration of 238U and 226Ra within the territory of PChP varies from hundreds to several thousands of Bq/kg; this may be compared with local soils which contain only 15–30 Bq/kg. The main long-lived radionuclides in the tailings are 234U, 238U, 230Th, 226Ra and 210Pb/ 210Po with activities of up to 105 Bq/kg. Aerosol pollution is also relatively high at the legacy site in comparison to naturally occurring background levels in the vicinity and is the result of wind driven resuspension and the dispersion of radon-progeny radionuclides over this area. The main contributor to radiation exposure in this territory is indoor radon. Concentrations of radon in some buildings used by workers in the industrial premises were found to be between 103 – 105 Bq/m3. The highest concentrations were found at some indoor working areas where highly contaminated facilities are still in place (uranium extraction facilities, transport tubes etc.). Maximum measured outdoor concentrations of radon are 2–4 102 Bq/m3. Preliminary dose and risk assessments carried out recently have shown that the current levels of alpha activity in surface water are rather low and lead to doses less than the permissible levels in Ukraine [1]. However, according to [3], the pore water in aquifers around tailing dumps is highly contaminated (the highest concentrations of alpha emitting radionuclides were 105 Bq/m3) and can pose a potential risk in the event of the protective dyke becoming damaged. This could result in the spillage of the highly polluted tailings pore water into the drainage canal and on to the Dnieper River. Under natural conditions, the pore water moves in the aquifer towards the Dnieper River very slowly. At present, the water in the drainage canal (Konoplyanka River) has gross alpha activity levels of between 0.3 and 0.6 Bq/L; this is 10 to 20 times higher than the background levels that have been found in the Dnieper River upstream of the drainage water inlet to the reservoir. The most significant source of Dnieper River pollution is tailings pile D, the closest pile to the Konoplyanka River. 213 TOPICAL SESSION 7 3. PRELIMINARY DOSE ASSESSMENT AND CONCLUSIONS BASED ON MONITORING DATA ANALYSES Radiation exposures due to external radiation, inhalation of contaminated aerosols and radon, and soil ingestion were calculated [2]. The results showed that external exposure and radon inhalation make the highest contribution to the total dose. Depending on the scenarios chosen, annual dose rates may exceed the dose limits for both Worker Categories A and B, i.e. 20 and 5 mSv per year, respectively. The radiation doses to people living in the vicinity of the PChP site are estimated to be less than 1 mSv per year for any potential scenario. However, an accidental situation which affected the tailing dams and removed the tailings cover could lead to significant radiological consequences which would still require long term surveillance for periods of 100 - 1000 years, or longer. For most workers whose workplaces are in buildings which are not contaminated or who are mainly working in non-contaminated areas of the site, annual doses are estimated to be in the range 0.1–0.5 mSv per year. The annual doses to workers whose workplaces are located near to tailing dumps or near to the contaminated buildings or who are regularly inspecting/monitoring the tailing dumps may vary from 1–12 mSv per year depending on their specific duties and the time spent in the contaminated areas or contaminated premises. The highest doses (30–45 mSv/a) will be received by those who have regular access to the contaminated premises and are involved in remediation activities involving the removal and utilization of the tailing materials and/or of the most contaminated equipment. The preliminary assessment concluded that the main priorities of the remediation plan should be the cleanup of the former uranium extraction facilities, proper surface coverage of the tailings or removal of the tailings to specially prepared tailing sites (with engineering barriers). Predictions based on the radionuclide migration model incorporated into the radiological assessment tool ‘Ecolego’ showed that proper soil coverage and removal of the tailing materials from the largest tailing site D would decelerate radionuclide transport into the Dnieper River for the next 500 years [4]. A new concept for remediation has been developed; it involves establishing the following pre-feasibility actions in further remediation planning: – To re-consider some of the legislative and regulatory norms - as a basis for safe management of the former uranium facilities (the new rules to be improved according to the principles of the International Basic Safety Standards [7]); – To extend the tailing dump characterization and inspection programmes taking into account the recommendations of the International Atomic Energy Agency; – To consider re-treatment (re-processing) options for some tailings materials as a part of the remediation process. The pre-feasibility studies are to be implemented by 2010 and will help in the selection of the most appropriate and economically justified options for remediation at the PChP industrial site. The experience gained from global best uranium facility remediation practices will be applied [5, 6]. Among the most pressing remediation problems still awaiting attention are: the highly contaminated buildings at the industrial sites; the phospogypsum cover, the integration of the largest tailing pile, Dnieprovskoe (tailing D), with other tailing materials; and the wet uranium Sukhachevskoe tailing pile (tailing S), which is still partly covered with water. One option to be considered is the deepening of the Konoplyanka creek to serve as a natural drainage canal for both the industrial site and the tailings pile D. 214 LAVROVA et al. The new concept considers, as the most preferable action, the removal of the relatively small tailing dumps over the territory and their transportation to the surface of the largest tailing D (about 1 km) with further conservation of the tailings pile using a multilayer soil cover. The State Programme of 2003 suggested removing all tailing dumps and contaminated materials to the tailing S – a distance of about 14 km. This would dramatically increase the project costs. However, both options are still to be finally evaluated taking into consideration social and long term ecological considerations by using multi-attribute assessment procedures. REFERENCES [1] [2] [3] [4] [5] [6] [7] INTERNATIONAL ATOMIC ENERGY AGENCY, Radiological Conditions in the Dnieper River Basin, IAEA Radiological Assessment Reports, IAEA, Vienna (2002). ENSURE: Assessment of Risks to Human Health and the Environment from Uranium Tailings in Ukraine, FACILIA, Phase-1, Final Report, Swedish Radiation Protection Institute – SIUS under contract UA401A/ 2007-09-24, Stockholm (2008). VOITSEKHOVYCH, O.V., et al., Substantiation of radionuclide transfer reduction to the environment and human body in uranium sites, Interim Project Report, Ukrainian Hydrometeorological Institute, STCU Project No. 3290 (2007). SKALSKY, A., et al., Problems of the hydrogeological monitoring at the Pridneprovsky Chemical Plant (Dneprodzerzhinsk, Ukraine), in Uranium Mining and Hydrogeology, September 2008, Freiberg, Germany, Springer (2008). UMTRA, Uranium Mill Tailings Remedial Action, U.S. Uranium production facilities: operating history and remediation cost under uranium mill tailings remedial action project as of 2000, Energy Information Administration, Official Energy Statistics from the US Government, (2005). http://www.eia.doe.gov/cneaf/nuclear/page/umtra/title1map.html INTERNATIONAL ATOMIC ENERGY AGENCY, Uranium Mine Remediation in Times of Revival of Production, UMREG Monograph, Selected Paper - limited distribution, IAEA, Vienna (2008). INTERNATIONAL ATOMIC ENERGY AGENCY, International Basic Safety Standards for Protection against Ionizing Radiation and for the Safety of Radiation Sources, Safety Series No. 115, IAEA, Vienna (1996). 215 EXPERIENCE GAINED IN TRANSFERRING WISMUT RADIATION PROTECTION KNOW–HOW TO INTERNATIONAL PROJECTS IN URANIUM MINING REMEDIATION P. SCHMIDT*, C. KUNZE**, J. REGNER* * Wismut GmbH, Chemnitz, Germany ** WISUTEC Wismut Umwelttechnik GmbH, Chemnitz, Germany Abstract Since 1990, the federal-owned corporation WISMUT GmbH has been rehabilitating the legacies left behind by some 40 years of intensive uranium ore mining and processing operations in Eastern Germany. Starting in 1996, WISMUT has been involved in transferring the know-how gained in the rehabilitation of the WISMUT sites to projects outside of Germany. As a rule, radiation protection management and radioecological issues are key elements of these activities. In this work, benefits have been obtained both from the substantial similarities prevailing in the countries of the former Soviet Union and in Eastern Germany after termination of uranium production and from the commonality of the problems to be resolved. This paper describes the possibilities and limits of transferring radiation protection know-how to countries where the rehabilitation of uranium mining liabilities is often to be carried out under circumstances of limited financial, material, and human resources. It also describes some lessons learnt. Conclusions for application to future projects are derived. 1. INTRODUCTION Forty years of intensive mining and processing of uranium ores in the heart of densely populated areas in Eastern Germany left behind considerable liabilities. They are being cleaned up by the federal-owned corporation WISMUT GmbH under an environmental restoration project which is unique in terms of complexity and size. Since 1996, the corporation has also been involved in transferring the know-how gained in the rehabilitation of WISMUT sites to projects outside of Germany. These projects have been funded by the European Community, the World Bank, and other international organizations. In 2002, the WISMUT subsidiary WISUTEC (Wismut Umwelttechnik GmbH) was established with a view to marketing the know-how gained during the rehabilitation of uranium mining sites in Eastern Germany. So far, more than 25 projects have been successfully implemented outside Germany. The know-how transfer has been primarily targeted at countries of the former ‘Eastern Bloc’, to the Russian Federation and countries of the Commonwealth of Independent States (CIS) in Central Asia, but also to countries in Africa and North America. As a rule, consulting activities focus on key elements such as radiation protection management and radioecological issues. Given the commonality of the inherited histories, the similarity of environmental problems to be resolved, and, last but not least, the former working-level contacts between the experts of WISMUT and their counterparts in countries in Eastern Europe and the former Soviet Union, WISMUT was (and still is) well positioned for the task of transferring knowhow to Eastern Europe and CIS countries. Examples of recent or ongoing projects are listed in Table 1 below. 217 TOPICAL SESSION 7 TABLE 1. EXAMPLES OF TRANSFER OF KNOW-HOW BY WISMUT/WISUTEC Project/beneficiary country Task Phare Project PH4.2 / BUL, CZ, EST, HU, PO, RO, SV Provision of means to assess radiological risks Environmental Impact Assessment (EIA), conceptual design, supervision EIA, identification of remedial measures, stakeholder involvement EIA, optimization of remedial measures, supervision of implementation Sillamäe Tailings Pond Remediation Project /Estonia EUROPAID Project Lermontov/Russia Disaster Hazard Mitigation Project Mailuu Suu/Kyrgyzstan 2. FromTo 19971999 Funded by EC 19992008 NEFCO 20042005 EC 2005- World Bank CHARACTERISTICS OF PRE-REMEDIAL CONDITIONS IN BENEFICIARY COUNTRIES AND PROBLEM DEFINITION The termination of uranium production in the beneficiary countries (and at WISMUT) was marked by the following features: (1) (2) Uranium production was often carried out in complete disregard for the most elementary rules of occupational health and safety and of environmental protection. As a consequence, an existing long term radiological situation was left behind which requires the application of radiological protection principles for intervention situations; Operations were chiefly terminated in a very abrupt way: no preparations had been made for closure, knowledge of remediation concepts and know-how on techniques were almost non-existent, regulations and methodology for rehabilitation design were usually absent, generally few expert personnel were available, and the technical equipment necessary for conducting remediation (including the means for radiological data acquisition and for radiological assessment) was lacking; During the production operations, no financial provisions had been made for rehabilitation. Due to the economic situation prevailing in the countries, the state-owned corporations were unable to carry out remediation according to international standards. Remediation had to be implemented under the conditions of constrained resources; The old culture of secrecy prevailed. Arrangements for communicating with the local population and the culture of ‘stakeholder involvement’ were hardly developed. (3) (4) The following is a typical list of issues which the experts from WISMUT/WISUTEC have had to deal with: – Definition of evaluation criteria, in collaboration with national authorities; – Radiological impact assessment as an integral part of an Environmental Impact Assessment (EIA); – Introduction of appropriate measurement techniques for the determination of contamination levels as well as procedures for measuring releases, including QA/QC procedures; – Development of a radiological monitoring system, including individual monitoring; – Optimization of remediation measures; – Introduction of procedures to document the progress of the remediation effort; 218 SCHMIDT et al. – Ensuring practical radiation protection of employees, minimization of remediationrelated radiological exposure of the population; – Management of radioactive waste and residues; – Licensing management; – Training and further education of employees involved, capacity building; – Public relations, stakeholder involvement. 3. EXPERIENCE WITH MEANS OF KNOW-HOW TRANSFER 3.1. Body of rules and regulations, licensing management There was a tendency in CIS countries for authorities to wish to retain the standards of the former Soviet Union. This phenomenon made it difficult to develop country-, site-, and object-specific solutions and to assign pertinent priorities. As an example, in the case of a geo-mechanically unstable waste dump located far from residential areas and in conditions of limited national financial resources, it seemed to be justified to limit remediation efforts to regrading (in order to eliminate immediate hazards), while refraining from capping (which is required by national standards). In this particular case, the idea was somewhat difficult to transmit to national authorities. In matters like these, WISMUT has been successful when presenting arguments based on international documents. The Safety Standards, Technical Reports and Technical Documents of the International Atomic Energy Agency [1–5] as well as the recommendations of the International Commission on Radiological Protection (ICRP) [6] and of other international agencies provided a sound basis. In addition, case studies of remediation actions conducted in Germany proved helpful in overcoming a reluctance to move from previous approaches. 3.2. Provision of means From the 1990s through to the present time, various programmes have provided countries with instrumentation and software for radiological measurements, modelling, and interpretation. There have been shortcomings in coordinating such provisions both in the donor organizations and within beneficiary countries. Also, issues related to providing practical training in the use of hardware and software, to providing for Quality Assurance/Quality Control (QA/QC) (e.g. in radiation metrology), and to long term funding of operating costs, did not always receive due attention. In implementing the European Union Phare Project PH4.2, under the terms of which technical equipment designed to establish the radiological situation at uranium mining sites was provided to seven East European countries from 1997 to 1999, WISMUT contributed, in almost the same proportion, to the purchase of hardware, on the one hand, and to the efforts for training, QA/QC means, and the continuation of operations, on the other. 3.3. Training Workshops and training courses are essential elements of assistance, irrespective of whether conducted in a beneficiary country or in the country of the project consultant. Choosing appropriate candidates is a key to success. Training courses should put a great deal of emphasis on imparting practical skills. WISMUT/WISUTEC’s project experience shows that best results are achieved by ‘on-the-job’ training schemes. Funded by the IAEA, the European Union, and other organizations, more than 10 experts have completed study visits at WISMUT on radiological aspects of uranium mining site remediation in recent years. 219 TOPICAL SESSION 7 Accompanied by WISMUT specialist staff, these experts went on field trips to perform joint measurements, carried out laboratory work or worked together on modelling etc. 3.4. Joint project work As a rule, projects begin with the acquisition of data and the subsequent radiological evaluation of that data. Rather than distinguishing between consultant and beneficiary, emphasis is again on joint efforts for concept building, acquisition and evaluation of data. Seeking and finding common ground and learning from each other – this approach has also provided benefits to WISMUT. In 2001 and 2002, for instance, WISMUT and the DIAMO Corporation (from the Czech Republic) initiated a project located in the German-Czech border region which was designed to adjust the methods used to acquire and evaluate radiological data. The project was conducted in the two neighbouring towns of Johanngeorgenstadt (on the German side) and Potucky (on the Czech side) along the common border in the Ore Mountains. Jointly performed measurements, modelling, exposure assessments, and the exchange of results brought about harmonization in dealing with radiological issues in adjacent former uranium mining regions. 3.5. Radiation protection management under conditions of constrained resources A ‘performance-based regulatory framework’ is better suited than a ‘prescriptive regulatory framework’ for supporting radiation protection management under conditions of constrained resources. State-of-the-art of science and technology are not always implementable under these conditions. Focussing on essentials, assigning priorities and selecting the proper degree of required accuracy can help to provide sufficient radiological data for the justification and optimization of radiation protection measures, irrespective of the scarcity of available means. An example of such an approach is WISMUT's combination of field and laboratory measurement methods by making use of statistical evaluation procedures and of problem-oriented follow-up calibration (see the flow chart in Fig. 1). Under such a scheme, the calibration and the laboratory measurement programme is reduced to a minimum while local experts on site perform field measurements with a limited but sufficient degree of accuracy. 3.6. Stakeholder involvement After forty years of uranium production in Eastern Germany, conducted to some extent under severe secrecy regulations, finding ways of dispelling mistrust and ‘building bridges’ with the local population was the only possible way for WISMUT to implement its environmental restoration project. This was achieved by active public relations work, by disclosing the whole range of environmental data and integrating the public concerned into the process of identifying optimized remedial options. Area rehabilitation was and is being carried out with the goal of returning reclaimed land to productive reuse (for example, the integration of rehabilitated mine dumps into the park landscape of the Schlema spa centre). In the framework of consulting projects performed in Eastern Europe, experience gained in stakeholder involvement was actively described and illustrated (for example, by inviting political and societal decision makers to attend site visits at WISMUT). As a result, diverging stakeholder interests in identifying remedial solutions in have been overcome. 220 SCHMIDT et al. Problem Definition Approach Large quantities of materials or large-area contaminations, respectively, require determination of representative activity levels Intelligent combination of field and laboratory measurements, statistical evaluation of field measurement series Step 1: Sampling, laboratory determination of nuclide vectors, identification of key nuclides or parameters, respectively Step 2: Selection of appropriate field measurement method to determine key parameter Step 3: Problem-oriented follow-up calibration between lab and field measurement methods Step 4: Field measurements, Quality Assurance by accompanying laboratory analyses Step 5: Establishment of representative activity levels by statistical evaluation of field data FIG 1. Flow chart of the combination of field and laboratory measurement methods for release measurements of materials and areas. 4. LESSONS LEARNED AND CONCLUSIONS Key elements in successfully transferring radiation protection know-how in the framework of international projects designed to remediate the legacies of uranium mining and processing operations are: – The application of international standards and technical documentation, in particular, those published by IAEA and ICRP; – Transferring personal experience gained, with due regard to country-specific conditions; – Development of site and object specific solutions; – Imparting practical skills by ‘learning on the job’ schemes; – Ensuring stakeholder involvement; and – Implementation of process-oriented solutions consistent with conditions of limited resources. 221 TOPICAL SESSION 7 REFERENCES [1] [2] [3] [4] [5] [6] 222 FOOD AND AGRICUTURE ORGANIZATION OF THE UNITED NATIONS, INTERNATIONAL ATOMIC ENERGY AGENCY, INTERNATIONAL LABOUR ORGANIZATION, OECD-NEA, PAN AMERICAN HEALTH ORGANIZATION, WORLD HEALTH ORGANIZATION, International Basic Safety Standards for Protection against Ionizing Radiation and for the Safety of Radiation Sources, Safety Series No. 115, IAEA, Vienna (1996). INTERNATIONAL ATOMIC ENERGY AGENCY, Decommissioning of Facilities for Mining and Milling of Radioactive Ores and Close Out of Residues, Technical Report Series No. 362, Vienna (1994). INTERNATIONAL ATOMIC ENERGY AGENCY, Planning for Environmental Restoration of Uranium Mining and Milling Sites in Central and Eastern Europe, TECDOC 982, Vienna (1997). INTERNATIONAL ATOMIC ENERGY AGENCY, Generic Models for the Use in assessing the Impact of Discharges of Radioactive Substances to the Environment, Safety Reports Series No. 19, Vienna (2001). INTERNATIONAL ATOMIC ENERGY AGENCY, Environmental and Source Monitoring for Purposes of Radiation Protection, Safety Standards Series, RS-G-1.8, Vienna (2005). INTERNATIONAL COMMISSION ON RADIOLOGICAL PROTECTION, 1990 Recommendations of the International Commission on Radiological Protection, Publication 60, ICRP (1990). JUSTIFICATION OF REMEDIATION STRATEGIES IN THE LONG TERM AFTER THE CHERNOBYL ACCIDENT S. FESENKO*, P. JACOB**, A. CHUPOV*, A. ULANOVSKY**, I. BOGDEVICH***, N. SANZHAROVA****, A. PANOV****, N. ISAMOV****, V. KASHPAROV*****, Y. ZHUCHENKA****** * International Atomic Energy Agency, Vienna, Austria ** Institute of Radiation Protection, Neuherberg, Germany *** Research Institute for Soil Science and Agrochemistry, Minsk, Belarus **** ***** ****** Russian Institute of Agricultural Radiology and Radioecology, Obninsk, Russia Ukrainian Institute of Agricultural Radiology, Chabany, Ukraine Gomel University, Gomel, Belarus Abstract Following the accident at the Chernobyl nuclear power plant, a number of different remedial actions were developed and implemented in Belarus, Russia and Ukraine. Recommendations on the application of countermeasures and remedial actions were published by the International Atomic Energy Agency in 1994. Since then, new information on the behaviour of radionuclides in the environment and on the effectiveness of countermeasures in the long term has been obtained. On this basis, a new approach has been developed on remediation strategies for contaminated areas and has been successfully implemented in the affected countries. 1. INTRODUCTION The accident at the Chernobyl nuclear power plant (NPP) was the most serious radiation accident in the history of nuclear energy generation. More than 4.5 million hectares of agricultural lands were contaminated in Belarus, Russia and Ukraine. Consumption of contaminated products was, and remains, one of the main radiation exposure pathways for the population of the affected regions [1]. To protect people against radiation exposure, various large-scale remedial actions have been implemented in the affected areas. In all three countries, there are laws or acts of government requiring the optimization of countermeasures so as to reduce annual doses to the population. In this context, the International Atomic Energy Agency initiated a regional technical collaboration project called ‘Radiological support for the rehabilitation of the areas affected by the Chernobyl nuclear power plant accident’. In the frame of this project, a software tool called ReSCA (Remediation Strategies after the Chernobyl Accident) has been developed [2]. The software is based on experiences over two decades with countermeasures against radioactive contamination in the aftermath of the Chernobyl accident [3]. The International Commission on Radiological Protection (ICRP) in its Publication No. 103 recommends, for radiation protection purposes, the assessment of 223 TOPICAL SESSION 7 the dose to a ‘representative person’. The representative person is defined as: “a hypothetical construct, receives a dose that is representative of the more highly exposed individuals in the population”. The present work utilises this concept and the dose to the representative person is one of the main quantities used in the optimization process for remediation. The present study summarizes information on settlements which have less than 10 000 inhabitants (rural settlements) and for which the effective dose to a representative person exceeds 1 mSv/y. Practically all of these settlements have a rural character. External radiation and intakes of radionuclides from the consumption of locally produced foodstuffs, especially milk from private cows and mushrooms, are the major factors causing radiation doses from contamination of Chernobyl origin. The objectives of this study were: (i) to assess the present and future numbers of inhabitants of the settlements with annual effective doses to the representative person still exceeding 1 mSv; (ii) to discuss possible remediation strategies, their costs and impacts on the dose distribution; (iii) to provide general recommendations on remediation strategies more than two decades after the Chernobyl accident. 2. MATERIALS AND METHODS Settlements with less than 10 000 inhabitants, which had, according to official dose catalogues for 2004, annual doses to individuals exceeding 1 mSv, were defined as study settlements1. The data collected for the study settlements included the number of inhabitants, the number of grassland areas for cows, the mean 137Cs ground contamination density, the mean 137Cs concentrations in pork, potatoes and mushrooms, and the average consumption of locally collected mushrooms relative to the average consumption of mushrooms in the country. The data for the grassland areas include the number of cows, the distribution of soil types, information about countermeasures previously or presently applied, and the mean 137Cs concentrations in milk and beef. 3. RESULTS AND DISCUSSIONS For each of the study settlements, calculations were performed to evaluate the effective dose to the representative person, defined by the sum of the averages of the upper 10% of the effective dose distributions from external and internal exposure. The internal dose estimates were validated with data sets on whole body measurements in the course of the study. The external dose estimates had been validated previously. All study settlements which have, according to the ReSCA calculations, annual doses to representative persons in 2004 exceeding 1 mSv were defined as ‘affected’ and eligible for consideration for the implementation of remedial actions. Six remedial actions were included in the current analysis: radical improvement of grassland (RI); application of ferrocyn to cows (FA); feeding pigs with uncontaminated fodder before slaughter (FP); application of mineral fertilizers to potato fields (MF); information campaign on mushrooms and other forest produce (IM); removal of contaminated soil from populated areas (RS). Among the 545 study settlements, there were 290 settlements in which the effective dose to the representative person exceeded 1 mSv in 2004. In total, these affected settlements had 78 172 inhabitants, most of them (57 960) in Russia. The number of settlements with annual effective doses to the representative person exceeding 1 mSv is predicted to decrease 1 Three of the affected towns in Russia (Klimovo, Klintsy and Novozybkov) are not considered in the present study as they are non-rural. 224 FESENKO et al. because of natural reduction processes and radioactive decay to 121 by 2020 with a total of 35 044 affected inhabitants. Thus, without remedial actions the decrease is quite slow. The collective dose assessed for 2004 in the affected settlements is about 130 person-Sv, three quarters of this being accumulated in Russia. The distribution of the dose between external and internal exposures is very different in the affected settlements of the three countries: in Belarus, external exposure dominates; in Russia, both pathways are equally important; in Ukraine, the dose is nearly exclusively due to internal exposure. In about half of the Belarusian and Russian affected settlements, the annual dose from mushrooms is comparable to the annual dose from milk. In Ukraine, however, milk is the dominant contributor to internal exposure in most of the affected settlements. To consider possible alternatives, the results of the assessments were summarized for two options: remediation strategies 1 and 2. In the frame of the first strategy, the ‘social strategy’, higher attention was given to the acceptability of the suggested remedial actions. Strategy 2 is based on lowering costs per averted dose. Remediation strategies have been evaluated using expected annual doses in 2010 based on data for year 2004. If only very limited resources are available for remediation, then Strategy 1 (focussing on a high degree of acceptability) consists nearly exclusively of radical improvement of grassland. This has a remedial effect on the milk contamination for several years. Strategy 2, focuses, first on application of ferrocyn to cows, which has to be applied continuously, and in Belarus and Russia, on removal of highly contaminated soil from populated areas, which, on the one hand, reduces the exposure for all time, but, on the other hand, requires the disposal of contaminated soil. In Belarus and Ukraine, Strategy 2 is considerably more cost-effective than Strategy 1. General information on the effectiveness of the remediation strategies is given in Table 1. TABLE 1. COSTS, AVERTED DOSES AND COSTS PER AVERTED DOSE FOR TWO REMEDIATION STRATEGIES CALCULATED UNDER THE ASSUMPTION THAT 1 M€ IS AVAILABLE FOR REMEDIATION IN EACH AFFECTED COUNTRY Country Cost of remediation, k€ Averted dose (person-Sv) Strategy 1 Strategy 2 Belarus 1003 1002 Russia 1011 1003 61.1 73.0 17 14 378 2383 45.3 127.8 23.5 123.9 30 27 16 19 Ukraine Total b 1372 3386 Strategy 1 Strategy 2 Costs of 1 person-Sv averted, k€ 21.4 Strategy 1 27.3 Strategy 2 47 37 In Belarus, Strategy 1 shares the resources between radical improvement (RI) or ferrocyn application (FA) and removal of contaminated soil from populated areas (RS), while Strategy 2 is totally focused on RS. In Russia, Strategy 1 focuses on RI and FA, while Strategy 2 shares the resources between RI and FA, on the one hand, and RS on the other hand. In Ukraine, Strategy 2 reduces annual doses in all affected settlements below 1 mSv with costs of less than 0.4 M€. Strategy 1 is considerably less cost-effective and requires larger amounts of money for the remediation of grasslands by radical improvement. A large collective dose in the order of 120–130 person-Sv can be averted by the remediation strategies. Nevertheless, the number of inhabitants in Belarusian and Russian settlements with annual doses exceeding 1 mSv remains substantial. Compared to international values for the cost-effectiveness of actions to reduce occupational exposures, the recommended remediation strategies for rural areas affected by the Chernobyl accident are quite cost-effective (about 20 k€/person-Sv). 225 TOPICAL SESSION 7 The effect of the remediation is dependent both on site-specific factors, which were directly included into the analysis, and on funds available for remediation purposes. If only very limited resources are available, then there are considerable differences between the two strategies discussed earlier (Fig. 1). Strategy 1 consists nearly exclusively of radical improvement of grassland. This has a remedial effect on the milk contamination for several years. Strategy 2, however, focuses first on the application of ferrocyn to cows, which has to be applied continuously, and in Belarus and Russia on the removal of highly contaminated soil from populated areas, which, on the one hand, reduces the exposure for all time, and on the other hand, requires the disposal of contaminated soil. As might be expected, in Belarus and in Ukraine, Strategy 2 is considerably more cost-effective than Strategy 1. If more than 1 M€ is available for remediation, the situation becomes country-specific. In Belarus, the two strategies become more similar in terms of the effectiveness of remediation with increasing resources. In Russia, the difference between the two strategies persists up to resources of several M€, because of the large number of affected settlements. Strategy 1 starts to become less cost-effective for higher expenditures (Fig. 1). In Ukraine, Strategy 2 reduces annual doses in all affected settlements below 1 mSv with costs of less than 0.4 M€. Strategy 1 is considerably less cost-effective and requests larger amounts of money for the remediation. 160 Averted collective dose (person-Sv) Averted collective dose (person-Sv) 40 Belarus 30 20 10 Strategy 1 Strategy 2 0 0.0 0.5 1.0 1.5 2.0 2.5 3.0 Total cost of remediation (MEuro) 140 Russia 120 100 80 60 40 Strategy 1 Strategy 2 20 0 0.0 0.5 1.0 1.5 2.0 2.5 Total cost of remediation (MEuro) Averted collective dose (person-Sv) 70 60 Ukraine 50 40 30 20 10 0 0.0 Strategy 1 Strategy 2 0.5 1.0 1.5 2.0 2.5 3.0 Total cost of remediation (MEuro) FIG 1. Averted dose versus available funds for remediation purposes in Belarus, Russia, and Ukraine. The number of settlements with annual doses exceeding 1 mSv after application of the two remediation strategies is quite similar in Belarus and Russia. In Ukraine, remediation 226 3.0 FESENKO et al. Strategy 2 is considerably more effective in terms of the number of settlements with annual doses exceeding 1 mSv than Strategy 1; with a relatively small expenditure of resources, the annual dose in all settlements can be reduced below 1 mSv. 4. CONCLUSIONS The present analysis of possible strategies for remediation of rural areas affected by the Chernobyl accident, i.e. where annual effective dose to the representative person exceeds 1 mSv, shows that, even two decades after the Chernobyl accident, the application of remedial actions is still cost-effective. Thus, further remediation of the affected areas will result in considerable reduction of the radiation exposure of rural populations. REFERENCES [1] [2] [3] INTERNATIONAL ATOMIC ENERGY AGENCY, Guidelines for agricultural countermeasures following an accidental release of radionuclides, Technical Reports Series No. 363, Vienna (1994). JACOB, P., FESENKO, S., FIRSAKOVA, S.K., et al., Remediation strategies for rural territories contaminated by the Chernobyl accident, J Environ Radioactivity 56 (2001) 51-76. ULANOVSKY, A., JACOB, P., FESENKO, S.V. et al., ReSCA – decision support tool for remediation planning after the Chernobyl accident, Radiat Environ Biophys 50 1 (2011) 67-83. 227 EXPERIENCES IN THE REMEDIATION OF CONTAMINATED LAND I. ADSLEY, R. MURLEY, L. FELLINGHAM, K. STEVENS Nuvia Limited, Didcot, United Kingdom Abstract This paper provides details of a series of projects related to the remediation of contaminated land. Sites with different contamination issues have been selected to show the extent of the problems that may be encountered. The sites described include a nuclear bomb testing range, a radium luminizing site, an old nuclear experimental facility, and a tritium factory. Relevant aspects of legislation, assay and safety issues are considered for each site. 1. INTRODUCTION The paper describes the remediation of four sites contaminated with radioactive materials and, in some cases, chemicals. The sites represent a range of contamination situations resulting from various nuclear processes. The sites considered are: (a) (b) (c) (d) 2. The Maralinga Nuclear Weapons Test Site in Australia; The former United Kingdom Admiralty Research Centre at Ditton Park; The Southern Storage Area at UK Atomic Energy Authority, Harwell; A tritium contaminated site at Hayes in London. CASE STUDIES 2.1. Maralinga The Maralinga test site occupies some 3200 km2 and is located on the northern edge of the Nullabor Plain in South Australia, approximately 900 km north-west of Adelaide. Between 1953 and 1963, the British Government carried out seven atmospheric nuclear weapons tests and approximately five hundred and fifty small scale experiments (‘minor trials’) using nuclear materials at the site. These latter trials resulted in the dispersal of over 23 kg of plutonium, 22 kg of enriched uranium, 8447 kg of natural and depleted uranium and 102 kg of beryllium, as well as smaller amounts of other materials at various locations over the range. During the operation of the test site, various ’housekeeping‘ radiation surveys and cleanup operations were undertaken. Some of the materials used in the trials were gathered up and buried in various numbered and unnumbered pits throughout the range. As part of the work, an initial helicopter-based aerial survey was undertaken of all the significant sites to map the distributions of the significant gamma-ray emitters: 241Am, 60Co and 137Cs. The rehabilitation programme for the site was specified as a ‘risk reduction exercise’, not as a ‘cleanup’. The underlying assumption was that the site would be returned to its former Aboriginal owners, the Maralinga Tjarutja. They would return to live in their semitraditional lifestyle, albeit supplemented by certain modern accompaniments, such as imported foodstuffs, motor vehicles and health care. This semi-traditional lifestyle is associated with the intake of much higher levels of dust than is characteristic in the life patterns of western societies. Hence, the inhalation of plutonium-contaminated dust has been identified as the dominant pathway for radiation dose accumulation. The critical group was identified as Aboriginal children and the rehabilitation strategy was devised to ensure that the 229 TOPICAL SESSION 7 annual dose to individuals did not exceed 5 mSv. This dose limit was translated by the Australian Radiation Laboratory (ARL) into acceptable residual contamination levels for various parts of the site. These levels ranged from 1.8 to 4 kBq/m2 of 241Am; this radionuclide was used as a marker for the plutonium present. The key components of the risk reduction works were: (a) The construction of three large, 15 m deep, burial trenches at Taranaki, TM100/101 and Wewak; (b) The removal of contaminated soil to an average depth of 150 mm from approximately 2.2 km2 at Taranaki, TM100/101 and Wewak and its placement into the corresponding disposal trenches; (c) The removal of the concrete caps from the twenty one numbered pits in central Taranaki, followed by in-situ vitrification of their contents, using the Geosafe process, and replacement of the concrete caps and restoration of the surfaces to their natural levels; (d) The excavation of various other pits containing plutonium-contaminated debris and placement of the contents in the burial trenches; (e) The restoration of various other numbered and unnumbered pits by collection and burial of surface debris, compaction, importation of clean soil, re-contouring and the re-introduction of vegetation; (f) The installation of 100 km of marker posts at 50 m intervals throughout the outer plume areas to warn the Aboriginal population that they may hunt and traverse the area, but should not camp there permanently; (g) The removal of access routes to certain areas by destroying roads; and (h) The re-vegetation of selected areas. The bulk of the soil was removed using scrapers; an excavator was used to remove small areas requiring further treatment. In some areas the soil cover was very limited, and vacuum and rotary brush attachments were used to clean rock surfaces. The major hazard to the operators arose from the generation of plutonium-bearing dusts. The dust also caused recontamination during the rehabilitation process. A variety of measures were undertaken to minimise such dust generation. These included modifying facilities to reduce dust generation, e.g. by covering loads, restricting plant operating spreads and spraying areas with water prior to working them. In order to minimize risks to workers, operations were designed to keep the number of personnel present during the removal of active materials as low as possible. All vehicles were modified to have positively pressurised, sealed cabins with absolute filtered air supplies. Contaminated areas were surveyed at the end of each day and material was removed in sequence during the following day. This enabled a ‘survey – removal’ process to be adopted and allowed the process of personnel surveying during dust generation processes during the day to be dispensed with. Areas were re-monitored after clearance of active material and reworked if found to be still contaminated. All treated areas were independently surveyed by ARL, using a specially modified vehicle with a boom mounted, high purity germanium detector, to certify that all clearance criteria had been met. Finally, areas to be re-vegetated were treated to return the site to a condition close to its original state. 2.2. UK admiralty research centre at Ditton Park Ditton Manor Park is a 68 ha site located adjacent to the M4 motorway some 2 km to the south east of the town of Slough in the United Kingdom. The site was formerly used by 230 ADSLEY et al. the UK Admiralty for the development, manufacture and testing of compasses. These activities involved the use of radium-based luminizing paints. In March 1998, Ditton Manor Park was purchased from the UK Ministry of Defence (MoD) to become part of the corporate headquarters of a major computer software company. It comprised a listed moated manor house with various out-buildings, which had been extended and used as workshops and laboratories. Investigations had revealed widespread localized radioactive contamination of the ground over much of the site. In addition, many of the buildings were contaminated with radium and mercury. A site waste tip had been used and this was contaminated with radium, heavy metals and polyaromatic hydrocarbons. A remediation programme was developed to remove all significant historic contamination from the ground and fabric of buildings and to leave the site suitable for redevelopment without the need for any future special precautions. The current and future risks to the environment were to be eliminated. The remediation criteria were set on the basis of a quantitative risk assessment in close consultation with the prime regulator, the Environment IAEA, and also with the Local Authority. The criteria were established, based upon the proposed uses of the site and with public access to all areas outside the moat. They were also compatible with sensitive multifunctional use, e.g. for housing. A novel feature was the extensive use of the GroundhogTM gamma area surveying system in the characterization, remediation and validation of all land clearance. The Groundhog system comprises a highly sensitive NaI scintillation radiation detector linked to a GPS detector for position location and a data logger. A plot of a Groundhog survey showing regions of contamination is shown in Fig. 1. FIG. 1. Regions of contamination at Ditton Manor Park. At the onset of the works, comprehensive surveys were undertaken to further characterize the contamination present. Surveys were either conducted manually with a portable Groundhog system, or with four detectors mounted on a vehicle. These surveys set the scope for the remedial works and helped to finalize the areas requiring excavation and backfilling. In addition, the advanced surveys identified contamination of the building structures and defined the areas requiring remediation. 231 TOPICAL SESSION 7 The remedial works involved: (a) (b) (c) (d) (e) (f) (g) (h) (i) Advance surveys; Remediation of ground contamination - both chemical and radioactive; Remediation of non-listed buildings prior to demolition; Remediation of ground after demolition of non-listed buildings; Remediation of radioactive (radium) contamination of listed buildings; Remediation of chemical (mercury) contamination of listed buildings; Investigation and moat sediments and their subsequent remediation; Remediation of the cottage gardens along the estate edge; Extensive consultation with all key stakeholders. Regular liaison was established with the prime regulator, the Environment IAEA, in order to ensure that remediation criteria, waste handling and disposal methods met with their approval. This was the largest remediation project which had been undertaken in the United Kingdom of a site contaminated with 226Ra from luminising operations - in terms of both scale and cost. The works were successfully completed within a period of 9 months. All identified contamination was removed to below levels of concern. 2.3. Remediation of the southern storage area at UK Atomic Energy Authority (UKAEA), Harwell The Southern Storage Area (SSA) is a separate, security-fenced site, which is located approximately 1 km south of the main Harwell nuclear licensed site in the UK. It is approximately 7.3 hectares in area. The site was the main munitions storage area for RAF Harwell, which was a Second World War bomber and training aerodrome. It was subsequently used for radioactive waste storage, treatment and disposal operations by UKAEA during the early UK nuclear research programmes. A cleanup of the site was carried out during 1988–90 in order to eliminate the need for the site to be licensed under the Nuclear Installations Act; this was also required for the main Harwell site. As a result of the historical operations on the site, there were three main liabilities. They were the chemical pits, the beryllium pits and the common land, which is the remainder of the site. It was known that radioactive and chemical contamination was present due to past storage in the various pits. The waste segregation strategy was a key component of the programme. It was based on the following key steps: (a) Use of previous characterization results plus in-situ and excavation bucket monitoring for radioactive and chemical contamination by gamma, beta surface, volatile organic compound and mercury probes to provide initial segregation into exempt/special/controlled and low-level waste streams; (b) Packaging of the bulk of waste, excepting large artefacts, etc, into 1 m3 cube bags, which became the standard packaging volume; (c) Sampling of the waste during the filling of the 1 m3 bags and other waste containers; (d) Gamma and contamination monitoring of the faces of each bag. The former provided evidence of any significant gamma sources in each bag; (e) Gross / analysis of the homogenized sample from each bag; (f) High-resolution gamma spectroscopy of every bag of the potentially exempt waste. All waste arising from the site was consigned as low-level, exempt, controlled and/or special waste. The latter was dependent upon the levels of chemical contaminants present. 232 ADSLEY et al. Finally, in order to facilitate the remedial works, two authorizations were granted by the Environment IAEA. The first authorization was to accumulate and dispose of radioactive waste on the site. The second authorization was granted for a gaseous discharge from the SSA. Special sampling arrangements were made to comply with these authorizations. 2.4. Tritium contamination on a storage site at Hayes An industrial unit at Hayes near London was vacated after a 25 year lease had expired. It had been used by a company which collected redundant gaseous tritium light devices (GTLD). It was found that low level tritium contamination was left after the removal of these devices. Nuvia Limited was initially contracted to undertake a detailed survey of the buildings. In this first stage of the survey, a limited number of building samples were taken to gauge the spread and penetration of the tritium into the building fabric. This showed the contamination to be much greater and more widespread than previously thought and resulted in a further extensive survey, which included concrete cores from the floor slab together with soil samples from below the slab. The outbuildings were found to have widespread contamination in the range of thousands of Bq/g of tritium on the concrete base. Tritium had also migrated into the soil below the concrete slab. The main building slab and sub-soil were also contaminated with tritium up to levels of hundreds of Bq/g. Nuvia led negotiations with the Environment IAEA on behalf of the landlord to establish and agree a remediation plan and an end-point. The landlord wished to re-use the contaminated site and also to enable the use of the large adjacent area of industrial and commercial buildings that he leased to other tenants. Although the environmental impact of the contamination was not excessive, the definition of radioactive waste in the UK means that any material with anthropogenic radiological contamination above 0.4 Bq/g is radioactive waste. The amount of building materials and soil contaminated above 0.4 Bq/g was estimated to be 1500 te. Disposal of this amount of material would cost several million pounds. Some investigations and trials were undertaken to establish whether soil and concrete washing would remove the tritium to acceptable levels. However, it was soon established that the cost and commercial risk of soil washing did not make this an attractive option. The only disposal site available in the UK for this material is the National Low Level Waste Depository at Drigg in Cumbria. This site is both costly for disposal and represents a limited national resource so it was not the ideal disposal solution. Nuvia established that a commercially operated active incinerator was prepared to accept the waste for treatment. This process would drive off the tritium contamination from both concrete and soil and it could then be either collected from the flue gas as a liquid or dispersed to atmosphere with acceptably low environmental impact. Further negotiation with the Environment IAEA resulted in agreement that the incineration method of waste treatment for the concrete and soil contaminated with higher levels of tritium was acceptable. It was also agreed that soils at greater depth and contaminated to a level slightly above 0.4 Bq/g could be left in place without conditions being imposed on the development of the site. It was shown that this would not influence the site development work and that after re-development, the tritium would disperse and decay from these areas over time with minimal environmental impact. Nuvia undertook all of the demolition work and remediated the site to the agreed standards. 233 TOPICAL SESSION 7 3. SUMMARY Four completed projects which required the identification, assessment and removal of a variety of radioactive contaminants in land and buildings have been briefly described. All of the work was conducted to prescribed safety standards and within relevant legal environmental requirements. 234 ASSESSMENT OF CURRENT DOSES FROM URANIUM TAILINGS R. AVILA*, O. VOITSEKHOVYCH**, I. ZINGER*, P. KEYSER*** * ** *** Facilia AB Stockholm, Sweden EcoMonitor, Kiev, Ukraine Swedish Radiation Safety Authority, Stockholm, Sweden Abstract Assessments of radiation doses have been carried out in and around existing uranium tailings in Ukraine, Tajikistan and Uzbekistan. Radioactive contamination at these sites can potentially impact human health as nearby areas are often heavily populated. As an example, the current doses to humans were assessed in detail for one site. These first assessments should help in building more realistic scenarios and dose estimates. This work may be used as part of decision making on the most suitable remediation options based on the long term intended uses of the sites. 1. INTRODUCTION This paper summarises studies carried out around existing uranium tailings in Ukraine, Tajikistan and Uzbekistan in 2008. Specific assessments were carried out in Ukraine as part of a collaborative project between Swedish and Ukrainian authorities [1] and as part of expert missions on behalf of the International Atomic Energy Agency to Tajikistan and Uzbekistan [2] to define scenarios for dose assessments for the uranium mill tailings disposal sites. 1.1. Brief description of sites The following is a brief overview of the sites studied; more details are included in [1, 2]. In general, contamination at all sites is not spatially homogeneous; large variations exist in radionuclide levels in different parts of a given site. – Dniprodzerzhinsk (Ukraine). Nine tailing impoundments were created in the area; they contain about 42 million tonnes of radioactive waste with a total activity of 3.2 × 1015 Bq. Some of the waste was deposited within the territory of the industrial zone of Dniprodzerzhinsk, and some at about 14 km to the southeast of the site. The sites are located in and near to the Pridneprovsky Chemical Plant (PChP) in the town of Dniprodzerzhinsk (about 280 000 inhabitants); – Taboshar (Tajikistan). Tailings occupy a 54 ha area and contain about 7.6 million tonnes of waste. They are located a few kilometres away from the town (12 000 inhabitants). Some of the tailings are without any cover and represent a source of highly contaminated drainage and seepage water, which is migrating into surface water and to the shallow groundwater table. Due to hot climatic conditions, the drainage waters evaporate resulting in the precipitation of carbonate, sodium and sulphate complexes of uranium. This creates a salt cover of white colour with yellow uranile crystals, containing concentrations around 10–20 Bq/g of 238U; 235 TOPICAL SESSION 7 – Degmay (Tajikistan). This is the largest single uranium mill tailings site in Central Asia. It extends over 90 ha and contains about 20 million tonnes of uranium residue waste. The estimated total activity is about 1.6 × 1013 Bq. It is located 2 km from the Chkalovsk settlement (22 000 people) and 10 km from the town of Khudjand (164 000 inhabitants). Due to hot climatic conditions, the water from the tailings’ surface has evaporated, and the tailings pile has cracked leading to high 222Rn exhalation (36–65 Bq/m2.s). The 222Rn ambient concentration in air at the site varied from 200 to 1000 Bq.m-3; – Charkesar in (Uzbekistan). This is a uranium legacy site located in the suburb of the village of Charkesar (2500 people). The site extends over 20.6 ha and contains 482 thousand m3 radioactive waste with a total activity of 3 x1013 Bq. The ventilation shaft currently discharges contaminated water containing 238U at concentrations ranging from 26 to 36 Bq/L. 2. METHODOLOGY The assessments to derive current radiation doses to humans living in the vicinity of these sites were performed using the same approach for each site: – First, monitoring data was used to identify the hazardous areas; – For each hazard, exposure pathways, and associated models, were determined; – The hazards were then quantified in term of radiation dose rates from each pathway per unit time or for a given use of contaminated media, such as water and food. Once the exposed groups had been identified it was then possible to assess the existing radiation doses to the particular exposed population groups based on defined scenarios. This approach produces results which are only indicative of the current situation. In order to quantify the actual risks to individuals, further analyses are needed based on both current and future scenarios. These steps are not described in this paper. 3. IDENTIFICATION OF HAZARDS In this study, a hazardous area is defined as an area with elevated radionuclide or radiation levels, as compared with background levels. These areas pose an additional radiological hazard, as their occupancy by the population can result in radiation doses above those due to natural background radiation. Radiological hazards can also be caused by elevated radionuclide levels in water bodies, such as underground and surface waters. Monitoring data were used for each site to identify the hazardous areas, using information such as: – Gamma radiation dose rates outside and inside of buildings; – Radionuclide concentrations in aerosols, soils and tailing materials; – Radon concentrations outside and inside of buildings; – Radionuclide concentrations in water and food products, such as milk and meat (not yet done at the Ukraine site). 236 AVILA et al. 3.1. Dniprodzerzhinsk – Ukraine The monitoring data helped to identify a number of contaminated locations: inside and outside contaminated buildings (closed to public and due to be demolished); the PChP north part; hot spots in the forest; tailing Zapadnoe; tailing Central Yar; tailing Yugovoctochnoye; tailing Dniprovskoye; ponds near tailing Central Yar. From the description of the current activities on the PChP territory, it is clear that workers on the site receive the highest radiation doses if they spend part of their working hours near the hot spots, in the contaminated buildings or working at the tailings surface where the cover is not sufficient. The development and analysis of scenarios has been focused on critical groups of workers. Expansion of the scenarios to address risks to members of the public is scheduled for 2009. 3.2. Taboshar – Tajikistan The following radiological hazards were identified at the Taboshar site: elevated radionuclide and radiation levels a) outdoors at the Taboshar settlement; b) indoors at the Taboshar settlement; c) at the uranium tailings piles, which may affect the population which have free access to the tailing sites and use the tailings surface for the grazing of domestic animals; d) at the uranium pits (waste rock piles), where some local citizens spend part of their time visiting the waste rock piles and former uranium pits for swimming and for other private needs; d) in waters contaminated by the uranium tailings; and e) in waters contaminated by the uranium pits. 3.3. Degmay – Tajikistan The main exposure pathways for persons visiting this site are external exposure to gamma radiation and inhalation of radon and particulate bearing dusts. The following radiological hazards were identified at the Degmay site: elevated radionuclide and radiation levels a) in the Degmay settlement; b) at the uranium tailings; and c) in ground waters (water from local wells). 3.4. Charkesar – Uzbekistan It was found that the main radiological problem at Charkesar is that local citizens, in many cases, use tailing materials for the construction of their houses. The following radiological hazards were identified in the Charkesar site: elevated radionuclide and radiation levels in a) areas of the Charkesar settlement that are close to the industrial site (‘near settlement’); b) areas of the Charkesar settlement that are far from the industrial site (‘far settlement’); c) at the industrial site; d) in spring waters; e) in the mine waters; and f) in the river waters. 4. CURRENT RADIATION DOSE RATES 4.1. Derivation of doses To provide a basis for exposure assessments at sites of this type, the German Federal Ministry for the Environment, Nature Conservation and Reactor Safety has published a document containing appropriate models and parameters [3]. This document provides equations for estimating radiation exposures through all pathways that can be relevant at uranium mining and processing sites, namely: 237 TOPICAL SESSION 7 – External exposure caused by soil contamination for reference persons inside and outside buildings; – Exposure through contaminated aerosols inside and outside buildings; – Radiation exposure from locally grown foodstuffs; – Exposure through the direct ingestion of soil; – Determination of activity concentration in foodstuff; and – Exposure from the inhalation of 222Rn and its short-lived progeny. According to this methodology [3], the radionuclides to be considered for calculating doses are included in the following three decay chains: 1) 238U > 234U > 230Th > 226Ra > 210Po > 210Pb; 2) 235U > 231Pa > 227Ac; and 3) 232Th > 228Ra > 228Th. In the present study, dose calculations were only performed for the seven radionuclides: 238 U, 234U, 230Th, 226Ra, 210Po, 210Pb and 228Th, due to limitations in the availablility of data. This may lead to a slight underestimation of doses. The equations for dose calculations from the German report [3] were implemented in the software package Ecolego [4]. 4.2. Predicted dose rates Table 1 summarises the estimated radiation dose rates for the exposure pathways used in the model calculations. The results [1, 2] showed that external exposure and radon inhalation contributed the most to the total doses. Fig. 1 compares the four sites. Similar results are found at the sites, except for Dniprodzerzhinsk, Ukraine, where the measurenents were taken in highly contaminated locations aimed at worker dose estimation rather than in areas occupied by the local population. TABLE 1. DERIVED DOSE RATE RANGES IN µSV/H FOR THE FOUR STUDIED SITES Site Hazard Taboshar, Tajikistan Settlement outdoors Settlement indoors Tailings Uranium pit Settlement Tailings Far outdoors Far indoors Near outdoors Near indoors Industrial site Outside polluted building Inside polluted building PChP north part Hot spots Tailing Yugovoctochnoye Tailing Zapadnoe Tailing Dniprovskoye Tailing Central Yar Ponds (near tailing Central Yar) Degmay, Tajikistan Charkesar, Uzbekistan Dniprodzerzhinsk, Ukraine * * Results based on experimental data. 238 Total dose rates µSv/h Minimum Maximum 0.10 0.53 0.11 0.53 0.11 0.77 0.15 2.40 0.04 0.31 2.70 13.00 0.22 1.20 0.22 2.70 0.28 1.30 0.56 4.40 0.22 1.90 0.56 7.17 5.70 21.80 0.15 0.49 4.93 18.40 1.30 30.60 0.09 2.65 0.15 0.49 0.52 3.29 0.53 2.35 AVILA et al. µSv/hr maximum minimum 35,00 30,00 25,00 20,00 15,00 10,00 5,00 0,00 S7 Dniprodzerzhinsk - Ukraine S5 Charkesar – Uzbekistan Degmay, Tajikistan S3 Taboshar, Tajikistan S1 FIG. 3. Minimum and maximum dose rates (µSv/h) in and around the four studied uranium tailings sites in Ukraine, Tajikistan and Uzbekistan. 4.3. Current doses to exposure groups Once the radiation doses from the exposure pathways have been evaluated it is possible to assess the doses that different groups of individuals may receive based on their life styles. Both studies [1, 2] present such results, but here one example is provided. At the Taboshar site, five groups were identified: – Group 1. People that live in Taboshar, relatively far from the tailing dump site, and stay most of the time in houses. The houses are not contaminated because materials from the tailing have not been used for house construction. They obtain all their drinking water from the non-contaminated river Utken-Suu; – Group 2. People from this group have the same occupancy of the hazardous areas as Group 1, but they use water from the mine for drinking and for irrigation of vegetables; – Group 3. People from this group use water from the mine for drinking and irrigation (as for Group 2). They also live in Taboshar, relatively far from the tailing dump site, and stay most of the time in houses, but they regularly visit the areas in the vicinity of town where the uranium waste rock piles are situated; – Group 4. People from this group make the same use of the water from the mine as people from Group 3. They differ from the other group in that spend some time at the tailings pasturing their cows and sheep and in that they obtain 30% of their meat and milk from cows that drink tailing waters; – Group 5. People from this group work 30 hours per week during 46 of the weeks of the year in areas near the uranium pit. Like the other groups, they live in Taboshar, relatively far from the tailings dump site, and stay most of the time in their houses. 239 TOPICAL SESSION 7 Table 2 presents the assumptions used and the derived annual radiation dose rates for the five groups. TABLE 2. ESTIMATED RADIATION DOSE RATES (MSV/Y) TO VARIOUS GROUPS OF THE POPULATION AT THE TABOSHAR SITE Exposure (h/y) to different hazards Group Outdoor at tailings Outdoor at waste rock piles Indoor in houses 1 2 3 4 5 0 0 0 1 460 0 0 0 730 730 1 380 5 840 5 840 5 110 5 110 5110 Group 1 2 3 4 5 5. Percentage of annual consumption % Meat and Irrigation of Drinking Outdoor at milk (water vegetables water the town from (water from from tailings) mine) mine 2 920 0 0 0 2 920 0 30 30 2 920 0 30 30 1 460 30 30 30 2 270 0 0 0 Dose mSv/y Minimum Maximum 0.93 4.70 1.20 5.10 1.20 6.50 1.30 6.80 1.00 7.20 Contribution % External Radon Others 12 88 0 11 80 9 32 59 8 39 49 12 48 50 2 SUMMARY A consistent approach for deriving radiation doses to groups of people exposed to uranium tailings contaminants has been applied at four locations. By identifying the hazards and quantifying them based on exposure pathways, radiation dose rates can be calculated and form the basis for quantifying the exposure to given groups of the population. As stated in the main report [2] “… the data generated will support prioritization of the legacy sites for remediation and preparation of the necessary remedial feasibility assessments”. Further work is being pursued at all four sites. ACKNOWLEDGEMENTS The authors would like to thank both the International Atomic Energy Agency and the Swedish Radiation Safety Authority for sponsoring part of the work that is presented in this paper as well as all local counterparts who assisted in the work. The authors also acknowledge that many staff at EcoMonitor and Facilia also contributed to producing the results that are presented in this paper. 240 AVILA et al. REFERENCES [1] [2] [3] [4] ZINGER, I. (Ed.), ENSURE: Assessment of Risks to Human Health and the Environment from Uranium Tailings in Ukraine – Phase 1 report, Facilia Report: TR/SIUS/01 for the Swedish Radiation Protection Authority, Sweden (2008). INTERNATIONAL ATOMIC ENERGY AGENCY, Annex: Assessment of doses from exposures to elevated levels of natural radionuclides in areas close to uranium tailings in Tajikistan and Uzbekistan, in Safe Management of Residues from former Mining and Milling Activities in Central Asia: project results 2005–2008, Regional Technical Cooperation Project RER/9/086, Draft report (in preparation), November 2008. BMU, Berechnungsgrundlagen zur Ermittlung der Strahlenexposition infolge bergbaubedingter Umweltradioaktivität (Berechnungsgrundlagen – Bergbau), [Assessment principles for estimation of radiation exposures resulting from miningrelated radioactivity in the environment (Assessment principles for mining)], German Federal Ministry for the Environment, Nature Conservation and Reactor Safety, Berlin 30.07.1999 (1999). AVILA, R., BROED, R. and PEREIRA, A., Ecolego – A toolbox for radioecological risk assessment, Proceedings of the International conference on the Protection from the Effects of Ionizing Radiation, Stockholm, IAEA–CN–109/80, International Atomic Energy Agency, Vienna (2003). 241 SUMMARY OF SESSION 7 B. Salbu Norway CASE STUDIES II From the eight presentations and the discussion in this session, a number of valuable lessons were learned. As a general lesson, it is clear that there is no substitute for competent regulators, operators and good science. This underscores the need for training, education and national capacity building in order to meet the challenges associated with contaminated sites. Life cycle planning (or lack of it) was a reoccurring theme in many of the presentations in the session. Life cycle planning is needed in order to prevent significant problems from occurring in the latter stages of a uranium mining and milling operation. A robust regulatory system (i.e. one that requires an environmental impact assessment prior to the start of a mining operation) and good coordination between the regulatory body, the operators and the research community, are also very important. The regulatory body should be independent of the operator. It was clearly demonstrated there is a strong need for stakeholder involvement throughout the whole period of a project. The experience gained in the remediation of a uranium extraction plant in Mexico showed that if the organization that is performing the remediation is different from that responsible for long term care of the site, there needs to be good coordination between them to ensure a smooth transition of responsibilities. The study showed the need for adequate compliance verification of the remediation plan, for example, by the use of proper institutional controls. One presentation discussed an innovative way to calculate radiation doses when background radiation makes the radiation caused by human activities difficult to measure. The presentation also emphasized the need to take due account of the habits of local potentially exposed population groups in dose assessments and provided an example of this in relation to the Aborigines in Australia. Radiation monitoring programmes and radiation dose assessments to workers involved in remediation activities at uranium mine sites and to the public were described in several presentations. The public perception of radiation risks was raised as an issue in at least one presentation and the need for improved approaches for risk communication was emphasized. Experience in the implementation of remediation schemes in different countries has shown that: – What may work in one part of the world may not work in another, e.g. for cultural, climatic and physical geographic reasons; – Having a site conceptual model is valuable for targeting limited resources towards the activities that will give the greatest risk reduction; – Stakeholder involvement may be more challenging than the technical solutions. Furthermore, it was noted that many of these legacy sites have common issues: – – – – 242 Operations were terminated abruptly; There was improper or no management of waste and residues; No funding exists for post mining/milling activities; and There was no stakeholder involvement due to the secret nature of the sites. SUMMARY OF SESSION 7 An important conclusion from the presented studies on the radiological impact of uranium mining and milling legacy sites is that, in almost every case, with a few localized exceptions, the radiation doses are low. This underscores the need to evaluate these legacy sites individually using a site-specific, evidence based approach. Only in this way can the true risks to the public and the environment be properly evaluated and addressed. 243 EXPEDITING AND ENHANCING EXPERIENCE EXCHANGE (TOPICAL SESSION 8) Chairperson D. LOUVAT IAEA THE ENVIRONET – NETWORK ON ENVIRONMENTAL MANAGEMENT AND REMEDIATION H. MONKEN-FERNANDES International Atomic Energy Agency, Vienna Abstract This paper describes ENVIRONET, a new initiative of the International Atomic Energy Agency to facilitate information exchange between persons concerned with environmental remediation projects in different counties. The rationale for the development of the ENVIRONET network and the main the functions and facilities of the network are described. 1. BACKGROUND The successful implementation of environmental remediation projects depends on the appropriate combination of factors that include both technical and non-technical issues. In most cases, the major constraint in implementing of these projects is the lack of financial resources. Environmental remediation activities tend to be very expensive and because, in the past, companies, both private and state-owned, did not provide the necessary financial provisions for environmental remediation, it is not uncommon that resources for remediation are unavailable. For these reasons, the costs of remediation projects have generally to be faced by the State. Often, the national organizations in charge of implementing remediation works rely on the support of international organizations to fund the projects – especially in the case of countries with weak economies. However, even if financial resources are available there are a number of other issues to be tackled. They include, but are not limited to: the technologies to be used, the availability of appropriate staff and the regulatory infrastructure (including laws, regulations, and regulatory organizations). Planning is a topic of crucial importance for the successful implementation of environmental remediation projects but in many cases it is not appropriately considered by those in charge of the implementation of projects. Finally, consideration has to be given to the role to be played by different stakeholders in the decision making process. Consideration has to be given to procedures for taking their views into consideration and for involving them effectively in the process. Solutions have to be found that are both technically and scientifically sound at the same time as being understood and accepted by the different stakeholders. Some countries have achieved more successful outcomes in the implementation of environmental remediation projects than others. As a result they have experience on how to deal with some of the issues mentioned above. However, solutions for environmental remediation problems are not universally applicable, i.e. a technology has proven to be effective at one site may not be the most appropriate one to be applied to another one. One example of this is the use of dry covers. A cover designed for an arid region may not be appropriate for use in humid conditions. There is a need to understand the scientific rationale behind the functioning of the cover in order to design an appropriate cover for a specific situation. Interaction with stakeholders is another example where universal solutions do not exist. The socio-political and cultural characteristics of communities and societies may often differ so that an approach used in one country may not be the best approach to be used in another. 247 TOPICAL SESSION 8 Taking all these elements into account the International Atomic Energy Agency has been working to provide its Member States with relevant support in this area. It has been promoting technologies that can aid in the implementation of environmental remediation projects. These are aimed at improving the environmental conditions in areas affected by radioactive contamination in the past. At the same time the IAEA has been encouraging the adoption of good environmental management practices with the objective of avoiding the creation of new legacy sites and/or the need of extensive remediation works after the termination of operations. The IAEA tries to fulfil this important mission by: i) publishing technical documents and safety standards, ii) organising training courses, workshops and seminars and providing for the implementation of scientific visits and experts missions under the activities of its Technical Cooperation Department, iii) organising international conferences and iv) providing and supporting peer-review missions. 2. NETWORKING It has been noted that there is room for improvement in the type of assistance that the IAEA provides to its Member States. One reason is that there are different types of potential recipients of IAEA assistance. Sometimes the guidance given in its technical documents may be too generic or superficial for use by some while for others it may not be achievable. The IAEA publications tend to consolidate the experience of more developed countries on a specific topic and this experience may not be readily applicable in a country with comparatively modest resources (human and/or finance). For various reasons countries often need more than published advice in order to be able to tackle the problems of environmental remediation. It has become evident from interaction with many of the Member States affected by environmental contamination that the IAEA should strive to provide help in more practical and tangible ways. 2.1. IAEA Networks – the ENVIRONET At the present time, the Waste Technology Section of the IAEA is operating four information networks: the first one to be created was the URL (Underground Research Laboratory Network). It was followed by the IDN (International Decommissioning Network) and the DISPONET (Waste Pre-disposal Network). The ENVIRONET, which was launched in 2009, is an information network dealing with legacy sites (existing contaminated sites) as well as life-cycle approaches for minimizing the need for future remediation measures due to the operations of nuclear facilities and NORM (naturally occurring radioactive materials) industries. It is intended to aid Member States in solving the problems created in the past by improving the efficiency of information exchange and the transfer of knowledge and assistance. Topics to be covered by the ENVIRONET include: i) Life-cycle planning of both facility operations and environmental remediation; ii) Project planning (quality control and assurance); iii) Data management, iv) Integration and communication; v) Site characterization; vi) Modelling (fate and transport, engineering design and economics); vii) Risk assessment; viii) Remediation technology development and selection; ix) Monitoring; x) Stakeholder involvement and communication; xi) Regulation and policy development; xii) Risk communication; xii) Stewardship – Institutional Control and xiii) Funding. The planned methods of work include a variety of products and services aimed at expediting the exchange of information and experiences. The ultimate goal is to build 248 MONKEN-FERNANDES capacity in Member States and to facilitate the full implementation of remediation projects. These products and services include: website (document repository of educational materials); discussion forum; partners directory (online profiles); schedule of events; workshops, conferences, training sessions, long-distance training, fellowships/internships and peer reviews. The products will be: proceedings; dedicated publications; training materials, case studies, annual reports and newsletters. The vision underlying the implementation of networks is that the involvement of interested groups through the network on a specific topic will promote an effective flow of information and experience sharing. ENVIRONET will also aim at the transfer of knowledge while providing for the education of those in need. In principle, information will flow from more experienced partners to those with less experience. However, in many situations the advantages of integration through a network is mutual, as a lot of positive and valuable information can flow in a reverse way. With the aid of the new tools provided by the development of the Internet, virtual forums can be established, and this will allow an intensive circulation of information amongst the participants of the network. Modern web-base resources will also allow new educational tools, such as video materials, to be posted on the web. Finally, networking will allow the IAEA to capture the needs of a greater number of technical people in the each Member State. More information and further contact with IAEA Waste Technology Section networks can be obtained at: www.iaea.org/OurWork/ST/NE/NEFW/wts_NETWORKS_homepage.html. For further contact with the ENVIRONET Scientific Secretary the email address environet@iaea.org is also available. 249 SUMMARY OF SESSION 8 D. Louvat IAEA INTERNATIONAL ASSESSMENT AND INFORMATION EXCHANGE In this short session there were three presentations covering an internationally sponsored review of uranium mining legacy sites in countries of Central Asia and the programmes of two international organizations in the field of environmental remediation. These presentations were followed by a final discussion. The secrecy surrounding the sites in former times led to a lack of disclosure of information. Nowadays, more data is available, but the reliability of the information is an issue. Therefore, it is essential for measurements to be carried out to validate and complete the information. The quality and accuracy of dose assessments depend on the reliability of the data used in the models. Under the NATO RESCA project a number of field missions have been carried out involving measurement and radioactive dose assessment, among other activities. The overall conclusion is that, in general, radiation levels are not very high, except at very specific locations within some sites or when there is easy access to radioactive material that potentially could be misused. The dose assessments were, however, very preliminary since the radiological characterization of the sites has not been completed. Indoor radon generally makes the highest contribution to the dose. Drinking water makes a smaller contribution and other pathways make even smaller contributions. A short summary of the goals of NATO in the field was presented and, in particular, the organization and objectives of the Science for Peace and Security Committee were described. The activities of the Committee are non-military and are for civil science cooperation. The main topics dealt with by the Committee are oriented towards defence against terrorism and other threats, including environmental security. The work is implemented in many cases in association with other international initiatives. Working groups and subgroups deal with a wide range of subjects connected to environmental hazards and man-made induced degradation of the world’s natural resources, among other topics. In particular, two large projects related to the former nuclear test site at Semipalatinsk in Kazakhstan have been implemented. In the final presentation, ENVIRONET, an IAEA initiative on a ‘network of centres of excellence on environmental remediation’ was described. The objectives of ENVIRONET are to provide coordinated support, to organize training and demonstration events, to foster information exchange and to establish a forum. ENVIRONET will cover a wide range of topics, e.g. site characterization and remediation, but its final structure is still being designed, including the roles and functions of the partners. The establishment of the network will be formally announced at the next General Conference of the IAEA in October 2009. The Chairperson started the discussion session by reminding the participants that there are several ongoing and planned international initiatives in relation to remediation of uranium legacy sites. In the subsequent discussion, the ENVIRONET project was generally appreciated and well supported. Detailed questions as to its scope, content, mechanisms and resources for its support were raised. While appreciating the ENVIRONET initiative, it was noted that a separate forum for regulators is needed. Most problems (no maintenance, lack of planning) have resulted from 251 SUMMARY OF SESSION 8 poor regulatory infrastructure and organization of the regulatory bodies. The establishment of a global network of regulators in this field is needed. It was pointed out that the issue of site maintenance had not been properly addressed at the conference. IAEA has issued guidance on this but it needs to be strongly emphasized in projects otherwise remediation actions will fail in the long term. The Conference participants heard of a number of international initiatives related to the remediation of legacy sites in Central Asia. It is important that these are properly coordinated so as to avoid wasting resources in the countries of Central Asia, in the international organizations and in their supporting Member States. The international organizations should urgently address this potential problem. 252 SUMMARY AND CONCLUSIONS OF THE CONFERENCE Report of the Conference President1 Mr Timur Zantikin Conference President Kazakhstan Atomic Energy Committee (KAEC) Ulitsa Lisy Chaikina, 4 050020 Almaty KAZAKHSTAN The need for the remediation of legacy sites resulting from nuclear weapons testing, nuclear accidents, poorly operated practices and abandoned facilities became evident after the end of the Cold War in 1989. Since then, the full extent of the global remediation problem has become clear and, in response, the International Atomic Energy Agency organized several radiological assessments of major affected sites around the world. In 1999, the IAEA held the International conference on the Restoration of Environments with Radioactive Residues in Arlington, USA. The Arlington conference was mainly focused on the remediation of areas affected by nuclear weapons testing and nuclear accidents and on the issue of radiological criteria to guide cleanup decisions. By 2009, the emphasis had moved to the remediation of uranium mining and milling legacy sites and the technology for use in site remediation. These are the main topics of this week’s conference in Astana, Kazakhstan. The Conference has attracted participants from all over the world and presentations from many countries and organizations, but the emphasis of our discussions this week has been on the problems caused by uranium mining and milling legacy sites in the countries of Central Asia. The conference addressed the important issue of international regulatory standards for remediation and noted the progress being made towards incorporating regulatory requirements and guidance for remediation into the revised International Basic Safety Standards on Radiation Protection (BSS). The revised BSS will include a radiological protection framework for remediation which allows criteria for remediation to be developed by a process of optimization, taking due account of national and local circumstances. In the context of regulations, the Norwegian Radiation Protection Authority (NRPA) announced a plan during the Conference to assist in the regulatory supervision of legacy sites in the Central Asian Republics. Based on its previous experience in the Russian Federation, in which it helped to improve the regulatory capabilities of the nuclear regulator, the NRPA proposes to assist the countries of the Central Asian Republics by improving regulatory infrastructures and, in particular, providing training to the regulatory body in procedures and regulatory supervision. It was also suggested that IAEA might wish to become involved, for example, by hosting meetings of the coordination forum. Many of the old uranium mines were developed in an era in which efficiency of uranium production was the only concern – with no attention being given to the damage inflicted on the environment or to the residues left behind. The environmental consequences of the first phase of uranium mining and milling were therefore often significant and could have been avoided. This has prompted concern that the same mistakes might be repeated in the new wave of uranium mining. The Conference supported the strategy of avoiding the creation of future legacy sites by proper planning (life cycle planning) and good operating 1 The views and recommendations expressed here are those of the President of the Conference and the participants, and do not necessarily represent those of the IAEA. 253 SUMMARY AND CONCLUSIONS OF THE CONFERENCE practices and by promoting an environmental protection culture among the mining companies. It was also recognized that much could be achieved by establishing appropriate regulations and a strong regulatory body in the country in which the mining operations are conducted. Many of the countries with legacy uranium mining sites share common problems, such as, a lack of funds to deal with the problem, a lack of local expertise and equipment and, as a result, inadequately characterized sites. Furthermore, the radiological conditions of people living near to the sites may not be known. In most of the major industrialized uranium producing countries of the world, the uranium mining sites have been successfully remediated. During the conference the experience obtained in attempting to transfer this experience to developing countries was shared with the participants. Some of the key points were: – It is necessary to build capacity through training so that the local organizations become capable of managing and regulating their own remediation activities; – In many countries, resources are limited and the remediation solutions which have been used in industrialized countries may not be ideally suited to the application; usually, simple rather than sophisticated solutions are to be preferred; – It is necessary to involve local stakeholders and to be sensitive to their concerns; sometimes it may not be appropriate to apply the most effective technical solutions because of social considerations, such as, maintaining the wellbeing of local people and securing their employment; – Precautions may need to be taken to ensure the long term viability of supplied equipment, for example, by providing spares and arrangements for maintaining and servicing it. New and innovative technologies were discussed at the Conference and information was provided on such technologies for application to monitoring, assessing and restricting the movement of radionuclides in soil and ground water. The Conference gave strong support to ENVIRONET – a new initiative of the IAEA which has the aim of promoting mutual interests and the sharing of information in the area of environmental remediation. Many presentations dealt with the characterization and radiological assessment of sites. In most of the cases considered, there are chemical (metals) hazards as well as those due to ionizing radiation and these must be taken into account in any assessment – too often only radiological hazards are considered. A number of posters were displayed throughout the week describing studies additional to those presented in the oral sessions; they were mainly related to uranium mining and milling. All of the conference papers and posters will be useful and a help to persons wishing to learn from the experience of others. The involvement in the Conference of many international organizations is a reflection of the importance being given to this problem. The World Bank, the United Nations Development Fund, the North Atlantic Treaty Organization, the World Health Organization, the European Bank for Reconstruction and Development, the Organization for Security and Cooperation in Europe, the European Commission and the IAEA have all been represented and almost all have made presentations. The aims of most of these organizations are similar in that they wish to provide assistance in the remediation of uranium mining and milling legacy sites in the countries of Central Asia. Most of them favour a regional approach and see the need for a well defined road map before proceeding with any project. They recognize the importance of developing regulatory capabilities in the countries and agree on the need to have well defined indicators of success. It is evident that they are already in contact with each 254 SUMMARY AND CONCLUSIONS OF THE CONFERENCE other, but this conference has shown more clearly that there is a need for increased coordination between them. In this context the IAEA has a special role. It is the only one of the organizations with formal international responsibilities and specialized knowledge in the areas of radiation protection and radioactive waste management. For this reason, if such a joint regional project were to be established, the IAEA would be the appropriate international organization to provide the technical safety justification for it on the basis of its safety standards. The discussions at the Conference have resulted in a number of initiatives and proposals being put forward for cooperative action at the regional level; these are elaborated in the Session Summaries of the conference. It is now up to the international organizations to deliberate on these and to decide if and when to take action, taking into account the demands from other sectors. I am sure that you have all benefitted from the exchange of information which has been possible during this conference and that you have made many useful contacts. These are often the main benefits from such meetings. 255 CHAIRPERSONS OF SESSIONS Opening Session Session 1 Session 2 Session 3 Session 4 Session 5 Session 6 Session 7 Session 8 Closing Session T. ZANTIKIN H. FORSSTROEM S. VORBIEV A. J. GONZALEZ V. ADAMS M. PAUL A. KIM B. SALBU D. LOUVAT T. ZANTIKIN Kazakhstan IAEA ISTC Argentina United States of America Germany Kazakhstan NATO IAEA Kazakhstan PRESIDENT OF THE CONFERENCE T. ZANTIKIN Kazakhstan SECRETARIAT OF THE CONFERENCE H. MONKEN-FERNANDES R. EDGE H. SCHMID E. POSTA G. LINSLEY H. RATCLIFFE A. JUNGER R. de SILVA Scientific Secretary (IAEA) Scientific Secretary (IAEA) Conference Services (IAEA) Conference Services (IAEA) Proceedings Editor Administrative Support Administrative Support Administrative Support PROGRAMME COMMITTEE Chairperson V. Adams United States of America Members T. Akhmetov S. Berezin P. Crouchon E. Fillion M. Iskakov I. Kadyrzhanova S. Nordstrom P. Stegnar H. Monken-Fernandes R. Edge Kazakhstan Kazakhstan France France Kazakhstan Kazakhstan Norway Slovenia IAEA IAEA 257 ORGANIZING COMMITTEE IN KAZAKHSTAN Chairperson S. Mynbaev Ministry of Energy and Mineral Resources Members A. Magauov Ministry of Energy and Mineral Resources Astana Mayor’s Office Ministry of Culture and Information Ministry of Environmental Protection Ministry of Trade and Industry Ministry of Foreign Affairs Ministry of Internal Affairs State Sanitary and Epidemiological Control Committee Customs Control Committee NAC Kazatomprom National Nuclear Centre Ministry of Energy and Mineral Resources T.Nurkenov B. Aytkazin A. Tauteev K. Alkeev B. Sadykov K. Zhanisbaev A. Askarov D. Tulemisov S. Yashin S. Lukashenko T. Akhmetov Local Coordination G. Yeligbayeva Ministry of Energy and Mineral Resources 258 AUTHOR INDEX AUTHOR INDEX Adsley, I.: 229 Akber, R.: 173 Aleshin, Y.G.: 147 Ashirov, G.E.: 147 Avila, R.: 235 Baechler, S.: 195 Balonov, M.I.: 51 Berta, Z.: 91 Berkovskyy, V.: 31 Bochud, F.: 195 Bogdevich, I.: 223 Bollhöfer, A.: 173 Buzinny, M.G.: 211 Carr, Z.: 31 Christie, D.H.: 31 Chupov, A.: 223 Csővári, M.: 91 Danilova, E.A.: 153 Daniska, V.: 131 Denham, M.: 97 Dinis, M.L.: 191 Edge, R.: 107 Eleyushov, B.: 165 Fabian Ortega, R.: 185 Fang, Y.L.: 79 Fellingham, L.: 229 Fesenko, S.: 223 Fiúza, A.: 191 Földing, G.: 91 Franklin, M.R.: 179 Froidevaux, P.: 195 González, A.J.: 21 Gudowski, W.: 41 Gwo, J.P.: 79 Hajkova, E.: 131 Iskakov, M.: 165 Isamov, N.: 223 Jacob, P.: 223 Jakubick, A.T.: 107 Li, M.H.: 79 Magauov, A.M.: 17 Metzler, D.R.: 107 Mirsaidov, U.: 67 Moϊse, K.N.: 195 Monken-Fernandes, H.: 247 Murley, R.: 229 Nurgaziyev, M.: 165 Oughton, D.H.: 127 Osborne, D.F.: 85 Panov, A.: 223 Radyuk, G.A.: 153 Radyuk, R.I.: 153 Regner, J.: 217 Reisenweaver, D.: 13, 119 Recio, M.: 139 Rudneva, V.: 41 Saïdou, S.: 195 Saint-Pierre, S.: 61 Salbu, B.: 159 Salikhbaev, U.S.: 153 Sanzharova, N.: 223 Schmidt, P.: 217 Shandala, N.K.: 51, 67 Sherstyuk, E.: 31 Siegel, M.D.: 79 Sneve, M.: 51, 67 Stanislavov. E.: 31 Stegnar, P.: 153 Stevens, K.: 229 Teunckens, L.: 131 Tolongutov, B.: 67 Toma, A.: 203 Torgoev, I.A.: 147 Ulanovsky, A.: 223 Vangelas, K.: 97 Van Velzen, L.P.M.: 131 Várhegyi, A.: 91 Vasidov, A.: 153 259 LIST OF PARTICIPANTS Karankevich, A.: 31 Kashparov, V.: 213 Kayukov, P.: 159 Kelly, J.: 136 Keyser, P.: 224 Kim, A.: 68 Kinker, M.: 136 Kiselev, M.F.: 52, 68 Kist, A.A.: 149 Kristofova, K.: 130 Kunz, C.: 207 Lavrova, T.V.: 202 Leshchenko, O.: 31 Lu, P.: 168 Luo, W.S.: 78 260 Vasko, M.: 130 Velicu, O.: 195 Vinton, L.: 31 Voitsekhovych, O.V.: 202, 224 Waggitt, P.: 104 Walker, S.: 57 Yabusaki, S.B.: 78 Yeh, G.T.: 78 Zhang, F.: 78 Zhuchenka, Y.: 213 Zhunussova, T.: 68 Zhuravlev, A.A.: 149 Zinger, I.: 224 LIST OF PARTICIPANTS LIST OF PARTICIPANTS Abdikarim, U. L.N. Gumilyov Eurasia National University, Munaitpassova Street 5, Astana, Kazakhstan Abdikhalikova, S. Kazakhstan Atomic Energy Committee, Orynbor Street, Ministries Building, 13 Entrance, 010000 Astana, Kazakhstan Adams, V. U.S. Department of Energy, EM-12/Cloverleaf Building, 1000 Independence Avenue S.W., Washington, D.C. 20585-2040, United States of America Email: vincent.adams@em.doe.gov Adsley, I. Nuvia Ltd, The Library, 8th Street, Harwell, Science Campus, Didcot OX11 ORL, United Kingdom Fax: +441235514857 Email: ian.adsley@nuvia.co.uk Aitbaeva, A. L.N. Gumilyov Eurasia National University, Munaitpassova Street 5, Astana, Kazakhstan Akhmetov, T Kazakhstan Atomic Energy Committee, Orynbor Street, Ministries Building, 13 Entrance, 010000 Astana, Kazakhstan Fax: +77172503074 Email: atz@kaec.kz Akhmetova, Z. Ministry of Health, State Sanitary-Epidemiological Surveillance Committee, Moskovskaya, 66, 473000 Astana, Kazakhstan Fax: +73172317811 Email: z.akhmetova@mz.gov.kz Arisheva, A. L.N. Gumilyov Eurasia National University, Munaitpassova Street 5, Astana, Kazakhstan Askay, B. Ministry of Energy and Mineral Resources, Kabanbay Batyra Street 22, Astana, Kazakhstan, Fax: +7717231729769 Atygaev, A. Ministry of Energy and Mineral Resources, Kabanbay Batyr Street, 22, 010000 Astana, Kazakhstan Aydarova, S. K. Satpaev National Technical University, Almaty, Kazakhstan Bahari, I. University Kebangsaan Malaysia, School of Applied Physics, 261 LIST OF PARTICIPANTS 43600 Bangi, Malaysia Email: ismailbaharisn@yahoo.com Bakhtin, M. Medical Academy, Sary Arka Street 35, Astana, Kazakhstan Email: radbiol7@mail.ru Basibekov, K. Kazakhstan Atomic Energy Committee, Orynbor Street, Ministries Building, 13 Entrance, 010000 Astana, Kazakhstan Beishenkulova, R. Department of the State Sanitary and Epidemilogical Survaillence, Ministry of Health, Frunze Street 535, P.O. Box 720033, Bishkek, Kyrgyzstan Fax: +996312263756 Email: r_beishenkulova@yahoo.com Belben, G. United Kingdom Atomic Energy Authority (UKAEA), Harwell Science and Innovation Campus, Didcot, Oxfordshire OX11 0RA, United Kingdom Fax: +441235431914 Email: gaey.belben@ukaea.co.uk Belorusov, V. Stepnogorksy Mining and Chemical Complex LLP, Microdistrict 4, Building 2, P.O. Box 021500, Akmolinskaya oblast, Stepnogorsk, Kazakhstan Fax: +77164562816 Email: info@sghk.kz Bensman, V. “Ecoservice S”, Tole bi 202a, 050009 Almaty, Kazakhstan Fax: +77272503408 Email: ecoservic@mail.ru Berezin, S. National Nuclear Centre, 071100 Kurchatov, Kazakhstan Fax: +73225123858448206 Email: berezin@nnc.kz Burkitbayev, M. Al-Farabi Kazakh National University, 95a Karasai-batyr Street, 050012 Almaty, Kazakhstan Fax: +77272923731 Email: mburkit@nursat.kz Carr, Z. World Health Organization, 20 ave Appia, 1211 Geneva, Switzerland Email: carrz@who.int Chakam Tagheu, P. MINRESI, P.O. Box 1457, Yaounde, Cameroon Fax: +23722221336 Email: pulchakam@yahoo.fr JC “Ecomet-C”, Moscow, Russian Federation Cheremisin, P. 262 LIST OF PARTICIPANTS Chunkibyeva, A. Kazakhstan Atomic Energy Committee, Orynbor Street, Ministries Building, 13 Entrance, 010000 Astana, Kazakhstan Email: A.Chunkibayeva@kaec.kz Cingaev, V. National Nuclear Centre, 6, Tauelsisdik, 071100 Kurchatov, Kazakhstan Crochon, P. AREVA NC/BU, Mines/DI/DQSSE, Tour AREVA, 1 place Jean Millier, 92084 Paris La Defense, France Fax: +33134693900 Email: philippe.crochon@areva.com Csovári, M. MECSEK-ÖKO Zrt, Esztergár L.u.19, 7633 Pécs, Hungary Fax: +3672535390 Email: csovarimihaly@mecsekoko.hu Dairbekov, T. Kazakhstan Atomic Energy Committee, Orynbor Street, Ministries Building, 13 Entrance, 010000 Astana, Kazakhstan Danenov, N. Ministry of Foreign Affairs, Tanelsizdik Street 20, Astana, Kazakhstan Danilova, E. Institute of Nuclear Physics Tashkent, Ulugbek, 100214 Tashkent, Uzbekistan Email: Danilova@inp.uz Dauletov, A. Ministry of Energy and Mineral Resources, Kabanbay batyra Street 22, Astana, Kazakhstan Fax: +7717231729769 Demin, V National Nuclear Centre, 6, Tauelsisdik, 071100 Kurchatov, Kazakhstan Dinis, M. de Lurdes Faculdade de Engenharia da Universidade do Porto, R. Dr. Roberto Frias, Porto, Portugal Email: mldinis@fe.up.pt Djenbaev, B. National Academy of Science, Institute of Biology and Pedology, Chui Avenue 265, 720071 Bishkek, Kyrgyzstan Fax: +996312657943 Email: bekmamat2002@mail.ru Djunushaliev, T. Ministry of Emergency Situations of the Kyrgyz Republic, 11 Mominov Street, 723500 Osh, Kyrgyzstan Fax: +996322220471 Email: mchs.osh@elcat.kg NRCN, P.O. Box 9001, Beer Sheva 84190, Israel Dody, A. 263 LIST OF PARTICIPANTS Fax: +9726567690 Email: dodik@bgu.ac.il Dogalova, G. Kazakhstan Atomic Energy Committee, Orynbor Street, Ministries Building, 13 Entrance, 010000 Astana, Kazakhstan Durucan, S. Imperial College London, Exhibition Road, London SW7 2AZ, United Kingdom Email: s.durucan@imperial.ac.uk Dyusekeev, T. Ministry of Energy and Mineral Resources, Kabanbay batyra Street 22, Astana, Kazakhstan Fax: +7717231729769 Edge, R. International Atomic Energy Agency, Division of Radiation, Transport and Waste Safety, Vienna International Centre, P.O. Box 100, 1400 Vienna, Austria Fax: +43126007 Email: R.Edge@iaea.org Egizbaev, A. Ministry of Emergency Situations, Beybitshilik 22, Astana, Kazakhstan Eleushov, B.-B. JSC National Atomic Company “Kazatomprom”, 168, Bogenbay Batyr, 050012 Almaty, Kazakhstan Fax: +77272503541 Email: beleushov@kazatomprom.kz Erkasov, R. Pavlodar University, Astana, Kazakhstan Ermatov, A. Kazakhstan Atomic Energy Committee, Orynbor Street, Ministries Building, 13 Entrance, 010000 Astana, Kazakhstan Esposito, A. Sogin, Centrale Nucleare del Garigliano, Via Appia km 160.400, Sessa Aurunca (CE), Italy Fax: +390823055930 Email: aesposito@sogin.it Fawaris, B. Tajoura Nuclear Research Centre, Algerian Square, P.O. Box 464, Tripoli, Libya Fax: +21821361414243 Email: nyrkj@yahoo.com 264 LIST OF PARTICIPANTS Faybishenko, B. Lawrence Berkeley National Laboratory, 1 Cyclotron Road, MS 90-1116, Berkeley, 94720 California, United States of America Fax: +5104865686 Email: bafaybishenko@lbl.gov Fillion, E. AREVA NC/D3SE, 33 rue La Fayette, 75442 Paris Cedex 09, France Fax: +33134960239 Email: eric.fillion@areva.com Földing, G. MECSEK-ÖKO Zrt, Esztergár L.u. 19, 7633 Pécs, Hungary Fax: +3675535390 Email: foldinggabor@mecsekerc.hu Forsstroem, H. International Atomic Energy Agency, Department of Nuclear Energy, Division of Nuclear Fuel Cycle and Waste Technology, Vienna International Centre, P.O. Box 100, 1400 Vienna, Austria Fax: +43126007 Franklin, M. Brazilian Nuclear Energy Commission, Institute of Radiation Protection and Dosimetry, Av. Salvador Allende, S/N-Recreio, P.O. Box 37750, Rio de Janeiro, ZIP 22780-160, Brazil Fax: +552124422699 Email: mariza@ird.gov.br Gigase, Y. European Commission/ADICO A4, Jozef II Straat 54 07/235, 1049 Brussels, Belgium Fax: +3222995206 Email: yves.gigase@ec.europa.eu Gluchshenko, V. Institute of Nuclear Physics, National Nuclear Centre, 1 Ibragimov, 050032 Almaty, Kazakhstan Fax: +77273866454 Email: vik@inp.kz Gomes Mortagua, V. Industrias Nucleares do Brasil S/A-INB, Rua Miguel Yunes 115, CEP 04444-000, Jurubatuba – São Paulo, Brazil Fax: +551156317611 Email: valtermortagua@inb.gov.br González, A.J. Autoridad Regulatoria Nuclear (ARN), Av. Del Libertador 8250, 1429 Buenos Aires, Argentina Fax: +541163231771 Email: agonzalez@arn.gob.ar Gorbatenko, O. JSC National Atomic Company “Kazatomprom”, 168, Bogenbay Batyr, 050012 Almaty, Kazakhstan Fax: +77272503541 Email: ogorbatenko@kazatomprom.kz 265 LIST OF PARTICIPANTS Halvorsen, D. Royal Norwegian Embassy, 12 Samal microdistrict, Astana Tower Busniess Centre, 13th Floor, 010000 Astana, Kazakhstan Fax: +77172580087 Email: dmh@mfa.no Harlander, E. European Bank for Reconstruction and Development, Exchange Square, Primrose Street, London, EC2A 2JN, United Kingdom Fax: +442073387175 Email: harlande@ebrd.com Hein, G. Cameco Corporation, 2121 11th Street West, Saskatoon, Saskatchewan S7M 1J3, Canada Fax: +77272506415 Email: ghein@inkai.kz Hulka, J. SURO – National Radiation Protection Institute, Bartoškova 28, 14000 Praha 4, Czech Republic Fax: +420241410215 Email: jiri.hulka@suro.cz Idrissova, M. Kazakhstan Atomic Energy Committee, Orynbor Street, Ministries Building, 13 Entrance, 010000 Astana, Kazakhstan Ilyas, Z. BAPETEN, Jl. Gajah Mada No. 8, Jakarta, Indonesia Fax: +622163851028 Email: z.ilyas@bapeten.go.id Imasheva, B. Medical Academy, Sary Aska Street 35, Astana, Kazakhstan Fax: +77172539439 Email: bagdat_imasheva@mail.ru Isaev, N. Ministry of Energy and Mineral Resources, Kabanbay Batyra Street 22, Astana, Kazakhstan Fax: +7717231729769 Isaeva, A. Research Institute of the South Kazakhstan University, Tauke-khan Avenue, 5, Chimkent City, Kazakhstan Iskakov, M. JSC National Atomic Company “Kazatomprom”, 168, Bogenbay Batyr, 050012 Almaty, Kazakhstan Fax: +77272503541 Email: m.iskakov@kazatomprom.kz Ivanov, A. Centre of Radiation Technology and Technical Diagnostics, Akatu, Kazakhstan Jakubick, A. UMREG, Am Reuteberg, Eichenweg 14, 78269 Volkertshausen, Germany Fax: +493718120107 Email: alexjakubick@gmail.com 266 LIST OF PARTICIPANTS Jamsangtong, J. Thailand Institute of Nuclear Technology, Division of Research and Development on Nuclear Science and Technology, 9/9 Moo 7, Sai Mun, Ongkarak, 26120 Nakornnayok, Thailand Fax: +6637392913 Email: jantanee11@yahoo.com John, G. AMEC, 601 Faraday Street, Birchwood Park, Birchwood, Warrington WA3 6GN, United Kingdom Fax: +441925675006 Email: Gordon.john@amec.com Jousten, N. European Commission/ADICO A4, Jozef II Straat 54 07/235, 1049 Brussels, Belgium Email: Norbert.jousten@ec.europa Kadirzhanov, K. National Nuclear Centre, 071100 Kurchatov, Kazakhstan Kadyrova, N. 2 Krasnoarmeiskaya Street, 071100 Kurchatov, Kazakhstan Fax: +77225122806 Email: kadyrova@nnc.kz Kaftaranov, M. State Enterprise “Uranlikvidrudnik”, Ministry of Energy and Mineral Resources, Abay 112/12, P.O. Box 76, 020000 Kokshetau, Kazakhstan Fax: +77162401905 Email: uranlikvidrudnik@mail.kz Kainarbayev, A. L.N. Gumilyov Eurasia National University, Munaitpassova Street 5, Astana, Kazakhstan Email: aset_mirabilieus@mail.ru Kaligozha, A. L.N. Gumilyov Eurasia National University, Munaitpassova Street 5, Astana, Kazakhstan Kamel, Nour-el-hayet Commissariat à l’énergie atomique, Centre de Recherche Nucléaire d’Alger, 2, Boulevard Frantz Fanon, B.P. 399, 16000 Alger – Gare, Algeria Fax: +21321433538 Email: kamelhayet@yahoo.fr Kamel, Nariman H.M. Atomic Energy Authority (AEA), Radiation Protection Department, Nuclear Research Centre, P.O. Box 13759, Cairo, Egypt Fax: +20222730261 Email: Narimankamel@hotmail.com Karigi, A. Radiation Protection Board, P.O. Box 19841, 00202 Nairobi, Kenya Fax: +254202714383 Email: alice_karigi@yahoo.co.uk 267 LIST OF PARTICIPANTS Karlin, Y. SIA “Radon”, Rostovky Lande, 7, 2/14, 119121 Moscow, Russian Federation Fax: +74992481941 Email: karlinyr@yandex.ru Kartoev, S. Ministry of Energy and Mineral Resources, Kabanbay Batyra Street 22, Astana, Kazakhstan Fax: +7717231729769 Kayukov, P. JSC “Volkovgeologia”, Bogenbay Batyr Street 156, 050012 Almaty, Kazakhstan Fax: +77272501359 Email: priemnaya-vg@kazatomprom.kz Kazimbet, B. Medical Academy, Sary Arka Street 35, Astana, Kazakhstan Keltchewsky, A. Organization for Security and Co-operation in Europe, OSCE Centre in Astana, Beibitshilik 10, 010000 Astana, Kazakhstan Fax: +77172328304 Email: aliya.orazbayeva@osce.org Kerouanton, D. AREVA/SGN, 1 Rue des Herons, 78180 Montigry le Bretonneux, France Fax: +139487737 Email: david.kerouanton@areva.com Kim, A. Atomic Energy Committee, 35 Street, Ministries House, 010000 Astana, Kazakhstan Fax: +77172503073 Email: a.kim@kaec.kz Kim, N. CDC/CAR, 41 Kazybek Bi Street, Park Palace Building, 050010 Almaty, Kazakhstan Fax: +7272501777 Email: nkim@kz.cdc.gov Kiyazova, A. Atomic Energy Committee of the Ministry of Energy and Mineral Resources, 8th Building, 35th Street, Left Bank District, 010000 Astana, Kazakhstan Fax: +77172503073 Email: A.Kiyazova@kaec.kz Kozhakhmetov, N. Republican Prophylactic-Epidemiological Station, Ministry of Health, Astana, Kazakhstan Kuchynskyi, V. Chernobyl Nuclear Power Plant, m/b 10, 11, 1 Voennykh Stroiteley Street, 07100 Slavutich, Ukraine Fax: +380447925946 Email: mishchuk@chnpp.gov.ua 268 LIST OF PARTICIPANTS Kueny, L. Autorité de Sûreté Nucléaire, Division de Marseille, 69 Avenue du Prado, 13286 Marseille Cedex 06, France Fax: +33491836410 Email: laurent.kueny@asn.fr Kunze, C. WISUTEC Wismut, Environmental Technologies GmbH, Jagdschänkestrasse 33, 09117 Chemnitz, Germany Fax: +493718120175 Email: c.kunze@wisutec.de Kupchenko, V. State Geology Enterprise “Urangeology”, 7a, Navoi, 700000 Tashkent, Uzbekistan Fax: +10998711339774 Email: ecology@albatros.uz Kusainov, A. Nuclear Technology Park, Lenin Street 6, Kurcahtov, Kazakhstan Kuttigul, T. L.N. Gumilyov Eurasia, National University, Munaitpassova Street 5, Astana, Kazakhstan Kuturbekov, K. Interdisciplinary Research Complex, Ablaihana Street 2/1, 010000 Astana, Kazakhstan Fax: +87172342078 Email: kkuterbekov@google.com Kuyanova, Y. Al-Farabi Kazakh National University, 95a Karasai-Batyr Street, Almaty 050012, Kazakhstan Email: k-yelena@mail.ru Lacroix, E. AREVA NC/BU Mines/DI/DQSSE, Tour AREVA, 1 place Jean Millier, 92084 Paris la Defense, France Fax: +33134963902 Email: emilie.lacroix@areva.com Lavrova, T. Ukrainian Hydrometeorological Institute, Nauki Avenue, 37, 03028 Kiev, Ukraine Fax: +380445255363 Email: lavrova@uhmi.org.ua Linsley, G. International Atomic Energy Agency, Private Consultant, 23 Radley Road, Abingdon, Oxfordshire OX14 3PL, United Kingdom Email: gordon_linsley@yahoo.com Logar, Z. Pod Plevno 14, 4220 Skofja Loka, Slovenia Email: logar.zmago@gmail.com Louvat, D. International Atomic Energy Agency, Vienna International Centre, P.O. Box 100 1400 Vienna, Austria Lu, P. Energy Resources Australia Pty Ltd, GPO Box 518, Darwin, NT 0801, Australia Fax: +61889425790 Email: ping.lu@riotinto.com 269 LIST OF PARTICIPANTS Lukashenko, S. National Nuclear Centre, Institute of Nuclear Physics, 2 Krasnoameiskaya Street, 07100 Kurchatov, Kazakhstan Magauov, A. Ministry of Energy and Mineral Resources, Kabanbai Batyr Street 22, 010000 Astana, Kazakhstan Fax: +77172976943 Email: kanc@memr.kz Mansurov, Z. Ministry of Energy and Mineral Resources, Kabanbai Batyr Street 22, bloc A, 010000 Astana, Kazakhstan Marignac, Y. World Information Service on Energy (WISE-Paris), Bureau – Office 31-33 Rue de la Colonie, 5013 Paris, France Fax: +3314654793 Email: yves.marignac@wise-paris.org Marinho, P.R. Brazilian Nuclear Energy Commission, Rua General Severiano, 90, 22290-901 Rio de Janeiro, Botafogo, Brazil Fax: +552121732603 Email: pmarinho@cnen.gov.br Masalimov, Z. L.N. Gumilyov Eurasia National University, Munaitpassova Street 5, Astana, Kazakhstan Massenov, C. Atomic Energy Committee of the Ministry of Energy and Mineral Resources, 8th Building, 35th Street, Left Bank District, 010000 Astana, Kazakhstan Fax: +73272646631 Email: masenov@atom.almaty.kz Meshin, M. National Nuclear Centre, Institute of Atomic Energy, Krasnoarmeyskaya ulitsa 10, 071100 Kurchatov, Kazakhstan Email: Meshin@nnc.kz Métivier, J.-M. Institut de Radioprotection et de Sûreté Nucléaire, Direction de l’Environnement et de l’Intervention, Service d’Études sur le Comportement des Radionucléides dans les Écosystèmes, Cadarache BP3, 13115 Saint Paul les Durance, France Fax: +33442199143 Email: jean-michel.metivier@irsn.fr Metzger, W. Organization for Security and Co-operation in Europe, OSCE Centre in Astana, Beibitshilik 10, 010000 Astana, Kazakhstan Email: willmetz@umich.edu 270 LIST OF PARTICIPANTS Migliore, G. Sogin, Centrale Nucleare de Gar, Gliano, Via Appia km 160.400, Sessa Aurunca (CE), Italy Fax: +390823055930 Email: migliore@sogin.it Minbaev, S. Ministry of Energy and Mineral Resources, Kabanbai Batyr Street 22, 010000 Astana, Kazakhstan Fax: +77172976943 Email: kanc@memr.kz Mirsaidov, U. Nuclear and Radiation Safety Agency, Academy of Sciences, 17a Khamza Khakimzoda Street, Dushanbe, Tajikistan Fax: +992372215548 Email: m.ulmas@nrsa.tj Mirzagalieva, A. L.N. Gumilyov Eurasia National University, Munaitpassova Street 5, Astana, Kazakhstan Monken Fernandes, H. International Atomic Energy Agency, Vienna International Centre, P.O. Box 100, 1400 Vienna, Austria Fax: +43126007 Email: H.Monken-Fernandes@iaea.org Morenko, S. Institute of Nuclear Physics of the National Nuclear Centre, Kurchatov, Kazakhstan Mukashev, Z. Prime Minister’s Office, Astana, Kazakhstan Mukhametzhanova, A. Kazakhstan Atomic Energy Committee, Orynbor Street, Ministries Building, 13 Entrance, 010000 Astana, Kazakhstan Myrkhaidarov, K. L.N. Gumilyov Eurasia National University, Munaitpassova Street 5, Astana, Kazakhstan Nurakhmetov, T. L.N. Gumilyov Eurasia National University, Munaitpassova Street 5, Astana, Kazakhstan Fax: +77172344361 Email: aset_mirabilicus@mail.ru Nurgaziyev, M. JSC National Atomic Company “Kazatomprom”, 168, Bogenbay Batyr, 050012 Almaty, Kazakhstan Fax: +77272503541 Email: MNurgaziev@kazatomprom.kz Nyssanov, L.N. Gumilyov Eurasia National University, Munaitpassova Street 5, Astana, Kazakhstan 271 LIST OF PARTICIPANTS O’Kane, M. O’Kane Consultants Inc., Suite 1740 – 246 Stewart Green S.W., AB. T3H 3C8, Calgary, Canada Email: mokane@okc-sk.com Ortega Fabián, R. Comision Nacional de Seguridad Nuclear y Salvaguardias, Barragan 779, Colonia Narvarte, 03020 Mexico City, Mexico Fax: +525550953293 Email: rfabian@cnsns.gob.mx Osborne, D. Linkforce Pty Ltd, Suite R1A Innovation House Technology Park, 5095 Mawson Lakes S.A., Australia Email: david.osborne@linkforceau.com Ostroverkhov, M. National Nuclear Centre, Lenin Street 6, Kurchatov, Kazakhstan Email: max@nnc.kz Oughton, D. NATO, Department of Environmental and Plant Science, Norwegian University of Life Sciences, P.O. Box 5003, 1432 Aas, Norway Fax: +4764948359 Email: Deborah.oughton@umb.no Paul, M. WISUTEC Wismut Environmental Technologies GmbH, Jagdschänkenstrasse 29, 09117 Chemnitz, Germany Fax: +49378120107 Email: m.paul@wismut.de Pavel, G. RosRAO, 24/26 Bolshaya Ordynka Street, 19017 Moscow, Russian Federation Email: rosrao@mail.ru Pipovarov, O. National Nuclear Centre, 6, Tauelsisdik, 071100 Kurchatov, Kazakhstan Poleshko, A. Institute of Nuclear Physics, National Nuclear Centre, 1 Ibragimov Street, 050032 Almaty, Kazakhstan Fax: +77273865260 Email: anp@inp.kz Polezhaev, E. “Ecoservice S”, Eastern Branch, Vinogradov Street 29/1, Ust-Kamenogorsk, Kazakhstan Fax: +87232222666 Email: ukecoservice@mail.ru Prokhodceva, T. Nuclear Technology Safety Centre (NTSC), Liza Chaykina Street 4, 050020 Almaty, Kazakhstan 272 LIST OF PARTICIPANTS Rahman, R. University of Liverpool, H3 Philharmonic Court, Catharine Street, Liverpool, L8 7SD, Merseyside, United Kingdom Fax: +441517942866 Email: rrahman@liv.ac.uk Rakhimzhanov, B. L.N. Gumilyov Eurasia National University, Munaitpassova Street 5, Astana, Kazakhstan Raposo de Almeida, R. Federal Fluminense University, Rua Passo Da Patria 156 S.133, Niteroi 24.210-240, RJ Brazil Fax: +552126295354 Email: rraposo@globo.com Rehman, S.-U. International Affairs and Training, Pakistan Atomic Energy Commission, P.O. Box 1114, Islamabad, Pakistan Fax: +926429260030 Email: psshafir@yahoo.com Reisenweaver, D. Alion Science & Technology, 1475 Central Ave, Suite 200, Los Alamos 97544, United States of America Email: dreisenweaver@alionscience.com Romanenko, O. Nuclear Technology Safety Centre (NTSC), Liza Chaykina Street 4, 050020 Almaty, Kazakhstan Fax: +73272646803 Email: romanenko@ntsc.kz Rudneva, V. International Science and Technology Centre (ISCT), Krasnoproletarskaya ul. 32-34, P.O. Box 20, 127473 Moscow, Russian Federation Fax: +74999784637 Email: rudneva@istc.ru Ryabko, L. L.N. Gumilyov Eurasia National University, Munaitpassova Street 5, Astana, Kazakhstan Ryabkov, V. ATOMTEX, 5 Gikalo Street, Minsk 220005, Belarus Email: e.bystrov@gmail.com Sadykov, B. Ministry of Foreign Affairs, Tanelsizdik Street 20, Astana, Kazakhstan Saidou, S. Institute for Geological and Mining Research (IRGM), Energy Research Laboratory, Nuclear Technology Section, B.P. 4110, Nlongkak-Yaounde, Cameroon Fax: +23722222431 Email: saidous2002@yahoo.fr 273 LIST OF PARTICIPANTS Saint-Pierre, S. World Nuclear Association (WNA), Carlton House, 221 St. James’s Square, London – SW1Y 4JH, United Kingdom Email: saintpierre@world-nuclear.org Saipov, A. L.N. Gumilyov Eurasia National University, Munaitpassova Street 5, Astana, Kazakhstan Salbu, B. Institute of Plant and Environmental Sciences, Norwegian University of Life Sciences, P.O. Box 5003, 1432 Aas, Norway Fax: +4764948359 Email: brit.salbu@umb.no Salimgereev, M. Ministry of Energy and Mineral Resources, Kabanbai Batir Street 22, bloc A, 10000 Astana, Kazakhstan Sametbyatova, D. Kazakhstan Atomic Energy Committee, Orynbor Street, Ministries Building, 13 Entrance, 010000 Astana, Kazakhstan Santinelli, R. Nucleco S.p.A., Via Anguillarese 301, 00123 Rome, Italy Email: r_santinelli@hotmail.it Sarsanbaev, K. Nuclear Technology Park, Lenin Street 6, Kurchatov, Kazakhstan Satibaev, E. Astana Mayor’s Office, Astana, Kazakhstan Saypov, A. Research Institute of the South Kazakhstan University, Tauke-khan Avenue, 5, Chimkent City, Kazakhstan Schmidt, P. Wismut GmbH, Jagdschänkenstrasse 29, 09117 Chemnitz, Germany Fax: +493718120107 Email: p.schmidt@wismut.de Serikbaeva, U. Ministry of Energy and Mineral Resources, Kabanbai Batir Street 22, bloc A, 10000 Astana, Kazakhstan Seysebayev, A. Medical Academy, Sary Arka Street 35, Astana, Kazakhstan Seytkul, Z. Ministry of Energy and Mineral Resources, Kabanbay Batyra Street 22, Astana, Kazakhstan Shadrack, A. Radiation Protection Board, Hospital Road, P.O. Box 849, 274 LIST OF PARTICIPANTS 40100 Kisumu, Kenya Fax: +2542020078 Email: shadrackanthony@yahoo.com Shaho, Y. Verkhovna Rada of Ukraine, Grushevskyi Street 5, 01008 Kiev, Ukraine Fax: +380442552542 Email: shaho@rada.gov.ua Shaimerdenova, M. L.N. Gumilyov Eurasia National University, Munaitpassova Street 5, Astana, Kazakhstan Shaldibaev, M. Kazakhstan Atomic Energy Committee, Orynbor Street, Ministries Building, 13 Entrance, 010000 Astana, Kazakhstan Shandala, N. Federal Medical Biophysical Centre, Zhivopisnaya 46, 123182 Moscow, Russian Federation Fax: +74991930585 Email: shandala-fmbc@bk.ru Sharipov, M. Atomic Energy Committee, Ministry of Energy and Mineral Resources, 8th Building, 35th Street, 010000 Astana, Kazakhstan Fax: +77272607220 Email: M.Sharipov@kaec.kz Shaymardanova, D. Ministry of Energy and Mineral Resources, Kabanbai Batyr Street 22, 010000 Astana, Kazakhstan Shiganakov, S. Kazakhstan Atomic Energy Committee, Orynbor Street, Ministries Building, 13 Entrance, 010000 Astana, Kazakhstan Fax: +77172976870 Email: ssb@memr.kz Shishkov, I. JSC “Volkovgeology”, The Central Experience Methodical Expedition, 68 Griboedova Street, Almaty, Kazakhstan Email: Vershina@come.kz Simo, A. Ministry of Scientific Research and Innovation, P.O. Box 1457, Yaoundé, Cameroon Fax: +23722221336 Email: augsimo@yahoo.fr Simone, G. Nucleco S.p.A., Via Anguillarese 301, 00123 Roma, Italy Email: g.simone@nucleco.it Sizov, A. Institute for Safety Problems of NPPS, National Academy of Sciences of Ukraine, 275 LIST OF PARTICIPANTS Kirova 36a, Kyiv Region, Chernobyl, Ukraine Fax: +380449351209 Email: asizov@gmail.com Slavik, O. VUJE, a.s., Okruzna 5, Trnava 91864, Slovakia Fax: +421335991494 Email: slavik@vuje.sk Smagulova, A. Organization for Security and Co-operation in Europe, OSCE Centre in Astana, Beibitshilik 10, 010000 Astana, Kazakhstan Email: asmagulova@osce.org Smiroldo, E. US Nuclear Regulatory Commission, 11555 Rockville Pike, MS O4E12, 20852 Rockville, United States of America Email: exs5@nrc.gov Sneve Karpov, M. Norwegian Radiation Protection Authority, Grini neringspark 13, P.O. Box 55, Osteras, 1332 Oslo, Norway Fax: +4767167407 Email: Malgorzata.Sneve@nrpa.no Solomatina, A. Chu Laboratory of Ecology St. Koshomberdieva, 722030 Karabalta, Kyrgyzstan Fax: +996313372477 Email: Solomatina_76@mail.ru Stegnar, P. Jozef Stefan Institute, Jamova cesta 39, 1000 Ljubljana, Slovenia Fax: +38612519385 Email: stegnar@gmail.com Sugralina, S. Ministry of Energy and Mineral Resources, Division of Nuclear Energy and External Affairs, Kabanbay Batyr Street 22, 010000 Astana, Kazakhstan Fax: +73172976874 Email: sugralina@memr.kz Takelekov, K. Ministry of Energy and Mineral Resources, Kabanbay Batyr Street 22, 010000 Astana, Kazakhstan Fax: +77172976850 Email: takelekov_k@memr.kz Takenov, Z. UNDP Office in Kyrgyzstan, 160 Chui Avenue, 72004 Bishkek, Kyrgyzstan Email: zharas.takenov@undp.org 276 LIST OF PARTICIPANTS Tazhibaeva, I. National Nuclear Centre, Institute of Atomic Energy, Krasnoarmeyskaya ulitsa 10, 071100 Kurchatov, Kazakhstan Tolongutov, B. M. The Chu Ecological Laboratory, Koshomberdieva Street 1A, 722030 Kara-Balta, Kyrgyzstan Fax: +996313372477 Email: ecolabug@yahoo.com Torgoev, I. Kyrgyzstan National Academy of Sciences, Scientific Engineering Centre GEOPRIBOR, 98 Mederowa Street, Bishkek, Kyrgyzstan Email: geopribor@mail.ru Tulegenov, M. Atomic Energy Committee of the Ministry of Energy and Mineral Resources, 8th Building, 35th Street, 010000 Astana, Kazakhstan Fax: +77172503073 Email: M.Tulegenov@kaec.kz Uralbekov, B. Al-Farabi Kazakh National University, 95a Karasay Batyr Street, Almaty 050012, Kazakhstan Fax: +77272923731 Email: bulat.ural@gmail.com Usupov, U. Government House, Bishkek 720003, Kyrgyzstan Fax: +996312626359 Email: usen@mail.gov.kg Van der Tembel, K. Embassy of the Netherlands in Kazakhstan, Astana, Kazakhstan Van Velzen, L. Nuclear Research and Consultancy Group, Utrechtseweg 310, P.O. Box 9034, 6812 AR Arnhem, Netherlands Fax: +31263568538 Email: vanvelzen@nrg.eu Varhegyi, A. MECSEK-ŐKO Zrt., Esytergar Lajos u. 19, 7633 Pecs, Hungary Fax: +3672564708 Email: varhegyiandras@mecsekoko.hu Vasilyeu, P. ATOMTEX, 5 Gikalo Street, 220005 Minsk, Belarus Email: vasiliev@atomtex.com Velicu, S.-O. National Commission for Nuclear Activities Control, 14, Libertatii Boulevard, P.O. Box 42-4, 050706 Bucharest, Romania Fax: +40213163244 Email: sovelicu@cncan.ro 277 LIST OF PARTICIPANTS Vorobiev, S. International Science and Technology Centre (ISTC), Krasnoproletarskaya ul, 32-34, P.O. Box 20, 127473 Moscow, Russian Federation Fax: +74999781331 Email: vorobiev@istc.ru Vurim, A. National Nuclear Centre, Institute of Atomic Energy, Krasnoarmeyskaya ulitsa 10, 071100 Kurchatov, Kazakhstan Fax: +77225123125 Email: vurim@nnc.kz Walker, S. EPA 14212 Golden Hook Road, Boyds, MD 20841, United States of America Fax: +7036039132 Email: Walker.Stuart@epamail.epa.gov Walker, N. UNDP Office in Kyrgyzstan, 160 Chui Avenue, 72004 Bishkek, Kyrgyzstan Fax: +996312611217 Email: neal.walker@undp.org Wellman, D. Pacific Northwest National Laboratory, 902 Battelle Blvd., P.O. Box 999, MS K3-62, Richland, WA 99352, United States of America Fax: +15093724600 Email: Dawn.Wellman@pnl.gov Yakovlev, I. Centre of the Radiation Technology and Technical Diagnosis, Almaty, Kazakhstan Yakovlev, V. National Nuclear Centre, Institute of Atomic Energy, Krasnoarmeyskaya ulitsa 10, 071100 Kurchatov, Kazakhstan Yeh, G.-T. University of Central Florida, 4000 Central Florida Blvd, 32816 Orlando, Florida, United States of America Fax: +14078233315 Email: gyeh@mail.ucf.edu Yeligbayeva, G. Kazakhstan Atomic Energy Committee, Orynbor Street, Ministries Building, 13 Entrance, 010000 Astana, Kazakhstan Fax: +77172503073 Email: G.Yeligbayeva@kaec.kz Yessenkulova, A. L.N. Gumilyov Eurasia National University, Munaitpassova Street 5, Astana, Kazakhstan 278 LIST OF PARTICIPANTS Yunusov, M. Deputy Director General State Enterprise Vostokredmet Ulitsa Oplanchuka 12 Sogdiyskaya Oblast 735730 Chkalovsk, Tajikistan Fax: 00992 3451 50945 E-mail: yunusov2001@mail.ru Zaytceva, I. L.N. Gumilyov Eurasia National University, Munaitpassova Street 5, Astana, Kazakhstan Zhantikin, T. Kazakhstan Atomic Energy Committee, Orynbor Street, Ministries Building, 13 Entrance, 010000 Astana, Kazakhstan Fax: +77172503073 Email: t.zhantikin@kaec.kz Zhetbaeva, S. Kazakhstan Atomic Energy Committee, Orynbor Street, Ministries Building, 13 Entrance, 010000 Astana, Kazakhstan Zhumabaev, A. L.N. Gumilyov Eurasia National University, Munaitpassova Street 5, Astana, Kazakhstan Zhumabaev, S. Prime-Minister’s Office, Astana, Kazakhstan Zhumabaeva, G. Ministry of Energy and Mineral Resources, Kabanbai Batyr Street 22, bloc A, 010000 Astana, Kazakhstan Zhumagaliev, A. Ministry of Energy and Mineral Resources, Kabanbai Batyr Avenue, 22 010000 Astana, Kazakhstan Zhunusbek, B. Nuclear Technology Park, Lenin Street 6, Kurchatov, Kazakhstan Zhunussova, T. Norwegian Radiation Protection Authority, Grini neringspark 13, P.O. Box 55, 1332 Osteras, Oslo, Norway Email: tamara.zhunussova@nrpa.no Zinger, I. Facilia AB, Gustavslundsvägen 151C, 16751 Bromma, Sweden Fax: +468259665 Email: irene@facilia.se 279