FORWARD SIMULATION ATM type "Real winds" transport Analyzed meteorology Anal. Met. Resolution Simulation time-step Simulation length Spin-up period Distribution of vert. levels Model grid Horizontal resolution CCAM LMDz GCM* GCM* YES YES YES (NCEP) YES (ECMWF) 12 hours 12 hours 1 hour 1 hour 1987 - 2004 1987 - 2004 4 years 4 years Sigma coord. system Sigma coord. system Genomic projection Latitude/longitude ~2°-2° 3.75° - 2.5° McGregor et al. Relevant model publication (1996) Hourdin et al. (2006) No. vertical levels 18 19 Text S2: Technical details of the four forward simulations FRCGC ATM** YES YES (NCEP/NCAR) 12 hours 40 min 1988 - 2004 3 years Sigma coord. system Latitude/longitude 2.5° - 2.5° Maksyutov et al. (2008) 15 TM3 CTM*** YES YES (NCEP) 6hr 1hr 1990 - 2004 6 years Sigma coord. system Latitude/longitude 4° - 5° Heimann & Körner (2003) 19 *General Circulation Model **Atmospheric Transport Model ***Chemical Transport Model REFERENCES Andres, R.J., G. Marland, I. Fung and E. 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