Supercond. Sci. Technol. 13 (2000) 183–186. Printed in the UK PII: S0953-2048(00)07485-6 Temperature dependence of filament-coupling in Bi-2223 tapes: magneto-optical study A V Bobyl†‡, D V Shantsev†‡, T H Johansen†, M Baziljevich†, Y M Galperin†‡ and M E Gaevski‡ † Department of Physics, University of Oslo, PO Box 1048 Blindern, 0316 Oslo, Norway ‡ Ioffe Physico-Technical Institute, Polytechnicheskaya 26, St Petersburg 194021, Russia Received 1 September 1999 Abstract. Coupling through random superconducting bridges between filaments in a multifilamentary Ag-sheathed Bi2 Sr2 Ca2 Cu3 O10+δ tape has been investigated by magneto-optical imaging at temperatures from 20 K up to Tc . Magnetic flux distributions have been measured on the surface of an intact tape in the remanent state on applying a strong perpendicular magnetic field. The flux distributions observed at low temperatures reflect the arrangement of individual filaments. At high temperatures, the distribution becomes more similar to that for a uniform monocore tape, indicating that superconducting connections appear between the filaments. To discuss the relative contributions of the intra- and inter-filament currents, a simple model based on the Bean critical state was proposed and applied to analyse the temperature dependent behaviour. The inter-filament coupling, increasing with temperature, reaches at 77 K a point where the currents flowing in large inter-filament loops are roughly equal to the intra-filament currents. 1. Introduction There is great interest in making use of high-Tc superconducting multifilamentary tapes in power applications. An important issue concerning multifilamentary tapes is the possible presence of superconducting connections between the filaments. Such a connection may appear through formation of random inclusions of the superconducting material, making up superconducting ‘bridges’ between neighbouring filaments. On the one hand, the coupling between filaments may be useful for maintaining the current flow when it encounters a structural defect within a single filament. on the other hand, however, this also leads to a substantial increase in ac loss, important for many applications, such as power transmission lines or ac magnets. Filament bridging was observed in Ag-sheathed Bi2 Sr2 Ca2 Cu3 O10+δ (Bi-2223) tapes and its effect on the magnetization loops was analysed in [1]. For multifilamentary samples, the measured susceptibility is considerably larger than that in isolated filaments, being although somewhat smaller than the value expected for a monocore tape. Studies of ac loss in a Bi-2223/Ag tape have shown that the filaments behave as if they were connected into bundles, a typical bundle being composed of eight filaments [2]. Although the filament bridging strongly affects the magnetic properties of a tape, its existence can be established unambiguously only by space-resolved studies. Indeed, these techniques have proved to be very successful in investigations of field and current distribution in mono- and 0953-2048/00/020183+04$30.00 © 2000 IOP Publishing Ltd multifilamentary tapes [3–7]. Hall-probe measurements of the remanent state after passing a transport current [5] and magneto-optical (MO) imaging at various applied fields [4] have both revealed the existence of superconducting bridges between filaments in Bi-2223/Ag tapes. In the present work we used the MO imaging method to investigate the temperature dependence of filament coupling. Since there are different mechanisms limiting the current inside individual filaments and the current leaking through the random superconducting interconnections, one would expect different temperature dependences of the corresponding critical currents. In order to separate the two contributions experimentally we constructed a model which can be fitted quantitatively to the MO images. Good agreement is achieved over a wide range of temperatures which allows the behaviour of both the intra- and inter-filament critical currents to be determined. 2. Experiment The object of study was a 55 filament Bi-2223 tape, prepared by the powder-in-tube method with subsequent drawing and rolling [8]. The tape width, including the Ag sheath, was 3.7 mm; the critical current was 45 A at 77 K. An optical image of the tape cross section is shown in figure 1(a). MO images of the magnetic field distributions were taken using a Faraday-active Bi:YIG indicator film with in-plane magnetization. The indicator, grown by liquid phase epitaxy 183 A V Bobyl et al (a) 15 (b) 10 19 K 41 K 57 K 62 K 69 K 76 K 80 K 86 K 93 K 102 K 108 K 5 B (mT) (c) 0 Figure 1. (a) Optical image of the tape cross section, with superconducting filaments appearing black. The arrows point to three filaments located near the tape surface, see the text. Magneto-optical images showing trapped flux (Ba = 0) in the tape after applying a large field at 19 K (b) and at 108 K (c). The images were taken with uncrossed polarizers, giving a monotonic relation between image brightness and the local flux density. Strong contrast enhancement was applied to the image (c). The stripes along the tape, clearly seen in the image (b), reflect the arrangement of the filaments. on GGG substrate, was mounted in contact with the large surface of an intact Ag-sheathed Bi-2223 tape. Details of the MO imaging technique itself are given in [9]. Contrary to the conventional procedure, we chose an angle between the polarizer and the analyser far from 90◦ . In this case the grey level in the MO images becomes a single-valued function of the flux density, i.e., the brightness grows with B, rather than with |B|. In this work we studied the remanent states obtained after applying a magnetic field of Ba = 105 mT, which much exceeds the full penetration field at all temperatures. MO images of the tape at 19 and 108 K are shown in figure 1. The major feature of the B-distribution at 19 K is a set of stripes that correspond to a particular arrangement of filaments. Secondly, the distribution also has common features with that expected for a uniform strip, namely a large peak of positive flux in the middle and regions of smaller negative flux near the edges (cf [4]). At 108 K the stripes can hardly be distinguished and the flux distribution is very close to that in a uniform strip. The flux density profiles across the tape are shown for different temperatures in figure 2. The peaks in the profiles correspond to the bright stripes in the MO images. It is evident that the remanent state flux distribution is strongly temperature dependent. Firstly, and quite as expected, the trapped flux decreases with increasing temperature owing to reduced pinning at elevated temperatures. Secondly, we notice a less obvious feature, namely that the profiles become smoother at higher temperatures. To reveal the loss of fine structure more clearly, we can focus on the region −0.9 (mm) < x < 0. At low temperatures one finds three distinct peaks in B profiles. As the temperature increases, the two minor peaks gradually vanish and finally disappear at 70 K. The three peaks coincide in space with three individual filaments near the tape surface (see arrows in figure 1(a)). Thus, we are confident that the peaks originate from current loops within these filaments. When the peaks vanish from the 184 −5 Tape −10 −0.5 0.0 x (mm) 0.5 1.0 Figure 2. Experimental profiles of the flux density in the remanent state on removing a strong field at different temperatures. The profiles are obtained from MO images as in figure 1(b, c) by averaging grey levels over a 100 µm band across the tape. The band is shown under the profiles. As the temperature increases, there occurs (i) a decrease of the trapped flux, and (ii) smoothening of the flux profiles. flux profile, this may only be due to changes in the current flow pattern, our configuration being fixed mechanically. We assign the merging of the three flux maxima into one broad peak to the creation of inter-filament current loops at elevated temperatures. Therefore, our conclusion is that there exists a temperature dependent redistribution of the intra- and interfilament currents in the tape. 3. Model We propose a simple model to describe the observed redistribution of currents. Individual filaments are considered to be thin infinite strips, while the inter-filament coupling is described by an additional (fictitious) wide strip. The positions and widths of the thin strips are taken from the optical image, figure 1(a). The position and width of the wide strip are determined from the B-profile at the highest temperature, where the inter-filament currents appear to be dominant. The spatial arrangement of the strips is shown in figure 3 and also specified quantitatively in table 1. We assume that all the strips behave according to the Bean model for a fully-penetrated remanent state, i.e., the critical current flows along the strip so that +Jc and −Jc are the current densities in each of its halves. We allow different critical current densities, Jcintra and Jcinter , for the narrow strips and additional wide strip, respectively. The latter is the critical current limiting the transport between the filaments, and, in general, one expects it to be different from Jcintra . Temperature dependence of filament-coupling in Bi-tapes: MO study Table 1. Widths and centre positions of the strips used in T = 108 K 0.2 modelling, see also figure 3. The origin of the x-axis is chosen as in figure 2. The strips 1–3 correspond to real filaments, and their dimensions are taken from the optical image of the tape, figure 1(a). The wide strip, 4, models the inter-filament coupling. 0.0 Number w (mm) xc (mm) −0.2 1 2 3 0.15 0.09 0.11 8 −0.79 −0.46 −0.09 4 0.6 −0.37 B (mT) 6 T = 57 K 4 2 0 15 T = 19 K 10 5 0 −1.0 −0.8 −0.6 −0.4 x (mm) −0.2 0.0 Figure 3. Experimental profiles (symbols) of the flux density across the tape at three temperatures. Full curves are fits by the model (2) which assumes a fully penetrated state of the filaments. The positions of the filaments are sketched at the bottom, and specified in more detail in table 1. The fitting parameters are the two critical sheet currents, Jcinter and Jcintra . very different temperatures. It is evident that our modelling successfully reproduces the important features of the flux profile variation. Some deviation between the fitting curves and the measured flux profiles can be assigned to the effect of the field trapped in the remaining filaments of the tape. The pronounced variation in the B-profiles with temperature leads to quite different temperature dependences of the fitting parameters Jcinter and Jcintra , as shown in figure 4. At low temperatures, the intra-filament critical current far exceeds the inter-filament current. This would be expected since in this temperature range the current transport through random interconnections between filaments is severely limited by weak links. At higher temperatures, however, Jcintra becomes very small, and essentially all the current flows in large inter-filament loops. These loops consist of filaments and interconnections, both having the same critical current Jcinter . This result is consistent with the observation that in Bi-2223 the depinning critical current decreases with temperature much more rapidly than the critical current through weak links does [10]. At 77 K, the operating temperature for most tape applications, Jcinter ≈ Jcintra . Hence, at this temperature the currents flowing in the large inter-filament loops are roughly equal to the intra-filament currents. Moreover, larger current loops obviously give larger contribution to ac From the Biot–Savart law it follows that the field distribution at a distance h above such a strip of width 2w is given by B(x) = Jc F (x, w) where 2 x 2 + h2 µ0 (1) ln F (x, w) = 4π (x + w)2 + h2 (x − w)2 + h2 50 with Jc the critical sheet current, and x the coordinate across the strip with x = 0 in the centre. The total field generated by currents in all the four strips is 30 B(x) = Jcintra inter-filament 40 Jc (kA m−1) 3 X intra-filament 20 F (x − xci , wi ) + Jcinter F (x − xc4 , w4 ) (2) i=1 where wi and xci are the strip widths and centre positions, respectively. Equations (1) and (2) were fitted to the experimental flux density profiles in the range −0.9 (mm) 6 x 6 0. The height h was chosen to be 0.17 mm, which is the separation between the MO indicator film and the top layer of filaments, the distance primarily defined by the silver sheath thickness. For each temperature the B-profile was fitted with two free parameters, Jcinter and Jcintra , using the least-squares method. The result of the fitting is shown in figure 3 for three 10 0 0 20 40 60 T (K) 80 100 Figure 4. Temperature dependence of the critical currents, Jcinter and Jcintra corresponding to inter- and intra-filament current loops, respectively. The data were obtained by fitting (2) to experimental flux density profiles. 185 A V Bobyl et al loss. Therefore, at 77 K losses due to inter-filament current even dominate over intra-filament losses. 4. Conclusion Magneto-optical imaging shows directly the existence of superconducting interconnections between filaments in multifilamentary Bi-2223/Ag tape. Using a Bean-model approach, we have extracted from such observations the temperature dependences of the intra-filament and interfilament critical currents. It is shown that the relative strength of inter-filament coupling grows steadily as the temperature is raised from 20 K to Tc . At the highest temperatures, the interfilament current becomes the dominant current component. Acknowledgments We thank P Vase (NST, Brøndby, Denmark) for sample preparation. 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