ENEL Società per azioni Main Features of ECART Enel Code for Analysis of Radionuclide Transport ECART is a computer code of ENEL-EDF common property Periodical revisions, updates and improvements are managed by ENEL Research Branch Requests of information can be addressed to: Flavio Parozzi - ENEL Research via Reggio Emilia 39 20090 Segrate (Milano) - Italy tel: +39-02-21.67.23.10 fax: +39-02-21.67.26.20 e-mail: flavio.parozzi@s1.cise.it SUMMARY SUMMARY.................................................................................................................................................... 2 INTRODUCTION TO ECART.................................................................................................................... 3 MAIN FEATURES AND CODE ARCHITECTURE ................................................................................ 3 BRIEF HISTORY OF THE CODE ....................................................................................................................... 3 CODE STRUCTURE AND MAIN ASSUMPTIONS ................................................................................................ 4 OVERVIEW OF THE THERMAL-HYDRAULIC MODELS ................................................................. 6 MAIN FEATURES .......................................................................................................................................... 6 CAPABILITY TO ANALYSE BOTH CONTAINMENT AND PRIMARY SYSTEM SCENARIOS ..................................... 6 CAPABILITY TO PROCESS EXPERIMENTAL DATA ........................................................................................... 7 OVERVIEW OF THE AEROSOL AND VAPOR MODELS ................................................................... 7 MAIN FEATURES .......................................................................................................................................... 7 TRANSPORT OF VOLATILE FISSION PRODUCTS .............................................................................................. 8 TRANSPORT OF AEROSOL PARTICLES ........................................................................................................... 8 OVERVIEW OF THE CHEMISTRY MODELS ..................................................................................... 10 RUNNING OF THE COUPLED MODULES ........................................................................................... 12 COMPUTER TIME REQUIREMENTS ............................................................................................................. 13 Tables Figure 1: Schematic of the linking among the three main modules of ECART: ................. 5 Figure 2: Control volume model adopted for ECART code................................................ 7 Figure 3: Schematics of the transport phenomena considered by the Aerosol and Vapour Transport Module in each control volume. ................................................................. 9 Figure 4: Example of log-normal aerosol particle size distribution and corresponding discretization.............................................................................................................. 10 Figure 5: Example of the fitting function used to calculate the decay specific power associated to an element, as a function of accident time and fuel irradiation time. .. 12 Figure 6: Example of ECART prediction of suspended masses of Caesium compounds transported from the primary circuit into the containment, for a typical PWR small break. ......................................................................................................................... 13 INTRODUCTION TO ECART The realistic calculation of the radionuclide transport within a nuclear plant and the release to external environment during an accident involving a severe damage of the fuel rods requires an appropriate evaluation of the thermal-hydraulic conditions influencing both the chemical equilibria among the involved chemical species and the radionuclide retention phenomena. Also, the path followed by the radioactive stream before being released to the environment through the potential containment leakages must be carefully simulated in relation to the aerosol removal mechanisms which may occur in the presence of heat structures and considering radionuclide scrubbing favoured by steam condensation and bubbling through liquid sumps. During the '80s, in connection with the increased interest in Source Term problems and in parallel with the large-scale experimental programs, several versions of computer codes for Source Term analysis were released. In the same period, the need to have well-known and well documented tools adapted to national studies, led to the development of dedicated versions differing from the original ones. In this context, the Italian utility ENEL built up an its own version of some STCP codes (Source Term Code Package) set up for US NRC, paying particular attention to the aerosol transport modelling. TRAPMELT and NAUA, for instance, were improved and tested by ENEL on the basis of the results of Marviken, LACE and DEMONA series of experimental tests on the aerosol behaviour. These tools, together with other ENEL-adapted versions of this type of codes, were successfully employed in the Italian Source Term studies for PWR and BWR plants, and in the preliminary sizing verifications for the EU/CEA Phebus-FP and EU/JRC Ispra STORM Projects. ECART was born starting from those experiences. This new code was aimed at representing the “container” of mechanistic radionuclide transport models developed in the framework of experimental programs, able to couple aerosol/vapour transport with thermal-hydraulic and chemical equilibria calculations, and taking into account, at the same time, the need to have a computer code reasonably utilisable for plant analyses. MAIN FEATURES AND CODE ARCHITECTURE Brief history of the code The work on ECART started at ENEL in 1989 with the valuable support of Synthesis, which defined the code architecture and built up the Aerosol/Vapour Transport Module. The first stand-alone version of this Module, in particular, was used in 1990 to run new aerosol models, like those for steam condensation within pipeworks and particle dry resuspension, developed in the framework of EU Reactor Safety Research Programs 1988-91 [Parozzi 1991; Borioli 1992]. In the following years, the Aerosol/Vapour Transport Module was continuously updated in the framework of a wide validation campaign. This module, often quoted in literature as the bulk of ECART itself [Wright 1994; Bowsher 1995], was widely used for research purposes, like the STORM Project and the RCA Source Term Project of the European Union [Eusebi 1992; Parozzi 1995b]. Since 1993, through an agreement between EDF-SEPTEN and ENEL related to joint research actions on LWR severe accident studies, EDF started a significant financial and technical contribution to the development and validation of ECART, involving its Research and Development Division of Chatou: the Aerosol/Vapour Transport Module, then, was submitted to a further revision in France by CNRS [Blawzdziewicz, 1995] and was used on reference primary circuit transport problems for a detailed comparison with the aerosol results given by MAAP [Hervouet 1995]. Still in the framework of EU Reactor Safety Research Programs 1988-91, ENEL carried out a phenomenological research related to the chemical behaviour of fission products in the gas stream after their release from the fuel and their dependence on parameters like temperature, pressure and hydrogen-to-steam ratio [Borioli 1992]. On the basis of that study, the Chemical Equilibria Module was set-up with a significant contribution of the Industrial Chemistry and Chemical Engineering Department of Politecnico of Milano: after a successful series of stand-alone tests on theoretical problems and chemistry benchmarks, this ECART module was completed in 1994 [Biardi 1993]. At the Mechanical and Nuclear Constructions Department of University of Pisa, starting from the experience on thermal-hydraulic analysis of nuclear accidents and FUMO containment code modelling, the Thermal-Hydraulic Module was developed with a significant support of Themas. A preliminary version of this module was completed in 1993 and successfully tested on a large series of theoretical problems and code benchmarks on experimental situations [Oriolo 1995]. In 1995, the fully-coupled version of ECART was finally employed on typical PWR severe accident scenarios and experimental benchmarks, like those on VANAM-M3 and Phebus FPT0 [Ambrosini 1995; Paci 1996; Parozzi 1996; Salina 1996]. Code structure and main assumptions ECART is designed to operate with three modules, linked together, but able to be activated separately (Figure 1): the Thermal-Hydraulic Module, providing the boundary conditions to the other two modules; the Aerosol and Vapour Transport Module, calculating the amount of radionuclides that can be retained or released; the Chemical Equilibria Module, evaluating chemical reactions occurring among radionuclides. The code applies to pure transport phenomenology (mass, energy, momentum transfer and physico-chemical processes in whatever part of a nuclear power plant). As designdependent models are not included (e.g. core degradation, releases from fuel, safety systems, etc.), the complete analysis of a severe accident requires the linking with other suitable code packages. The structure of ECART is designed to treat the thermal-hydraulic phenomena and the radionuclide transport in an arbitrary flow system, that the user can subdivide into a series of control volumes connected by flow junctions in an arbitrary way, and chosen on the basis of considerations regarding geometrical features, thermal-hydraulic conditions and relevant radionuclide phenomena. As shown in the following, the detail level of aerosol and vapour transport analyses can be also decided by the user (i.e. the number of chemical species, the number of aerosol size discretization bins, the occurrence of agglomeration and the multicomponent description). These choices have obviously great influence on the computing time. Inside each control volume, a two-region model is adopted, being the liquid sump separated from the atmosphere. Within each region, thermal equilibrium is always assumed. Therefore, non-equilibrium effects related to superheated vapour injected in the pool or subcooled water sprayed in the atmosphere are separately accounted for. Also aerosols are assumed to be well-mixed inside the volumes. This assumption requires that the amount of vapour and/or aerosol removed within the control volume is “small” in relation to the total amount of material transported throughout the control volume itself. A corrective action is provided for those volumes, like long pipes, having only a radial mixing (concentration gradient along the pipe). The direction and the rate of the flow can be directly assigned as input, together with other thermal-hydraulic boundary data, or can be predicted by the thermal-hydraulic module. The direction of flow can change with time, although the aerosol transport through junctions is treated as one-dimensional (i.e. there is not simultaneous mixing through a junction). Two-dimensional flows, however, required to simulate accident scenarios or large-scale experimental situations where the natural convection currents could enhance the mixing among the volumes, can be accounted for using two junctions to describe the exchanges between two volumes. Recirculation phenomena promoted by density gradients of the carrier gas at the inlet of large components (e.g. chimney-effect caused by hot gas or hydrogen injection) are taken into account by aerosol models, in the absence of any sub-nodalization, through the estimate of a “recirculation velocity” [Masnaghetti 1987]. THERMAL HYDRAULICS 5 1 CHEMICAL EQUILIBRIA 4 2 3 AEROSOL TRANSPORT Figure 1: Schematic of the linking among the three main modules of ECART: 1. 2. 3. 4. 5. t-h boundary conditions for chemical equilibria; selection of quantity of each chemical compound in gaseous phase; species concentrations for updating chemical equilibria; t-h boundary conditions for aerosol and vapours transport phenomena; decay heat sources associated to transported fission products and aerosol concentrations capable to modify gas physical properties. OVERVIEW OF THE THERMAL-HYDRAULIC MODELS Main features The study of the thermal-hydraulics of primary system and containment during last decades provided a plenty of possible options to simulate the thermal-hydraulic behaviour of nuclear light water reactors. Specific modelling requirements are generally identified for the simulation of DBAs or severe accidents and of primary system or containment phenomena, suggesting different choices in the selection of models and of the level of detail to be used in plant description. Basing on previous experience in the development and application of models for analysing the thermal-hydraulic behaviour of LWRs during postulated accidents [Ambrosini 1987, Manfredini 1992, Ambrosini 1992, Ambrosini 1996] and considering the peculiarities of the existing Aerosol and Vapour Module, the following characteristics were agreed for the Thermal-Hydraulic Module: capability of describing LWR thermal-hydraulic transients, with the degree of detail required by the aerosol module, and of processing incomplete experimental data providing the lacking information on local behaviour; solution of mass, energy and momentum balance equations in order to provide for realistic representations of flow and heat transfer; transport simulation of the aerosol carrier gases expected within LWR plants under accident conditions and usually employed in experimental test (steam, argon, helium, hydrogen, carbon dioxide, carbon monoxide, krypton, nitrogen, oxygen and xenon); calculation of pool levels in the control volumes and evaluation of steam suppression effects to support the aerosol scrubbing phenomenology; steam condensation modelled by splitting bulk and wall condensation (influencing, respectively, aerosol growth and aerosol diffusiophoretic deposition); allowance for counter-current flow conditions at junctions; capability of evaluating wall heat transfer taking into account wall thermal conductivity changes due to aerosol deposition and radioactive decay heat sources; possibility of characterising heat structure surfaces with local hydraulic parameters having strong influence on aerosol deposition and resuspension mechanisms (i.e. hydraulic diameter, local fluid velocity and Reynolds number, etc.). Capability to analyse both containment and primary system scenarios The assumption of complete stratification adopted in ECART control volumes is fairly well suited for severe accident containment analyses, but has some limitations in simulating primary system conditions. These limitations are accepted considering that, under core melt-down conditions, single-phase flow (superheated steam-hydrogen mixture) or stratified flow (formation of water sumps in cold components) is likely to occur within the reactor coolant system. A complete solution of the problem, obviously, would require flow regime maps and constitutive laws for interfacial area and heat transfer under the various regimes. However, this kind of accident scenarios, expected to be of minor importance in terms of radiological consequences (e.g. TMI accident or steam generator tube rupture), would imply removal mechanisms of fission products differing from those mainly influencing the source term associated to the severe accidents normally considered for probabilistic safety assessments. External Spray Door Heat Sink Blowdown jet Deentrainment Evaporation Liquid Film Junction Figure 2: Control volume model adopted for ECART code. Capability to process experimental data The capability to process incomplete experimental data to supply the lacking information consists in imposing the value of pressure, temperatures and void fraction in outer environments located upstream or downstream a given junction or to assign flow rates through particular fluid injection or removal devices, according to different possible choices (e.g., tables of flow as a function of time, pressure or level). OVERVIEW OF THE AEROSOL AND VAPOR MODELS Main features The Aerosol and Vapour Transport Module is based primarily on the validation and development work carried out for US NRC codes, and the knowledge coming from the participation in ATT-Marviken V, LACE, and DEMONA experimental programs [Parozzi 1988a; Parozzi 1988b]. The more recent results and models produced in the frame of the European Union Reactor Safety Research Programs, like the dry physical particle resuspension or the multicomponent description, are included [Borioli 1992; Parozzi 1995b]. Although ECART adopts the classical well-mixed assumption to describe the transport within each control volume, the deposition and resuspension phenomena can be described by dividing each control volume into sub-regions, where local thermalhydraulic conditions (temperature, gas flow velocity, etc.) can be taken into account. In this way, removal mechanisms associated to small pipes can be detected, without using too short time steps and ad-hoc running the aerosol equation. As already shown in Figure 2, each control volume can simulate the presence of liquid water at the bottom. A BWR suppression pool, large water tanks of advanced LWRs or time-varying sumps caused by steam condensation can be then modelled. Within each control volume, all phenomena that can be responsible for retention or re-entrance of radionuclides are taken into account using the same criteria (Figure 3). Transport of volatile fission products Because of their negligible latent heat, condensation and evaporation of volatile species onto and from airborne particles and structure surfaces are dynamically calculated by diffusion equations. Conversely, steam-water phase changes can be either calculated by the Thermal-Hydraulic Module or assigned as input data. The condensation and evaporation onto and from airborne particles promotes aerosol growth or shrink, while the presence of a liquid phase in an aerosol deposit can inhibit its resuspension. Irreversible sorption of I2, HI, CsOH and Te vapours onto internal surfaces is also modelled by adopting the usual deposition velocity approach. Transport of aerosol particles ECART works with discretized size distributions both for airborne and deposited particles (Figure 4) and always uses mono-component basic aerosol equations to compute the evolution of aerosol particles. The number of size bins is an input choice. Ordinary differential equations solvers with implicit integration methods allow to save computing time and prevent from numerical instabilities. Optionally, in order to give a multicomponent description of both airborne and deposited particles, the code can individually track the transported species in each size bin, accounting for all transport mechanisms. In more detail, the current particles mass in each size bin is distributed among the involved chemical species following all the particle transport phenomena accounted by the code (sources, particle growths or shrinking, depositions, resuspensions, etc.). The computational correctness and the stability of this algorithm, that represents the only available possibility to manage the multicomponent behaviour of aerosols with large catalogues of species, was tested through theoretical tests simulating typical LWR primary circuit conditions [Kourti 1995]. To simulate asphericity of aerosol particles, an aerodynamic shape factor (accounting for different resistance to motion of the actual particles if compared to the mass-equivalent sphere) and a collision shape factor (accounting for the increased effective collision crosssection) are adopted as size-dependent by the code. Agglomeration of suspended particles is based on the three classical mechanisms, usually modelled in this type of codes: : Brownian (Smoluchowski); Gravitational (collision between particles having different settling velocities); Turbulent, shear and inertial (Saffman and Turner). Particle growth due to bulk vapour/steam condensation is modelled taking into account the Kelvin effect (the condensation of steam is inhibited for particles having radii smaller than the critical radius), while particle deposition and resuspension onto and from surfaces is computed as the sum of several phenomena [Borioli 1992]: inertial impaction from turbulent flow (Liu-Agarwal); diffusion from turbulent flow (Davies); diffusion from laminar flow (Gormley-Kennedy); thermophoresis (Brock-Talbot); gravitational settling (Stokesian and non-Stokesian); centrifugation in curved pathways (Stokesian and non-Stokesian) accounting the trapping effect within bent pipes; diffusiophoresis (Schmitt-Waldmann); dry physical resuspension (force-balance correlation). In water sumps, the formation of bubbles and their evolution (growth, asphericity, breakup and rise velocity) are calculated on the basis of experimental data, while particle scrubbing is modelled accounting for inward and condensing steam, gravitational settling, particle diffusion and centrifugation. STEAM VAPORS DEPOSITION SURFACES PHYSICAL RESUSPENSION LAMINAR DEPOSITION TURBULENT DEPOSITION THERMOPHORESIS GRAVITATIONAL SETTLING WATER SUMP AEROSO L GROWTH CENTRIFUGAL DEPOSITION DIFFUSIOPHORESIS SUMP BUBBLING AEROSOLS Figure 3: Schematics of the transport phenomena considered by the Aerosol and Vapour Transport Module in each control volume. Number of particles 0.01 0.10 1.00 Particle radius [m] Figure 4: Example of log-normal aerosol particle size distribution and corresponding discretization OVERVIEW OF THE CHEMISTRY MODELS To set-up the Chemical Equilibria Module, it was necessary to identify the chemical species that can originate, under reference PWR severe accident conditions, in the gas stream after the release of the elements from the fuel. To meet this objective, a wide set of sensitivity calculations, exploring the dependence of the chemical speciation on gas temperature, pressure and hydrogen-to-steam ratio, was performed with SOLGASMIX code [Borioli 1992]. The Chemical Equilibria Module contains information for the most representative chemical species selected with that method (Table 1) and the solver algorithm is based on Gibbs free energy minimisation at constant pressure and temperature of the system: this allows the calculation of the equilibrium composition of the mixture in terms of molar fractions for the gaseous phase and in terms of the moles for the condensed phase. In order to manage the formation and evolution of radionuclide species within LWR primary circuits, this module is dimensioned for environments characterised by temperatures in the range from 1000 to 2500 K with pressures up to 15 MPa [Biardi 1993]. Within the ECART architecture, the possible reactants and reaction products considered by the Chemical Equilibria Module are the carrier gas components, with the exception of nitrogen and noble gases, and most of the transported species which are airborne as gases or vapours. To match with the phase change models of the Aerosol and Vapour Transport Module, supersaturation conditions of the predicted vapours are accepted. The databases of the Chemical Equilibria Module are also used by ECART to determine the temperature-dependent saturation pressures of all volatile species. Table 1: Catalogue of the chemical species available in ECART. Species Ag AgI B BI3 B2O3 Ba BaI BaI2 BaO BaOH Ba(OH)2 C Cd CdI CdI2 CdO Cd(OH)2 CdTe CH4 Cr CrI CrI2 CrO Cr2O3 Cs CsBO2 CsI CsO CsOH Cs2 Cs2CrO4 Cs2MoO4 Cs2O Cs2(OH)2 Cs2Te Cs2TeO3 Cs2ZrO3 Fe FeI2 FeO Fe2I4 Fe2O3 Fe3O4 H HBO2 HI H2O H2Te H3BO3 I I2 Silver silver iodide Boron boron triiodide boron sesquioxide Barium barium monoiodide barium iodide barium oxide barium hydroxide barium dihydroxide Carbon Cadmium cadmium monoiodide cadmium diiodide cadmium oxide cadmium dihydroxide cadmium telluride Methane Chromium chromium monoiodide chromium diiodide chromium oxide chromium sesquioxide Caesium caesium borate caesium iodide caesium monoxide caesium hydroxide diatomic caesium caesium chromate caesium molybdate caesium oxide caesium dihydroxide caesium telluride caesium tellurite caesium zirconate Iron iron iodide iron oxide iron iodide iron sesquioxide iron tetraoxide elemental hydrogen boric acid hydrogen iodide Water hydrogen telluride boric acid elemental iodine molecular iodine Evap. cond. Chem. reactive yes yes yes no yes yes no yes yes no yes no yes no yes yes no no no yes no yes no no yes no yes no yes no no yes yes no no no no yes yes yes no no no no no no yes no no no yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes no yes yes yes yes Table 1 - Catalogue of the chemical species available in ECART (cont'd). Species In InI InTe In2O In2O3 In2Te MnI2 MnO Mn2O3 Mn3O4 MoO2 MoO3 NG Ni Ni(CO)4 NiI2 NiO O OH PA PM PS RbI RbOH Ru RuO2 RuO3 Sb SbTe Sb2 Sb2O3 Sb2Te3 Sb4 Sn SnH4 SnI2 SnO SnO2 SnTe Sr SrI2 SrO SrOH Sr(OH)2 Te TeO2 Te2 Zn ZnO ZrI4 ZrO2 Indium indium monoiodide indium telluride indium suboxide indium sesquioxide diindium telluride manganese diiodide manganese oxide manganese sesquioxide trimanganese tetraoxide molybdenum dioxide molybdenum trioxide noble gases nickel nickel carbonyl nickel iodide nickel monoxide elemental oxygen hydroxyl aggregate aggregate aggregate rubidium iodide rubidium hydroxide ruthenium ruthenium dioxide ruthenium trioxide antimony antimony monotelluride diatomic antimony antimony trioxide antimony tritelluride tetraatomic antimony tin tin tetrahydride tin iodide tin monoxide tin dioxide tin monotelluride strontium strontium iodide strontium oxide strontium hydroxide strontium dihydroxide tellurium tellurium dioxide diatomic tellurium zinc zinc oxide zirconium tetraiodide zirconium dioxide Evap. cond. Chem. reactive yes yes no no no no no no no no yes yes no yes no no yes no no no no no yes no yes no no yes no no no no no yes no yes yes no yes yes yes no no yes yes yes no yes no yes yes yes yes yes yes yes yes yes yes yes yes yes yes no yes yes yes yes yes yes no no no yes no yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes yes RUNNING OF THE COUPLED MODULES The coupling among the three modules is explicit. As the Thermal-Hydraulic Module and the Aerosol and Vapour Transport Module are advanced with different time steps, depending on their own convergence criteria, a proper logic of synchronism is adopted. The thermal-hydraulic problem is firstly solved over the time interval between two synchronous conditions (of the order of the lowest Courant limit in the nodalization), often adopting short time steps. The aerosol-vapour and chemical equilibria calculations follow, with implicit integration methods allowing time steps usually longer than the thermal-hydraulics ones: this technique gives the possibility to smooth out the data related to flow rates and pressures calculated by the Thermal-Hydraulic Module in the case of oscillations due to limited instabilities. In the coupling, the influence of high airborne aerosol concentrations on the gas physical properties (apparent density and viscosity) is taken into account. Decay heat can be accounted for the most powerful elements undergoing transport processes (Kr, Rb, Sr, Mo, Ru, Ag, Sn, Sb, Te, I, Xe, Cs and Ba) through time-dependent and specific power correlations (Figure 5) deduced for typical LWRs [Parozzi 1995a]. The Chemical Equilibria Module updates the gaseous phase composition whenever significant changes in temperatures, pressures or vapour species amounts are calculated by the other modules. Possible phase changes, however, are dynamically accounted for in the diffusive model employed by the Aerosol and Vapour Transport Module (Figure 6). 1E+9 400 days [W•days/kg] 1E+8 600 days 1200 days 1800 days 1E+7 1E+6 1E+5 0.0E+0 5.0E+5 1.0E+6 1.5E+6 2.0E+6 Time after shutdown [s] Figure 5: Example of the fitting function used to calculate the decay specific power associated to an element, as a function of accident time and fuel irradiation time. CsOH 1E+5 CsI 1E+4 Cs 1E+3 1E+2 Suspended mass [g] 1E+1 Cs2Te 1 CsO 0.1 Cs2 1E-2 1E-3 1E-4 1E-5 1E-6 Cs2O 1E-7 1E-8 1E-9 1E-10 11000 12000 13000 14000 15000 16000 17000 18000 19000 20000 21000 Time [s] Figure 6: Example of ECART prediction of suspended masses of Caesium compounds transported from the primary circuit into the containment, for a typical PWR small break. Computer Time Requirements The ECART code can be compiled with Microsoft FORTRAN Power Station (with no DEBUG option) and executed with a PC 486 or Pentium under DOS control. In these environments, the CPU time required for complete reactor coolant system transients turns out to be some tenths of hours, depending on the scenario, the nodalization and the number of models activated. The code has also successfully installed and used on other computers, such as IBM Power PC (RISC) workstation and IBM-9021/740 mainframe, with a performance of about 5 times as fast for the former and 13 times as fast for the latter. These computing times are not excessively long if compared with the times taken by other mechanistic severe accident codes, and it is likely they will be reduced introducing optimisation criteria and improvements in the numeric. REFERENCES [Ambrosini 1987] W. Ambrosini, G. Fruttuoso, M. Mazzini, F. Oriolo, “FASTRAP : a Very Fast-Running Code for the Analysis of Special Transients and SB-LOCAs in PWRs”, ANS Anticipated and Abnormal Transients Topical Meeting, Atlanta (USA), April 1987. [Ambrosini 1992] W. Ambrosini, P. Barbucci, G. Fruttuoso, A. Manfredini, G. Mariotti, F. Oriolo, “An Integrated Model for Evaluating the Thermal-Hydraulic Behaviour of Primary System and Containment in Innovative LWRs”, International Conference on Design and Safety of Advanced Nuclear Power Plants, October 1992, Tokyo (J). [Ambrosini 1995] W. Ambrosini, G. Fruttuoso, F. Oriolo, S. Paci, F. Parozzi, "Assessment and Validation of ECART Code in Support to SA Radionuclide Transport" IAEA TCM on "Advanced in and Experience with Accident Consequences Analysis", Vienna (A), September 1995. [Ambrosini 1996] W. Ambrosini, F. Oriolo, G. Fruttuoso, A. Manfredini, F. Parozzi, M. Valisi "Heat and Mass Transfer Phenomena in Innovative LWRs" Energia Nucleare, Vol. 1, 1996. [Biardi 1993] G. Biardi, E. Borioli, L. Pellegrini, "A chemical equilibrium solver under development at ENEL". 5th European Severe Accident Chemistry Group Meeting, AEA Winfrith (UK), September 1993. [Blawzdziewicz 1995] J. Blawzdziewicz, T.B. Diep, F. Feuillebois, “Physical Study of Aerosol Transport in the ECART Code”, Report CNRS Laboratoire de Physique et Mécanique des Milieux Hétérogènes - École Supérieure de Physique et de Chimie Industrielles de la Ville de Paris, for EDF, 1995. [Borioli 1992] E. Borioli, F. Parozzi, “Computer Models on Fission Product and Aerosol behaviour in the LWR Primary Coolant System”, EC DG XII Report 14676 EN, November 1992. [Bowsher 1995] B.R. Bowsher, "A strategy for source term work in the European Union", European Commission DG XII Report, EUR 16501 EN, 1995. [Eusebi 1992] M. Eusebi, F. Parozzi, M. Valisi, J. A. Capitao, G. De Santi, “Preparatory Calculations for a New Experimental Program on Dry Aerosol Resuspension Mechanisms (STORM Project)”, European Aerosol Conference, Oxford (UK), September 1992, Journal of Aerosol Science, Vol. 23 Suppl. 1, S1-S1026, Pergamon Press, 1992. [Hervouet 1995] Hervouet, C., W. Ranval, M. Eusebi, F. Parozzi (1995), “Fission Product Transport in RCS. Part I - Comparison between MAAP and ECART Predictions of Radionuclide Transport throughout a Typical PWR Reactor Coolant System”, ENEL-ATN Final Report for CEC RCA Source Term Project ST(95)-P234, June 1995. [Kourti 1995] N. Kourti, F. Parozzi, D. Utton, K. Taylor, D. Williams, A. Smethurst, A. Schatz, "Multicomponent aerosol effects", Report IKE - Universität Stuttgart, IKE 2 - 122, Final Report for CEC RCA Source Term ST(95) P-173, June 1995. [Manfredini 1992] A. Manfredini, M. Mazzini, F. Oriolo, S. Paci, “FUMO Code Manual Volume 1: System Models”, University of Pisa, Dipartimento di Costruzioni Meccaniche e Nucleari, RL 533 (92), 1992. [Masnaghetti 1987] A. Masnaghetti, F. Parozzi, “Influence of Recirculation Phenomena on the Aerosol Retention in Large Components of LWR Primary Circuits”, NEA/CEC Workshop on Water-cooled Reactor Aerosol Code Evaluation and Uncertainty Assessment, Brussels (B), September 1987. [Oriolo 1995] F. Oriolo, W. Ambrosini, G. Fruttuoso, F. Parozzi, R. Fontana, “Thermal-Hydraulic Modelling and Severe Accident Radionuclide Transport”, Nuclear Technology, vol. 112, n. 2, November 1995. [Paci 1996] S. Paci, "Analysis of the Phebus FPT-0 Test using the ECART Integrated Code", Report Themas, NT TH 129(96), February 1996. [Parozzi 1988a] F. Parozzi, G. Sandrelli, A. Masnaghetti, “Italian Contribution to TRAP-MELT Code Development”, IAEA International Symposium on Severe Accidents in Nuclear Power Plants, Sorrento (I), March 1988. [Parozzi 1988b] F. Parozzi, “Relevance of Marviken and LACE Project Results in Validating TRAPMELT2/ENEL Code”, MARVIKEN-V/DEMONA/LACE Workshop, Montreux (CH), June 1988. [Parozzi 1991] F. Parozzi, “The Vapour and Aerosol Transport Module in ECART Code”, European Aerosol Conference, Karlsruhe (D), September 1991, Journal of Aerosol Science, Vol. 22 Suppl. 1, S751, Pergamon Press, 1991. [Parozzi 1995a] F. Parozzi, G. Sandrelli, F. De Rosa, D. Diamanti, R. Fontana, "Fission Product Transport in RCS - Thermal-Hydraulic Input. Part III -Estimate of specific radioactive decay power associated to elements undergoing transport processes", ENEL-ATN Final Report for CEC RCA Source Term Project ST(95)-P233, June 1995. [Parozzi 1995b] F. Parozzi T. Albiol, A. Alonso, N. Kourti, P. Merker, D.A. Williams, “Fission Product Transport in the Reactor Coolant System”, FISA-95 Symposium EU Research on Severe Accidents, Luxembourg (L), November 1995. [Parozzi 1996] F. Parozzi, F. Oriolo, S. Paci, "Analysis of the OECD CSNI ISP-37 on VANAM M3 Test using the ECART integrated code", ENEL-ATN Report, January 1996, Comparison Workshop of International Standard Problem N. 37, Cologne (D), February 1996. [Salina 1996] E. Salina, R. Fontana, M. Eusebi, F. Parozzi, "Fission Product Transport in RCS Thermal-Hydraulic Input. Part IV - Preliminary verification tests of the Integrated ECART", ENEL-ATN Final Report for CEC RCA Source Term Project, February 1996. [Wright 1994] A.L. Wright., “Primary System Fission Product Release and Transport: a SOAR to the CSNI”, NRC, NUREG/CR-6193, NEA/CSNI/R(94)2, June, 1994.