CH 7: Carbohydrates First Biochemistry Chapter • Biochemistry – study of substances found in living organisms and their interactions with each other • Most important branch of science in medicine • Substances can be bio-inorganic or bio-organic • Bio-inorganic = water, ions, and ionic compounds • Bio-organic: • Carbohydrates: C, H, O • Lipids: C, H, O • Proteins: C, H, O, N, S • Nucleic Acids: : C, H, O, N, P Carbohydrates • Carbohydrates are the most abundant bio-orainc substance on the planet • Made by photosynthetic (PHS) organisms • PHS reaction – see board • Plants use the carbs made for 2 (really 3) purposes: 1. Source of energy – glucose (not a separate purpose in text) 2. Make starch – storage form of glucose 3. To make cellulose – structural polysaccharide found in cell walls Functions of Carbohydrates in Animals 1. Source of energy - glucose 2. Storage form of energy – glycogen • Made and stored in liver and muscles 3. Use carbons to make other bio-organic substances 4. 5 Carbon sugars are key component of DNA and RNA • Deoxyribose – DNA • Ribose – RNA 5. Short, often branched carbohydrates attach to proteins and lipids on the outside of the plasma membrane • Called glycoproteins and glycolipids Classifying Carbohydrates • Carbohydrate = polyhydroxyl aldehyde or ketone • Aldehyde carb = aldose sugar* • Ketone carb = ketose sugar* * monosaccharides and disaccharides are also referred to as sugars Classes of Carbohydrates 1. Monosaccharides – single polyhyroxyl ald/ketone unit 2. Oligosaccharides – 2-~10 monos. units joined by covalent bonds, may be branched • Disaccharides – 2 monos. units joined by covalent bond • Sucrose, lactose, maltose, cellobiose 3. Polysaccharides – MANY monos. units joined by covalent bonds • Glycogen • Starch – amylose and amylopectin • Cellulose Chiral Compounds • Many carbohydrates are chiral compounds • Chiral objects have mirror images that are cannot be superimposed (like your hands). • Chiral compounds have the same number of atoms arranged differently in space. • A chiral carbon atom has four different groups attached • Called a chiral center • Page 238 7 Determine if there is a chiral carbon in each compound. 8 ? Chiral Carbons ? D and L Notation - Cabohydrates • D,L tells which of the two chiral isomers of a carbohydrate we are referring to. • If the –OH group on the next to the bottom carbon atom points to the right , the isomer is a D-isomer; if it points left, the isomer is L. • The D form is usually the isomer found in nature. 10 D or L ? 11 Fischer Projections • Simplified way to show chiral centers Draw Fischer Projection for….. Terms • Chiral center (carbon) • Chiral compound – non-superimposable mirror images • chiral center present • Achiral compound - superimposable mirror images • no chiral centers New Types of Stereoisomers • Enantiomers – stereoisomers with non-superimposable mirror images • Diastereomers – stereoisomers that are not mirror images • Cis-trans isomers fit here as well as the carb isomers we’re working on • Epimers – diastereomers that differ at just one chiral center Examples…… • See board for examples…then from the book, COVER answers • 7.2 – example or practice exercise • 7.3 – “ “ • 7.4 – both example and practice exercise • Page 246 may be useful Properties of Enantiomers • Constitutional isomers differ in most chemical and physical properties • Enantiomers (a stereoisomer) have the same: • Boiling points, melting points • Density • Solubility and reactivity with achiral compounds • Enantiomers differ in: • Rotation of polarized light • Solubility in chiral solvents • Reactivity with chiral reactants Chiral Compounds and Polarized Light Enantiomers and Polarized Light • Enantiomers are optically active – rotate polarized light • May rotate in clockwise or counter-clockwise direction • Clockwise rotation = Dextrorotary (+) • Counter-clockwise rotation = Levorotary (-) • D & L enantiomers rotate light in opposite directions • Which direction they rotate is unrelated to the D/L designation and must be determined experimentally • The degree of rotation depends on the concentration of the solution and the identity of the substance. Monosacchrides - describing • Aldoses sugars are monosacchrides with an aldehyde group and many hydroxyl (-OH) groups. • Ketoses sugars are monosacchrides with a ketone group and many hydroxyl (-OH) groups. 20 Monosacchrides - describing • Three Carbons = Triose • Four Carbons = Tetrose • Five Carbons = Pentose • Six Carbons = Hexose • Page 251 21 Identify each as tetrose, pentose or hexose, and as aldose or ketose, D or L? 22 Hexose Monosaccharides CH2OH CHO H HO OH C H O O H O H HO H H O H H OH H O H H OH H CH2OH D-Glucose (aldohexose) O H C H 2 D-Galactose (aldohexose) OH H H OH H OH CH2OH D-Fructose (ketohexose) D-Glucose CHO H HO OH H H OH H OH •Also called blood sugar or dextrose* •70 - 100 mg/100 mL of blood •All other nutritionally important sugars are converted to glucose in the liver. •Forms a 6 membered cyclic hemiacetal CH2OH D-Glucose (aldohexose) * Name related to the clockwise rotation of light D-Galactose • D-galactose is an epimer of D-glucose • Rarely found as free monos. in nature • Find in Lactaid milk • Not very sweet CHO H OH HO H HO H H OH • Find galactose as a component of glycoproteins CH2 OH D-Galactose on brain and other nerve cells, also an (aldohexose) important carbohydrate in blood typing D-Fructose • Also known as fruit sugar and levulose • Rotates polarized light counter-clockwise • Sweetest of all monosacharides • High fructose corn syrup • Glucose and fructose differ in just the location of the carbonyl group CH2OH O HO H H OH H OH CH2OH D-Fructose (ketohexose) D-Ribose & D-Deoxyribose • Pentose Sugars – not nutritionally important • Components of RNA and DNA in hemiacetal (cyclic) forms Hemiacetal Formation – Cyclic Carbohydrates • Monosaccharides form cyclic hemiacetals • Formation of the hemiacetal • Alpha versus beta form (anomers) • Showing structure – Haworth projections • Chiral OH on right goes down on structure • Chiral OH on left goes up on structure Cyclic Hemiacetal Forms of D-Glucose 2 forms of cyclic D-glucose: • Alpha-form: -OH of C1 and CH2OH of C5 are on opposite sides • Beta-form: -OH of C1 and CH2OH of C5 are on 6 6 same sides CH OH CH OH 2 5 4 OH 2 O 1 OH 2 3 OH OH 4 OH O OH 2 3 OH -D-Glucose Copyright © Cengage Learning. All rights reserved 5 -D-Glucose 30 OH 1 Glucose in solution CHO H HO H H 6 6 OH CH2OH CH 2OH H 5 OH OH CH2OH D-Glucose (aldohexose) Less than .01% 4 OH O 1 OH 2 3 OH OH -D-Glucose 37% glucose 5 4 OH O OH 2 OH 1 3 OH -D-Glucose 63% glucose D-Ribose D-Fructose CH2OH O HO •Forms a 5 membered cyclic form H H OH H OH CH2OH CH2OH D-Fructose (ketohexose) CH2OH O CH2OH O OH OH OH OH -D-Fructose OH OH -D-Ribose Skip 7.12 (for now!) Disaccharides • Monosaccharides in their cyclic form react to form acetals……aka…disacharrides or a glycoside • Bond is called a glycosidic linkage • Disaccharides we will consider: 1. Maltose 2. Cellobiose 3. Lactose 4. Sucrose • Goal is to: • Know constituent monosaccharides • Recognize type of bond • Know how body handles – digestible or not? • Identify sugar as a reducing sugar or not • Page 262 Formation of Maltose Maltose CH2 OH CH2 OH O O OH OH O OH OH OH • - D –glucose -- D-glucose Copyright © Cengage Learning. All rights reserved OH (1-4) 37 Cellobiose • - D –glucose -- D-glucose CH2OH O (1-4) CH2OH O H OH O OH OH OH OH Cellobiose Copyright © Cengage Learning. All rights reserved 38 OH Lactose • - D –galactose -- D-glucose CH2OH CH2OH O OH O (1-4) H OH O OH OH OH Lactose Copyright © Cengage Learning. All rights reserved 39 OH Sucrose – , (1->2) linkage CH2 OH O CH2 OH OH O OH OH OH OH -D-Glucose OH OH + CH2 OH , (1->2) linkage OH O CH2 OH OH O (1-2) Linkage O OH CH 2OH OH -D-Fructose CH 2OH OH Sucrose Polysaccharides - Consider 1. Sugars present in polymer • Homopolysaccharide or heteropolysaccharide 2. Length of chain 3. Extent of branching 4. Type of linkage between monomers and at branch points Polysaccharides 1. Starch • Amylose • Amylopectin 2. Glycogen 3. Cellulose 4. Chitin (not covered) Starch • Starch: • Polymer of glucose • Storage form of glucose in plants • Two forms • Amylose • Amylopectin Copyright © Cengage Learning. All rights reserved 43 Amylose • 15 - 20% of starch • Straight chain polymer • coils • Up to ~1000 glucose units • (1 4) glycosidic bonds Amylopectin • 80 - 85 % of the starch • Branched chain polymer of glucose • (14) glycosidic bond for straight chain and (16) at the branch • Branch every ~25-30 glucose • up to 100,000 glucose units • Humans can hydrolyze alpha linkages in starch Glycogen • Polymer of glucose, up to 1,000,000 glucose units • Excess glucose in blood stored in the form of glycogen – animal storage form of glucose • Bonding? • Branch every ~8-12 glucose • ~2-3x more branched than amylopectin Cellulose HO O HO O HO O HO O O O (1-4) OH OH O (1-4) OH O (1-4) OH OH OH OH OH • Structural polysaccharide – made by plants, bacteria, and others (not humans) • Straight chain polymer of glucose, up to ~ 5,000 glucose units • (1 4) glycosidic bonds between glucose • Humans don’t have enzymes that hydrolyze (1 4) - so humans cannot digest cellulose O Cellulose chains crosslink with H bonds to form bundles/fibers – Cotton ~95% cellulose and wood ~50% cellulose Reactions of Monosaccharides Oxidation Reactions (3) 1. Mild oxidizing agent such as Tollen’s or Benedict’s o All monosaccharides and disaccharides except sucrose react – called reducing sugars o Hemiacetal group opens to reform the aldehyde or ketone group o o o Ketone group rearranges to form an aldehyde Reaction oxidizes the aldehyde to a carboxylic acid No hemiacetal to open in sucrose Oxidation of Monosaccharides 2. Strong oxidizing agents can oxidize both ends of a monosaccharide • the carbonyl group and the terminal primary alcohol group oxidize to produce a dicarboxylic acid. 3. Enzymes can oxidize the primary alcohol end of an aldose such as glucose, without oxidation of the aldehyde group! • VERY difficult to do in the lab Reduction to a Sugar Alcohol • The carbonyl group in a monosaccharide (either an aldose or a ketose) is reduced to a hydroxyl group using hydrogen as the reducing agent. • The product is the corresponding polyhydroxy alcohol - sugar alcohol. • Sorbitol CHO H HO OH H H OH H OH CH2OH D-Glucose (aldohexose) Sorbitol Reactions of Monosaccharides • Glycoside formation – already covered • Hemiacetal of one carb. Reacts with an alcohol group on another carb to produce a glycosidic linkage/bond