Spin Hall effect J. Wunderlich(1), B. Kästner(1,2), J. Sinova (3), T. Jungwirth (4,5) (1) (2) (3) (4) (5) Hitachi Cambridge Laboratory, UK National Physical Laboratory, UK Texas A&M University, USA Institute of Physics ASCR, Czech Republic University of Nottingham, UK Collaborators: Allan MacDonald, Dimitri Culcer, Ewelina Hankeiwc, Qian Niu, Kentaro Nomura, Nikolai Sinitsyn, Laurens Molenkamp, Winfried Teizer SHE - Theory (http://unix12.fzu.cz/msnew) Entin-Wohlman:2005_a O. Entin-Wohlman, A. Aharony, Y. M. Galperin, V. I. Kozub, and V. Vinokur, "Orbital ac spin-Hall effect in the hopping regime", (2005), preprint cond-mat/0502478: on-line Liu:2005_a S. Y. Liu and X. L. Lei, "Vanishing of the Dissipationless Spin Hall Effect in a Diffusive Two-Dimensional Electron Gas with Spin-Orbit Coupling", (2005), preprint cond-mat/0502392: on-line Yao:2005_a Y. Yao, and Z. 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OUTLINE: - Theory remarks - Comments on experiments Kerr microscope Co-planar spin LED 10 µm p n SHE in a 2D hole gas [Wunderlich et. al., Phys. Rev. Lett. 94, 047204] SHE in a bulk semiconductor [Kato et. al., Science 306, 1910] Ordinary and quantum Hall effects B Lorentz force deflect like-charge particles _ _ _ _ _ _ _ _ _ _ _ Ordinary: +++++++++++++ Sign and density of carriers; holes in SC V Quantum FL I Resistance standard; fractional-charge carriers Anomalous Hall effect Spin-orbit coupling “force” deflects like-spin particles majority __ FSO _ FSO I H R0 B 4πRs M minority V InMnAs Simple electrical measurement of magnetization Spin Hall effect Spin-orbit coupling “force” deflects like-spin particles _ FSO __ FSO non-magnetic I V=0 Spin-current generation in non-magnetic systems without applying external magnetic fields Spin accumulation without charge accumulation excludes simple electrical detection Spin-orbit coupling (relativistic effect) Produces an electric field Ingredients: - potential V(r) E - motion of an electron In the rest frame of an electron the electric field generates and effective magnetic field - gives an effective interaction with the electron’s magnetic moment k E H SO Beff 1 E V (r ) e μ Beff k E Beff cm Skew scattering off impurity potential (Extrinsic SHE/AHE) H SO 2s 2 2 k Vimp(r) m c skew scattering If only this SO effect then much too weak to give a sizable SHE/AHE SO-coupling from host atoms (Intrinsic SHE/AHE) H SO E es k 1 dV (r ) Beff r s l mc mc er dr l=0 for electrons weak SO l=1 for holes strong SO E Enhanced in asymmetric QW v Intrinsic AHE approach explains many experiments • (Ga,Mn)As systems [Jungwirth et al PRL 02, APL 03] • Fe [Yao et al PRL 04] Experiment sAH 1000 (W cm)-1 Theroy sAH 750 (W cm)-1 • Layered 2D ferromagnets such as SrRuO3 and pyrochlore ferromagnets [Onoda and Nagaosa, J. Phys. Soc. Jap. 01,Taguchi et al., Science 01, Fang et al Science 03, Shindou and Nagaosa, PRL 01] • Manganites, [Ye et al. PRL 99] • Ferromagnetic spinel CuCrSeBr [Lee et al. Science 04] INTRINSIC SPIN-HALL EFFECT: [Murakami et al Science 2003 (cond-mat/0308167) Sinova et al PRL 2004 (cont-mat/0307663)] Let’s start with a simple model: Rashba SO coupling in a 2DEGs Inversion symmetry no R-SO Broken inversion symmetry R-SO 2k 2 2k 2 Hk ( k xsy k ys x ) s ( z k ) 2m 2m [Bychkov and Rashba 84] Heuristic argument: z-component of spin due to precession in effective "Zeeman" field dk Classical dynamics in k-dependent (Rashba) field: ( z k ), x eE x dt LLG equations for small drift adiabatic solution: dy x nz dt x dt dn y nz x 2 eEx y ( t ) ny ( t ) x Spin Hall conductivity js ,y ~ d p( nz , p p y ) 2 s sH js , y / E x e / 8 Classical and Kubo formula give the same spin-Hall conductivity s xysH Color plot of spin-Hall conductivity: yellow=e/8π and red=0 e m 2 2 * for n2 D n2 D 4 8 e n2 D * for n n 2D 2D 8 n*2 D Disorder effects: finite lifetime (Born approximation) for Rashba 2DEG ε F /(/τ) F ( / ) SO k F / intrinsic SHE Disorder effects: beyond the Born approximation for Rashba 2DEG Question: Are there any other major effects beyond the finite life time broadening? Can vertex corrections be ignored? Inoue, Bauer, Molenkamp PRB 04 Ladder sum vertex correction: Mal'shukov et al, PRL 04 Raimondi et al, PRB 04 Khaetskii, cond-mat/0408136 Loss et al, cond-mat/0407342 v2 ~ 0 s xysH 0 Spin Hall effect ? Extrinsic too weak to give any sizable effect Intrinsic cancelled by vertex corrections for infinitely weak disorder Ways to solve (go around) the controversy: - Skew scattering in SO-coupled bands not done yet - Intrinsic SHE in Rashba-SO systems beyond perturbation theory by solving Kubo formula exactly inconclusive (finite-size effects) [Nomura et al. PRB '05] - Other than Rashba-SO systems (intrinsic AHE explains experiments here) [Bernevig, Zhang, cond-mat/0411457, vertex corrections vanish in all other studied SO-systems (bulk, 2DHG,..) cond-mat/0412550 - Look at transport in mesoscopic systems instead of conductivity in the thermodynamic limit [Hankiewicz et al., PRB 04] [Nikolic et al., cond-mat/0412595] - Measure the effect Kato, Myars, Gossard, Awschalom, [Science 306, 1910] "Observation of the spin Hall effect in semiconductors" Local Kerr effect in n-type GaAs and InGaAs: ~0.03% polarization Bulk semiconductor stronger disorder n-type material weaker SO-coupling SO / Not in the intrinsic SHE regime Wunderlich, Kästner, Sinova, Jungwirth, [Phys. Rev. Lett. 94, 047204] Experimental observation of the spin-Hall effect in a two dimensional spin-orbit coupled semiconductor system Experiment “A” LED 1 a IP -Ip LED 1 p n n z LED 2 0 LED 1 y -Ip Experiment “B” +Ip x Ip x -1 LED 1 1 0 z ILED 1 ILED 2 y LED 2 1.505 1.510 1.515 -1 1.520 E [eV] Co-planar spin LED in GaAs 2D hole gas: ~1% polarization CP [%] 1.5m channel zI x y 1 CP [%] Ip +Ip y z Self-consistent LDA & 6-band calculations for the [001] QW etched GaAs p-AlGaAs 2DHG 2DEG i-GaAs n-AlGaAs E [meV] 20 a 0 s+ s20 HH+ 9 2.5 5 1.5 1 0. 5 10 20 30 p2D [1011 cm-2] 0 HH- LH -20 -0.2 0.0 Modulation doping weak disorder p-type asymmetric QW strong SO 0,2 ky [nm-1] SO / Close to the intrinsic SHE regime sS [e/8] 3D electron-2D hole Recombination / η [meV] GaAs/AlGaAs superlattice GaAs substrate A dissipationless remark ... Dissipative spin-polarized currents in non-magnetic systems at B=0 Spin-current is along the applied electric field proportional to non-equilibrium distribution function asymmetric scattering involving spin-flip [Ganichev et al., cond-mat/0403641, Silov et al. APL 04] Dissipationless intrinsic spin Hall effect ● Heuristic argument: transverse spin current generated between scattering events Sinova, Culcer, Niu, Sinitsyn, Jungwirth, MacDonald, PRL 92, 126603 (2004) ● Boltzman equation for current: transverse anomalous velocity in the equilibrium band structure due to combined E and SO effects Jungwirth, Niu, MacDonald, Phys. Rev. Lett. (2002) Murakami, Nagaosa, Zhang, Science 301, 1348-1351 (2003). anomalous velocity Berry curvature: M.V. Berry, Proc. Royal Soc. London (1984) normal group velocity Caution: the dissipationless transverse intrinsic SHE is accompanied by a dissipative longitudinal response to the electric field