AP* Chapter 21 Transition Metals and Coordination Chemistry AP Learning Objectives LO 1.10 Students can justify with evidence the arrangement of the periodic table and can apply periodic properties to chemical reactivity. (Sec 21.1) LO 1.11 The student can analyze data, based on periodicity and the properties of binary compounds, to identify patterns and generate hypotheses related to the molecular design of compounds for which data are not supplied. (Sec 21.1) Section 21.1 The Transition Metals: A Survey AP Learning Objectives, Margin Notes and References Learning Objectives LO 1.10 Students can justify with evidence the arrangement of the periodic table and can apply periodic properties to chemical reactivity. LO 1.11 The student can analyze data, based on periodicity and the properties of binary compounds, to identify patterns and generate hypotheses related to the molecular design of compounds for which data are not supplied. Section 21.1 The Transition Metals: A Survey Transition Metals Show great similarities within a given period as well as within a given vertical group. Copyright © Cengage Learning. All rights reserved 4 Section 21.1 The Transition Metals: A Survey The Position of the Transition Elements on the Periodic Table Copyright © Cengage Learning. All rights reserved 5 Section 21.1 The Transition Metals: A Survey Forming Ionic Compounds More than one oxidation state is often found. Cations are often complex ions – species where the transition metal ion is surrounded by a certain number of ligands (Lewis bases). Copyright © Cengage Learning. All rights reserved 6 Section 21.1 The Transition Metals: A Survey The Complex Ion Co(NH3)63+ Copyright © Cengage Learning. All rights reserved 7 Section 21.1 The Transition Metals: A Survey Ionic Compounds with Transition Metals Most compounds are colored because the transition metal ion in the complex ion can absorb visible light of specific wavelengths. Many compounds are paramagnetic. Copyright © Cengage Learning. All rights reserved 8 Section 21.1 The Transition Metals: A Survey Electron Configurations Example V: [Ar]4s23d3 Exceptions: Cr and Cu Cr: [Ar]4s13d5 Cu: [Ar]4s13d10 Copyright © Cengage Learning. All rights reserved 9 Section 21.1 The Transition Metals: A Survey Electron Configurations First-row transition metal ions do not have 4s electrons. Energy of the 3d orbitals is significantly less than that of the 4s orbital. Ti: [Ar]4s23d2 Ti3+: [Ar]3d1 Copyright © Cengage Learning. All rights reserved 10 Section 21.1 The Transition Metals: A Survey CONCEPT CHECK! What is the expected electron configuration of Sc+? Explain. [Ar]3d2 Copyright © Cengage Learning. All rights reserved 11 Section 21.1 The Transition Metals: A Survey Plots of the First (Red Dots) and Third (Blue Dots) Ionization Energies for the First-Row Transition Metals Copyright © Cengage Learning. All rights reserved 12 Section 21.1 The Transition Metals: A Survey Atomic Radii of the 3d, 4d, and 5d Transition Series Copyright © Cengage Learning. All rights reserved 13 Section 21.2 The First-Row Transition Metals 3d transition metals Scandium – chemistry strongly resembles lanthanides Titanium – excellent structural material (light weight) Vanadium – mostly in alloys with other metals Chromium – important industrial material Manganese – production of hard steel Iron – most abundant heavy metal Cobalt – alloys with other metals Nickel – plating more active metals; alloys Copper – plumbing and electrical applications Zinc – galvanizing steel Copyright © Cengage Learning. All rights reserved 14 Section 21.2 The First-Row Transition Metals Oxidation States and Species for Vanadium in Aqueous Solution Copyright © Cengage Learning. All rights reserved 15 Section 21.2 The First-Row Transition Metals Typical Chromium Compounds Copyright © Cengage Learning. All rights reserved 16 Section 21.2 The First-Row Transition Metals Some Compounds of Manganese in Its Most Common Oxidation States Copyright © Cengage Learning. All rights reserved 17 Section 21.2 The First-Row Transition Metals Typical Compounds of Iron Section 21.2 The First-Row Transition Metals Typical Compounds of Cobalt Section 21.2 The First-Row Transition Metals Typical Compounds of Nickel Copyright © Cengage Learning. All rights reserved 20 Section 21.2 The First-Row Transition Metals Typical Compounds of Copper Section 21.2 The First-Row Transition Metals Alloys Containing Copper Copyright © Cengage Learning. All rights reserved 22 Section 21.3 Coordination Compounds A Coordination Compound Typically consists of a complex ion and counterions (anions or cations as needed to produce a neutral compound): [Co(NH3)5Cl]Cl2 [Fe(en)2(NO2)2]2SO4 K3Fe(CN)6 Copyright © Cengage Learning. All rights reserved 23 Section 21.3 Coordination Compounds Coordination Number Number of bonds formed between the metal ion and the ligands in the complex ion. 6 and 4 (most common) 2 and 8 (least common) Copyright © Cengage Learning. All rights reserved 24 Section 21.3 Coordination Compounds Ligands Neutral molecule or ion having a lone electron pair that can be used to form a bond to a metal ion. Monodentate ligand – one bond to a metal ion Bidentate ligand (chelate) – two bonds to a metal ion Polydentate ligand – more than two bonds to a metal ion Copyright © Cengage Learning. All rights reserved 25 Section 21.3 Coordination Compounds Coordinate Covalent Bond Bond resulting from the interaction between a Lewis base (the ligand) and a Lewis acid (the metal ion). Copyright © Cengage Learning. All rights reserved 26 Section 21.3 Coordination Compounds The Bidentate Ligand Ethylenediamine and the Monodentate Ligand Ammonia Section 21.3 Coordination Compounds The Coordination of EDTA with a 2+ Metal Ion ethylenediaminetetraacetate Copyright © Cengage Learning. All rights reserved 28 Section 21.3 Coordination Compounds Rules for Naming Coordination Compounds [Co(NH3)5Cl]Cl2 1. Cation is named before the anion. “chloride” goes last (the counterion) 2. Ligands are named before the metal ion. ammonia (ammine) and chlorine (chloro) named before cobalt Section 21.3 Coordination Compounds Rules for Naming Coordination Compounds [Co(NH3)5Cl]Cl2 3. For negatively charged ligands, an “o” is added to the root name of an anion (such as fluoro, bromo, chloro, etc.). 4. The prefixes mono-, di-, tri-, etc., are used to denote the number of simple ligands. penta ammine Copyright © Cengage Learning. All rights reserved 30 Section 21.3 Coordination Compounds Rules for Naming Coordination Compounds [Co(NH3)5Cl]Cl2 5. The oxidation state of the central metal ion is designated by a Roman numeral: cobalt (III) 6. When more than one type of ligand is present, they are named alphabetically: pentaamminechloro Copyright © Cengage Learning. All rights reserved 31 Section 21.3 Coordination Compounds Rules for Naming Coordination Compounds [Co(NH3)5Cl]Cl2 7. If the complex ion has a negative charge, the suffix “ate” is added to the name of the metal. The correct name is: pentaamminechlorocobalt(III) chloride Copyright © Cengage Learning. All rights reserved 32 Section 21.3 Coordination Compounds EXERCISE! Name the following coordination compounds. a) [Co(H2O)6]Br3 hexaaquacobalt(III) bromide b) Na2[PtCl4] sodiumtetrachloro-platinate(II) Copyright © Cengage Learning. All rights reserved 33 Section 21.4 Isomerism Some Classes of Isomers Section 21.4 Isomerism Structural Isomerism Coordination Isomerism: Composition of the complex ion varies. [Cr(NH3)5SO4]Br and [Cr(NH3)5Br]SO4 Linkage Isomerism: Composition of the complex ion is the same, but the point of attachment of at least one of the ligands differs. Copyright © Cengage Learning. All rights reserved 35 Section 21.4 Isomerism Linkage Isomerism of NO2– Section 21.4 Isomerism Stereoisomerism Geometrical Isomerism (cis-trans): Atoms or groups of atoms can assume different positions around a rigid ring or bond. Cis – same side (next to each other) Trans – opposite sides (across from each other) Copyright © Cengage Learning. All rights reserved 37 Section 21.4 Isomerism Geometrical (cis-trans) Isomerism for a Square Planar Compound a) cis isomer b) trans isomer Section 21.4 Isomerism Geometrical (cis-trans) Isomerism for an Octahedral Complex Ion Copyright © Cengage Learning. All rights reserved 39 Section 21.4 Isomerism Stereoisomerism Optical Isomerism: Isomers have opposite effects on plane-polarized light. Copyright © Cengage Learning. All rights reserved 40 Section 21.4 Isomerism Unpolarized Light Consists of Waves Vibrating in Many Different Planes Copyright © Cengage Learning. All rights reserved 41 Section 21.4 Isomerism The Rotation of the Plane of Polarized Light by an Optically Active Substance Copyright © Cengage Learning. All rights reserved 42 Section 21.4 Isomerism Optical Activity Exhibited by molecules that have nonsuperimposable mirror images (chiral molecules). Enantiomers – isomers of nonsuperimposable mirror images. Copyright © Cengage Learning. All rights reserved 43 Section 21.4 Isomerism A Human Hand Exhibits a Nonsuperimposable Mirror Image Copyright © Cengage Learning. All rights reserved 44 Section 21.4 Isomerism CONCEPT CHECK! Does [Co(en)2Cl2]Cl exhibit geometrical isomerism? Yes Does it exhibit optical isomerism? Trans form – No Cis form – Yes Explain. Copyright © Cengage Learning. All rights reserved 45 Section 21.5 Bonding in Complex Ions: The Localized Electron Model Bonding in Complex Ions 1. The VSEPR model for predicting structure generally does not work for complex ions. However, assume a complex ion with a coordination number of 6 will have an octahedral arrangement of ligands. And, assume complexes with two ligands will be linear. But, complexes with a coordination number of 4 can be either tetrahedral or square planar. Copyright © Cengage Learning. All rights reserved 46 Section 21.5 Bonding in Complex Ions: The Localized Electron Model Bonding in Complex Ions 2. The interaction between a metal ion and a ligand can be viewed as a Lewis acid–base reaction with the ligand donating a lone pair of electrons to an empty orbital of the metal ion to form a coordinate covalent bond. Copyright © Cengage Learning. All rights reserved 47 Section 21.5 Bonding in Complex Ions: The Localized Electron Model The Interaction Between a Metal Ion and a Ligand Can Be Viewed as a Lewis Acid-Base Reaction Copyright © Cengage Learning. All rights reserved 48 Section 21.5 Bonding in Complex Ions: The Localized Electron Model Hybrid Orbitals on Co3+ Can Accept an Electron Pair from Each NH3 Ligand Section 21.5 Bonding in Complex Ions: The Localized Electron Model The Hybrid Orbitals Required for Tetrahedral, Square Planar, and Linear Complex Ions Section 21.6 The Crystal Field Model Focuses on the energies of the d orbitals. Assumptions 1. Ligands are negative point charges. 2. Metal–ligand bonding is entirely ionic: strong-field (low–spin): large splitting of d orbitals weak-field (high–spin): small splitting of d orbitals Copyright © Cengage Learning. All rights reserved 51 Section 21.6 The Crystal Field Model Octahedral Complexes d z and d x y point their lobes directly at the pointcharge ligands. d xz , d yz ,and d xy point their lobes between the point charges. 2 2 2 Copyright © Cengage Learning. All rights reserved 52 Section 21.6 The Crystal Field Model An Octahedral Arrangement of Point-Charge Ligands and the Orientation of the 3d Orbitals Copyright © Cengage Learning. All rights reserved 53 Section 21.6 The Crystal Field Model Which Type of Orbital is Lower in Energy? Because the negative point-charge ligands repel negatively charged electrons, the electrons will first fill the d orbitals farthest from the ligands to minimize repulsions. The d xz , d yz ,and d xy orbitals are at a lower energy in the octahedral complex than are the d z and d x y orbitals. 2 2 2 Copyright © Cengage Learning. All rights reserved 54 Section 21.6 The Crystal Field Model The Energies of the 3d Orbitals for a Metal Ion in an Octahedral Complex Copyright © Cengage Learning. All rights reserved 55 Section 21.6 The Crystal Field Model Possible Electron Arrangements in the Split 3d Orbitals in an Octahedral Complex of Co3+ Section 21.6 The Crystal Field Model Magnetic Properties Strong–field (low–spin): Yields the minimum number of unpaired electrons. Weak–field (high–spin): Gives the maximum number of unpaired electrons. Hund’s rule still applies. Copyright © Cengage Learning. All rights reserved 57 Section 21.6 The Crystal Field Model Spectrochemical Series Strong–field ligands to weak–field ligands. (large split) (small split) CN– > NO2– > en > NH3 > H2O > OH– > F– > Cl– > Br– > I– Magnitude of split for a given ligand increases as the charge on the metal ion increases. Section 21.6 The Crystal Field Model Complex Ion Colors When a substance absorbs certain wavelengths of light in the visible region, the color of the substance is determined by the wavelengths of visible light that remain. Substance exhibits the color complementary to those absorbed. Copyright © Cengage Learning. All rights reserved 59 Section 21.6 The Crystal Field Model Complex Ion Colors The ligands coordinated to a given metal ion determine the size of the d–orbital splitting, thus the color changes as the ligands are changed. A change in splitting means a change in the wavelength of light needed to transfer electrons between the t2g and eg orbitals. Copyright © Cengage Learning. All rights reserved 60 Section 21.6 The Crystal Field Model Absorbtion of Visible Light by the Complex Ion Ti(H2O)63+ Copyright © Cengage Learning. All rights reserved 61 Section 21.6 The Crystal Field Model CONCEPT CHECK! Which of the following are expected to form colorless octahedral compounds? Zn2+ Cu+ Fe3+ Fe2+ Cr3+ Cu2+ Mn2+ Ti4+ Ni2+ Ag+ Section 21.6 The Crystal Field Model Tetrahedral Arrangement None of the 3d orbitals “point at the ligands”. Difference in energy between the split d orbitals is significantly less. d–orbital splitting will be opposite to that for the octahedral arrangement. Weak–field case (high–spin) always applies. Copyright © Cengage Learning. All rights reserved 63 Section 21.6 The Crystal Field Model The d Orbitals in a Tetrahedral Arrangement of Point Charges Copyright © Cengage Learning. All rights reserved 64 Section 21.6 The Crystal Field Model The Crystal Field Diagrams for Octahedral and Tetrahedral Complexes Copyright © Cengage Learning. All rights reserved 65 Section 21.6 The Crystal Field Model CONCEPT CHECK! Consider the Crystal Field Model (CFM). a) Which is lower in energy, d–orbital lobes pointing toward ligands or between ? Why? b) The electrons in the d–orbitals – are they from the metal or the ligands? Copyright © Cengage Learning. All rights reserved 66 Section 21.6 The Crystal Field Model CONCEPT CHECK! Consider the Crystal Field Model (CFM). c) Why would electrons choose to pair up in d– orbitals instead of being in separate orbitals? d) Why is the predicted splitting in tetrahedral complexes smaller than in octahedral complexes? Copyright © Cengage Learning. All rights reserved 67 Section 21.6 The Crystal Field Model CONCEPT CHECK! Using the Crystal Field Model, sketch possible electron arrangements for the following. Label one sketch as strong field and one sketch as weak field. a) Ni(NH3)62+ b) Fe(CN)63– c) Co(NH3)63+ Copyright © Cengage Learning. All rights reserved 68 Section 21.6 The Crystal Field Model CONCEPT CHECK! A metal ion in a high–spin octahedral complex has 2 more unpaired electrons than the same ion does in a low–spin octahedral complex. What are some possible metal ions for which this would be true? Metal ions would need to be d4 or d7 ions. Examples include Mn3+, Co2+, and Cr2+. Copyright © Cengage Learning. All rights reserved 69 Section 21.6 The Crystal Field Model CONCEPT CHECK! Between [Mn(CN)6]3– and [Mn(CN)6]4– which is more likely to be high spin? Why? Copyright © Cengage Learning. All rights reserved 70 Section 21.6 The Crystal Field Model The d Energy Diagrams for Square Planar Complexes Copyright © Cengage Learning. All rights reserved 71 Section 21.6 The Crystal Field Model The d Energy Diagrams for Linear Complexes Where the Ligands Lie Along the z Axis Copyright © Cengage Learning. All rights reserved 72 Section 21.7 The Biological Importance of Coordination Complexes Metal ion complexes are used in humans for the transport and storage of oxygen, as electron-transfer agents, as catalysts, and as drugs. Copyright © Cengage Learning. All rights reserved 73 Section 21.7 The Biological Importance of Coordination Complexes First-Row Transition Metals and Their Biological Significance Copyright © Cengage Learning. All rights reserved 74 Section 21.7 The Biological Importance of Coordination Complexes Biological Importance of Iron Plays a central role in almost all living cells. Component of hemoglobin and myoglobin. Involved in the electron-transport chain. Copyright © Cengage Learning. All rights reserved 75 Section 21.7 The Biological Importance of Coordination Complexes The Heme Complex Section 21.7 The Biological Importance of Coordination Complexes Myoglobin The Fe2+ ion is coordinated to four nitrogen atoms in the porphyrin of the heme (the disk in the figure) and on nitrogen from the protein chain. This leaves a 6th coordination position (the W) available for an oxygen molecule. Section 21.7 The Biological Importance of Coordination Complexes Hemoglobin Each hemoglobin has two α chains and two β chains, each with a heme complex near the center. Each hemoglobin molecule can complex with four O2 molecules. Copyright © Cengage Learning. All rights reserved 78 Section 21.8 Metallurgy and Iron and Steel Production Metallurgy Process of separating a metal from its ore and preparing it for use. Steps: Mining Pretreatment of the ore Reduction to the free metal Purification of the metal (refining) Alloying Copyright © Cengage Learning. All rights reserved 79 Section 21.8 Metallurgy and Iron and Steel Production The Blast Furnace Used In the Production of Iron Copyright © Cengage Learning. All rights reserved Section 21.8 Metallurgy and Iron and Steel Production A Schematic of the Open Hearth Process for Steelmaking CaCO3 CaO + CO2 Heat 4Al + 3O2 2Al2O3 Copyright © Cengage Learning. All rights reserved 81 Section 21.8 Metallurgy and Iron and Steel Production The Basic Oxygen Process for Steelmaking Much faster. Exothermic oxidation reactions proceed so rapidly that they produce enough heat to raise the temperature nearly to the boiling point of iron without an external heat source.