Phenolic Assays: What do the Numbers Mean? James A. Kennedy Department of Viticulture and Enology California State University, Fresno Wine Flavor 101C The Impact of Phenolic Management on Wine Style Options February 15, 2013 Davis, CA Outline • Phenolic compounds – General wine phenolic composition – Specific compounds in grapes/wine and importance • Analyzing for phenolics – Non-specific – Specific – Combination • Using analytical information – Fruit development – Fermentation/Maceration – Aging • Future trends Wine Composition-Phenolics Waterhouse, A., Ann. N.Y. Acad. Sci. 2002, 957:21-36 Volatile Phenols 4-ethylphenol • Low molecular weight, volatile • Associated with Brettanomyces sp. Infections – 4-ethylphenol (4-EP), 4-ethylguaiacol (4-EG) – Increase in proportion of 4-EG related to spiciness – >500 g/L generally detectable, 3000 g/L high Brett. • Smoke tainted wines – Guaiacol, 4-methylguaiacol, 4-EP, 4-EG – Glycosides (non-volatile) also present • Analyzed by GC-MS or HPLC • Concentrations – Clean wine: not detectable – Problematic wines: free guaiacol >200 g/L Hydroxycinnamic Acids t-caftaric acid • Present in all wines (present in the mesocarp) • Produced as tartaric acid esters • Major hydroxycinnamic acid ester is trans-caftaric acid ester • Tartaric acid portion hydrolyzed over time • Vicinal dihydroxy phenol susceptible to oxidation – Glutathione adduct of caftaric acid (GRP) can provide information on oxidation of must/juice • Useful for white wine production • Involved in white wine color Stilbenes t-resveratrol • Belong to a group of compounds called phytoalexins (antimicrobials) – Upregulated in grapes in response to fungal infection • • • • trans-resveratrol most abundant Glycosides (piceids) and polymers (viniferins) also found Provides indication of “rot” presence Some monitor for labeling purposes – “wine and health” Catechins • Other names: (-)-epicatechin – flavan-3-ol monomers, (+)-catechin, (-)-epicatechin • Almost exclusively seed-derived • Ratio of [catechin] to [tannin] can provide information on relative seed extraction • High concentrations suggestive of bitterness • Concentration declines with fruit maturity – Amount relative to extractable tannin concentration also declines Flavonols quercetin • Present as glycosides in grape, partially cleaved in wine • Concentration in grapes provides information on fruit exposure – Indirectly related to exposure and flavor • Concentration in wine indicates skin extraction (can be useful in white wine production). • Poorly soluble in wine – Low color and low tannin wines, with high flavonol concentrations are prone to physical instability (e.g.: Sangiovese) Anthocyanins malvidin-3-glucoside • Responsible for initial color in red wine • Higher concentrations associated with darker red wine • Several equilibrium forms – pH sensitive – Colored and non-colored forms – Red form is not the major component Tannins • Other names: – Proanthocyanidins, procyanidins, prodelphinidins, condensed tannins, leucoanthocyanidins • • • • • • Responsible for astringency in red wine procyanidin B2 Found in skin, seed, pulp and stem tissue Pulp tannin generally not present in wine Stem tannin present only when extracted Concentration related to perceived astringency Lower molecular weight tannins (less than 600 MW) considered bitter • Considered to be essential for long term color stability in red wine. Pigmented Tannin • Other names: – Pigmented polymer, polymeric color, polymeric anthocyanins • Stable form of red wine color • Generally thought to be a softening component of red wine astringency Other Phenolic Products • Generally of interest from mouthfeel and color stability standpoint. • Active area of research – Structure identification – Sensory relevance oxidation products vitisin A acetaldehyde – vitisin B decarboxylated hydroxycinnamic acids – pinotins vinylcatechin-vitisin A - portisins For phenolic analytical information to have value, results should relate (directly or indirectly) to perception. Analyses and Maturity/Management • White Wines – Grapes • Flavonols • Smoke taint • Catechin/tannin – Fermentation/Maceration • GRP/caftaric • Catechins (solids contact) • Polymer at 360 nm – Aging • Red Wines – Grapes • • • • • Catechin/tannin Flavonols Anthocyanins Phenolic extractability Smoke taint – Fermentation/Maceration • Catechin/tannin • Anthocyanins/Pigmented tannin • Tannin – Aging • • • • Flavonols (phys. stability) Anthocyanins/Pigmented tannin Tannin Volatile phenols Analytical Methodology - non specific • UV/Vis absorbance spectrophotometry – – – – Relates absorbance information to phenolic composition UV/Vis of wine at single wavelength (360, 420, 520, 620 nm) Folin Ciocalteu Disadvantages • With exception of red color, measurements have historically lacked specificity – Advantages • Generally rapid and cheap • Pretreatment can provide specificity (e.g.: protein precipitation) – Subsequent direct UV/Vis measurement at multiple wavelengths can provide specificity – Useful for color and tannin measurements Red Wine Absorbance Somers, 1998 Analytical Methodology - specific - • Specific phenolic compound(s) are separated from the matrix and quantified • Volatile phenols: gas chromatography – 4-EP, 4-EG . . . • Non-volatile phenols: HPLC – Hydroxycinnamic acids – Flavonoids • Advantages – Excellent specificity • Disadvantages – Expensive Phloroglucinol-Subunit Adduct Analysis OH OH O OH (+)-catechin OH OH OH HO OH OH O OH (-)-epicatechin OH OH OH OH OH OH HO OH O OH OH (-)-epigallocatechin OH OH HO OH OH OH O OH (-)-epicatechin-3-O-gallate OH O OH OH O HO OH OH OH OH Kennedy and Jones, J. Agric. Food Chem., 2001 Skin Proanthocyanidins Seed Proanthocyanidins 400 Day 4 300 200 100 51% Skin 54% Skin 51% Skin 50% Skin 53% Skin Proanthocyanidin concentration (mg/L) Proanthocyanidin concentration (mg/L) Berry Integrity: Skin and Seed Tannin Extraction 0 Skin Proanthocyanidins Seed Proanthocyanidins 400 300 200 100 45% Skin 71% Skin 54% Skin 20 40 60 80 100 0 20 40 Skin Proanthocyanidins Seed Proanthocyanidins 400 79% Skin 73% Skin 72% Skin 300 60 80 100 % Crushed berries 200 59% Skin 50% Skin Day 9 0 Proanthocyanidin concentration (mg/L) % Crushed berries Proanthocyanidin concentration (mg/L) 69% Skin 61% Skin 0 0 100 Day 5 Skin Proanthocyanidins Seed Proanthocyanidins 400 56% Skin 63% Skin 55% Skin 53% Skin 300 51% Skin 200 100 Day 17 0 0 20 40 60 % Crushed berries 80 100 0 20 40 60 80 100 % Crushed berries Cerpa-Calderon and Kennedy, J. Agric. Food Chem., 2008 Wine Analysis: Using HPLC-Based Data catechin tannin polymeric anthocyanins total catechin anthocyanins tannin ratio A 23 Oct 6 799 51 1097 0.01 B 25 Oct 7 621 32 1128 0.01 1 Nov 19 1072 51 944 0.02 24 Oct 35 390 23 925 0.09 26 Oct 70 888 39 1003 0.08 1 Nov 92 1313 58 809 0.07 C 10 Brix Combination • Combines simplicity of UV/Vis absorbance, with specificity • Has been very useful in assessing tannins in red wine • Measurement based upon precipitating tannins from solution and measuring absorbance of wine before and after precipitation – Measurement of absorbance at multiple wavelengths • Relating to precipitation has resulted in correlation of UV/Vis absorbance information to tannin concentration – – Enartis/Vinquiry: MCP Wine X-ray: A-H 22 23 Your samples Comparison samples 24 Tannin: Napa Valley Cabernet Future Trends • Phenolic structure-relationships are reasonably well developed • Access to analytical information is increasing – In house: UV/Vis spectrophotometry – Analytical labs: Enartis/Vinquiry, ETS Labs, Wine Xray • Challenges – Reduce cost and increase throughput further – Astringency quality in vineyard and winery Tannin-Protein Interaction Most analytical methods measure tannin concentration/composition and use information to predict astringency Tannin Response to Temperature Barak and Kennedy, Anal. Chem., In Review Tannin Response to Temperature Barak and Kennedy, Anal. Chem., In Review Tannin: Interaction vs. Size seed skin CS2010 CS2012 Regression lines - H, kJ/mol Increasing “grippiness” 100 10 1 11.0 11.5 12.0 12.5 13.0 13.5 14.0 14.5 15.0 GPC Retention, min Decreasing Tannin Size Barak and Kennedy, Anal. Chem., In Review Acknowledgements UC Davis Anita Oberholster Linda Bisson Kay Bogart Analytical Laboratories AWRI Paul Smith Enartis Vinquiry John Katchmer ETS Labs Gordon Burns Steve Price Funding American Vineyard Foundation