Infinite Randomness Fixed Point of the disordered Mott transition? Eric Castro Andrade1,2 E. Miranda1 Vlad Dobrosavljević2 1Campinas, Brazil 2Florida State University FL, U.S.A. REVIEW: Reports on Progress in Physics 68, 2337–2408 (2005) Disorder and QCP: The Cold War Era (1960-1990) Criticality and Collectivization There is not, nor should there be, an irreconcilable contrast between the individual and the collective, between the interests of an individual person and the interests of the collective.” (Joseph Stalin) Collectivization: Theory Long wavelength modes rule! Ken Wilson’s RG GRIFFITHS singularities, Harris criterion: “Weak” disorder corrections Trouble Starts (circa 1990) Dissidents run away over the Berlin Wall Weak coupling RG finds run away flows for QCPs with disorder (Sachdev,...,Vojta,...) Quantum Griffiths phases and IRFP (1990s) • D. Fisher (1991): new scenario for (insulating) QCPs with disorder (Ising) T clean phase boundary Griffiths phase (Till + Huse): ordered phase g Griffiths phase P(L) ~ exp{-ρLd} P(Δ) ~ Δα-1 ; χ ~ Tα-1 α → 0 at QCP (IRFP) Rare, dilute magnetically ordered cluster tunnels with rate Δ(L) ~ exp{-ALd} E.Miranda, V. Dobrosavljevic, Reports on Progress in Physics 68, 2337 (2005) How generic is IRFP? Quantum insulating magnets + disorder (D. Fisher et al.) • Ising (and other discrete symm.) models – YES • Heisenberg (and other continuous symm.) – NO More recently (2003-2008) Dissipative (itinerant?) magnets + disorder • Ising model: transition “rounding” – NO (T. Vojta, 2003) • Heisenberg (and other continuous symm.) – YES!!! (T. Vojta, J. Schmalian, J. Hoyos, 2005-2008) • Heisenberg + RKKY interactions – cluster glass – NO (V.D. and E. Miranda, 2005) Metal-Insulator Transition? • Example: Doped semiconductors Si:P,B Paalanen et al, Physica B 169, 223 (1991) Uncompensated Si:P Compensated Si:P, B 2-Fluid Phenomenology • Strongly localized states dominate the spin response even in the metallic state. Spin and charge seem to decouple. insulator M. J. Hirsch et al., PRL 68, 1418 (1992) metal Two transitions? • Possible phase diagram Fermi-liquid metal (T=0)=o Non-Fermi-liquid metal (T=0)= Insulator MIT Disorder • Previous studies: – (Milovanović, Sachdev, and Bhatt, PRL 63, 82 (1989)) Mean-field theory of the disordered Hubbard model • Shows localized magnetic states in the presence of delocalized singleparticle states. • The mean-field theory (Anderson, 1962) is known to break down at low T due to the Kondo effect: need to describe the scales at which this occurs? – R. N. Bhatt and D. S. Fisher, PRL 68, 3072 (1992): Kondo vs. RKKY; non-Fermi liquid behavior, divergent thermodynamics slower than any power-law: need quantitative calculation (fluctuations of the density of states). Incorporating the Kondo effect • Statistical Dynamical Mean Field Theory (Kotliar and Dobrosavljević, PRL 78, 3943 (1997)): assume local (though spatially non-uniform) self-energiesEach local site is governed by an impurity action: Local renormalizations : hybridization to the neighboring sites Physics content of statDMFT • Treat each impurity action within the Gutzwiller approximation (PRL 10, 159 (1963)); equivalent to the Kotliar-Ruckenstein slave boson formalism (PRL 57, 1362 (1986)). • Clean case (W=0): Mott metal-insulator transition at U=Uc, where Z (Brinkman and Rice, 1970). • Fermi liquid approach in which each fermion acquires a quasiparticle renormalization and each site-energy is renormalized: Results in d=∞ (D. Tanasković et al., PRL 2003; M. C. O. Aguiar et al., PRB 2005) • For U Uc(W), all Zi vanish (Mott transition) like in the clean case (Brinkman and Rice, PRB 2, 4302 (1970)). • If we re-scale all Zi by Z0 ~ Uc(W)-U, we can look at P(Zi /Z0) • In the limit of infinite coordination (dynamical mean field theory), P(Z/Z0) tends to a universal form at Uc. Z0 gap Results in d=2 (E. C. Andrade, Eduardo Miranda, V. D., PRL, 2009) • In low dimensions, the environment of each site (“bath”) has strong spatial fluctuations • New physics: rare evens due to fluctuations and spatial correlations DMFT However, in d=2, the distribution P(Z/Z0) acquires a low-Z tail: Results: thermodynamics • Remembering that the local Kondo temperature and Singular thermodynamic response The exponent is a function of disorder and interaction strength. =1 marks the onset of singular thermodynamics. Quantum Griffiths phase (see, e.g., E. Miranda and V. D., Rep. Progr. Phys. 68, 2337 (2005); T. Vojta, J. Phys. A 39, R143 (2006)) Phase diagram (W<U) Ztyp = exp{ < ln Z> } Infinite randomness at the MIT? • Most characterized Quantum Griffiths phases are precursors of a critical point where the effective disorder is infinite (D. S. Fisher, PRL 69, 534 (1992); PRB 51, 6411 (1995); ….) Compatible with infinite randomness fixed point scenario -1 – variance of log(Z) Quantum Griffiths phases and IRFP • D. Fisher (1991): new scenario for (insulating) QCPs with disorder (Ising) T clean phase boundary Griffiths phase (Till + Huse): ordered phase g Griffiths phase P(L) ~ exp{-ρLd} P(Δ) ~ Δα-1 ; χ ~ Tα-1 α → 0 at QCP (IRFP) Rare, dilute magnetically ordered cluster tunnels with rate Δ(L) ~ exp{-ALd} E.Miranda, V. D., Reports on Progress in Physics 68, 2337 (2005)) “Size” of the rare events? Typical sample Rare event! Replace the environment of given site outside square by uniform (DMFT-CPA) effective medium. Reduce square size down to DMFT limit. Rare events due to rare regions with weaker disorder The rare event is preserved for a box of size l > 9: rather smooth profile with a characteristic size. U=0.96Uc;W=2.5D Size of the rare events: a movie Killing the Mott droplet Spectrosopic signatures: disorder screening • The effective disorder at the Fermi level is given by the distribution of: Width of the vi distribution This quantity is strongly renormalized close to the Mott MIT is pinned to Fermi level (Kondo resonance) Energy-resolved inhomogeneity! • However, the effect is lost even slightly away from the Fermi energy: Aspen E=EF - 0.05D E=EF The strong disorder effects reflect the wide fluctuations of Zi Similar to high-Tc materials, as seen by STM, tunneling (e.g. K. McElroy et al. Science 309, 1048 (2005)) Tallahassee U=0.96Uc;W=0.375D Generic to the strongly correlated materials? Mottness-induced contrast Conclusions and... • An electronic Griffiths phase emerges as a precursor to the disordered Mott MIT (non-Fermi liquid metal) • Strong-correlation-induced healing of disorder at low energies, but very inhomogeneous away • Infinite randomness fixed point: new type of critical behavior for disordered MIT??? • (Weak) localization vs. interactions: is there a true 2D metal in D=2???