Stability of the analytical perturbation for nonlinear coupled kinetics equations Ahmed E. Aboanber1,2, Abdallah A. Nahla1, Faisal A. Al-Malki3 1 Department of Mathematics, Faculty of Science, Tanta University, Tanta 31527, Egypt. 2 Department of Mathematics, Faculty of Science and Arts, Qassim University, QassimBuraidah, P.B 1300, Buraidah 51431, Saudi Arabia. 3 Department of Mathematics, Faculty of Science, Taif University, Taif 888, Saudi Arabia. E-mails: aboanber@tu.edu.eg, nahla@tu.edu.eg, faisal_malki1@hotmail.com Abstract: The critical problem in nuclear-reactor kinetics is to predict the evolution in time of the neutron population in a multiplying medium. Point kinetics allows the study of the global behavior of the neutron population from the average properties of the medium. In this paper, an efficiency improved technique based on the small parameter approximation is developed for the analytical solution of stiff system kinetics equations for linear and/or nonlinear coupled differential equations. The variations of neutron density, precursors, fuel temperature and reactivity are obtained in terms of time. Furthermore, the stability criterion of the perturbed method is investigated and discussed. The procedure is tested by using a variety of reactivity functions, including step reactivity insertion, ramp input and oscillatory reactivity changes. The solution of the developed method is compared to other analytical and numerical solutions of the point reactor kinetics equations; the results proved that the approach is both efficient and accurate to several significant figures. The proposed method can be used in real time forecasting for power reactors in order to prevent reactivity accidents. Keywords: Point kinetics , Neutron population, Stiff system kinetics equations, Reactivity, Stability 1 1. Introduction The sub-critical reactor kinetics analysis is important to determine the neutron density as function reactivity insertion rate with respect to the initial sub-criticality. The analytical and numerical solutions of the point kinetics equations in the presence of temperature feedback reactivity are useful to estimate the transient behavior of the reactor power and other parameters of the reactor cores. There are many analytical and numerical solutions available to study the reactor kinetics in the presence the adiabatic feedback model. Chen (1990) studied a nonlinear time dependent point power reactor problem with delayed temperature feedback on reactivity. Dam (1996) analyzed the point reactor kinetics equations in combination with linear temperature feedback for the reactivity and an adiabatic heating of the core after loss of cooling. Damen and Kloosterman (2001) used a simple reactor model with one delayed neutron group and first order fuel and temperature feedback mechanisms to calculate the linear transfer function from reactivity to reactor power that was subsequently used in a root-locus analysis. Aboanber and Nahla (2002) introduced a solution of the point kinetics equations in the presence of Newtonian feedback model using different cases of Padé approximations via analytical inversion method. Aboanber and Hamada (2003) reduced the point kinetics equations in the presence of Newtonian feedback to a differential equation in a simple matrix form convenient for explicitly power series solution involving no approximation beyond the usual space-independent assumption. Aboanber (2006) studied stability and efficiency improved class of generalized Runge-Kutta methods for several sample problems of the stiff system point kinetics equations with reactivity feedback. Chen et al. (2006 and 2007) presented a new analysis for the prompt supercritical process of nuclear reactor with temperature feedback and initial power while inserting large step reactivity 0 and small step reactivity 0 . Nahla and Zayed (2010) developed the analytical approximation and numerical solution of the point nuclear reactor kinetics equations with average one-group of delayed neutron and the adiabatic feedback model. Sathiyasheela (2009) presented power series solution method for solving point kinetics equations with lumped model temperature and 2 feedback. Tashakor et al. (2010) presented a numerical solution of the point kinetics equations with fuel burn-up and temperature feedback using an implicit time method. Kinard and Allen (2004) described and investigated an efficient numerical solution for the point kinetics equations in nuclear reactor dynamics. Quintero-Leyva (2008) developed a numerical algorithm (CORE) to solve the point kinetics equations of nuclear reactors. Sathiyasheela (2010a) solved analytically the sub-critical point reactor kinetics equations with one group of delayed neutrons using incomplete gamma functions and binomial expansions. Sathiyasheela (2010b) solved analytically inhomogeneous point kinetics equations for step and linear reactivities using the prompt jump approximation. Theler and Bonetto (2010) studied the stability of the point kinetics equations. Espinosa et al. (2011) derived and analyzed the fractional point-neutron kinetics model for the dynamic behavior in a nuclear reactor In this work, the analytical perturbation for the point reactor kinetics equations with one-group delayed neutrons and the adiabatic feedback model is presented. This analytical perturbation method based on the expansion of the neutrons density in powers of the small parameter. The time dependent neutron density, and the average density of delayed neutron precursors as functions of reactivity are derived. The relations of reactivity, neutron density and temperature with time are calculated. The stability of the analytical perturbation method is investigated. Finally, comparison between the results of the method and the conventional methods is introduced. 2. Mathematical Model (Analytical Perturbation) The point kinetics equations with one group delayed neutrons in the presence of Newtonian temperature feedback are a stiff nonlinear coupled ordinary differential equations (Ash, 1979; Glasstone and Sesonske, 1981; Hetrick, 1993; Stacey, 2001) which given by: dn(t ) (t ) = n(t ) C (t ) dt l (1) dC(t ) = n(t ) C (t ) dt l (2) 3 (t ) = 0 [T (t ) T0 ] (3) dT (t ) = K c n(t ) dt (4) where, n(t ) is the neutron density, (t ) is the reactivity as function of time t, is the total fraction of the delayed neutrons, l is the prompt neutrons generation time, is the decay constant of delayed neutron precursors, C (t ) is the precursor concentrations of delayed neutron, T (t ) is the temperature of the reactor, T0 is the initial temperature of the reactor, is the temperature coefficient of reactivity, and K c is the reciprocal of the thermal capacity of reactor. From Eqs. (1), (2), (3) and (4) we have: d (t ) = K c n(t ) dt (5) d 2 n(t ) dn(t ) d (t ) l = ( (t ) l ) (t ) n(t ) 2 dt dt dt (6) Starting Eq. (5) into Eq. (6) and multiplied by ( K c ), we get d 3 (t ) d 2 (t ) d (t ) d (t ) l = ( ( t ) l ) ( t ) dt dt 3 dt 2 dt 2 (7) Treating Eq. (7) with the initial conditions given by: d d 2 (0) = K c n0 yield: (0) = 0 and n(0) = n0 , (0) = 0 , 2 dt dt l where d 2 (t ) d (t ) 2 = ( ( t ) l ) ( 2 (t )) 2 dt 2 dt (8) 2 = 02 2K c n0 ( l 0 )/ Beginning Eqs. (5) and (8): dn(t ) ( 2 2 (t )) l = (t ) l n(t ) dt 2K c and consequently, we get: 4 (9) dn(t ) d (t ) ( 2 2 (t )) l = ( (t ) l )n(t ) d dt 2K c (10) Eqs. (5) into (10) gives dn(t ) ( 2 2 (t )) lK c n(t ) ( (t ) l )n(t ) = d 2K c (11) Starting from the fact that (lK c ) is very small, equal 2.5 10 10 for a pressurized- water reactor with U as fissile material, let us consider = lK c and = /K c into Eq. 235 (12), then n(t ) dn(t ) ( (t ) l )n(t ) = ( 2 2 (t )) d 2 (12) Assume the neutron density are perturbed so that: n(t ) = n1 (t ) n2 (t ) (13) An application of Eq. (12) yields [n1 (t ) n2 (t ) ] d [n1 (t ) n2 (t ) ] d ( (t ) l )[ n1 (t ) n2 (t ) ] = 2 (14) ( 2 2 (t )) Therefore, 2 2 (t ) n1 (t ) = 2 l (t ) n2 (t ) = (15) 2 2 2 (t ) 2 2 (t )( l ) 2 (t ) 4 l (t ) ( l (t )) 3 (16) And consequentely, the neutron density in terms of reactivity can be obtained as follow: n(t ) = 2 2 (t ) 2 2( l ) (t ) 2 (t ) 1 2 l (t ) 2 ( l (t )) 3 (17) The rate of change for reactivity in terms of neutron density is obtained by combining Eqs. (13) and (5), neglecting the somallest term with the coefficient K c so that: d (t ) = K c n1 (t ) dt (18) 5 Combining with Eq. (15) yields t= 1 l 0 l 0 1 1 ln ln (t ) (t ) (19) 3. Stability discussion 3.1. Bounded of solution: The bounded values for the variation of reactivity with time can be estimated by taking the limit of Eq. (19) when the reactivity tends to : l 2 2 1 0 ( 0 )( (t )) ln 2 = (20) lim t = lim 2 (t ) ( (t ))( 0 ) ( t ) ( t ) which can be rewite as: lim (t ) = , That is lim n(t ) lim n(t ) t t ( t ) Furthermore, the limit of Eq. (19) when the reactivity tend to : 2 2 (t ) 2 2 (t )( l ) 2 (t ) 1 = 0 (21) lim 3 2 ( t ) 2 l (t ) ( l ( t )) Eqs. (20) and (21) show that: lim n(t ) = 0 , in this particular instance the neutron flux t given by Eq. (19) is bounded function. 3.2. Stability of solution The stability of the solution n(t ) obtained by Eq. (17), which satisfy the nonlinear ordinary differential equation (12) is considered. Let us add a small function (t ) to the solution n(t ) such that n* (t ) = n(t ) (t ) which assure Eq. (12) also, [n(t ) (t )] d [n(t ) (t )] ( l (t ))[n(t ) (t )] = ( 2 2 (t )) (22) d 2 applying into Eq. (12), neglecting the term (t ) d (t ) and dividing by (t )n(t ) yields d 1 d (t ) 1 dn(t ) l (t ) = (t ) d n(t ) d n(t ) Combining Eqs. (17) and (23): 6 (23) 1 d (t ) (t ) d 1 dn(t ) 2 l (t ) n(t ) d (t ) (t ) 2 = ( l ) 2 2 (24) 2 2 (t )( l ) (t ) (t ) (t ) 2 2 (t )( l ) 2 (t ) 4 2 The solution of Eq. (23) taking the following form: 2 0 (t ) 4 0 (t ) 2 (t ) = (0) exp ( l )2 ( l )( l ) 2 4( l )( l ) 1 0 2 2 (t ) ( l )2 ( l )( l ) 2 4( l )( l ) 1 (t ) 2 2 0 ( l )2 2 l ( l ) 2 2 l ( l ) 2 2 2 0 2 2 l (t ) ( l ) ( l )2 2 l ( l ) 2 2 2 l ( l ) 2 2 0 2 2 l (t ) ( l ) l (t ) 4n0 3 2 l (t ) 2 2 (t ) l 2 (t ) 4 (25) (4) Taking the limit, lim (t ) = lim (t ) = 0 t (26) ( t ) That is, the perturbed solution of Eq. (17) is stable. 3.3. Liapunov stability: The stability of the solution of the autonomous system is also analyzed according to Jordan and Smith, 2007, as follows: 7 Assume that n (t ) is an equivalent solution as n(t ) given by Eq. (17) so that: 2 2 (t ) 2 2( l ) (t ) 2 (t ) 1 n (t ) = 2 l (t ) 2 ( l (t )) 3 (27) where 2 = 02 2K c n0 ( l 0 )/ From Eqs. (17) and (27), for which | 02 02 |< , the inequality is: 2 ( 2 2 2( l ) (t )) | n(t ) n (t ) |< 2( l (t )) 4( l (t )) 4 (28) Taking the limit of Eq. (28) when time tend to which means the reactivity tend to which = min { , } . 2 ( 2 2 2 ( l )) < lim | n(t ) n (t ) |< t 2( l ) 4( l ) 4 (5) Then, the perturbation solution n(t ) of Eq. (19) is Liapunov stable. 4. Results and discussions Consider the prompt supercritical process in a pressurized-water reactor with 235 U as fissile material. It is assumed that = 0.0065, l = 0.0001 s, = 0.07741s1 , K c = 0.05 K/MW s, and = 5 10 5 K 1 . The supercritical process will take place when three initial reactivities are inserted into the reactor. This reactor is operating in critical state with initial power n0 = 10.0MW . The comparison between conventional numerical and analytical solution for the neutron density is shown in Fig (1). Variation of neutron density n(t ) as a function of time t at the initial reactivity 0 = 0.25 , 0.5 and 0.75 is drawn in Fig (1). It is found that variation of neutron density with time for different methods, developed analytical perturbation, Chen (1990) approximation and numerical method, is corresponding. Furthermore, the relation between reactivity and time at the initial reactivity 0 = 0.25 , 0.5 and 0.75 is shown in Fig (2). Finally, the relation between time, reactivity, neutron density and temperature using 8 the analytical perturbation, Chen approximation and numerical methods is presented in Tables (1), (2) and (3) with initial reactivity 0 = 0.25 , 0.5 and 0.75 respectively. The numerical method based on Taylor's series method (Nahla and Zayed, 2010). It is found that the difference between the developed analytical perturbation results, Chen approximation and numerical reaults are small less than 10 3 . 5. Conclusions The developed analytical perturbation method for nonlinear couple reactor kinetics equations with one group of delayed neutrons in presence of temperature feedback have been derived. The analytical perturbation technique based on the small term, l Kc which equal 2.5 10 10 for a pressurized-water reactor with 235 U as fissile material. The stability of the analytical perturbation technique are studied with different method. The analytical results of the supercritical process in a pressurized-water reactor with 235 U as fissile material are drawn and tabulated. It is found that the neutron density using the analytical perturbation method are identical with the neutron density using Chen approximation and numerical method which based on Taylor's series. References [1] Aboanber, A.E., 2006. Stability of generalized Runge-Kutta methods for stiff kinetics coupled differential equations. Journal Physics A: Mathematics and General 30, 1859-1876. [2] Aboanber, A.E., Hamada, Y.M., 2003. Power series solution (PWS) of nuclear reactor dynamics with newtonian temperature feedback. Annals of Nuclear Energy 30, 11111122. [3] Aboanber, A.E., Nahla, A.A., 2002. Solution of the point kinetics equations in the presence of Newtonian temperature feedback by Padé approximations via the analytical inversion method. Journal Physics A: Mathematics and General 35, 96099627. [4] Ash, M., 1979. Nuclear reactor kinetics. McGraw-Hill, Inc., USA. [5] Chen, G.S., 1990. A nonlinear study in a reactor with delayed temperature feedback. 9 Progress in Nuclear Energy 23 (1), 81-91. [6] Chen, W.Z., Buang, B., Guo, L.F., Chen, Z.Y., Zhu, B., 2006. New analysis of prompt supercritical process with temperature feedback. Nuclear Engineering Design 236, 1326-1329. [7] Chen, W.Z., Guo, L. F., Zhu, B. and Li, H., 2007. Accuracy of analytical methods for obtaining supercritical transients with temperature feedback. Progress in Nuclear Energy 49 (4), 290-302. [8] Dam, V.H., 1996. Dynamics of passive reactor shutdown. Progress in Nuclear Energy 30 (3), 255-264. [9] Damen, P.M.G., Kloosterman, J.L., 2001. Dynamics aspects of plutonium burning in an inert matrix. Progress in Nuclear Energy, 38 (3-4), 371-374. [10] Espinosa-Paredes, G., Polo-Labarrios, M.A., Espinosa-Martnez, E.G., ValleGallegos, E., 2011. Fractional neutron point kinetics equations for nuclear reactor dynamics. Annals of Nuclear Energy, 38 (2-3), 307-330. [11] Glasstone, S., Sesonske, A., 1981. Nuclear Reactor Engineering. Chapman & Hall Inc. [12] Hetrick, D.L., 1993. Dynamics of Nuclear Reactors. American Nuclear Society, La Grange Park. [13] Jordan, D.W., Smith, P., 2007. Nonlinear Ordinary Differential Equations. Fourth edition, Oxford University Press. [14] Kinard, M., Allen, E.J., 2004. Efficient numerical solution of the point kinetics equations in nuclear reactor dynamics. Annals Nuclear Energy 31, 1039-1051. [15] Nahla, A.A., Zayed E.M., 2010. Solution of the nonlinear point nuclear reactor kinetics equations. Progress in Nuclear Energy 52(8), 743-746. [16] Quarteroni, A., Sacco, R., Saleri, F., 2000. Numerical Mathematics. Springer-Verlag New York, Inc. USA. [17] Quintero-Leyva, B., 2008. CORE: A numerical algorithm to solve the point kinetics equations. Annals of Nuclear Energy 35, 2136-2138. [18] Sathiyasheela, T., 2009. Power series solution method for solving point kinetics equations with lumped model temperature and feedback. Annals of Nuclear Energy 36, 246-250. 10 [19] Sathiyasheela, T., 2010. Sub-critical reactor kinetics analysis using incomplete gamma functions and binomial expansions. Annals of Nuclear Energy 37, 12481253. [20] Sathiyasheela, T., 2010. Inhomogeneous point kinetics equations and the source contribution. Nuclear Engineering and Design 240, 4083-4090. [21] Stacey, W.M., 2001. Nuclear Reactor Physics. John Wiley and Sons, Inc. USA. [22] Theler, G.G., Bonetto, F.J., 2010. On the stability of the point reactor kinetics equations. Nuclear Engineering and Design 240, 1443-1449. [23] Tashakor, S., Jahanfarnia, G., Hashemi-Tilehnoee, M., 2010. Numerical solution of the point reactor kinetics equations with fuel burn-up and temperature feedback. Annals of Nuclear Energy 37, 265-269. 11 Table1: Reactivity, Neutron density and Temperature as functions of time at initial reactivity 0.25 . Time Reactivity Neutron Density (s) ($) Chen App. Anal. Pert. Num. Meth. (K ) 0.0 0.25 10.0 10.0 10.0 300.0 10.0 0.207752 11.920335 11.916985 11.916994 305.492219 20.0 0.158941 13.368069 13.365992 13.366050 311.837653 30.0 0.105789 14.155938 14.155193 14.155254 318.747375 40.0 0.050948 14.249263 14.249636 14.249701 325.876708 50.0 -0.003053 13.742208 13.743366 13.743446 332.896942 60.0 -0.054208 12.796830 12.798441 12.798521 339.547050 70.0 -0.101164 11.585716 11.587518 11.587613 345.651356 80.0 -0.143195 10.257042 10.258853 10.258986 351.115344 90.0 -0.180073 8.921237 8.922945 8.923002 355.909445 100.0 -0.211921 7.651384 7.652932 7.653634 360.049753 110.0 -0.239085 6.489769 6.491133 6.491833 363.581103 115.0 -0.251051 5.956452 5.957721 5.958417 365.136628 12 Temperature Table2: Reactivity, Neutron density and Temperature as functions of time at initial reactivity 0.5 . Time Reactivity Neutron Density (s) ($) Chen App. Anal. Pert. Num. Meth. (K ) 0.0 0.5 10.0 10.0 10.0 300.0 10.0 0.446517 18.220153 18.195046 18.195158 306.952849 20.0 0.359572 26.743477 26.725939 26.726191 318.255655 30.0 0.245386 31.900591 31.894813 31.895273 333.099883 40.0 0.120072 32.594130 32.596224 32.597210 349.390656 50.0 -0.001244 30.096715 30.102094 30.103104 365.161749 60.0 -0.109559 26.074489 26.080507 26.081541 379.242696 70.0 -0.201433 21.691699 21.697222 21.698225 391.186282 80.0 -0.276824 17.572978 17.577644 17.578548 400.987074 90.0 -0.337342 13.984105 13.987887 13.988706 408.854429 100.0 -0.385198 10.991478 10.994473 10.995258 415.075780 110.0 -0.422648 8.564157 8.566497 8.567273 419.944209 120.0 -0.451736 6.631089 6.632902 6.633668 423.725630 130.0 -0.474206 5.110976 5.112373 5.113089 426.646742 140.0 -0.491496 3.926056 3.927128 3.927845 428.894540 147.0 -0.501146 3.259237 3.260127 3.260785 430.148962 13 Temperature Table3: Reactivity, Neutron density and Temperature as functions of time at initial reactivity 0.75 . Time Reactivity Neutron Density (s) ($) Chen App. Anal. Pert. Num. Meth. (K ) 0.0 0.75 10.0 10.0 10.0 300.0 10.0 0.647415 47.877804 47.691231 47.691120 313.336018 20.0 0.405342 71.467363 71.455316 71.456192 344.805479 30.0 0.135590 66.159691 66.179999 66.181404 379.873244 40.0 -0.094510 53.134130 53.153026 53.154675 409.786287 50.0 -0.273940 40.439861 40.453927 40.455536 433.112263 60.0 -0.408680 30.010027 30.020056 30.022448 450.628466 70.0 -0.507961 21.967440 21.974528 21.976612 463.534940 80.0 -0.580334 15.950425 15.955435 15.957500 472.943463 90.0 -0.632747 11.522864 11.526410 11.528276 479.757136 100.0 -0.670554 8.296181 8.298697 8.300844 484.672014 110.0 -0.697738 5.960236 5.962025 5.963708 488.205908 120.0 -0.717256 4.275238 4.276512 4.278079 490.743231 130.0 -0.731262 3.062159 3.063066 3.065639 492.564088 140.0 -0.741275 2.193012 2.193659 2.195231 493.865788 150.0 -0.748468 1.567664 1.568125 1.571112 494.800892 153.0 -0.750188 1.418068 1.418485 1.421002 495.024410 14 Temperature Fig.1: Variation of neutron density for different initial reactivity. 15 Fig.2: Variation of reactivity for different initial reactivity. 16