Interaction of Neutrons with Matter Vasily Arzhanov Reactor Physics, KTH Overview • • • • • • • Chain Reaction in a Nuclear Reactor Classification of Neutron Interactions Interaction Cross-Sections Neutron Flux and Reaction Rates Elastic Scattering: X(n,n)X or simply (n,n) Inelastic Scattering: (n,n') 1/v and non-1/v absorbers HT 2008 Neutron Interactions 2 Chain Reaction n 2 MeV β H2O 235U n 2 MeV E ~ 0.1 eV β Scattering ν n ν H2O γ 235U ν γ ν γ β Fission 400 KeV γ 238U β 239Pu Capture HT 2008 Neutron Interactions Breeding 3 Fission Cross Section 10 4 235 σ (barns) 10 U 3 10 2 fission 10 1 10 0 capture 10 -1 10 -2 -3 10 10 -2 10 -1 10 0 10 1 10 2 10 3 10 4 10 5 10 6 10 7 Energy (eV) HT 2008 Neutron Interactions 4 2 MeV N1 ν n/fission Energy Leakage N2 N2 k≡ N1 Fast fission Resonance abs. ν ≈ 2.5 Non-fissile abs. Slowing down E Physical Principles of Nuclear Reactor Non-fuel abs. 1 eV Fission 200 MeV/fission HT 2008 Leakage Neutron Interactions 5 Important ν ≈ 2.5 n/fiss εf ≈ 200 MeV/fiss MeV = 1.602 × 10-13 J Pthermal = Nfissions • εf • MeV [W] = [fiss/s] • [MeV/fiss] • [J/MeV] Nfissions may be evaluated through n(r,E,t) n(r,E,t)d3rdE = Number of neutrons in d3r about r with energies in dE about E. HT 2008 Neutron Interactions 6 Conclusion The behaviour of a nuclear reactor is governed by the distribution in • space • energy • time of the neutrons in the system. The central problem is to predict this distribution, or equivalently to derive an equation for the neutron density, n(r,E,t) or more generally, n(r,E,Ω,t). The first step to this end is to study the neutron interaction with matter. HT 2008 Neutron Interactions 7 Classification of Neutron Interaction with Matter Neutron Interaction Scattering Elastic HT 2008 Inelastic Absorption Fission Capture (n,γ) Neutron Interactions N. mult. (n,2n) (n,3n) ... (n,p) (n,α) 8 Reactions (n,xn) HT 2008 63 29 1 Cu+ 01 n →62 Cu+2 29 0n 63 29 Cu(n,2n) 62 29Cu 203 81 200 Tl+ 01 n →81 Tl+4 01 n 203 81 Tl(n,4n) 200 81 Tl Neutron Interactions 9 Reactions (n,p) (n,d) (n,α) N + 10 n → 146C + 11 H p 14 7 d 31 15 α production in the atmosphere 31 P + 10 n → 14 Si + 21 H 10 5 B+ n → or HT 2008 14C 1 0 10 5 ( B) 11 5 * → 73 Li + 42 He B(n,α ) 7 Li Neutron Interactions 10 Definition of Cross-Section Each instance of interaction will be called collision. Detector Area of the beam, A cross section σ Monoenergetic beam of neutrons θ # [I ] = 2 cm s Detector Vol = A×L L Experiments: Rcoll(Vol) = σ×I×N×Vol [σ ] = cm 2 HT 2008 Neutron Interactions 11 Macroscopic Cross Section Collimated monoenergetic neutron beam, n/(cm2sec) I0 Number of neutrons at distance x: I(x) -dI(x) x It was observed in experiments that the fraction of neutrons which suffer their first collision in dx around x is constant. x+dx dI ( x) − = dx ⋅ Σ ⎡⎣cm −1 ⎤⎦ I ( x) Neutrons have no memory HT 2008 Neutron Interactions 12 Microscopic Cross Section It was observed further in experiments that this constant is proportional to the density of the background medium. Σ =σN σ ⎡⎣cm 2 ⎤⎦ Cross-sectional unit: 1 barn = 10-24 cm2 Σ → Σt σ → σt HT 2008 (total cross-section) Neutron Interactions 13 Example 1 0.5 A beam of 1-MeV neutrons of intensity 5×108 n/(cm2s) strikes a thin 12C target. The area of the target is 0.5 cm2 and is 0.05 cm thick. The beam has a cross-sectional area of 0.1 cm2. At 1 MeV, the total cross-section of 12C is 2.6 b and density is 1.6 g/cm3. cm2 12C target 0.1 cm2 Question (a): At what rate do interactions take place in the target? Question (b): What is the probability that a neutron in the beam will have a collision in the target? 0.05 cm Rcoll(Vol) = σ×I×N×Vol Number density of the target material HT 2008 Neutron Interactions 14 Solution 1 Rcoll (Vol) = σ × I × N × Vol N= ρ ⋅ NA M 1.6 × 6.02 ⋅ 10 23 = ≈ 8 × 10 22 12 Rcoll ( Vol) = 2.6 × 10 −24 × 5 × 10 5 × 8 × 10 22 × 0.1 × 0.05 = 5.2 × 10 5 # s Rcoll 5.2 × 10 5 −2 Pr {neutron interacts} = = = 1.04 × 10 I × A 5 × 10 8 × 0.1 HT 2008 Neutron Interactions 15 Neutron Attenuation Number of neutrons survived traveling distance x. dI ( x) I ( x) − = Σt dx −dI ( x) dI ( x) − I ( x) Σt HT 2008 I ( x) = I ( 0 ) e −Σt x I ( x) Pr {No collision} = = e −Σt x I (0) Number of neutrons that survived penetrating the distance x and made their first collision within dx. = Probability of the first collision within dx = Σt dx = Probability of some interaction per unit path length Neutron Interactions 16 Probability of Uncollided Flight 1 Probability of uncollided flight within distance x F(x) P(x) = e−Σt x Probability of at least one collision within distance x F(x) = 1 − P(x) = 1 − e −Σt x 0 HT 2008 Neutron Interactions P(x) x 17 First Collision Probability Independent events: P { A ∩ B} = P { A} ⋅ P {B} Let p(x)dx be the probability that a neutron will have its first collision in dx around x. p ( x ) dx = Pr {( Survives x ) ⋅ ( Collides in dx )} = = Pr {Survives x} ⋅ Pr {Collides in dx} = e −Σt x Σt dx First collision probability: p ( x ) = Σt e −Σt x ∞ ∫ p ( x ) dx = 1 0 HT 2008 Neutron Interactions 18 Mean Free Path The mean free path, average distance traveled by a neutron in the medium is ∞ ∞ 0 0 mfp = λ = ∫ xp ( x ) dx = Σt ∫ xe −Σt x dx = 1 Σt For example, mean free path of 100-keV neutrons in liquid sodium is 11.6 cm. σt = 3.4 b; N = 2.54×1022; Σt = 0.0864 cm-1; HT 2008 Neutron Interactions λ = 1/Σt = 11.6 cm 19 Mean Time Collision probability per unit path length is Collision probability per unit time is Alternatively HT 2008 1 Σt ⇒ = λt Σt 1 vΣt ⇒ = τt vΣt Mean free path Mean time λt 1 = = τt v vΣt Neutron Interactions 20 Cross-Sections of Mixtures Homogeneous mixture of 2 nuclide species, X and Y. Probability per unit path length that a neutron collides with X is ΣX = σXNX Probability per unit path length that a neutron collides with Y is ΣY = σYNY Total probability per unit path length that a neutron collides with either nuclides Σ = σ X N X + σ Y NY It generalizes to Σ = ∑ σ i N i i HT 2008 Neutron Interactions 21 Cross-Sections of Molecules N X = mN , If there are N molecules XmYn per cm3 then σ= Σ σ X N X + σ Y NY = = mσ X + nσ Y N N NY = nN (except elastic scattering) Elastic scattering in water 0.0253 eV 1 MeV HT 2008 H 21 3 O 4 8 2σs(H) + σs(O) 46 14 σs(H2O) 103 14 Neutron Interactions 22 Elastic Scattering from Molecules Feels only H τ coll ∼ 0 Fast neutron Ek Echem σ s (H 2O) = 2σ s (H) + σ s (O) Feels whole molecule Slow (thermal) neutron τ coll ≠ 0 Ek ∼ Echem HT 2008 Neutron Interactions 23 Elastic Scattering in Water σ s [barn] Chemical binding is unimportant important 150 100 50 2σ s (H) + σ s (O) 0.01 HT 2008 0.1 1 Neutron Interactions 10 E [eV] 24 Neutron Flux I One-beam experiment: I = vn Collision rate: Rcoll ( Vol ) = σ × I × N × Vol Rt ≡ Rcoll ( Vol ) = Σt I = Σt vn Vol Except for crystals, the interaction of neutrons with nuclei is independent of the angle. ID Rt = Σt ( I A + I B + IC + I D ) = Σt v ( nA + nB + nC + nD ) IC IA n = nA + nB + nC + nD φ ≡ vn IB HT 2008 Rt = Σt vn Rx = Σ xφ ⎡⎣ n cm 2 s ⎤⎦ Neutron Interactions 25 Meaning of cm2 in Flux I I = vn ⎡ # ⎤ 2 ⎥ ⎣ cm s ⎦ φ ≡ vn ⎢ HT 2008 Neutron Interactions 26 Physical Meaning of Neutron Flux φ (r ) ≡ vn(r ) = ∑ vni = ∑ φi i φi = v i neutrons from direction i dN i da dN φ =v da r dN is the number of neutrons entering the sphere with a cross section da per unit time unit area for direction i Flux is the number of neutrons entering the sphere with a unit cross section around point r per unit time HT 2008 Neutron Interactions 27 Another Interpretation φ(r) = v ⋅ n(r) distance traveled by 1 neutron per unit time number of neutrons having velocity v in unit volume Total distance (track length) traveled by all neutrons in unit volume around r per unit time HT 2008 Neutron Interactions 28 Reaction Rate Reaction rate, Rx = number of interaction of kind x per unit volume in unit time Probability per unit path length Distance per unit time Rx (r , t) = Σxvn(r , t) = Σxφ(r , t) Probability per unit time HT 2008 Number of neutrons in unit volume Neutron Interactions 29 Neutron Flux Units φ ≡ v⋅n Rx = Σxφ ⎡ # ⎤ ⎡ # ⎤ n(r , t) ⎢ 3 ⎥ ⇒ φ(r , t) ≡ v ⋅ n(r , t) ⎢ 2⎥ cm s cm ⋅ ⎣ ⎦ ⎣ ⎦ ⎡ # ⎤ ⎡ # ⎤ n(r , E, t) ⎢ 3 ⎥ ⇒ φ(r , E, t) ≡ v ⋅ n(r , E, t) ⎢ ⎥ 2 cm J s cm J ⋅ ⋅ ⋅ ⎣ ⎦ ⎣ ⎦ ⎡ ⎤ ⎡ ⎤ # # n(r , E, Ω, t) ⎢ 3 ⎥ ⇒ φ(r , E, Ω, t) ≡ v ⋅ n(r , E, Ω, t) ⎢ ⎥ 2 cm J sr s cm J sr ⋅ ⋅ ⋅ ⋅ ⋅ ⎣ ⎦ ⎣ ⎦ HT 2008 Neutron Interactions 30 Reactor Power ∞ P(t) = ε f ⋅ ∫∫ Σ f (r , E)φ(r , E, t)dEd3r V 0 ∞ P(t) = ε f ⋅ ∫∫ Σ f (r , E)vn(r , E, t)dEd3r V 0 J 1 # J 3 × ×J×cm = = W ⎡⎣P⎤⎦ = × 2 # cm s×cm ×J s HT 2008 Neutron Interactions 31 Example 2 A certain research reactor of a cubic shape has a flux of 1×1013 n/cm2s and a side of 0.8 m. If the fission cross-section, Σf, is 0.1 cm-1, what is the power of the reactor? HT 2008 Neutron Interactions 32 Solution 2 P = ε f R f V = ε f Σ f φV P = 200 3 MeV J 1 # × 0.1 × 1013 × = 16.4 MW 1.6 × 10 −13 80cm ( ) 2 # MeV cm cm s Typical NPP produces 1000 ÷ 3000 MWth HT 2008 Neutron Interactions 33 Cross Section Hierarchy Total cross section σt Scattering σs Elastic σe Inelastic σi Absorption σa Fission σf Capture σγ n. mult. σ2n σ3n σp σα ... HT 2008 Neutron Interactions 34 Neutron Cross-Sections σs = σe +σi σ a = σ γ + σ f + σ p + σ α + σ 2n + … Often: σa = σγ +σ f σt = σs +σa HT 2008 Neutron Interactions 35 Compound Nucleus Formation To explain nuclear reactions, Niels Bohr proposed in 1936 a two-stage model comprising the formation of a relatively long-lived intermediate nucleus and its subsequent decay. Fe + n → ( Fe ) 57 26 * Fe + n Fe + n′ Fe + γ Fe + 2n (elastic scattering) 32 30 (inelastic scattering) 28 26 (radiative capture) (n,2n) reaction Cross-sections of nuclear reactions exhibit maxima at certain incident neutron energies. The maxima are called resonances. Energy levels 34 24 Energy, MeV 56 26 56 26 56 26 56 26 56 26 12C 22 20 18 16 14 12 10 8 6 4 2 0 HT 2008 Neutron Interactions 36 Elastic Scattering X(n,n)X Regions: Potential scattering Elastic scattering cross-section as a function of incident neutron energy, E σ e = 4π R2 Resonances Smooth region HT 2008 Neutron Interactions 37 Elastic Scattering for 16O Resonance region σ e = 4π R2 ~50 keV Potential scattering 0.01 eV HT 2008 100 keV Neutron Interactions Smooth region 38 Elastic Scattering for 238U Density increases ~10 eV 1 eV HT 2008 Neutron Interactions 1 keV 39 Summary on Elastic Scattering • Elastic scattering cross-sections for light elements are more or less independent of neutron energy up to 1 MeV. • For intermediate and heavy elements, the elastic crosssection is constant at low energy and exhibit some variation at higher energy. • We are usually more interested in light elements as far as elastic scattering is concerned; so a good approximation is, σs = const, for all elements of interest. • Nearly all elements have scattering cross-sections in the range 2 to 20 barns. • The important exception is water and heavy water. HT 2008 Neutron Interactions 40 Odd vs. Even Nuclides 10000 1000 100 10 1 0,1 500 1000 50 100 5 10 1 0,5 10 30 Incident neutron data / ENDF/B-VII.0 / U238 / Resonances / Resonances data Resolved parameters : 1.0E-5 < E < 20000.0 Incident Energy (eV) 20 30 Incident neutron data / ENDF/B-VII.0 / U235 / Resonances / Resonances data Resolved parameters : 1.0E-5 < E < 2250.0 Incident Energy (eV) 20 40 40 T=300.0 K T=300.0 K 50 50 41 Neutron Interactions HT 2008 0,1 10 0 Resonances (b) Resonances (b) 50 (eV) 238U 235U E Summary for Resonance Levels • For light nuclei resonance levels are scarce with distance of about 100 keV or more. For heavy nuclei distance between the levels is of the order of few eV • Density of levels increase with energy. Pronounced effect of EVEN - UNEVEN nuclei. When neutrons interact with nuclei with EVEN mass number resonances are at larger distances than for UNEVEN mass numbers HT 2008 Neutron Interactions 42 Inelastic Scattering n n AX θ A+1X* γ (1) Light (2) Heavy 1 MeV 50 KeV Ground HT 2008 Li, Be 238U 2-3 MeV 40 KeV Neutron Interactions 43 General Conclusion on In. Sc. • Inelastic scattering cross section is relatively small for light nuclei. • Heavy nuclei cannot serve as good moderators in thermal reactors. • Inelastic scattering may be significant: – Heterogeneous reactors – Highly enriched fuel – Fast reactors HT 2008 Neutron Interactions 44 Radiative Capture Potential scattering The radiative capture cross-section as a function of the incident neutron energy 1 1 σγ ∝ ∝ E v Resonances Smooth region There are a few important nuclei that do not show exact 1/v behaviour. They are called non-1/v absorbers. HT 2008 Neutron Interactions 45 Radiative Capture for 197Au 1/v region HT 2008 Neutron Interactions 46 Breit-Wigner Formula Statistical factor Neutron width Wavelength of neutrons with energy Er Radiation width ΓnΓγ γ r2 g σ γ ( E) = 4π ( E − Er )2 + Γ2 4 Total width, Γ = Γn + Γγ HT 2008 Neutron Interactions 47 Single-Level Resonance Peak width at half-maximum Breit-Wigner formula: σ x ( E) = σ max σ max 2 Γ σ s ( E) = Er HT 2008 σ x,max 2 ⎛ E − Er ⎞ ⎜ ⎟ +1 ⎝ Γ2 ⎠ Er ⋅ E σ s,max 2 ⎛ E − Er ⎞ ⎜ ⎟ +1 ⎝ Γ2 ⎠ E Neutron Interactions 48 Charged-Particles Reactions As a rule, the (n,p), (n,α) are endothermic and do not occur below some threshhold energy. Their cross-sections tend to be small, even above the threshhold, especialy for heavier nuclei. En > 9 MeV 16 8 16 O ( n, p ) N ⎯⎯⎯ → 8O + γ 7 sec 16 7 β− Eγ > 6÷7 MeV However, there some important exothermic reactions in light nuclei: 10 5 6 3 HT 2008 B( n,α ) 73 Li Li ( n,α ) 31 H Neutron Interactions 1/v absorber 1/v absorber Tritium production 49 Several orders Cross-Section of (n,α) for 10B Several orders HT 2008 Neutron Interactions 50 Total Cross-Section At low energy C σ t = 4π R + E 2 239Pu Total Fission Capture Elastic Inelastic HT 2008 Neutron Interactions 51 Hydrogen and Deuterium The nuclides, 1H and 2H, interact differently • No formation of compound nucleus. • No resonances. • No excited states. • No inelastic scattering. σs is constant up to 10 keV. σγ is 1/v up to 1 MeV. HT 2008 Neutron Interactions 52 Cross-Sections for 1H Both total and elastic scattering 1/v region 0.1 eV HT 2008 100 keV Neutron Interactions 53 Example 3 σ γ ( E) C σ γ ( E) = ⎯⎯ → = σ γ ( E0 ) E E0 E0 ⎯⎯ → σ γ ( E ) = σ γ ( E0 ) E E At E = 0.253 eV, σγ(1H) = 0.032 b. What is σγ at 1 eV ? σ γ ( 1eV ) = 0.332 × HT 2008 0.253 = 0.0528 b 1 Neutron Interactions 54 Polyenergetic Neutrons We define n(E) such that n(E)dE is the number of neutrons per unit volume with energies in dE about E. Polyenergetic neutron beam Differential collision rate dI ( E ) = v( E)n( E)dE dRt ( E ) = Σt ( E ) v( E)n( E)dE ∞ Total collision rate Rt = ∫ Σt ( E ) v( E)n( E)dE 0 ∞ Absorption collision rate Ra = ∫ Σ a ( E ) v( E)n( E)dE 0 HT 2008 Neutron Interactions 55 1/v Absorbers Σ a ( E ) v( E) = Σ a ( E0 ) v0 ∞ ∞ 0 0 Ra = ∫ Σ a ( E ) v( E)n( E)dE = Σ a ( E0 ) v0 ∫ n( E)dE = Σ a ( E0 ) v0 n For 1/v absorbers, the absorption rate is independent of the energy distribution. Equivalently, the absorption rate is the same as that for a monoenergetic beam of neutrons with arbitrary energy E0 and intensity v0n. Standard practice: to specify 1/v X-sections at the single energy E0 = 0.0253 eV corresponding to v0 = 2200 m/s. The values of X-sections at 0.0253 eV are loosely referred to as thermal cross-sections. The quantity v0n is called 2200 m/s flux and denoted as φ0 ≡ v0 n ⎯⎯ → Ra = Σ a ( E0 ) φ0 HT 2008 Neutron Interactions 56 Non-1/v Absorbers There are a comparatively few important non-1/v absorbers. ∞ Ra = ∫ Σ a ( E ) v( E)n( E)dE It is dependent on the neutron energy distribution n(E). 0 Assuming Maxwellian distribution of n(E), C.H. Wescott computed Ra numerically. Ra = ga (T ) Σ a ( E0 ) φ0 Non 1/v factor HT 2008 Equilibrium temperature Neutron Interactions 57 Non-1/v Factors Cd In 135Xe 149Sm ga ga ga ga ga gf ga gf ga ga gf 20 1.3203 1.0192 1.1581 1.6170 0.9983 1.0003 0.9780 0.9759 1.0017 1.0723 1.0487 100 1.5990 1.0350 1.2103 1.8874 0.9972 1.0011 0.9610 0.9581 1.0031 1.1611 1.1150 200 1.9631 1.0558 1.2360 2.0903 0.9973 1.0025 0.9457 0.9411 1.0049 1.3388 1.2528 400 2.5589 1.1011 1.1864 2.1854 1.0010 1.0068 0.9294 0.9208 1.0085 1.8905 1.6904 600 2.9031 1.1522 1.0914 2.0852 1.0072 1.0128 0.9229 0.9108 1.0122 2.5321 2.2037 800 3.0455 1.2123 0.9887 1.9246 1.0146 1.0201 0.9182 0.9036 1.0159 3.1006 2.6595 1000 3.0599 1.2915 0.8858 1.7568 1.0226 1.0284 0.9118 0.8956 1.0198 3.5353 3.0079 T ºC 233U 235U 238U 239Pu Ra = ga (T ) Σ a ( E0 ) φ0 A small indium foil is placed in a reactor where 2200 m/s flux is 5×1012 n/cm2s. The neutron density can be represented by a Maxwellian distribution with a temperature of 600 ºC. At what rate are neutrons absorbed per cm3 in the foil? NIn = 0.0383×1024 and σa(E0) = 194 b. Ra = 1.15×7.43 cm-1×5×1012 n/(cm2s) = 4.27×1013 abs/(cm3s) HT 2008 Neutron Interactions 58 Summary • • • • Cross-Section Definition and Meaning Mean Free Path, Mean Time Flux Definition and its Meanings Flux Attenuation HT 2008 Neutron Interactions 59 The END HT 2008 Neutron Interactions 60 Classification of Neutron Sources • Radioisotope neutron sources (small, portable, reliable, low-cost, no maintenance) – Fission source based on 252Cf (overwhelming favourite) – (α,n) sources – (γ,n) sources • Nuclear reactors • Accelerator-based neutron sources – proton and deuterium bombardment – electron bombardment and photo-nuclear reactions – Spallation neutron sources HT 2008 Neutron Interactions 61 NEUTRON SOURCES Source 124Sb-Be Half-life Reaction Neutron yield (n×s-1×g-1) Neutron energy (MeV) 60.9 d (γ,n) 2.7×109 140La-Be 40.2 h (γ,n) 107 210Po-Be 138 d (α,n) 1.28×1010 4.3 241Am-Be 458 y (α,n) 1.0 ×107 ~4 226Ra-Be 1620 y (α,n) 1.3×107 ~4 227Ac-Be 21.8 y (α,n) 1.1×109 ~4 239Pu-Be 24400 y (α,n) 109 ~4 228Th-Be 1.91 y (α,n) 1.7 ×1010 ~4 252Cf 2.65 y fission 2.3×1012 2.3 stibium-antimony HT 2008 Neutron Interactions 0.024 2.0 62 Californium Source 252 98 248 96 Cf Channel 1: 97% 252 98 N ∼ e −0.88 E sinh Cm ( 2E ) α (6 MeV) Cf γ γ Channel 2: 3% 252 98 3.8 n (185 MeV) Cf FP FP HT 2008 Neutron Interactions 63 Fission and Spallation HT 2008 Neutron Interactions 64 Neutron Discovery • In 1930 W. Bothe and H. Becker in Germany: α → light elements (Be, B, Li); unussually strong penetrating radiation was produced. • In 1932 Irène Joliot-Curie and Frédéric Joliot in Paris: (unknown) radiation → paraffin or any other hydrogen containing compound it ejected protons of very high energy. • Finally (later in 1932) the physicist James Chadwick in England performed a series of experiments showing that the gamma ray hypothesis was untenable. HT 2008 Neutron Interactions 65 NEUTRON DISCOVERY Sir James Chadwick, 1932 (Nobel prize - 1935) 210Po α Neutrons from 9 4 Be ( α,n ) 126 Be Converter: H, Li, Be, B, N α Be target Aluminum sheets Ionization chamber Signal H2, Ne, N2, O2 Elastic scattering Mme I. Curie and F. Joliot had an idea: 9 4 Be + 42 He → 136 C + γ Chadwick guessed: 9 4 Be + 42 He → 126 C + 01 n + γ HT 2008 Neutron Interactions 66 Mass Evaluation n,m M v1 v0 Applying collision laws Chadwick derived: V1 M - nucleus mass m - neutron mass v0 - neutron velocity before collision v1 - neutron velocity after collision V1 - nucleus velocity after collision ⎧ m ( v0 + v1 ) = MV1 2m ⎪ ⎯⎯ → V1 = v0 1 ⎨1 2 2 2 M+m ⎪⎩ 2 MV1 = 2 m ( v0 + v1 ) V1 was determined for two types of recoil nuclei. Masses of 11 5 11 5 B and 14 7 N were known, so through the reaction B + 42 He → 147 N + 01 n Chadwick evaluated m = 1.2 mp . Current measurement: m = 1.0014 mp HT 2008 Neutron Interactions 67 Neutron Composition (udd) Family Fermion Interaction u Gravity, Electromagnetic, Weak, Strong Antiparticle Antineutron Discovered J. Chadwick Electric charge 0 (qn < 4×10-20 e) Magnetic mom. µn = -1.04187564 × 10-3 µB Spin 1/2 d d n → p + e− +ν + 1.29 MeV Decay t1 2 = 10.3min; τ = 14.9min mn = 1.6749543 × 10-27 kg = 1.008665012 u Mass = 939.5731 MeV/c2 = 1.0014 × mp = 1839× me HT 2008 Neutron Interactions 68 NEUTRON SOURCES: Fission, Fusion, Spallation Nuclear Reaction T (d,n) W (e,n) Be (d,n) Fission 235U (n,f) Fusion (T,d) Pb spallation 235U spallation HT 2008 Number of Energy neutrons per (MeV) particle or event 0.2 8×10-5 n/d 35 1.7×10-2 n/e 15 1.2×10-2 n/d 2.2 ~1 ~ GeV ~ GeV 2.5 n/fission 1 n/fusion 20 n/p 40 n/p Neutron Interactions Heat deposition (MeV/n) 2500 2000 1200 80 17 23 50 69 Photo Neutron Sources H+ γ → 11 H+ 01 n Q = −2.226 MeV Be + γ → 84 Be + 01 n Q = −1.666 MeV 2 1 9 4 All other target particles have much higher binding energy HT 2008 Neutron Interactions 70 Charged Particle Bombardment These neutron sources are based on electro static accelerators or cyclotrons. Isotope 7Li(p,n)7Be Hydrogen Nucleus 1H 1H+ = p proton Deuterium D = 2H 2H+ = d deuteron T = 3H 3H+ = t triton 3H(d,n)3He 2H(d,n)3He 3H(d,n)4He 1H(t,n)3He 1H(7Li,n)7Be Tritium HT 2008 Neutron Interactions 71 Nuclear Reactors: HFL (High Flux Reactor in Grenoble) 1. Core. 2 Heavy water reflector. 3 Light water pool. 4 Cold source. 5 Hot source. 6 Horizontal channel. 7 Concrete shield. HT 2008 Thermal neutron spectrum of HFR Neutron Interactions 72 IBR-2 Reactor in Dubna (Russia) HT 2008 Neutron Interactions 73 IBR-2 HT 2008 Neutron Interactions 74 Important ν ≈ 2.5 n/fiss εf ≈ 200 MeV/fiss MeV = 1.602 × 10-13 J Pthermal = Nfissions • εf • MeV [W] = [#fiss/s] • [MeV/fiss] • [J/MeV] n(r,E,t)d3rdE = Number of neutrons in d3r about r with energies in dE about E. ∞ Pth ( t ) = ε f ∫ ∫ σ f ( r , E ) N F ( r ) vn ( r , E, t ) d 3 rdE 0V HT 2008 Neutron Interactions 75