Session I.4.6 Part I Review of Fundamentals Module 4 Sources of Radiation Session 6 Basic Reactor Physics Theory 4/2003 Rev 2 IAEA Post Graduate Educational Course Radiation Protection and Safe Use of Radiation Sources I.4.6 – slide 1 of 63 Overview In this session we will discuss fission and fusion reactions We will also discuss criticality 4/2003 Rev 2 I.4.6 – slide 2 of 63 Fission fission fragment free neutron beta nucleus alpha energy free neutron 4/2003 Rev 2 gamma free neutron fission fragment I.4.6 – slide 3 of 63 Fission Sample fission reactions: 235U + n 141Ba + 92Kr + 3n + 170 MeV 235U + n 94Zr + 139La + 3n + 197 MeV 4/2003 Rev 2 I.4.6 – slide 4 of 63 Fission Follows neutron capture Thermal neutrons fission 233U, 235U, 239Pu which have odd number of neutrons For isotopes with even number of neutrons, the incident neutron must have energy above about 1 MeV 4/2003 Rev 2 I.4.6 – slide 5 of 63 Fission 4/2003 Rev 2 I.4.6 – slide 6 of 63 Fission Neutron Name/Title Cold Neutrons Thermal Neutrons Epithermal Neutrons Cadmium Neutrons 0 < 0.025 0.025 0.025 < 0.4 0.4 < 0.6 Epicadmium Neutrons 0.6 < 1 Slow Neutrons 1 < 10 Resonance Neutrons Intermediate Neutrons Fast Neutrons Relativistic Neutrons 4/2003 Rev 2 Energy (eV) 10 < 300 300 < 1,000,000 1,000,000 < 20,000,000 >20,000,000 I.4.6 – slide 7 of 63 Fission 4/2003 Rev 2 I.4.6 – slide 8 of 63 fission products and transuranics from neutron capture 4/2003 Rev 2 I.4.6 – slide 9 of 63 Fission Source of energy released during fission: Kinetic energy of fission fragments Gamma rays Kinetic energy of neutrons emitted Prompt Delayed 4/2003 Rev 2 I.4.6 – slide 10 of 63 Criticality Neutrons ejected during fission equal neutrons producing more fissions + neutrons absorbed + neutrons lost from system Criticality is constant if balance exists. Fission rate (power) can be changed by varying the number of neutrons absorbed and/or controlling the number lost 4/2003 Rev 2 I.4.6 – slide 11 of 63 Criticality Multiplication Factor (4 factor formula) Nf+1 Keff = Nf Nf+1 is the number of neutrons produced in the “f+1” generation by the Nf neutrons of the previous “f” generation 4/2003 Rev 2 I.4.6 – slide 12 of 63 Criticality Sub-Critical (keff < 1) – more neutrons lost by escape from system and/or non-fission absorption by impurities or “poisons” than produced by fission. Critical (keff = 1) – one neutron per fission available to produce another fission Super-Critical (keff > 1) – rate of fission neutron production exceeds rate of loss 4/2003 Rev 2 I.4.6 – slide 13 of 63 Criticality Keff depends on the availability of neutrons with the required energy and the availability of fissile atoms As a result, keff depends on composition, arrangement and size of fissile material If assembly is infinitely large, no neutrons are lost and Keff = L x k , where L is the non-leakage probability and K depends on 4 factors 4/2003 Rev 2 I.4.6 – slide 14 of 63 Criticality Let’s follow “n” fission neutrons through their life cycle is mean number of neutrons emitted per absorption in uranium if “n” fission neutrons are captured, n x fission neutrons will be produced 4/2003 Rev 2 I.4.6 – slide 15 of 63 Criticality is the mean number of neutrons emitted per fission which depends on the fuel (2.5 for 235U and 3 for 239Pu) not every uranium absorption results in fission (238U can absorb thermal neutrons without fission) mean number of fission neutrons per absorption is less than 4/2003 Rev 2 I.4.6 – slide 16 of 63 Sample Calculation For 100% enrichment of 235U, = 2.1. What is for natural uranium? f = x a f = (N5 x f 5) a = (N5 x a 5) + (N8 x a 8) = macroscopic cross section = microscopic cross section = average number of neutrons per fission N = atoms per cm3 a = absorption (5 = 235U) f = fission (8 = 238U) 4/2003 Rev 2 I.4.6 – slide 17 of 63 Sample Calculation (N5 x f 5) (f 5) f = = a (N5 x a 5) + (N8 x a 8) (a 5) + ( N8 x a 8) N5 f 5 = 549 barns a 5 = 650 barns a 8 = 2.8 barns = 2.5 for 235U For natural U, N8 = 139 N5 549 = x 2.5 = 1.32 for natural U 650 + (139 x 2.8) 4/2003 Rev 2 I.4.6 – slide 18 of 63 Criticality 238U has a small cross section for fission by fast neutrons (not thermal) = 0.29 barns Fast fission factor is total number of fission neutrons = number of thermal fission neutrons 4/2003 Rev 2 I.4.6 – slide 19 of 63 Criticality depends on 3 factors: ratio of moderator to fuel ratio of inelastic scattering cross section to fission cross section geometrical relationship between fuel and moderator capture of n thermal neutrons will produce n x x fission neutrons 4/2003 Rev 2 I.4.6 – slide 20 of 63 Criticality For unmoderated pure U metal, = 1.29 which is the maximum value For homogenous fuel (such as a solution) is very close to 1 4/2003 Rev 2 I.4.6 – slide 21 of 63 Criticality while fast neutrons are being slowed, they may be captured by 238U without fission resonance for this capture occurs between 5 and 200 eV p is the probability that a neutron will escape this resonance capture 4/2003 Rev 2 I.4.6 – slide 22 of 63 Criticality p = resonance escape probability (fraction of fast, fission produced neutrons that become thermalized) p depends on ratio of moderator to fuel for high ratio of moderator to fuel, p 1 for a low ratio of moderator to fuel, p small for pure unmoderated natural U, p = 0 4/2003 Rev 2 I.4.6 – slide 23 of 63 Criticality from the original n thermal neutrons we have n x x x p thermal neutrons some of the thermal neutrons are absorbed by non-fuel atoms some are absorbed by 235U without fission (only 84% of thermal neutrons absorbed by 235U cause fission) 4/2003 Rev 2 I.4.6 – slide 24 of 63 Criticality f = thermal utilization factor which is the fraction of all the thermal neutrons which are absorbed by the fuel (all of the U) the total number of new neutrons produced by the original n thermal neutrons is n x x x p x f 4/2003 Rev 2 I.4.6 – slide 25 of 63 Criticality aU f= aU + aM + ap aU = macroscopic cross section for U aM = macroscopic cross section for moderator ap = macroscopic cross section for other stuff 4/2003 Rev 2 I.4.6 – slide 26 of 63 Criticality K = Nf+1 npf = = pf n Nf depends only on the fuel , p and f depend on the composition and arrangement of the fuel varies from 1.29 for unmoderated U to almost 1 for homogeneous dispersion of fuel and moderator p is about 0.8 to 1 (for pure 235U, p = 1) 4/2003 Rev 2 I.4.6 – slide 27 of 63 Reactivity and Reactor Control in a nuclear reactor the factors are combined to produce a controlled, sustained chain reaction excess reactivity (k) is an increase in the multiplication factor (k) above 1 k = k - 1 4/2003 Rev 2 I.4.6 – slide 28 of 63 Reactivity and Reactor Control For n neutrons in one generation, the number of additional neutrons in the next generation is nk If the lifetime of a neutron generation is L sec, the time rate of change of neutrons is dn = nk dt L 4/2003 Rev 2 I.4.6 – slide 29 of 63 Reactivity and Reactor Control dn = nk dt L when integrated from no to n we get n =e no k t L The reactor period (T) is the time during which the neutrons (power level) increase by factor of “e” 4/2003 Rev 2 I.4.6 – slide 30 of 63 Reactivity and Reactor Control 1 k = T L or the reactor period is: L T= k The mean lifetime of a neutron (birth to absorption) in pure 235U is about 0.001 sec 4/2003 Rev 2 I.4.6 – slide 31 of 63 Reactivity and Reactor Control The mean lifetime of a neutron (birth to absorption) in pure 235U is about 0.001 sec Assume excess reactivity = 0.1% (k = 0.001) 0.001 T= = 1 sec 0.001 And the power level would increase by 2.718 each second 4/2003 Rev 2 I.4.6 – slide 32 of 63 Reactivity and Reactor Control If k is increased to 0.5% 0.001 T= = 0.2 sec 0.005 The power level increase each second would be n =e no t T = e 1 0.2 = 150 This would be hard to control 4/2003 Rev 2 I.4.6 – slide 33 of 63 Reactivity and Reactor Control The actual mean generation time in a reactor is much greater than 0.001 because 0.6407% of fission neutrons are delayed from 0.3 seconds to 80 seconds. This delay permits the reactor to be controlled. 4/2003 Rev 2 I.4.6 – slide 34 of 63 Reactivity and Reactor Control Delayed Neutrons Group ni (%) Ti (sec) ni x Ti 1 0.0267 0.33 0.009 2 0.0737 0.88 0.065 3 0.2526 3.31 0.836 4 0.1255 8.97 1.125 5 0.1401 32.78 4.592 6 0.0211 80.39 1.688 ni = 0.6407 4/2003 Rev 2 nixTi = 8.315 I.4.6 – slide 35 of 63 Reactivity and Reactor Control The mean generation time for all fission neutrons is delayed prompt 8.315 + (99.359 x 0.001) niTi T = n = = 0.084 sec 100 i If k 0.006407 the reactor is prompt critical – the reaction can be sustained by prompt neutrons alone If k < 0.006407 the reactor is delayed critical – the delayed neutrons are needed to sustain the reaction 4/2003 Rev 2 I.4.6 – slide 36 of 63 Sample Calculation What is the reactor period and the increase in power level in 1 second for a generation time of 0.084 sec for excess reactivity (k) of 0.1% and 0.5% For k = 0.001 T = 0.084 = 84 sec 0.001 n =e no 1 84 = 1.012 For k = 0.005 0.084 T= = 16.8 sec 0.005 4/2003 Rev 2 n =e no 1 16.8 = 1.06 I.4.6 – slide 37 of 63 Reactivity and Reactor Control Excess reactivity is measured in units of “dollars” and “cents” (one dollar = 100 cents) and “inhours” (inverse hours) One “dollar” worth of reactivity will cause the reactor to go prompt critical One “inhour” is the amount of excess reactivity which results in a reactor period of 1 hour 4/2003 Rev 2 I.4.6 – slide 38 of 63 Fission Control of Fission Fission typically releases 2-3 neutron (average 2.5) One is needed to sustain the chain reaction at a steady level of controlled criticality The other 1.5 leak from the core region or are absorbed in non-fission reactions 4/2003 Rev 2 I.4.6 – slide 39 of 63 Fission Control of Fission Boron or cadmium control rods absorb neutrons When slightly withdrawn the number of neutrons available for fission exceeds unity and the power level increases When the power reaches the desired level, the control rods are returned to the critical position 4/2003 Rev 2 I.4.6 – slide 40 of 63 Fission Control of Fission ability to control the reaction is due to presence of delayed neutrons without delayed neutrons, change in the critical balance of the chain reaction would lead to a virtually instantaneous and uncontrollable rise or fall in the neutron population safe design and operation of a reactor sets strict limits on departures from criticality 4/2003 Rev 2 I.4.6 – slide 41 of 63 Fission Control of Fission fission neutrons initially fast (energy above 1 MeV) fission in 235U most readily caused by slow neutrons (energy about 0.02 eV) moderator slows fast neutrons by elastic collisions For natural (unenriched) U only graphite and “heavy” water suitable moderators For enriched uranium “light” water may be used 4/2003 Rev 2 I.4.6 – slide 42 of 63 Fission Control of Fission commercial power reactors designed to have negative temperature and void coefficients if temperature too high or excessive boiling occurs rate of fission is reduced and temperature reduced 238U absorbs more neutrons as the temperature rises, pushing neutron balance towards subcritical steam within water moderator reduces density which pushes neutron balance towards subcritical 4/2003 Rev 2 I.4.6 – slide 43 of 63 Fission Control of Fission fuel gradually accumulates fission products and transuranic elements which increases neutron absorption (control system has to compensate) after about three years, fuel is replaced due to: build-up in absorption metallurgical changes from constant neutron bombardment burn-up effectively limited to about half of the fissile material 4/2003 Rev 2 I.4.6 – slide 44 of 63 Fission Summary 4/2003 Rev 2 I.4.6 – slide 45 of 63 Fusion In 1920 Arthur Eddington suggested that the energy of the sun and stars was a product of the fusion of hydrogen atoms into helium In the core of the sun at temperatures of 10-15 million degrees Celsius, hydrogen is converted to Helium Since the 1950's, great progress has been made in nuclear fusion research however, the only practical application of fusion technology to date has been the "hydrogen" or thermonuclear bomb 4/2003 Rev 2 I.4.6 – slide 46 of 63 Fusion Fusion has an almost unlimited potential The hydrogen isotopes in one gallon of water have the fusion energy equivalent of 300 gallons of gasoline A fusion power plant would have no greenhouse gas emissions and would not generate high level radioactive waste Experts predict the world is still at least 50 years and billions of dollars away from having fusion generated electricity largely due to the enormous size and complexity of a fusion reactor 4/2003 Rev 2 I.4.6 – slide 47 of 63 Fusion Hydrogen atoms merged to create helium Helium mass is slightly less (1%) than the original mass with the difference being given off as energy Rather than using hydrogen atoms, it is easier to promote fusion by using two isotopes of hydrogen, deuterium and tritium Deuterium is a naturally occurring isotope of hydrogen which has one extra neutron One hydrogen atom in 6700 occurs as deuterium and can be separated from the rest 4/2003 Rev 2 I.4.6 – slide 48 of 63 Fusion 4/2003 Rev 2 I.4.6 – slide 49 of 63 Fusion Energy per Nucleon (MeV) 0 -2 Fission A 56 -4 -6 -8 -10 0 4/2003 Rev 2 Fusion A 56 50 100 150 200 Atomic Mass Number 250 I.4.6 – slide 50 of 63 Fusion Tritium very rare because it is naturally radioactive and decays quickly Tritium can be made by bombarding the naturally occurring element lithium with neutrons Tritium could be created by having a "blanket" made of lithium surrounding a fusion containment vessel (this would result in a breeder reactor) Fusion can only be accomplished at temperatures typical of the centre of stars, (100 million degrees Celsius 4/2003 Rev 2 I.4.6 – slide 51 of 63 Fusion The fusion components exist in the form of a plasma, where atoms are broken down into electrons and nuclei No known solid material could withstand the temperatures involved in nuclear fusion, so that a powerful confinement system is required to keep the plasma away from the walls of the vessel in which it is contained 4/2003 Rev 2 I.4.6 – slide 52 of 63 Fusion Fuels Deuterium can be extracted from water (If all the world's electricity were provided by fusion, deuterium would last for millions of years) Tritium does not occur naturally and will be manufactured from lithium within the machine Lithium, the lightest metal, is plentiful in the earth's crust (if all the world's electricity were to be provided by fusion, known reserves would last for at least 1000 years) Even though fusion occurs between Deuterium and Tritium, the consumables are Deuterium and Lithium 4/2003 Rev 2 I.4.6 – slide 53 of 63 Fusion Fuels For example, 10 grams of Deuterium which can be extracted from 500 litres of water and 15g of Tritium produced from 30g of Lithium would produce enough fuel for the lifetime electricity needs of an average person in an industrialised country 4/2003 Rev 2 I.4.6 – slide 54 of 63 Current Fusion Research Fusion research was big news in 1989 when it was reported that scientists had achieved fusion at room temperatures with simple equipment Unfortunately, the scientists involved could not prove their claims There are currently two methods of confining the hot plasma which are being studied around the world, "magnetic confinement" and "inertial confinement" 4/2003 Rev 2 I.4.6 – slide 55 of 63 Current Fusion Research Magnetic confinement has the greatest potential and most of the recent research has been based on the "TOKOMAK" system (Tokomak is an acronym for the Russian words "torroidal magnetic chamber“) The tokomak system was developed in the former U.S.S.R. and is under study in the U.S., Japan and Europe A torroidal magnetic chamber is a doughnut shaped steel structure in which the fusion plasma is confined by means of powerful coils of super-conducting material which create a strong magnetic field I.4.6 – slide 56 of 63 4/2003 Rev 2 Current Fusion Research The other method is inertial confinement (small amounts of a deuterium-tritium mixture are rapidly heated to extremely high temperatures with a high powered laser beam or a beam of charged particles) The most advanced test reactors, the Tokomak Fusion Test Reactor (TFTR) in the U.S. and the Joint European Torus (JET), use the tokomak design To be useful the energy produced must be many times that required to sustain the reaction Even the most optimistic researchers feel that this will not be achieved until the next century 4/2003 Rev 2 I.4.6 – slide 57 of 63 Fusion Power Plants A fusion reactor capable of generating 1000 MW of electricity would be very large and complex While fission reactors can be made small enough to be used in submarines or satellites, the minimum size of a fusion reactor would be similar to that of today's largest commercial nuclear plants the difficult part is creating a sustainable fusion reaction - capturing the energy to generate electricity is very similar to a fission reactor A 1000 MW fusion generator would consume only 150 kg of deuterium and 400 kg of lithium annually 4/2003 Rev 2 I.4.6 – slide 58 of 63 Advantages and Disadvantages of Fusion The fuels required for fusion reactors, deuterium and lithium, are so abundant that the potential for fusion is virtually unlimited Oil and gas fired power plants as well as nuclear plants relying on uranium will eventually run into fuel shortages as these non-renewable resources are consumed Unlike fossil plants, fusion reactors have no emission of carbon dioxide (contributor to global warming) or sulphur dioxide (cause of acid rain) 4/2003 Rev 2 I.4.6 – slide 59 of 63 Advantages and Disadvantages of Fusion Barriers to the widespread use of nuclear power have been public concern over operational safety, and the disposal of radioactive waste Accidents such as Chernobyl are virtually impossible with a fusion reactor because only a small amount of fuel is in the reactor at any time It is also so extremely difficult to sustain a fusion reaction (should anything go wrong, the reaction would invariably stop) 4/2003 Rev 2 I.4.6 – slide 60 of 63 Advantages and Disadvantages of Fusion Long lived highly radioactive wastes are generated by conventional nuclear plants Radioactive wastes generated by a fusion reactor are the walls of the vessel exposed to neutrons Although the quantity of radioactive waste produced by a fusion reactor might be slightly greater than that from a conventional nuclear plant, the wastes would have low levels of short lived radiation, decaying almost completely within 100 years. 4/2003 Rev 2 I.4.6 – slide 61 of 63 Advantages and Disadvantages of Fusion The major disadvantages of nuclear fusion are the vast amounts of time and money which will be required before any electricity is generated by fusion Development of other electricity supply technologies such as photovoltaic cells which convert sunlight directly into electricity could eliminate the need for fusion before it is operational 4/2003 Rev 2 I.4.6 – slide 62 of 63 Where to Get More Information Cember, H., Introduction to Health Physics, 3rd Edition, McGraw-Hill, New York (2000) Firestone, R.B., Baglin, C.M., Frank-Chu, S.Y., Eds., Table of Isotopes (8th Edition, 1999 update), Wiley, New York (1999) International Atomic Energy Agency, The Safe Use of Radiation Sources, Training Course Series No. 6, IAEA, Vienna (1995) 4/2003 Rev 2 I.4.6 – slide 63 of 63