Measuring fluid-fluid interfacial curvatures using x

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2012
Measuring fluid-fluid interfacial curvatures using x-ray
microtomography
R.T. Armstrong1, M.L. Porter2 and D. Wildenschild
1
School of Chemical, Biological, and Environmental Engineering, Oregon State University,
Corvallis, OR, USA
2
Los Alamos National Laboratory, Earth and Environmental Sciences Division, Los Alamos,
NM, USA
ABSTRACT:
Synchrotron-based tomographic datasets of oil-water drainage and imbibition cycles have been
analyzed to quantify phase saturations and interfacial curvature, as well as, connected and
disconnected fluid configurations. This allows for close observation of the drainage and
imbibition processes, assessment of equilibrium states, and studying the effects of fluid phase
disconnection and reconnection on the resulting capillary pressures and interfacial curvatures.
Based on this analysis, estimates of capillary pressure (Pc) calculated from interfacial curvature
can be compared to Pc measured externally with a transducer. Results show good agreement
between curvature-based and transducer-based measurements, when connected phase
interfaces are considered. Curvature measurements show a strong dependence on whether an
interface is formed by connected or disconnected fluid and the time allowed for equilibration.
The favorable agreement between curvature-based and transducer-based Pc measurements
shows promise for the use of image-based estimates of Pc for interfaces that cannot be probed
with external transducers, as well as opportunities for a detailed assessment of interfacial
curvature during drainage and imbibition.
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