Ruolo delle correlazioni superconduttive in conduttori mesoscopici: utilizzo per l’implementazione di rilevatori quantistici Francesco Giazotto NEST Istituto Nanoscienze-CNR & Scuola Normale Superiore Pisa, Italia Universita’ di Perugia 15 Aprile 2010 Collaboration J. T. Peltonen M. Meschke J. P. Pekola Low Temperature Laboratory, Helsinki University of Technology, 02015TKK, Finland Outline • Part I: Andreev reflection and proximity effect in superconducting hybrid systems – impact on the density of states • Basic concepts of electron transport in hybrid systems: AR and PE •Proximity-induced modification of the DOS • Probing the proximized DOS: experiments with tunnel junctions and STM spectroscopy • Consequences • Part II: Superconducting quantum interference proximity transistor (SQUIPT) • Theoretical behavior of the SQUIPT • Structure fabrication details • Experimental results and comparison with theory • Advantages • Future perspectives Andreev reflection in SN contacts Andreev reflection BdG equations BTK, PRB 25, 4515 (1982) Proximity effect and supercurrent Metallic contact between a normal metal and a superconductor S N S Andreev reflection Normal metal (Semiconductor) Electron-hole correlations: proximity effect S N S Superconductor Cooper pair Incident electron Reflected hole Supercurrent Andreev bound states (ABS) Proximity effect in SNS systems: basic formalism Diffusive mesoscopic N wire: quasi-1D geometry L >L >> le D = diffusion coefficient = superconducting order parameter = macroscopic phase of the order parameter ETh = D/L2 Thouless energy Usadel equations LDOS properties: LDOS N(-E) = N(E) Eg for |E| Eg Eg( = 0) 3.2ETh for >>ETh Eg( = ) = 0 Modification of the LDOS in SNS systems due to proximity effect Length and position dependence J. C. Cuevas et al., PRB 73, 184505 (2006) Phase dependence J. C. Hammer et al., PRB 76, 064514 (2007) Spatial spectroscopy of PE probed with tunnel junctions Al/Cu SN structure with tunnel probes Phase-dependence of PE probed with STM spectroscopy Al/Ag SNS proximity SQUIDs Phase-dependence of PE probed with STM spectroscopy Phase-evolution of PE Full phase-control of the minigap amplitude Experiment to theory comparison H. le Sueur et al., PRL 100, 197002 (2008) I) -tuning of specific heat: quantum control of a thermodynamic variable Electron entropy H. Rabani, F. Taddei, F. G. and R. Fazio, JAP 105, 093904 (2009); H. Rabani, F. Taddei, R. Fazio, and F. G., PRB 78, 012503 (2008) Electron specific heat II) -tuning of e-ph interaction: quantum control of relaxation T. T. Heikkila and F. G., PRB 79, 094514 (2009) Sensitivity through proximity SQUIPT: a novel quantum interferometer Active manipulation of the DOS of a proximity N metal Phase control (through magnetic flux) SQUIPT Detection (through tunnel junctions) High sensitivity for flux detection SQUIPT: fabrication details and configurations Fabrication details Shadow-mask evaporation 27 nm Al @ 25 Oxidation 4.4 mbar 5’ (tunnel junctions) 27 nm Cu @ -25 60 nm Al @ 60 (clean SN interfaces) Geometry and materials details L 1.5 m Probe width 200 nm N wire width 240 nm SN overlapping 250 nm Rt 50-70 k LG 40 pH IJ 3 A = 200 eV SQUIPT (theo): prediction of its behavior in the current-bias mode A-type configuration quasiparticle current Usadel equations SQUIPT (theo): current-voltage characteristic vs N-region DOS 2 ETh = 4 eV Low-temperature I-V characteristic /0 DOS () 3 0 1/8 1/4 3/8 1/2 /0 0.0 1/8 1/4 3/8 1/2 1 I(nA) 2 0 -23 -4.0x10 1 to V transformer 0 V 160 4.0x10 -23 (J) I = const. 0 0.0 200 V(V) 240 modulation amplitude Calculation parameters from the samples: T = 0.1 Tc Tc = 1.3 K ETh = 4 eV D = 110 cm2/s (Cu) = 200 eV Rt = 50 k SQUIPT (theo): voltage modulation and transfer function Voltage modulation V() 2.8 50 I(nA) V/ [V/0] V(V) 240 Transfer function V/ 2.4 2.0 220 1.6 0.8 1 / 0 -25 1.2 200 0 25 2 Features: • nonmonotonic behavior in I • change of concavity 3 -50 0.0 0.5 1.0 /0 1.5 Features: • nonmonotonic behavior in I • change of sign 2.0 A-type SQUIPT (exp): current-voltage characteristic vs 4 Rt = 50 k T = 68 mK Rt = 50 k T = 53 mK 3 /0 3.0 2 2.5 Theory 3 /0 0 I (nA) -1 -2 -3 2.0 -5 -300 2 1.5 -4 1 I = const. -150 0 150 300 0 1/8 1/4 3/8 1/2 I(nA) I (nA) 1 0.0 0.15 0.29 0.5 I = const. 1.0 V (V) 0 V 0.5 V 160 200 0 240 280 V (V) Coherent modulation of the N DOS 160 200 V(V) 240 A-type SQUIPT (exp): Josephson coupling in the proximity metal Rt = 50 k T = 53 mK 40 20 20 10 I (pA) I (pA) Rt = 50 k T = 68 mK 0 -20 -10 -40 -200 0 -20 -100 0 V (V) IJ 17 pA 100 200 100 V V 0 0.17 Oe A 120 m2 A-type SQUIPT (exp): voltage modulation vs theory 2.8 240 I (nA) I(nA) 2.4 3.0 V(V) 10 V Rt = 50 k T = 54 mK 2.6 2.2 1.8 2.0 220 1.6 1.2 V Change of concavity 0.8 1.4 200 0 1.0 1 / 2 exp 50-60% theory 0.6 0.2 -4 -2 0 /0 2 V 7V @ 1 nA 4 • device parameters • non ideal phase-biasing 3 A-type SQUIPT (exp): transfer function theory 50 V/ [V/0] V/ (V/0) Rt = 50 k T = 54 mK I (nA) 0.2 1.0 1.6 2.2 3.0 20 0 0 -25 -50 0.0 1 2 /0 3 V/ 30 V/0 @ 1 nA 4 Max |V /| (V/0) -20 0 25 0.5 30 20 10 0 0 1 2 I (nA) 3 1.0 /0 1.5 2.0 B-type SQUIPT (exp): voltage modulation vs and transfer function Rt = 70 k T = 53 mK I (nA) Max |V /| (V/0) 20 V Rt = 70 k T = 53 mK 3.0 2.6 2.2 V 1.8 1.4 60 40 20 1.0 1 2 I (nA) 0.6 V/ 60 V/0 @ 0.6 nA 0.2 -4 0 0 -2 0 /0 2 V 12V @ 1 nA 4 doubled response in B-type SQUIPT 3 A-type SQUIPT (exp): temperature dependence Rt = 50 k I = 1 nA T (mK) 730 618 512 452 411 376 353 313 288 Max |V /| (V/0) V 20 V Rt = 50 k I = 1 nA 244 200 123 50 40 30 20 10 54 -4 -2 0 /0 2 4 0 0 400 T (mK) change of concavity between 376 mK and 411 mK 800 SQUIPT: dissipation and flux sensitivity Power dissipation lowered Pdiss = VI 100 fW DC SQUIDS increasing the probing junction resistance 4-5 orders of magnitude smaller in the SQUIPT Ultralow dissipation cryogenic applications Flux sensitivity NEF = <V2N>1/2/|V/|1/2 NPre 1.2 nV/Hz1/2 NEF 2 10-5 0/Hz1/2 NEF 4 10-7 0/Hz1/2 with Nb (1.5 meV) and L = 150 nm SQUIPT: advantages •simple DC readout scheme, similar to DC SQUID • current- or voltage-biased measurements • flexibility in farication parameters and materials (semiconductors NWs, carbon nanotubes, graphene) • Nb or V to enhance response and operating temperature • ultralow dissipation (1-100 fW) • implementation in series or parallel array for enhanced output • implementation with S coolers to “actively” tune the working temperature SQUIPT: future perspectives (i) Short junction limit (<<ETh) Al and L = 150 nm (ii) V SNS junction SQUIPT C. Pascual Garcia and F. G., APL 94, 132508 (2009) (iii) Noise? Both theory and experiment