Experimental study on the characteristics of low power microwave plasma jet within local vacuum environment Juan Yang* Yang Qiao Xu Bing Zhu Gen Wang Mao Liang Ming Zhu College of Astronautics, Northwestern Polytechnic University, Xi’an 710072, China A microwave plasma jet based on a coaxial cavity can be generated in atmosphere and vacuum environment. It is shown that with argon gas and a power range of 53~60W, cavity efficiency ranges from 54 to 68%. The electron density distribution and the microwave return loss of the confined plasma jet adjacent to a metal object and their dependency on argon mass flow rate and power have been studied by applying emission/Langmuir probe and spatial reflected wave diagnostic equipments in a low scatter vacuum environment. The results show that the electron density ranges from 8.8×1014 to 7.53×1016 /m3, the electron density on the centerline of the jet decreases exponentially from the nozzle exit plane, but its distribution off the centerline is in up heaved curve. Increasing mass flow rate at constant power and increasing power at constant mass flow rate increase electron density mildly. From typical measurements of microwave return loss, it is noted that the plasma jet attenuates microwaves in 6 to 8GHz range. *yangjuan@nwpu.edu.cn Ⅰ. Introduction Plasma can be generated through electron-impact and photon ionization. In the electron-impact process, energy for sustaining the plasma can be provided via hot arcs and radio frequency waves of all frequencies. Of all the possibilities, microwave ionization for sustaining the plasma has the advantage of low power, cathodeless operation than the hot arc. The microwave generated plasma has been applied in deep space detection1-2 and is under study for future applications in space propulsion3-4. Another possible application is radar cloaking in which an object with high scattering coefficient is covered with a plasma cloud which absorbs incident microwave radiations. Plasma concealment is more effective and flexible5-8 compared with body design and wave absorbing coating methods. According to the theory of microwave propagation, effective wave absorption by non-collision plasma is governed by the relationship between the microwave and plasma frequency. The condition of microwave 2 2 2 propagation and absorption in a plasma is electron density n p n cr , where n cr 4π m e ε 0f /e is the cutoff density. When n p n cr , the wave can not penetrate the plasma and is reflected. For collision plasma, the relationship among wave attenuation, wave and plasma frequency, and particle collisional frequency is complicated. The plasma characteristics such as electron density and particle collisional frequency greatly affect wave attenuation9-10. Therefore, to be an attractive wave absorber, the plasma must have an appropriate electron density for a given background pressure and given wave parameters. For application study of radar cloaking, a large number of references cover numerical simulations11-15 and a few experimental research16 related to the interaction between microwaves and plasmas. Numerical simulations assume the plasma model as uniform or non-uniform slabs or balls with special electron density distributions. However, actual plasma can not be represented by these regular shapes. It is a complicated task to simulate wave propagations in plasma when it has a non-regular shape. Based on the aforementioned background, it is necessary to experimentally study the characterization of the actual plasma jet. As shown in Figure 1a), our experimental model consists of a low power microwave plasma generator operating at 2.45GHz and less than 60W, and a quartz container and metal plate. The experimental model is positioned in a large vacuum chamber to create a vacuum background. A plasma jet from an exit hole of the generator cavity is sprayed into the container. Its electron density distribution is characterized by 1 emission/Langmuir probe. The metal plate and the end of the cavity are strong scatter objects, and the plasma jet enveloping them can be considered a microwave absorbent coating. When the experiment model is put into a low scatter vacuum chamber, the microwave return loss in the near field of a measuring antenna can be obtained using the spatial reflected wave measurement method. Experimental results and analysis explain the effects of an actual plasma jet on microwave absorption in the near field of the antenna. a) b) Fig.1 Experimental system (dimensions in mm)a) Integrated experimental set upb) Cavity structure and field distribution Ⅱ.Experimental Setup A.Microwave plasma generator and experimental model As shown in Figure 1a), a low power microwave plasma generator is composed of three parts: solid state microwave source, a cavity and a gas supply subsystem. The solid state microwave source changes the electric power into microwave energy at 2.45GHz and less than 60W, which is transferred to the cavity through a coaxial circulator with three ports. The reflected microwave energy from the cavity can be transmitted to the attenuated detector for examination. Figure 1b) shows the cavity, in the form of coaxial structure with a concentrated capacitance. It is composed of an inner and outer conductor and a coupling probe. Radial and axial electric intensity Er and Ez, tangential magnetic intensity HΦ exist in the cavity. Near the end tip of the inner conductor, Er and Ez become stronger, creating a favorable condition for gas breakdown. Also, the gap between the end tip of inner conductor and the inner side of outer conductor forms a concentrated capacitance, which results in the cavity length being less than a quarter wave length. When gas is injected, it is ionized in the strong electric field zone and the resultant plasma jet is accelerated through the nozzle. In Figure 1b), the inside surface diameter of the outer conductor and outside surface diameter of the inner conductor are chosen to be 40 and 10 mm, respectively, based on the consideration that the structure must suppress the appearance of an inhomogeneous wave mode and support maximum power. Another compromise is that the cavity must have high quality factor. The length of the cavity is chosen to be 31mm, which is less than the quarter wave length at 2.45GHz. The nozzle throat diameter is chosen as 0.6mm in order to sustain appropriate gas pressure in the cavity and appropriate mass flow rate. Including the microwave plasma generator, the experimental model is built up as shown in Figure 1a). It is composed of the cavity, metal plate and quartz container with 260mm in diameter and 300mm in length. A pipe is joined on the metal plate, which is used to vacuum the container when this model is placed in a large vacuum chamber. B.Emission/Langmuir probe The Langmuir probe is an effective tool for diagnosing the distribution of plasma electron density. The theory of the Langmuir probe is based on the assumption that the probe radius is small compared to the collision mean free paths but large compared to the Debye length, which means when charged particles impact the probe biased from negative to positive voltage, they must be completely absorbed by the probe. It is important to define the charged particle collecting area of the probe surface in order to calculate the electron and ion collection current. 2 Also, obtaining the electron saturation current is important for calculating the electron density according to the I-V characteristics of probe. But when the probe is immersed in the plasma jet there will appear a wake region, in which the charged particles may not be absorbed normally. Sometimes, the thickness of this plasma shell increases slowly with an increase in the probe potential, which causes the electron collecting area and current to increase slowly. This circumstance makes it difficult to accurately define the charged particle collecting area and electron saturation current. Therefore, another method is needed to specify the point at which the electron saturation current appears on the probe’s I-V curve. The emission probe is an effective tool for doing this. The emission probe is a tungsten filament heated by current. When the current is too low to induce the filament to emit electrons, the I-V characteristic of the probe is same as that of the Langmuir probe. But when current is increased to a high level, the filament emits electrons. As shown in Figure 2, in the ion saturation region, the filament potential is lower than that of the plasma, and the emission electrons can come into space without resistance to generate greater emission electron or ion current than Langmuir probe. At the electron saturation region, the filament potential is higher than that of the plasma, which leads the surrounding electrons to be absorbed by the filament but the emission electrons are turned back. In this region, although the emission probe is heated by current, the I-V curve is same as Langmuir probe. When the filament potential counterbalances with that of plasma, the emission electrons will begin to come into the surrounding area and the I-V curve drops suddenly. In this situation, plasma spatial potential can be defined accurately and electron density can be calculated. According to the similarity and difference between I-V characteristics of emission and Langmuir probes, the emission probe can be applied to diagnose not only the plasma spatial potential but also electron density. The diagnostic arrangement is illustrated in Figure 1a). Since the experimental setup is fixed in a large vacuum Fig.2 I-V characteristics measured by emission probe chamber, the probe penetrating through the metal plate is mounted on a stand that allows it to be shifted in the axial direction of the cavity. C.Low scatter vacuum experimental environment and microwave measuring equipment The integrated experimental system is also shown in Figure 1a), in which the vacuum chamber of 1.2m in diameter and 3m in length is lined with a rubber wave absorber for a low scatter vacuum environment. The chamber is pumped by two sets of Lobe-type vacuum pumps. They maintain a background pressure of less than 10Pa throughout the experiments. Testing has shown that the chamber wall lined with the rubber wave absorber can attenuate microwaves by 10dB from 4 to 10GHz. The experimental model is mounted in this environment to investigate the effect of the plasma jet on shielding the metal plate from microwaves. One pair of transmitting and receiving antennas is mounted 520mm from the metal plate. The distance between the centerlines of the two antennae is 170mm. The antenna exit plane faces the metal plate, such that the transmitting antenna emits a test wave supplied by the network analyzer toward the metal plate and cavity, through the quartz container and the plasma jet. The receiving antenna receives the reflected microwave passing through the reverse path and transmits it back to the network analyzer. The measured parameter is the wave return loss Lr 10lg Pr Po , where P0 is the microwave power induced by the network analyzer and Pr is the reflected power. When the transmitting antenna propagates the test wave toward the metal plate and cavity, the plate and cavity will reflect wave toward all sides. Neglecting the quartz effect on the microwave, the received microwave power Pr by the receiving antenna is composed of Pr1 and Pr2. Pr1 is directly from the metal plate and cavity, Pr2 is from the rubber wave absorber lining on the chamber wall. Pr2 is less than Pr1 because the absorber will attenuate 3 the incident microwave power by about 90 percent (10dB return loss). Before generating plasma, Lr is first calibrated to zero, which means that Pr is at a reference level. After plasma is generated, the plasma may also ' reflect microwaves in all directions. Assuming the total power received by the receive antenna is Pr , which is also ' ' ' ' composed of Pr1 and Pr2 , Pr1 comes directly from the metal plate and plasma jet. Pr2 is from the absorber. Pr1' contains the main part of Pr' . Therefore the return loss L' r of the test wave propagating into the plasma jet surrounding the metal plate and cavity can be obtained and gives the shield effect of the plasma jet. One pair of horn antennas, operating frequency ranges from 6 to 8GHz, is used in the measurement. One Fig.3 Antenna structure of their structures is shown in Figure 3, where the E and H plane is defined as that parallel and perpendicular to the electric intensity. The dimensions of their exit planes are chosen as 200mm×200mm for matching the cross section of the plasma. Ⅲ.Experimental results and analysis A. Microwave plasma jet generation In order to reduce the reflected microwave power from the cavity to a minimum level, the cavity of plasma generator must be regulated on network analyzer and the microwave source with low output power respectively to match the impedances of cavity and its input. Then plasma can be formed within the cavity with high efficiency and exits through the nozzle, at microwave output power up to 40W. Experimental results: (1) Microwave power for sustaining plasma can be reduced after the gas discharge. After the plasma is started at 40W, it can be steadily sustained at 30W. Before an equilibrium state is reached, electrons diffuse rapidly to the boundary and electrons determine the plasma diffusion coefficient. After the ionized gas reaches equilibrium, plasma shell is formed and induces additional ion diffusion, which establishes the plasma ambipolar diffusion coefficient as defined by fast electron and low speed ion movements. Electrons in the equilibrium plasma will be confined by the static bipolar electric field. This makes the electron diffusion coefficient less than that in a free moving environment and thus decreases the microwave power required to maintain equilibrium plasma. (2) Pressure required to sustain large volume plasma jet. Experiments shows that 0.5~2atm absolute pressure within cavity can produce a large volume plasma jet. When the cavity absolute pressure is greater than 2atm, the volume of cold gas passing through the discharge zone is too large for the available microwave energy. This decreases the ionization percentage. On the other hand, when the cavity absolute pressure is less than 0.5atm, although gas can absorb enough microwave energy and, thus, there is a high degree of ionization, lower pressure produces lower plasma exit speed and a smaller jet volume. (3) Strong cavity coupling will reduce the reflected power from the cavity and stabilize operation. The loaded quality factor QL is a performance parameter of the plasma generator cavity. It is defined as 1 QL =1 Q0 +1 Qe , where Q0 is the intrinsic quality factor of the cavity which is defined only by its structure, Qe is the plasma load quality factor. Defining Pd as the power loss on the cavity wall and Pe as the power absorbed by plasma within the cavity, results in a coupling coefficient β= Pe Pd = Q0 Qe , and QL = Q0 1+ 17. At 4 given cavity structure, QL is defined by β, which is affected by the coupling probe shape and the gap between the probe and the inner conductor. Resonant experiments show that a high coupling coefficient corresponds to a small gap between probe and inner conductor, and a low loaded quality factor QL reduces reflected microwave power from the cavity and increases the operating frequency band, which makes the generator operation more stable. Defining Fig.4 Cavity coupling efficiency vs. mass flow rate eff Pout Pr Pout as the cavity coupling efficiency, where Pr is the reflected power from the cavity and Pout is the output power from microwave source, the efficiency curves as a function of the variation in argon mass flow rate at atmosphere and vacuum conditions are given in Figure 4. The curves show that the cavity efficiency ranges from 54 to 68% at microwave output power levels of 53 to 60W. At a fixed mass flow rate, cavity efficiency increases as output power increases. At fixed output power and mass flow rate, the cavity efficiency in vacuum is greater than that in atmosphere. B.Electron density Three bend probes are installed in the experimental model as shown in Figure 1a), in which one filament is on the centerline, and the other two are 50mm and 80mm from the centerline. Although the probes can be moved continuously in the axially direction, diagnostics are taken starting at 20mm from the nozzle exit plane and in 25mm intervals. The probe insertion depth into the experiment model is limited to 170mm because of the interference between the probe stand and the experiment model. At each location, three points of power and five points of argon mass flow rate are applied: 46W, 52W and 59W, 21 mg/s, 42 mg/s, 63 mg/s, 84 mg/s and 105mg/s. (1) Spatial distribution at constant power and dependency on mass flow rate. Figure 5 shows electron density profiles in the axial directions with various mass flow rates at microwave output power of 59W. L and r are the distances from the nozzle exit plane and the centerline of the plasma jet, respectively. The diagnosed density ranges from 9.6×1014 to 1016/m3. It can be seen from the profiles showed in Figure 5a) that axial electron density along the centerline decreases exponentially from the nozzle exit plane at every mass flow rate. The dependence is consistence with that presented in Reference 18. The difference is due to the effect of the quartz container on the plasma jet. The same variation of mass flow rate induces less discrepancy in electron density in a confined plasma jet, but noticeable variation in a free plasma jet. Figures 5b) and c) show that the plasma in the middle part of jet is denser and diffuses farther than the two ends, which was anticipated since it is known that the nozzle plume has the same characterization. Electron density is more sensitive to the mass flow rate when the position is far from the centerline and close to the nozzle exit plane. a) b) c) Fig.5 Axial electron density distribution with various mass flow rates at 59W output power a) r=0, b) r=50, c) r=80mm 5 (2) Spatial distribution at constant mass flow rate and its dependency on output power. Figure 6 shows electron density profiles in the axial directions at various microwave output powers and mass flow rate of 63mg/s. Electron densities range from 8.8×1014 to 7.52×1016/m3. All the profiles show that increasing microwave output power increases the electron density in the plasma jet. This is consistent with Figure 4 in the plasma generation experiment. When the microwave power is transmitted into the cavity filled with about 1atm gas, the collision frequency of the particles in the induced plasma is very high which means power is absorbed without the limitation of the electron cutoff density. This results in an increasing percentage of ionization and electron density with increasing microwave power. The profiles show that at far distances from the centerline and nozzle exit plane, electron density is more sensitive to microwave power. a) b) c) Fig.6 Axial electron density distribution with various power levels at 63mg/s mass flow rate a) r=0, b) r=50, c) r=80mm C.Microwave return loss The antennas are mounted such that the E plane is parallel to the ground level, which is called horizontal polarization. Two points of power and three points of argon mass flow rates are applied: 46W, and 59W; 21 mg/s, 63 mg/s, and 105mg/s. Calibration of the experimental model is accomplished by pumping the chamber to 0.1 Pa, then adjusting the mass flow rate to 105 mg/s which causes the background pressure to increase to about 5 Pa. Figure 7 shows the calibration plot with antennas in horizontal direction. The plot shows deviation amplitude of 0.135dB, which can not be zeroed out after many calibrations. It is caused by the vibration of the experimental system. The measurements of the horizontal polarized wave return losses in the plasma jet are given in Figure 8. Different symbols present the different experimental data taken at different power, and different lines present the associated curve fits. Experimental data shows an obvious frequency oscillation, which can be explained by the vacuum chamber and plasma jet being regarded as a big resonant cavity with a disturbance object in it. At a given frequency point, if the plasma state is in resonance with the chamber, more detection power will be absorbed by the plasma and the chamber. Fig.7 Calibration profile of experimental model We call this abnormal absorption. The return loss measured at a non resonant frequency can actually give the wave attenuation in the plasma jet. Otherwise, curve fits can correct the data at the resonant frequency. Profiles in Figure 8a) show wave return loss at mass flow rate of 21mg/s is nearly zero because of the small volume of generated plasma. Figure 8b) gives the wave return loss at a mass flow rate of 63mg/s and microwave power of 59W and 46W. The profiles show the wave return loss decreases gradually from 5dB to 0. Figure 8c) gives the wave return loss at a mass flow rate of 105mg/s and microwave power of 59W and 46W. The profiles have the same variation as Figure 8b), but Figure 8c) shows from 6 to 8GHz the maximum of the wave return loss reaches 7dB. Reference 19 reports that the plasma plume of an arcjet operating at back ground pressure of 53Pa has the 6 same electron density magnitude as this microwave plasma jet. The arcjet can only attenuate microwaves from 1 to 4GHz. The attenuation decreases with increasing frequency. The reason is the increasing wave frequency induces low wave spatial damping rate. The variation trend reflected by Figure 8 is same as Reference 19, but their magnitude is different, which is caused by the different experiment conditions. a) b) c) Fig.8 Wave return loss a) at 21mg/s flow rate, b) at 63mg/s flow rate, c) at 105mg/s flow rate Ⅳ. Conclusions A solid state microwave source at 2.45GHz frequency and a coaxial cavity comprises a compact, low power microwave plasma jet generator. It produces a stable plasma jet in atmosphere and vacuum at a microwave power of less than 60W. The present work is unique in two respects. First, an emission probe is applied to diagnose the plasma jet confined by a quartz container and enveloping a metal plate. This probe characterizes the shape of the plasma jet, the electron density distribution and its dependence on mass flow rate and microwave power. At microwave powers of 46W, 52W and 59W, and mass flow rates of 21mg/s to 105mg/s, the diagnosed electron density ranges from 8.8×1014 to 7.53×1016/m3. The electron density on the centerline of jet decreases exponentially beyond the nozzle exit plane. Its distribution off the centerline is in the shape of up heaved curve. Second, using spatial reflected wave measurement diagnostic equipments, the attenuation of the horizontal polarized wave by the confined plasma jet enveloping a metal plate is measured in a low scatter vacuum environment. The data shows that the plasma jet can attenuate the incident microwave. For construction of a low scatter environment, we can choose a different type of wave absorber, a soft rubber with small bubbles and plain rubber. Although the soft rubber can attenuate microwaves more than 30dB and provide a very low scatter environment, its volume is too large for the vacuum chamber, and out gassing from its small bubbles overwhelms the vacuum system. Therefore, we chose plain rubber which is small in volume and has a solid interior. 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