Design of Nuclear Reactor Protection Systems

Design of Nuclear Reactor Protection Systems:

Lessons from Fukushima

by

Christopher Michael Fennell Petty

An Engineering Project Submitted to the Graduate

Faculty of Rensselaer Polytechnic Institute in Partial Fulfillment of the

Requirements for the degree of

MASTER OF ENGINEERING IN MECHANICAL ENGINEERING

Approved:

_________________________________________

Dr. Ernesto Guitierrez-Miravete, Project Adviser

Rensselaer Polytechnic Institute

Hartford, Connecticut

May 2012

© Copyright 2012 by

Christopher Petty

All Rights Reserved ii

CONTENTS

Design of Nuclear Reactor Protection Systems: Lessons from Fukushima ....................... i

LIST OF TABLES ............................................................................................................. v

LIST OF FIGURES .......................................................................................................... vi

LIST OF EQUATIONS ................................................................................................... vii

LIST OF EXAMPLES .................................................................................................... viii

NOMENCLATURE ......................................................................................................... ix

GLOSSARY .................................................................................................................... xii

ACKNOWLEDGMENT ................................................................................................ xiv

ABSTRACT .................................................................................................................... xv

1.

Introduction / Background ........................................................................................... 1

1.1

Nuclear Physics .................................................................................................. 2

1.1.1

Elements & Isotopes .............................................................................. 2

1.1.2

Mass Defect & Binding Energy ............................................................. 2

1.1.3

Nuclear Force ......................................................................................... 4

1.1.4

Coulomb Force ....................................................................................... 4

1.1.5

Nuclear Stability..................................................................................... 5

1.2

Uranium.............................................................................................................. 8

1.3

Nuclear Reactions .............................................................................................. 9

1.3.1

Fission .................................................................................................... 9

1.3.2

Moderation ........................................................................................... 10

1.3.3

Fission Energy Release ........................................................................ 12

1.3.4

Reactor Coolant .................................................................................... 16

2.

Theory / Methodology ............................................................................................... 17

2.1

Nuclear Reactors .............................................................................................. 17

2.2

Boiling Water Reactors .................................................................................... 17

2.3

Pressurized Water Reactors.............................................................................. 23 iii

2.4

Nuclear Reactor Protection Systems ................................................................ 29

2.4.1

Pressure Protection ............................................................................... 29

2.4.2

Thermal Protection ............................................................................... 32

2.5

2011 Japan Catastrophic Earthquake and Tsunami ......................................... 35

2.5.1

Fukushima Daiichi Nuclear Power Plant Accident .............................. 35

2.5.2

Pressure Protection System Failure ...................................................... 35

2.5.3

Thermal Protection System Failure ...................................................... 37

3.

Discussion .................................................................................................................. 38

3.1

Pressure Relief Valves ..................................................................................... 38

3.1.1

Pilot-Actuated Pressure Relief Valves Description ............................. 38

3.1.2

Pressure Relief Valve Size Determination ........................................... 41

3.1.3

Pressure Relief Valves Setpoint Determination ................................... 41

3.2

Operational Power History & Decay Heat ....................................................... 45

3.2.1

Operational Power History ................................................................... 45

3.2.2

Radioactive Decay ............................................................................... 45

3.2.3

Decay Heat Generation ........................................................................ 46

3.2.4

Decay Heat Calculation........................................................................ 48

3.2.5

Decay Heat Removal............................................................................ 56

3.3

Passive Decay Heat Removal........................................................................... 57

3.3.1

Natural Circulation ............................................................................... 58

4.

Conclusions................................................................................................................ 60

5.

References .................................................................................................................. 61 iv

LIST OF TABLES

Table 1 - Calculated Binding Energies ............................................................................ 13

Table 2 - Fission Radiation and Released Particles ......................................................... 14

Table 3 - Average Energy from Uranium-235 Fission .................................................... 15

Table 4 - Relief Valve Setpoint Calculation .................................................................... 44

Table 5 - Coefficients for thermal fission of U

235

, Pu

239

, Pu

241

and fast fission of U

238

.. 52

Table 6 - Power Fractions for Fission of U

235

, Pu

239

, U

238 and Pu

241

............................... 52

Table 7 - Calculated Decay Heat versus Time ................................................................ 54 v

LIST OF FIGURES

Figure 1-1- Proton to Neutron Ratio .................................................................................. 5

Figure 1-2 - Binding Energy per Nucleon versus Mass Number ...................................... 6

Figure 1-3 - Nuclear Fission .............................................................................................. 9

Figure 1-4 - Neutron Cross-Sections for Fission of Uranium and Plutonium ................. 12

Figure 2-1 - Boiling Water Reactor Systems Overview .................................................. 18

Figure 2-2 - Main Steam System Overview .................................................................... 20

Figure 2-3 - Typical Main Steam Isolation Valve ........................................................... 20

Figure 2-4 - Internals of a BWR Reactor Vessel ............................................................. 22

Figure 2-5 - Pressurized Water Reactor Systems Overview ........................................... 24

Figure 2-6 - Internals of a PWR Reactor Vessel ............................................................. 28

Figure 2-7 - Typical Pressure Relief Valve ..................................................................... 30

Figure 2-8 - PWR Primary Relief System ....................................................................... 31

Figure 2-9 - PWR Secondary Relief System ................................................................... 31

Figure 2-10 - BWR Emergency Core Cooling System ................................................... 32

Figure 2-11 - Fukushima Containment Buildings for Reactor Units 1 - 4 ...................... 36

Figure 3-1- Unitized Pilot Relief Valve ........................................................................... 40

Figure 3-2 - Separated Pilot Relief Valve ........................................................................ 40

Figure 3-3 - Uranium 238 Radioactive Decay Chain ...................................................... 46

Figure 3-4 - Overview Calculated Decay Heat Versus Time .......................................... 55

Figure 3-5 - Residual Heat Removal System .................................................................. 56 vi

LIST OF EQUATIONS

Equation [1] – Mass Defect ............................................................................................... 3

Equation [2] – Coulomb’s Force

1

...................................................................................... 4

Equation [3] – Change of Binding Energy ...................................................................... 13

Equation [4] – Theoretical Decay Heat ........................................................................... 46

Equation [5] – Fissions Per Second ................................................................................. 47

Equation [6] – Decay Heat .............................................................................................. 47

Equation [7] – Immediate Rector Heat Production Rate

2

................................................ 48

Equation [8] – Reactor Decay Heat Production Rate ...................................................... 49

Equation [9] – Combination of Equations 7 & 8 ............................................................. 49

Equation [10] – Decay Heat Production Rate Over Time

3

.............................................. 50

Equation [11] – Decay Heat Production Rate at Time Zero ............................................ 50

Equation [12] – Time Dependant Decay Heat Concentration at Equilibrium

4

............... 50

Equation [13] – Total Decay Heat Rate ........................................................................... 51

Equation [14] – Total Decay Heat Rate at Equilibrium .................................................. 51

Equation [15] – Final Decay Heat Production Rate ........................................................ 51

Equation [16] – Decay Heat Production Rate with ANSI/ANS-5.1-2005 Substitutions

5

51

1

http://en.wikipedia.org/wiki/Coulomb%27s_law

2

Glasstone. Page 119.

3

Nichols. Page 69.

4

Ibid.

5

ANSI/ANS-5.12005. Pages 20 – 21. vii

LIST OF EXAMPLES

Example 1 - Mass Defect of Uranium-235.................................................................2

Example 2 - Binding Energy of Uranium-235............................................................3

Example 3 - Amount of Energy Released during Fission of Uranium-235...............13

Example 4 - Theoretical Average Decay Heat...........................................................46

Example 5 - Fissions per Second Calculation…………………………….………...47

Example 6 - Decay Heat of 7% Power.......................................................................47 viii

σ a

ABWR

α

AC

ASME

υ

A amu

Z

T c

T h

T ave

β -

β +

BE

BWR

BTU

N i

UTC

F

λ i

Q

ୈୌ

Q

ୈୌ

,

େ୦ୟ୧୬ୱ

DHR

DOE

ECCS

E

ε

NOMENCLATURE

absorption microscopic cross section advanced boiling water reactor alpha particle alternating current

American Society of Mechanical Engineers antineutrino atomic mass number (number of nucleons) atomic mass units atomic number (number of protons) average cold leg primary coolant temperature average hot leg primary coolant temperature average overall primary coolant temperature beta-minus (electron) decay beta-plus (positron) decay binding energy boiling water reactor

British Thermal Units concentration of the fission products (nuclei/cm

3

)

Coordinated Universal Time

Coulomb Force decay constant (sec

-1

) decay heat production rate decay heat production rate from the fission products

(energy/time-cm

3

) decay heat removal

Department of Energy emergency core cooling system

Energy fast fission factor (~0.32 typically) ix

fm

σ f

γ i

F

GE

I

E

Q

୍ୌ

JST kW-hr

ଶଷହ

்ு m

∆ m m e m atom m n m p

MeV

MWe

MWt

υ

NRC

N/S

PDHR q

1 q

2

PSI

PWR

k e

RCIC

V c

P femtometer (1.0x10

-15

meters) fission microscopic cross section fission yield of the fission products (nuclei/fission) fissions

General Electric immediate energy released per fission, 185.6 MeV immediate heat production rate

Japan Standard Time

Kilo-Watt Hour macroscopic thermal fission cross section for uranium-235 (cm

-1

) mass mass defect (amu) mass of electron (0.000548597 amu) mass of nuclide (amu) mass of nuetron (1.008665 amu) mass of proton (1.007277 amu)

Mega-Electron Volt

Mega-Watt Electric (MWt * 0.33 = MWe)

Mega-Watt Thermal neutrino

Nuclear Regulatory Commission

Nuclear Ship, commercial ship’s propulsion plant designator passive decay heat removal point charge 1 point charge 2 pounds per square inch pressurized water reactor proportionality constant reactor core isolation cooling reactor core volume (cm

3

) reactor power (MWt) x

RPI

RHRS

σ s

r

c

φ

2 t f t s

Q

ୖଡ଼

E

D,Chains

V

Rensselaer Polytechnic Institute residual heat removal system scattering microscopic cross section separation distance speed of light thermal neutron flux (neutrons/cm

2

-sec) time at constant fission rate (forming time) time after shutdown total reactor heat production rate useable energy released by each decay of a fission product decay chain (energy/decay) volume xi

GLOSSARY

Advanced Boiling Water Reactor (ABWR): is a newer design boiling water reactor.

Usually applied to boiling water reactors designed after 1980.

Boiling Water Reactor (BWR): is a type of light water nuclear reactor used for the generation of electrical power. In a boiling water reactor, the reactor heats water which turns to steam and then drives a steam turbine.

Decay Heat: is the heat released as a result of radioactive decay.

Department of Energy (DOE): is a Cabinet-level department of the United States government concerned with the United States' policies regarding energy and safety in handling nuclear material.

Emergency Core Cooling (ECCS): is a series of systems that are designed to safely shut down a nuclear reactor during accident conditions.

Japan Standard Time (JST): is the standard time zone of Japan, and is 9 hours ahead of

Coordinated Universal Time (UTC).

Nuclear Regulatory Commission (NRC): is an independent agency of the United States government that was established by the Energy Reorganization Act of 1974 from the

United States Atomic Energy Commission, and was first opened January 19, 1975. The

NRC oversees reactor safety and security, reactor licensing and renewal, radioactive material safety, and spent fuel management (storage, security, recycling, and disposal).

Passive Decay Heat Removal (PDHR): is a process to removal decay heat without pumps, power or other support systems. xii

Pressurized Water Reactor (PWR): is a type of light water nuclear reactor used for the generation of electrical power. In a pressurized water reactor, the reactor heats highly pressurized water (primary water) which in turn transfers the heat to an isolated water loop (secondary water). The secondary water is boiled off during the heat transfer process to create steam and then drive a steam turbine.

Reactor Core Isolation Cooling (RCIC): is a reactor safety system that can inject high pressure water into a reactor.

Radioactive Decay: is the process by which an atomic nucleus of an unstable atom loses energy by emitting ionizing particles.

Residual Heat Removal System (RHRS): is a system used to remove decay heat during a normal shutdown of the reactor.

SCRAM: is an operation that shuts down a nuclear reactor. In a reactor, a SCRAM is achieved by a large insertion of negative reactivity by insertion of the control rods. xiii

ACKNOWLEDGMENT

The author would like to thank his family, especially his wife Kristen, who has been so supportive throughout the entire Masters of Engineering in Mechanical Engineering curriculum. He would also like to thank the faculty of Rensselaer Polytechnic Institute in Hartford and Groton, for sharing their experience and expertise throughout the curriculum. xiv

ABSTRACT

Economic instability in today's world markets have caused the price of traditional fuel commodities, e.g. crude oil and coal, to rise to record levels. This sharp increase in fuel prices has forced the general public to demand cheaper power generation alternatives.

Construction of nuclear power plants would alleviate these cost burdens; however in the light of the crises at: Fukushima, Chernobyl and Three Mile Island, the general public is concerned about the safety of these plants near their homes and businesses. Despite recent disasters, nuclear power has the potential to be a safe and reliable way to produce electrical energy.

These catastrophes have shown the need for robust and reliable reactor protection systems. Complex reactor protection systems are designed to shutdown and cool down an operating nuclear reactor in an emergency, to protect the integrity of the reactor containment. The two most important protection issues are system over pressurization and fuel element overheating. Reactor protection equipment, such as pressure relief valves, prevent catastrophic destruction of vital reactor systems by relieving pressure buildup. Other reactor protection systems, such as passive decay heat removal, prevent the reactor fuel elements from overheating during the weeks and months of decay heat generation after the reactor is shutdown. This engineering project evaluates these protection systems by: determining the heat load required to be removed by the cooling systems through decay heat calculation, determining the layout of the cooling systems to promote passive decay heat removal flow modes, and determining the appropriate relief valve setpoints of the over pressure protection systems. The analyses of these systems will include an examination of the lessons learned from the events at the Fukushima

Daiichi nuclear power station in Japan. xv

1.

Introduction / Background

Recent catastrophic events at the Fukushima Daiichi nuclear power station in Japan have reemphasized the importance of reliable reactor protection systems. The failure of these systems, caused by two beyond-design-basis events (i.e., earthquake, tsunami), has increased awareness in the general public regarding the safety of nuclear power plants around the world. In light of recent disasters, public opinion of nuclear power is that it is not safe. In reality, complex safety systems are integrated into every reactor design.

Regulatory committees provide specific criteria for the design of the reactor protection systems to protect against failure for a series of potential, realistic causalities. Design agencies use these criteria to develop methodologies for implementing reactor safety into their plant designs. This project evaluates one methodology for designing the reactor protection systems required for a 1600 MWe Boiling Water Reactor nuclear power plant.

There are three major factors in overall reactor safety: 1. the capability of cooling systems to remove heat generated during decay of fission daughter products (commonly known as decay heat removal), 2. the capability of protection systems to relieve high pressure before a catastrophic failure occurs and 3. redundancy of these safety systems.

The objective of this study was to review how the three major factors in reactor safety failed in the catastrophic events at the Fukushima Daiichi nuclear power station in

Japan, as well as, reviewing lessons learned to design more robust reactor protection systems in future nuclear power plants. This report describes design strategies for safer nuclear power operations and reactor casualty minimization. This report is organized in the following way: 1. an overview of nuclear power and nuclear plant designs, 2. an overview of the Fukushima Daiichi nuclear power disaster, 3. an updated approach to calculations used in determining the: operational power history, decay heat generation, and pressure relief valve setpoints, and 4. an analytical analysis of the results, utilizing lessons learned from the Fuskushima Daiichi disaster, to properly size and locate the reactor protection systems within a reactor plant design.

1

1.1

Nuclear Physics

A review of basic principles of nuclear physics is presented. For further details see details presented in USNRC Technical Training Center’s Reactor Concepts Manual.

Nuclear power is an unique way to produce heat and thus steam used in turbine generators to produce electricity. Nuclear power generation is possible because of special properties of the nucleus of certain elements.

1.1.1

Elements & Isotopes

All elements, on the periodic table, are described and differentiated by the number of protons (atomic number) contained within the nucleus of the element (e.g.,

Hydrogen (1 proton), Carbon (6 protons), Uranium (92 protons)). The nucleus of an element will always contain the same number of protons, but may contain a different number of neutrons. Nuclei that are related in this way are called isotopes (e.g.,

Uranium-235 (92 protons, 143 neutrons), Uranium-236 (92 protons, 144 neutrons),

Uranium-238 (92 protons, 146 neutrons)).

1.1.2

Mass Defect & Binding Energy

When examining an isotope, the atomic mass of the isotope never exactly matches the combined masses of the proton(s) and neutron(s). This difference is called the mass defect. The mass defect is defined as the missing mass in an isotope. See

Example 1 for the mass defect of uranium-235.

2

Example 1 - Mass Defect of Uranium-235

= ∆ =

+

+ −

− where:

∆ m = mass defect (amu)

௔௧௢௠

6

[ 1] m p

= m e

= m n

= m atom

=

Z =

A = mass of proton (1.007277 amu) mass of electron (0.000548597 amu) mass of neutron (1.008665 amu) mass of nuclide for U

235

(235.043924 amu) atomic number (number of protons = 92) mass number (number of nucleons = 235)

∆ = 92 1.007277 + 0.000548597

+ 235 − 92 1.008665

− 235.043924

∆ = 1.915125

In classical physics, mass defect is not possible, however this phenomenon is explained through the conservation of energy and Albert Einstein's mass-energy equivalence equation =

. The lost mass of the nucleus is converted to energy (commonly referred to as Binding Energy) when the isotope is formed.

Therefore, binding energy (BE) represents the amount of energy required to split the nucleus of an atom. See Example 2 for the binding energy for uranium-235.

Example 2 - Binding Energy of Uranium-235

From example 1, the mass defect of uranium-235 is 1.915125 amu.

∆ = 1.915125

Since 1 amu = 931.5 MeV

= = ∆

931.5

!

"

= 1.915125 ∗ 931.5

= 1783.94

!

6

Department of Energy. www.ne.doe.gov/

3

1.1.3

Nuclear Force

Certain elements have a stable nucleus because of the presence of the nuclear force. In the nucleus of an isotope, there is a collection of closely packed protons and neutrons. The protons (with like charges), in close proximity to each other, exert large repulsive electrostatic forces. This repulsion should cause the nucleus to fly apart.

However, the nuclear force, at short distances, and allows the nuclei to remain intact.

The nuclear force is defined as the interaction force that holds the nucleons in a nucleus together.

The nuclear force is powerfully attractive between nucleons at distances between

1 and 2 femtometers (fm) (1.0 x 10

−15

meters and 2.0 x 10

−15

meters), but rapidly decreases to insignificance at distances beyond about 2.5 fm. At very short distances of less than 0.7 fm, the nuclear force becomes repulsive, and is therefore responsible for the physical size of nuclei. This phenomenon results in a minimum separation distance between the nucleons.

1.1.4

Coulomb Force

The protons in a nucleus attach to each other via the nuclear force, and at the same time they repel each other with a large repulsive electrostatic force, the Coulomb force. The Coulomb force is governed by Coulomb's law. Coulomb's law is a law of physics describing the electrostatic interaction between electrically charged particles.

The law states that electrical charges of the same sign have a force that is repulsive; on the other hand, the electrical charges of opposite signs have a force that is attractive.

The magnitude and sign of the electrostatic force between two idealized point charges

(q

1

) and (q

2

), is given by:

#

=

$

࢘ ૛

[2] where:

F k e r q

1 q

2

=

=

=

=

=

Coulomb Force proportionality constant separation distance point charge 1 point charge 2

4

1.1.5

Nuclear Stability

Figure 1-1 is a plot of the number of protons versus the number neutrons, with all stable isotopes high-lighted in the "belt of stability". Note that light nuclei are the most stable if they contain equal numbers of protons and neutrons. Furthermore, heavy nuclei are more stable if the number of neutrons exceeds the number of protons. We can understand this by recognizing that as the number of protons increases, the strength of the Coulomb force increases, which tends to break the nucleus apart. As a result, more neutrons are needed to keep the nucleus stable, since the neutrons experience only attractive nuclear forces. Eventually, the repulsive forces between protons cannot be compensated for by the addition of more neutrons; this occurs when the number of protons ≈ 83. Elements that contain more than 83 protons do not have stable nuclei.

Figure 1-1- Proton to Neutron Ratio

7

7

http://chemed.chem.wisc.edu/chempaths/GenChem-Textbook/Nuclear-Stability-748.html

5

The stability of an isotope can be determined by the summation of all the forces

(binding energy) per nucleon. The total binding energy of an isotope increases as the number of particles in the nucleus increases. However, the rate of the binding energy increase is not uniform with the rate of number of particle increase, resulting in a variation in the amount of binding energy associated with each nucleon within the nucleus. This variation in the binding energy per nucleon (BE/A) is easily seen among different nuclei when the average BE/A is plotted versus atomic mass number (A), as shown in Figure 1-2. It is apparent from Figure 1-2 that the most stable isotope is iron-

56 (Fe

56

). (Located at the top of the curve.)

Figure 1-2 - Binding Energy per Nucleon versus Mass Number 8

8

http://www.euronuclear.org/info/encyclopedia/bindingenergy.htm

6

Because iron-56 is the most stable isotope, other isotopes will undergo radioactive decay to become iron-56; essentially becoming more stable. Isotopes that are larger and heavier than iron-56 will fission to become stable; likewise, isotopes that are smaller and lighter than iron-56 will combine, through fusion, to become more stable. The nuclear force also affects the binding energy of a nucleus and its probability to decay.

For a small isotope (small A), the nuclear radius is small and each of the isotope nucleons can interact strongly with other nucleons. Thus, for light nuclei, the BE/A curve rises rapidly as A increases because the number of interacting nucleon pairs increases. As mentioned earlier, the nuclear force is strong, but has a very short range of effect, therefore as the nucleus grows in size, the nuclear forces holding it together decrease. This is noticeable for heavier nuclei on the BE/A curve where BE/A decreases gradually as the nuclear radius increases. This is because strong bonds can form only between the nearest neighboring nucleons.

As the atomic mass number (A) increases further and the nucleus becomes larger still, a point at which the field of each nucleon cannot reach all the remaining nucleons occurs, and the nuclear force is saturated. The binding energy per nucleon shows little change as more nucleons are added. At this point (A ≈ 70) the nuclear radius corresponds roughly to the range of the nuclear force. If the nuclear force were the only phenomenon acting on the nucleus, the value of BE/A would remain constant at its maximum value as A increases beyond 70. There is another phenomenon, however, which shifts the maximum in the BE/A curve to A ≈ 60 and results in the gentle downward slope observed beyond that value. This effect is a consequence of the

Coulomb force, described in section 1.1.4. As A increases beyond ≈ 60, the mutual repulsion of the protons in the nucleus opposes the attractive nuclear force and tends to destabilize the nucleus. The Coulomb force is a powerful over a larger range than the nuclear force, further destabilizing the nucleus with the addition of more neutrons and protons. The result is a net decrease in binding energy per nucleon beyond A ≈ 60. This fundamental understanding of isotope nucleus formation is the reason heavy isotopes are used for fission.

7

1.2

Uranium

Uranium, a heavy element found abundantly in the earth's crust, is obtained through milling and enrichment. Naturally occurring uranium contains various isotopes; uranium-238, uranium-235 and uranium-234. The majority (99.2745%) of all the atoms in natural uranium are uranium-238. Most of the remaining natural uranium atoms

(0.72%) are uranium-235, and the remainder (0.0055%) uranium-234. Although all isotopes of uranium have similar chemical properties, each isotope's nuclear properties differ significantly. The difference in nuclear properties allows one isotope, uranium-

235, to be useful for thermal fission. To allow a commercial power reactor to operate approximately two years before new fuel is required, the fuel must be enriched.

Enriching the uranium fuel increases the number of uranium-235 atoms in a given volume thus increasing the usefulness of the field.

8

1.3

Nuclear Reactions

1.3.1

Fission

As described in Section 1.2, uranium-235 is used as reactor fuel because of its nuclear properties. Uranium-235 has a high probability of absorbing a thermal (low energy) neutron causing fission. Fission occurs because the arrangement of particles in the nucleus is unstable and allows it to disintegrate easily to become more stable. When the uranium-235 nucleus absorbs a thermal neutron, it becomes uranium-236.

Uranium-236 is not found in nature and is highly unstable, therefore it quickly disintegrates into two or more smaller element isotopes; commonly known as daughter products. See Figure 1-3 for a pictorial description of the fission process. Each time a fission event occurs and the nucleus is split into daughter products, there is a release of two or three neutrons and a substantial amount of energy. The energy released from the fission process is utilized to heat the reactor coolant; while the neutrons released allow the fission chain reaction to continue.

Figure 1-3 - Nuclear Fission

9

The neutrons released by the fission process can be divided into two categories, prompt neutrons and delayed neutrons. Prompt neutrons constitute 99.35 percent of the

9 http://web.mit.edu/nrl/www/reactor/fission_process.htm

9

total neutrons released. They are released within 10

-14

seconds (or less) of the instant of fission.

10

The average lifetime of prompt neutrons is 26 microseconds. Delayed neutrons are expelled from the daughter products over a period of several minutes after fission. The average lifetime of delayed neutrons is between 0.2 seconds and 1 minute.

The presence of delayed neutrons prevents the chain reaction from increasing too rapidly therefore controlling the fission process.

1.3.2

Moderation

In nuclear fission, moderation plays an important role. During each fission process, two to three neutrons can be released with high energy ( ≥ 2 MeV), called fast neutrons. In order for the chain reaction of fission to continue; a released neutron must have the proper energy to be absorbed by another uranium-235 nucleus. Uranium-235 undergoes fission more readily when the neutrons are of low energy, called slow neutrons or thermal neutrons. Thus, for a neutron to be absorbed by uranium-235 it must slow down or reduce its energy. The process of reducing the energy of a neutron to the thermal region (~0.00625 MeV) by elastic scattering is referred to as thermalization or moderation.

The material used for the purpose of thermalizing neutrons is called a moderator.

During the fission process, neutrons are released at different energies depending on when the neutrons are released, prompt versus delayed. Prompt neutrons born during the fission process have energies greater than 0.1 MeV with an average energy of 2 MeV.

These high energies are well above the thermal region and require thermalization to be useful for fission. In contrast, delayed neutron energies are lower than those for the prompt; with the delayed neutron average energy being approximately 0.4 MeV. These higher energy neutrons are thermalized through scattering events where they lose some of their kinetic energy to the surrounding bulk material and coolant.

Elastic and inelastic scattering reactions are the only types of interactions that cause the neutrons to lose energy without removing them from the fission cycle. Of the two types of scattering reactions, elastic scattering collisions are the most important since they occur at all neutron energies.

10

Glasstone. Page 106.

10

The collisions are not possible unless there is an effective moderator in the reactor core. Effective moderators are classified as mediums that create a large energy loss per collision. They have large scattering cross sections, and low absorption cross sections. The maximum energy lost in any single collision increases as the mass of the target nucleus decreases. This means that light nuclei, for example hydrogen, contribute more effectively to the slowing down process and are considered effective moderators.

A practical example is a “pool” ball can transfer all of its energy to another “pool” ball that results in stopping of the first “pool” ball and the movement of the second “pool” ball. However, on the other hand, a “pool” ball will transfer some of its energy to a

“bowling” ball. This energy transfer may occur without visibly moving the “bowling” ball.

Moderation allows a neutron to be useful for fission by "increasing" its absorption cross section. While the physical size of a neutron does not change, the absorption cross section of the nucleus represents its probability to fission, and changes with speed and energy. At fast speeds and high energy, a neutron has a large scattering cross section, σ s

, and a small absorption cross section, σ a

; indicating that the neutron has a higher probability to scatter instead of fission. Likewise, at slow speeds and low energy a neutron has a large absorption cross section and a small scattering cross section; indicating that the neutron has a higher probability to be absorbed and fission.

See Figure 1-4. The absorption cross section decreases faster than the inverse of velocity (1/V) so it is generally smaller than the scattering cross section at fast energies.

The highest probability of neutrons to induce fission events occurs in the thermal energy range where the absorption cross section is the highest.

11

Figure 1-4 - Neutron Cross-Sections for Fission of Uranium and Plutonium

11

1.3.3

Fission Energy Release

As mentioned in section 1.3.2, neutrons can be released from the fission process with high amounts of energy. This energy is proportional to the decrease in mass of the system described in section 1.1.2. The relationship between mass and energy was explained in section 1.1.2. Therefore the amount of energy released as usable energy during the fission process, a conservation of mass-energy equation can be analyzed. The energy released from the system will be equivalent to the difference in binding energy

(BE) between the reactants and the products. See Example 3 for the amount of energy release during a specific fission event.

11

http://world-nuclear.org/education/phys.htm

12

Example 3 - Amount of Energy Released during Fission of Uranium-235

Assumptions: urnaium-235 will fission into Yttrium-98 (

ଽ଼

ଷଽ

%

) and Iodine-135 (

ଵଷହ

ହଷ

ܫ )

+

ଶଷହ

ଽଶ

&

ଶଷ଺

ଽଶ

&

∗ →

ଽ଼

ଷଽ

%

+

ଵଷହ

ହଷ

'

+ 3

Using example 1, we can determine the binding energies:

Table 1 - Calculated Binding Energies

Nuclide

ଶଷହ

ଽଶ

ܷ

Atomic Mass (amu)

235.043924

Binding Energy (MeV)

1783.940

Total Reactants

ଽ଼

ଷଽ

ܻ

ଵଷହ

ହଷ

ܫ

Total Products

97.9222195

134.9100503

1783.940

832.960

1131.993

1964.953

()

= ∆

()

ࡼ࢘࢕ࢊ࢛ࢉ࢚࢙

− ∆

()

ࡾࢋࢇࢉ࢚ࢇ࢔࢚࢙

[3]

∆ =

%

+

ଵଷହ

ହଷ

'

ଶଷହ

ଽଶ

&

∆ = 1964.953 − 1783.940 = 181.013

!

Example 3 demonstrates the amount of prompt energy that is released from uranium-235 when the fission products are yttrium-98 and iodine-135. This example, however, doesn't demonstrate all the energy released during the fission process. Energy in the form radiation and particles are also released. The radiation released during the fission can come in different forms. See Table 2 for the types of radiation and released particles.

13

Table 2 - Fission Radiation and Released Particles 12

Particle

Gamma (Photon)

Beta-minus

(electron)

Beta-plus

(positron)

Neutrino

Antineutrino

Alpha

Radiation

Type

Gamma

Radiation

Beta Decay

Alpha Decay

Symbol

β

β

γ

υ

υ

Α

-

+

*

Notation

*

ିଵ

υ

υ

+

Charge Mass (amu)

0

- 1

+ 1

0

0

+ 2

0

0.000548597

0.000548597

0

0

4.002602

12

Glasstone. Page 330.

14

Taking into consideration the prompt energy, radiation and particle release, the average total amount of energy released per fission of one uranium-235 atom is summarized in

Table 3.

Table 3 - Average Energy from Uranium-235 Fission 13

Emitted Energy

(MeV)

Instantaneous Energy

Kinetic energy of fission fragments 165.6

Kinetic energy of fission neutrons

Fission gamma rays

Neutron capture gamma rays

4.8

7.7

7.5

Total instantaneous energy 185.6

Delayed Energy

Kinetic energy of beta particles 7.2

Delayed neutrons

Fission product decay gamma rays

Antineutrinos

Total delayed energy

~0

7.2

10.2

24.6

Total energy released per fission 210.2

Recoverable Energy

(MeV)

165.6

4.8

7.7

7.5

185.6

7.2

~0

7.2

0

14.4

200.0

13

Glasstone. Page 17.

15

1.3.4

Reactor Coolant

In a nuclear reactor, the reactor coolant also plays an important role. As described in sections 1.3.1 and 1.3.3, the fission process releases thermal energy as part of the energy conservation process. The medium that removes the thermal energy generated during the fission process, in a reactor, is called the reactor coolant. The thermal energy resulting from the fission process establishes a temperature difference between the reactor fuel elements and the circulating reactor coolant. This temperature difference results in a transfer of energy from the fuel elements to the reactor coolant.

Along with the fission thermal energy, most of the kinetic energy in the neutron is transferred directly to the reactor coolant as heat during the thermalization process, described in section 1.3.2. During the thermalization process, neutron elastic collisions with hydrogen nuclei dominate the slowing-down process, along with the inelastic scattering collisions with heavier elements such as zirconium (typically used in fuel element construction). These elastic and inelastic collisions also generate heat that needs to be removed by the reactor coolant. This energy is then used to create steam and ultimately generate electrical power.

16

2.

Theory / Methodology

2.1

Nuclear Reactors

Nuclear power plants currently in operation and under design, in the United States, fall into two main categories: boiling water reactors (BWR) and pressurized water reactors

(PWR). The basic concepts between the two types of plants are similar but the details of the reactor designs of these reactor types vary drastically. These variations account for multiple heat transfer loops as well as designs involving different components.

2.2

Boiling Water Reactors

In the United States, BWRs encompass approximately 33 percent of all commercial nuclear power plants in operation. There are two operating BWR types, an older variation BWRs and advanced boiling water reactors (ABWR). BWRs have been in operation since 1960; with the original BWRs being developed by General Electric (GE) in the 1950s. The first BWR nuclear power station was Dresden Unit-1 (200 MWe) commissioned in July 1960. This first BWR was a dual cycle plant like a PWR, as will be described in section 2.3. However, subsequent designs were modified to adopt a single direct cycle. The Fukushima Daiichi Nuclear Power station had six separate

BWRs.

BWRs utilize light water (normal H

2

0 as opposed to “heavy” water commonly known as deuterium) as the reactor coolant and moderator to generate electricity by directly boiling the light water in a reactor core to make steam that is delivered to a turbine generator to produce electricity. A BWR and ABWR nuclear power plant consists of: a nuclear reactor, a reactor coolant recirculation system, main steam system, condensate system, feed system, turbine equipment, generator equipment and other important secondary systems (e.g., purification, sampling) and equipment. Along with the reactor operational systems, engineered safety features including: pressure protection system, emergency core cooling system, reactor core isolation cooling, containment cooling system and injection system is provided for emergency operations. See Figure

2-1 for a systems overview of a typical BWR.

17

14 http://www.ge-energy.com/

Figure 2-1 - Boiling Water Reactor Systems Overview 14

18

A BWR provides cooling to the reactor and generates steam with utilizing a single loop system called the reactor coolant recirculation system. The reactor coolant recirculation system circulates subcooled water for neutron moderation and for removal of the heat generated in the core. The heat transfer in the reactor core, from the fuel elements to the reactor coolant, generates steam inside the reactor vessel and supplies the steam to the main steam system. The main steam system transports the steam from the reactor vessel to the electrical generation turbines. Once all the steam energy is used the steam is condensed back to liquid. This water is supplied to the condensate and feed systems which direct the water back to the reactor vessel for the heat transfer cycle to be repeated.

The reactor coolant recirculation system is located inside the primary containment and is divided into multiple units; with the exact number depending on the size of the reactor, with a common reactor vessel. The principal components of each unit are a steam separator and reactor coolant recirculation pump(s); typically between two and four units per reactor. Water discharged by the reactor coolant recirculation system passes through the reactor core which heats the water to a mixture of water and steam. The steam-water mixture is discharged by the reactor to risers. The risers convey the steam-water mixture to the steam separators which separate and dry the steam. The steam separators dry the steam, aka increase the quality, and remove residual moisture; which is fed back to the reactor for reuse.

The main steam system transports the dry and saturated steam from the steam separators to the main turbines to produce electrical power, see Figure 2-2 for a detailed main steam system overview. The number of main steam headers depends on size of the reactor; typically between two and five main steam headers per reactor. The main steam system originates at the steam outlets of the steam separator and passes through the primary containment into the turbine building. The system consists of the necessary piping, valves, and instrumentation required to transport steam from the steam separators to the inlet of the main electrical turbines. A set of primary containment isolation valves are located on either side of the containment boundary for isolation of the reactor, see

Figure 2-3. These isolation valves, see Figure 2-3, isolate the reactor and primary containment from the manned spaces in an emergency or during maintenance evolutions.

19

Figure 2-2 - Main Steam System Overview 15

Figure 2-3 - Typical Main Steam Isolation Valve 16

15 http://www.ge-energy.com/

16 Ibid.

20

Once the steam has expelled all of its energy in the turbines, its temperature and pressure are reduced. Spent, low-pressure steam exits the turbines and enters the condenser where it flows over tubes cooled by water. As the remainder of the energy is removed from the steam, by cooling in the turbine condensers, a liquid called condensate is formed. The condensate system then transports the deaerated condensate from the condenser hot well to the reactor feed pumps for return to the reactor coolant recirculation system. Each condensate system, one for each main steam header and turbine generator, consists of condensate pumps connected to the condenser hot well, associated valves and a recirculation line. The condensate pumps increase the pressure of the water to approximately half the required pressure and then discharges it into a common header. The condensate header directs the condensate to the reactor feed system, specifically the reactor feed pump suction header.

The reactor feed system completes the heat transfer cycle by transporting the water from the condensate system back to the reactor vessel. The reactor feed system completes the pressure increase of the water to a pressure that is greater than reactor operating pressure. This water enters the reactor pressure vessel through feed nozzles high on the vessel, well above the top of the fuel assemblies but below the water level to prevent splashing and causing a thermal shock on the feed nozzle piping. The feed water is pumped into the reactor pressure vessel after going through feed water heaters to raise its temperature; so the reactor vessel is not thermally shocked by "cold" feed water. Without these heaters and proper feed piping placement, the shock to the system could cause brittle fracture cracks and/or failures. The feed water enters the reactor vessel in the downcomer region and combines with excess water exiting the steam separators. The feed water then flows down the downcomer region and goes through either jet pumps or reactor coolant pumps that provide additional pumping power. The water, now called reactor coolant again, makes a 180 degree turn and moves up through the lower core plate into the core where the fuel elements heat the water and restart the process. See Figure 2–4 for the internals of BWR reactor vessel.

21

Figure 2-4 - Internals of a BWR Reactor Vessel

17

17

http://www.euronuclear.org/e-news/e-news-18/HP-BWR.htm

22

2.3

Pressurized Water Reactors

In the United States, pressurized water reactors (PWR) encompass the majority of commercial nuclear power plants. A PWR is considerably different than a BWR in its heat transfer and steam generation location details. These details add complexity through multiple loops and components. In the US, PWRs were originally designed at the Oak Ridge National Laboratory for use as a nuclear submarine power plant. The remaining designs were conducted by Westinghouse's Bettis Atomic Power Laboratory.

The first purely commercial nuclear power plant was a PWR built at Shippingport

Atomic Power Station and went critical on December 2, 1957.

A PWR is fundamentally different than a BWR because a PWR is designed to preclude boiling in the reactor vessel. In a PWR heat is removed from the reactor and steam is generated utilizing a two loop system configuration, called the primary and secondary loops; see Figure 2-5. The primary loop system removes the heat generated by the fission process by circulating reactor coolant and transfers that thermal energy to the secondary loop; via the steam generator. The purpose of the secondary loop system is to: "cool" the primary loop, generate steam, transport the steam to the turbine generators and resupply makeup water to the steam generator. The steam generated in the steam generator is transported to the main turbine building to rotate the main electrical turbines and generate electricity. Once all the steam energy is expelled, the steam is condensed. The condensed water is fed to the condensate and feed systems to raise the water's pressure and direct it back to the steam generator for the heat transfer cycle to repeat.

The primary system is a pressurized, enclosed loop that removes heat from the reactor core and prevents boiling in the reactor vessel. The primary system in a PWR is maintained at high temperatures ( ≥ 400°F) and high pressure ( ≥ 1500 psia). Boiling in the primary system is prevented because heat generated from fission in the reactor fuel could cause excessive temperatures and distorting or melting of core components if not properly removed. These problems would occur due to the steam heat transfer properties being less effective than liquid water heat transfer properties. The primary system obtains its required operating pressure by electrically heating a tank of water, the

23

Figure 2-5 - Pressurized Water Reactor Systems Overview

18

18 http://aboutnuclearphysics.blogspot.com/2010_07_01_archive.html

24

pressurizer, and raising the temperature of the water in the pressurizer to the saturation temperature corresponding to the desired primary system pressure. The pressurizer's temperature is maintained well above reactor coolant temperatures in the reactor so that boiling occurs in the pressurizer and not in the reactor core.

Reactor coolant is continuously circulated in the primary system loop which connects the reactor to the steam generator and the steam generator back to the reactor.

"Hot" reactor coolant leaves the reactor, and flows through the hot-leg piping of the primary loop and enters the steam generator. Inside the steam generator, the reactor coolant transfers its heat energy to the secondary loop for steam generation. "Cold" reactor coolant leaving the steam generator, due to the heat energy transfer, flows through the cold-leg piping and pump(s) of the primary loop and reenters the reactor vessel, completing the primary heat cycle. The primary system has a temperature difference of only approximately 50°F (375°F - 425°F) if the average reactor coolant temperature is 400°F. This constitutes the "hot" leg having a temperature of 425°F reactor coolant and the "cold" leg having a temperature of 375°F reactor coolant; for this example. If the reactor coolant flow rate is reduced or lost and/or reactor coolant liquid volume is lost, heat generated in, but not removed from the reactor, could result in excessive temperatures and ultimately damage to the reactor fuel elements.

A main aspect to the primary system is the reactor coolant pressurizing system.

The reactor coolant pressurizing system serves two main purposes: 1. to develop and maintain the reactor coolant system pressure during operation and 2. to provide a means of removing non-condensable gases from the primary system so that gas concentrations are kept within specifications. Although inherent self-regulation of the reactor tends to keep the average reactor coolant temperature (T ave

) constant, the cold-leg temperature

(T c

), and the hot-leg temperature (T h

) vary during steam demand transients. These temperature changes affect the density and, hence, the volume of the primary system.

Changes in reactor coolant volume, in turn, produce pressure changes in a closed system.

The pressurizing system handles these volume changes without requiring the reactor coolant system to have water added or removed; all while maintaining the system pressure below the maximum design pressure.

25

The secondary system cycle consists of: the steam generator, a main turbine, a condenser, a condensate pump, a feed pump, feed heaters and associated piping and valves. Heat transferred from the reactor coolant to the secondary fluid generates highpressure and low-quality steam. After the steam generator dries the steam, the secondary system directs the high-pressure high-quality steam that exits the steam generator to the main turbine generators where the steam's potential energy is changed to kinetic energy through turbine work. As steam completes work in the turbines, its temperature and pressure are reduced. Spent, low-pressure steam exits the turbines and enters the condenser where it flows over tubes cooled by water. As the remainder of the energy is removed from the steam, by cooling in the turbine condensers, a liquid called condensate is formed. To complete the secondary cycle, this condensate is returned to the steam generator by the combined pressure addition of the condensate and feed pumps. The condensate pump is designed to operate with a low suction pressure such as that in the condenser, and protects the feed pump from damage due to cavitation by providing sufficient pressure at the inlet to the feed pump. The feed pump completes the heat transfer cycle by increasing the pressure of the secondary coolant above the steam generator operating pressure and returning the fluid to the steam generator for reuse.

The primary purpose of the steam generating system is to transfer heat from the reactor coolant to secondary water. The region above the tube sheet and outside the Utubes in the generator is the secondary side. In this region, heat is transferred through the U-tubes from the reactor coolant to the secondary water. The combined action of heat transferred from the reactor coolant and the colder water returned by the feed system establishes an internal circulation of secondary water.

As secondary water is heated by the U-tubes, its temperature increases, its density decreases, and it rises up through the tube bundle region. When its temperature reaches saturation temperature, it begins to boil, forming a mixture of steam and liquid water. This mixture flows upward into the riser region above the U-tubes. The internal steam generator structure guides the upward-flowing steam-water mixture toward the moisture separators in the upper part of the steam generator. The moisture separators reduce the quality of the steam and permit dry saturated steam to exit the steam

26

generator through the steam nozzle, into the main steam system, while returning saturated liquid to the downcomer region.

The main steam, condensate and feed systems function exactly the same way as the boiling water reactor's main steam, condensate and feed systems perform. The main steam system transports the dry and saturated steam from the steam separators to the main electrical turbines to produce electrical power. The condensate system transports the deaerated condensate from the condenser hot well to the feed pumps. The reactor feed system transports the condensate from the condensate system to the steam generator. The final destination of the feed water is the only difference between the

PWR system (steam generator) and BWR system (reactor vessel).

27

Figure 2-6 - Internals of a PWR Reactor Vessel

19

19

http://www.nrc.gov/reading-rm/basic-ref/teachers/04.pdf

28

2.4

Nuclear Reactor Protection Systems

Robust reactor protection systems are common to both types of nuclear reactor plants. A reactor protection system is a set of nuclear safety components in a nuclear power plant designed to protect and/or safely shutdown the reactor while preventing the release of radioactive materials. In a nuclear power plant, protection systems are broken down into two main categories; pressure protection and thermal protection. The pressure protection systems have the responsibility to protect the reactor and various systems' pressure integrity. The thermal protection systems have the responsibility to keep the reactor fuel elements covered at all times and, when necessary, reduce the temperature of the reactor coolant to a safe and stable temperature.

There are three major factors in overall reactor protection design:

1. Capability of the pressure protection systems to relieve high pressure before a catastrophic failure occurs,

2. Capability of the thermal protection systems to remove heat generated during decay of fission daughter products (commonly known as decay heat removal) and,

3. Redundancy of these safety systems to prevent any single point failures.

These major factors directly affect the design of the nuclear power plants.

2.4.1

Pressure Protection

The purpose of a pressure relief system is to prevent the plant pressure from exceeding the design system pressure. This is accomplished by discharging liquid or steam through a relief valve when the pressure exceeds the relief valve's set pressure.

See Figure 2-7 for a typical nuclear power plant relief valve. The consequences of excessive pressure can include leakage through pressure boundaries in valves, distorting and/or weakening of system components, and in the worst case, rupture of the system's pressure boundary. A rupture of a pressure boundary could potentially release fission products and radioactivity to the primary containment or to the environment in extreme cases.

29

Figure 2-7 - Typical Pressure Relief Valve

20

In a BWR, there is only one set of relief valves required to protect the reactor pressure vessel due to the simplicity of having a single direct steam generation cycle, see

Figure 2–2. In a PWR however, there are multiple relief valves sets required. A set of relief valves protect the over pressurization of the primary loop, usually installed in the pressurizer, and a set of relief valves to protect the secondary loop, usually installed near the steam generator in the main steam piping. See Figures 2–8 and 2–9.

In both reactor designs there are multiple relief valves for redundancy. Every high pressure system in a reactor design must account for ASME codes and catastrophes, specifically the possibility of a relief valve failing to open. If reactor plant designs did not have redundancy and a single relief valve failed to open, with no other means of relieving the pressure; the chances of a pressure boundary rupturing would dramatically increase. Also, while multiple relief valves provide valuable backup protection, their set pressure must differ enough to prevent two from lifting simultaneously and reducing

20

http://www.process-safety-design.com/safely-relief-valves.html

30

pressure too rapidly. Properly addressing over pressure protection will be addressed in

Section 3.

Figure 2-8 - PWR Primary Relief System

21

Figure 2-9 - PWR Secondary Relief System

22

21

http://www.nrc.gov/reading-rm/basic-ref/teachers/04.pdf

22

Ibid.

31

2.4.2

Thermal Protection

The purpose of the emergency core cooling system (ECCS) is to provide the capability to remove design decay heat from the reactor when normal reactor cooling is unavailable. Other reactor protection systems, e.g., SCRAM, stop the chain reaction of fission. The ECCS is responsible for removing heat generated during the fissions and decays of the daughter fission products after the reactor plant is shutdown. The quantity of decay heat required to be removed will be discussed in section 3.2. There are two types of emergency core cooling; electrically powered and passive. See Figure 2-10.

Figure 2-10 - BWR Emergency Core Cooling System

23

23

http://www.ge-energy.com/

32

In a BWR and PWR there are multiple emergency core cooling systems; one high pressure core cooling system, one intermediate pressure injection system, cold-leg accumulators, and a low pressure core injection (reflooder) system (see Figure 2–10).

These emergency safety systems are not nuclear plant type specific; they are mandated by the regulating governing agencies, Department of Energy (DOE) and Nuclear

Regulatory Commission (NRC) and ASME codes. All of these systems are completely independent and redundant divisions of safety systems. The emergency systems are mechanically separated and have no cross connections to prevent one failure from destroying all the ECCS. These systems are also electronically separated so that each division has access to redundant sources of AC power and, for added safety, its own dedicated emergency diesel generator. Each system division is located in a different quadrant of the reactor building, separated by fire walls for redundancy reasons. A fire, flood or loss of power which disables one division has no effect on the capability of the other systems. Finally, each division contains both a high and low pressure system and each system has its own dedicated heat exchanger to control core cooling and remove decay heat.

The high pressure injection system uses special dedicated pumps to deliver this water to the reactor vessel. Upon receipt of an emergency actuation signal, the system will automatically realign to take water from the refueling water storage tank and pump it into the reactor coolant system. The high pressure injection system is designed to provide water to the core during emergencies in which reactor coolant system pressure remains relatively high (such as small break in the reactor coolant system, steam break accidents, and leaks of reactor coolant through a steam generator tube to the secondary side).

The intermediate pressure injection system is also designed for emergencies in which the primary pressure stays relatively high, such as small to intermediate size primary breaks. Upon an emergency start signal, the intermediate pressure injection system pumps will take water from the refueling water storage tank and pump it into the reactor coolant system.

The cold leg accumulators do not require electrical power to operate. These tanks contain large amounts of borated water with a pressurized nitrogen gas bubble in

33

the top. If the pressure of the primary system drops below the pressure of cold leg accumulators, the nitrogen will force the borated water out of the tank and into the reactor coolant system. These tanks are designed to provide water to the reactor coolant system during emergencies in which the pressure of the primary drops very rapidly, such as large primary breaks.

The low pressure injection system (also known as residual heat removal) is designed to inject water from the refueling water storage tank into the reactor coolant system during large breaks, which would cause a very low reactor coolant system pressure. In addition, the residual heat removal system has a feature that allows it to take water from the containment sump, pump it through the residual heat removal system heat exchanger for cooling, and then send the cooled water back to the reactor for core cooling. This is the method of cooling that will be used when the refueling water storage tank goes empty after a large primary system break. This is called the long term core cooling or recirculation mode.

In an event where there is a station blackout or total loss of all AC power, one of the high pressure systems, the reactor core isolation cooling (RCIC) system, is powered by steam provided by the reactor. The RCIC is provided to inject the condensed water of residual heat removal system or condensate storage tank water, etc. into the reactor core with a steam turbine-driven pump. As long as steam is available, the RCIC is able to utilize it for use in the high pressure injection pump.

When there is an event that causes a plant and electric casualty, a passive emergency cooling system is needed. In both a BWR and PWR, the reactor cooling utilizing the passive emergency cooling system must be independent of electrical power.

Therefore, it is designed to use natural circulation produced by a thermal driving head.

A thermal driving head is a difference in pressure caused by a temperature difference and thus a density difference between two columns of water. The warmer water, less dense water tends to flow upward, while cooler, denser water tends to flow downward by gravity. The pressure difference caused by this phenomenon allows flow in the reactor coolant system without a recirculation pump assistance. Passive decay heat removal will be described in detail in section 3.3.

34

2.5

2011 Japan Catastrophic Earthquake and Tsunami

On Friday March 11, 2011, a magnitude 9.0 earthquake hit off the coast of Japan at

14:46 Japan Standard Time (JST). The earthquake occurred with the epicenter approximately 43 miles east of the Oshika Peninsula of Tohoku and the hypocenter at an underwater depth of approximately 20 miles. It was the most powerful known earthquake ever to have hit Japan, and one of the five most powerful earthquakes in the world since modern record-keeping began in 1900. The earthquake triggered powerful tsunami waves that reached heights of up to 133 feet in Miyako in T ō hoku's Iwate

Prefecture, and which, in the Sendai area, travelled up to 6 miles inland.

24

2.5.1

Fukushima Daiichi Nuclear Power Plant Accident

Prior to the disaster, Fukushima had six operable reactors, three units were operating (units 1, 2 and 3) and three units were shut down for planned maintenance

(units 4, 5, and 6). After the earthquake occurred, reactor protection safety measures automatically shutdown, e.g., SCRAMed, the three operating reactors. As the reactor operators were completing the post SCRAM procedures on the reactors, the tsunami struck the Fukushima Daiichi nuclear power plant operating stations approximately 30 to

60 minutes following the earthquake. This catastrophic event started a series of events and failures that led to a loss of all primary and backup electrical power systems. This loss of all electrical power, known as a complete station blackout, resulted in the three operating reactors becoming uncontrollable with respect to reactor core cooling. At the

Fukushima Daiichi plant, substantial fuel damage and core meltdowns have occurred in units 1, 2 and 3. These meltdowns led to explosions in units 1, 2, 3 and 4.

2.5.2

Pressure Protection System Failure

Events from Fukushima highlight the important use of pressure relief valves.

The pressure relief valves worked the way they should work. Unfortunately, the discharge of the valves was directed to an undesirable location, within the secondary containment building. Because of the meltdown occurring in the core, the fuel element coating, zirconium, was heating up and releasing hydrogen gas into the pressure vessel.

24

http://en.wikipedia.org/wiki/2011_T%C5%8Dhoku_earthquake_and_tsunami

35

Zircaloy, undergoes an exothermal chemical reaction with water at high temperatures, causing a release of hydrogen gas. When the relief valves were manually operated to vent the steam out, hydrogen gas also escaped into the containment building. Once the hydrogen found an ignition source, the containment building exploded destroying the second containment. See Figure 2–11 showing the exploded secondary containment buildings; Unit 1, Unit 3 and Unit 4.

The lesson learned from this catastrophe, related to pressure relief, is to direct the pressure relief discharge to an explosion proof, radiological controlled area. If the plants in Fukushima were designed in this manner, the primary containment and secondary containment building would not have failed due to an explosion. This could have prevented (or minimized) the release of radiation and contaminants from the building; which would have resulted in minimizing the environmental damage and personnel radiation exposure. Since the primary and secondary containments failed, the high levels of radiation and contamination being released slowed the emergency responder actions due to the high exposure concerns. This problem resulted in a delay of restarting reactor cooling and thus caused more reactor damage from failure to remove decay heat.

Unit 4 Unit 3

Unit 2 Unit 1

Figure 2-11 - Fukushima Containment Buildings for Reactor Units 1 - 4

25

25

Ragheb, M. Page 67

36

2.5.3

Thermal Protection System Failure

The catastrophe at Fukushima occurred because the reactor operators were unable to remove the decay heat from the reactors. After the earthquake occurred, the reactors were SCRAMed to stop the prompt fissions from occurring. RCIC and ECCS were activated to cool the reactor core. Unfortunately, the tsunami destroyed all primary and backup AC power sources and internal emergency diesel generators. Once all power was drained from the final safety backup battery banks, the reactor was left with only natural circulation cooling utilizing PDHR.

The design of the reactor coolant recirculation system wasn't adequate enough to maintain natural circulation flow without power. Once natural circulation flow was lost the decay heat from the reactor core caused a pressure increase. This pressure increase caused the relief valves lifted causing a loss of reactor coolant. One lesson learned from this disaster is to design reactor coolant recirculation loops to never lose natural circulation flow. The second lesson learned is to better protect the last line of defense; the emergency diesel generators. These generators were placed in pits to prevent fuel spills from leaking into the environment but the tsunami ended up filing those fuel spill pits with water and destroying the generators. If the emergency diesel generators were able to operate, the decay heat generation might have been able to be controlled.

37

3.

Discussion

3.1

Pressure Relief Valves

Pressure relief valves are special valves designed in accordance with ASME standards to protect the integrity of a pressure vessel by relieving abnormally high pressures before a catastrophic failure occurs. These valves are designed to open automatically whenever pressure exceeds certain valves and to terminate the discharge automatically when the pressure decreases below a preset value. There are many types of pressure relief valves depending on the system requirements. Most nuclear power plants use pilot-actuated relief valves for their protection.

3.1.1

Pilot-Actuated Pressure Relief Valves Description

A pilot-actuated relief valve is made up of two sections: a main section and a pilot section. In the unitized pilot-actuated relief valve, the two sections are coupled directly to each other, see Figure 3–1. In de-coupled pilot-actuated relief valve design, the main section and the pilot section are separate units connected by a length of pipe, see Figure 3–2. The main section is a hydraulically operated reverse-seated globe valve.

Use of a reverse seated globe valve allows the reactor plant pressure to help keep the valve tightly shut. The valve stem extends through the seat port and connects to an actuating piston in the valve body. A helical compression spring in the valve body holds the valve stem disc in the shut position.

The pilot section contains its own valve disc, seat, valve stem and a spring bellows assembly. The pilot disc is held shut by differential pressure acting on the disc and (at low pressure) by a force exerted by a stretched bellows. The lower end of the bellows is anchored to the pilot valve body; the upper free end is capped and is mechanically attached to the pilot valve stem. The capped bellows assembly prevents inlet pressure from entering the pilot valve upper bonnet.

The differential pressure established across the bellows actuates the main section of the valve via flow from the pilot section as follows. System pressure, introduced to the bellows via the sensing port, internally pressurizes the bellows and tends to extend the bellows linearly. As system pressure increase and approaches the established

38

pressure relief setting, the extending bellows mechanically unseats the pilot valve disc and allows steam or water to flow into the actuating piston chamber of the main valve section. System pressure then acts on the main valve actuating piston, forcing the piston downward and overcoming both the force of the main relief spring and the system pressure acting under the disc of the main valve. This action fully opens the relief valve and permits steam or water to discharge and relieve the overpressure condition. Relief valve pressure settings are adjusted by varying the normal position of the pilot valve stem to require more or less bellows travel before engaging the pilot valve disc. For relief valves, system pressure must increase above the relief setpoint before the designed flow rate is achieved. The difference between the pressure at the design steam flow or design water flow is achieved and the relief setpoint is called accumulation.

As system pressure decrease, the pilot bellows contracts and system pressure reseats the pilot disc. When flow from the pilot valve is shut off, pressure in the main valve piston chamber discharges at a controlled rate to the outlet side of the valve through specially designed piston orifices and via space around the piston rings. As the piston chamber pressure decreases, the spring force, assisted by system pressure, reseats the main valve. The difference between the relief setpoint and the pressure at which the relief reseats is called blowdown. If the plant pressure again exceeds the pilot valve setting, the lifting action is automatically repeated.

39

Figure 3-1- Unitized Pilot Relief Valve

26

Figure 3-2 - Separated Pilot Relief Valve

27

26

http://www.patentgenius.com/image/6318406-2.html

27

http://www.separation-process.com/pilot-operated-relief-valves.html

40

3.1.2

Pressure Relief Valve Size Determination

Pressure relief valve sizing criteria is controlled by ASME pressure vessel code section III, subsection NC. Pressure relief valve sizing is completed once the majority of the reactor coolant recirculation system has been finalized. The size of the relief valve is dependent on the volumetric flow rate required to protect the plant. A reactor plant designer must determine the pressure relief volumetric flow rate from the total volume of the specific system and from a determination of rate in which the pressure will increase in the system. Once the fastest pressure increase situation is determined, this becomes the most limiting protection operation. The relief valve size must accommodate this limit case, with margin, to assure that there is not a failure.

3.1.3

Pressure Relief Valves Setpoint Determination

As described in section 2.4.1.1, multiple relief valves are employed to ensure protection even when one has failed. While multiple relief valves provide backup protection from single valve failure, their set pressures must differ enough to prevent the multiple relief valves from lifting simultaneously and reducing pressure too rapidly. To prevent multiple pressure relief valves from lifting simultaneously, the set pressures are staggered. To accomplish this, there is a PSI margin built into the relief valve set point determination criteria. Also, the valve with the lowest set pressure must not lift during normal operational transients, and the valve with the highest set pressure must not allow pressure to exceed the system design pressure. Using design guidance from ASME pressure vessel code section III, subsection NC to determine the proper setting of a relief valve, the following must be taken into account: 1. the system normal operating pressure

(NOP), 2. the maximum design transient, 3. instrumentation error, 4. relief valve setpoint tolerance and 5. maximum design pressure of the system.

Once a NOP of a system is determined, the maximum design pressure is set to

150% of the NOP. In a 1600 MWe BWR nuclear power plant, the reactor coolant recirculation system is typically operated around 800 PSIG. With this knowledge, the maximum design pressure can be determined: 800 PSIG * 150% = 1200 PSIG. Once the

NOP has been set, reactor plant designers determine all the operational and pressure changes, commonly called transients that the reactor plant will go through. A design

41

transient is a temporary increase or decrease in pressure (and/or temperature) that occurs as a result of other changes occurring in the plant. For example, if the reactor was operating at 100% power and then decreased to 50% power, there would be a transient that would cause a sudden rise in temperature and pressure in the reactor. Once the reactor power reaches 50% power, the reactor will eventually return to a stable pressure and temperature and the transient is complete. Because there are a large amount of possible changes within the core, a 12.5% margin in pressure is assumed (for this project) to account for the worse case high pressure transient; 800 PSIG * 112.5% = 925

PSIG. The exact transient margin would be calculated to determine if 12.5% was a conservative assumption. If a relief valve was to lift below 925 PSIG, a normal operational change in the reactor could potentially cause the first relief valve to lift. To prevent this from occurring, the first relief valve lift pressure is designed to lift above this maximum transient with some margin (assume 25 PSI) to account for instrument error and prevent relief valve cycling.

After the relief valve size is determined and a specific valve is chosen, using methods described in section 3.1.2, the relief valve setpoint tolerance is obtained.

Manufactures can not guarantee a relief valve will lift at an exact pressure due to manufacturing / machining differences thus a range of relief valve set pressures are given. Upon review of a few relief valve manufacturing component data sheets, a 100

PSI relief valve setpoint tolerance is common; ± 50 PSI.

For this example, the first relief valve would be set at 1000 PSIG ± 50 PSI. This would account for relief valve worse case low opening pressure of 950 PSIG (925 PSIG to account for the maximum transient and 25 PSI margin). The second relief valve would be set at 1105 PSIG ± 50 PSI. The second relief valve set pressure would give a 5

PSI margin to prevent both relief valves from opening simultaneously (worse case high opening of first pressure relief valve at 1050 PSIG (1000 PSIG + 50 PSI) and worse case low opening of the second pressure relief valve at 1055 PSIG (1105 PSIG - 50 PSI)).

The final margin band to incorporate in the pressure relief system design is above the second relief valve setpoint and below the maximum design pressure. A reactor plant designer would not want the second relief valve to lift at exactly the maximum design pressure. If a relief valve was set at the maximum design pressure, a

42

manufacturing error / defect or a localized material fatigue issue could cause the pressure vessel to rupture before the second relief valve lifts. A margin (assume 45 PSI) assures the second relief valve will lift before a catastrophic failure occurs in the pressure vessel.

See Table 4 for a breakdown of the relief valve setpoints.

43

Table 4 - Relief Valve Setpoint Calculation

PSIG Tolerance Description

%

Above

NOP

Setpoint

1200

1155 – 1200

1105 – 1155

1105

1055 – 1105

(45 PSI) Margin to Design Pressure

(50 PSI) Upper Tolerance Band of 2nd Relief Valve

(50 PSI) Lower Tolerance Band of 2nd Relief Valve

50% 1200 PSIG - Design Pressure

38.125% 1105 PSIG - 2nd Relief Valve Setpoint

1050 – 1055

1000 – 1050

1000

950 – 1000

(5 PSI) Margin to Prevent Simultaneous Valve Lifts

(50 PSI) Upper Tolerance Band of 1st Relief Valve

(50 PSI) Lower Tolerance Band of 1st Relief Valve

925 – 950 (25 PSI) Margin to Prevent Unnecessary Lifting

800 – 925 (125 PSI) Margin to Account for Maximum Design Transient 12.5%

800

25% 1000 PSIG - 1st Relief Valve Setpoint

800 PSIG - Normal Operating Pressure (NOP)

44

3.2

Operational Power History & Decay Heat

3.2.1

Operational Power History

Operational power history is a calculation that summarizes the operating power history of a reactor plant. This calculation is dependent on the reactor power history (i.e.

0% - 100%) and time the reactor spent at each power level. For this project, an operational power history of 100% power for 10,000 hours is assumed for calculations described later. Since every reactor plant has a different power rating, operates at different power levels, and spends different lengths of time at a particular power level; the operational power histories per plant vary drastically. The operational power history and power rating directly influences the amount of decay heat generated in the reactor.

For commercial power plants, the operational power histories are relatively close in comparison to similar reactor power size plants because the power companies' ultimate goal is for the plant to be operating at 100 percent power all year. In a perfect scenario, all the commercial plants of the same power rating would operate at 100% power all the time, thus they would have the exact same operational power history and the same amount of decay heat. However, in contrast, ships (ex. nuclear powered cargo ship N/S Savannah) and research reactors (ex. RPI research reactor) have operational power histories that vary dramatically due to a constant change in reactor power and operating history; thus creating different operational power histories and decay heat generation profiles.

3.2.2

Radioactive Decay

Radioactive decay or radioactivity is the phenomenon of an unstable atom or nucleus becoming more stable through the spontaneous emission of radiation. This radiation can be in the form of emitted particles such as alpha or beta particles or electromagnetic emissions such as gamma rays or x-rays. The decay of radioactive isotopes occurs in a random manner, and the precise time at which a single nucleus will decay can't be determined. The fundamental nature of radioactivity is that it is a statistical process that can be described as a probability that the atoms or nuclei of a

45

substance will undergo a spontaneous transmutation. See Figure 3–3 for a uranium-238 decay chain.

→ → →

→ →

→ →

→ → → → →

→ → →

→ → →

(

)

Figure 3-3 - Uranium 238 Radioactive Decay Chain

α = alpha decay

β = beta decay

*Note - All information in Uranium-238 decay chain was obtained from the chart of isotopes.

3.2.3

Decay Heat Generation

Unlike all other forms of electrical power generation, upon shutdown of a nuclear power plant, the power from the core does not instantaneously stop. This remaining power is generated when fission products release energy by undergoing radioactive decay, typically β - decay and γ decay for uranium-235 fission daughter products. This power is commonly referred to as the decay heat production rate or decay heat.

When a reactor is abruptly shut down by the insertion of the control rods, all of the prompt energy sources are eliminated because virtually all fissions stop. β - decay and γ decay, however, do not stop. Reactor thermal output does not drop to zero immediately after shut down; instead it drops to approximately 7 percent of the preshutdown power and continues to decrease at a slower and slower rate as the fission fragments β - decay and γ decay to stable daughter products. See Example 4 demonstrating theoretical decay heat using average fission energy values from Table 3.

Example 4 - Theoretical Average Decay Heat

=

.

.

.

= .

% ≈ % [4]

46

The decay heat production rate is proportional to the number of fission fragments in the reactor. For example, a reactor which has been operating at full power, in this case a 1600 MWe (4800 MWt) BWR, for a long time contains approximately 1.62x10

20 fissions fragments undergoing β - decay and γ decay each second. See Example 5.

Example 5 - Fissions per Second Calculation

= ∗ !

1

1.6

!

10

"#$

"#

"

=

$%&'()*+ ,

'

&'-

.

,

/011023

=

,

/0110231

1 -

[ ]

&4 -

*

*

.

)*+ "

,

&4

5267-

= 4800

!

10

%

1

185.6

1

1.6

!

10

"#$

= 1.62

!

10

&' ,

89::9;<:

:=> -

Where:

F

P

=

= fissions reactor power (MWt)

I

E

= immediate energy released per fission, 185.6 MeV (from Table 3)

All of the β - particles and most of the γ particles are absorbed within the core, causing the reactor coolant within the reactor vessel to heat up. In a large nuclear power plant, approximately 7 percent of the power is still a significant amount of heat, see Example 6.

This heat generation is large enough to cause reactor damage if not removed from the core by the reactor coolant. For this reason, reactor power plant designers are careful to ensure that sufficient coolant flow can be maintained, even in a shutdown reactor.

Example 6 - Decay Heat of 7% Power

?@

() =

?@

*+ ∗

+

.

+

[5]

A@

,-

A@

,-

= 4800

BC

∗ 0.07 = 336

BC

= 336

BC

3.41214

BDEF

BC

GH

47

A@

,= 1146.48

BDEF

GH

= 1.14648 ∗ 10

.

DEF

GH

3.2.4

Decay Heat Calculation

Fission product decay heat (excluding neutron capture) is able to be calculated using methods and data developed in the American National Standard for Decay Heat

Power Generation, ANSI/ANS-5.1-2005. The procedures described in the standard are applicable for calculation of decay heat for both irrated PWR and BWR reactor assemblies. The contribution of fission products to the decay heat power, uncorrected for neutron capture, is calculated from the individual contributions from fission of the four major fissionable isotopes in low-enriched uranium fuel: uranium-235 (U

235

), plutonium-239 (Pu

239

), uranium-238 (U

238

), and plutonium-241 (Pu

241

). These four isotopes account for more than 99 percent of the fissions in a typical fuel. Fission of other isotopes is considered by treating them as uranium-235, which is conservative for most cooling times. The standard also corrects for neutron capture, but it is not necassary for the scoping of this project. For a detailed analysis of decay heat generation, reactor design companies use high performance computers and all the data from this standard to complete an accurate analysis. The assupmtions and procedure utlized for this project allow these calculations to become managable, using excel; while still providing the appropriate amount of accuracy.

To accurately determine the decay heat production rate a detailed calculation could be considered by reviewing all the decay chains of all fission products versus time.

However due to the extreme complexity of this approach, decay heat can be realistically predicted with sufficient accuracy by a few-group representation (e.g. 13 groups).

ANSI/ANS-5.1-2005 provides details for 23 groups, however the amount of value added in the calculation is small. To determine the decay heat production rate, first the heat generated during the operation of the core (from the β - decay and γ decay), commonly called immediate heat, must be analyzed. The immediate heat production rate ( Q /0 ) from fission is found using equation 7.

?@

1) =

.

I 4

2

3

J

K L "4

4)

2 [ ]

48

Where:

ε

φ

2

V c

=

=

=

= fast fission factor macroscopic thermal fission cross section for uranium-235 (cm thermal neutron flux (neutrons/cm reactor core volume (cm

3

)

2

-sec)

-1

)

The decay heat production rate ( Q 70 ) is the sum of the contributions due to the decay of several groups of decay chains. Using ANSI/ANS-5.1-2005, the decay chains that are consentrated on are: uranium-235, plutonium-239, uranium-238 and plutonium-241.

A@

,-

<

=

K A@

,-

,

89:;<=

;>#

[ ]

Where:

Q 70

,

?@ABCD = decay heat production rate from the fission products decay chains

(energy/time-cm

3

)

The decay heat production rate from the fission products decay chains is equal to the energy released by each decay times the decay rate.

A@

,=

N

,

,

E9:;<= ∗

O I PQ

E [

R

]

λ

N

Where:

E

D,chain s

=

=

= useable energy released by each decay of a fission product decay chain (energy/decay) decay constant (sec

-1

) concentration of the fission products decay chains (nuclei/cm

3

)

49

Since the concentration of the fission products (N) is position-dependent, it must be integrated over the core volume to obtain the total number of fission products in the core. The time aspect of the decay heat production rate depends on how the concentration of the fission products changes. The differential equation describing the rate of change of N is described in equation 10:

P

=

S

; ∗

T

K U

6-

& −

O

P

[

*+

]

γ i

Where:

= fission yield of the fission products (nuclei/fission)

The solution to the differential equation, equation 10, for the initial concentration (time =

0) of fission products is given by equation 11:

PVW

=

S

; ∗

T

∑ U

&

O

X

1 −

= "F

G Y

[

**

] t f

Where:

= time at constant fission rate

As shown in the in equation 11, the time dependence of the fission product concentration, N, is governed by

X

1 −

= "F

G Y

. Once a reactor operates a long time at a constant power, the fission products concentration will reach equilibrium. This extended operation at a constant power (and constant fission rate), will reach an equilibrium concentration given by equation 12:

P

HI =

S

; ∗

T

∑ U

&

O

[

*Z

]

50

If you substitute equation 12 into equation 9, the total decay heat rate versus time during the buildup to equilibrium is given by equation 13:

<

A@

,-

X

J

Y

=

K N

,

,

89:;<=

;>#

O

I Q

E ∗

P

;

,

HI

Q

E

X

1 −

= "F

G Y

[

*[

] and the equilibrium decay heat rate is equation 14:

A@

,-

<

V

W

=

K N

,

,

89:;<=

;>#

O

I Q

E ∗

P

HI

Q

E [

*\

]

When the reactor is shutdown, the fission products will decay with a time dependence given by

= "F

G

where t s

is the time after shutdown. Therefore, the decay heat production rate following shutdown is given by equation 15:

A@

,-

X

J ,

<

=

Y

=

K N

,

,

89:;<=

;>#

O

I Q

E ∗

P

HI

Q

E

X

1 −

= "F

G Y= "F

G

[

*

]

Since most of the variables in the equation above are constant, we can substitute many of these variables with constants from the ANSI/ANS-5.1-2005 specification to make the calcuation more managable. Equation 15 then becomes equation 16:

A@

,-

X

J ,

#$

=

Y

=

K

;>#

]

;K

O

;K;

X

1 −

= "F

G Y= "F

G

[

*

]

51

Table 5 - Coefficients for thermal fission of U

235

, Pu

239

, Pu

241

and fast fission of U

238

Term index j

U-235 (thermal) Pu-239 (thermal) U-238 (fast) Pu-241 (thermal)

α

1j

λ

1j

α

2j

λ

2j

α

3j

λ

3j

α

4j

λ

4j

1 5.28E-04 2.72E+00 1.65E-01 8.92E+00 3.94E-01 4.34E+00 3.09E-01 2.90E+00

2 6.86E-01 1.03E+00 3.69E-01 6.90E-01 7.46E-01 1.71E+00 5.44E-01 6.49E-01

3 4.08E-01 3.14E-01 2.40E-01 2.36E-01 1.22E+00 6.06E-01 4.08E-01 2.56E-01

4 2.19E-01 1.18E-01 1.03E-01 1.01E-01 5.28E-01 1.94E-01 1.58E-01 8.71E-02

5 5.77E-02 3.44E-02 3.49E-02 3.72E-02 1.48E-01 6.98E-02 4.16E-02 2.51E-02

6 2.25E-02 1.18E-02 2.30E-02 1.43E-02 4.60E-02 1.88E-02 1.48E-02 1.33E-02

7 3.34E-03 3.61E-03 3.91E-03 4.51E-03 1.04E-02 6.13E-03 5.82E-03 6.38E-03

8 9.37E-04 1.40E-03 1.31E-03 1.32E-03 1.70E-03 1.38E-03 1.95E-03 2.02E-03

9 8.09E-04 6.26E-04 7.03E-04 5.35E-04 6.91E-04 5.28E-04 9.52E-04 6.29E-04

10 1.96E-04 1.89E-04 1.43E-04 1.73E-04 1.47E-04 1.61E-04 1.82E-04 1.75E-04

11 3.26E-05 5.51E-05 1.76E-05 4.89E-05 2.40E-05 4.84E-05 1.53E-05 4.02E-05

12 7.58E-06 2.10E-05 7.35E-06 2.02E-05 6.93E-06 1.56E-05 4.50E-06 1.53E-05

13 2.52E-06 9.99E-06 1.77E-06 8.37E-06 6.49E-07 5.36E-06 9.83E-07 7.61E-06

Table 6 - Power Fractions for Fission of U

235

, Pu

239

, U

238 and Pu

241

Burnup

5 MWd/KgU

U-235

0.808

4 % U-235 Enrichment

Pu-239

0.129

U-238

0.061

Pu-241

0.002

Since there are not equal amounts of uranium-235, plutonium-239, uranium-238 and plutonium-241 in the fuel at any one time, a percentage of the elements is assumed in

Table 5. This assumption is of uranium-235 at 4 percent enrichment and 5 MWd/KgU burned (aka short operating history). Calculation of the fission product decay heat power requires the fraction of fission power contributed by each of the fissionable nuclides at each irradiation time step. The fractions are required because each fission nuclide has a unique decay heat power curve as represented by the coefficients described in Table 6. For low uranium typically used in power reactors, the initial power comes mainly from uranium-235 and uranium-238. During irradiation and the depletion of uranium-235, fission power shifts uranium-235 to the plutonium-239 and plutonium-241

52

isotopes. Using equation 16 and values from Tables 5

28

and 6

29

, the decay heat versus time can be calculated for each isotope. Each isotope's values are added together to get a total energy (MeV) per second per fission result. These values can be adjusted to the size of the reactor (1600 MWe, 4800 MWt) and operational power history (100% power for 10,000 hours) to get energy per hour. The results of the calculations are summarized in Table 7 and graphed in Figures 3–4.

28

ANSI/ANS-5.1–2005. Pages 20 - 21

29

Nichols. Page 19.

53

Table 7 - Calculated Decay Heat versus Time

Decay Heat Decay Heat Decay Heat Decay Heat Decay Heat

2.5

3.0

3.5

4.0

4.5

5.0

6.0

7.0

8.0

Time

(Seconds after shutdown)

(Minutes after shutdown)

(MBTU/hr)

0.0001 1140.17777

(MBTU/hr)

0.5 1096.92471

(Hours after shutdown)

(Days after shutdown)

(MBTU/hr) (MBTU/hr)

662.00457 244.65818 65.11453

1.0

1.5

2.0

1062.27526

1032.42310

1006.45754

573.66449

523.94278

490.67066

189.22595

161.29388

143.64593

46.16239

37.88684

33.14985

983.66103

963.46656

945.42458

929.17693

914.43727

900.97545

877.17600

856.66551

838.68986

466.29932

447.36009

432.02950

419.23951

408.30991

131.02682

121.34784

113.60579

107.23549

101.87895

30.06799

27.88128

26.22310

24.89935

23.80049

398.78217 97.29233 22.86083

382.73856 89.78461 21.30764

369.46769 83.81489 20.04812

358.07529 78.88495 18.98871

9.0

10.0

15.0

20.0

25.0

30.0

35.0

40.0

822.72279

808.38598

753.29481

714.87020

685.61332

662.00457

642.18694

625.09449

45.0

50.0

60.0

70.0

610.06892

596.67657

573.66449

554.46092

80.0

90.0

538.10156

523.94278

100.0 511.52832

110.0 500.52209

120.0 490.67066

348.04433 74.70275 18.07759

339.05708 71.08721 17.28201

304.22644 58.33431 14.42356

279.39351 50.54007 12.60864

260.19665 45.24009 11.31482

244.65818 41.36823 10.32785

231.71756 38.39913 9.54493

220.72791 36.04678 8.90810

211.25559 34.13463

202.99165 32.54932

189.22595 30.06799

178.16343 28.20201

169.02205 26.73137

161.29388 25.52762

154.63610 24.51203

148.81021 23.63424

143.64593 22.86083

8.38028

7.93562

7.22557

6.67741

6.23380

5.86124

5.53955

5.25626

5.00352

3.00515

2.82223

2.26708

1.97638

1.78726

1.65722

1.56148

1.49027

1.43625

1.39418

1.33300

1.28919

1.25437

1.22426

1.19677

1.17094

1.14615

(Months after shutdown)

(MBTU/hr)

14.33254

10.25585

8.32058

7.17469

6.39945

5.81856

5.35279

4.96399

4.63217

4.34548

3.87718

3.51526

3.23136

54

700

650

600

550

500

450

400

350

300

250

200

150

100

50

0

1200

1150

1100

1050

1000

950

900

850

800

750

0

Decay Heat versus Time

Seconds

Minutes

Hours

10 20 30 40 50

Time

60 70 80

Figure 3-4 - Overview Calculated Decay Heat Versus Time

90 100 110 120

55

3.2.5

Decay Heat Removal

The decay heat that is created after the nuclear reactor is shutdown is removed using the normal active decay heat removal system (residual heat removal system

(RHRS)). This system consists of an independent loop, consisting of dedicated heat exchangers and pumps to cool the reactor coolant and fuel elements. See Figure 3–5 for a typical decay heat removal system.

Figure 3-5 - Residual Heat Removal System

30

30

http://www.nrc.gov/reading-rm/basic-ref/teachers/04.pdf

56

3.3

Passive Decay Heat Removal

Passive decay heat removal (PDHR) is utilized when active decay heat removal, described in section 3.2.5, is unavailable. If active decay heat removal capability should be lost, decay heat generation within the core will cause reactor plant temperatures to increase. PDHR, on the other hand, doesn't require AC power to operate. PDHR uses natural circulation, described in section 3.3.1, along with ambient heat loses to lower the temperature in the reactor core. Heat losses from the reactor plant to its surrounding structures, the primary containment, and adjacent buildings will increase as the plant temperature increases. Hence, heat losses to ambient will increase as the decay heat generation rate falls off.

In a BWR, during the first hours of the PDHR operations, the decay heat generation will exceed the ambient heat loss rate. This thermal energy generation will be dissipated by the heating and boiling of the reactor coolant. Excess steam pressure may cause relief valve cycling to dissipate the pressure buildup in the reactor vessel.

Unfortunately this action, while helping to reduce the pressure in the reactor vessel and main steam system, causes a loss of reactor coolant inventory. This loss of reactor coolant will allow the creation of more steam within the reactor vessel. Once the steam bubble becomes large enough to cover the feed water return nozzle, the steam will stop all flow of makeup water into the reactor vessel. This will cause the water level to continuously decrease, due to the lack of makeup water, and uncover the fuel elements.

In a PWR, during the first hours of the PDHR operations, the decay heat generation will also exceed the ambient heat loss rate similar to a BWR. The thermal energy generation is dissipated by the heating of the primary and secondary plant systems. First, secondary system water inventory will be lost by boiling off the steam generator inventory and cause steam generator relief valve cycling. This loss of steam generator water inventory prolongs the heating of the reactor coolant due to the heat transfer within the steam generator. This heat transfer increases the probability of success to cool the plant. Following loss of all steam generator inventory, decay heat continues to heat the primary coolant and may lift a primary relief valve. The lift of a primary relief valve will cause a loss of reactor coolant volume and potentially uncover the fuel elements.

57

In both cases, if the decay heat generation rate exceeds the ambient heat loss rate, reactor coolant inventory will be lost through a relief valve, the fuel channels could begin to boil dry, and the fuel could overheat and be damaged. If the reactor decay heat generation falls below the ambient heat loss rate before the fuel uncovers, the reactor will cool and the fuel will remain submerged and undamaged.

3.3.1

Natural Circulation

During PDHR operations, natural circulation is important in maintaining reactor coolant flow. Active DHR requires pumping power, with various pumps called forced circulation, to move water. Natural circulation, on the other hand, achieves flow without the use of a mechanical source, e.g., no pump.

If there is little or no flow of the reactor coolant, the temperature will increase rapidly and the creation of steam would increase. Therefore, a reactor plant is designed to use natural circulation produced by a thermal driving head. A thermal driving head is a difference in pressure caused by a temperature difference and thus a density difference between two columns of water. The warmer water, less dense water tends to flow upward, while cooler, denser water tends to flow downward by gravity. The pressure difference caused by this phenomenon allows flow in the reactor coolant system without a reactor coolant recirculation pump assistance.

In reactor plants, natural circulation in the coolant loops may be lost by 1. steam voiding of a high point or 2. cold trapping in the reactor coolant recirculation loops low points.

In a PWR, steam voiding can occur as the pressurizer cools off and depressurizes and the plant reaches saturation. Once saturated plant conditions exist, the bubble in the pressurizer can transfer into the reactor vessel and reactor plant and interrupt liquid flow.

In a BWR, steam voiding can occur when the steam bubble stops all make-up water from entering the vessel, thus interrupting fluid flow. This casualty will reduce ambient losses since the steam is less effective heat transfer properties than liquid-filled piping.

Cold trapping can occur when a portion of the loop piping experiences some localized cooling. At some point, the flow may stop if the plant lacks sufficient thermal driving head to push out the column of cooler, denser water that has formed. This can

58

reduce ambient losses by isolating the vessel from a portion of the reactor coolant recirculation loop heat transfer surfaces.

59

4.

Conclusions

Events at the Fukushima Daiichi nuclear power station in Japan have reemphasized the importance of reliable reactor protection systems. While design requirements were complex and robust, in a post Fukushima era, reactor plant designs must account for many new scenarios that were deemed improbable in the past designs. The probability and severity of the design basis accidents, analyzed in the future design process, will increase due to the recent nuclear plant accidents as well as the increase in major natural disasters around the world. These new analyses will help improve the robustness of the reactor plant safety requirements.

The reactor plant safety requirements are, and will continue to be, stringent because personnel and environmental safety is paramount. The recent events have brought skepticism to the general public about the safety posture of all current plants. In order to prove to the general public that nuclear power is safe and have them remain tolerant of nuclear power plant risks, the safety posture of every plant must be proven to be undeniably safe.

Using correct pressure relief protection sizing and setpoint determinations, described in section 3.1, and updated decay heat generation values, described in section

3.2 and shown in Figure 3–4, and; new nuclear power plant concepts can be designed with robust integrity. Applying the natural circulation criteria and PDHR concepts, described in section 3.3, to the reactor plant design will also help improve the safety posture of the future reactor plants while reducing their dependence on outside AC power.

Incorporating the design guidance described in this project and applying the lessons learned from Fukushima, future nuclear power plants will be better equipped to handle major natural disasters while minimizing the damage of the reactor. This improved design information will ease the public's worry about the chances of another catastrophic disaster like Fukushima occurring near their homes and businesses.

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