APPLIED PHYSICS LETTERS 98, 151107 共2011兲 A half wave retarder made of bilayer subwavelength metallic apertures Z. Marcet,1,2 H. B. Chan,2,a兲 D. W. Carr,3 J. E. Bower,4 R. A. Cirelli,4 F. Klemens,4 W. M. Mansfield,4 J. F. Miner,4 C. S. Pai,4 and I. I. Kravchenko5 1 Department of Physics, University of Florida, Gainesville, Florida 32611, USA Department of Physics and William Mong Institute of Nano Science and Technology, The Hong Kong University of Science and Technology, Clear Water Bay, Kowloon, Hong Kong 3 Symphony Acoustics, Rio Rancho, New Mexico 87124, USA 4 Bell Laboratories, Alcatel-Lucent, Murray Hill, New Jersey 07974, USA 5 Center for Nanophase Materials Sciences, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37830, USA 2 共Received 26 January 2011; accepted 27 March 2011; published online 13 April 2011兲 We demonstrate a half wave plate whose principle of operation is based on the strong evanescent field coupling between two metal layers with arrays of subwavelength slits. The device is divided into two kinds of pixels in which the slits are oriented in orthogonal directions. By tuning the phase delay of the transmitted light through the lateral displacement between the top and bottom layers, the polarization of linearly polarized light at 1.55 m can be rotated by up to 90°. The polarization extinction ratio of the transmitted light exceeds 22 dB. © 2011 American Institute of Physics. 关doi:10.1063/1.3579245兴 Nano optical devices exploit the interaction between near field and far field radiations in subwavelength metallic and dielectric structures to achieve novel optical capabilities. For example, the excitation of surface plasmons is responsible for the remarkable transmission1 and beaming properties2 of periodic subwavelength metallic apertures. The subwavelength features on the metal surface can be engineered to control the strong evanescent fields associated with the surface excitations.3 Here, we describe the fabrication of a half wave plate where the retardation in one polarization is achieved through tailoring the evanescent field coupling between two metal layers with arrays of subwavelength apertures. Polarization state controllers are essential components in optical systems. Conventional wave plates rely on birefringent crystals to impart a phase delay to one of the polarizations. The wavelength of operation is determined by the material properties and therefore is not readily tunable. Moreover, it is challenging to integrate them with other optical components due to their bulkiness. Alternative ways to control the polarization have recently emerged, including liquid-crystals,4–6 waveguides,7–10 micromechanical devices,11,12 and chiral metamaterials.13 In particular, chiral metamaterials offer a compact, planar platform to rotate the polarization of transmitted or reflected light. However, the difficulty in generating strong optical activity has limited the polarization azimuth rotation to ⬃30°.14 The device reported here is a half wave retarder based on the enhanced transmission through bilayer subwavelength metallic slit arrays at resonance. By utilizing the controllable phase delay of the transmitted light through the lateral displacement of the two arrays and the strong dependence of the transmission on the polarization of the incident light, the polarization of linearly polarized light at 1.55 m can be rotated by up to 90° in the zero order transmission. The polarization extinction ratio of the transmitted light exceeds 22 dB. a兲 Electronic mail: hochan@ust.hk. 0003-6951/2011/98共15兲/151107/3/$30.00 Our sample is made of two 0.2 m thick aluminum films separated by 0.34 m, each with subwavelength slit apertures arranged in specific orientations. The slits in the aluminum layers are created by reactive ion etching with a photoresist etch mask defined by deep ultraviolet lithography.15 As shown in Fig. 1共a兲, the top aluminum layer is divided into a checkerboard pattern with two kinds of square pixels. Each pixel 共25⫻ 25 m2兲 consists of an array of long slits with width of 0.49 m and periodicity of 1 m. The orientations of the slits are perpendicular to each other in adjacent pixels. For pixels labeled as type 1 in Fig. 1共a兲, the slit array is oriented along the y direction. In the bottom layer, an identical array of slits is present, almost laterally aligned to the top array 关Fig. 1共b兲兴. For type 2 pixels with slits along the x direction, the array of slits in the bottom layer is laterally shifted from the top layer by about half the period 关Fig. 1共c兲兴. The two aluminum layers are completely surrounded by silicon oxide. Fabrication of the metal layers was performed on a silicon substrate. Completed structures were then transferred onto a quartz wafer for optical measurements.15 To understand the working principle of the above structure as a half wave retarder, we first consider the transmission properties of a nonpixilated, single-layer structure with all slits oriented along the y direction. Linearly polarized light with electric field along the x 共y兲 axis is denoted as Ex 共Ey兲 polarized. We measured a transmission peak of up to 75% at 1.55 m for Ex polarized light. Taking into account the refractive index of silicon oxide 共n = 1.47兲, the peak wavelength is slightly higher than the periodicity of the slit array 共1 m兲. It is well-known that when Ex polarized light impinges on metallic gratings oriented along the y direction, the transmission can exceed the diffraction limit at wavelengths comparable to the period of the slits. Such extraordinarily high transmission has been attributed to the excitation of surface plasmons,1 surface evanescent waves16 and/or guided modes.17 When two such single layers are placed in close proximity so that the strong evanescent fields on their surface couple, both the intensity15 and the phase18 of Ex 98, 151107-1 © 2011 American Institute of Physics Downloaded 02 Aug 2011 to 143.89.149.207. Redistribution subject to AIP license or copyright; see http://apl.aip.org/about/rights_and_permissions 151107-2 Marcet et al. FIG. 1. 共Color兲 共a兲 Top view optical image of the half-wave retarder. Cross sectional scanning electron micrograph of 共b兲 aligned and 共c兲 misaligned double layer slit arrays, in structures similar to the sample. 共d兲 Measured transmission spectrum of Ex-polarized 共red line兲 and Ey-polarized 共blue line兲 light through the pixilated structure. 共e兲 RCWA calculations of transmission through both aligned 共red兲 and misaligned 共blue兲 double layer arrays. 共f兲 Phase delay of transmitted light changes by about radians when the lateral shift between the top and bottom arrays is increased from zero to half the period. Field distribution calculated by RCWA for 共g兲 aligned and 共h兲 misaligned double layer arrays. Light at 1.55 m is incident from the bottom with unit amplitude. The color scale is associated with the magnitude and direction of the magnetic field that is directed into and out of the page. The electric field that points along the page is not shown. polarized light can be controlled by the lateral shift in the two layers. The transmitted intensity for Ey polarized light, in contrast, is lower by several orders of magnitude and is practically negligible. Therefore, the pixilated bilayer structure acts as a polarization beam splitter followed by a polarization beam combiner, in the sense that Ex polarized light passes through type 1 pixels and Ey polarized light passes through type 2 pixels. As we will explain below, the phases acquired by these two components in this process differ by . Figure 1共d兲 shows the measured transmission through the pixilated structure for Ex 共red line兲 and Ey 共blue line兲 polarizations at normal incidence, measured with a Fourier transform infrared specrometer. The transmitted intensity depicted by the red 共blue兲 line originates from type 1 共2兲 pixels because light impinging on the other kind of pixels is entirely blocked. For instance, the maximum transmission of ⬃32% for Ey polarized light in Fig. 1共d兲 originates from ⬃64% transmission through type 2 pixels. The transmission of both types of pixels for the corresponding polarization components remains strong due to the efficient coupling of the surface waves excited on the two layers.15 It should be noted that the lateral shift s1 between the two slit arrays within pixel 1 is about 0.1 m instead of exactly perfectly aligned. We choose a sample with this value of s1 共out of many samples covering a wide range of s1兲 so that the transmissions of the Ex polarization through pixel 1 and the Ey polarization through pixel 2 are identical at our laser wavelength of Appl. Phys. Lett. 98, 151107 共2011兲 ជ I of the incident light makes an angle FIG. 2. 共Color兲 共a兲 The electric field E with the x-axis of the pixilated slit array. 共b兲 The y component of the electric field 共blue arrow兲 acquires an extra half-wave phase delay relative to the x component 共red arrow兲, leading to a rotation of the electric field from ជ I to Eជ T, by an angle of 2. 关共c兲–共e兲兴 Transmission measurement 共crosses兲 at E a wavelength of 1.55 m as a function of the angle ␣ of the second polarizer 共before the photodetector兲 relative to the first polarizer 共that polarizes the incident light兲. Full scale transmitted intensity is 16%. The pixilated slit array is inserted between the two polarizers at equal to 共c兲 0°, 共d兲 15°, and 共e兲 45°. The purple lines represent the expected cos2共␣ − 2兲 dependence of the transmitted light intensity on ␣. 1.55 m 关Fig. 1共d兲兴. As described later, equal transmission intensity of the Ex and Ey polarizations is a crucial factor in determining the performance of this device as a half wave retarder. Figure 1共e兲 shows the transmitted intensity calculated with rigorous coupled wave analysis 共RCWA兲 共Ref. 19兲 using the slit array dimensions of the two kinds of pixels and tabulated optical properties of aluminum.20 The calculated transmission is in good qualitative agreement with measurement. The different lateral shifts in the orthogonal pixels produce a phase delay that is close to half-wave in the transmission of the two polarizations. Figure 1共f兲 shows that the calculated phase of the transmitted light varies by almost as the top array is laterally shifted from the bottom array between zero and half the period. To achieve a phase shift between light transmitted through pixels 1 and 2 that is closer to , the sample was tilted about the y-axis by a small angle of 2.5°. The transmission intensity remains largely unchanged. Figures 1共g兲 and 1共h兲 compare the spatial distribution of the magnetic fields for the two pixels, showing the same field directions on the incident side 共bottom兲 but opposite field directions on the transmitted side 共top兲. Such phase delay can be understood in terms of the surface electromagnetic fields on the two individual layers coupling differently depending on whether the fields are parallel or opposite to each other, as explained in Ref. 18. The half-period lateral shift in the type 2 pixels reverses the direction of the electromagnetic field for the transmitted Ex polarization relative to the Ey polarization that was transmitted through the type 1 pixels. We use a 1.55 m laser to demonstrate the capability of the pixilated structure to rotate the polarization. Through a shadow mask, the linearly polarized, collimated laser beam illuminated a sample area of 400⫻ 400 m2 共about 256 pixels兲. As shown in Fig. 2共a兲, the x-axis of the sample was oriented at an angle relative to the electric field of the linearly polarized incident light. A second linear polarizer in Downloaded 02 Aug 2011 to 143.89.149.207. Redistribution subject to AIP license or copyright; see http://apl.aip.org/about/rights_and_permissions 151107-3 Appl. Phys. Lett. 98, 151107 共2011兲 Marcet et al. front of a photodetector serves as an analyzer to measure the polarization of light transmitted through the pixilated sample relative to the polarization of the incident light. Depending on , the electric field of the incident light decomposes into different x and y components along the sample axis 关Fig. 2共b兲兴. For = 0°, all the light is transmitted through the type 1 pixels. The polarization of the transmitted light remains unchanged, as shown in Fig. 2共c兲 by the square cosine dependence of the measured intensity at the photodetector on the angle ␣ of the second polarizer with respect to the first one. When is changed to 45°, half of the incident light is transmitted through the type 1 pixels. The other half is transmitted through the type 2 pixels with the direction of the electromagnetic field reversed, as illustrated in Fig. 2共b兲. Consequently, the transmitted light remains linearly polarized with polarization rotated by 90°, as shown in Fig. 2共e兲. The structure therefore acts as a half wave plate that rotates the polarization of the incident linearly polarized light by 2. Figure 2共d兲 shows measured polarization rotation of 30° for = 15°. For all our measurements at different , the polarization extinction ratio of the transmitted light is found to exceed 22 dB. It is important to note that since the maximum intensities in Figs. 2共c兲–2共e兲 are largely independent of , the pixilated bilayer structure is not a simple polarizer that projects the polarization component along a certain direction, but is a polarization controller that imparts a polarization rotation to the transmitted light. Unlike conventional wave plates, the half-wave retarder described here is not based on birefringence of the material. The wavelength of operation can be chosen by creating slit arrays with different periodicity to tune the surface wave resonance. Using similar principles, quarter wave plates can also be created to generate elliptically polarized light from linearly polarized incident light. Most importantly, it offers the possibility of dynamical control of polarization in future designs if one of the two metal plates can be suspended to allow controlled motion between the two layers. One such configuration involves a lower metal layer fixed to the substrate and a movable upper layer supported by springs. When the top layer moves in the x direction by half the array period, the top and bottom slit arrays become aligned in both types of pixels. As a result, the polarization rotating effect can be completely turned off. Such capability of dynamic polarization control by nanomechanical motion could prove to be useful in optical systems, telecommunication networks and interchip data communications. This work was supported by the National Science Foundation under Grant No. ECS-0621944. Z. Marcet acknowledges support from South East Alliance for Graduate Education and the Professoriate. A portion of this research was conducted at the Center for Nanophase Material Sciences, which is sponsored at Oak Ridge National Laboratory by the Division of Scientific User Facilities, U.S. Department of Energy. 1 T. W. Ebbesen, H. J. Lezec, H. F. Ghaemi, T. Thio, and P. A. 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