List of Publications – Kurt V. Gothelf
Papers – peer reviewed
August 2011
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DNA- programmed Glaser-Eglinton reactions for the synthesis of conjugated
molecular wires
Ravnsbæk, J. B.; Jacobsen, M. F.; Rosen, C. B.; Voigt, N. V.; Gothelf, K. V. Angew. Chem.
Int. Ed., 2011, in press.
Chiral induction by seeding surface assemblies of chiral switches
Masini, F.; Kalashnyk, N.; Knudsen, M. M.; Cramer, J. R.; Lægsgaard, E.; Besenbacher, F.;
Gothelf, K. V.; Linderoth, T. R. J. Am. Chem. Soc., 2011, 7, 13910–13913.
Control of self-assembled 2D nanostructures by methylation of guanine
Bald, I.; Wang, Y.-g.; Dong, M.; Rosen, C. B.; Ravnsbæk, J. B.; Zhuang, G.- l.; Gothelf, K.
V.; Wang, J.-g.; Besenbacher, F., Small, 2011, 7, 939–949.
Single molecule microscopy methods for the study of DNA origami structures
Birkedal, V.; Dong, M.; Golas, M. M.; Sander, B.; Andersen, E. S.; Gothelf, K. V.;
Besenbacher, F.; Kjems, J. Microscopy Research and Technique 2011, 74, 688–698.
"Off–On" electrochemical hairpin-DNA-based genosensor for cancer diagnostics
Farjami, E.; Clima, L.; Gothelf, K. V.; Ferapontova, E. E. Anal. Chem. 2011, 83, 1594–
1602.
Recent advances in electrochemical aptamer-based sensors
Ferapontova, E. E.; Gothelf, K. V. Curr. Org. Chem. 2011, 15, 498–505.
β-olefination of 2-alkynoates leading to trisubstituted 1,3-dienes
Jacobsen, M. J.; Funder, E. D.; Cramer, J. R.; Gothelf, K. V. Org. Lett. 2011, 13, 3418–
3421.
Site-specific chemical labeling of long RNA molecules
Jahn, K.; Olsen, E. M.; Nielsen, M. M.; Tørring, T.; MohammadZadegan, R.; Andersen, E.
S.; Gothelf, K. V.; Kjems, J. Bioconjugate Chem. 2011, 22, 95–100.
Functional patterning of DNA origami by parallel enzymatic modification
Jahn, K.; Tørring, T.; Voigt, N. V.; Sørensen, R. S.; Kodal, A. L. B.; Andersen, E. S.;
Gothelf, K. V.; Kjems, J. Bioconjugate Chem. 2011, 22, 819–823.
Controlling chiral organization of molecular rods on Au(111) by molecular design
Knudsen, M. K.; Kalashnyk, N.; Masini, F.; Cramer, J. R.; Lægsgaard, E.; Besenbacher, F.;
Linderoth, T. R.; Gothelf., K. V. J. Am. Chem. Soc. 2011, 133, 4896–4905.
Combining aryltriazenes and electrogenerated acids to create well-defined aryltethered films and patterns on surfaces
Kongsfelt, M.; Vinther, J.; Malmos, K.; Ceccato, M.; Torbensen, K.; Knudsen, C. S.;
Gothelf, K. V.; Pedersen, S. U.; Daasbjerg, K. J. Am. Chem. Soc. 2011, 133, 3788–3791.
Design and construction of double-decker tile as a route to three-dimensional
periodic assembly of DNA
Majumder, U.; Rangnekar, A.; Gothelf, K. V.; Reif, J. H.; LaBean, T. H. J. Am. Chem. Soc.
2011, 133, 3843–3845.
Development of a lipase-based optical assay for detection of DNA
Pinijsuwan, S.; Shipovskov, S.; Surareungchai, W.; Ferapontova, E. E.; Gothelf, K. V. Org.
Biomol. Chem. 2011, 9, 6352–6356
Design and synthesis of DNA four-helix bundles
Rangnekar, A.; Gothelf, K. V.; LaBean, T. H. Nanotechnology 2011, 22, 235601.
DNA origami: a quantum leap for self-assembly of complex structures
Tørring, T.; Voigt, N. V.; Nangreave, J.; Yan, H.; Gothelf, K. V. Chem. Soc. Rev. 2011,
Advance Article DOI: 10.1039/C1CS15057J.
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A DNA tile actuator with eleven discrete states
Zhang, Z.; Olsen, E. M.; Kryger, M.; Voigt, N. V.; Tørring, T.; Gültekin, E.; Nielsen, M.;
MohammadZadegan, R.; Andersen, E. S.; Nielsen, M. M.; Kjems, J.; Birkedal, V.; Gothelf,
K. V. Angew. Chem. Int. Ed. 2011, 50, 3983–3987.
A nucleic acid dependent chemical photocatalysis in live human cells
Arian, D.; Cló, E.; Gothelf, K. V.; Mokhir, A. Chem,. Eur. J. 2010, 16, 288–295.
Steering organizational and conformational surface chirality by controlling
molecular chemical functionality
Bombis, C.; Weigelt, S.; Knudsen, M. M.; Nørgaard, M.; Busse, C.; Lægsgaard, E.;
Besenbacher, F.; Gothelf, K. V.; Linderoth, T. R., ACS Nano 2010, 4, 297–311.
DNA interactions with a methylene blue redox indicator depend on the DNA length
and are sequence specific
Farjami, E.; Clima, L.; Gothelf, K. V.; Ferapontova, E. E. Analyst 2010, 135, 1443–1448.
Electrochemical DNA sandwich assay with a lipase label for attomole detection of
DNA
Ferapontova, E. E.; Hansen, M. N.; Saunders, A. M.; Shipovskov, S.; Sutherland, D. S.;
Gothelf, K. V. Chem. Commun. 2010, 46, 1836–1838.
Synthesis and application of a triazene–ferrocene modifier for immobilization and
characterization of oligonucleotides at electrodes
Hansen, M. N.; Farjami, E.; Kristiansen, M.; Clima, L.; Pedersen, S. U.; Daasbjerg, K.;
Ferapontova, E. E.; Gothelf, K. V. J. Org. Chem. 2010, 75, 2474–2481.
Weave tile architecture construction strategy for DNA nanotechnology
Hansen, M. N.; Zhang, A. M.; Rangnekar, A.; Bompiani, K. M.; Carter, J. D.; Gothelf, K. V.;
LaBean, T. H. J. Am. Chem. Soc. 2010, 132, 14481–14486.
Single molecule atomic force microscopy studies of photosensitized singlet
oxygen behavior on a DNA origami template
Helmig, S.; Rotaru, A.; Arian, D.; Kovbasyuk, L.; Arnbjerg, J.; Ogilby, P. R.; Kjems, J.;
Mokhir, A.; Besenbacher, F.; Gothelf, K. V. ACS Nano 2010, 4, 7475–7480.
Small molecule induced control in duplex and triplex DNA-directed chemical
reactions
Jacobsen, M. F.; Ravnsbæk, J. B.; Gothelf, K. V. Org. Biomol. Chem. 2010, 8, 50–52.
DNA-templated covalent coupling of G4 PAMAM dendrimers
Liu, H.; Tørring, T.; Dong, M.; Rosen, C. B.; Besenbacher, F.; Gothelf, K. V. J. Am. Chem.
Soc. 2010, 132, 18054–18056.
Selective dsDNA-templated formation of copper nanoparticles in solution
Rotaru, A.; Dutta, S.; Jentzsch, E.; Gothelf, K. V.; Mokhir, A. Angew. Chem. Int. Ed. 2010,
49, 5665–5667.
DNA nanotechnology: Steps towards automated synthesis
Rotaru, A.; Gothelf, K. V. Nat. Nanotech. 2010, 5, 760–761.
A novel secondary DNA binding site in human topoisomerase I unravelled by
using a 2D DNA origami platform
Subramani, R.; Juul, S.; Rotaru, A.; Andersen, F. F.; Gothelf, K. V.; Mamdouh, W.;
Besenbacher, F.; Dong, M.; Knudsen, B. R. ACS Nano 2010, 4, 5969–5977.
Reversible pH-regulated control of photosensitized singlet oxygen production
using a DNA i-motif
Tørring, T.; Toftegaard, R.; Arnbjerg, J.; Ogilby, P. R.; Gothelf, K. V. Angew. Chem. Int.
Ed. 2010, 49, 7923–7925.
Single-molecule chemical reactions on DNA origami
Voigt, N. V.; Tørring, T.; Rotaru, A.; Jacobsen, M. F.; Ravnsbæk, J. B.; Subramani, R.;
Mamdouh, W.; Kjems, J.; Mokhir, A.; Besenbacher, F.; Gothelf, K. V. Nat. Nanotech. 2010,
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Supramolecular porous network formed by molecular recognition between
chemically modified nucleobases guanine and cytosine
Xu, W.; Wang, J.-g.; Jacobsen, M. F.; Mura, M.; Yu, M.; Kelly, R. E. A.; Meng, Q.-q.;
Lægsgaard, E.; Stensgaard, I.; Linderoth, T. R.; Kjems, J.; Kantorovich, L. N.; Gothelf, K.
V.; Besenbacher, F. Angew. Chem. Int. Ed. 2010, 49, 9373–9377.
Synthesis of functional molecular rod oligomers
Andersen, C. S.; Gothelf, K. V. Org. Biomol. Chem. 2009, 7, 58–60.
Distance dependent interhelical couplings of organic rods incorporated in DNA 4helix bundles
Andersen, C. S.; Knudsen, M. M.; Chhabra, R.; Liu, Y.; Yan, H.; Gothelf, K. V. Bioconjugate
Chem. 2009, 20, 1538–1546.
Self-assembly of a nanoscale DNA box with a controllable lid
Andersen, E. S.; Dong, M.; Nielsen, M. M.; Jahn, K.; Subramani, R.; Mam- douh, W.;
Golas, M. M.; Sander, B.; Stark, H.; Oliveira, C. L. P.; Pedersen, J. S.; Birkedal, V.;
Besenbacher, F.; Gothelf, K. V.; Kjems, J. Nature 2009, 459, 73–76.
Optimization of the electrochemical RNA-aptamer based biosensor for
theophylline by using a Methylene Blue redox label
Ferapontova, E. E.; Gothelf, K. V. Electroanalysis 2009, 21, 1261–1266.
Effect of serum on an RNA aptamer-based electrochemical sensor for theophylline
Ferapontova, E. E. ; Gothelf, K. V. Langmuir 2009, 25, 4279–4283.
A yoctoliter-scale DNA reactor for small-molecule evolution
Hansen, M. H.; Blakskjær, P.; Petersen, L. K.; Hansen, T. H.; Højfeldt, J. W.; Gothelf, K.
V.; Hansen, N. J. V. J. Am. Chem. Soc. 2009, 131, 1322–1327.
Synthesis and electrochemical studies of an anthraquinone-conjugated nucleoside
and derived oligonucleotides
Jacobsen, M. F.; Ferapontova, E. E.; Gothelf, K. V. Org. Biomol. Chem. 2009, 7, 905–908.
Effect of polymer cross-links on oxygen diffusion in glassy PMMA films
Klinger, M.; Tolbod, L. P.; Gothelf, K. V.; Ogilby, P. R. ACS Appl. Mater. Interfaces 2009, 1,
661–667.
Self-assembly of artificial nucleobase 1H-benzimidazole-4,7-dione at the
liquid/solid interface
Mamdouh, W.; Kelly, R. E. A.; Dong, M.; Jacobsen, M. F.; Ferapontova, E. E.; Kantorovich,
L. N.; Gothelf, K. V.; Besenbacher, F. J. Phys. Chem. B 2009, 113, 8675–8681.
Bridging one helical turn in double-stranded DNA by templated dimerization of
molecular rods
Andersen, C. S.; Yan, H.; Gothelf, K. V. Angew. Chem. Int. Ed. 2008, 47, 5569–5572.
DNA origami design of dolphin-shaped structures with flexible tails
Andersen, E. S.; Dong, M.; Nielsen, M. M.; Jahn, K.; Lind-Thomsen, A.; Mamdouh, W.;
Gothelf, K. V.; Besenbacher, F.; Kjems, J. ACS Nano 2008, 2, 1213–1218.
Labeling of DNA via rearrangement of s-2-aminoethyl phosphorothioates to n-(2mercaptoethyl)phosphoramidates
Chen, M.; Gothelf, K. V. Org. Biomol. Chem. 2008, 6, 908–911.
An RNA aptamer-based electrochemical biosensor for detection of theophylline in
serum
Ferapontova, E. E.; Olsen, E. M.; Gothelf, K. V. J. Am. Chem. Soc. 2008, 130, 4256–4258.
Toward reliable gold nanoparticle patterning on self-assembled DNA nanoscaffold
Sharma, J.; Chhabra, R.; Andersen, C. S.; Gothelf, K. V.; Yan, H.; Liu, Y. J. Am. Chem.
Soc. 2008, 130, 7820–7821.
Molecular self-assembly from building blocks synthesized on a surface in
ultrahigh vacuum: Kinetic control and topo-chemical reactions
Weigelt, S.; Bombis, C.; Busse, C.; Knudsen, M. M.; Gothelf, K. V.; Lægsgaard, E.;
Besenbacher, F.; Linderoth, T. R. ACS Nano 2008, 2, 651–660.
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Surface synthesis of 2D branched polymer nanostructures
Weigelt, S.; Busse, C.; Bombis, C.; Knudsen, M. M.; Gothelf, K. V.; Lægsgaard, E.;
Besenbacher, F.; Linderoth, T. R. Angew. Chem. Int. Ed. 2008, 47, 4406–4410.
Chiral ordering and conformational dynamics for a class of oligo-phenyleneethynylenes on Au(111)
Busse, C.; Weigelt, S.; Petersen, L.; Lægsgaard, E.; Besenbacher, F.; Linderoth, T. R.;
Thomsen, A. H.; Nielsen, M.; Gothelf, K. V. J. Phys. Chem. B. 2007, 111, 5850–5860.
Rearrangement of s-(2-aminoethyl) thiophosphates to n-(2mercaptoethyl)phosphoramidates
Chen, M.; Maetzke, A.; Knak Jensen, S. J.; Gothelf, K. V. Eur. J. Org. Chem. 2007, 5826–
5833.
Control and selectivity of photosensitized singlet oxygen production: Challenges
in complex biological systems
Cló, E.; Snyder, J. W.; Ogilby, P. R.; Gothelf, K. V. ChemBioChem 2007, 8, 475–481.
An electrochemical sensor based on the human estrogen receptor ligand binding
domain
Hansen, J. A.; Sumbayev, V. V.; Gothelf, K. V. Nano Lett. 2007, 7, 2831–2834.
Synthesis of rigid homo- and heteroditopic nucleobase-terminated molecules
incorporating adenine and/or thymine
Jacobsen, M. F.; Andersen, C. S.; Knudsen, M. M.; Gothelf, K. V. Org. Lett. 2007, 9, 2851–
2854.
Model systems for activation of nucleic acid encoded prodrugs
Jacobsen, M. F.; Cló, E., Mokhir, A.; Gothelf, K. V. ChemMedChem 2007, 2, 793–799.
Covalent interlinking of an aldehyde and an amine on a Au(111) surface in
ultrahigh vacuum
Weigelt, S.; Busse, C.; Bombis, C.; Knudsen, M. M.; Gothelf, K. V.; Strunskus, T.; Wöll, C.;
Dahlbom, M.; Hammer, B.; Lægsgaard, E.; Besenbacher, F.; Linderoth, T. R. Angew.
Chem. Int. Ed. 2007, 46, 9227–9230.
Influence of molecular geometry on the adsorption orientation for
oligophenylene-ethynylenes on Au(111)
Weigelt, S.; Busse, C.; Nielsen, M.; Gothelf, K. V.; Lægsgaard, E.; Besenbacher, F.;
Linderoth, T. R. J. Phys. Chem. B 2007, 111, 11342–11345.
Synthesis of an elongated linear oligo(phenylene ethynylene)-based building
block for application in DNA-programmed assembly
Blakskjær, P.; Gothelf, K. V. Org. Biomol. Chem. 2006, 4, 3442–3447.
DNA-programmed control of photosensitized singlet oxygen production
Cló, E.; Snyder, J. W.; Voigt, N. V.; Ogilby, P. R.; Gothelf, K. V. J. Am. Chem. Soc. 2006,
128, 4200–4201.
Femtomolar electrochemical detection of DNA targets using metal sulfide
nanoparticles
Hansen, J. A.; Mukhopadhyay, R.; Hansen, J. Ø.; Gothelf, K. V. J. Am. Chem. Soc. 2006,
128, 3860–3861.
Quantum-dot/aptamer-based ultrasensitive multi-analyte electrochemical
biosensor
Hansen, J. A.; Wang, J.; Kawde, A.-N.; Xiang, Y.; Gothelf, K. V.; Collins, G. J. Am. Chem.
Soc. 2006, 128, 2228–2229.
A cleavable amino-thiol linker for reversible linking of amines to DNA
Højfeldt, J. W.; Blakskjær, P.; Gothelf, K. V. J. Org. Chem. 2006, 71, 9556–9557.
Efficient N-arylation and N-alkenylation of the five DNA/RNA nucleobases
Jacobsen, M. F., Knudsen, M. M.; Gothelf, K. V. J. Org. Chem. 2006, 71, 9183–9190.
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Chiral switching by spontaneous conformational change in adsorbed organic
molecules
Weigelt, S.; Busse, C.; Petersen, L.; Rauls, E.; Hammer, B.; Gothelf, K. V.; Besenbacher,
F.; Linderoth, T. R. Nature Mater. 2006, 5, 112–117.
Effect of water on the palladium-catalyzed amidation of aryl bromides
Dallas, A. S.; Gothelf, K. V. J. Org. Chem. 2005, 70, 3321–3323.
A modular approach to DNA-programmed self-assembly of macromolecular
nanostructures
Gothelf, K. V.; Brown, R. S. Chem. Eur. J. 2005, 11, 1062–1069.
DNA-programmed assembly of nanostructures
Gothelf, K. V.; LaBean, T. H. Org. Biomol. Chem. 2005, 3, 4023–4037.
Preparation temperature dependence of size and polydispersity of alkylthiol
monolayer protected gold clusters
Jørgensen, J. M.; Erlacher, K.; Pedersen, J. S.; Gothelf, K. V Langmuir 2005, 21, 10320–
10323.
Electrochemical properties of mixed self-assembled monolayers on gold
electrodes containing mercaptooctylhydroquinone and alkylthiols
Larsen, A. G.; Gothelf, K. V. Langmuir 2005, 21, 1015–1021.
Two-photon photosensitized production of singlet oxygen: Sensitizers with
phenylene-ethynylene-based chromophores
McIlroy, S. P.; Cló, E.; Nikolajsen, L.; Frederiksen, P. K.; Nielsen, C. B.; Mikkelsen, K. V.;
Gothelf, K. V.; Ogilby, P. R. J. Org. Chem. 2005, 70, 1134–1146.
DNA-directed coupling of organic modules by multiple parallel reductive
aminations and subsequent cleavage of selected DNA sequences
Nielsen, M.; Dauksaite, V.; Kjems, J.; Gothelf, K. V. Bioconjugate Chem. 2005, 16, 981–
985.
Formation and structure of conjugated salen-cross-linked polymers and their
application in asymmetric heterogeneous catalysis
Nielsen, M. M.; Thomsen, A. H.; Jensen, T. R.; Jakobsen, H. J.; Skibsted, J.; Gothelf, K. V.
Eur. J. Org. Chem. 2005, 2005, 342–347.
Self-assembly of aluminium-salen coupled nanostructures from encoded modules
with cleavable disulfide DNA-linkers
Brown, R. S.; Nielsen, M.; Gothelf, K. V. Chem. Commun. 2004, 1464–1465.
Modular DNA-programmed assembly of linear and branched conjugated
nanostructures
Gothelf, K. V.; Thomsen, A.; Nielsen, M.; Cló, E.; Brown, R. S. J. Am. Chem. Soc. 2004,
126, 1044–1046.
An electrochemical quartz crystal microbalance study of the etching of gold
surfaces in the presence of tetramethylthiourea
Larsen, A. G.; Johannsen, K.; Gothelf, K. V. J. Coll. Int. Sci. 2004, 279, 158–166.
Synthesis of linear and tripoidal oligo(phenylene ethynylene)-based building
blocks for application in modular DNA-programmed assembly
Nielsen, M.; Thomsen, A. H.; Cló, E.; Kirpekar, F.; Gothelf, K. V. J. Org. Chem. 2004, 69,
2240–2250.
Catalytic asymmetric Henry reactions of silyl nitronates with aldehydes
Risgaard, T.; Gothelf, K. V.; Jørgensen, K. A. Org. Biomol. Chem. 2003, 1, 153–156.
Nucleophilic addition of nitrones to ketones: Development of a new catalytic
asymmetric nitrone-aldol reaction
Bøgevig, A.; Gothelf, K. V.; Jørgensen, K. A. Chem. Eur. J. 2002, 8, 5652–5661.
Catalytic asymmetric 1,3-dipolar cycloaddition reactions of azomethine ylides – a
simple approach to optically active highly functionalized proline derivatives
Gothelf, A. S.; Gothelf, K. V.; Hazell, R. G.; Jørgensen, K. A. Angew. Chem. Int. Ed. 2002,
41, 4236–4238.
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Attachment of alkyltrichlorosilanes to the terminal 3,5-dihydroxyphenyl moiety of
a self-assembled thiol monolayer on gold
Gothelf, K. V.; Larsen, A. G. J. Coll. Int. Sci. 2002, 255, 356–362.
lectron transfer reactions of self- assembled monolayers of
thio(phenylacetylene)n-substituted chiral metal-salen complexes
Nielsen, M.; Larsen, N. B.; Gothelf, K. V. Langmuir 2002, 18, 2795–2799.
Density functional theory study of enantiospecific adsorption at chiral surfaces
Sljivancanin, Z.; Gothelf, K. V.; Hammer, B. J. Am. Chem. Soc. 2002, 124, 14789–14794.
The first catalytic asymmetric Aza-Henry reaction of nitronates with imines: A
novel approach to optically active β-nitro-α-amino acid- and α,β-diamino acid
derivatives
Knudsen, K. R.; Risgaard, T.; Nishiwaki, N.; Gothelf, K. V.; Jørgensen, K. A. J. Am. Chem.
Soc. 2001, 123, 5843–5844.
Synthesis and catalytic properties of p-acylthio(phenylacetylene)n substituted
chiral manganese salen complexes
Nielsen, M.; Gothelf, K. V. J. Chem. Soc., Perkin Trans. 1 2001, 2440–2444.
Catalytic enantioselective addition of nitro compounds to imines – a simple
approach for the synthesis of optically active β-nitro-α-amino esters
Nishiwaki, N.; Rahbek Knudsen, K.; Gothelf, K. V.; Jørgensen, K. A. Angew. Chem. Int. Ed.
2001, 40, 2992–2995.
Self-assembled monolayers of long-chain xanthic acids on gold studied by
voltammetry
Gothelf, K. V. J. Electroanal. Chem. 2000, 494, 147–150.
Cheminform abstract: Asymmetric catalysis of 1,3-dipolar cycloaddition reactions:
The concepts of activation and induction of asymmetry
Gothelf, K. V.; Jensen, K. B.; Jørgensen, K. A. ChemInform 2000, 31, no.
Catalytic enantioselective 1,3-dipolar cycloaddition reactions of nitrones
Gothelf, K. V., Jørgensen, K. A. Chem. Commun. 2000, 1449–1458. Feature Article.
Asymmetric catalysis of 1,3- dipolar cycloaddition reactions – The concepts of
activation and induction of asymmetry.
Gothelf, K. V.; Jensen, K. B.; Jørgensen, K. A. Science Prog. 1999, 82, 327–350.
Catalytic enantioselective inverse-electron demand 1,3-dipolar cycloaddition
reactions of nitrones with alkenes
Simonsen, K. B.; Bayón, P.; Hazell, R. G.; Gothelf, K. V.; Jørgensen, K. A. J. Am. Chem.
Soc. 1999, 121, 3845–3853.
Molecular sieve dependent absolute stereoselectivity in asymmetric catalytic 1,3dipolar cycloaddition reactions
Gothelf, K. V.; Hazell, R. G.; Jørgensen, K. A. J. Org. Chem. 1998, 63, 5483–5488.
Asymmetric 1,3-Dipolar cycloaddition reactions
Gothelf, K. V.; Jørgensen, K. A. Chem. Rev. 1998, 98, 863–910.
A simple synthetic approach to 3,3’-diaryl BINOLs
Simonsen, K. B.; Gothelf, K. V.; Jørgensen, K. A. J. Org. Chem. 1998, 63, 7536–7538.
On the structure of C,N-diphenylnitrone in 1,3-dipolar cycloaddition reactions
Gothelf, K. V.; Hazell, R. G.; Jørgensen, K. A. Acta Chem. Scand. 1997, 51, 1234–1235.
On the trans-cis controversy in Ti-TADDOLate-catalysed cycloadditions.
Experimental indications for the structure of the reactive catalyst-substrate
intermediate
Gothelf, K. V.; Jørgensen, K. A. J. Chem. Soc., Perkin Trans. 2 1997, 111–116.
Improvement of TADDOLate-TiCl2-catalyzed 1,3-dipolar nitrone cycloaddition
reactions by substitution of the oxazolidinone auxiliary of the alkene with
succinimide
Jensen, K. B.; Gothelf, K. V.; Hazell, R. G.; Jørgensen, K. A. J. Org. Chem. 1997, 62,
2471–2477.
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Control of regio-, diastereo-, and enantioselectivity in the
[Ti(OTs)2(TADDOLato)]-catalyzed 1,3-dipolar cycloaddition reaction between 3acryloyloxazolidin-2-one and nitrones
Jensen, K. B.; Gothelf, K. V.; Jørgensen, K. A. Helv. Chim. Acta 1997, 80, 2039–2046.
Lanthanide-catalyzed endo- and enantioselective 1,3-dipolar cycloaddition
reactions of nitrones with alkenes
Sanchez-Blanco, A. I.; Gothelf, K. V.; Jørgensen, K. A. Tetrahedron Lett. 1997, 38, 7923–
7926.
Control of diastereo- and enantioselectivity in metal-catalyzed 1,3-dipolar
cycloaddition reactions of nitrones with alkenes. Experimental and theoretical
investigations
Gothelf, K. V.; Hazell, R. G.; Jørgensen, K. A. J. Org. Chem. 1996, 61, 346–355.
Metal-catalyzed asymmetric 1,3-dipolar cycload- dition reactions
Gothelf, K. V.; Jørgensen, K. A. Acta Chem. Scand. 1996, 50, 652–660.
A highly diastereoselective and enantioselective Ti(OTos)2-TADDOLate-catalyzed
1,3-dipolar cycloaddition reaction of alkenes with nitrones
Gothelf, K. V.; Thomsen, I.; Jørgensen, K. A. J. Am. Chem. Soc. 1996, 118, 59–64.
Crystal structure of a chiral titanium catalyst-alkene complex. The intermediate in
catalytic asymmetric Diels-Alder and 1,3-dipolar cycloaddition reactions
Gothelf, K. V.; Hazell, R. G.; Jørgensen, K. A. J. Am. Chem. Soc. 1995, 117, 4435–4436.
On the mechanism of Ti-TADDOLate-catalyzed asymmetric Diels-Alder reactions
Gothelf, K. V.; Jørgensen, K. A. J. Org. Chem. 1995, 60, 6847–6851.
Transition-metal catalyzed asymmetric 1,3-dipolar cycloaddition reactions
between alkenes and nitrones
Gothelf, K. V.; Jørgensen, K. A. J. Org. Chem. 1994, 59, 5687–5691.
Synthesis of 2,8-diarylpyrano[3,2-g]chromene-4,6-diones
Gothelf, K. V.; Torssell, K. B. G. Acta Chem. Scand. 1994, 59, 165–168.
Synthesis of flavones via application of nitrile oxide and the Stille reactions
Gothelf, K. V.; Torssell, K. B. G. Acta Chem. Scand. 1994, 48, 61–67.
A convenient synthesis of flavones. Synthesis of apigenin
Gothelf, K. V.; Thomsen, I.; Torssell, K. B. G. Acta Chem. Scand. 1992, 46, 494–495.
Book Chapters
3)
2)
1)
Self-assembling DNA Nanostructures for Patterned Molecular Assembly
in Nanobiotechnology II: More Concepts and Applications, (eds. C. Niemeyer & C. Mirkin),
LaBean T. H.; Gothelf, K. V.; Reif, J. H., Wiley-VCH, Weinheim, 2007.
Asymmetric Reactions
Gothelf, K. V.; Jørgensen, K. A. in Applications of 1,3-Dipolar Cycloaddition Chemistry
Towards Heterocycles and Natural Products Padwa and Pearson (Eds.), Wiley, 2002.
Asymmetric Metal-Catalyzed 1,3-Dipolar Cycloaddition Reactions
Gothelf, K. V. in Cycloaddition Reactions in Organic Chemistry, pp. 211-247, Kobayashi,
Jørgensen (Eds.), Wiley-VCH, 2001.
Others
2)
1)
Steps towards automated synthesis
Rotaru, A.; Gothelf, K.V. Nature Nanotech. 2010, 5, 760–761 (News and Views).
DNA Origami
Voigt, N. V.; Tørring, T.; Gothelf, K. V. DANSK KEMI 2010, s. 18.
Patents
a)
b)
Bis-heterocyclic Derivatives
Gothelf, K. V. WO9734881
Macromolecular Architectures
Gothelf, K. V.;Thomsen, A. H.; Nielsen, M.; Brown, R. S. WO2004050231