A direct mathematical method to calculate the efficiencies of 4πNaI (Tl) scintillation detector Salam Noureddeena, Mahmoud I. Abbas1, a, b, Mahmoud Koreka a) Physics Department, Faculty of Science, Beirut Arab University, Beirut, Lebanon b) Physics Department, Faculty of Science, Alexandria University, 21511 Alexandria, Egypt Abstract A direct mathematical method is applied to calculate the total and geometrical efficiencies of a 4π NaI(Tl) scintillation detector for an arbitrarily positioned radiating point source. The 4π NaI(Tl) scintillation detector is made up of 8 square large NaI(Tl) detectors[1]. The central square is left void, see figure (1), so the radiating source can be moved easily. The results are compared with previous experimental treatment. Keywords: 4π NaI(Tl) gamma detectors; Geometrical efficiency; Total efficiency and Extended sources. 1. Introduction Scintillation detectors are widely applied for gamma-ray detection. Gamma rays could be emitted from a point, line, disc or cylindrical sources. The detection of these radiations is done by different detectors [1-12]. These detectors were designed with different efficiencies, depending on the shape of the detector and on the material of its active medium. The geometrical and total efficiencies for the source – detector system were determined experimentally and theoretically [1]. In the present work we will take into consideration the photon path length through the detector active medium in order to determine the efficiency of the 4πNaI (Tl) scintillation detector [11]. The work described below involves the use of straightforward analytical formulae for the computation of the 4πNaI(Tl) detector array geometrical and total efficiencies. Section 2 presents direct mathematical formulae for the geometrical and total efficiencies in the case of isotropic radiating axial point, non-axial point, plane and volumetric sources. Section 3 contains comparisons between the calculated efficiency using the formulae derived in this work 1 Corresponding author, email: mabbas@physicist.net with the published experimental and simulated values illustrating the validity of the present mathematical formulae. The conclusions are presented in section 4. 2. Mathematical viewpoint The position of the isotropic point source is defined by (ρ,h), where, is the lateral displacement between the source and the detector axis, whereas h is the height of the source from its center. The polar (θ) and azimuthal (φ) angles represent the direction of the photon when it enters the detector active volume. The effective rays which enter the detector active volume traverse a distance d until it emerges from detector [10]. 2.1. Axial point source placed inside the detector void part The incident photon may enter the detector’s inner side and emerges from see figure (2) i) lower base 1(LB1): d = 1 ii) (1) detector side (1): d = 2 iii) a - a1 2 sin(θ ) cos(φ) (2) lower base (2) (LB2): d = 3 iv) a c 2 sin(θ ) cos(φ) cos(θ ) b c 2 sin(θ ) cos(φ) cos(θ ) (3) detector side (2): d = 4 b - b1 2 sin(θ ) cos(φ) (4) The polar angle θ takes the steps a tan - 1 1 1 (5) a (6) 2c θ 2 = tan - 1 θ3 = tan 2c - 1 b1 (7) 2c b θ 4 = tan - 1 1 2c (8) The azimuthal angle φ takes the steps 2 Φ 1 = tan - 1 b a (9) Φ π -1 a = + tan 2 2 b Φ = π + tan - 1 3 a Φ4 (10) b = (11) a 3π + tan - 1 2 b (12) The total efficiency can be calculated by 1 1 2 /2 1 / 2 2 4 2 ∫ ∫f1dd ∫ ∫f 2dd ∫ ∫f3dd ∫ ∫f 4dd 3 4 0 0 1 1 1 1 3 / 2 3 /2 4 4 4 4 f dd ∫ ∫f dd ∫ ∫f dd ∫ ∫f dd ∫ ∫ 4 1 3 3 1 2 3 3 2 1 3 3 2 2 (13) 2 / 2 ∫∫f1dd ∫ ∫f 2dd 0 4 1 f i = (1 - e - μdi ) sin( θ ) . e - 2 μ1.t sin( θ ) , i=1,2….10. (14) where, μ and μ1 are the total attenuation coefficient of the detector and its housing [13](with thickness t cm) material for gamma-ray photon with energy Eγ, respectively. 2.2 Non-axial point source placed inside the detector void part The incidence photon may enter the detector’s inner side and emerges from see figure (3) i) lower base 1 (LB1): d1 = a 2 ρ cos(Φ) c 2 sin( θ ) cos(Φ) cos(θ ) (15) ii) detector side (1): a - a1 d2 = 2 sin( θ ) cos(Φ) (16) iii) lower base 2 (LB2): d3 = a + 2 ρ cos(Φ) c - 1 cos(θ ) 2 sin( θ ) cos(Φ) (17) 3 iv) detector side 2 a - a1 2 sin( θ ) cos(Φ) d4 = (18) v) detector side 3 b - b1 2 sin( θ ) cos(Φ) d5 = (19) vi) lower base 3 (LB3) d6 = b1 c ρ sin( α) + cos(θ ) 2 sin(θ ) sin( Φ) sin(θ ) (20) vii) detector side 4 d7 = b - b1 2 sin( θ ) cos(Φ) viii) (21) lower base 4 (LB4) b1 c ρ sin( α) cos(θ ) 2 sin( θ ) sin( Φ) sin( θ ) d8 = (22) The final expression of the total efficiency of a non-axial point source at different positions is given by: 5 2 /2 2 2 5 2 ∫ ∫f dd ∫ ∫ f 1 dd ∫ ∫ f 2 dd 1 0 0 8 1 1 /2 2 / 2 7 8 7 ∫ ∫f 2 dd ∫ ∫f 3 dd ∫ ∫f 4 dd 2 8 2 6 7 6 4 (23) 6 8 8 6 /2 /2 6 8 ∫ ∫f 5 dd ∫ ∫f 6 dd ∫∫f 7 dd ∫ ∫f 8 dd 4 3 5 5 5 7 7 6 The polar angle θ takes the steps a - 2 ρcos(α) -1 1 θ1 = tan θ 2 = tan - 1 θ 3 = tan - 1 (24) 2.c. cos(Φ) a - 2 ρcos(α) (25) 2.c. cos(Φ) b1 - 2 ρsin( α) (26) 2.c. sin( Φ) 4 θ 4 = tan - 1 θ5 = tan - 1 θ 6 = tan - 1 θ 7 = tan - 1 θ8 = tan - 1 b - 2 ρsin( α) (27) 2.c. sin( Φ) b1 + 2 ρsin( α) (28) 2.c. sin( Φ) b + 2 ρsin( α) (29) 2.c. sin( Φ) a1 + 2 ρ cos(α) (30) 2.c. cos(Φ) a + 2 ρ cos(α) (31) 2.c. cos(Φ) The azimuthal angle φ takes the steps a - sin( ) 2 1 tan 5 b - cos( ) 2 (32) b cos( ) 2 1 tan 6 2 b sin( ) 2 (33) tan - 1 7 (34) a sin ( ) 2 b - cos( ) 2 a - cos( ) 3 2 1 tan 8 2 b sin ( ) 2 (35) 2.3 Line source placed inside the detector void part The efficiency of a 4πNaI (Tl) scintillation detector arising from a line of length ℓ cm is derived as [3] h2 ξ1dh ∫ ξL = h1 (36) h2 - h1 where, ξ1 is the total efficiency of an axial point source as identified before in equation 13. The total efficiency of the line source is determined at different positions along the axial axis of the detector. 5 2.4 Disc source placed inside the detector void part The efficiency of 4πNaI (Tl) scintillation detector arising from a disc source is derived as [3] s 2 ∫ 2 d D 0 (37) s2 Where ξ2 is the total efficiency of a non-axial point source as identified before in equation 23. The total efficiency of the disc source is determined at different positions along the axis of the detector. 2.5 Cylindrical source placed inside the detector void part The efficiency of 4πNaI (Tl) scintillation detector arising from a cylindrical source is derived as [3] h2 ξ D dh ∫ ξC = h1 (38) h2 - h1 where ξD is the total efficiency of a disc source as identified before in equation 37. 3. Results The direct mathematical method is applied for both geometrical and total efficiencies for the 4πNaI(Tl) detector array using isotropic point source. The 4πNaI scintillation detector is made up of 8 square large NaI(Tl) detectors as shown in Figure 1. The central square is left void so the radiating source can be moved easily. The cross sectional size and the length of a NaI(Tl) crystal are 10.2 cm×10.2 cm and 40.6 cm, respectively. The housing of the NaI(Tl) crystal is 1 mm thick Stainless steel. The solid angle of the detection geometry is high, so that more than 95% can reach the detector surface. The total efficiency values of a point source placed at different positions along the axial axis and at different energies have been calculated for 4πNaI (Tl) scintillator detector by the direct mathematical method and compared with Byun et al. [1, 12] as shown in figures 4 and 5. The total efficiency is also determined at lateral distances ρ from the central axis of the detector as shown in figure (6). The figure shows no variation of the total 6 efficiency as the lateral distance changes for the same height. Three different sources non-axial point, line source of length 5 cm and disc source of radius 2 cm have been used in the theoretical calculations for this detector. As shown in figures 7, 8 and 9 as the height of the source from the center increases the total efficiency decreases for the different sources which is consistent with the results obtained by Byun et al [1, 12]. In our work the height is taken from zero which is the center to 20.3 cm which is at the surface of the detector. The same calculations are repeated again on the lower side of the detector and the graph is drawn between the efficiency and the position. It is clear also that the total efficiency for disc source is greater than that of line and point sources. The percentage difference between the calculated values and the measured ones is given by Diff (%) cal meas *100 (39) meas 4. Conclusions Direct mathematical expressions to calculate the total and the full-energy peak efficiencies of 4πNaI(Tl) scintillation detector have been derived in the case of axial point, non-axial point and extended to line, disk and cylindrical sources. In addition, the attenuation of photons by the source container and the detector housing materials is also presented in simple straight forward mathematical expressions. The agreement between the results calculated in this work and the published values is very good, the high discrepancies being less than 4 % (point source). 7 Sample access Fig (1) TThreeThe 4π NaI(Tl) scintillation detector is made up of 8 square large NaI(Tl) detectors dimension al view of the cylindrical Phoswich scintillatio n detector Dector 8 Fig (2) The position of point source for an axial point source 9 Fig (3) The position of point source for a non- axial point source. 10 Present work Experimental work 1.0 Relative Total Efficiency 0.9 0.8 0.7 0.6 0.5 0.4 0.3 -20 -10 0 10 20 Source position in cm Fig (4) The variation of the relative total efficiency with energy for a point source moves around the center of the detector . Present work Experimental 0.95 0.90 0.85 Total Efficiency 0.80 0.75 0.70 0.65 0.60 0.55 0.50 0.45 0.0 0.5 1.0 1.5 2.0 2.5 3.0 Energy in Mev Fig (5) The variation of the total efficiency with energy for a point source placed at the center of the detector 11 0.5 Total effeciency 0.4 0.3 0.2 0.1 0.0 0 1 2 3 4 5 6 Lateral distance p (cm) Fig (6) The variation of the total efficiency with lateral distance Total efficiency Relative total efficiency 1.00 0.95 Efficiency 0.90 0.85 0.80 0.75 0.70 0.65 0.60 -20 -10 0 10 20 Position in (cm) Fig (7) The variation of the total and relative efficiency with the position of the point source placed at the non-axial point 12 Total efficiency Relative total efficiency 1.00 0.95 Efficiency 0.90 0.85 0.80 0.75 0.70 0.65 0.60 -20 -10 0 10 20 Position in (cm) Fig (8) The variation of the total and relative efficiency with the position of the line source placed at the axis of the detector Total Effeciency Relative Total Effeciency 1.0 Effeciency 0.9 0.8 0.7 0.6 0.5 -20 -10 0 10 20 Position in (cm) Fig (9) The variation of the total and relative efficiency with the position of the disc source placed at the axial point 13 References: [1] Byun SH, Prestwich WV, Chin K, McNeill FE, Chettle DR (2006) IEEE Trans. Nucl.Sci. NS-53 (5), 2944. [2] Abbas MI (2001). HPGe detector photopeak efficiency calculation including self-absorption and coincidence corrections for Marinelli beaker sources using compact analytical expressions. Appl. Radiat. Isot. 54, 761– 768. [3] Abbas MI (2001). A direct mathematical method to calculate the efficiencies of a parallelepiped detector for an arbitrarily positioned point source. Radiat. Phys. Chem. 60, 3–9. [4] Abbas MI, Basiouni MM (1999). Direct mathematical calculation of the photopeak efficiency for gamma rays in cylindrical NaI(Tl) detectors. American Inst. Phys. CP450, 268–272. [5] Blaauw M (1998). Calibration of the well-type germanium gamma-ray detector employing two gamma-ray spectra.Nucl. Inst. Meth. A 419, 146– 153. [6] Selim YS, Abbas MI (2000). Analytical calculations o gamma scintillators efficiencies. II: total efficiency for wide co-axial disk sources. Radiat. Phys. Chem. 58, 15–19. [7] Selim YS, Abbas MI, Fawzy MA (1998). Analytical calculation of the efficiencies of gamma scintillators. I: total efficiency for co-axial disk sources. Radiat. Phys. Chem. 53,589–592. [8] Wang TK, Hou IM, Tseng CL (1999). Well-type HPGe detector absolute peak-efficiency calibration and true-coincidence correction. Nucl. Instr. and Meth. A 425, 504–515. [9] Huber JS, Moses WW, Andreaco MS, Petterson O (2001). Trans. Nucl.Sci.vol 48,pp 684-688 [10] Abbas MI (2009) Nucl. Technol. 168, 41. [11] Abbas MI (2010) Nuclear Instruments and Methods in Physics Research A 615, 48–52. [12] Byun SH, Prestwich WV, Chin K, McNeill FE, Chettle DR (2004) Nucl. Instr. Meth.Phys. Res. A 535, 674. [13] Hubbell JH, Seltzer SM (1995) NISTIR 5632, USA. 14