Ferromagnetic Resonance and Magneto-transport Behavior Correlation via Interparticle Interactions in Cu100–xCox Nanogranular Films Dinesh Kumar*, Sujeet Chaudhary, and Dinesh K. Pandya Thin Film Laboratory, Physics Department, Indian Institute of Technology Delhi, New Delhi 110016, India. *Corresponding author, e-mail:dinesh1.goyal@gmail.com, Tel.:+911126586521 Abstract Increasing demagnetizing field and anisotropic response of the magnetoresistance with the increase of ‘x’ in Cu100-xCox films indicate the presence of interparticle interactions. The correlation between magnetoresistance and ferromagnetic resonance is established by interpreting the interparticle interactions in terms of resonance field and line width of the ferromagnetic resonance spectra. Keywords: Nanogranular, Superparamagnetic, Ferromagnetic resonance, Magnetoresistance, Interactions. Introduction Nanogranular magnetic systems have been widely studied, yet the degree of correlation between the magnetoresistance (MR) response and the associated changes in the overall magnetic states continues to be one of the challenges in understanding these systems. Independently, magnetoresistance [1-2], magnetization [3], and ferromagnetic resonance (FMR) [4] studies are reported on the magnetic properties of these films. Few of them [4-5] are trying to interpret the FMR spectra with percentage MR, but no efforts are made to correlate the evolution of MR behavior with FMR spectra. In this work, the correlation between the two independent measurements of MR and FMR have been attempted on 100 nm thick sputtered Cu100-xCox (x=17.8-33.3 at%) films. The interparticle interactions probing ability of FMR is presented to understand the MR behavior of Cu100-xCox films. Results The MR and FMR spectra are recorded at room temperature with magnetic field (H) parallel (H||) and perpendicular (H) to the sample plane. It is found that for x≤20.9 films MR is isotropic and Co particles present are of superparamagnetic nature. Evolution of perpendicular demagnetizing field and in plane anisotropy as a function of ‘x’ indicates the presence of ferromagnetic and superparamagnetic particles in x>20.9 films. This finding is interpreted in terms of particle size and interparticle interactions. Fig. 1(a) shows the resonance field (Hr) determined from FMR spectra. Hr is moving towards low (high) H for field parallel (perpendicular) to film plane and the difference of resonance field ∆Hr increases monotonically with the increase of ‘x’, evidenced the presence of interparticle interactions and established the role of increased interactions for the observed MR behavior. The increase in line width (∆H) with the increase of ‘x’ (fig 1(b)) depicts the increase of particle size and further confirmed the role of interparticle interactions for the detected MR behavior. Fig. 1: Dependence of (a) resonance field (Hr) and the difference of resonance filed (∆Hr) (b) line width (∆H) on ‘x’ in H|| and H┴ geometries. Acknowledgment One of the authors D.K. acknowledges MHRD-Government of India for the SRF Fellowship. References [1] D. Kumar, S. Chaudhary, and D. K. Pandya, J. Appl. Phys., 112, (2012), 083924. [2] D. Kumar, S. Chaudhary, and D. K. Pandya, J. Appl. Phys., 114, (2013), 023908. [3] L. Peter, Z. Rolik, L. F. Kiss, J. Toth, V. Weihnacht, C. M. Schneider, and I. Bakonyi, Phys. Rev. B, 73, (2006), 174410. [4] H. K. Lachowicz, A. Gierlowski, and A. S.Waniewska, J. Appl. Phys., 88, (2000), 368. [5] A. G. Prieto, M. L. F.-Gubieda, L. Lezama, and I. Orue, J. Appl. Phys., 111, (2012), 07C105.