GEOPHYSICAL RESEARCH LETTERS, PAI,EOINTENSITY OF THE EARTH'S VOL. 16, MAGNETIC NO. FIELD 10, PAGES 1189-1192, AND K-AR DATING OCTOBER 1989 OF THE LOUCHADIERE VOLCANIC FLOW (CENTRAL FRANCE): NEW EVIDENCE FOR THE LASCHAMP EXCURSION Annick Chauvin Laboratoirede G6ophysiqueInterne,Universit6de RennesI Robert A. Duncan Collegeof Oceanography, OregonStateUniversity Norbert Bonhommet Laboratoirede G•ophysiqueInterne,Universit•de RennesI Saul Levi Collegeof Oceanography, OregonStateUniversity Abstract.We reportpaleointensityresultsof the Earth's magnetic field from a Late Pleistocene lava flow (Louchadi•re,CentralFrance),whichrecordedan intermediate geomagneticfield direction (5 sites, mean declination=114.1 ø, inclination=58.2ø, k=130, a95=6.7ø). New K- Ar agedeterminations confirmthatthisflow is contemporaneouswith the Laschampand Olby flows, and that this excursionoccurredaround45ka ago.UsingtheThellier double heatingmethod,reliablepaleointensities havebeenobtained for ten samplesfrom threedifferentsites,providingan average field strengthof 12.9 gT (+3.3). This low value and previousresultsof theLaschampexcursionfromFranceand Icelandconfirm that the Earth'smagneticfield was in an intermedlatestateduringtheLaschampexcursion. Introduction Analysesof the magneticpolaritytime scaleindicatethat reversals are essentially Poisson-distributed in time [McFadden and Merrill, 1984], first suggestedby Cox [ 1968].Thisimpliesthatmanyadditionalshort-lived polarity subchrons(or excursions)might exist in the geological record. The Brunheschron is an apparentlong period of normalpolarityin whichseveralexcursions or shortpolarity episodes havebeenreported[Champion et al., 1988].Interest in upperPleistocene excursions stemsfrom thefactthatthey shouldbe moreeasilyidentifiedat differentsitesaroundthe world,providingan opportunityfor studyingtheglobalmor- phologyof the geomagnetic field duringsuchmagneticdisturbances. In addition,geomagnetic excursions canbe valu- plagioclasesperformedby Gudrin [1983], on samplesfrom two sites (BO and BP) of the Louchadi•re flow provided similarages( 33.8 + 2.7 and 36.4 + 3.1 ka) to thoseobtained by the samemethodon samplesfrom theLaschampflow (35 + 3.0 and 33.5 + 5.0 ka) [Gillot et al., 1979]. In thispaper,we reporta moredetailedpaleomagnetic investigation and paleointensitydata from the Louchadi•re flow. New K-Ar agedeterminations showthat thisvolcanic unit is contemporaneous with the Laschampexcursion. SamplingandPaleomagnefic method A total of 41 cores were drilled ductedin vacuum(10-2 Torr).Samples withminimumsec- nallydiscovered in twovolcanicflowsof Laschamp andOlby (ChainedesPuys,CentralFrance).Becausethesetwo lava flows recordeda field directionthatis nearlyreversed,a full polarityreversalwasconsidered, andnumerous detal•edpaleomagnetic andradiomet.icstudies wereconducted o,l these two volcanic units. Recently, a paleointensitystudy has shownthat the strengthof the Earth'smagneticfield during theLaschampfeaturewasabout8gT [Roperchet al., 1988], suggesting thatthefieldwasin anintermediate stateandthat the Laschampshouldbe moreproperlyclassifiedas a geomagneticexcursion.Othertransitional directionswerealso found in the same volcanic province, notably the one at several sites of the Louchadi•re the ondaryremanences(Figure2a) and which showeda single, high Curie point above 500øC and relatively reversible thermomagneticcurves were selectedfor paleointensity experiments. ablefor stratigraphic correlations. The Laschampexcursionwasthefirst eventident:.fied in the Brunhesperiod[Bonhommet andBabkine,1967],origi- recorded at five sites within Louchadi•re flow (BP: Beauloup, BO: le Bouchet, FOU' Foug•res, BEAU: Beauregardand CHAU: Chausselles), separatedby at leastseveralkilometers(Figure 1). Two sites (BP and CHAU) were situatedin a less-oxidizedpart of the flow, while the other three comprisedmore oxidized rock and scotia. Small areas at two sites (FOU and BEAU) were clearlyaffectedby lightning,showing significantdeviations of the magneticcompass.Paleomagneticmeasurements and progressive demagnetizations by alternatingfields(AF) were performedwith Schonstedt equipment.Paleointensity determinations were doneby the originalversionof the Thellier and Thellier [ 1959] stepwisedoubleheatingmethod,where the laboratory field was applied during both heating and coolingcyclesand the field directionwas reversedbetween two heatingsat each temperaturestep.Heatingswere con- Paleomagnetic results Directions ProgressiveAF demagnetization of the naturalremanent magnetizations (NRM) indicatedtwo kindsof overprints:(1) a viscouscomponent(VRM) in the directionof the present day field and (2) a secondarycomponentwith shallowinclinationsand scattereddeclinationsfor samplesat the edgesof the areasaffected by lightning. However, several samples have NRM flow directions close to the characteristic direction (Figure 2a). Samplescarrying a viscouscomponenthave [Bonhommet,i972]. Thermoluminescence dating (TL) on NRMintensities typically between 1to5 Am-1andaremostly from sitesCHAU and BP. Samplesaffected by lightning Copyright 1989 by the American Geophysical Union. have much higher NRMintensities (upto30Am'l). Samples Paper number 89GL02916. 0094-8276/89/89GL-02916503.00 for which the strongmagneticoverprintwasnot completely removedduringAF demagnetization wereomittedin calculating thecharacteristic meansitedirections. 1189 1190 Chauvinet al.' Geomagnetic Paleointensity at Louchadi•re TABLE Volcano 53' 1. Site mean directions 45 ø 51' FOU .' CHAU Flow I nøuchadi/•re ! I Sites n/N D (o) I (o) k et95 Fou Beau Chau BP 130 6/10 8/11 5/6 6/8 6/6 119.0 123.1 102.3 109.8 117.0 Mean 5 114.1 Lat Long 62.8 59.3 62.3 48.6 57.2 130 84 107 75 237 5.9 6.1 7.4 7.8 4.4 15.0 9.9 22.8 8.5 10.9 43.4 43.5 53.0 58.8 48.7 58.2 130 6.7 13.2 49.8 n/N: nmnberof samplesusedin the meancalculation/measured Fig. 1. Locationmap and samplingsites(BO, BEAU, FOU, BP and CHAU) of the Louchadi•reflow, Chainedes Puys, parameterestimate,{x95:95% confidenceconeaboutthe mean; France. Lat, Long:latitudeandlongitudeof thevirtualgeomagnetic pole. N N ß ß (a) ß + .e o + ee W +30 (b) o 4•60 '+ß++*•..+ ++ eS• ß + s s Fig. 2. a) Stereographic projectionsof NRM directionsof all samplescollectedfrom the Louchadi•reflow. Solid symbols (open symbols) are on the lower (upper) hemisphere. Diamondsare the directionsof the samplesselectedfor the paleointensity determinations. b) Mean directionper si•esand {x95confidencecones,after af andthermalcleaning.The star represents the dir•tion of the axial dipolefield. The averagedirectionof thecharacteristic magnetization at eachsiteis reportedin Table 1 and shownin Figure2b. The mean direction of the flow (D= 114.1ø, I= 58.2 ø) shows a large departure(42ø) from the axial dipole field and a low VGP latitude (13.2ø). Paleointensity Eleven samplesfrom three sites(FOU, BEAU anJ BO) wereusedfor paleointensity experiments. They were sel•ted on the basisof havingminimumoverprint(Figure 2a), high Curie points, and good reversibility between heating and coolingin thermomagnetic tests.Strongfield thermomagnetic experimentson samplesfrom sitesBP and CHAU indicated low Curie temperaturesdue to the relatively low oxidation state of the Ti-rich titanomagnetites.Becausethis type of mineralogyoftenlead to mineralogicalchangesduringheating, no samplesfrom thesetwo siteswere selected.During the Thellier experiment,the sampleswere treatedin various applied fields: 10, 15 and 20 gT. Numerouspartial thermoremanentmagnetization(TRM) checkswereperformedin order to test the stability of TRM acquisitionduring the heating[Pr6votet al., 1985]. Among the elevenselectedsamples,only one did not provide a paleointensity resultdueto a drasticdecreasein the capacity of TRM acquisitionat temperaturesabove 410øC. Table 2 summarizesthe paleointensityresults.From each site,oneexampleof an NRM-TRM diagram andevolutionof the NRM vector during the heatingare shownin Figure 3. samples; D, I: meandeclinationandinclinationpersite;k: precision Althoughcoreswith large overprintswere avoided,samples selectedfor paleointensity measurements werenot completely free from small secondary¾RM components.However, thesesecondarymagnetizationswere commonlyremovedat temperaturebetween200 and 350øC.With the exceptionof sample Beau-06a which is from a core that broke during drilling, the NRM directions,in the temperatureintervalused for paleointensitydeterminations,are similar to thosedeterminedby AF demagnetization. At least 9 to 10 steps,and a large fraction of the NRM, were usedto determinethepaleointensity. The qualityfactor q and the standarderror for single sampledeterminations were calculatedfollowing the statisticalmethoddevelopedby Coe et al. [1978]. The weightedaveragepaleointensity of the flow was obtainedusing the weightingfactor proposedby Pr6vot et al. [ 1985]. The maximum error that CRM acquisition might have caused,in percentof the laboratoryf':eld,is indicatedby the index R (Table 2), as definedby Coe et al. [ 1984]. For our data,thisindexis typicallylessthan 10%. The paleointensityresultsrange from 11 to 15 gT, with only one determination,(22 gT, sampleBO-01), out of this range. BO-01 has the lowestquality factor of all our specimens,soits contributionto the weightedmeanis least.•.mportant. The unweightedmean intensityof the flow is 17.9 gT, and the weightedmean [Pr6votet al., 1985] consideredto be thebestestimateof thepaleointensity of the Louchadi•reflow is 12.9 gT. This resultis one third to onequarterthe strength of thepresentday field. The virtualdil•olemoment(¾DM) associated to thisflow is 2.2 1022Am2, whichis considerably less than the averageVDM obtainedfor the last 10 ka [McElhinny and Senanayake, 1982] or the last 5 m.y.[McFadden and McElhinny, 1982], which is about 8.7 1022Am2. Dating K-Ar radiometricagedetermination from samples fromsite BP providesan age (42 + 4 ka, Table 3) slightlyolderthan thosedeterminedby thermoluminescence [Gu6rin,1983]. A 40Ar-39Ar incremental heatingexperiment yieldeda poorlyconstrained plateauageof 39+28 ka. The agedeterminedby K-Ar is also very similar to new measurements'•n the LaschampandOlby flows (Table3). A goodinter-laboratory consistency betweenthesenewK-Ar dataandthoseobtained 'for Laschamp andOlby samples[Gillotet al., 1979;Hall and York, 1978] is observed.Significantagedifferencesseemto occur betweenresultsobtainedby TL and K-Ar methods, rather than between three different volcanic units. Discussion Another volcanic unit in the Chaine des Puys, the Royat lava, recorded a magnetic direction (D=284.7ø; I=68.2 ø) which deviatessignificantlyfrom normal secularvariation. Chauvinet al.: Geomagnetic Paleointensity at Louchadibre 1191 TABLE 2. Paleointensity results Samples Beau-02a Beau-06a Bo-01a Bo-02a Bo-03a Bo-250a Bo-252a Fou-03a Fou-04a Fou-05a D(ø) 145.0 104.0 110.5 111.5 117.0 123.0 126.5 108.0 113.0 110.0 I(ø) 60.0 86.0 57.5 54.5 64.0 53.0 58.0 59.5 63.0 60.5 N Hlab JNRM 10 10 9 15 11 11 10 10 10 10 10 15 20 10 15 10 10 20 10 10 4.4 3.8 1.4 1.5 2.0 2.2 1.2 2.2 1.9 4.2 370-530 200-500 350-515 250-550 250-520 350-540 300-510 350-525 300-510 200-500 f g q 0.700 0.672 0.419 0.891 0.697 0.701 0.533 0.704 0.724 0.914 0.868 0.854 0.860 0.908 0.860 0.879 0.860 0.883 0.873 0.863 36.4 8.4 7.7 30.3 12.1 28.9 14.9 61.8 36.0 19.0 r 0.998 0.981 0.992 0.995 0.989 0.998 0.996 0.999 0.998 0.993 R% Fe+sFe 18.6 3.4 11.5 1.9 2.6 10.3 7.9 3.2 3.6 3.5 11.0+_0.2 13.5+_0.9 22.4+_1.0 15.1_+0.4 15.5+0.8 11.2+-0.3 12.1+-0.4 12.3+_0.1 12.7+0.2 13.35:0.5 VDM = 2.2 x1022Am 2 <Fe> = 12.9 Mean: Fe q-s.d.= 13.9 !xT+-3.3 AT D, I: magneticdeclination andinclinationof theNRM left in theAT temperature interval;N: numberof temperature stepsin the AT interval; Hhb: laboratory field(in!.tT); JNRM: initial intensity ofmagnetization inAm-1'AT:interval oftemperature used tocalculate thepaleointensity; f, g, q: NRM fractionused,gapfactorandqualityfactorrespectively [Coeet al., 1978];r: linearcorrelation coefficient;R%: maximunpercentage of CRM; Fe: paleointensity estimatefor individualspecimen in !xT;sFe:standarderror,Fe+-s.d.: unweighted averagepaleointensity of theLouchadiirelavaflow plusor minusits standard deviation;<Fe>: weightedmeanin !xT. NRM TABLE 3. K-Ar Ages Up N 1A/m •1• BEAU-02A •zo iwn ONRM o N BO-03A 52 ' 1A/m Down 1 NRM 250• NRMo TRM N "• .• FOU-03A525•• E 'own I 1 40At* %40At* Age:!:1o (x10 -13mole/g) (ka) Laschamp Olby 1.857 1.733 1.578 1.148 2.8 1.8 49.0+-6.7 38.2+_6.3 Louchadi•re 1.677 1.213 3.0 41.7+_3.9 Decay andabundance constants usedin agecalculations: •,e=0.581x10-10 yr-1,•,[5=4.962x10-10yr-1, 40K/K=l.167x10 -4 TRM NRM 1 %K mole/mole, 40Ar*:Radiogenic 40Ar I 1 LavaFlow TRM Paleointensity determinations,performed by the Thellier methodon sedimentsbakedby the Royat flow [Barbettiand Flude, 1979], suggesta low field closeto 15 I.tT. The Royat flow has been dated by TL at around 40-46 ka [Gu6rin, 1983]. Thus the Royat flow may have been eruptedat the time of the Laschampexcursion. The globalor regionalextentof the Laschampexcursionis not, well defined.The only excursionrecordedin lavascorrelated with Laschampis in Iceland (D=258.0 ø, 1=-15.0ø) [Kristjanssonand Gudmundsson,1980]. Palcointensitydeterminationsby the ThelEermethodhave beenperformedby two groups and provide paleofields as low as 4.3 gT [Marshall et al., 1988] and 4.2 gT [Levi et al., 1989]. K-Ar radiometricage determinationsshow that theseflows were eruptedaround40-50 ka and suggestcontemporaneitywith the Laschampexcursion[Levi et al., 1989]. (A reverseddirection recorded in welded tuffs in Japan [Tanaka and Tachibana,1981], was originallydatedat around30 ka, and was first correlatedwith the Laschampexcursion.New dating of the tuff givesan agearound0.7 Ma, showingthat the reversed direction was probably acquired during the Fig. 3. Examplesof reliable paleointensitydeterminations (NRM-TRM diagrams),for 3 samplesfrom the sitesBEAU, BO, and FOU. Black dots are used to calculatethe slope; trianglesrepresentPTRM checks;the associated orthogonal vector plots of the thermaldemagnetizationof the NRM are shownin geographical(in situ) coordinateson the right of eachNRM-TRM plot.Temperature stepsareindicatedin øC. 1192 Chauvinet al.' GeomagneticPaleointensity at Louchadibre Matuyama period [Tanaka, 1988, personnalcommunication]).A very well definedintermediate direction(D= 101.1ø, I= -36.1o) wasrecentlymeasured at 63 sitesof 8 distinctlava flows of the AlbuquerqueVolcanos (New Mexico, USA) [Geissmanet al., 1989]. Preliminary K-Ar age determinationssuggestlatestPleistocene (i.e. 20 to 100ka) asthe time of theextrusion.More preciseagedeterminations arerequired priorto moreexactcorrelation withproposed LatePleistocene excursions. Three modelshave been appliedto explain geomagnetic excursions:(1) a dramaticchangein directionof the dipole field; (2) a large increasein strengthof non-dipolesources; and(3) a decreasein strengthof themaindipolefield causing non-dipoledominationoverlargerportionsof theglobe.The last hypothesiswasrecentlyusedin orderto interpretdirectionsandlow paleointensities obtainedon the Laschampand Olby flows [Roperchet al., 1988]. The low paleointensity value observedat Louchadi•rereinforcesthis interpretation. For example,a dipoleonly one fourthof the presentvalue with non-dipole fields of the same order as presentnondipolefield valuescan produceregionalintermediatedirections.We may speculatethat sucha decreasein the dipole field mighthavebeena first stepin an attemptedandfinally abortedpolarityreversal. Acknowledgments. The authorsare gratefulto P. Roperch for his help throughoutthis study.Financial supportfrom INSU (France)and NSF are acknowledged. References Barbetti, M. and K. 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Turrin and of the Laschampexcursion.In pressEarth Planet. Sci. Lett. , (ReceivedApril 3, 1989; acceptedSeptember1, 1989)