1 Synoptic scale dust emissions over the Sahara desert initiated by a convective cold 2 pool in early August 2006 3 Diana Bou Karam1, Earle Williams2, Matthew Janiga3, Cyrille Flamant1, Michael McGraw- 4 Herdeg2, Juan Cuesta4, Antoine Auby1 and Chris Thorncroft 3 5 1 6 7 2 Parsons Laboratory, Massachusetts Institute of Technology, Cambridge, MA, USA. 3 8 LATMOS/IPSL, CNRS and Université Pierre et Marie Curie, Paris, France. Department of Earth and Atmospheric Sciences, University at Albany, NY, USA. 4 9 LISA/IPSL, CNRS and Université Paris 12, Créteil, France. 10 11 Abstract 12 This paper is concerned with a dust-raising cold pool over the Sahara desert that occurred on August 13 3-5, 2006. Both the quantity of the uplifted dust and its spatio-temporal evolution are examined using 14 satellite observations and a high-resolution numerical simulation. The dust emission during this event 15 was initiated by a mesoscale cold pool emanating from mesoscale convective systems (MCSs) that 16 developed over northern Niger and Mali on August 3. This event is one of several exceptional 17 northward extensions of the West African monsoon during the 2006 wet season. We examine the 18 propagation of the cold pool and associated dust lofting using high temporal resolution false color dust 19 product images from the Meteosat Second Generation Spinning Enhanced Visible and Infrared Imager 1 20 (MSG-SEVIRI). Observations from Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation 21 (CALIPSO) are used to characterize the vertical structure of the dust cloud as it spreads over the 22 Sahara and across the Atlantic coast. The European Centre for Medium-Range Weather Forecasting 23 African Monsoon Multidisciplinary Analysis (ECMWF-AMMA) special reanalysis was used to 24 describe the synoptic conditions that accompanied this event. Furthermore, a numerical simulation 25 using the mesoscale model MesoNH was performed to quantify the emissions and the westward 26 transport of dust during this event. 27 The dusty cold pool covered southern Algeria and a large part of northern Mali and Western Niger 28 attaining a total area close to 500,000 km2. It extended over 2-3 km in altitude and had an aerosol 29 optical depth on the order of 1.5 and a total dust load of about 2 Tg on average. Following daytime 30 heating, the dusty cold pool and associated northward surge of moisture favored the development of 31 additional precipitation and dust lofting. The dusty cold pool and monsoon surge were accompanied 32 by a collapse of the Saharan heat low. About 0.4 Tg of dust produced during this event was subjected 33 to westward transport over the Atlantic Ocean after being mixed upward by the diurnal heating over 34 the Sahara to altitudes as high as 5 km. 35 Comments: You mentioned that you preferred a methodology then results order to the abstract, that is 36 fine. I suggest reordering the sentences in the second paragraph so that if follows a chronological 37 order. 38 . 39 Key Words: West African Monsoon, Mesoscale convective systems, CALIPSO, SEVIRI, ECMWF, 40 mineral dust, MesoNH. 2 41 1. Introduction 42 Satellite observations consistently indicate the most widespread and persistent aerosol plumes found 43 on Earth are associated with dust [e.g. Prospero et al., 2002]. Dust emitted from arid and semiarid 44 regions and transported in the atmosphere has been recognized to be an important component of the 45 Earth’s climate system because of its influence on the Earth’s radiation budget [e.g., Haywood et al., 46 2003; Forster et al., 2007]. In many regions, they are the biggest contribution to atmospheric optical 47 thickness [Tegen et al., 1997],. This is particularly true over North and West Africa, the world’s 48 strongest summertime dust source. Here emission and transport have been shown to be highly variable 49 in time and space although they are typically controlled by turbulent processes within the Saharan 50 boundary layer small-scale high-wind events [e.g. Prospero et al., 2002; Engelstaedter and 51 Washington, 2007]. There is now evidence that dust emission over the Sahara and Sahel is associated 52 with different meteorological processes occurring on a variety of scales, from small scale features like 53 dust devils through mesoscale phenomena including mesoscale convective features to synoptic scale 54 forcing features (like midlatitude cold fronts). These forcing mechanisms for dust emission over 55 Sahara and Sahel have been identified in recent work particularly in the framework of the African 56 Monsoon Multidisciplinary Analyses program [Redelsperger et al., 2006]. 57 Comments: Above two paragraphs merged into one. I think its important to provide contrast between 58 what typically occurs over the Sahara and the big events like our case study which are the topic of the 59 next paragraph. 60 Over the Sahara, dust storms have been documented to be associated with high near-surface wind 61 speeds resulting from the downward mixing and dissipation of momentum from the nocturnal low- 62 level jets (LLJs) during the morning build-up of the planetary boundary layer. Such LLJs are most 63 active during the summer and are associated with the Saharan heat low (SHL). Dust outbreaks occur in 3 64 response to collapses of the SHL [e.g. Knippertz, 2008] or are connected to LLJs generated in the lee 65 of complex terrain as is the case in the Bodélé region of Northern Chad [e.g. Washington and Todd, 66 2005; Todd et al., 2008]. Dust emission over the Sahara has also been shown to be connected to the 67 low level dynamics associated with the penetration during spring of an upper-level trough to low 68 latitudes [e.g. Jankowiak and Tanré, 1992]. Lastly, emission can occur in response tomesoscale 69 density currents [e.g. Wakimoto, 1982; Simpson, 1997] caused by strong evaporational cooling of 70 precipitation along cloud-bands on the Saharan side of the Atlas Mountain chain in southern Morocco 71 [Knippertz et al., 2007]. 72 73 Over the Sahel, cold pools associated with the outflows of mesoscale convective systems (MCSs) have 74 long been known to produce large outbreaks of dust called ‘haboobs’ particularly at the beginning of 75 the monsoon season, before the growing vegetation begins to reduce local dust emission and are 76 frequently observed during the afternoon and nighttime [Sutton, 1925, 1931; Williams et al., 2009; 77 McGraw-Herdeg, 2010]. They represent an efficient mechanism for dust mobilization by virtue of 78 their strong near-surface winds. This can be followed by mixing associated with daytime heating 79 which lofts the dust to altitudes favourable for long-range transport in summertime [e.g. Sterk, 2002; 80 Flamant et al., 2007; Bou Karam et al., 2008; Marsham et al., 2008]. Furthermore, Bou Karam et al., 81 [2008] and [2009] have identified another mechanism for dust emission over the Sahel during summer, 82 in which highly turbulent winds at the leading edge of the monsoon nocturnal flow in the Inter 83 Tropical Discontinuity (ITD) region generate dust uplifting and transport to high altitude. 84 However, the relative importance of dust activity in Sahelian and Saharan sources for dust export from 85 Africa during summertime is currently debated. Also, our understanding of the factors controlling the 86 dust cycle and the interannual variability of the cross-Atlantic dust transport from sources in these two 4 87 regions, activated by meteorological processes discussed above, is still limited. Thus, accurate 88 simulation of dust generating mechanisms during summertime over Sahara and over Sahel is crucial 89 for quantifying the total dust load observed annually and estimating the relative contribution of 90 Sahelian and Saharan source region to the overall dust transport out of Africa. 91 Despite the importance of MCS outflows in terms of dust emissions [Tetzlaff and Peters, 1986], only a 92 few studies [e.g. Knippertz et al., 2009] have documented their behavior over the Sahara desert during 93 summertime, where the surface is unprotected by vegetation and deflatable materials are often 94 abundant. Hence, the dust activity linked to cold pools over the Sahara may have significant 95 contribution to the total dust production over North and West Africa in summertime. 96 Taking advantage of the recent availability of convection-permitting numerical models, we aim in this 97 study to quantify for the first time the dust uplifted over the Sahara by a MCS cold pool of synoptic 98 scale. The main objectives of this study are: 1) To examine, using satellite observations with high 99 spatio-temporal resolution, dust emission and transport over and out of the Sahara in connection with 100 the MCS outflows, 2) to evaluate the impact of such features on the atmospheric conditions over the 101 Sahara particularly in terms of supply of moisture and temperature perturbation, 3) to evaluate the 102 ability of a mesoscale atmospheric model (MesoNH) to represent the dust lifting by the cold pool over 103 the Sahara and 4) to estimate the emissions and the westward transport of dust during this event 104 The paper is organized as follows: Section 2 provides an overview of the data sources used in this 105 study. In section 3, the meteorological conditions that accompanied this event are addressed. The 106 spatio-temporal evolution of the dusty cold pool, including its impact on the atmospheric conditions 107 over the Sahara Desert is treated in section 4. Section 5 describes the main characteristics of the dusty 5 108 cold pool including the estimate of the dust load and transport. Finally, discussion and conclusions are 109 treated in section 6. 110 6 111 112 2. Data sources 2.1 Ground based measurements 113 Hourly surface measurements are used to describe the meteorological conditions accompanying the 114 advance of the dusty gust front to the north. Surface wind (10 m above ground level, agl), temperature 115 (2 m agl) and visibility were obtained from meteorological station instruments deployed at 116 Tamanrasset (Algeria; 22.80°N, 5.52°E) and In Salah (Algeria; 27.19°N, 2.47°E). The location of 117 these stations is shown in Figure 1. These data are from the Integrated Surface Hourly (ISH) database 118 (dataset 3505), provided by the National Climatic Data Center (NCDC). 119 2.2 Space-borne observations 120 The horizontal distribution of the dust associated with the cold pool is described using the Spinning 121 Enhanced Visible and Infra-Red Imager (SEVIRI) images of the Meteosat Second Generation (MSG) 122 computed from a combination of three infrared channels (8.7, 10.8, and 12 μm).. MSG-SEVIRI is in 123 geostationary orbit at 0°W over the equator and provides images of Africa with 15-minute and 0.03° 124 resolution. False-color images are created using an algorithm developed by the European organization 125 for the Exploitation of Meteorological Satellites (EUMETSAT) which colors red the difference in 126 brightness temperature (BTD) between the 12.0 and 10.8 μm channels, green the BTD between the 127 10.8 and 8.7 μm channels and blue the 10.8 μm channel [e.g. Schepanski et al., 2007]. On these 128 composite images, dust appears pink or magenta and clouds appear orange or brown. The effect of the 129 dust on the BTD depends on its altitude [e.g. Pierangelo et al., 2004] suggesting that these composite 130 images may favor the dust which is elevated so that its radiating temperature differs significantly from 131 the ground. 7 132 Additionally, aerosol optical depth (AOD) obtained from the Moderate Resolution Imaging 133 Spectroradiometer (MODIS) /AQUA Deep Blue Collection 5.1 over desert surfaces (MYD08_D3 134 product) with horizontal resolution of 1°x1° is used to characterize the optical depth of the dust in the 135 cold pool. In addition, the 3B42 TRMM Satellite product [Huffman et al., 2007] is used to document 136 the precipitating convection over the Sahara Desert where no other radars are available. 137 Finally, information about the vertical distribution of dust during the event under scrutiny is provided 138 from attenuated backscatter profiles at 532 nm retrieved from the space-borne Cloud-Aerosol LIdar 139 with Orthogonal Polarization (CALIOP) on board the CALIPSO (Cloud-Aerosol Lidar and Infrared 140 Pathfinder Satellite Observation; Winker et al., [2003]) satellite with vertical and horizontal resolution 141 of 60 m and 12 km, respectively. It is worth noting that MODIS and CALIPSO are part of the A-Train. 142 The A-train orbit crosses North Africa twice a day, once during the daytime (between 1230 and 1430 143 LST) and once during the nighttime (between 0030 and 0230 LST), and has a revisit time period of 16 144 days for the same orbit [Stephens et al., 2002]. 145 2.3 Model data 146 2.3.1 Reanalyses 147 The analyses used to provide the synoptic-scale context for this event came from the 0.5º European 148 Centre for Medium-Range Weather Forecast (ECMWF) African Monsoon Multidisciplinary Analysis 149 (AMMA) Reanalysis. This analysis was achieved by running the ECMWF data assimilation system 150 using the radiosonde data collected and archived during AMMA [Augusti-Panareda et al., 2009]. 151 However, over the Sahara, the ECMWF AMMA Ranalyses are mainly dominated by model physics 8 152 and assimilated satellite data due to the paucity of synoptic stations and radiosondes data in this region 153 [e.g. Knippertz et al., 2009]. 154 Finally, toward understanding the fate of the dust raised by this event, the calculation of the back 155 trajectories was performed using the FLEXPART model [Stohl et al., 2005] which is a Lagrangian 156 particle dispersion model driven by the ECMWF AMMA Reanalyses that simulates the synoptic scale 157 and mesoscale transport of tracers released from a defined point [e.g. De Villiers et al., 2010]. In the 158 following, the term ‘ECMWF analysis’ denominates the ECMWF AMMA Reanalysis data. 159 2.3.2 Numerical simulations 160 Simulations have been carried out using MesoNH [Lafore et al., 1998], a non-hydrostatic mesoscale 161 atmospheric model with an on-line dust emission and transport module. MesoNH includes 162 parameterizations of various processes including cloud microphysics [Cohard and Pinty, 2000], 163 turbulence [Bougeault and Lacarre, 1989], deep and shallow convection [Bechtold et al., 2001], 164 chemical aerosol [Tulet et al., 2005] and dust aerosol [Grini et al., 2006].MesoNH is coupled to an 165 externalised surface model which handles heat and water vapour fluxes between the low-level 166 atmosphere and four types of surface: vegetation, towns, oceans and lakes [Masson et al., 2003]. 167 Natural land surfaces are described by interactions treated in the Soil Biosphere and Atmosphere 168 model (ISBA) [Noilhan and Mahfouf, 1996]. 169 170 The dust emission scheme is the Dust Entrainment And Deposition (DEAD) model [Zender et al., 171 2003], implemented as a component of MesoNH [Grini et al., 2006], that calculates dust flux from 172 wind friction velocity. DEAD includes entrainment thresholds for saltation, moisture inhibition and 173 saltation feedback. The ORILAM model [Tulet et al., 2005] simulates transport and loss processes by 9 174 following the evolution of two moments of three lognormal modes defined by Alfaro and Gomes 175 [2001]. Dust advection and diffusion are treated using the transport processes of MesoNH including 176 mixing within the planetary boundary layer, shallow convective transport and advection by winds. 177 MesoNH uses the radiative scheme of the European Centre for Medium-range Weather Forecasts 178 (ECMWF), which computes shortwave and longwave radiative fluxes. Shortwave radiative fluxes are 179 computed for 6 wavelengths using the extinction coefficients, asymmetry factors and single scattering 180 albedo provided by look-up tables for spherical aerosol particles. 181 182 In this study a five-day simulation (3-7 August 2006) was performed. The study area covering Niger, 183 Eastern Mali and southern Algeria forms a domain of 3000 km x 2500 km (centred on 20°N / 7°E, see 184 Fig. 1) with a horizontal mesh size of 10 km. In the vertical, 72 levels were used with 35 of them 185 within the planetary boundary layer. The lowermost level is at 10 m above the ground, while the 186 highest level is at 28 km above the ground. Initial and lateral boundary conditions were taken from the 187 ECMWF analyses. The ability of MesoNH to simulate dust emission and transport over West Africa 188 has been highlighted in several recent studies [e.g., Grini et al., 2006; Chaboureau et al., 2007; Tulet 189 et al., 2008; Crumeyrolle et al., 2008; Bou Karam et al., 2009a; Bou Karam et al., 2010]. 190 191 3. The synoptic situation 192 Figure 2 shows Hovmoller plots (Latitude versus time) of Mean Sea Level Pressure (MSLP), 193 geopotential at 850 hPa, meridional winds and specific humidity at 925hPa derived from the ECMWF 194 AMMA reanalysis and averaged over 5 °W-5° E are used to address the synoptic situation between 2 195 and 8 August 2006 (Figure 2). These fields have been smoothed with a 2 day low-pass Lanczos filter 196 to remove the substantial variability associated with the diurnal cycle. The analysis of these Hovmoller 10 197 plots suggest three distinct periods based on the large-scale flow and thermodynamic environment: 198 pre-dust outbreak, rapid northward dust movement, and a more gradual northward dust movement 199 associated with reduced dust emission. 200 201 The first period, between 2 August at 0000 UTC and 4 August at 0000 UTC preceded the dust event. 202 This period was characterized by a deep surface low (~1004 hPa) between 19 and 22° N located over 203 southern Algeria and northeastern Mali (Fig. 2a). The intertropical front (ITF), the interface between 204 two opposing surface winds: the cool moist south-westerly monsoon flow and the warm dry 205 northeasterly Harmattan [e.g. Hastenrath, 1988; Bou Karam et al., 2008; Pospichal et al., 2009] was 206 found around 20°N (Fig. 2c and 2d) with a core of intense southerlies between 15 and 20 °N (Fig. 2c). 207 . The second period. between 4 August at 0000 UTC and 5 August 0000 UTC coincided with the 208 rapid northward movement of the dusty cold pool. The surface low of 1004 hPa moved westward and 209 northward to northern Mauritania and western Algeria (Fig. 2a). At low-levels (i.e. 925hPa), strong 210 southerlies were seen between 14 and 24°N (Fig. 2c) and the ITF moved northward to 22°N (Fig. 2d). 211 A dramatic northward surge of the monsoon air (up to 24°N) was observed during this period (Fig. 212 2d). At this latitude, the total column water vapor (TCWV) increased from approximately 15 to 25 g 213 kg-1. Decreases in the 925 hPa potential temperature of 2-3 K were observed during this period over a 214 large region centered at 20°N. 215 The period following 5 August at 0000 UTC was characterized by a more gradual northward 216 movement of the dust front. The low-level southerlies persisted between 14°-24°N until 6 August at 217 1200 UTC. The weakening southerly flow seen in the Hövmoller was associated with a continued 11 218 westward movement and reduction in the strength of the SHL and southerlies. Continued but gradual 219 increases in TCWV and reductions in 925 hPa temperature were observed over the Sahel. Following 220 the cessation of southery flow on 6 August the ITF retreated back to ____ N. 221 Comments: I have tried to better define this three period idea although I’m not sure which figure you 222 are going to use. I think its very important to have each period have its own paragraph and a “name” 223 I’ve termed them “pre-dust”, “rapid surge”, and “gradual surge followed by cessation”. Also, there 224 needs to be specific mention of how we are denoting the ITF. Lastly, the conservation naturally moves 225 in and out of the Hovmoller diagram as there is information that is not apparent on it. I think when 226 specific latitudes are mentioned we need to be very clear as to whether these are in the Hovmoller (ie 227 a longitudinal average) or if they are determined by a separate examination of maps. 228 12 229 230 4. Spatio-temporal evolution of the dusty cold pool 4.1 The initiation phase: 3-4 August 2006 231 On 3 August, an isolated cumulonimbus cloud developed southwest of the Aїr Mountains (i.e. 8°E, 232 17°N) and expanded to a MCS to the southwest of the Aїr Massif. At 1500 UTC, a second MCS began 233 to develop over northeastern Mali. These two MCSs continued to grow and at 2100 UTC they merged 234 and formed a squall line nearly 1000 km across (Fig. 3a). On 3 August at 1800 UTC, the first visible 235 cold pool in SEVIRI imagery emanated from the MCS over western Niger, a region recognized as an 236 active dust source during the monsoon season by virtue of its location in the vicinity of mountain 237 foothills where fluvial sediment from weathering provides fine material for deflation [e.g. Bou Karam 238 et al., 2008; Schepanski et al., 2009; Bou Karam et al., 2009b]. The strong surface winds associated 239 with the MCS density current and the turbulent winds at the leading edge of the monsoon flow (e.g. 240 Bou Karam et al., 2008) produced strong dust emission and the cold pool was visible on the SEVIRI 241 images as an arc of dust (purple colors, Figs. 3a). 242 The MCS density current continued to mobilize dust as it moved northward and by 4 August at 0600 243 UTC the cold pool formed an arc of dust, over 1000km across, encompassing northern Mali, southern 244 Algeria and western Niger (Fig. 3b). 245 13 246 4.2 The northward transport of dust: 4-5 August 2006 247 The large dust cold pool continued its northward expansion over Algeria. On 4 August at 0900 UTC, 248 the dust front arrived over Tamanrasset (Fig. 3c) and reached In Salah on 5 August at 0600 UTC (Fig. 249 3d). At Tamanrasset, the arrival of the dust front was associated with a dramatic reduction in visibility 250 (< 500 m for several hours, Fig. 4a) accompanied with a short-term increase in surface wind speed to 251 7.5 m s-1. A small decrease in surface temperature (3°C) was observed in Tamanrasset at the time of 252 the dust front arrival together with an increase of about 2 hPa in surface pressure and of about 4 g kg-1 253 in water vapor mixing ration (Fig. 4a). Moreover, this event seemed to perturb the diurnal cycle in 254 surface temperature at Tamanrasset where the temperature during the morning hours on 5 August (9- 255 12 UTC) was about 5°C less than the previous days. This could be due to the development of 256 precipitating clouds over the Hoggar Mountains as will be discussed in section 4.3, or also to the 257 shielding of shortwave radiation by the heavy dust cloud. At In Salah, the arrival of the dust front over 258 the station was evident in the change in wind direction, the drop in visibility (less than 2 km visibility 259 for most of 5 August) and a 1 hPa increase in surface pressure (Fig. 4b). However, no significant 260 decrease in surface temperature was discernible in the surface observations at In Salah (Fig. 4d). 261 Figure 5a shows a Hovmoller of SEVIRI observations (latitude versus time) at 2° E and Figure 5b 262 shows the full space-time evolution of the dust front observable in SEVIRI imagery. From these 263 figures, we can discern and characterise three phases during the northward advance of the dust front: i) 264 through the lifetime of the MCS (i.e. between 3 August at 2100 UTC and 4 August at 0900 UTC), the 265 dusty cold pool propagated with speeds up to 18 m s-1, (ii) between 0900 UTC on 4 August and 0300 266 UTC on 5 August the propagation speed of the dust front decreased to 9 m s-1 on average, and (iii) 14 267 between 0300 UTC and 1500 UTC on 5 August where a final northward surge of the dust front with a 268 propagation speed of 5 m s-1 was observed (Fig. 5a and 5b). 269 The rapid northward surge of the dusty cold pool into the Sahara desert during the first phase was due 270 to the strong density contrast caused primarily by the difference in temperature between the cold air of 271 the convective downdraft and the hot Saharan air [e.g. Wakimoto, 1982; Simpson, 1997; McGraw- 272 Herdeg, 2010]. 273 During the second phase, the active convection had stopped and the cold pool was no longer being 274 replenished. Also, in the daytime, the turbulent mixing in the boundary layer tends to mix the cold 275 layer with the environmental air thereby decreasing the density contrast across the density current- 276 Saharan air interface and hence slowing the propagation of the dust front (Fig. 5b). During this phase, 277 synoptic conditions played the major role in the advance of the dust cloud over the Sahara where the 278 northern progression of the dust cloud was driven by a strong latitudinal pressure gradient and the 279 associated pronounced southerly winds (i.e. Fig 2a and 2c). This analysis is supported by the absence 280 of a distinct temperature drop (that usually characterizes the passage of density currents [e.g. Simpson, 281 1997]) at In Salah when the dust cloud passed over. 282 Finally, the last northward surge of the dust front was dominated by the emanation of outflows from 283 new convection that developed over the original dust cloud over central Algeria (i.e. over In Salah Fig. 284 5a and 6b) A diminishing role was likely played by the large-scale southerlies associated with the 285 weakening and westward moving SHL duing this phase.. Similar behavior of the dust front was 286 highlighted in the model results as well. A Hovmoller at 2° E of the vertically integrated dust 287 concentration simulated by MesoNH (Fig. 5c) shows a dust front loaded by at least 1.2 g m-2 and 288 advancing northward from 18°N on 3 August to 26 °N on 6 August 2006. 15 289 16 290 4.3 The impact of the cold pool on the atmospheric conditions over the Sahara 291 The intrusion of the cold pool into the Sahara desert impacted its environment mainly by the supply of 292 moisture which helped on the development of new convection, resulting in weak precipitation. 293 The transport of moisture into the Sahara was evident in the water vapor mixing ration (WVMR) fields 294 simulated by MesoNH (Fig. 5c right panel). The area covered by the dust front seen in pink in Fig. 5a 295 and in red in Fig. 5c (left panel) was associated with WVMR of about 12 g kg-1 at 925hPa and 296 reaching 20 g kg-1 in some hours (Fig. 2d and Fig. 5c right panel) which is more than three times the 297 WVMR over the desert (3 to 6 g kg -1, Fig. 5c right panel). A sharp gradient in WVMR was seen 298 across the dust front-Saharan air interface with 10 g kg-1 difference over less than 1° in latitude (Fig. 299 5c right panel). Moreover, in Tamanrasset an increase in WVMR from 8 to 12 g kg-1 was observed on 300 4 August after midnight with the arrival of the dust front. The WVMR remained high (13 g kg-1) till 301 the morning of the 6th of August (Fig. 4a). Also, with the advance of the cold pool into the Sahara, 302 WVMR at In Salah increased by 6 g kg-1 on the morning of the 5th of August and remained high (15 g 303 kg-1) till the evening of 6 August (Fig. 4b). 304 Under these unusual conditions over the Sahara desert, new convective clouds developed at several 305 locations over the Sahara (Fig. 6a and 6b). We also emphasize the faithful representation by MesoNH 306 of the dust features seen in the SEVIRI observations as well as the occurrence of new convection over 307 the Sahara (Fig. 6c and 6d). On 4 August at 1800 UTC (Fig. 6a and 6c), new convection developed 308 over southern Algeria in response to the supply of moisture and favored by the orographic lifting 309 associated with the Hoggar Mountains [e.g. Cuesta et al., 2010]. Based on the SEVIRI images, the 310 dominant type of cloud associated with the convection over the Hoggar was thick mid-level clouds 311 (Fig. 6a). From the model results, these clouds were around 6 km in altitude (Fig. 6c) and they resulted 17 312 in localized precipitation over southern Algeria of about 2.5 mm per hour as reported in the TRMM 313 observations (Fig. 6e). On 5 August at 1800 UTC, convection developed over central Algeria around 6 314 km in altitude (Fig. 6b and 6d). This convection resulted on shallower precipitation than the one over 315 the Hoggar and precipitation rates derived from TRMM did not exceed 2 mm per hour over central 316 Algeria (Fig. 5f). 317 I think mention needs to be made that the convection did not develop until ~12 h after the passage of 318 the dusty gust front. As Dave Schultz mentioned in his review one would not expect convection to 319 develop over the cold pool as they are very stable. The soundings showed that the initial arrival of the 320 cold pool (0600 UTC) resulted in a shallow layer of cool moist air (~50 hPa) and an inversion over 321 Tamanrasset. However, throughout the day this inversion was mixed out providing a more favorable 322 environment for the secondary episode of convection. 323 Furthermore, the dusty cold pool appears to have had a significant impact on the Saharan Heat Low 324 (SHL). An increase of 5 hPa in the mean sea level pressure was seen after the arrival of the dusty cold 325 pool over the desert and a collapsing of the SHL from August 5 to 6 was observed after the dust front 326 reached the central Sahara (i.e. Fig 2a and 2b). This could be the result of the advection of cold air 327 within the southerlies into the SHL or a result of the dust and clouds radiative forcing by reflecting the 328 incoming shortwave radiation and thus decreasing the heating at the surface. Also, the new deep 329 convection that developed over the desert could have impacted the energy budget and played a role in 330 the SHL collapsing. 331 18 332 333 5. The characteristics of the dusty cold pool 5.1 Dust loads in the cold pool 334 On 5 August at 1200 UTC, the large arc-shaped plume of dust generated by the MCS cold pool lay 335 over southern Algeria, northern Mali and northwestern Niger (Fig. 7a). The MODIS Deep Blue 336 observations of AOD on 5 August at 1200 UTC showed the same horizontal extent of the dust cloud to 337 be associated with AODs between 0.5 and 1.5 (Fig. 7b). The largest AODs were observed over central 338 Algeria (Fig. 7b). Figure 7c shows the dust AOD at 550 nm simulated by MesoNH on 5 august at 1200 339 UTC. The model reproduced quite well the horizontal extent of the dust cloud as well as the AODs 340 associated with and observed in the MODIS Deep Blue data (Fig. 7c). In order to estimate the dust 341 load generated by the cold pool, we averaged the simulated dust mass over the area covered by the 342 dust cold pool and having a dust load of 0.5 g m-2 and more. An evolution between 3 and 7 August of 343 the dust load over the area affected by the cold pool is shown in Figure 7d. The total dust load was 344 simulated to range between 1.8 Tg and 2.8 Tg on 3 and 5 August with an average of 1.7 Tg for the rest 345 of the period (Fig. 7d). 346 Bou Karam et al., [2009b] have estimated the average dust load in the ITD region over a domain 347 encompassing 11°W-17°E, 11°-28°N to be on the order of 2.5 Tg and those associated with the 348 monsoon leading edge (only to the south of the ITD) to range between 0.5 and 0.8 Tg. This indicates 349 that the dust load produced during this event is significant compared to the dust emitted in the ITD 350 region. 351 19 352 5.2 Vertical distribution of dust in the cold pool 353 The vertical distribution of dust in the cold pool was analyzed using the CALIPSO observations during 354 two nighttime orbits of the spaceborne lidar on 4 and 5 August. Seven hours after the initiation of dust 355 emissions over western Niger by the MCS density current, CALIPSO passed over the arc of dust on 4 356 August at 0100 UTC (Fig. 8a). A sharp dust front was seen in the CALIPSO observations shown in 357 Fig. 8b (see the red marker). A dense dusty layer associated with lidar reflectivity at 532 nm in excess 358 of 7 x10-3 km-1 Sr-1 was observed between the ground and 2 km in altitude. The height of the dusty 359 layer decreased with latitude forming a sharp front at 21°N. Note that the shape of the dust front 360 observed here by CALIPSO is similar to the one shown by Williams et al., [2009] derived from a 361 vertically-pointing W-band radar data and by Flamant et al., [2007] and Bou Karam et al., [2008] 362 using an airborne lidar. The dust front was associated with potential temperature on the order of 312 K 363 with colder atmosphere behind (i.e. 308 K at 18°N) and was advancing into the desert characterized by 364 320 K in potential temperature over 5 km in altitude (Fig. 8b). 365 The following day, CALIPSO crossed over the part of the dust cloud located over northern Mali (Fig. 366 9a). On 5 August, the dust extended to higher altitude reaching 3 km (Fig. 9b). It was associated with 367 lidar reflectivity at 532 nm of about 4 x10-3 km-1 sr-1 and potential temperature on the order of 312 K. 368 Mid-level clouds between 6 and 9 km in altitude were seen over central Mali to the south of the dust 369 layer (Fig. 9a and 9b). 370 20 371 5.3 The westward transport of the dust out of the continent 372 The role of this large scale dust-lofting event on the export of dust out of Africa has also been 373 examined in this study based on back-trajectory analyses (using the FLEXPART model) and 374 CALIPSO observations on 6 and 7 August 2006 near the West African coast, to the west of the area of 375 dust emission produced by the cold pool on 4 August 2006. Also, an attempt to estimate the dust mass 376 transported westward resulting from this event has been made based on the model results. 377 Although the development of new convection over the Hoggar may have scavenged a large amount of 378 the airborne dust, a westward transport over the Atlantic Ocean of the remaining dust was evident in 379 the CALIPSO observations shown in figures 10a and 10c. On 6 August 2006 at 0237 UTC, CALIPSO 380 observations showed a layer of dust over 18-27°N between 3 and 5 km in altitude (Fig. 10a). The 381 backtrajectory analysis starting on 6 August from the location and the height of this layer showed that 382 the dust originated two days before over the region bounded by 2°W-2°E and 19-22°N (Fig. 10b). This 383 corresponds to the dust produced by the cold pool over Algeria on 4 August as now discussed. 384 The transport of dust to the west was not favorable before the evening on 4 August. This is due to the 385 fact that the dust front was confined between the surface and 2 km in altitude as was evidenced by the 386 CALIPSO observations shown in Fig. 8b. The wind at these altitudes (i.e. below 2 km) is generally 387 northerly or southerly and so unfavorable for westward advection. In the daytime, the dust was 388 subject to vertical transport throughout the depth of the Saharan boundary layer and the height of the 389 dust layers was set by the daytime thickness of the Saharan boundary layer. Over Tamanrasset, the 390 height of the Saharan boundary layer was observed from soundings to reach roughly 4 km at 1200 391 UTC and 5 km at 1800 UTC (See Fig. 7a in Cuesta et al, 2008). At these altitudes (i.e. 3-5 km), 392 consistent easterly flow is present in the vicinity of the African Easterly Jet (AEJ) and westward 21 393 transport by these winds was responsible for carrying the dust from above the area of the cold pool to 394 the location observed by CALIPSO near the coast. 395 http://weather.uwyo.edu/cgi- 396 bin/sounding?region=africa&TYPE=GIF%3ASKEWT&YEAR=2006&MONTH=08&FROM=0400& 397 TO=0600&STNM=60680 398 399 On 7 August 2006, CALIPSO observations show a much more elevated dust layer (4-6 km) over 15- 400 25°N to be associated with much higher values of backscatter coefficient (> 3 x10-3 km-1 sr-1) than in 401 the previous day (Fig. 10c). The back-trajectory analysis initiated on 7 August at the location and the 22 402 height of this layer of dust showed that the dust was carried westward on 4 August 2006 from above 403 the area 0-5° E and 20-25° N (i.e. the location of the dust cloud caused by the cold pool) at 5-6 km in 404 altitude (i.e. Fig. 10d). This is also consistent with the fact that for a typical 8 m s-1 wind speed at 700 405 hPa, the transport of dust from its origin over the continent to the ocean (i.e. over ~2000 km) requires 406 ~ 3 days, which corresponds to the time interval from the initial raising of dust on 4 August to the time 407 of the observed dusty layer on CALIPSO near the Atlantic coast on 7 August. 408 In order to estimate the westward transport of dust resulting from this event, a vertical cross section at 409 longitude 4°W of dust concentration simulated by MesoNH was made on 6 August at 1200 UTC i.e. 410 after the emission processus has ended. The longitude 4°W was chosen because it is far enough from 411 the original area of dust lofting and represents a reasonable location for the dust to exit the continent 412 (i.e. Fig 11a). The model-simulated dust concentrations range between 300 and 400 µg.m-3 over 2.5 to 413 4.5 km in altitude near 22 °N (Fig. 11b). Along the same vertical cross section, the AEJ stands out 414 clearly between 2.5 and 6 km in altitude with a core of high wind (15 m s-1 )between 3 and 6 km in 415 altitude and 12-22°N (Fig. 11c). From Figures 11c and 11b, we can estimate the mass flux of dust 416 transported westward by the AEJ. To do so, we derive the mass flux of dust from the product of the 417 mean wind speed (15 m s-1) and the mean dust concentration (350 µg m-3) over the atmospheric 418 column 2-5 km and latitude range 20° N–22° N. Therefore, the result represents the net westward 419 export of dust mass from this area toward the Atlantic. The westward dust flux leaving the region at 4 420 W is 0.2 Tg per day. If we consider that the dust transport, due only to this event, occurred over 2 days 421 (from 5 to 6 August); then the contribution of this event to the total dust export from the Sahara toward 422 the Atlantic is about 0.4 Tg. 23 423 Todd et al., [2008], using the same approach, have estimated the dust emissions downstream of the 424 Bodélé Depression to be between 0.9 and 2.9 Tg per day. This indicates that the dust transported 425 westward during a single event of the like is significant comparing to the dust emitted daily from the 426 Bodélé Depression for example. 427 24 428 6. Discussion and conclusions 429 The evolution and the characteristics of an intense dust event that occurred over the Sahara desert on 430 August 3-5, 2006 have been documented using a combination of satellite observations and mesoscale 431 numerical modelling.The mesoscale model MesoNH was able to reproduce quite well the spatio- 432 temporal distribution of dust and clouds associated with this event. The dusty cold pool originated 433 from a large MCS that occurred over West Africa on 3 August 2006 propagated northward greater 434 than 1000 km over 3 days with an initial speed of 18 m s-1. The cold pool that expanded initially as a 435 density current raised a large quantity of dust (~ 2 Tg) and advected abundant moisture (with water 436 vapor mixing ratio 12 g kg -1) into the Saharan desert. The arc-shaped plume of dust extended over 437 2000 km in length and was associated with AOD values on the order of 1.5. Mass flux of dust in the 438 order of 0.2 Tg per day was transported out of the Sahara toward the Atlantic Ocean by the AEJ after 439 being mixed within the Saharan boundary layer up to altitudes of 3-5 km. The general synoptic scale 440 wind conditions and position of the AEJ in the period of the observations are rather common 441 conditions over West Africa. As a consequence, any dust raised to the level of the AEJ by deep dry 442 boundary layer convection will be advected westward over the Atlantic. 443 On August 4-5 moisture advection associated with the cold pool together with topographic lifting 444 associated with the Hoggar Mountains were responsible for the development of new convection over 445 the Sahara. The new convection resulted in weak precipitation over the Sahara (rainfall rate of 3 mm 446 hr-1 or less). This could be due to the fact that in arid regions most of the precipitation evaporates 447 before reaching the ground [e.g. Srivastava, 1985; Knippertz et al., 2009]. This study has 448 demonstrated for the continent of Africa that cold pool dynamics can link a single thunderstorm to 449 vigorous dust storms thousands of kilometers away. A similar expansion of a cold pool in which new 25 450 convection feeds cold air into the cold pool as it propagates, have been documented in North America 451 [e.g., Carbone et al., 2002; Tuttle et al., 2004]. 452 The present study also suggests that the occurrence of MCSs at high latitudes (i.e. > 18°N) during the 453 monsoon season has an important contribution in terms of dust emissions and transport towards the 454 Americas. Furthermore, such events may contribute importantly to the high dust activity observed 455 annually over West and North Africa in summertime. In 2006 for example, at least four events of the 456 like occurred over the Sahara, some of which have been explored in other studies [Cuesta et al., 2010; 457 Knippertz and Todd, 2010]. All these events are characterized by extraordinary latitudinal extensions 458 of the West African monsoon known as the monsoon surges. The latitudinal extents of these dust pools 459 (900 km for Cuesta et al. [2010]; 2000 km in this study and in Knippertz and Todd [2010]) exceed by 460 a substantial margin the mean value of 450 km for 30 MCS-related gust front events in the same 461 season that occurred over the Sahel [McGraw-Herdeg, 2010]. Climatologically speaking, the monsoon 462 flow is bounded by the Inter-Tropical Front (ITF) to the north, and the southerly flow stops well short 463 of the Saharan heat low. But in these exceptional events, the expanding dust pool pushes the ITD 464 northward strongly deforming it (Figure 2c and 2d), and brings sufficient moisture into the dry Sahara 465 Desert for weak precipitation to form there (Figure 6), both in this study and in Cuesta et al. [2010] for 466 another monsoon surge event in July 2006. 467 A second exceptional aspect of these monsoon surge events, in their exceptional latitudinal reach, they 468 often cause the collapse of the heat low to the north [Cuesta et al., 2010, and this study]. Though the 469 physical mechanism of this collapse has not been fully resolved in this study, observations here and 470 elsewhere provide additional constraints on suggested mechanisms. Lavaysse et al. [2010] discuss the 471 role of temperature decrease in contributing to heat low collapse, but it is important to note that 26 472 temperature drops in surface air at northernmost desert stations were difficult to discern (against 10- 473 15C diurnal variations) in both the present study and in Cuesta et al. [2010]. In this study, when the 474 dusty air pushed northward into the desert, a temperature drop is discernible at Tamanrasset (Figure 475 4a), but not further north at In Salah (Figure 4b). Likewise, Cuesta et al. [2010] identify no 476 temperature drop in dust arrival at Tamanrasset in their surge event, but only when rainfall events 477 occur. The absence of temperature drops points to the exhaustion of the density current and casts doubt 478 on the use of “cold pool” to characterize the event at this advanced stage of its evolution. The 479 continued northward progression of the dusty air, clearly evident in Figure 5, is pressure-gradient 480 driven (consistent with the findings in Knippertz and Todd [2010] for this event), and this conclusion 481 is supported in the present study by the model simulations. 482 Cuesta et al. [2010] present evidence that shading by cloud (and consequent temperature reduction) is 483 causing the heat low collapse in their event. The evidence presented here for the existence of 484 cloudiness in the SEVERI imagery (orange color in Figure 7) is consistent with that idea. However, 485 the area of lofted dust is substantially greater than water cloud at the higher latitude, and the abrupt 486 drops in surface visibility (Figures 4a, 4b) at all stations involved provide strong evidence that surface 487 shading by dust will occur and thereby suppress surface heating and sensible heat flux at high latitudes 488 where the heat low is found initially (Figure 2a). Future observations within the collapsing heat low 489 would shed important new light on this issue. Also, the radiative impact of the dust uplifted during 490 such events and its feedback on the atmospheric circulation and particularly on the Saharan Heat Low 491 dynamics are envisaged for future work via numerical simulations, necessary to sort out the radiative 492 effects of water cloud and dust. Finally, the evaluation of the frequency of the occurrence of these 493 events during a complete monsoon season and over many years is recommended for future studies. 27 494 Acknowledgement 495 "Based on a French initiative, AMMA was built by an international scientific group and is currently 496 funded by a large number of agencies, especially from France, UK, US and Africa. It has been the 497 beneficiary of a major financial contribution from the European Community's Sixth Framework 498 Research Programme. Detailed information on scientific coordination and funding is available on the 499 AMMA International web site http://www.amma-international.org". 500 MODIS observations used in this study were produced with the Giovanni online data system, 501 developed and maintained by the NASA Goddard Earth Sciences (GES) Data and Information 502 Services Center (DISC). The authors wish to thank the SATMOS, ICARE and Climserv for providing 503 SEVIRI and CALIPSO data. Some of the data used in this study were acquired as part of the Tropical 504 Rainfall Measuring Mission (TRMM). The data were processed by the TRMM Science Data and 505 Information System (TSDIS) and the TRMM Office; they are archived and distributed by the Goddard 506 Distributed Active Archive Center. D. Bou Karam’s work on this study was supported by the ‘Centre 507 National des Etudes Spatiales’ (CNES), and the authors wish to thank particularly Didier Renaut and 508 Carole Deniel. Earle Williams, Chris Thorncroft, Matthew Janiga and Michael McGraw-Herdeg 509 received partial support for this study from grant ATM0734806 from Atmospheric Dynamics (Jay 510 Fein) of the US National Science Foundation. 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