Supplementary Materials for Variability of Modeled Runoff over China and its links to climate change Li Mingxing, Ma Zhuguo, Lv Meixia RCE-TEA, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China This file includes: Supplementary text Methodology S1 Statistical analyses S1.1 Estimating multiple rates of change S1.2 Correlation, curve fitting, and envelope methods S2 Links assessment between runoff and climatic covariates Fig3. S1–S9 Tab. S1 References Methodology S1 Statistical analysis S1.1 Estimating multiple rates of change Runoff time series are often characterized by unequal variations owing to the complex feedback from the determinants, i.e., precipitation, vegetation cover, and geomorphology. Estimating multiple rates of change (slopes) provides a more complete picture of the runoff evolution and its interaction with climatic covariates. In this study, we adopt the quantile regression (QR) method to estimate the functional relations between runoff and climate variables (precipitation and temperature) for all portions of a probability distribution rather than the mean. QR is a collection of statistical methods for estimating and drawing inferences about conditional quantile functions. Compared with the widely used ordinary least squares regression (OLS), it is more suitable to model the heterogeneous variance of nonstationary change rates in heterogeneous data. Since its introduction by Koenker and Bassett (1978), QR has been used extensively in economics (Alagidede and Panagiotidis, 2012), ecology (Cozzoli et al., 2013), climate change (Barbosa et al., 2011; Bremnes, 2004; Hirschi et al., 2011; Meng and Shen, 2014), and so on. In this study, we used the sparsity method to compute the confidence intervals of the regression slopes. S1.2 Correlation, curve fitting, and envelope methods We used the Pearson correlation coefficient and the Student’s t-test to estimate its significance. The variation trends in the time series expressed as linear slopes were estimated using least squares, with significance tested by Student’s t-test. The correlation coefficient R between simulations (r) and observations (f) is defined as 1 π =π ∑π π=1(ππ −π)(ππ −π) ππ ππ , (1) where N is the sample size, π and π are means of the simulated and observed series, respectively, and σf and σr are the standard deviations of the simulated and observed series, respectively. Curve fitting was performed using polynomials of the form y ο½ c ο« ax ο« bx 2 . (2) The envelope calculations were performed by using the local maximum method combined with cubic spline interpolation and smoothed by the two-point adjacent averaging (Adler 1978). S2 Link assessment between runoff and climatic covariates The links between runoff and covariates are complex owing to the land–atmosphere and ocean–atmosphere interactions in variable spatiotemporal scales. Understanding the mechanisms behind them is beyond the scope of this study. Building on the observations of precipitation and temperature herein, we provide the relation patterns for runoff and covariates (precipitation and temperature) for the in-depth understanding of the nature of runoff variability. For simplicity, the relations are quantified using the correlation coefficient (eq. 1) and the Student’s t-test for its significance. The annual correlation is derived from 12-month averaged time series with sample size of 48 (1961–2008). Similarly, the summertime correlation is calculated from three-month (JJA) averaged values. The spatial structures of the links between runoff and climatic covariates are described by the correlation coefficients for each grid cell. The sensitivity of the runoff to covariates is represented by nonparametric regression, the quantile slopes, and the 0.1 and 0.9 quantiles for lower and upper end responses, respectively (see section 1). The slope significance is assessed with the standard errors of the quantile slopes by local estimates of sparsity. Fig S1 Comparison of normalized model monthly terrestrial water storage with those of GRACE over China from February 2004 to December 2008, a monthly time series, b averaged annual variations, c time series without annual variations. Fig S2 Spatial patterns for ratios (%) of annual and summer mean runoff to precipitation over 1961–2008 Figure S2 shows that high ratios cover the humid southeast and gradually decrease to the arid northwest, with maxima over 90% and minima close to zero across China. Summer runoff ratios likewise are characterized by the southeast–northwest gradient, although high-end percentages extend notably over southeastern China. The spatial structure of runoff ratio across China is largely related to that of soil moisture and precipitation (Li et al. 2011). Generally, in the humid regions with high soil moisture contents, saturation excess runoff model dominants runoff generation and leads to great runoff ratio; in the arid regions, infiltration excess runoff is the major model of runoff. The runoff ratios decline with precipitation drops and soil dryness. However, the mechanisms for runoff–precipitation interaction are complex, especially in the areas of plateau, mountain, glacial, permafrost (Huntington and Billmire 2014; Xu 2015). Fig S3 Spatial patterns for means of surface runoff and subsurface runoff (mm mo−1) across China over 1951–2008, and linear trends patterns (mm mo−1). The black lines indicate significance at the 0.05 level. Fig S4 Spatial patterns for runoff trends (mm mo−1) at quantiles 0.1, 0.3, 0.5 0.7, and 0.9, respectively, over 1951–2008. The black lines denote significance at the 0.05 level. Figure S4 shows that the spatial patterns of runoff trends for quantiles from 0.1 to 0.9 are characterized by the generally similar spatial gradient: significant increasing trends in the humid south, large-area decreasing trends in the wet–dry transition zone, and non-significant and mixed trends in the arid northwest. Moreover, the upper quantile trends are generally much steeper than those at lower quantiles. Discrepancies in trends from lower to upper quantiles manifest mainly over parts of northeastern China, northwestern high latitudes, and the Tibetan Plateau, where the trends tend to be upward at upper quantiles, but downward or slightly upward at lower quantiles. The changes in quantile trends of runoff imply generally intensified runoff variability from 1951 to 2008, which is associated with increased extreme precipitation (Zhai et al., 2005), groundwater level variations, and climate-warming introduced thawing/melting of glacial and permafrost (Chen et al. 2012; Xu 2015). Fig S5 Evolutions of runoff in the regions with significant ling-term trends. Fig S6 The time series of summer (JJA) runoff, precipitation, and temperature for the two critical regions in 1961-2008. The runoff is modeled by CLM driven with observation-based forcing. Precipitation (Prec-CMA) and temperature (Temp-CMA) series are taken from gridded observations by CMA, along with the precipitation from GPCP (Prec-GPCP) for 1979–2008. Fig S7 Quantile regression slopes at the 0.1–0.9 quantiles for the summer (JJA) monthly runoff versus monthly precipitation (a, c) and temperature (b, d) for two critical regions, along with 95% confidence interval of the estimated slopes shown as shadings. The horizontal lines indicate a slope of 0 (no trends). Red lines indicate regression slopes by the ordinary least squares regression with 95% conο¬dence intervals (red dash lines). Fig S8 Spatial patterns of correlation coefficients for annual runoff versus a precipitation and b temperature in 1961-2008. Figure S8 shows that the spatial patterns of correlation between annual runoff and precipitation and temperature over 1961–2008 are similar to the spatial structure of precipitation climate (not show the figure). The positive correlation locates over the humid regions, the negative (or weak positive) correlation over the arid regions, and the transition zone mostly covered by weak correlation, largely analogous to that in Interim ECMWF (European Centre for Medium-Range Weather Forecasts) ReAnalysis [ERA-Interim (Dee et al. 2011), not show the figures]. The negative correlation over arid and mountainous regions and plateaus is associated with relatively less proportion contributed from local precipitation but increasing effects of lateral groundwater transport, glacial melt (Gao et al. 2012). With respect to temperature, the spatial characteristics resemble that for runoff versus precipitation, with negative correlation over arid regions but the positive over humid regions. In the humid regions, the runoff-temperature correlation is remarkably less than those between runoff and precipitation. The relation of temperature to runoff showed a more mixed spatial structure, with significantly negative correlation over the South China, North China, and most of arid regions, but positive relation over the most part of Tibetan Plateau, Sichuan Basin, and northern coastal areas. Such correlation changes reflect the evident regional characteristics of the interactions between runoff and climate covariates. Fig S9 Spatial patterns of quantile slopes for summer (JJA) runoff versus precipitation and runoff versus temperature at quantile 0.1. Table S1 Quantile slopes (mm mo-1) of runoff and corresponding standard errors for Fig 3 Domains Region A Region B 0.1 -0.61 (0.22) 0.48 (0.22) 0.3 -0.56 (0.09) 0.69 (0.18) Quantile 0.5 0.7 -0.44 -0.54 (0.14) (0.06) 0.69 0.74 (0.14) (0.13) 0.9 -0.24 (0.26) 1.08 (0.25) References Adler R (1978) On the envelope of a Gaussian random field Journal of Applied Probability:502513 Alagidede P, Panagiotidis T (2012) Stock returns and inflation: Evidence from quantile regressions Economics Letters 117:283-286 Barbosa SM, Scotto MG, Alonso AM (2011) Summarising changes in air temperature over Central Europe by quantile regression and clustering Natural Hazards and Earth System Sciences 11:3227-3233 doi:10.5194/nhess-11-3227-2011 Bremnes JB (2004) Probabilistic forecasts of precipitation in terms of quantiles using NWP model output Monthly Weather Review 132:338-347 Chen RS, Qing WW, Liu SY, Han HD, He XB, Wang J, Liu GY (2012) The relationship between runoff and ground temperature in glacierized catchments in China Environmental Earth Sciences 65:681-687 doi:10.1007/s12665-011-1115-8 Cozzoli F, Bouma TJ, Ysebaert T, Herman PMJ (2013) Application of non-linear quantile regression to macrozoobenthic species distribution modelling: comparing two contrasting basins Marine Ecology Progress Series 475:119-+ doi:10.3354/meps10112 Dee DP et al. (2011) The ERA-Interim reanalysis: configuration and performance of the data assimilation system Quarterly Journal of the Royal Meteorological Society 137:553597 doi:10.1002/qj.828 Gao H, He X, Ye B, Pu J (2012) Modeling the runoff and glacier mass balance in a small watershed on the Central Tibetan Plateau, China, from 1955 to 2008 Hydrological Processes 26:1593-1603 doi:10.1002/hyp.8256 Hirschi M et al. (2011) Observational evidence for soil-moisture impact on hot extremes in southeastern Europe Nat Geosci 4:17-21 doi:10.1038/ngeo1032 Huntington TG, Billmire M (2014) Trends in Precipitation, Runoff, and Evapotranspiration for Rivers Draining to the Gulf of Maine in the United States Journal of Hydrometeorology 15:726-743 doi:10.1175/jhm-d-13-018.1 Koenker R, Bassett G (1978) REGRESSION QUANTILES Econometrica 46:33-50 doi:10.2307/1913643 Li MX, Ma ZG, Niu GY (2011) Modeling spatial and temporal variations in soil moisture in China Chinese Science Bulletin 56:1809-1820 doi:10.1007/s11434-011-4493-0 Meng L, Shen Y (2014) On the Relationship of Soil Moisture and Extreme Temperatures in East China Earth Interactions 18 doi:10.1175/2013ei000551.1 Xu JX (2015) Complex response of runoff-precipitation ratio to the rising air temperature: the source area of the Yellow River, China Regional Environmental Change 15:35-43 doi:10.1007/s10113-014-0617-9