1 Supplementary material for “The effect of smoke emission amount on changes in cloud 2 properties and precipitation: A case study of Canadian boreal wildfires of 2007” 3 Zheng Lu and Irina N. Sokolik 4 School of Earth and Atmospheric Sciences, Georgia Institute of Technology, 311 Ferst Drive, 5 Atlanta, Georgia, 30332-0340, USA 6 7 Table S1. WRF-Chem-SMOKE configurations selected for the present study Model aspect Grid Setting Arakawa C grid; Horizontal grid: Δx=Δy=5km, 842 (EW)×602(SN) grids; 36 vertical layer Meteorology initialization NCEP Global Forecast System (GFS) reanalysis data Time step 20 seconds Simulation period 20-25 July, 2007 Microphysics Morrison two-moment scheme Radiation RRTM longwave radiation scheme Goddard shortwave radiation scheme 8 Cumulus No cumulus parameterization Land surface NOAH land surface model Planetary boundary layer YSU PBL scheme Gas chemistry CBM-Z gas chemistry module Aerosol MOSAIC aerosol module 9 Meteorological evaluations of WRF-Chem-SMOKE 10 Meteorological fields modeled with WRF-Chem-SMOKE were extensively validated against 11 data from ground-based meteorological stations provided by the Canadian National Climate Data 12 and Information Archive (http://www.climate.weatheroffice.gc.ca/climateData/canada_e.html). 13 Daily mean data of surface temperature, sea level pressure, and wind speed for 22, 23, and 24 14 July 2007 from about 300 stations were compared to model outputs (the SMOKE10 case) of 15 corresponding model grids (see Figures S1-S3). In addition, we perform regression and 16 correlation analyses, the results of which are summarized in Table S2. 17 18 19 Figure S1. Observed vs. modeled surface temperatures on 22, 23, and 24 July 2007. Blue lines 20 indicate the regression lines. 21 22 23 Figure S2. Observed vs. modeled sea level pressure on 22, 23, and 24 July 2007. Blue lines 24 indicate the regression lines. 25 26 Figure S3. Observed vs. modeled wind speed on 22, 23, and 24 July 2007. Blue lines indicate 27 the regression lines. 28 29 30 31 32 33 Table S2. The results of regression and correlation analyses between observations (X) and model 34 outputs (Y) for surface temperature, sea level pressure, and wind speed on 22, 23, and 24 July. Intercept of Correlation No. of model regression coefficient grids (stations) Slope of regression 35 36 Surface temperature (22 July) 0.68 6.7 0.70 340 Surface temperature (23 July) 0.70 6.4 0.72 356 Surface temperature (24 July) 0.74 6.27 0.70 350 Sea level pressure (22 July) 0.91 82.5 0.92 240 Sea level pressure (23 July) 0.87 133.6 0.93 274 Sea level pressure (24 July) 0.81 185.9 0.87 267 Wind speed (22 July) 0.44 2.7 0.61 328 Wind speed (23 July) 0.57 2.0 0.62 342 Wind speed (24 July) 0.58 1.9 0.64 340