Chemical Reactions: Bonding and Changes in Physical Properties - Part 2 Dr. Pedro M. Pereyra Holy Trinity 2006, 2007, 2008, 2012 © Version 2 Rev 1 Expectations Matter and its changes • • • • explain how different elements combine to form covalent and ionic bonds using the octet rule demonstrate an understanding of the formation of ionic and covalent bonds and explain the properties of the products demonstrate an understanding of the relationship between the type of chemical reaction (e.g., synthesis, decomposition, single and double displacement) and the nature of the reactants relate the reactivity of a series of elements to their position in the periodic table (e.g., compare the reactivity of metals in a group and metals in the same period; compare the reactivity of non-metals in a group). Dr. Pedro M. Pereyra ©) 2006 Index • • • • • Bonding Continuum Types of Compounds & Bond properties Molecular and Ionic Compounds Intermolecular Forces & Interactions Physical properties arising from intermolecular interactions Dr. Pedro M. Pereyra ©) 2006 Bonds & Bond Formation Bonds and Bond Formation Applications and extension of the concept of Electronegativity (÷) Lewis Dot Diagrams • Types of Bonds: • Ionic, Pure Covalent, Polar Covalent and Coordination bonding Network bonding Metallic Bonding Electronegativity (÷) • Difference in Electronegativity (Ä÷) and % Ionic Character • Bonding Continuum • Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Bonds and Bond Formation • Bonds - binding atoms together Linus Pauling's definition of the chemical bond: "whatever is convenient to the chemist to define as a bond" • • Source: http://www.iupac.org/general/about.html Some other less “convenient” definitions: In general a bond is established between atoms by the balance of the electrostatic (e.g. charge attraction or repulsions) and electromagnetic forces (e.g. those responsible fro the structure of the electrons in an atom) acting between the valence electrons and the residual nuclear attractions (e.g electron affinity) of the atoms involved. • A covalent bond is considered when a pair of electrons share the valence shell of the combining atoms • A coordination bond is considered when a pair of electrons is donated by only one of the combining atoms. • An ionic bond is considered when the available valence electrons of one atom are donated to the valence shell of an other atom forming a positively and a negatively charged species that are predominantly attracted by electrostatic forces Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Bonds and Bond Formation Bonding and the Concept of Valence • • • Valence, also known as valency or valency number, is a measure of the number of chemical bonds formed by the atoms of a given element. The concept was developed in the middle of the nineteenth century in an attempt to rationalize the formulae of different chemical compounds. Although it has fallen out of use in higher level work with the advances in the theory of chemical bonding, it is still widely used in elementary studies where it provides a heuristic introduction to the subject. • Source: http://en.wikipedia.org/wiki/Valence_(chemistry) Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Bonds and Bond Formation Bonding and the Concept of Valence • The number of bonds formed by a given element was originally thought to be a fixed chemical property and in fact, in many cases, this is a good approximation. • However it soon became apparent that, for many elements, the valence could vary between different compounds. • For example, in virtually all of their compounds, carbon forms four bonds, oxygen two and hydrogen one. One of the first examples to be identified was phosphorus, which sometimes behaves as if it has a valence of three and sometimes as if it has a valence of five. One method around this problem is to specify the valence for each individual compound although it removes much of the generality of the concept, this approach has given rise to the idea of oxidation numbers (used in Stock nomenclature) and to lambda notation in the IUPAC nomenclature of inorganic chemistry. • Source: http://en.wikipedia.org/wiki/Valence_(chemistry) Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Types of Bonds • Ionic Bonding When an atom, generally a metal atom, loses one or more of its electrons, a positive ion or Cathion is formed. Na 6 Na+ + eG • When an atom, generally a non-metal atom, gains one or more electrons, a negative ion or Anion is formed. Cl 2 + 2eG 6 2ClG • Just as with the opposite poles of a magnet, when positive and negative ions approach one another a very strong force of attraction is formed. • • Source: http://www.rjclarkson.demon.co.uk/found/found3.htm Kind: group of individuals that share features: a group or class of individuals connected by shared characteristics Microsoft® Encarta® Reference Library 2004. © 1993-2003 Microsoft Corporation. All rights reserved. Type: a category of things or people whose members share some qualities Microsoft® Encarta® Reference Library 2004. © 1993-2003 Microsoft Corporation. All rights reserved. Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Types of Bonds • Ionic Bonding This is called an ionic bond, though more accurately it is a strong ionic force of attraction. + Na + + ClG 6 Na GCl or NaCl • • • • • Source: http://www.rjclarkson.demon.co.uk/found/found3.htm In strict terms, an ionic bond refers to the electrostatic attraction experienced between the electric charges of a cation and an anion, in contrast with a purely covalent bond where electrons are shared between atoms. Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Types of Bonds Covalent Bonding • covalent bond is a chemical bond that involves sharing pairs of electrons between atoms in a molecule • • http://www.wordreference.com/definition/covalent%20bond The following kind of covalent bonding are recognized: Single covalent bond: when a single covalent bond is established between two atoms • • Double covalent bond: when two covalent bonds are established between two atoms perpendicular to each other. Two possibilities are recognized: • • One sigma bond and one pi bond are formed Two pi bonds are formed Triple covalent bond: when three covalent bonds are established between two atoms. • • Along the axis of encounter: Sigma bond ( ó). Perpendicular to the axis of encounter: Pi bond ( ð). Usually formed when one sigma bond and two pi bond are. established coordinate bond or dative bond is a covalent bond in which both electrons are provided by one of the atoms. Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Types of Bonds Ionic - Covalent Bonds and %Ionic Character • • In practice, it is preferable to consider the amount of ionic character of a bond rather than referring to purely ionic or purely covalent bonds. The relationship was proposed (L.Pauling) for the estimation of ionic character of a bond between atoms A and B: • • • • where ÷A and ÷B. are the Pauling electronegativities of atoms A and B. Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Electronegativity and % Ionic Character Electronegativity (÷) • "Electronegativity is the power of an atom when in a molecule to attract electrons to itself." The electronegativity will depend upon a number of factors including other atoms in the molecule, the number of atoms coordinated to it, and the oxidation number for the atom. There are a number of ways to produce a set of numbers which represent electronegativity scales. The Pauling scale is perhaps the most famous. Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Electronegativity and % Ionic Character Difference in Electronegativity (Ä÷) and % Ionic Character • Pauling noticed that the bond energy E(AB) in a molecule AB is always greater than the mean of the bond energies E(AA) + E(BB) in the homonuclear species AA and BB. • E (AB) > (E(AA) + E(BB))/2 • • Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Electronegativity and % Ionic Character Difference in Electronegativity (Ä÷) and % Ionic Character • His argument was that in an "ideal" covalent bond, E(AB) should equal this mean, and that the "excess" bond energy is caused by electrostatic attraction between the partially charged atoms in the heteronuclear species AB. In effect, he was saying that the excess bond energy arises from an ionic contribution to the bond (% Ionic Character) . Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Electronegativity and % Ionic Character Difference in Electronegativity (Ä÷) and % Ionic Character • He managed to treat this ionic contribution by the equation • E (AB) = [E(AA) + E(BB)]/2 + 96.48(÷A -÷B)2 • in which E(AB is expressed in kJ mol-1 and ÷A -÷B represents the difference in "electronegativity" between the two elements, whose individual electronegativities are given the symbols ÷A and ÷B. • Using this equation, Pauling found that the largest electronegativity difference was between Cs and F. Pauling set F arbitrarily at 4.0 (today, the value for F is set to 3.98) and this gives a scale in which the values for all other elements are less than 4 but still with a positive number. Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 % Ionic Character vs Ä÷ Calculation of % Ionic Character in terms of Pauling's Electronegativity and in terms of Hannay & Smyth: ( ) 2 IC(Dc) := 1 - e - .25 ×Dc Dc := 0, .1.. 4 2 ICHS(Dc) := 0.16Dc + 0.035Dc % Ionic Character vs Electronegativity Dc = 1.2 1 0.8 IC(Dc) = ICHS(Dc) = 2.497•10 -3 0 0.016 9.95•10 -3 0.033 0.3 0.022 0.051 0.4 0.039 0.07 0 0.1 0.2 0 0.5 0.061 0.089 IC( Dc) 0.6 0.086 0.109 ICHS( Dc) 0.6 0.7 0.115 0.129 0.8 0.148 0.15 0.9 0.183 0.172 1 0.221 0.195 1.1 0.261 0.218 1.2 0.302 0.242 1.3 0.345 0.267 1.4 0.387 0.293 1.5 0.43 0.319 0.4 0.2 0 0.5 1 1.5 2 2.5 3 3.5 4 Dc Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Bonding Continuum Pure vs Polar Covalent vs Ionic Bonding Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Bonding Continuum Pure vs Polar Covalent vs Ionic Bonding • Pure covalent bonds are considered to have very little if no ionic character at all. %Ionic Character corresponding to electronegativity differences between 0 and 0.50 Charge density distribution is symmetrical. For example Hydrogen gas (H2) The term polarity refers to the presence in the same particle (e.g. molecule or atom) of a positively charged and a negatively charged regions The term charge density refers to the volume in space around and between atoms where the bonding electrons are concentrated Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Bonding Continuum Pure vs Polar Covalent vs Ionic Bonding Covalent bond is interpreted as a bonf formed by “sharing” a pair of electrons between two atoms. • It actually represents the formation of an energy level common to the two bonding atoms known as a Molecular Orbital (MO). • • Every MO has two possible states • A high energy state where the two electrons have unpaired spins (88) also known as anti-bonding state • A low energy state where the two electrons have a paired spins (89) also known as bonding state For atoms to bond covalently the bonding state of the bonding MO must exist at a lower energy level than the energy level of the atomic orbitals where the electrons originated from Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Bonding Continuum Pure vs Polar Covalent vs Ionic Bonding • • As we learned before the electron of hydrogen atoms exist in an energy level with the value of -13.6eV The bonding Molecular Orbital of the hydrogen molecule has a value of -17.6eV. A state 4eV lower in energy favouring the formation og hydrogen gas. Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Bonding Continuum Pure vs Polar Covalent vs Ionic Bonding • Polar covalent bonds are considered to have some to considerable ionic character due to the difference in electronegativity of the bonding atoms %Ionic Character corresponding to electronegativity differences larger then 0.50 and up to about 1.6 Charge density distribution is asymmetrical due to the electrostatic effect of the atom with higher electronegativity. A MO is present because such an energy level is still of lower energy than the atomic orbital supplying the electrons For example • Carbon Monoxide gas (CO) with Ä÷ = 1.0, or Hydrogen Chloride (HCl) with Ä÷ = 0.8 Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Bonding Continuum Pure vs Polar Covalent vs Ionic Bonding • Ionic bonds are considered to have considerable ionic character due to the difference in electronegativity of the bonding atoms %Ionic Character corresponding to electronegativity differences larger then 1.60. Charge density distribution is biased to the atom or group with highest electronegativity duue to the strong electrostatic effect. The energy level of the MO is higher or equal to that of the atomic orbital of the atom with the strongest electronegativity For example Lithium Chloride. Noticed the charge density concentrated in the chlorine atom only Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Na Cl Types of Compounds Types of Compounds Tetrahedron of Material Type Just like we considered before a bonding continuum between ionic and molecular compounds, we can incorporate the other bonding types to build a tetrahedron of material types known erroneously as Laing Tetrahedron. http://www.meta-synthesis.com/webbook/38_laing/tetrahedra.html Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Types of Compounds Tetrahedron of Material Type Dr. Pedro M. Pereyra ©) 2006 Types of Compounds Tetrahedron of Material Type We have become empirically familiar with some of the concepts related to the continuum between molecular and network compounds when we observed the drastic changes in physical properties of sulfur as it was heated, changing from a molecule (S8)to polymeric chains (Sn) and back to molecules. (S2 6 S8) We are also familiar with this molecular dimensionality in plastics and biological macromolecules S8 6 S n 6 S 2 6 S 8 160EC Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties 600EC 20EC Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Types of Compounds Tetrahedron of Material Type The range of ionic to network bonding compounds is associated with many ceramics and refractory oxides and the range of metallic to ionic bonding compounds is associated with many known alloys Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Types of Compounds Tetrahedron of Material Type Dr. Pedro M. Pereyra ©) 2006 Types of Compounds Molecular compounds Molecules are made of atoms covalently bonded and with a definite geometry defined by fix average bond lengths and bond angles • The geometries are defined by • • the balance of attractive and repulsive forces among the atoms making up the molecule. The number and type of covalent bonds made by each atom The number of unused electrons remaining in the valence shell after bonding (electron pairs or free radicals). When assessing the possible geometries these electrons count as a bond (for every unused pair or for every free radical) The following basic geometries are recognized: Linear (180E) Triangular Planar (120E) Tetrahedral (109.5E) Triangular bipyramidal (120E and 90E) Square bipyramidal (90E) Pentagonal bipyramidal (72E and 90E) Hexagonal bipyramidal (60E and 90E) Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Types of Compounds Molecular compounds Atoms with valence electrons in “s” and “p” orbitals can only contain up to 4 pairs of electrons or 4 bonds; their geometries are restricted to linear, triangular planar, and tetrahedral. • Atoms with “d” valence electrons can also contain electrons in “s” and “p” type orbitals allowing for higher order geometries • BeBr2 ; 180E Linear BF3 ; 120E Triangular Planar Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties CH4 ; Tetrahedral Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Net Polarity Polar Molecular compounds Molecules with polar covalent bonds exhibit a collective property known and Net Dipole Moment • In general, each polar bond will contribute to the total, or net polarity of the molecule in a predictable way determined by the average geometry of the molecule. • In Beryllium Bromide’s case the strong polarity arising from the difference in electronegativity (Ä÷ = 1.3) between Beryllium and Bromine is cancelled by the overall symmetrical geometry of the molecule giving rise to a Net Dipole Moment of zero • BeBr2 ; 180E Linear Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Net Polarity Polar Molecular compounds • In a similar way Boron Trifluoride and Methane will display also a Net Dipole Moment of zero. BF3 ; 120E Triangular Planar CH4 ; Tetrahedral Symmetrical Molecules will display a Net Dipole Moment of zero Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Net Polarity Polar Molecular compounds • • • • Some molecules, as mentioned before, will contain also unbonded or lone pairs of electrons in their valence shell. These electrons will contribute to the overall geometry of the molecule. Water and ammonia are two important molecules that display a geometry influenced by the valence electron pairs In the case of water, Oxygen has two electron pairs, that together with the two bonded Hydrogen requires a tetrahedral geometry. In the case of ammonia, Nitrogen has one electron pair and is bonded to three Hydrogen requiring also a tetrahedral geometry Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties Angle between Hydrogens = 104.5E Angle between Hydrogens = 109.5E Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Net Polarity Polar Molecular compounds • The resultant molecules are not totally symmetric and the polarity of their bonds becomes enhanced resulting in a definite and significant Net Dipole Moment Angle between Hydrogens = 104.5E The Net Dipole Moment gives water a strong net polarity that determines much of its unique physical properties The H-O dipoles cancel in their horizontal, but not in their vertical components Reactions Types Mechanisms Bonding Intermolecular Interactions Physical properties Bond types Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Application Exercises We are now in a position to predict some of the fundamental structural properties of simple molecular compounds by applying what we have learned about bonding and bonds in a systematic manner: • We start with the compositional formula of the compound and: • • Determine the electronegativity difference (Ä÷) for each atom pair involved in the compound’s bonds. Using Lewis Dot diagrams, determine the bonding pattern among the atoms making up the compound With this information we can determine The types of bonds, their polarity, as well as, their % Ionic Character (%IC). The number and kind of bonds in the compound, and The number of electron pairs or free radicals not involved in bonding As a last step we can now determine the most likely geometry of the arrangement of the atoms around the central atom of the compound and if the molecule will or not display a net polarity • For example: CO2 • Application Exercises From the Ä÷ we can determine that the bonds between Carbon and Oxygen must be polar covalent, indicating that it is a molecular compound. Application Exercises From the Ä÷ we can determine that the bonds between Carbon and Oxygen must be polar covalent, indicating that it is a molecular compound. From the Lewis Dot bonding diagram we can infer that carbon is linked to oxygen by double bonds Application Exercises From the Ä÷ we can determine that the bonds between Carbon and Oxygen must be polar covalent, indicating that it is a molecular compound. From the Lewis Dot bonding diagram we can infer that carbon is linked to oxygen by double bonds Because carbon has no other electrons in its valence shell we can distribute the two Oxygens 180E apart, thus as far as possible from each other; giveing the moleclule a linear geometry. Because of this, the polarity of the Carbon-Oxygen bonds is cancelled giving the molecule a net polarity of zero Application Exercises Intermolecular Forces and Bulk Physical Properties Intermolecular interactions Effects of ionic and polar bonding • Van der Waals Forces(§) (<0 - 10 kJ/mol) • Dispersion or London Forces (London 1930) • Induced dipole-induced dipole interactions in particles with no or very weak permanent polarity Dipole-dipole interactions (Keesom 1912) • In particles with a permanent net-dipole Ion-dipole and ion-induced dipole interactions H-bonding (~24 kJ/mol) (§)There's a bit of a problem here with modern syllabuses. The majority of the syllabuses talk as if dipole-dipole interactions were quite distinct from van der Waals forces. Such a syllabus will talk about van der Waals forces (meaning dispersion forces) and, separately, dipole-dipole interactions. All intermolecular attractions are known collectively as van der Waals forces. The various different types were first explained by different people at different times. Dispersion forces, for example, were described by London in 1930; dipole-dipole interactions by Keesom in 1912. http://www.chemguide.co.uk/atoms/bonding/vdw.html Reactions Types Mechanisms Intermolecular Interactions Bonding Bond types Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Intermolecular interactions Dispersion Forces The dynamic nature of electrons in all atoms and molecules (particles) allows for the momentary polarization of the particle creating a weak dipole, even if the particle shows no or only a very weak net polarity. • Neighboring particles within a critical distance will be influenced by this momentary polar force allowing for the formation, on the neighboring particles, of an induced-dipole. • In its turn, so long as the particles are close to each other, this induced-dipoles will reinforce the induce-dipoles in all the particles involved. • The larger the particle the stronger this induced-dipole interactions are going to be. Shape of the particle also influences dispersion force effects. • Reactions Types Mechanisms Intermolecular Interactions Bonding Bond types Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Intermolecular interactions Dispersion Forces • The dynamic nature of electrons in all atoms and molecules (particles) allows for the momentary polarization of the particle creating a weak dipole, even if the particle shows no or only a very weak net polarity. Reactions Types Mechanisms Intermolecular Interactions Bonding Bond types Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Intermolecular interactions Dispersion Forces • • Neighboring particles within a critical distance will be influenced by this momentary polar force allowing for the formation, on the neighboring particles, of an induced-dipole. In its turn, so long as the particles are close to each other, this induced-dipoles will reinforce the induce-dipoles in all the particles involved. Dr. Pedro M. Pereyra ©) 2006 Intermolecular interactions Dispersion Forces and Physical Properties • The effect of dispersion forces at the bulk level translates into important physical behaviors such as the trends in the melting or boiling point of pure non-metal elements and molecular substances, as well as, their behaviour in mixtures. For example: Noble Gases b.p. of Noble gases 0 -50 -100 -150 -200 -250 -300 Helium Neon Argon Krypton Xenon Radon Helium Neon Argon Krypton Xenon Radon -269 -246 -186 -152 -108 -62 Dr. Pedro M. Pereyra ©) 2006 Intermolecular interactions Dispersion Forces and Physical Properties • The effect of dispersion forces at the bulk level translates into important physical behaviors such as the trends in the melting or boiling point of pure nonmetal elements and molecular substances, as well as, their behaviour in mixtures. For example: Hydrocarbons are particularly good examples of the effects of dispersion forces on boiling and melting points as a function of molecular size and carbon chain. 300 200 100 0 -100 -200 m.p. (C) Methane CH4 Butane C4H10 Heptane C7H16 Dacane C10H22 Methane CH4 Ethane C2H6 Propane C3H8 Butane C4H10 Pentane C5H12 Hexane C6H14 Heptane C7H16 Octane C8H18 Nonane C9H20 Dacane C10H22 Tetradecane C13H28 b.p. (C) Ethane C2H6 Pentane C5H12 Octane C8H18 Tetradecane C13H28 Propane C3H8 Hexane C6H14 Nonane C9H20 -182 -182 -190 -138 -125 -95 -91 -57 -53 -30 3 -161 -88 -44 -0.5 36 68 98 126 151 174 254 Dr. Pedro M. Pereyra ©) 2006 Intermolecular interactions Dispersion Forces and Physical Properties • The effect of dispersion forces is strongly dependent of the number of electrons present in the molecule. This is shown below for molecules with the same number of carbons and hydrogens -an therefore the number of electrons. As is evident, the dispersion effect on melting and boiling points is barley affected by the shape of the molecule 100 50 0 -50 -100 -150 m.p. (C) 2,2 Dimethylpentane 2,2 Dimethylpentane 2,3 Dimethylpentane 2,4 Dimethylpentane 2 Methylhexane 2,3 Dimethylpentane b.p. (C) 2,4 Dimethylpentane 2 Methylhexane -124 -124 -119 -118 79 90 80 90 Dr. Pedro M. Pereyra ©) 2006 Intermolecular interactions dipole-dipole interactions • • • Dipole-dipole interaction forces work on similar principles as dispersion force interactions. They are stronger due to the permanent net-dipole nature of the molecules due to the presence of an element in the molecule with a high electronegativity (e.g. F, Cl, O, etc.) The effect of the net-dipole sometimes enhances the attraction among molecules, however, the combined effect of all dispersion forces in a molecule can sometimes be more significant. Reactions Types Mechanisms Intermolecular Interactions Bonding Bond types Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Intermolecular interactions dipole-dipole interactions • Case study: monocarbon chloride compounds CH4 CH3Cl CH2Cl2 CHCl3 CCl4 m.p.°C -182 -91 -75 -63 -23 b.p.°C -161 -26 40 61 77 100 50 0 -50 -100 -150 -200 CH4 CH3Cl CH2Cl2 CHCl3 m.p m.p b.p Reactions Types Mechanisms Intermolecular Interactions Bonding Bond types Physical properties -182 -161 Bond properties -91 -26 CCl4 b.p -75 40 -63 61 -23 77 Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Intermolecular interactions Ion - Dipole and Ion-Induced dipole • • Ions are permanently charged particles that will interact strongly with polar substances The solubilization of many ionic compounds in polar solvents like water is a classic example of ion-dipole interactions Reactions Types Mechanisms Intermolecular Interactions Bonding Bond types Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Intermolecular interactions hydrogen bonding • • • Hydrogen bonding or H-bonding is a unique type of intermolecular interaction somewhere between dipole-dipole interactions and coordination bonding. The term H-bonding was coined by Huggins in 1912 and widely publicized by Pauling’s “Nature of the Chemical Bond” and published in 1930. The idea however was first discussed by Nerst in 1891 working with hydroxides H-bonding is unique to a limited number of compounds containing Oxygen, Nitrogen or Fluorine Hydrogen bonds • O-H, N-H, or F- H. The interaction is established between a pair of “active” non-bonding valence electrons in the strong electronegative element (F, O, or N) and the Hydrogen bonded to a similar strong electronegative element: e.g: N: ----- H - N http://www.chemguide.co.uk/atoms/bonding/hbond.html#top http://www.hbond.de/ Reactions Types Mechanisms Intermolecular Interactions Bonding Bond types Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Intermolecular interactions hydrogen bonding • • Evidence of H-bonding is easily demonstrated by comparing the boiling points of the “hydrides” of the group 4, 5, 6, and 7 elements The hydrides of the group 4 elements follow the expected increase of boiling point with increasing molecular size due to dispersion force effects http://www.chemguide.co.uk/atoms/bonding/hbond.html#top Reactions Types Mechanisms Intermolecular Interactions Bonding Bond types Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Intermolecular interactions hydrogen bonding • When the “hydrides” of the group 5, 6, and 7 elements are compared, however, the hydrides of Fluorine, Oxygen and Nitrogen depart dramatically from the expected pattern by showing very elevated boiling points http://www.chemguide.co.uk/atoms/bonding/hbond.html#top Reactions Types Mechanisms Intermolecular Interactions Bonding Bond types Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Intermolecular interactions hydrogen bonding • The strong electronegativity of these three elements (F, O, and N) coupled with the presence of “active” unoccupied (lone) electron pairs in their valence shell, lead to a very strong dipole that makes the Hydrogen atom strongly positive. http://www.chemguide.co.uk/atoms/bonding/hbond.html#top Reactions Types Mechanisms Intermolecular Interactions Bonding Bond types Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Intermolecular interactions hydrogen bonding • • This polarization is further enhanced as the hydride interacts with other similar hydrides; effectively allowing the electrons from two strong electronegative atoms to nearly coordinate with one Hydrogen atom In Nitrogen and Oxygen containing hydrides the effect is the formation of extensive intermolecular bonding networks See article Ultrafast h-bond dynamics (AAAS) Reactions Types Mechanisms Intermolecular Interactions Bonding Bond types Physical properties http://www.chemguide.co.uk/atoms/bonding/hbond.html#top Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Application Exercises Let us consider the following pairs of compound and the respective melting and boiling point data a. b. c. d. • NO2 and NO H2O and H2S O2 and O3 CH4 and SiH4 Which difference in meting point and boiling points are best explained by: dispersion force effects only? dipole interactions only? H-bonding only? a combination of effects? Other Physical Properties Physical Properties arising from intermolecular interactions In some of the previous discussions we learned how dispersion forces determine the melting and boiling point of many compounds. • The presence of a strong dipole, H-bonds and ions will enhance or decrease the effects of dispersion forces • H-bonds contribute greatly to the “adhesivness” of intermolecular interactions, particularly in mixtures containing compounds capable of forming H-bonds between each other • Reactions Types Mechanisms Bonding Bond types Intermolecular Interactions Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Physical Properties arising from intermolecular interactions • Other physical properties affected by intermolecular bonds are solubility surface tension and flash point viscosity and fluidity density elasticity and plasticity torsional and tensor strength, etc. • The shape and geometry of a compound plays also a very important role in • melting/fusion point viscosity and fluidity density The size of the particles play a very important role in solubility viscosity and fluidity Reactions Types Mechanisms Bonding Bond types Intermolecular Interactions Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Physical Properties Solubility • • • • • Solubility is a physical property that arises from the intermolecular interactions between at least two different substances. Solutions are considered homogenous mixtures made of a solute that dissolves in a solvent. Solutes can be gases, liquids, or solids. Solvents can also be gases, liquids or solids. Most solutions encountered are made of a solid or liquid solute dissolved in water which functions as a solvent. Reactions Types Mechanisms Bonding Bond types Intermolecular Interactions Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Physical Properties Solubility Substances that are not soluble or partially soluble will form two separate “phases”; e.g. air and water • The space where the two phases meet is known as the “interphase”. This is a realm with unique physical properties important in chemical reactions and intermolecular interactions. • “Miscible” is an other term used to denote the fact that a substance mixes with an other to form a solution; • its is normally used in the context of liquids or gases mixing with a liquid solvent phase. e.g. ethanol is miscible in water. or to indicate only partial solubility Reactions Types Mechanisms Bonding Bond types Intermolecular Interactions Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Physical Properties expressing the extent of solubility of substances • • • The solubility of solids is measured most often in terms of the number of grams of solute that dissolve at a given temperature (usually 25EC) in a fix volume of solution (usually 100mL). The solubility of gases is measured in terms of the mL of gas dissolved in a liter of solution. The most commonly referred solubility is with respect to water, however, many compounds are not soluble in water and their solubility is assessed with respect to other solvents. Reactions Types Mechanisms Bonding Bond types Intermolecular Interactions Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Physical Properties general description of solubility in terms of vapourization, mixing and ionization energies • • Solubilization of a molecular solute in a molecular solvent can be considered to be equivalent as the dispersion of the solute’s molecules among the solvent’s molecules. To disperse the solute’s molecules one would need to apply energy to break the intermolecular forces holding the solute in its original solid or liquid state. • Energy of fusion and/or vapourization For the molecules of solute to inter-disperse in the solvent requires for at least some of the solvent’s molecules to break their intermolecular interactions. It is easiest to consider the complete vapourization of the solvent. Energy of fusion and/or vapourization Reactions Types Mechanisms Bonding Bond types Intermolecular Interactions Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Physical Properties general description of solubility in terms of vapourization, mixing and ionization energies • • If all the molecules are now in a “gaseous state” they can mix Once mixed a release of energy would bring the mixture back to a liquid or a solid state. • As well as, it would establish new intermolecular bonding between solute and solvent molecules. This interactions for a soluble solute would normally release energy • Energy of condensation or fusion (-ÄE) Energy of solvation (-ÄE) The net process can result in a net amount of energy being released (exothermic process) or some energy being still needed to form the mixture (endothermic process. Net Energy of mixing Reactions Types Mechanisms Bonding Bond types Intermolecular Interactions Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Physical Properties general description of solubility in terms of vapourization, mixing and ionization energies Reactions Types Mechanisms Bonding Bond types Intermolecular Interactions Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Physical Properties general description of solubility in terms of vapourization, mixing and ionization energies • • Solubilization of an ionic solute in a molecular solvent can be considered to be equivalent as the dispersion of the solute’s cathions and anions among the solvent’s molecules. To disperse the solute’s ions one would need to apply energy to break the intermolecular forces holding the ions together in its original solid state. • Energy of ionic dissociation For the molecules of solute to inter-disperse in the solvent requires for at least some of the solvent’s molecules to break their intermolecular interactions. It is easiest to consider the complete vapourization of the solvent. Energy of fusion and/or vapourization Reactions Types Mechanisms Bonding Bond types Intermolecular Interactions Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Physical Properties general description of solubility in terms of vapourization, mixing and ionization energies • • If all the solvent molecules are now in a “gaseous state” and all the ions are separated they can mix Once mixed a release of energy would bring the mixture back to a liquid or a solid state. • As well as, it would establish ion- dipole or ion - induce dipole interaction between the ions and solvent molecules. This interactions for a soluble ionic compound would normally release energy • Energy of condensation or fusion (-ÄE) for the solvent Energy of ion solvation (-ÄE) The net process can result in a net amount of energy being released (exothermic process) or some energy being still needed to form the mixture (endothermic process). Net Reactions Types Mechanisms Bond types Energy of mixing Bonding Intermolecular Interactions Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Physical Properties general description of solubility in terms of vapourization, mixing and ionization energies Reactions Types Mechanisms Bonding Bond types Intermolecular Interactions Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Physical Properties effect of temperature on solubility • • Different compounds and substances show different solubility behaviours in water. Some of these behaviours can be generalized Reactions Types Mechanisms Bonding Bond types Intermolecular Interactions Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Physical Properties effect of temperature on solubility • The solubility of sucrose and NaCl both increase with increasing temperatures. • The increase of solubility of sucrose is greater than for NaCl. • Analyze the properties of sucrose and NaCl and build a general hypothesis for the solubility of solid compounds in water. Reactions Types Mechanisms Bonding Bond types Intermolecular Interactions Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Physical Properties effect of temperature on solubility • The solubility of Ammonia, Oxygen and Carbon Dioxide decreases with temperature, roughly to the same extent. Reactions Types Mechanisms Bonding Bond types Intermolecular Interactions Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Physical Properties solubility of solids in water solubility of gases in water • Hypothesis #1: The solubility of all solids in water increases with the temperature of the solution • Hypothesis #2: The solubility of ionic solids is only slightly affected by temperature • Hypothesis #3: The solubility of polar molecular compounds is greatly affected by temperature • Hypothesis # 4: The solubility of both nonpolar and polar gases in water decreases with temperature to a similar % Reactions Types Mechanisms Bonding Bond types Intermolecular Interactions Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Physical Properties testing the hypotheses using published solubility data • • Use the table of solubilities provided in the back of your table of elements and Collect the temperature solubility data for as many of the above compounds using the CRC Handbook of Chemistry & Physics (library) Reactions Types Mechanisms Bonding Bond types Intermolecular Interactions Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Physical Properties testing the hypotheses using published solubility data • • Plot the data to produce a graph similar to the one on the right and test the 4 hypotheses. Collect data for 25EC and group them according to periodic trends and cathion and anion group trends Reactions Types Mechanisms Bonding Bond types Intermolecular Interactions Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Physical Properties general qualitative behaviour of different substances in water solutions • • • Most gases will have a reduced solubility in water with increasing temperatures. When a substance is considered insoluble in water it means that their solubility is very very low , sometimes below detection levels. All substances are miscible with each other to some extent. Only when that extent is significant for our purposes we say that the substance is soluble In general substances are miscible if their intermolecular forces are similar in nature. “Similar dissolves similar”. Reactions Types Mechanisms Bonding Bond types Intermolecular Interactions Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Physical Properties general qualitative behaviour of different substances in water solutions • Nearly all solids will have their solubility in water increased by increasing the temperature of the solution. • The solubility of polar molecular compounds, nitrates, and bases are the most significantly affected by the temperature of the solution. • All nitrates are soluble • Most polyvalent cathion oxide/hydroxides are slightly soluble or insoluble. • The solubility of salts is less affected by temperature, but is affected by • the type of metal cathion-anion combination. • Most monovalent or polyvalent cathion salts bonded to halogens are soluble. • Most polyvalent cathion salts bonded to polyatomic anions are insoluble • Most monovalent cathion salts bonded to polyatomic anions are soluble • the relative size of the alkaline metal cathion • smaller cathions are more soluble than larger ones (Li>Na>K). • the relative size of the halogen anion • smaller anions are less soluble than larger ones (F<Cl<Br<I). Reactions Types Mechanisms Bonding Bond types Intermolecular Interactions Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Physical Properties saturated solutions • As we learned in previous slides, a solid will display an increase solubility as the temperature of the solution increases. • At any given temperature only so much solute can be dissolved in the water. We say that the solution is saturated for that given temperature. It is important to check the saturation concentration of a given solute at a given temperature before preparing solutions. • This phenomenon will, however, reach a limit after which no further increase in temperature will dissolve any more of the solid. • If a saturated solution is allowed to cool to a lower temperature, usually room temperature (~25EC), the excess solute will precipitate out of solution forming a super-saturated solution. this behaviour is used to purify substances by crystallization Reactions Types Mechanisms Bonding Bond types Intermolecular Interactions Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006 Physical Properties solutions applications • • Isolating a substance by crystallization of saturated solutions Isolating and purifying molecular compounds based on their different solubilities and adhesion properties in a liquid, gaseous or solid phase system chromatography electrophoresis Reactions Types Mechanisms Bonding Bond types Intermolecular Interactions Physical properties Bond properties Types of Compounds Dr. Pedro M. Pereyra ©) 2006