Research statement – Dr. Yonatan Sivan My research involves a variety of subjects in nano-photonics including linear and nonlinear optical effects in plasmonic and semiconductor nanostructures, graphene, metamaterials and photonic crystals. The research relies on a combination of analytical, asymptotical and numerical techniques, but almost always involves collaboration with an experimental group. Some of the specific projects that occupy us are: 1. The use of metallic nanoparticles for performance improvement in super-resolution microscopy. This project is based on my recent prediction that metallic nanoparticles can be used to improve the resolution and signal brightness in Stimulated-emission-depletion microscopy (Y. Sivan et al., ACS Nano 2012; Y. Sivan, Appl. Phys. Lett. 2012), see Fig. 1. The project involves analytical work, heavy computations, nanofabrication and optical characterization (spectroscopy, imaging, lifetime imaging etc.). The work is done in collaboration with 2 groups at Imperial College London, as well as with the group pf Nobel Laurate in Chemistry, Prof. S Hell at Gottingen, Germany. Fig. 1. A schematic illustration of a (NP-) STED nanoscope with excitation beam shape (green), depletion doughnutshaped beam (dark red), hybrid plasmonic-fluorescent emitter (yellow-red metal shell nanoparticle) and overall subdiffraction fluorescence signal (light red). Insets show the transverse cross sections of the field distributions and signal. We were recently able to perform proof-of-concept measurements of the technique. Using metal nano-shells of about 150nm in size, we demonstrated a 4-fold reduction of the intensity required to obtain super-resolution, see Fig. 2 and [Sonnefraud et al. Nano Lett. 2014]. Further work demonstrated similar performance with gold spheres coated by fluorescent silica of sizes 30-60nm. More recently, we also repeated these measurements with 10 by 30 nm metal rods coated with fluorophores attached to actin chains. We are now in advanced stages of testing the viability of the technique for live cell imaging. Fig. 2. Resolution improvement using core-shell NPs, as a function of the STED depletion power density used. Blue disks: bare doped silica cores only. Black dotted circles: core-shell nanoparticles. The red dashed (resp. green dotted) line is a least square fit of the bare silica (resp. core-shell) data. 2. Ultrashort optical pulse reversal in semiconductor nano-photonic structures. This project is based on a series of joint publications with Prof. Sir J. Pendry (Sivan and Pendry, Phys. Rev. Lett. 2010; Sivan and Pendry, Opt. Express 2010; Sivan and Pendry, Phys. Rev. A 2010) whereby we showed how to employ dynamically tuned photonic crystals for extreme manipulations of ultrashort pulses such as ultrafast switching, time-resolved spectroscopy, time-reversal, storage and stopping. The current theoretical work on light and charge carrier dynamics in semiconductor waveguides accompanies the experimental effort done in the University of Twente, The Netherlands. Specifically, we showed in [Sivan at al., Optics Express 2015] that transient gratings enable optical switching at femtosecond features, i.e., orders of magnitude faster than the conventional limits. This is enabled by diffusion of the free carriers along the periodicity of the grating, so that the grating contract self-erase on sub-picosecond time scales. Fig. 3. A spatiotemporal contour map of wave evolution in the switchable mirror time-reversal scheme developed by Sivan and Pendry. The illustration shows the splitting of the incident wave to a forward and a backward (timereversed) wave. Another direction is to explore additional applications of the technique such as short pulse generation. This is done by turning on a Bragg grating that partially overlaps a longer signal pulse. This work is done in collaboration with the group of Amiel Isha’aya at BGU using silica fibers. We also explore some additional material platforms for these applications such as plasmonic waveguides or graphene ribbons. All the above work is accompanied by a careful derivation of a simplified and accurate set of governing equations by extending the standard coupled-mode theory to pulse propagation and for time-varying optical properties. This work is currently will be submitted for publication soon. 3. Nonlinear nanofocusing in plasmonic waveguides. In this project we are studying the prospects of focusing intense beams into nanometric light spots. We study the interplay between linear focusing provided by the plasmonic environment, nonlinear focusing and losses in the metal. 4. Novel designs of magnetic and negative refractive index metamaterials. This work is based on a modal analysis of metal wire clusters. The work is done in collaboration with a group at Tel Aviv University. As part of that, we performed the first ever multipole expansion for wire media under general oblique incidence conditions, and provided a simple polarization-based explanation to the seemingly contradictory assigning of magneto-electric coupling to these structures. These findings appear in [P.Y. Chen, Y. Ben-Yakar and Y. Sivan, Phys. Rev. B, submitted]. 5. Frequency up-conversion using plasmonic waveguides and nano-particles. Here we aim to exploit various recent ideas from nonlinear optics to realize highly efficient frequency mixing processes in short plasmonic waveguides. We employ heavy analytical methods such as the spectral decomposition and transformation optics. We also study these processes in various nanoparticle complexes.