International Atomic Energy Agency ASSESSMENT OF OCCUPATIONAL EXPOSURE DUE TO EXTERNAL RADIATION SOURCES AND INTAKES OF RADIONUCLIDES Personal Dosimeters Personal Dosimeters - Unit objectives The objective of this unit is to provide an overview of personal dosimeters used for occupational radiation protection. It is intended to provide a review of the radiation detection mechanisms that are employed, methods for readout, advantages and limitations of dosimetry systems, and the radiation types for which these systems are appropriate. It also provides a comparison of traditional passive systems and newer electronic dosimeters. At the completion of this unit, the student will be able to understand how dosimetry systems function, and make informed judgements on dosimetry system selection. International Atomic Energy Agency Personal Dosimeters - Module outline Introduction Passive, integrating dosimeters Photon Dosimetry Photographic Film Thermoluminescence Photoluminescence Optically Stimulated Luminescence Beta and Low Energy Photon Dosimetry Neutron Dosimetry Nuclear Track Emulsions Solid State Nuclear Track Detectors TLD Albedo Bubble Detectors International Atomic Energy Agency Personal Dosimeters - Module outline Electronic Dosimeters Introduction Pocket Dosimeters Charged fiber (electroscope) pocket dosimeters Ion chambers Commercial Electronic Dosimeters Geiger Mueller Silicon Diode Direct Ion Storage International Atomic Energy Agency Introduction International Atomic Energy Agency A basic objective of personal dosimetry Provide a reliable measurement of the operational quantities, independent of type, energy and direction of incidence of the radiation, and with a prescribed overall accuracy. No dosimetry system can meet these requirements without additional information from workplace monitoring and information about the type of work involved. International Atomic Energy Agency Workplace characteristics dictate dosimetry needs Different dosimeters may be required for low energy x-rays and gamma fields. Different dosimeter types may be needed for photons and neutrons. Complication exists at nuclear power stations, high energy accelerators, fuel reprocessing plants, etc., where there is a mixed radiation hazard. Beta dosimetry is difficult, particularly in mixed fields. International Atomic Energy Agency Exposure geometry is also important Workers at different glove boxes (+, +n) are dealing with sources for exploration or radiography will primarily have A-P exposure. Workers at X-ray diagnostic machines are in a scattered, low photon energy, mostly isotropic radiation field. Operators of radiation sources may be exposed largely from the back: P-A exposure. Places where collimated beams are in operation can be characterized by a rotational geometry. International Atomic Energy Agency Personal dosimeters can be considered to fall into five classes. Photon dosimeters only for Hp(10). Beta-photon dosimeters giving information on Hp(0.07) and Hp(10). Discriminating photon dosimeters that, in addition to Hp(10), provide some indication of radiation type and effective energy, and detection of high energy electrons. Extremity dosimeters for beta-photon radiation only giving information on Hp(0.07), and Neutron dosimeters giving information on Hp(10). International Atomic Energy Agency Passive, Integrating Dosimeters International Atomic Energy Agency Detection mechanisms for personal dosimeters Passive, integrating dosimeters Photographic film Thermoluminescence Photoluminescence Optically stimulated luminescence Solid state nuclear track detection International Atomic Energy Agency A wide range of passive dosimeter designs has been developed International Atomic Energy Agency Photographic Film Dosimetry International Atomic Energy Agency Photographic film Film emulsion is made of AgBr crystals suspended in a gelatinous medium. A thin emulsion layer is coated on a plastic base. Ionizing radiation interacts with emulsion grains to produce a latent image. In development, silver ions in the latent image produce permanent blackening. Blackening is measured with a densitometer. International Atomic Energy Agency Photographic film Degree of blackening is a function of film type, developing process, temperature, and radiation type and energy. Film has been used to determine personnel exposure to photons, betas and thermal neutrons. For personnel monitoring, films are commonly placed inside suitable holders, or "film badges”. Compensation for energy dependence of the film dosimeter is achieved either by the use of one or more filters having different atomic numbers. International Atomic Energy Agency Illustration of exposed film showing filter density pattern A B Film Package C D E C B A D E O A - Plastic filter B to E - Metallic filters O - Open window Film dosimeter with film packet and filters. International Atomic Energy Agency Photographic film One filter is adequate for photons > 0.1 MeV. Multiple filters (e.g. Cu, plastic and open window) are used for lower energy photons. Blackening produced by gamma rays from neutron capture in a cadmium filter is often used to detect thermal neutrons. Type and dose of incident radiation can be estimated from the ratio of responses behind different filters. International Atomic Energy Agency Film density patterns following exposure to radiation fields of different qualities FOG * FILM INVERTED 50 kV X-rays 0.25 mGy 100 kV X-rays 0.25 mGy 75 kV X-rays 1.50 mGy International Atomic Energy Agency Film has a strong photon energy dependence 1.5 Relative sensitivity Normal - 0° 1.0 35° 80° 0.5 45° Kodak RM 0.71 mm Sn + 0.31 mm Pb 0 10 20 50 100 200 500 1000 2000 Photon energy - keV International Atomic Energy Agency Photographic film Optical density does not vary linearly with dose. At higher doses, a reversal of optical density solarization - takes place. Dose Linear combination of the responses behind suitable filters can be used to determine the dose. International Atomic Energy Agency Typical photographic film calibration curve 6 Net optical density 5 4 0.6 Sv/s 11. Sv/s 0.3 mSv/s 3 2 0.013 Sv/s 1 0 10-1 1 10 102 103 104 105 106 Hp(10) - mSv International Atomic Energy Agency Films with different sensitivities extend the measurable dose range of the film badge 7 6 Net density 5 4 A 3 B 2 1 0 0.1 1 10 102 103 104 Hp(10) - mSv International Atomic Energy Agency Photographic film New calibrations are necessary for each new film batch, or the developing process changes. Operational films are often calibrated by using identical standard films irradiated to known doses and processing them simultaneously with the operational dosimeters. Perform calibrations at doses that cover the full range for which the dosimeter is used. Film badges are used for issue periods up to one month. International Atomic Energy Agency For longer periods, fading is a problem 1.0 30% relative humidity Relative optical density 0.8 0.6 60% 0.4 Kodak RM 80% 0.2 0 0 2 4 6 8 10 Storage time - weeks International Atomic Energy Agency Photographic film Film can be used in discriminating dosimeters to give qualitative information in addition to dose. Film dosimetry can be economical depending upon the degree of automation adopted. Film disadvantages include fading and energy dependence, requiring a complex and expensive holder. Film dosimeters can be designed for HP(10) and HP(0.07), and beta radiation with (Emax) > 0.5 MeV. International Atomic Energy Agency Commercial film supply information Dosimetry suppliers ICN Dosimetry Service http://www.dosimetry.com/dx/external/default.html Radiation Detection Company http://www.radetco.com/film.htm Landauer, Inc http://www.landauerinc.com/products.htm General product source listing Double Film Badge Wrist Film Badge Health Physics Society Buyer’s Guide http://hps.org/aboutthesociety/affiliates/services.html Exposed Film International Atomic Energy Agency Thermoluminescence International Atomic Energy Agency Thermoluminescent dosimeters - TLD The thermoluminescence mechanism is complex, and each TL phosphor is unique. After exposure the latent measure of the absorbed dose is the number of electrons which remain trapped in the various trapping levels. TLD readout consists of heating, light detection and data recording. International Atomic Energy Agency Thermoluminescent dosimeters - TLD TLD heating can be done in a number of ways Electrical heating with a hot finger Hot nitrogen gas Radio frequency heating Infrared light International Atomic Energy Agency Thermoluminescent dosimeters - TLD Luminescent brightness vs. temperature at a constant heating rate is called the "glow curve”. A photomultiplier or other light-sensitive device measures the TL glow emission during readout. Entire glow curve or the peak brightness is recorded. Area under the curve or glow peak brightness is used as a measure of dose. International Atomic Energy Agency Illustration of TLD readout High voltage supply D.C. amplifier PM tube Recorder Suitable filter Phosphor material Heater power supply International Atomic Energy Agency Modeling the TL effect TLD Gamma rays, X-rays, etc. The number of photons emitted is proportional to the energy of the ionizing radiation Heat PMT International Atomic Energy Agency Simplified thermoluminescent process Electron Conduction band Thermal release E T L Ionization T T L L Light Hole Valence band a) Irradiation b) Storage c) Heating International Atomic Energy Agency Time-temperature profile (TTP) Anneal temp. Temperature °C Max. temp. Max. temp. ramp rate Preheat temp. Ambient Preheat Acquisition Anneal Ambient Time Time-temperature profile and glow curve for LiF:Mg,Ti freshly exposed to 1 Gy International Atomic Energy Agency Relative thermoluminscent intensity Sample glow curves 100 80 CaSO4 CaF2 LiF 60 40 20 0 0 100 200 300 400 Temperature - Degrees C International Atomic Energy Agency Glow curves for various TL phosphors LiF:Mg,Ti 195 °C Lithium fluoride CaF2:Mn 260 °C Calcium fluoride manganese LiF:Mg,Cu,P 220 °C Lithium fluoride Al2O3:C 185 °C Aluminum oxide CaF2:Dy 180 °C Calcium fluoride dysprosium CaSO4:Dy 220 °C Calcium sulfate dysprosium International Atomic Energy Agency TLD is attractive for radiation protection dosimetry Some TL materials are nearly tissue-equivalent. TL offers high sensitivity, accuracy, low detection limit and linearity over a wide dose range. Many TL materials are commercially available as small solid detectors adaptable for automatic processing. Particularly suited to beta skin and extremity dosimetry. International Atomic Energy Agency General characteristics of commercially available TLDs TLD type LiF:Ti,Mg LiF:Na,Mg LiF:Mg,Cu,P Li2B4O7:Mn Li2B4O7:Cu MgB4O7:Dy BeO CaSO4:Dy CaSO4:Tm CaF2:Mn CaF2 (natural) CaF2:Dy Al2O3 Effective atomic number Zeff 8.3 8.3 8.3 7.3 7.3 8.4 7.1 14.5 14.5 16.3 16.3 16.3 10.2 Main peak (°C) 200 200 210 220 205 190 190 220 220 260 260 215 360 Emission maximum (nm) 400 400 400 605 368 490 200-400 480-570 452 500 380 480-570 699 Relative sensitivity 1 1 25 0.20 2 10 0.20 30 30 5 23 15 4 Fading (at 25 °C) 5%/year 5%/year 5%/year 4%/month 10%/2 months 4%/month 8%/2 months 1%/2 months 1-2%/2 months 16%/2 weeks very slight 8%/ months 5%/2 weeks International Atomic Energy Agency Calculated relative response Photon energy dependence of various TLDs 101 1 10-1 101 102 103 104 Photon energy - keV International Atomic Energy Agency Thermoluminescent fading Unintentional release of trapped electrons before readout is called fading. Fading may be due to thermally or optically stimulated release of the electrons. International Atomic Energy Agency Fading of various phosphors 110 LiF CaF2:Dy 90 CaSO4:Dy Relative dosimeter reading - % 110 90 70 50 25 °C, 97% RH 25 °C, 50% RH 20 50 °C, 31% RH 100 40 60 CaSO4:Dy LiF 80 60 50 50 °C 40 0 60 60 CaSO4:Dy LiF 40 0 40 20 80 20 20 0 100 20 0 Li2B4O7:Mn 60 CaF2:Dy Li2B4O7:Mn 40 CaF2:Dy CaSO4:Dy 70 Li2B4O7:Mn 0 LiF CaF2:Dy Li2B4O7:Mn 0 20 40 60 Storage time - days International Atomic Energy Agency TL signal ratios under different filters Theoretical chip ratios 10. PTFE/Sn(0.33 mm) PTE/Cu Ratio 5. PTFE/Sn(1.3 mm) PTFE/Sn(0.635 mm) 2. 1. 0.5 10 100 1000 Photon energy - keV International Atomic Energy Agency X-ray and response of a 4-element dosimeter using LiF 3.5 Relative response 3.0 Deep dose photon energy response 2.5 1000 mg/cm2 Copper filter Open window 300 mg/cm2 2.0 1.5 1.0 0.5 0 10 100 1000 Photon energy - keV International Atomic Energy Agency Thermoluminescent dosimeters - TLD Dosimeters have excellent long term stability. Dose evaluation is rapid, and dosimeters are reusable. TLD currently used for personnel beta dose monitoring have energy threshold problems because the detector is too thick, or non-tissue equivalent. Multi-element method is complex and can be inaccurate. International Atomic Energy Agency Thermoluminescent dosimeters - TLD Neutron response of TL materials depends on detector composition, TLD encapsulation and neutron energy. Some TL phosphors have high thermal neutron sensitivity, but low fast neutron response. Techniques to increase TL fast neutron response include use of a moderator to thermalize the neutrons. International Atomic Energy Agency Short time exposure dating with LiF Time post exposure - Hours International Atomic Energy Agency Long time exposure dating with LiF TLD Time post exposure - Days International Atomic Energy Agency Harshaw 7776/8814 badge International Atomic Energy Agency Panasonic badge International Atomic Energy Agency Harshaw 6600 automated TLD reader International Atomic Energy Agency ENDOS automated TLD reader International Atomic Energy Agency Commercial TLD supply information Dosimetry suppliers ThermoRMP www.thermormp.co.uk/ Landauer, Inc www.landauerinc.com/products.htm ICN Dosimetry Service www.dosimetry.com/dx/external/default.html Panasonic www.panasonic.com/industrial/other/other_components_radiation_measurement_home.htm International Atomic Energy Agency Photoluminescence International Atomic Energy Agency Photoluminescent Dosimeters - PLD Photoluminescence is based on formation of induced luminescent centers in silver doped phosphate glass. When exposed to UV light, fluorescent light of a larger wave length is emitted with intensity linearly related to absorbed dose up to 30 Sv. Unlike TL centers are not destroyed by normal read-out and are extremely stable. Fading at room temperature is negligible. International Atomic Energy Agency Photoluminescent dosimeters - PLD Dose information can be obtained at any time during long-term dose accumulation. Commercial phosphate glass has good reproducibility and constant sensitivity. Individual calibration of dosimeters is not needed. Pulsed UV laser read-out reduces the pre-dose of unirradiated glasses to a value of about 10 µSv. Because of the high Z value of the glass materials, energy compensation filters are required. International Atomic Energy Agency Sensitivity relative to 60Co Energy dependence of a typical PL glass Photon energy - keV International Atomic Energy Agency Relative RPL intensity - % Example of an PL dosimeter design Photon energy - keV International Atomic Energy Agency Photoluminescence dosimeters - PLD Newer generation flat glass dosimeters have an energy dependence ±15% for photons >15 kev. Automated phosphate glass dosimetry systems are a possible alternative to TLD or film based systems. PLDs have been used in accident dosimeters. In criticality accidents, fast and thermal neutrons can be measured using the 31P(n,p)32Si and 31P(n,)32P reactions and counting the emitted betas. International Atomic Energy Agency Photoluminescence dosimeters - PLD PLD advantages include permanent and long-term integration of dose information, good accuracy, negligible fading and remeasurability. A PLD disadvantage is need for energy compensation filters, excluding measurement of low energy photons. International Atomic Energy Agency Commercial PLD supply information Dosimetry supplier Chiyoda Technol http://www.c-technol.co.jp International Atomic Energy Agency Optically Stimulated Luminescence International Atomic Energy Agency Optically stimulated luminescence - OSL Pulsed OSL dosimetry - A narrow spectrum of light repetitively illuminates an aluminum oxide film. Optical energy releases a small fraction of the trapped charge carriers created during exposure. Released charge carriers combine with luminescent centers to emit light detected with a PMT tube. Each luminescence accumulation period ranges from 25 msec to 100 msec. International Atomic Energy Agency Optically stimulated luminescence - OSL With 10 accumulation periods per dose measurement, the analysis time is approximately 250 msec. The wavelength of the stimulation beam is 532 nm. A series of optical filters between the OSL film and photomultiplier tube reject the green stimulation light and pass the blue luminescence which has a peak wavelength of 420 nm. International Atomic Energy Agency Commercial dosimeter based on OSL International Atomic Energy Agency Optically stimulated luminescence - OSL In the commercial version, aluminum oxide powder is obtained by grinding solid crystals and sifting the powder into the desired size range. The powder is mixed with a polyester binder and coated onto a roll of clear polystyrene film. The coating is 18 mm wide by 0.15 mm thick and each roll is generally 150 meters long. The film roll is cut to produce film chips with an aluminum oxide coating area of 18 mm x 17 mm. International Atomic Energy Agency Optically stimulated luminescence - OSL Each film chip contains approximately 80 mg of aluminum oxide powder. Dosimetry is performed by stimulating three circular areas 4 mm in diameter; each containing 3.3 mg of aluminum oxide powder. Absorbers placed on both sides of the OSL film alter the dose response of the film so that the personal dose quantities can be assessed. International Atomic Energy Agency Optically stimulated luminescence - OSL A fourth area, 6 mm x 6 mm, serves to image determine static and dynamic exposure conditions. A special absorber containing an array of perforations projects a distinctive image on the film. A research grade, image intensified CCD camera captures the luminescent image. Computer programs interpret the image data and can display the image in various configurations. International Atomic Energy Agency Relative response for several photon energiesa ISOb X Ray Quality Average Energy (keV) Response Relative to 137Cs M30 20 1.95 M50 29 2.30 M60 34 2.22 M100 50 1.96 M150 71 1.48 H150 117 0.96 137Cs 662 1.00 a From data of Landauer, Inc. b INTERNATIONAL ORGANIZATION FOR STANDARDIZATION, X and Gamma Reference Radiations for Calibrating Dosemeters and Doserate Meters and for Determining Their Response as a Function of Photon Energy, ISO 4037/Part 1: Radiation Characteristics and Production Methods, ISO, Geneva (1996). International Atomic Energy Agency Commercial OSL supply information Dosimetry suppliers Landauer, Inc www.landauer.com/poducts.htm International Atomic Energy Agency Beta and Low Energy Photon Dosimetry International Atomic Energy Agency Beta and low energy photon dosimetry Beta sources external to the body do not cause significant irradiation of deeper-lying tissue in the body. Can contribute significant exposure of the eye lens. Particularly important in causing irradiation of the hands, and especially of the finger-tips. International Atomic Energy Agency Beta and low energy photon dosimetry If photon or beta irradiation is fairly uniform, a single dosimeter worn on an appropriate part of the body is sufficient, however, Beta irradiation of the body is usually non-uniform. For non-uniform irradiation, additional dosimeters on other parts of the body may be necessary. Frequently, it is necessary to wear an additional suitable dosimeter on the hands or fingers. International Atomic Energy Agency Beta and low energy photon dosimetry Commercial dosimetry services offer finger rings in addition to conventional badges. International Atomic Energy Agency Beta and low energy photon dosimetry Dosimeter may need to measure skin dose from a mixture of beta rays and photons. Dosimeters based on a high Z detector materials are not appropriate because of photon energy dependence. Better to use tissue equivalent dosimeter material. Most photon dosimeter types can be used. International Atomic Energy Agency Ideal dosimeter for beta/gamma skin dose Tissue equivalent detector approximately 5 mg•cm-2 thick in close contact with a tissue equivalent filter of the same thickness and kept in a tissue equivalent holder. Would provide a good estimate of tissue dose at 7 mg•cm-2 depth, independent energy, angle of incidence, or source configuration and geometry. Dosimeter should be easy to handle and suited to manual as well as automatic processing. International Atomic Energy Agency Beta and low energy photon dosimetry Several practical solid state detectors with good dosimetric characteristics have been developed. Thin layers of TL materials on a nonthermoluminescent graphite base Mixed MgB4O7:Dy TLDs BeO TSEE detectors Threshold detection levels as low as 100 µSv (or about 20 µSv for BeO TSEE detector). Small ion chambers adapted to electron measurements by use of a thin entrance window. International Atomic Energy Agency Neutron Dosimetry International Atomic Energy Agency Neutron dosimetry presents unique challenges Neutron interactions produce more densely ionizing charged particles than photons. Photons Electrons Neutrons Recoil protons Alpha particles Heavy charged particles Neutron energies span 9 orders of magnitude vs. 3 for photons. wR 5. International Atomic Energy Agency wR is very important for neutron dosimetry 30 ICRP Recommendation 25 ICRP Approximation 20 WR 15 10 5 0 10-8 10-7 10-6 10-5 10-4 10-3 10-2 10-1 Neutron energy - MeV 1 10 International Atomic Energy Agency 102 Dosimeter energy response is very important 103 E H*(10) Hslab(10) 102 10 1 10-8 10-7 10-6 10-5 10-4 10-3 10-2 10-1 1 10 102 103 Neutron energy - MeV International Atomic Energy Agency Nuclear Track Emulsions International Atomic Energy Agency Neutron dosimetry - Nuclear track emulsions Fast neutrons interact with the hydrogen in the emulsion and film, producing recoil protons. Protons pass through the emulsion to create latent images or tracks which leads to film darkening after processing. Below 10 eV, neutrons interact with nitrogen nuclei of the gelatin and produce recoil protons. Tracks are counted with high magnification microscopes. International Atomic Energy Agency Neutron dosimetry - Nuclear track emulsions NTA energy threshold is about 0.7 MeV. Saturates at relatively low doses (about 50 mSv). Accuracy depends on operator skill. Thermal neutron sensitivity is undesirable, dosimeter should be kept under a filter of neutron absorbing material such as 6LiF or 10B carbide. International Atomic Energy Agency Recoil proton tracks from 14 MeV neutrons International Atomic Energy Agency NTA detects only fast neutrons Relative response 103 102 NTA response 101 Slab phantom conversion coefficients 1 10-8 10-7 10-6 10-5 10-4 10-3 10-2 10-1 1 10 Neutron energy - MeV International Atomic Energy Agency 102 Neutron dosimetry - Nuclear track emulsions High fading is a disadvantage of emulsion. Fading is severe when used without protection in high temperatures and humidity (~ 75% per week). Fading can be controlled if the films are desiccated and sealed in a moisture-proof pouch prior to use. Photon sensitivity is also a serious disadvantage. Other methods are replacing film. International Atomic Energy Agency Solid State Nuclear Track Detectors International Atomic Energy Agency Solid state track detectors (SSNTD) Heavy charged particles such as fission fragments, alpha particles or neutron induced recoils produce damage along their path in dielectric materials. Tracks are etched chemically and become visible under a microscope. Electrochemical etching (ECE) enlarges the track diameter to make large area counting possible. International Atomic Energy Agency Solid state track detectors (SSNTD) Three SSNTD techniques have been used for neutron dosimetry : Fission track detectors Recoil track detectors Track detectors based on (n,p) reactions International Atomic Energy Agency Fission track detectors Detector has 2 components; Fissionable material (radiator or converter) The fission fragment detector All SSNTD materials can be used to detect high LET fission fragments. Efficiency is typically between 85 and 92%. International Atomic Energy Agency Fission track detectors Fission reactions have neutron energy thresholds; 0.6 MeV for 237Np 1.3 MeV for 232Th 1.5 MeV for 238U or very high cross sections for thermal neutrons (e.g. 235U or 239Pu). International Atomic Energy Agency Fission track detectors Neutron energy can be determined using different radiators. Thermal neutron shields (e.g. Cd or 10B) can be used to separate thermal neutrons from those at higher energies. Use of fissionable radiators leads to increased radiation risk. Use of fissionable materials in dosimeters is restricted or forbidden in certain countries. International Atomic Energy Agency Recoil track detectors Neutron interactions in the track detector or radiator may produce recoil charged particles such as protons, carbon, oxygen and nitrogen. Recoils produce latent tracks which also can be visualized by etching. A combination of chemical etching and electrochemical etching (ECE) or a two-step ECE technique can be used to detect recoil tracks. International Atomic Energy Agency Recoil track detectors Track density can be counted with a microfiche reader or an automatic particle counter. Response depends on the detector and energy. Etching techniques are optimized for each combination of radiator, absorber and detector material. Energy response curves must be experimentally established and are only valid for conditions used. International Atomic Energy Agency Recoil track detectors Most common detector materials are polycarbonate, cellulose nitrate and CR39. Polycarbonate is simple, inexpensive and very stable, with an energy threshold is between 2 and 5 MeV. CR39 has a low threshold (~100 keV) and high sensitivity. A number of services use CR39. International Atomic Energy Agency Electrochemical etch tracks Plastic surface Side view ~50 m Early tree formation Etched track Top view for counting International Atomic Energy Agency CR39 is a fast neutron detector Relative response 103 102 CR39 (ECE*) 10 Slab phantom conversion coefficients * Electrochemically etched 1 10-8 10-7 10-6 10-5 10-4 10-3 10-2 10-1 1 10 Neutron energy - MeV International Atomic Energy Agency 102 (n,) Track Detectors Uses neutron induced alpha particles in an external particle radiator or “converter”: 6Li (n,) 3H or 10B (n,) 7Li Cross sections are high for thermal neutrons and decrease as 1/v with increasing energy. Efficiency depends on the type of material and etching conditions. Limit of detection for intermediate neutrons is as low as a few mSv, and 1 mSv for fast neutrons. International Atomic Energy Agency TLD Albedo Dosimeters International Atomic Energy Agency TLD albedo dosimeters Detection of low energy neutrons reflected from the body with thermal detector. TLD with 6LiF (TLD 600) and 7LiF (TLD 700) with various shields. Neutron dose is determined by difference between 6LiF and 7LiF detector readings. Relative response can vary by a factor of 50. Energy response can be improved slightly by the dosimeter encapsulation. International Atomic Energy Agency Albedo response is poor for fast neutrons 103 Relative response Bare 6Li Hankins albedo 102 101 1 10-8 Slab phantom conversion cofficients 10-7 10-6 10-5 10-4 10-3 10-2 10-1 1 10 102 Neutron energy - MeV International Atomic Energy Agency TLD albedo dosimeters For albedo dosimeters, neutron fields can be put in 4 categories: Reactors, linear accelerators and accelerators for medical therapy Nuclear fuel fabrication areas Radioactive neutron sources High energy accelerators with little or no shielding Within a neutron field class, relative neutron response does not vary by more than a factor of 2. International Atomic Energy Agency TLD albedo dosimeters Very large energy dependence is a disadvantage. Energy dependence can be improved with a second detector for fast neutrons. Albedo dosimeters detect neutrons of all energies coupled and have simple, automatic TLD read out. Extensive field calibrations of each dosimeter type is necessary. International Atomic Energy Agency TLD albedo dosimeters Calibration curves for working areas can reduce of albedo response within 30%. Depending on neutron field the lowest detectable dose using TLD albedos varies from 50 to 200 µSv. Albedo dosimeters can be combined with track detectors for separate measurement of fast neutrons. Albedo detector serves as the basic neutron detector for screening purposes. International Atomic Energy Agency Bubble Detectors International Atomic Energy Agency Bubble Damage Polymer Detector Superheated droplets are suspended in a firm elastic polymer. Neutrons trigger droplets giving rise to formation sites. Number of bubbles is a measure of the neutron dose. Completely passive device which can be stored until required for use. International Atomic Energy Agency Bubble damage polymer detector Does not require electronic readout. Automatic reader can be used for a large number of detectors. Extremely sensitive to neutrons (in µSv range). Completely insensitive to gamma rays. Can be made with neutron energy thresholds from <20 keV to several MeV. International Atomic Energy Agency Bubble damage polymer detector Set of detectors can be used for crude spectrometry. One type of a bubble detector has flat energy response for dose equivalent from about 200 keV to >15 MeV. Significant temperature dependence. Limited dose range, so several dosimeters with different sensitivities must be worn. Finally, bubble detectors can be expensive. International Atomic Energy Agency Superheated Drop and Bubble detectors use different detection mechanisms Bubble Technology BD-100R Bubble Dosimeter TM APFEL Liquid Matrix Superheated Drop Detector Cap Glass or Plastic Tube Elastic Polymer Event Acoustical Transducer Event Acoustical Transducer (Gel) Trapped Bubbles ~1 mm diam. Superheated Liquid Drops ~0.025 mm diam. Anti-Coincidence Circuitry Counting and Display Circuitry Noise Acoustical Transducer International Atomic Energy Agency Bubble detectors can have a wide energy range International Atomic Energy Agency Electronic Dosimeters International Atomic Energy Agency Passive dosimeters have limitations Lack of direct dose display. No alarm or indication of high dose rate or dose. Limited sensitivity. Limited accuracy in some cases. Need for significant laboratory investment. International Atomic Energy Agency Why are electronic dosimeters needed? Instant or direct readout where the potential for high exposures exists. Alarm at given levels of dose and dose rate. Indication of Hp(10) and Hp(0.07). Better characteristics for neutron dosimetry. Data transfer to and from computer networks. International Atomic Energy Agency Commercial electronic dosimeters also have limitations Potential dosimeter cost. Passive dosimeters are used extensively. Market is not growing vastly for photon and beta dosimeters. Market is very small for neutron dosimeters. International Atomic Energy Agency Detection mechanisms for electronic (active) dosimeters Charged fiber (electroscope) pocket dosimeters. Ion chambers. Silicon diodes. Geiger-Müller counters. Direct ion storage. Charged particle radiators for neutrons. International Atomic Energy Agency Pocket Dosimeters International Atomic Energy Agency Pocket dosimeters Based on ionization of gases in a small chamber. Suitable for monitoring different types of radiation. Direct-reading devices with and without built-in charger: pocket electrometers. Indirect-reading devices: Condenser type pocket ion chambers require a readout device. International Atomic Energy Agency Direct reading pocket dosimeter International Atomic Energy Agency Pocket dosimeters Useful when immediate indication of the worker's radiation exposure is required. Commonly used as supplementary dosimeters. Should have appropriate wall materials and thicknesses for adequate response to electron, photon or neutrons. Single dosimeters will have a limited dose range. International Atomic Energy Agency Pocket dosimeters Care should be taken against erroneous readings due to electrical leakage. Such dosimeters are called alarm and warning devices. A high degree of accuracy is not important, but reliability is. Proper functioning may be crucial to the safety of personnel. International Atomic Energy Agency Commercial Electronic Dosimeters International Atomic Energy Agency Electronic dosimeters Over 20 types of electronic dosimeters are commercially available. Several GM devices for photons >30 keV. Electronic dosimeters for Hp(10) have been developed based on a single silicon diode. Commercial dosimetry system based on 3 silicon diode detectors, suitable for the simultaneous measurement of HP(10) and HP(0.07) for photons and betas. International Atomic Energy Agency Commercial electronic dosimeters Large variation in specifications and quality. Some photon dosimeters are well advanced. Few photon/beta dosimeters are available. Neutron dosimeters are new. Careful evaluation needed. International Atomic Energy Agency Commercial electronic dosimeters A credit card size routine individual dosimeter has been developed, silicon diode detector measures dose and dose rate adjustable alarm stores daily integrated dose for 12 months. International Atomic Energy Agency Selected commercial electronic dosimeters International Atomic Energy Agency Selected dosimeters - Eurisys Very small and lightweight dosimeter for photon radiation with EEPROM memory for detailed dose history. One of the first advanced systems, today in various applications. International Atomic Energy Agency Selected dosimeters - Fuji Electric Small and lightweight dosimeter with versions for photon or photon, beta and neutron radiation. “Trend dose collection” (i.e. dose data stored every minute). In use in Japanese nuclear power plants. International Atomic Energy Agency Selected dosimeters - MGP Small, rugged and lightweight dosimeter for photon, or photon and beta radiation. Different versions of this system are in numerous applications, including military. International Atomic Energy Agency Selected dosimeters - RADOS Systems with silicon detectors for photon radiation. Small, rugged and lightweight dosimeter with various applications, including civil defense. International Atomic Energy Agency Selected dosimeters - RADOS Passive electronic system with Direct Ion Storage (DIS). Small and rugged devices for measurement of Hp(10) and Hp(0.07) for photon and beta radiation of wide energy range. Especially rugged version for military application and special version for neutron radiation. International Atomic Energy Agency Selected dosimeters - Siemens Sophisticated dosimeter with standard version for measuring Hp(10) and Hp(0.07) for photon and beta radiation. Special version for neutron radiation. Photon and beta version approved for legal dosimetry in UK. International Atomic Energy Agency Electronic dosimeter energy responses International Atomic Energy Agency Electronic dosimeters encounter several problems Lack of security of data storage. No adequate mechanical and climatic resistance. Mass and size of dosimeter. Battery type and life span. International Atomic Energy Agency Electronic dosimeters encounter several problems Poor low energy photon energy dependence. Poor beta radiation response. Sensitivity to electromagnetic fields. Saturation at high dose rates. International Atomic Energy Agency Basic features of Direct Ion Storage (DIS) systems Nondestructive readout Tissue equivalent detector Passive operation Small dimensions Low production cost Suitable for data networks Options for various applications International Atomic Energy Agency Analog EEPRom memory cell Control gate Silicon oxide Oxide Electron tunneling paths Floating gate Source Drain Si International Atomic Energy Agency Cross section of DIS Fill gas Oxide Opening Floating gate Electron tunneling path Source Drain Si Modified Transistor with ion chamber International Atomic Energy Agency DIS photon detector Electrons Gas Photons Graphite or teflon International Atomic Energy Agency DIS-2 Detector Element International Atomic Energy Agency DIS-2 system International Atomic Energy Agency Personal alarm neutron dosimeters P.A.N.D.s are based on several techniques: Counter for measuring recoil protons. 3He Tissue equivalent proportional counter with a microprocessor. Silicon surface-barrier detector to detect recoil ions from polyethylene and 10B radiators. detector in a small CH3 moderator with thermal neutron shield. International Atomic Energy Agency Commercial neutron dosimeters Aloka PDM-313 (Si diode) Fuji Electric NRY-22001 (Si diode) Overhoff Technology Corporation Neutron /Gamma electronic Dosemeter (Si diode) Rados DIS-N (passive), (Ion chamber) Siemens EPD-N (Si diode) International Atomic Energy Agency Example of a silicon diode based neutron dosimeter International Atomic Energy Agency Prototype TEPC dosimeter International Atomic Energy Agency Bubble detector dosimeter Event acoustical transducer Anti-coincidence circuitry Event acoustical transducer Counting and display circuitry Noise acoustical transducer An active dosimeter, based on bubble detection, has been produced commercially. It is based on acoustical detection of bubble formation and includes noise rejection anticoincidence circuitry. International Atomic Energy Agency Energy dependence of prototype electronic neutron dosimeters Relative response 10 SDD MC-TEPC ME-TEPC-24 ME-TEPC-144 ME-TEPC-PD DIS SWD 1 01 10-8 10-2 10-1 1 10 102 Neutron energy - Mev International Atomic Energy Agency DIS neutron detector thermal neutrons particles fast neutrons protons photons electrons A-150 tissue equivalent plastic with BN International Atomic Energy Agency RADOS DIS-N dosimeter International Atomic Energy Agency Conclusions and outlook Several electronic dosimeter types are commercially available. Small number of types fulfill demanding requirements. Some electronic dosimetry systems are legally approved for photon and beta radiation. New products are available and development is ongoing on neutron dosimetry. Quality and application of electronic dosimetry are expected to increase significantly. International Atomic Energy Agency References BARTHE, J., et al., New devices for individual neutron dosimetry, Radiat. Prot. Dosim. 54 (1994) 365-368. BORDY, J.M., BARTHE, J., BOUTRUCHE, B., SEGUR, P., A new proportional counter for individual neutron dosimetry, Radiat. Prot. Dosim. 54 (1994) 369-372. BURGKHARDT, B., ROBER, H.G., PIESCH, E., Phosphate glass energy compensation filters for the measurement of operational dose quantities, Radiat. Prot. Dosim. 6 (1983) 287-289. CHRISTENSEN, P., Review of personnel monitoring technique for the measurement of absorbed dose from external beta and low energy photon radiation, Radiat. Prot. Dosim. 14 (1986) 127-135. GRIFFITH, R.V. and TOMMASINO, L., “Etch track detectors”, Radiation Dosimetry: The Dosimetry of Ionizing Radiation, Vol. III (KASE, K.R., BJARNGARD, B.E., ATTIX, F.H., Eds), Academic Press, New York (1990) Ch. 4. HARRISON, K.G., TOMMASINO, L., Damage track detectors for neutron dosimetry: II. Characteristics of different detection systems, Radiat. Prot. Dosim. 10 1-4 (1985). HARVEY, J.R., BATES, J.R., MACKFARLINE, B., “An assessment of a commercial individual dosemeter suitable for low penetrating radiation”, paper presented at Symp. on Personnel Radiation Dosimetry, Knoxville, 1984. HÖFERT, M., PIESCH, E., Neutron dosimetry with nuclear emulsions, Radiat. Prot. Dosim. 10 1-4 (1985). ING, H., The status of the bubble damage polymer detector, Nucl. Tracks Radiat. Meas. 12 (1986) 49-54. INTERNATIONAL ATOMIC ENERGY AGENCY, Assessment of Occupational Exposure Due to External Sources of Radiation, Safety Guide RS-G-1.3 (1999) INTERNATIONAL ATOMIC ENERGY AGENCY, Neutron Monitoring for Radiological Protection, Technical Reports Series No. 252, IAEA, Vienna (1985). INTERNATIONAL ATOMIC ENERGY AGENCY, Personnel Dosimetry Systems for External Radiation Exposures, Technical Reports Series No. 109, IAEA, Vienna (1970). International Atomic Energy Agency References INTERNATIONAL ORGANIZATION FOR STANDARDIZATION, X and Gamma Reference Radiations for Calibrating Dosemeters and Doserate Meters and for Determining Their Response as a Function of Photon Energy, ISO 4037/Part 1: Radiation Characteristics and Production Methods, ISO, Geneva (1996). LACOSTE, F., LUCAS, M., Le système Dosicard, Radioprotection 28 1 (1993) 77-81. MARSHALL, T.O., POOK, E.A., BARTLETT, D.T., HALLAM, J., “An approved personal dosimetry service based on an electronic dosemeter”, paper presented at International Radiation Protection Association Conf. Montreal, 17-22 May 1992. PIESCH, E., BURGKHARDT, B., “Albedo neutron dosimetry”, Neutron Dosimetry in Radiation Protection (ING, H., PIESCH, I., Eds), Nuclear Technology Publishing, Ashford (1985) 175-188. PIESCH, E., BURGKHARDT, B., “LiF albedo dosimeters for personnel monitoring in a fast neutron radiation field”, Neutron Monitoring for Radiation Protection Purposes, (Proc. Symp. Vienna, 1972), Vol. 2, IAEA, Vienna, (1973) 31-35. PROKI‚ M.S., Beta dosimetry with newly developed graphite mixed TL detectors, Phys. Med. Biol. 30 4 (1985) 323-329. Wernli, C., Neutron Dosimetry with Ion Based DIS System, Proc. 10th International Congress of the International Radiation Protection Association, Hiroshima, Japan, Paper T-13-4 (2000). International Atomic Energy Agency