1 SUPPLEMENTARY MATERIAL INVERSION SETUP ATM No. regions* Time resolution Inversion Transport Inv. full period Data period Spin-up period Sfc. data Smoothed obs/real obs No. stations Interp/extrap sfc. data Pre-subtracted fluxes Fossil Fuel Biosphere Flux Ocean Flux Data weights Prior information Prior spatial/temporal correl. Lab Country Personnel Publication CCAM CCAM 146 (94 land, 52 ocean) Monthly Monthly response functions Fwd simul. cycling 1999** 1987 - 2004 1989 - 2004 2 years GLOBALVIEW-CO2 (2005) Smoothed observations 74 (77 records) NO/NO YES Andres et al. (1996) Randerson et al. (1997) Takahashi et al. (2002) Following Baker et al. (2006) LMDz LMDz Model-grid scale Monthly Monthly response functions Retro-plumes 1986 - 2004 1989 - 2004 2 years GLOBALVIEW-CO2 (2005) Smoothed observations 82 YES/NO YES Andres et al. (1996) Randerson et al. (1997) Takahashi et al. (2002) Following Baker et al. (2006) FRCGC FRCGC 64 Monthly Monthly response functions Fwd simulation 1988 - 2004 1988 - 2004 0 years GLOBALVIEW-CO2 (2005) Smoothed observations 87 YES/YES YES Andres et al. (1996) Randerson et al. (1997) Takahashi et al. (2002) Following Patra et al. (2005) A priori flux PDF NO/NO CSIRO-MAR Australia Pickett-Heaps, Rayner & Law Rayner et al. 2008 A priori flux PDF YES/NO LSCE - CEA/CNRS France A priori flux PDF NO/NO FRCGC Japan Peylin & Bousquet Following Peylin et al. (2005) Patra & Maksyutov Patra et al. (2005a) 2 Text S1: Technical details of the four inversion models 3 *’Model-grid based’ indicates that flux estimates are obtained at the model grid resolution rather than pre-defined flux regions. TM3 TM3 Model-grid scale Daily Forward/adjoint runs 1990 - 2006 1996 - 2005 6 years Raw data (flask/hourly obs.) Real observations 51 NO/NO YES van Aardenne et al. (2001) Sitch et al. (2003) Gloor et al. (2003) Following Rödenbeck (2005)*** NO YES/YES MPI-BGC Germany Rödenbeck & Heimann, Marshall Rödenbeck et al. (2003)**** 4 **Forward simul. cycling 1999 refers to the use of a forward simulation to generate monthly response functions for 1999 only. These response functions are then used 5 repeatedly for each year of the inversion. 6 *** http://www.bgc-jena.mpg.de/mpg/websiteBiogeochemie/Publikationen/Technical_Reports/tech_report6.pdf 7 ****Available at: http://www.bgc-jena.mpg.de/~christian.roedenbeck/download-CO2/ 8 9 10 11 12 REFERENCES 13 Andres, R.J., G. Marland, I. Fung and E. Matthews (1996), A 1 degree * 1 degree distribution of carbon dioxide emissions from fossil fuel 14 consumption and cement manufacture, 1950 – 1990, Glob. Biogeochem. Cyc., 10, 419 – 429. 15 16 Baker, D. F., R. M. Law, K. R. Gurney, P. Rayner, P. Peylin, A. S. Denning, P. Bousquet, L. Bruhwiler, Y. –H Chen, P. Ciais, I. Y. Fung, M. 17 Heimann, J. John, T. Maki, S. Maksyutov, K. Masarie, P. Prather, B. 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