PM2.5 Co-benefits of Climate Change Legislation Part 1: California’s AB 32 Christina Zapata1, Nicholas Muller2, and Michael J. Kleeman1* 1 Department of Civil and Environmental Engineering, University of California, Davis. 1 Shields Avenue, Davis CA 95616. 2Department of Economics, Environmental Studies Program, Middlebury College, Middlebury VT 05770. *Corresponding author. Tel.: +1 530 752 8386; fax; +1 530 752 7872. E-mail address: mjkleeman@ucdavis.edu (M.J. Kleeman). Reference Acronyms: CARB – California Air Resources Board CEC – California Energy Commission FRA – Federal Railroad Administration CDWR – California Department of Water Resources SWRCB - State Water Resources Control Board S.1. Emission Changes from Individual AB 32 Measures Table S1 summarizes the business as usual (BAU) emissions and Table S2 summarizes changes to emissions for source categories impacted by AB 32 control measures. The “Levels” defined in the current study were designed to inform the reader about which economic sectors provided the greatest benefits from AB 32 emissions changes. The individual measures assigned to each “Level” are taken directly from AB 32. Supplemental information sources were used to determine thresholds for source inclusion in various AB 32 measures when these thresholds were not directly provided by AB 32. In cases where supplemental information was not available or the resulting thresholds seemed impractical, we provided our own expert opinion. Table S1 only summarizes information for the emission sources that are influenced by AB 32 measures. Table 2 in the main text provides insight about the magnitude of the emissions change for the entire sector. The Public Health and Environmental Benefits Analysis for AB 32 (CARB 2008) estimated changes in NOx and PM2.5 emissions for a variety of mobile and stationary sources. In the present study, the same fraction of emission reduction (or increase) was applied to TOG, NMOG, CO, SOx, and/or NH3 if those emissions were non-zero in the BAU inventory. Emissions from sources in the petroleum industry were scaled based on controls applied to methane or hydrocarbon emissions. Level 1: Industrial Measures BAU emissions from industrial sources include emissions from on-site electricity generation at a major facility that is used directly at that same facility. The energy efficiency measures applied under Level 1 were assumed to reduce demand for electrical power in this sector. Roughly 70 major industrial facilities including refineries, cement plants, high emitting oil and gas extraction plants, hydrogen plants, and mineral plants were affected by the energy efficiency measures in Level 1 controls. See discussion in the main text for further details. Level 2: Commercial and Institutional Electricity Generation Measures The effect of AB 32 measures related to commercial electricity consumption/generation were summed and the net change in electrical generation was then applied using the following priority: reductions in electrical generation were applied first to out-of-state fossil fuel electricity generation, and then to instate fossil fuel electricity generation as described in the main text. For the Renewable Electricity Standard, “electricity generation from other” includes the increase in emissions associated fossil-fueled boilers and heaters attached to solar thermal electrical generation units. Many solar thermal power plants have boilers and heaters that assist in the startup phase of the plant and that provide protection against freezing of the working fluids. The Green Buildings measure was applied to new and existing state, residential, and commercial buildings (including schools). It was assumed that the adoption of energy efficient building standards and the use of more energy efficient appliances would decrease emissions associated with electricity and natural gas consumption in buildings. Estimates for reduced energy consumption associated with water use were obtained from multiple sources. A 20% improvement in “end use” water efficiency was assumed to reduce electricity demand for end use water supplies and wastewater treatment by a proportional amount (CEC Nov 2005, CEC 2009a, Pacific Institute Sep 2005). Utilization of urban runoff, water recycling, and improvements to water system energy efficiency were assumed to reduce electrical consumption for water treatment by a further 10% (CEC Nov 2005, CEC 2009a, CDWR Jun 2003, SWRCB Mar 2008 NRDC Aug 2009). The projected net effect of all water-related measures in 2030 is a 5% reduction in total electricity consumption in California. Level 3: Agriculture Measures AB 32 stipulates an increase in electricity generation from renewable sources. Central California and southern California have large dairy farms that produce methane gas through the decomposition of dairy waste. The installation of combustion systems to produce electricity from this methane source satisfies the definition of renewable energy production. Large dairies were not explicitly defined by AB 32, but EPA provides a definition for a large dairy as ≥500 dairy cows per facility (Ed. K.F. Roos 2004). Over 1000 dairy farms in California have ≥500 dairy cows, accounting for over 90% (1.67 million) of all CA dairy cows in 2007 (USDA 2009). Implementing biogas digesters on each of these facilities would require an investment of ~$2B, which seemed prohibitively expensive. The current study assumes that the largest dairy facilities emitting ≥5100 kg/hr of TOG would install biogas digesters (<20 dairies in total meet this criterion) as a more practical threshold for implementation. Level 4 and Level 5: On-road and Other Mobile Transportation Measures The Low Carbon Fuel Standard specifies emission reductions for advanced passenger vehicles and increases in emissions for transport of biofuel feedstock via rail and heavy duty trucks. All on-road vehicles using biofuels were assumed to have reduced tailpipe emissions factors. The measures associated with Port Drayage Trucks regulation were applied within an 80 mile radius from the 6 ports mentioned in the main text based on survey results describing the average distance traveled by trucks servicing the ports. High Speed Rail emissions were based on the HST Investment-grade scenario analysis (FRA Aug 2005). Investment-grade ridership forecasts were used to approximate the potential VMT reductions from 26.6 million annual trips from highway travel and 15.4 million trips for air travel. Regional transportation related greenhouse gas targets were assumed to apply to gasoline vehicles. Brake wear and road dust was included in the BAU emissions totals for on-road gasoline vehicles and these emissions were not scaled by AB 32 measures. The goods movement statewide efficiency improvements were assumed to apply to diesel vehicles, the same source assumed in the CARB Sep 2008 reference. Clean/Green ship measures were assumed to apply equally to all ships including commercial and ocean-going vessels during all modes of operation (maneuvering, berthing, and intransit). Industrial off-road equipment excludes construction and farming equipment. S.2. Impact of AB 32 on PM2.5 Component Concentrations Figures S1 through S4 illustrate the effect of AB 32 defined Implementation Levels on PM2.5 component concentrations including organic carbon (OC), elemental carbon (EC), sulfate (S(VI)), and nitrate (N(V)). Implementation Level 2 produces the largest reduction in OC and EC concentrations but these large changes are highly localized around the industrial emissions point source. The most widespread reductions of OC and EC during the simulated winter stagnation event are produced by electric utility and on-road mobile Implementation Levels 2 and 4, respectively, with OC concentrations reduced by ~0.3 µg m-3 over large portions of the state. Dairy biogas combustion for electricity generation increases PM2.5 organic and elemental carbon concentrations by ~0.06 µg m-3 in the SJV. PM2.5 sulfate concentrations are expected to decrease by ~1.49 µg m-3 in the port regions due to ship controls under Implementation Level 5 and increase in the SJV by ~0.1 µg m-3 due to the combustion of dairy biogas under Implementation Level 3. This agrees with the sulfur content of the fuel that will be combusted less or more for those sources as specified by the measures. All AB 32 defined Implementation Levels produce reductions in regional nitrate concentrations ranging from 0.17-0.3 µg m-3 with the exception of Implementation Level 3 that increases nitrate concentrations in the SJV by 0.5 µg m-3. It is evident that due to the diverse range of emission sources and rates for specific California regions as well as the implementation of multiple GHG measures, each California region differs from one another in PM2.5 mass and composition concentration benefit or disbenefit. Table S.1. Business as Usual emissions for sources impacted by AB 32 measures in tonnes per day. Simulated Sources Level Industrial Electricity Generation Oil and Gas Production Equipment 1 Natural Gas Transmission Petroleum Refining Flares Petroleum Fugitive HC Pipeline Valves Commercial and Governmental Waste Disposal Electricity Generation from Coal Electricity Generation from Distillate Oil Electricity Generation from Coke Electricity Generation from LPG Electricity Generation from Jet Fuel 2 Electricity Generation from Diesel Electricity Generation from Natural Gas Electricity Generation from Geothermal Electricity Generation from Landfill Gas Electricity Generation from Other Residential and Commercial Natural Gas 3 4 5 Dairy Manure Waste On-Road Gasoline Vehicles On-Road Diesel Vehicles Transportation Refrigeration Units Industrial Off-road Equipment 6 Commercial Harbor Craft Ocean Going Vessels Commercial Aircraft Freight Trains TOG NMOG CO NOx SOx NH3 TSP PM10 PM2.5 5.12E+01 2.60E+00 2.40E+02 9.27E+00 2.37E+00 6.66E+01 2.43E-02 3.70E-01 4.04E-01 5.82E-02 5.80E-04 4.10E-04 2.61E+01 1.37E+01 9.83E+00 7.64E-03 9.12E+00 1.04E+03 2.06E+02 1.51E+01 6.10E+00 8.04E+00 5.51E+00 3.04E+01 1.09E+01 1.46E+01 1.21E+01 1.32E+00 1.51E+01 7.08E+00 1.69E+00 1.15E+00 3.93E-03 3.42E-01 6.80E-02 5.38E-02 5.24E-04 3.79E-04 7.31E+00 1.92E+00 2.25E+00 5.92E-03 3.86E+00 3.13E+02 1.95E+02 1.39E+01 5.64E+00 5.74E+00 5.10E+00 2.62E+01 9.78E+00 1.35E+01 9.68E+01 1.30E+00 0.00E+00 1.34E+00 0.00E+00 4.86E-01 4.00E-01 1.16E+00 3.82E-01 1.81E-01 2.02E-02 1.15E-03 8.82E+01 6.82E-03 5.88E+00 1.23E-02 3.14E+01 0.00E+00 1.55E+03 2.24E+02 6.90E+01 2.87E+02 2.13E+01 8.64E+01 6.40E+01 5.26E+01 5.02E+01 2.64E+00 0.00E+00 1.28E+00 0.00E+00 5.00E-01 1.20E+00 4.19E+00 7.55E-01 6.21E-01 2.30E-02 4.64E-03 4.08E+01 4.13E-01 1.82E+00 2.33E-01 4.87E+01 0.00E+00 1.31E+02 1.61E+02 3.37E+01 2.29E+01 4.02E+01 7.33E+02 4.57E+01 1.40E+02 3.71E+00 2.44E+00 0.00E+00 1.43E+01 0.00E+00 9.38E-02 1.21E+00 1.39E-01 8.05E-01 1.99E-01 2.10E-03 1.76E-03 9.82E-01 1.20E-01 2.32E-01 7.25E-03 5.09E-01 0.00E+00 4.69E+00 9.97E-01 8.25E-02 8.93E-02 3.05E-01 3.54E+02 1.26E+00 1.60E-01 3.35E+00 7.90E-03 0.00E+00 0.00E+00 9.30E-04 0.00E+00 0.00E+00 8.08E-03 0.00E+00 3.70E-04 0.00E+00 0.00E+00 3.32E+00 0.00E+00 1.74E-02 0.00E+00 0.00E+00 3.28E+02 3.49E+01 2.69E-01 0.00E+00 0.00E+00 0.00E+00 0.00E+00 0.00E+00 0.00E+00 1.19E+01 1.00E+00 0.00E+00 1.27E-01 0.00E+00 4.73E-01 8.10E-02 3.08E-01 1.88E-02 7.60E-02 8.30E-04 3.50E-04 1.05E+01 6.17E-01 2.92E-01 9.95E-03 6.27E+00 1.96E+01 4.71E+01 7.74E+00 1.79E-01 6.74E-01 1.51E+00 5.44E+01 7.11E-01 4.28E+00 1.18E+01 1.02E+00 0.00E+00 1.27E-01 0.00E+00 3.68E-01 3.24E-02 3.00E-01 7.50E-03 7.42E-02 8.10E-04 3.36E-04 1.06E+01 4.31E-01 2.89E-01 9.71E-03 6.32E+00 1.37E+01 3.12E+01 7.62E+00 1.73E-01 6.36E-01 1.50E+00 5.11E+01 6.93E-01 4.22E+00 1.16E+01 1.02E+00 0.00E+00 1.27E-01 0.00E+00 2.73E-01 1.21E-02 2.97E-01 2.81E-03 7.35E-02 8.03E-04 3.28E-04 1.06E+01 2.59E-01 2.89E-01 9.62E-03 6.32E+00 8.23E+00 2.66E+01 7.31E+00 1.66E-01 6.27E-01 1.43E+00 4.98E+01 6.87E-01 4.02E+00 Table S2: Emission changes associated with AB 32 measures (tonnes/day). Please refer to the References section of the main article for full reference information. Simulated AB 32 Scoping Plan Measure Level 1 2 Sources Energy Efficiency and Co- Benefits Audits for Large Industrial Sources Industrial Electricity Generation Oil and Gas Extraction GHG Emission Reduction Oil and Gas Extraction Equipment Natural Gas Transmission and Distribution GHG Emission Reduction Natural Gas Transmission Refinery Flare Recovery System Improvement Petroleum Refining Flares Removal of Methane Exemption from Existing Refinery Regulations Petroleum Fugitive HC Pipeline Valves Landfill Methane Control Measure Commercial and Governmental Waste Disposal Green Buildings Electricity Generation from Coal Increasing Combined Heat and Power Use by 30,000 GWh Million Solar Roofs: 3,000MW by 2017 Electricity Generation from Distillate Oil Water Use Efficiency Electricity Generation from LPG Water Recycling Electricity Generation from Jet Fuel Water System Energy Efficiency Electricity Generation from Diesel Reuse Urban Runoff Electricity Generation from Natural Gas Electricity Generation from Coke Electricity Generation from Geothermal Renewable Electricity Standard Electricity Generation from Landfill Gas Electricity Generation from Other 3 4 5 6 Energy Efficiency (Natural Gas) Residential and Commercial Natural Gas Water Use Efficiency Residential and Commercial Natural Gas Green Buildings Residential and Commercial Natural Gas Solar Water Heating: AB1470 Residential Natural Gas Methane Capture at Large Dairies Dairy Manure Waste Dairy Biomethane Digester Combustion Pavley (AB 1493) On-Road Gasoline Vehicles Pavley II On-Road Gasoline Vehicles Low Carbon Fuel Standard On-Road Gasoline Vehicles Regional Transportation- Related Greenhouse Gas Targets On-Road Gasoline Vehicles Tire Tread Program, Tire Pressure Program On-Road Gasoline Vehicles High Speed Rail On-Road Gasoline Vehicles Medium- and Heavy-Duty Vehicle Hybridization On-Road Gasoline Vehicles Port Drayage Trucks On-Road Diesel Vehicles Heavy-Duty Vehicle GHG Emission Reduction (Aerodynamic Efficiency) On-Road Diesel Vehicles Medium- and Heavy-Duty Vehicle Hybridization On-Road Diesel Vehicles Goods Movement System- Wide Efficiency Improvements On-Road Diesel Vehicles Low Carbon Fuel Standard On-Road Diesel Vehicles Transport Refrigeration Units Cold Storage Prohibition and Energy Efficiency Transportation Refrigeration Units Cargo Handling Equipment- Anti-Idling, Hybrid, Electrification Industrial Off-road Equipment Commercial Harbor Craft- Maintenance and Design Efficiency Commercial Harbor Craft Clean Ships All Ocean Going Vessels Clean Ships Commercial Vessels Vessel Speed Reduction In-Transit Ocean Going Vessels Ship Electrification at Ports Berthing Ocean Going Vessels High Speed Rail Commercial Aircraft Low Carbon Fuel Standard Freight Trains TOG NMOG CO NOx SOx NH3 TSP PM10 PM2.5 -5.28E+00 -4.47E-01 -2.00E+00 -4.64E+00 -1.44E-01 -2.63E+01 -2.43E-02 -3.70E-01 -4.04E-01 -5.77E-02 -5.80E-04 -4.10E-04 -1.94E+01 0.00E+00 5.69E+00 4.86E-02 -5.55E-01 -4.71E-01 -1.27E+00 -1.85E-02 -1.00E+01 2.29E+01 -3.41E+00 -4.90E+00 -4.38E+00 -5.97E+00 -8.53E-01 -3.04E+00 -6.34E+00 0.00E+00 -1.34E-01 -4.13E-01 -1.43E+00 2.27E-01 -3.42E+00 -4.20E-01 -1.93E+00 -1.62E+00 -2.73E-03 -7.49E-01 -1.42E+00 -8.67E-01 2.11E-01 -1.24E+00 -1.55E-01 -1.00E-01 -3.54E+00 -1.01E-01 -3.68E-01 -3.93E-03 -3.42E-01 -6.80E-02 -5.34E-02 -5.24E-04 -3.79E-04 -5.25E+00 0.00E+00 1.31E+00 3.76E-02 -4.19E-01 -1.50E-01 -4.06E-01 -1.40E-02 -1.00E+00 1.72E-04 -3.27E+00 -4.70E+00 -4.20E+00 -5.72E+00 -8.17E-01 -2.75E+00 -5.74E+00 0.00E+00 -1.26E-01 -3.88E-01 -1.34E+00 2.29E-01 -3.16E+00 -2.81E-01 -1.78E+00 -1.30E+00 -2.42E-03 -5.92E-01 -1.21E+00 -7.82E-01 3.09E-01 -3.18E+00 0.00E+00 0.00E+00 -6.68E-01 0.00E+00 0.00E+00 -4.00E-01 -1.16E+00 -3.82E-01 -1.77E-01 -2.02E-02 -1.15E-03 -5.72E+01 2.52E-03 5.52E+00 1.60E-03 -4.56E+00 -1.67E+00 -4.28E+00 -1.86E-01 0.00E+00 8.70E+01 -2.59E+01 -3.62E+01 -2.33E+01 -3.63E+01 -2.37E+01 -2.25E+01 -4.94E+01 0.00E+00 -2.13E+00 -6.57E+00 -2.27E+01 3.99E-01 -3.86E+01 -1.66E+01 -1.02E+01 -4.18E+00 -1.02E-02 -1.80E+00 -4.03E+00 -1.73E+01 0.00E+00 -5.09E+00 -1.16E+00 0.00E+00 -6.38E-01 0.00E+00 0.00E+00 -1.20E+00 -4.19E+00 -7.55E-01 -6.18E-01 -2.30E-02 -4.64E-03 -2.87E+01 2.40E-02 1.14E+00 9.00E-03 -9.47E+00 -2.67E+00 -6.11E+00 -2.73E-01 0.00E+00 2.29E+01 -1.94E-01 -1.36E+00 -7.44E+00 -3.39E+00 -1.94E-01 -4.54E+00 -3.68E+00 -3.46E+01 -1.57E+00 -4.30E+00 -1.74E+01 1.32E+00 -1.89E+01 -2.54E+00 -1.93E+01 -7.49E+01 -5.63E-02 -1.88E+01 -5.10E+01 -5.95E+00 2.07E+00 -3.53E-01 -2.33E-02 0.00E+00 -7.15E+00 0.00E+00 0.00E+00 -1.21E+00 -1.39E-01 -8.05E-01 -1.93E-01 -2.10E-03 -1.76E-03 -6.68E-01 0.00E+00 1.12E-01 2.90E-04 -9.37E-02 -2.60E-02 -7.35E-02 0.00E+00 0.00E+00 8.35E-02 -7.71E-02 -1.08E-01 -1.34E+00 -1.07E-01 -7.05E-02 -1.15E-01 -1.46E-01 -8.33E-02 -2.96E-03 -9.12E-03 -3.16E-02 7.57E-03 -4.62E-02 -5.32E-03 -1.46E-01 -2.32E+01 -2.70E-03 -1.10E+01 -2.60E+01 -1.64E-01 8.84E-03 6.66E-03 0.00E+00 0.00E+00 0.00E+00 0.00E+00 0.00E+00 0.00E+00 -8.08E-03 0.00E+00 0.00E+00 0.00E+00 0.00E+00 -2.26E+00 0.00E+00 9.07E-03 0.00E+00 0.00E+00 0.00E+00 0.00E+00 0.00E+00 -1.52E+02 0.00E+00 -5.62E-01 -7.86E-01 0.00E+00 -7.84E-01 -5.14E-01 -8.38E-01 -1.07E+00 0.00E+00 -2.00E-03 -6.18E-03 -2.14E-02 0.00E+00 0.00E+00 0.00E+00 0.00E+00 0.00E+00 0.00E+00 0.00E+00 0.00E+00 0.00E+00 0.00E+00 -2.52E-01 -7.06E-02 0.00E+00 -6.38E-02 0.00E+00 -1.81E-01 -8.10E-02 -3.08E-01 -1.88E-02 -7.56E-02 -8.30E-04 -3.50E-04 -7.06E+00 1.60E-01 1.74E-01 3.15E-03 -7.53E-01 -3.33E-01 -8.76E-01 -2.82E-02 0.00E+00 2.75E+00 -6.90E-01 -7.67E-01 -1.51E+00 -6.58E-01 -8.77E-01 -5.37E-01 -7.71E-01 -2.41E+00 -7.01E-02 -2.41E-01 -7.23E-01 -8.15E-01 -1.00E-01 -1.90E-02 -9.08E-01 -7.99E-01 -7.06E-04 -1.55E+00 -3.64E+00 -3.56E-02 4.21E-02 -2.50E-01 -7.26E-02 0.00E+00 -6.38E-02 0.00E+00 -1.27E-01 -3.24E-02 -3.00E-01 -7.50E-03 -7.38E-02 -8.10E-04 -3.36E-04 -7.15E+00 1.12E-01 1.74E-01 3.09E-03 -7.55E-01 -3.36E-01 -8.82E-01 -2.83E-02 0.00E+00 2.73E+00 -6.24E-01 -6.93E-01 -1.37E+00 -5.94E-01 -7.92E-01 -4.85E-01 -6.28E-01 -2.37E+00 -6.81E-02 -2.37E-01 -7.12E-01 -8.03E-01 -9.69E-02 -1.90E-02 -9.02E-01 -7.63E-01 -7.06E-04 -1.47E+00 -3.50E+00 -3.45E-02 4.11E-02 -2.46E-01 -7.26E-02 0.00E+00 -6.38E-02 0.00E+00 -7.61E-02 -1.21E-02 -2.97E-01 -2.81E-03 -7.31E-02 -8.03E-04 -3.28E-04 -7.15E+00 6.71E-02 1.73E-01 3.08E-03 -7.55E-01 -3.36E-01 -8.82E-01 -2.83E-02 0.00E+00 2.73E+00 -6.64E-01 -7.37E-01 -1.10E+00 -6.32E-01 -8.43E-01 -5.16E-01 -6.94E-01 -2.30E+00 -6.35E-02 -2.30E-01 -6.90E-01 -7.40E-01 -9.32E-02 -1.90E-02 -8.60E-01 -7.57E-01 -7.05E-04 -1.46E+00 -3.41E+00 -3.43E-02 4.12E-02 References CARB Dec 2009, Worrel et al. 2008, Worrel et al. 2005, Coito 2005, XENERGY Inc. 2001 CARB Sep 2008 CARB Sep 2008 CARB Dec 2008 CARB Sep 2008 R.W. Beck Inc. and Group Jun 2006, EPA 2011a, EPA 2011b CEC Dec 2009b, CEC Dec 2005 CARB Dec 2008 CARB Dec 2008 CEC Nov 2005, CEC 2009a, Pacific Institute Sep 2005 CEC Nov 2005, CEC 2009a, CDWR Jun 2003 CEC Nov 2005, CEC 2009a, SWRCB Mar 2008 CEC Nov 2005, CEC 2009a, NRDC Aug 2009 CARB Apr 2010 CARB Apr 2010 CARB Apr 2010 CARB Sep 2008 CEC Nov 2005, CEC 2009a, Pacific Institute Sep 2005 Flex Your Power 2007 CARB Sep 2008 Shaw et al. 2007 See S.I. and text. CARB Apr 2007 CARB Sep 2008 CARB Mar 2009 CARB Sep 2008 CARB Sep 2008 FRA Aug 2005 CARB Mar 2009 CARB Sep 2008 CARB Sep 2008 CARB Sep 2008 CARB Sep 2008 CARB Mar 2009 CARB Sep 2008 CARB Sep 2008 CARB Sep 2008 CARB Sep 2008 CARB Sep 2008 CARB Sep 2008 CARB Sep 2008 FRA Aug 2005 CARB Mar 2009 a) PM2.5 Mass Change b) PM2.5 EC Change c) PM2.5 OC Change d) PM2.5 Sulfate Change e) PM2.5 Nitrate Change f) PM2.5 Ammonium Change a) Cumulative PM2.5 OC Change b) Level 1 Industry PM2.5 OC Change c) Level 2 Elec. & NG PM2.5 OC Change d) Level 3 Agriculture PM2.5 OC Change e) Level 4 On-road Mobile PM2.5 OC Change f) Level 5 Other Mobile PM2.5 OC Change Fig. S1. January 2050 episode average PM2.5 Organic Carbon (OC) concentration changes (µg m-3) for all defined AB 32 Implementation Levels. Panel (a) illustrates cumulative effects of all Levels while (panels b-f) illustrate individual changes associated with each Level relative to the previous level. Red indicates increased concentrations while blue indicates decreased concentrations. a) Cumulative PM2.5 EC Change b) Level 1 Industry PM2.5 EC Change c) Level 2 Elec. & NG PM2.5 EC Change d) Level 3 Agriculture PM2.5 EC Change e) Level 4 On-road Mobile PM2.5 EC Change f) Level 5 Other Mobile PM2.5 EC Change Fig. S2. January 2050 episode average PM2.5 Elemental Carbon (EC) concentration changes (µg m-3) for all defined AB 32 Implementation Levels. Panel (a) illustrates cumulative effects of all Levels while Panels (b-f) illustrate individual changes associated with each Level relative to the previous level. Red indicates increased concentrations while blue indicates decreased concentrations. a) Cumulative PM2.5 S(VI) Change b) Level 1 Industry PM2.5 S(VI) Change c) Level 2 Elec. & NG PM2.5 S(VI) Change d) Level 3 Agriculture PM2.5 S(VI) Change e) Level 4 On-road Mobile PM2.5 S(VI) Change f) Level 5 Other Mobile PM2.5 S(VI) Change Fig. S3. January 2050 episode average PM2.5 Sulfate (S(VI)) concentration changes (µg m-3) for all defined AB 32 Implementation Levels. Panel (a) illustrates cumulative effects of all Levels while (panels b-f) illustrate individual changes associated with each Level relative to the previous level. Red indicates increased concentrations while blue indicates decreased concentrations. a) Cumulative PM2.5 N(V) Change b) Level 1 Industry PM2.5 N(V) Change c) Level 2 Elec. & NG PM2.5 N(V) Change d) Level 3 Agriculture PM2.5 N(V) Change e) Level 4 On-road Mobile PM2.5 N(V) Change f) Level 5 Other Mobile PM2.5 N(V) Change Fig. S4. January 2050 episode average PM2.5 Nitrate (N(V)) concentration changes (µg m-3) for all defined AB 32 Implementation Levels. Panel (a) illustrates cumulative effects of all Levels while (panels b-f) illustrate individual changes associated with each Level relative to the previous level. Red indicates increased concentrations while blue indicates decreased concentrations.