Revision 2 March 2015 Neutron Life Cycle Student Guide GENERAL DISTRIBUTION GENERAL DISTRIBUTION: Copyright © 2014 by the National Academy for Nuclear Training. Not for sale or for commercial use. This document may be used or reproduced by Academy members and participants. Not for public distribution, deli to, or reproduction by any third party without the prior agreement of the Academy. All other rights reserved. NOTICE: This information was prepared in connection with work sponsored by the Institute of Nuclear Power Operations (INPO). Neither INPO, INPO members, INPO participants, nor any person acting on behalf of them (a) makes any warranty or representation, expressed or implied, with respect to the accuracy, completeness, or usefulness of the information contained in this document, or that the use of any information, apparatus, method, or process disclosed in this document may not infringe on privately owned rights, or (b) assumes any liabilities with respect to the use of, or for damages resulting from the use of any information, apparatus, method, or process disclosed in this document. ii Table of Contents INTRODUCTION ..................................................................................................................... 1 TLO 1 NEUTRON MODERATION ............................................................................................ 2 Overview .......................................................................................................................... 2 ELO 1.1 Neutron Moderation .......................................................................................... 3 ELO 1.2 Moderator Characteristics ................................................................................. 9 TLO 1 Summary ............................................................................................................ 11 TLO 2 PROMPT AND DELAYED NEUTRONS ......................................................................... 12 Overview ........................................................................................................................ 12 ELO 2.1 Production of Prompt and Delayed Neutrons ................................................. 12 ELO 2.2 Delayed Neutron Fraction ............................................................................... 15 ELO 2.3 Prompt and Delayed Neutrons ........................................................................ 16 ELO 2.4 Delayed Neutrons and Reactor Control .......................................................... 18 TLO 2 Summary ............................................................................................................ 19 TLO 3 NEUTRON FLUX ....................................................................................................... 20 Overview ........................................................................................................................ 20 ELO 3.1 Prompt Neutron Energy .................................................................................. 21 ELO 3.2 Neutron Energy Spectrum ............................................................................... 22 ELO 3.3 Neutron Flux Spectrum Shape ........................................................................ 23 TLO 3 Summary ............................................................................................................ 25 TLO 4 NEUTRON LIFE CYCLE AND REACTOR CONTROL..................................................... 26 Overview ........................................................................................................................ 26 ELO 4.1 Neutron Life Cycle Terms .............................................................................. 26 ELO 4.2 Describe Each Term in the Six-Factor Formula ............................................. 30 ELO 4.3 Core Physical Changes and the Six-Factor Formula....................................... 34 ELO 4.4 Core Operating Parameter Changes and the Six-Factor Formula ................... 39 TLO 4 Summary ............................................................................................................ 46 NEUTRON LIFE CYCLE SUMMARY ...................................................................................... 49 iii This page is intentionally blank. iv Neutron Life Cycle Revision History Revision Date Version Number Purpose for Revision Performed By 10/31/2014 0 New Module OGF Team 12/10/2014 1 Added signature of OGF Working Group Chair OGF Team 3/4/2015 2 ο· Aligned answer of knowledge check on PPT OGF Team slide 28 to IG page 11. Aligned answer d in IG/SG to align with PPT. ο· Corrected fast nonleakage probability factor (Lf) on PPT slide 95. ο· Adjusted Lf to Lf on IG/SG page 33. ο· Corrected slide title for PPT slide 113 to read “Moderator-to-Fuel Ratio.” Introduction In thermal reactors, the neutrons that cause fission are born during the fission process at a much higher energy level than required. To make Rev 1 1 fission more probable, these neutrons must be slowed down to what is known as thermal energy. To reduce high-energy neutrons to thermal energy levels a process known as moderation must take place. Pressurized water reactors (PWRs) utilize water as a moderator for thermalizing neutrons. During the process of moderating fast neutrons, neutrons are subject to other events resulting in gains and losses before they cause fission and start the process all over again. The neutron life cycle describes this process. The neutron life cycle is important as it provides a tool for explaining the factors involved in controlling the nuclear fission rate. Proper management of the neutron life cycle makes control of a nuclear reactor possible. Objectives At the completion of this training session, the trainee will demonstrate mastery of this topic by passing a written exam with a grade of 80 percent or higher on the following Terminal Learning Objectives (TLOs): 1. Describe the process of neutron moderation in a nuclear reactor and the characteristics of desirable moderators. 2. Describe the production of prompt and delayed neutrons from fission and how these neutrons affect nuclear reactor control. 3. Describe the neutron flux spectrum in thermal reactors. 4. Describe the neutron life cycle throughout the lifetime of a thermal reactor and how core design and variation in operating parameters affect it. TLO 1 Neutron Moderation Overview Fission neutrons are born at an average energy of 2 mega electron volt (MeV) or fast neutrons and at high temperature. Fission neutrons immediately begin to reduce their energy levels as they undergo numerous scattering reactions with nuclei in the nuclear reactor core. A number of collisions with nuclei reduce the neutron’s energy to approximately the same average kinetic energy as its surrounding atoms or molecules. This energy reduction occurs in a medium known as the moderator. A neutron in energy equilibrium with its surrounding atoms is a thermal neutron. Since the kinetic energy depends on temperature (molecular movement), the energy of a thermal neutron also depends on temperature. At 68° Fahrenheit (F), the energy of a thermal neutron is 0.025 electron volt (eV). Energies less than 1eV yield neutrons designated or known as slow neutrons. 2 Rev 1 Objectives At the completion of this training session, you will be able to do the following: 1. Describe the following: a. Thermalization b. Moderator c. Moderating ratio d. Average logarithmic energy decrement e. Macroscopic slowing down power 2. Describe the four desirable characteristics of a good moderator and explain how moderator density affects neutron moderation. ELO 1.1 Neutron Moderation Introduction Lowering the energy level of a neutron is essential because thermal fission requires a neutron to be at thermal equilibrium. In a nuclear reactor, fast energy neutrons born from a fission event must be slowed to the thermal energy region to maintain a chain reaction. Thermalization or moderation is the process of reducing neutron energy to the thermal range by elastic scattering. Moderation Terms Thermalization Thermalization or moderation is the process of reducing neutron energy to the thermal range by elastic scattering. Moderator A moderator is the material used to thermalize neutrons. A desirable moderator is one that reduces the velocity of the fission neutrons, using a minimum number of scattering collisions with a low probability of neutron absorption. Slowing the neutrons in as few collisions as possible reduces their travel distance, thereby reducing the number of neutrons that leak out of the core. This shorter travel distance also reduces the number of resonance absorptions in non-fuel materials. Neutron leakage and resonance absorption are discussed in detail later in this module. Average Logarithmic Energy Decrement The average logarithmic energy decrement is the measure of neutron energy loss per collision. This term is the average decrease per collision of the logarithm of the change in neutron energy, denoted by the symbol ξ (Xi). Rev 1 3 π = ππ πΈπ πΈπ Where: ξ = logarithmic energy decrement Ei = initial energy level of neutron Ef = final energy level of neutron Macroscopic Slowing Down Power The logarithmic energy decrement is a convenient measure of the ability of a material to slow neutrons, but does not consider the probability of collisions taking place. Another measure of a moderator is the macroscopic slowing down power (MSDP), defined as the product of the logarithmic energy decrement and the macroscopic cross-section for scattering in the material. The equation below calculates the macroscopic slowing down power. πππ·π = ππ΄π Where: ξ = logarithmic energy decrement π΄π = Macroscopic scattering cross-section Moderating Ratio Macroscopic slowing down power calculates how rapidly a neutron will thermalize in the chosen moderator. However, it does not yet fully explain the effectiveness of the material as a moderator. An element such as boron has a high logarithmic energy decrement and good MSDP, but it is a poor moderator because of its high probability of absorbing neutrons. The moderating ratio considers absorbing probability as well as slowing down power; and therefore, is a more complete measure of moderator effectiveness. Moderating ratio is the ratio of the microscopic slowing down power to the microscopic cross-section for absorption. The higher the moderating ratio, the more effectively the material performs as a moderator. This equation shows the calculation for the moderating ratio (MR): ππ = πππ ππ The moderating ratio characterizes the effectiveness of a material as a moderator. It considers the ratio between the absorption and scattering cross-sections factoring in neutron energy levels. It does not consider the 4 Rev 1 density of the moderator. The table below compares moderating properties of different materials. Moderating properties of different materials are compared in the table below. Material ξ Number of Collisions to Thermalize Microscopic CrossSections σa–σs Moderating Ratio Water (H2O) also known as light water 0.948 19.0 0.66 – 103.0 148.0 Deuterium Oxide (D2O) also known as heavy water 0.570 35.0 0.001 – 13.6 7,752.0 Beryllium (Be) 0.209 86.0 0.0092 – 7.0 159.0 Carbon (C) 0.158 114.0 0.003 – 4.8 253.0 A good moderator is one with a high moderating ratio. Any of the materials shown in the table above make good moderators; however, commercial nuclear power applications often use light water (H2O) because it is plentiful, easily obtained, and inexpensive. Another benefit of using water is that water can serve as both a moderator and a coolant. Heavy water (D2O) is by far the best performing moderator; however, its higher cost precludes its use in U.S. commercial PWRs. Calculate Energy Loss Per Collision The symbol ξ is called the average logarithmic energy decrement because of the fact that a neutron loses, on average, a fixed fraction of its energy per scattering collision. Since the fraction of energy loss per collision for a given material is constant, ξ is also a constant. Because it is a constant and does not depend on the initial neutron energy, ξ is a convenient quantity for assessing the moderating ability of a material. Varieties of sources have tabulated ξ values for the lighter nuclei. With atomic mass numbers (A) greater than 10, the formula below is a relatively accurate approximation for ξ: π= 2 2 π΄+3 Rev 1 5 Since ξ equals the average logarithmic energy loss per collision, the total number of collisions necessary for a neutron to lose a given amount of energy may be determined by dividing ξ into the difference of the natural logarithms of the energy range in question. The equations below show this calculation. π= π= ππ πΈβππβ − ππ πΈπππ€ π πΈβππβ ππ ( πΈ ) πππ€ π If it is desirable to work with an average fractional energy, loss per collision as opposed to an average logarithmic fraction the following relationship is useful: πΈπ = πΈπ (1 − π₯)π Where: πΈπ = initial neutron energy πΈπ = neutron energy after N collisions x = average fractional energy loss per collision N = number of collisions Average Logarithmic Energy Decrement The table below presents the steps to determine the number of collisions necessary for a neutron to reach certain energy. This information is important when determining the moderator properties. Step Action 1. Determine the average logarithmic energy decrement for A > 10 2. Determine the average logarithmic energy decrement for A < 10 3. 6 Determine the number of collisions (N) to reach a lower energy Calculation π = ππ π= π= πΈπ πΈπ 2 2 π΄+3 πΈβππβ ππ ( πΈ ) πππ€ π Rev 1 Step Action 4. Determine the energy level after a number of collisions Calculation πΈπ = πΈπ (1 − π₯)π Example 1 How many collisions are required to slow a neutron from an energy of 2 MeV to a thermal energy of 0.025 eV, using water as the moderator? For water, ξ = 0.948. π= πΈβππβ ππ ( πΈ ) πππ€ π ππ ( π= 2 × 106 ππ ) 0.025 ππ 0.948 π = 19.2 ππππππ ππππ Example 2 If the average fractional energy loss per collision in hydrogen (H) is 0.63, what will be the energy of a 2 MeV neutron after... a. 5 collisions? b. 10 collisions? a) πΈπ = πΈπ (1 − π₯)π E5 = (2 × 106 eV)(1 − 0.63)5 = 13.9 kilo electron volt (keV) b) EN = Eo (1 − x)N E10 = (2 × 106 eV)(1 − 0.63)10 = 96.2 eV Rev 1 7 Knowledge Check A _______________ is a material within a reactor which is responsible for thermalizing neutrons. A. fuel rod B. moderator C. poison D. reflector Knowledge Check The process of reducing the energy level of a neutron from the energy level at which it is produced to an energy level in the thermal range is known as _______________. 8 A. moderating ratio B. resonance absorption C. thermalization D. inelastic scattering Rev 1 Knowledge Check The average logarithmic energy decrement is important because... A. it can be used to determine if a material is a good moderator. B. it can be used to determine the amount of energy released from fission. C. it accounts for the change in binding energy change during fission. D. it accounts for the change in mass during fission. ELO 1.2 Moderator Characteristics Introduction The ideal moderator requires the following nuclear properties: ο· ο· ο· ο· Large scattering cross-section Small absorption cross-section Large energy loss per collision High atomic density Desirable Moderator Properties A material with a mass equal to a neutron, but with a large scattering crosssection is desirable as a moderator. A substance having a high absorption cross-section, acts as a poison, removing available neutrons for fission. A moderator with a low atomic density has few atoms available to thermalize neutrons. Carbon, hydrogen, beryllium, and water (both heavy and light) are moderators used in nuclear reactors. In the U.S., most reactors use light water as the moderator. Water is a good moderator because the hydrogen atoms in water are close in mass (good for elastic scattering) to the thermalized neutrons. A neutron loses more energy in a collision with an atom of nearly its own mass than in a collision with an atom whose mass is much greater than the incident neutron (inelastic scattering — billiard ball effect). Water moderators, rather than other materials, thermalize neutrons in fewer collisions, reducing both the time and distance required for thermalization. Rev 1 9 Moderator Density Effects Temperature changes affect moderator density in an operating reactor. These density changes affect the moderator’s ability to thermalize neutrons. This in turn affects the number of neutrons available for fission. Consider a PWR (light water moderator and coolant) as an example. If the moderator temperature increases, the density of the water decreases. Decreasing water density means there are fewer water atoms per unit volume to thermalize neutrons. The neutrons will have to travel further to thermalize, and this larger travel distance will take longer. Because of this and other factors discussed later, there is now an increased chance that these neutrons will not be available for fission. Fewer neutrons available for fission, means fewer fissions, resulting in less reactor power. Knowledge Check Which of the items below is not a desirable property for a neutron moderator? A. Large absorption cross-section B. Large scattering cross-section C. Large energy loss per collision D. High atomic density Knowledge Check The density of a moderator is important because... 10 A. it can affect the number of target nuclei available for collisions. B. it can affect the number of target nuclei available for absorption. C. it can affect the number of collisions. D. it can affect the energy loss per collision. Rev 1 TLO 1 Summary In this lesson, you learned about neutron moderation: how thermalization works with a moderator to reduce the velocity of the fission neutrons, average logarithmic energy decrement, and macroscopic slowing down power and moderating ratio. The listing below provides a summary of sections in this TLO. 1. Slowing, or lowering, a neutron’s energy level is impacted by the following factors: Thermalization — the process of reducing the energy level of a neutron from its birth energy to the energy level of the surrounding atoms. ο· The moderator is the reactor material present for thermalizing neutrons. ο· Moderating ratio — the ratio of the microscopic slowing down power to the microscopic cross-section for absorption. This ratio characterizes the effectiveness of a material as a moderator. ο· The average logarithmic energy decrement, ξ — the average change in the logarithm of neutron energy per collision. ο· Macroscopic slowing down power — the product of the average logarithmic energy decrement, and the macroscopic crosssection for scattering. 2. There are four desirable characteristics of a moderator: ο· Large scattering cross-section ο· Small absorption cross-section ο· Large energy loss per collision ο· High atomic density — The density of the moderator affects its ability to moderate neutrons. A less dense moderator results in neutrons taking longer and traveling further to thermalize. — The equation below calculates the energy loss after a specified number of collisions. ο· πΈπ = πΈπ (1 − π₯)π Now that you have completed this lesson, you should be able to do the following: 1. Describe the following: a. Thermalization b. Moderator c. Moderating ratio d. Average logarithmic energy decrement e. Macroscopic slowing down power 2. Describe the four desirable characteristics of a good moderator, and explain how moderator density affects neutron moderation. Rev 1 11 TLO 2 Prompt and Delayed Neutrons Overview Not all neutrons are born immediately following fission. Fission releases most neutrons virtually instantaneously; these are referred to as prompt neutrons. The remaining neutrons (a very small fraction), are born after the decay of certain fission products and are referred to as delayed neutrons. Although delayed neutrons are a very small fraction of the total number of neutrons, they play an extremely important role in controlling the reactor. Objectives Upon completion of this lesson, you will be able to do the following: 1. Describe the origin and production of prompt and delayed neutrons. 2. State the approximate fraction of neutrons that are born as delayed neutrons from the fission of the following fuels: a. Uranium-235 b. Plutonium-239 3. Define prompt and delayed neutron lifetimes and their generation times. 4. Explain the effects of delayed neutrons on reactor control. ELO 2.1 Production of Prompt and Delayed Neutrons Introduction There are two ways to classify neutrons. One is to categorize according to energy, such as fast or thermal. Another is to classify according to birth time relative to a fission event. Those neutrons born immediately after a fission event are prompt neutrons, those born later from the decay of certain fission products are delayed neutrons. 12 Rev 1 Glossary Prompt Neutrons Within about 10-14 seconds of a fission event, a majority (≈ 99.36 percent) of the neutrons are released (born). These are prompt neutrons. The number of prompt neutrons emitted during a fission event depends on the type of fuel used (U-235 averages 2.4 per fission event). The most probable energy for a prompt neutron is approximately 1 MeV, and the average energy is approximately 2 MeV. Delayed Neutrons A small portion of the neutrons born of fission, are born delayed from delayed neutron precursors. Delayed neutrons are neutrons that are born significantly after the fission process has taken place. On average, delayed neutrons are born approximately 12.7 seconds after the fission event. Delayed neutrons are born fast but at a lower energy than prompt neutrons (≈ 0.5 MeV). Delayed Neutron Precursors A delayed neutron precursor refers to delayed neutrons emitted immediately following the first beta decay of a fission fragment. An example of a delayed neutron precursor is bromine-87 (Br), shown below. Br-87 is the fission product; Kr-87 (Krypton) is the delayed neutron precursor, with Kr86 (Krypton) the result of the delayed neutron birth. 86 π΅π 35 π π½− 87 86 → πΎπ πΎπ → 36 πππ π‘πππ‘πππππ’π 36 π π‘ππππ 55.9 π ππ Example It is convenient to combine the known delayed neutron precursors into groups with appropriately averaged half-life properties. These groups will vary somewhat depending on the fuel or mixture of fuel in the reactor. The table below lists the characteristics for the six delayed neutron precursor groups resulting from the thermal fission of uranium-235. Group Half Life (Seconds) Delayed Neutron Fraction Average Energy (MeV) 1 55.7 0.00021 0.25 2 22.7 0.00142 0.46 3 6.2 0.00127 0.41 Rev 1 13 Group Half Life (Seconds) Delayed Neutron Fraction Average Energy (MeV) 4 2.3 0.00257 0.45 5 0.61 0.00075 0.41 6 0.23 0.00027 N/A Total N/A 0.0065 N/A Knowledge Check Which one of the following types of neutrons has an average neutron generation lifetime of 12.5 seconds? A. Prompt B. Delayed C. Fast D. Thermal Knowledge Check Delayed neutrons are the neutrons that... A. have reached thermal equilibrium with the surrounding medium. B. are expelled within 10-14 seconds of the fission event. C. are produced from the radioactive decay of certain fission fragments. D. are responsible for the majority of U-235 fissions. Knowledge Check In a comparison between a delayed neutron and a prompt neutron produced from the same fission event, the prompt neutron is more likely to... 14 Rev 1 A. require a greater number of collisions to become a thermal neutron. B. be captured by U-238 at a resonance energy peak between 1 eV and 1,000 eV. C. be expelled with a lower kinetic energy. D. cause thermal fission of a U-235 nucleus. ELO 2.2 Delayed Neutron Fraction Introduction The fraction of all neutrons produced by each delayed neutron precursor is the delayed neutron fraction for that precursor. The total fraction of all neutrons born as delayed neutrons is the delayed neutron fraction (β). Each nuclear fuel has different delayed neutron fraction (β). Delayed Neutron Fraction (β) The fraction of delayed neutrons (β) varies depending on the predominant fissile nuclide in use. The delayed neutron fractions (β) for the nuclides of most interest are as follows: ο· ο· ο· ο· Uranium-233 β = 0.0026 Uranium-235 β = 0.0065 Uranium-238 β = 0.0148 Plutonium-239 β = 0.0021 It is significant to note that uranium-235 and plutonium-239 are the two major fuels in use in PWRs. Although the β values are small, β for uranium-235 is considerably larger than plutonium-239. Over core life, uranium-235 concentration will decrease, while plutonium239 increases. This will result in lower delayed neutron fraction over core life. Knowledge Check What is the delayed neutron fraction of uranium-235? Rev 1 A. 0.0065 B. 0.0148 C. 0.0021 D. 0.0026 15 ELO 2.3 Prompt and Delayed Neutrons Introduction Neutron lifetime is the time that a free neutron exists, from its birth until its loss either from leakage or by absorption. Neutron generation time is the time for a neutron from one generation to cause fission that produces the next generation of neutrons. Prompt Neutron Lifetime Prompt neutron lifetime is the average time span from prompt neutron birth until its loss from either leakage or absorption in another nucleus. This time is the sum of thermalization time and diffusion time. Diffusion time relates to absorption time of the thermal neutron and is a function of the absorption mean free path, λa, divided by the average velocity of the thermal neutron. Thermalization time is small (microseconds) compared to diffusion time (milliseconds) and is usually ignored in calculations. Simply stated, prompt neutron lifetime is the time from birth to loss by either leakage or absorption. Delayed Neutron Lifetime Delayed neutron lifetime begins at its birth from a delayed neutron precursor and ends at loss from leakage or absorption in another nucleus. We calculate delayed neutron lifetime similarly to prompt neutron lifetime. The key difference is the time of birth, which is not at the time of fission but at the time of birth from decay of one of the delayed neutron precursors. Prompt Neutron Generation Time The generation time for prompt neutrons (β* — pronounced ell-star) is the total time from birth of a fast neutron in one generation to birth in the next generation. Prompt neutron generation time is equal to the prompt neutron lifetime added to the time required for a fissionable nucleus to emit a fast neutron after absorption. In water-moderated reactors, thermal neutrons exist for about 10-4 seconds before absorption. Taking into account losses due to leakage, the prompt neutron lifetime is equal to about 10-4 to 10-5 seconds (leakage occurs quicker). Following absorption, fission, and the birth of fast neutron(s) occurs in about 10-13 seconds — quickly. Therefore, in water-moderated thermal reactors, β* is about 10-4 seconds to 10-5 seconds. Delayed Neutron Generation Time Similar to prompt neutron generation time, delayed neutron generation time equals the time of birth of a delayed neutron from a delayed neutron precursor to the time of birth of a neutron(s) in the next generation. 16 Rev 1 The significant difference between prompt and delayed neutron generation time is the delay in birth from their delayed neutron precursors. As previously mentioned, the average time for decay of the delayed neutron precursors from fission of uranium-235 is 12.7 seconds. With this relatively large time interval, the delayed neutron lifetime is insignificant. Therefore, the average delayed neutron generation time is equal to approximately 12.7 seconds. This significance of this time is shown next. Average (or Effective) Generation Time Slowing the neutron generation time from 10-4 seconds to a more reasonable time period is necessary for improved reactor control. Adding delayed neutrons makes this possible. Delayed neutrons with their long generation time have a large effect on the overall average neutron generation time. To determine the average generation time, we calculate a weighted average taking into consideration the prompt neutron generation time, and the delayed neutron generation. The following equation shows this mathematically: ππππ ππ£πππππ = ππππ ππππππ‘(1 − π½) + ππππ πππππ¦ππ(π½) Demonstration Assume a prompt neutron generation time for a particular reactor of 1 x 10-4 seconds and a delayed neutron generation time of 12.7 seconds. If β is 0.0065, calculate the average generation time. ππππ ππ£πππππ = ππππ ππππππ‘(1 − π½) + ππππ πππππ¦ππ(π½) = (1 × 10−4 π ππππππ )(0.9935) + (12.7 π ππππππ )(0.0065) = 0.0827 π ππππππ Knowledge Check __________ begins when it is released from a precursor and ends when it is absorbed in another nucleus. Rev 1 A. Delayed neutron lifetime B. Prompt neutron lifetime C. Fast neutron fraction D. Thermal neutron fraction 17 Knowledge Check Neutron generation time describes... A. time from one generation to the next generation of neutrons. B. time that it takes for a neutron to become thermalized. C. time it takes for neutron precursors to emit neutrons. D. time that neutrons are born after a fission event. Knowledge Check What effect on the average neutron generation time would a smaller β value produce? A. The result would be a longer average generation time. B. The result would be a shorter average generation time. C. More information is needed to determine the effect on average generation time. D. β does not have any effect on average generation time. ELO 2.4 Delayed Neutrons and Reactor Control Introduction Rapid power excursions result from the prompt neutron generation time of 10-4 seconds or faster (prompt neutrons only), which makes safe control of the reactor difficult. As seen in the previous section, delayed neutrons increase overall neutron generation time and slow down the power excursions. Delayed Neutrons and Reactor Control If a reactor was operating using only prompt neutrons (β = 0), the generation time would be about 1 x 10-4 seconds. This means that a fractional change in power would occur every 1 x 10-4 seconds. However, by operating the reactor with delayed neutrons, the average or effective neutron generation time extends to approximately 0.0827 seconds. While this seems fast, it is more than eight (8) times slower than the rate on 18 Rev 1 prompt neutrons alone, and leads to a more controllable rate of power change, which increases operator control. Although delayed neutrons make up only a small fraction of the total neutron population, they are important to the safe control of a fission chain reaction and changes in reactor power level. Knowledge Check If a reactor fueled with U-235 was operating and not dependent on delayed neutrons, the average generation time would be... A. 12.5 seconds. B. 0.0001 seconds. C. 80 seconds. D. 0.0065 seconds. TLO 2 Summary During this lesson, you learned about prompt and delayed neutrons: their origin and production, the approximate fraction of neutrons born delayed from the fission of Uranium-235 and Plutonium-239, the lifetime and generation times of both prompt and delayed neutrons, and the effects of delayed neutrons on reactor control. The listing below provides a summary of sections in this TLO. 1. Neutrons are classified by energy, such as fast or thermal, or by birth time relative to a fission event, and are considered either prompt or delayed. ο· Prompt neutrons are born directly from fission within 10-14 seconds of the fission event. ο· Delayed neutrons are born from the decay of fission products are called delayed neutron precursors. Delayed neutrons are born on the average, about 12.7 seconds after the fission event. ο· When a delayed neutron precursor undergoes a β- decay, it results in an excited daughter nucleus which ejects a neutron. Delayed neutrons are born based on the half-life of the delayed neutron precursor. ο· Delayed neutron precursors are grouped according to half-life. Half-lives vary from fractions of a second to almost a minute. 2. The fraction of neutrons born as delayed neutrons is different for each fuel isotope; fractions for two common fuel materials are: ο· Uranium-235 — 0.0065 ο· Plutonium-239 — 0.0021 Rev 1 19 3. Define the prompt and delayed neutron lifetimes and their generational times. ο· The prompt neutron lifetime begins when a prompt neutron is born, and ends when it is lost through leakage or is absorbed in another nucleus. ο· The delayed neutron lifetime begins when a delayed neutron is released from a delayed neutron precursor, and ends when it is lost through leakage or is absorbed in another nucleus. ο· Prompt neutron generation time is the sum of the time between a fissionable nuclide absorbing a neutron and fission neutrons being released (10-13 seconds), and the prompt neutron lifetime. ο· Prompt neutron generation time is about 1 x 10-4 seconds. ο· Delayed neutron generation time is the sum of the time between a fissionable nuclide absorbing a neutron and fission neutrons being born (10-13 seconds), and the delayed neutron lifetime. ο· The half-life of the delayed neutron precursors dominates the delayed neutron generation time. ο· Average (or effective) delayed neutron generation time is about 12.7 seconds. — Weighted average — ππππ ππ£πππππ = ππππ ππππππ‘(1 − π½) + ππππ πππππ¦ππ(π½) 4. Explain the effects of delayed neutrons on reactor control. ο· Delayed neutrons slow the rate of power changes. ο· If only prompt neutrons existed, reactor control would not be possible due to the rapid power changes. Now that you have completed this lesson, you should be able to do the following: 1. Describe the origin and production of prompt and delayed neutrons. 2. State the approximate fraction of neutrons that are born as delayed neutrons from the fission of the following fuels: a. Uranium-235 b. Plutonium-239 3. Define prompt and delayed neutron lifetimes and generation times. 4. Explain the effects of delayed neutrons on reactor control. TLO 3 Neutron Flux Overview The neutron population in a reactor consists of neutrons at many different energy levels. This spectrum of energy levels is the neutron flux spectrum. For graphical purposes, it is plotted either by the fraction of neutrons or by the neutron flux at a given energy, versus neutron energy levels. Different types of reactors will have different neutron energy spectrums to match their design. This lesson will discuss neutron energy spectrums associated with PWR thermal reactors. 20 Rev 1 Objectives Upon completion of this lesson, you will be able to do the following: 1. Describe the average energy at which prompt neutrons are produced. 2. Describe the shape of the neutron energy spectrum in a thermal reactor. 3. Explain the reason for the shape of the neutron energy spectrum for a thermal reactor, including variable(s) that have the most effect on thermal neutron velocity. ELO 3.1 Prompt Neutron Energy Introduction All neutrons born of fission are high-energy neutrons (fast neutrons), and most of them range in energy between 0.1 MeV and 10 MeV. Their birth energy affects the shape of the neutron energy spectrum. Prompt Neutron Birth Energy Plotting the fraction of fission neutrons per MeV as a function of neutron energy provides a graphic illustration of the neutron energy distribution for prompt neutrons, or spectrum. The figure below shows the prompt neutron energy spectrum for uranium-235 thermal fissions. Values vary according to fuel nuclides. The figure shows that the most probable neutron energy (highest fraction) is about 0.7 MeV. By analyzing the curve, we determine that the average neutron energy is about 2 MeV. Figure: Prompt (birth) Neutron Energy Spectrum for Thermal Fission of Uranium-235 Rev 1 21 Knowledge Check All prompt neutrons are born at the same energy level. A. True B. False ELO 3.2 Neutron Energy Spectrum Introduction The spectrum of prompt energies at birth varies significantly from the energy spectrum of all neutrons existing in the reactor at any given time. The next figure shows neutron flux spectrums for a thermal reactor and a fast breeder reactor. In either case, the prompt neutron spectrum at birth is approximately the same. However, overall the energy spectrum of all neutrons is considerably different between these two reactors due to design and moderator effects. A fast breeder reactor requires a larger fast neutron flux, where a thermal reactor needs slower thermal neutrons for fission. Thermal reactors have a neutron energy spectrum that has two pronounced peaks, one in the thermal energy region where the neutrons are in thermal equilibrium with the core materials and another in the fast region at energies where neutron production occurs. Figure: Comparison of Neutron Flux Spectra for Thermal and Fast Breeder Reactor 22 Rev 1 Knowledge Check A graph of the neutron energy spectrum for a thermal reactor would… (choose the most correct answer) A. have a distinct peak at approximately 2 MeV. B. have the same approximate shape as the prompt neutron energy spectrum. C. have the same approximate shape as the delayed neutron energy spectrum. D. have two peaks, one in the thermal energy region and another in the fast region. ELO 3.3 Neutron Flux Spectrum Shape Introduction The shape of the neutron energy spectrum in a thermal reactor depends on neutron energy losses during the slowing down process and the temperature of the moderator. Thermal reactors have a neutron energy spectrum with two pronounced peaks. The first peak is in the thermal energy region where the neutrons are in thermal equilibrium with the core materials. The second peak is in the fast region at energies where neutron production occurs. The large number of fast neutrons born from fission combined with delayed neutrons from precursors that start to slow down explains the initial higher energy peak. During the neutron thermalization process, elastic collisions remove a constant fraction or average of neutron energy per collision, meaning that the neutrons lose larger amounts of energy per collision at higher energies than at lower energies. Note the following about the neutron energy spectrum: 1. There is a flat flux level between one (1) eV and 100 kiloelectron volt (keV). This area represents mostly intermediate range neutrons that have few losses in this energy range as they slow. 2. The neutron energy losses per collision are smaller at lower energy levels; this results in neutron flux peaking at lower energies before absorption occurs. This is also near the energy level where diffusion occurs before absorption – remember diffusion time is longer than slowing down time. This results in the lower energy flux peak at approximately 0.1 eV. Rev 1 23 Figure: Comparison of Neutron Flux Spectra for Thermal and Fast Breeder Reactor Most Probable Neutron Velocities In the thermal region (0.025eV), neutrons achieve thermal equilibrium with the atoms of the moderator material. In any given collision, they may gain or lose energy (velocity), and over successive collisions gain as much energy as they lose. These thermal neutrons, even at a constant temperature, do not all have the same energy or velocity. There is a distribution of energies, known as the Maxwell Distribution, which determines the most probable neutron velocity (energy) for a given temperature. Most thermal neutrons remain close to this most probable energy, but with a spread above and below this value. The most probable velocity (vp) of a thermal neutron is determined by the temperature of the medium and is decided by: π£π = √ 2ππ π Where: vp = most probable velocity of neutron (centimeter [cm]/second [sec]) k = Boltzmann’s Constant (138 x 10-16 ergon (erg)/ Kelvin [°K]) T = absolute temperature in degrees Kelvin (°K) m = mass of thermal neutron (1.66 x 10-24 grams) 24 Rev 1 Knowledge Check Thermal neutrons are at what energy level? A. < 1 eV B. 10 eV C. > 1 MeV D. 0.1 MeV TLO 3 Summary During this lesson, you learned about neutron flux: the average energy that produces prompt neutrons, the shape of the neutron energy spectrum in a thermal reactor, and the reason for the neutron energy spectrum’s shape for a thermal reactor, including variable(s) that have the most effect on thermal neutron velocity. The listing below provides a summary of sections of this TLO. Prompt neutrons are born at energies between 0.1 MeV and 10 MeV. ο· The average prompt neutron energy is about 2 MeV. 2. The neutron energy spectrum for thermal reactors has two pronounced peaks, one in the thermal energy region where the neutrons are in thermal equilibrium with the core materials and another in the fast region at energies where neutrons are born. 3. The neutron flux spectrum for the fast energy region of a thermal reactor has a shape similar to that of the spectrum of neutrons born by the fission process. ο· Because of the smaller neutron energy losses per collision at lower energy levels the neutrons pile up at lower energies before absorption occurs (diffusion time). This results in the lower energy flux peak at approximately 0.1 eV. 1. Now that you have completed this lesson, you should be able to do the following: 1. Describe the average energy at which prompt neutrons are produced. 2. Describe the shape of the neutron energy spectrum in a thermal reactor. 3. Explain the reason for the shape of the neutron energy spectrum for a thermal reactor including variable(s) that have the most effect on thermal neutron velocity. Rev 1 25 TLO 4 Neutron Life Cycle and Reactor Control Overview Some of the fast neutrons born by fission in one generation cause fission in the next generation. Fission neutrons travel through a series of events as they slow to thermal energies, leak, or are absorbed in the reactor. The neutron life cycle describes these events, and is the topic of this chapter. For simplicity, the following assumptions provide an outline of the neutron life cycle. ο· ο· ο· ο· ο· ο· ο· ο· ο· All neutrons are born as fast neutrons. Some fast neutrons are absorbed by fuel and cause fast fission. Some fast neutrons leak out of the reactor core. Some fast neutrons undergo resonance capture while slowing down. All remaining fast neutrons become thermalized. Some thermal neutrons leak out of the core. Some thermal neutrons are absorbed by non-fuel material. Some thermal neutrons are absorbed by fuel and do not cause fission. All remaining thermal neutrons are absorbed by fuel and cause thermal fission. Objectives Upon completion of this lesson, you will be able to do the following: 1. Define the following terms associated with the neutron life cycle: a. Infinite multiplication factor (k∞) b. Effective multiplication factor (keff) c. Subcritical d. Critical e. Supercritical 2. Describe each term in the six-factor formula using the ratio of the number of neutrons present at different points in the neutron life cycle. 3. Explain how the physical design of the reactor core affects each of the terms in the six-factor formula. 4. Explain how a change to plant operating parameters affects each of the factors of the six-factor formula. ELO 4.1 Neutron Life Cycle Terms Introduction Several key terms require understanding in order to relate to the neutron life cycle, including the following: ο· ο· ο· 26 Infinite multiplication factor (k∞) Effective multiplication factor (keff) Subcritical Rev 1 ο· ο· Critical Supercritical Infinite Multiplication Factor Glossary Not all of the neutrons produced by fission are available to cause new fissions. Some are absorbed by nonfissionable material, some are absorbed parasitically in fissionable material and do not cause fission, and others leak out of the reactor. Fortunately, to maintain a selfsustaining chain reaction, it is not necessary that every neutron produced in fission initiate another fission reaction. The minimum condition required for a selfsustaining chain reaction is that each nucleus undergoing fission produces at least one neutron that ultimately causes fission of another nucleus. All of the possible things that can happen to the neutron from birth to fission are expressed in terms of a multiplication factor. If the multiplication factor equals one (1), it means that a self-sustaining chain reaction is occurring. The infinite multiplication factor (k∞) is used to consider a reactor of infinitely large size where no neutron leakage can occur. k∞ is defined as the ratio of neutrons produced by fission in one generation to the number of neutrons lost through absorption in the preceding generation. It is also known as the four-factor formula. It is expressed mathematically as: πππ’π‘πππ πππππ’ππ‘πππ ππππ πππ π πππ ππ πππ πππππππ‘πππ π∞ = πππ’π‘πππ πππ ππππ‘πππ ππ π‘βπ πππππππππ πππππππ‘πππ Rev 1 27 Effective Multiplication Factor (keff) Glossary The infinite multiplication factor only represents a reactor that is infinitely large assuming no neutrons leaking out of the reactor. To describe the neutron life cycle in a real, finite reactor, it is necessary to account for neutrons that leak. This factor is the effective multiplication factor (keff). It is expressed mathematically: ππππ πππ’π‘πππ πππππ’ππ‘πππ ππππ πππ π πππ ππ πππ πππππππ‘πππ = πππ’π‘πππ πππ ππππ‘πππ πππ’π‘πππ πππππππ ππ π‘βπ πππππππππ + ππ π‘βπ πππππππππ πππππππ‘πππ πππππππ‘πππ Effective Multiplication Factor (keff) Versus Infinite Multiplication Factor (k∞) The balance between production of neutrons and their absorption in the core and leakage out of the core determines the value of the multiplication factor. If the leakage is small enough to be neglected, the multiplication factor depends only on the balance between production and absorption. This is called the infinite multiplication factor (k∞) since by definition an infinitely large core has no leakage. The infinite multiplication factor, also called the four-factor formula, considers the four factors shown below: π∞ = (πππ π‘ πππ π πππ ππππ‘ππ)(πππ ππππππ ππ ππππ ππππππππππ‘π¦) (π‘βπππππ π’π‘ππππ§ππ‘πππ ππππ‘ππ)(πππππππ’ππ‘πππ ππππ‘ππ) To include leakage, the effective multiplication factor (keff) is used. The effective multiplication factor (keff) for a finite reactor is expressed mathematically in terms of the infinite multiplication factor and two additional factors, which account for neutron leakage as shown below. ππππ = π∞ (πππ π‘ ππππππππππ ππππππππππ‘π¦)(π‘βπππππ ππππππππππ ππππππππππ‘π¦) These multiplication factors are explained in the next section. Effective Multiplication Factor (keff) Versus Criticality When the value of keff is 1, a self-sustaining chain reaction of fissions occurs where the neutron population neither increases nor decreases. This is referred to as critical or critical reactor and is expressed as keff = 1. 28 Rev 1 ο· When neutron production is greater than the losses due to absorption and leakage, the reactor is called supercritical. A supercritical reactor has a keff greater than one (keff > 1), and the neutron flux is increasing each generation. This is normal on power increases. ο· When the neutron production is less than the losses due to absorption and leakage, the reactor is called subcritical. A subcritical reactor has a keff less than one (keff < 1), and the neutron flux is decreasing each generation. This is normal on a power decrease. When keff is not equal to exactly one, neutron flux and therefore reactor power will change. For this reason, it is important to understand how changes in reactor operating conditions affect keff. Knowledge Check A thermal neutron is about to interact with a uranium238 (U-238) nucleus in an operating nuclear reactor core. Which one of the following describes the most likely interaction and the effect on core keff? A. The neutron will be scattered, thereby leaving keff unchanged. B. The neutron will be absorbed and U-238 will not undergo fission, thereby decreasing keff. C. The neutron will be absorbed and U-238 will undergo fission, thereby increasing keff. D. The neutron will be absorbed and U-238 will undergo radioactive decay to Pu-239, thereby increasing keff. Knowledge Check A nuclear reactor is initially subcritical with the effective multiplication factor (keff) equal to 0.998. After a brief withdrawal of control rods, keff equals 1.000. The reactor is currently _______________. Rev 1 A. prompt critical B. exactly critical C. supercritical D. subcritical 29 ELO 4.2 Describe Each Term in the Six-Factor Formula Introduction As mentioned in the introduction to this chapter, a number of assumptions can be made regarding the possible paths a fission neutron may take during its lifetime. This section will take these assumptions and place them into ratios, the product of which equals keff or k∞. Infinite Multiplication Factor or Four Factor Formula A group of fast neutrons produced by fission can enter into several reactions. Some of these reactions reduce the neutron population and some increase the neutron population. There are four factors independent of the size and shape of the reactor and do not consider any neutron leakage from the reactor. This infinite multiplication factor considers all factors, but excludes fast and thermal neutron leakage. The equation below states the infinite multiplication factor. π∞ = ππππ Where: ε = fast fission factor ρ = resonance escape probability f = thermal utilization factor η = reproduction factor Each of these four factors represents a process that adds to or subtracts from the initial neutrons born in a generation by fission. Six-Factor Formula Because reactors are finite in size, two additional factors need consideration, including: ο· ο· Fast non-leakage probability (Lf) Thermal non-leakage probability (Lth) With the inclusion of these last two factors, we can determine the fraction of neutrons that remain after each of the events that occur as the neutrons complete their generation time. The effective multiplication factor (keff) can then be determined by the product of six terms: ππππ = ππΏπ ππΏπ‘β ππ 30 Rev 1 Note Note A pneumonic device to help you remember the sixfactor formula is “Every Little Person Loved the Funny Navy.” Fast Fission Factor (ε) The first event that the neutrons incur after birth is fast fission. Fast fission is fission caused by neutrons that are in the fast energy range, and results in a net increase in the fast neutron population of the reactor core. The crosssection for fast fission in uranium-235 or uranium-238 is small. However, there are still a significant number of fast neutrons that cause fission in uranium-235, uranium-238, and plutomium-239. Even though uranium-235 enrichment is small compared to uranium-238, a large fraction of fast fissions occur with uranium-235 because of its wider fission energy spectrum. The fast fission factor (ε) is defined as the ratio of the net number of fast neutrons produced by all fissions to the number of fast neutrons produced by thermal fissions. The equation below shows the mathematical expression of this ratio. π= ππ’ππππ ππ πππ π‘ πππ’π‘ππππ πππππ’πππ ππ¦ πππ πππ π ππππ ππ’ππππ ππ πππ π‘ πππ’π‘ππππ πππππ’πππ ππ¦ π‘βπππππ πππ π ππππ Value of Fast Fission Factor For a fast fission to occur, fast neutrons must pass close enough to a fuel nucleus while they are still fast neutrons. The value of ε is affected by fuel concentration and its physical arrangement proximity to the moderator. The fast fission factor is essentially 1.00 for a homogenous reactor where the fuel atoms are surrounded by moderator atoms (rapid moderation). However, in a heterogeneous reactor, a PWR for example, fuel atoms are packed closely together in fuel pellets within fuel rods and assemblies. Because of this, neutrons emitted from the fission of one fuel atom have a good chance of passing near another fuel atom before substantially slowing down. This arrangement results in some fast fission. For PWRs, 1.02 is a good value for ε; most heterogeneous reactors have a ε value in the range of 1.02 to 1.05. Fast Non-Leakage Probability (Lf) In a real reactor of finite size, some of the fast neutrons leak out of the boundaries of the reactor core before they begin the slowing down process. Of concern are the neutrons that do NOT leak out, as these remain to contribute to the fission process. The fast non-leakage probability (Lf) is the ratio of the number of fast neutrons that do not leak from the reactor Rev 1 31 core to the number of fast neutrons produced by all fissions. The equation below states this ratio: πΏπ = ππ’ππππ ππ πππ π‘ πππ’π‘ππππ π‘βππ‘ ππ πππ‘ ππππ ππππ πππππ‘ππ ππ’ππππ ππ πππ π‘ πππ’π‘ππππ πππππ’πππ ππ¦ πππ πππ π ππππ The fast non-leakage probability represents a net loss in neutron population and has value range of 0.85 to 0.97. Resonance Escape Probability (ρ) After fast fissions occur, neutrons continue to diffuse throughout the reactor. As they travel, they collide with nuclei of fuel, non-fuel material, and the moderator, losing part of their energy in each collision and slowing down. All nuclei within the reactor core have some probability of absorbing neutrons, as indicated by the microscopic cross-section for absorption (σa) for each material. The microscopic cross-section for absorption is not a constant value but is dependent on the energy level of the incident neutron. Normally, absorption cross-sections increase as neutron energy level decreases. However, certain nuclei, such as uranium-238 and plutonium240 in particular, show extremely high absorption cross-section peaks for neutrons at specific energy levels. At certain neutron energy levels, these absorption cross-sections are as much as 1,000 times higher than the cross-section for a slightly higher or lower energy neutron. These peaks in absorption cross-sections are referred to a resonance peaks or resonance peaking. For example, while neutrons are slowing down through the resonance peak region of uranium-238, about 6 eV to 200 eV, there is a chance that some of the neutrons will be captured (resonance capture). These captured neutrons are lost to the fission process for that particular generation of neutrons. For mathematical purposes, rather than considering those captured neutrons, the six-factor formula considers the number of neutrons that are not captured. The probability that a neutron will not be absorbed by a resonance peak is called the resonance escape probability. The resonance escape probability (ρ) is defined as the ratio of the number of neutrons that reach thermal energies to the number of fast neutrons that start to slow down. This ratio is shown below. π= ππ’ππππ ππ πππ’π‘ππππ π‘βππ‘ ππππβ π‘βπππππ ππππππ¦ ππ’ππππ ππ πππ π‘ πππ’π‘ππππ π‘βππ‘ π π‘πππ‘ π‘π π πππ€ πππ€π Value of Resonance Escape Probability 32 Rev 1 The value of the resonance escape probability is determined largely by the fuel-moderator arrangement and the amount of enrichment of uranium-235. To undergo resonance absorption, a neutron must pass close enough to a uranium-238 nucleus to be absorbed while slowing down. In a homogeneous reactor, neutrons slow down in the vicinity of fuel nuclei, easily meeting this condition. This means that a neutron has a high probability of being absorbed by uranium-238 while slowing down, making its resonance escape probability low. In a heterogeneous reactor, the neutron slows down in the moderator where there are no atoms of uranium-238 present. This means resonance absorption is less likely to occur and therefore, resonance escape probability is high. The value of the resonance escape probability is always less than one and ranges from 0.75 to 0.90 with a value of 0.87 a good approximation for a PWR. Thermal Non-Leakage Probability (Lth) Neutrons leak out of a finite reactor core after they reach thermal energies. Like fast leakage, our interest is in the neutrons that do NOT leak out, rather than in the ones that do. The thermal non-leakage probability (Lth) is defined as the ratio of the number of thermal neutrons that do not leak from the reactor core to the number of neutrons that reach thermal energies. The equation below shows this ratio: πΏπ‘β = ππ’ππππ ππ π‘βπππππ πππ’π‘ππππ π‘βππ‘ ππ πππ‘ ππππ ππππ πππππ‘ππ ππ’ππππ ππ πππ’π‘ππππ π‘βππ‘ ππππβ π‘βπππππ ππππππππ The thermal non-leakage probability represents a net loss in neutron population and has a value range of 0.85 to 0.99. Thermal Utilization Factor (f) The thermalized neutrons are still dispersed throughout the core where they are subject to absorption by either fuel or non-fuel material. The thermal utilization factor describes how effectively thermal neutrons are being absorbed by the fuel or underutilized by non-fuel materials within the reactor. The thermal utilization factor (f) is defined as the ratio of the number of thermal neutrons absorbed in the fuel to the number of thermal neutrons absorbed in all reactor materials. The equation below presents this ratio. π= ππ’ππππ ππ π‘βπππππ πππ’π‘ππππ πππ πππππ ππ π‘βπ ππ’ππ ππ’ππππ ππ π‘βπππππ πππ’π‘ππππ πππ πππππ ππ πππ πππππ‘ππ πππ‘ππππππ Rev 1 33 The thermal utilization factor is always less than one because some of the thermal neutrons absorbed within the reactor are not absorbed by atoms of the fuel, but are lost to the fission process. The thermal utilization factor ranges from 0.70 to 0.80. Reproduction Factor (η) Most of the neutrons absorbed in the fuel cause fission, but some do not. The reproduction factor (η) is defined as the ratio of the number of fast neutrons produced by thermal fission to the number of thermal neutrons absorbed in the fuel. The reproduction factor is shown below. π= ππ’ππππ ππ πππ π‘ πππ’π‘ππππ πππππ’πππ ππ¦ π‘βπππππ πππ π πππ ππ’ππππ ππ π‘βπππππ πππ’π‘ππππ πππ πππππ ππ π‘βπ ππ’ππ The reproduction factor represents net gain in neutron population and has a value range of 1.65 to 2.0. The reproduction factor can also be stated as a ratio of rates as shown below. π= π ππ‘π ππ πππππ’ππ‘πππ ππ πππ π‘ πππ’π‘ππππ ππ¦ π‘βπππππ πππ π πππ π ππ‘π ππ πππ ππππ‘πππ ππ π‘βπππππ πππ’π‘ππππ ππ¦ π‘βπ ππ’ππ Total Non-Leakage Probability (LT) The fast non-leakage probability (Lf) and the thermal non-leakage probability (Lth) may be combined into one term that gives the fraction of all neutrons that do not leak out of the reactor core. This term is called the total non-leakage probability and is given the symbol (LT). The equation below shows the formula for LT. πΏπ = πΏπ + πΏπ‘β The total non-leakage probability can be substituted for the fast and thermal non-leakage terms in the six-factor formula. Knowledge Check Neutrons that are not absorbed in fuel are insignificant and do not have any effect on reactor operation. A. True B. False ELO 4.3 Core Physical Changes and the Six-Factor Formula Introduction 34 Rev 1 Core physical design characteristics such as fuel enrichment, fuel temperature, and moderator-to-fuel ratio affect various factors of the sixfactor formula. This section concentrates on the design attributes of the reactor, while the next section focuses on operating parameter changes during power operation, such as power, temperature, poisons, core age, etc. Since keff is the product of these factors, knowledge of these effects is important to the operator for safe operation of the reactor. Design Factors Affecting the Value of the Fast Fission Factor (ε) Reactor design establishes most parameters that affect the value of the fast fission factor during plant operation. Variables such as temperature, pressure, enrichment, or neutron poison concentration have little effect on ε. Reactor design affects ε in the following ways: Fuel atomic density — as fuel atomic density decreases, ε decreases. Fuel pellet diameter — as fuel pellet diameter decreases, ε decreases. — Fuel pellets are encased in a fuel rod; multiple fuel rods are assembled to make a fuel element. ο· Moderator — ε decreases with the ability to slow fast neutrons more rapidly. ο· Enrichment — a higher concentration of uranium-235 atoms results in a very slightly higher fast fission factor. — Impact is relatively small and may change ε from 1.04 for a new core to 1.03, for a depleted core. ο· ο· Design Factors Affecting Resonance Escape Probability (ρ) Moderator-to-fuel ratio, fuel temperature, and fuel enrichment are parameters that affect the value of resonance escape probability. Importantly, these parameter are set by design, but are also affected during plant operation. For example, fuel temperature is affected by power level and moderator-to-fuel ratio is affected by moderator temperature, which is discussed further in the next section. Moderator-to-Fuel Ratio Moderator-to-fuel ratio has a large impact on the value of the resonance escape probability and thermal utilization factor in an operating nuclear reactor. Changing fuel element design or moderator density can modify this ratio. The fuel element design and loading is set by reactor design and is not controlled by the reactor operator. However, moderator density in a pressurized water reactor (PWR) is affected by moderator temperature changes, which the operator can directly control. In the case of the resonance escape probability, as moderator temperature decreases, density increases, neutrons spend less time in the resonance capture energy range, moderator-to-fuel ratio increases, and ρ increases. The figure below shows this relationship. Rev 1 35 Figure: Resonance Escape Probability Versus Moderator-to-Fuel Ratio Fuel Temperature The resonance escape probability varies with changes in fuel temperature. In water moderated, low uranium-235 enrichment reactors, raising the temperature of the fuel will increase the resonance absorption in uranium238 due to the Doppler Effect (broadening of the normally narrow resonance absorption peaks due to thermal motion of nuclei). The increase in resonance absorption decreases the resonance escape probability. Figure: Resonance Escape Probability Change With Fuel Temperature 36 Rev 1 Fuel Enrichment Increasing fuel enrichment (concentration of uranium-235 atoms) in the core will result in a minor increase in resonance escape probability. This is due to the corresponding decrease in uranium-238 concentration, reducing the probability that neutrons will undergo resonance absorption by uranium238 nuclei. Design Factors Affecting Thermal Utilization Factor (f) Several design factors affect the value of the thermal utilization factors. The largest is the moderator-to-fuel ratio and the second is uranium-235 enrichment. Other operating parameter affects are discussed in the next section. Moderator-to-Fuel Ratio Moderator-to-fuel ratio has the largest impact on the value of the resonance escape probability and thermal utilization factor in an operating nuclear reactor. Changing fuel element design or moderator density can modify this ratio. The fuel element design and loading is set by reactor design and is not controlled by the reactor operator. However, moderator density in a PWR is affected by moderator temperature changes, which the operator can directly control. In the case of the thermal utilization factor, as the moderator-to-fuel ratio increases (temperature decrease) thermal utilization decreases, which results from the increased total number of thermal neutrons absorbed specifically by the moderator. Figure: Thermal Utilization Factor Versus Moderator-To-Fuel Ratio Rev 1 37 Uranium-235 Enrichment The amount of enrichment of uranium-235 will affect the thermal utilization factor by increasing the number of thermal neutrons absorbed in the fuel. π= ππ’ππππ ππ π‘βπππππ πππ’π‘ππππ πππ πππππ ππ π‘βπ ππ’ππ ππ’ππππ ππ π‘βπππππ πππ’π‘ππππ πππ πππππ ππ πππ πππππ‘ππ πππ‘ππππππ In an operating nuclear reactor, higher fuel enrichment is used to allow for extended power operations (typically 18 months or longer). This increased enrichment means more thermal neutrons absorbed in the fuel compared to fuel plus all other absorptions, increasing f. Recall that the thermal neutron macroscopic cross-section for absorption for uranium-235 is greater than that for uranium-238. Design Factors Affecting Reproduction Factor (η) Uranium-235 enrichment is the design factor affecting the value of the Reproduction Factor (π). Other operating parameter affects are discussed in the next section. Enrichment The value of η increases with uranium-235 enrichment because there is less uranium-238 in the reactor making it more likely that a neutron absorbed in the fuel will be absorbed by uranium-235 and cause fission. Refer to the equation below. π π−235 ππ π−235 π£ π−235 π = π−235 π−235 π ππ + ππ−238 ππ π−238 Design Factors Affecting Fast Non-Leakage Probability (Lf) The ability for a fast neutron to leak out of a reactor depends on how far the neutron travels as well as its distance from the core boundary. Because of this, beyond the core design, Lf is primarily a function of the moderator density. Because the physical core size is so large for a commercial nuclear reactor (nearly infinite for neutrons), moderator density actually has a very minor effect on the value of Lf. Because of this, Lf is often neglected. Design Factors Affecting Thermal Non-Leakage Probability (Lth) The thermal non-leakage probability is affected by the same parameters, effective core size and moderator density, as the fast non-leakage probability. The effect of core size and moderator density changes is reduced because the distance that a neutron travels in the thermal energy range is much less than that of a fast neutron. 38 Rev 1 As with fast non-leakage probability, this leakage term is often neglected due to the relative infinite size of a commercial nuclear reactor core. Knowledge Check An increase in moderator temperature results in a decrease in all of the factors in a six-factor formula except... A. resonance escape probability (p). B. fast fission factor (ε). C. thermal utilization factor (f). D. fast non-leakage factor (Lf). ELO 4.4 Core Operating Parameter Changes and the Six-Factor Formula Introduction This section focuses on operating parameter changes during power operation, that is power, temperature, poisons, core age, etc., and how they affect the factors in the six-factor formula. In order to control reactor power, a reactor operator must be able to control the thermal neutron population in the core. The operator controls thermal neutron population in the core by controlling the various factors of the six-factor formula. This section explains the following summary table: Figure: Core Parameter Changes Affecting keff - S = Slight Effect Rev 1 39 Core Life Increasing Fast fission — the most significant effect to fast fission. Decreases slightly from depleting uranium-235, reducing a number of fast fissions occurring. (U-235 has a higher cross-section for fast fissions than U-238.) Resonance escape probability — as the core ages, some uranium-238 is converted to plutonium-240, by the following reaction. π½ − 239 238 1 239 π½− 239 239 1 240 π+ π → π→ ππ → ππ’, ππ’ + π → ππ’ 92 0 92 93 94 94 0 94 Uranium-238, which has high resonance absorption cross-section peaks, depletes and plutonium-240 increases. However, plutonium-240 has even higher resonance absorption cross-section peaks than uranium-238 (approximately 30 times higher). The result is an increase in resonance capture over core life or a decrease in resonance escape probability over core life. Thermal utilization — as the core ages, fuel enrichment decreases with the burnup of uranium-235 resulting in a decreasing number of uranium-235 atoms causing a decrease in the value of the thermal utilization factor. Additionally, as the fuel concentration decreases, the moderator-to-fuel ratio increases, and the probability of neutron absorption by the moderator increases. With fewer neutrons available for absorption in the fuel, the thermal utilization factor decreases. Furthermore, soluble boron, control rods, and burnable poisons are used in the nuclear reactor to control the excess amount of reactivity present in the core from fuel loading. Throughout the life of the core, control rods are normally maintained fully withdrawn (except during startup and shutdown) so the thermal utilization factor would not be affected at full power by control rods. However, boron concentration and burnable poison concentrations are reduced to compensate for fuel burnup and fission product poisons over core life. Additionally, the reactor operator can change boron concentration to control reactor power. Lowering the concentration of boron decreases the probability that thermal neutrons will be absorbed by the boron (soluble in the moderator), resulting in an increase to thermal utilization factor. Control rods would have the same affect when used. There is one more affect with increasing core life. As previously described, plutonium-239 builds up over core life from the uranium-238 neutron capture. This results in an increase in fuel concentration, in turn causing a thermal utilization factor increase. 40 Rev 1 The overall effect over core life of these factors may be a slight increase in the thermal utilization factor due to the changing boron concentration in the coolant. Reproduction factor — as the core ages, plutomiun-239 is produced from neutron capture by uranium-238. Although neutron yield per fission for plutomium-239 is slightly higher than for uranium-235, production of plutonium-239 lags the depletion of uranium-235. The result is a slight decrease in the reproduction factor over core life. Non-Leakage factors — no significant changes over core life. keff — decreases without operator action. Moderator Temperature Increasing Fast fission factor — as moderator temperature increases, moderator density decreases, and neutrons take longer to thermalize, causing a greater chance of fast fission. Therefore, ε increases slightly with increasing moderator temperatures. Non-Leakage, resonance escape probability, and thermal utilization factors – these factors combine to provide for the most basic inherent safety feature of PWR thermal reactors. This is the negative moderator temperature coefficient. Much more detail on this is provided later in the course, especially in regards to the effect soluble boron concentration has on the coefficient. For the following explanation, only pure light water as the moderator is considered, with no soluble boron. Non-leakage factors — as moderator temperature increases, density decreases, neutron collisions are further apart, neutrons travel further, and there is a greater chance of leakage. Therefore, the non-leakage probabilities decrease. The opposite is true for a temperature decrease. ο· Moderator-to-fuel ratio — moderator temperature affects density, which affects the moderator-to-fuel ratio. This affects both the resonance escape and thermal utilization factors. Refer to the following figure for the following explanation. ο· Rev 1 41 Figure: keff Versus Moderator-To-Fuel Ratio Water density decreases as temperature increases. At higher temperatures (550°F), the decrease in water density is greater per degree change in temperature than at lower temperatures (120°F), as shown in the figure below. Restated: for the same change in temperature, the change in water density is greater at higher temperatures. Figure: Density of Water Versus Moderator Temperature The change in moderator-to-fuel ratio (Nmod/Nfuel) versus temperature change is proportional to the water density change. Therefore, as moderator temperature increases, the moderator-to-fuel ratio (Nmod/Nfuel) decreases. As previously stated the magnitude of this change is greater at higher temperatures. 42 Rev 1 At power, a nuclear reactor is designed to operate at a tight temperature range (approximately 30°F) and small pressure changes. Significant moderator temperature changes do occur in a reactor plant during heatup to operating temperature; however, the reactor will not be made critical until at normal operating temperatures and pressures. Under moderation PWRs are designed to be under moderated — less than ideal moderation of all neutrons in the core. This condition leads to a negative temperature coefficient, the inherent safety feature as previously mentioned. In an undermoderated reactor, as moderator temperature increases and density decreases (causing the non-leakage factors to decrease), a drop in moderator-to-fuel ratio also occurs causing resonance escape probability to decrease (neutrons travel further, greater chance of resonance capture) and thermal utilization to increase because fewer moderator atoms are available for absorbing thermal neutrons compared to fuel. The effect on resonance escape probability is greater than for thermal utilization. By multiplying each term of six-factor formula, the result is that keff decreases for an increase in moderator temperature. This can be seen on the moderator-to-fuel ratio figure to the left of the keff curve peak. An increase in temperature lowers keff, decreasing the neutron population in the core, resulting in reactor power level decreasing and the temperature increase stopping. This, along with the fuel temperature coefficient, provides for the inherent stability for controlling reactor power. Over moderation In a reactor where the moderator-to-fuel ratio is high, an over moderated condition exists. In this case, on a temperature increase, keff increases. Unlike the under moderated condition, the decrease in resonance escape probability is smaller and the increase to the thermal utilization factor is larger. Refer to the moderator-to-fuel ratio curve. This along with the non-leakage factors causes an increase in keff for a moderator temperature increase. This is referred to as a Positive Moderator Temperature Coefficient. While this condition could exist in a PWR with high soluble boron concentrations, or directly following a reactor refueling, this is not a desirable situation and requires close monitoring and understanding by the operator. Boron Concentration Decreasing or Control Rods Withdrawn Fast fission factor — no effect. Non-leakage factors — no significant effect, rod withdrawal may affect flux shape that could increase the non-leakage factors very slightly. Resonance escape probability — no effect. Rev 1 43 Thermal utilization — concentration of non-fuel neutron absorbing materials decrease, thermal utilization increases. Reproduction factor — no effect. keff — increases from thermal utilization increase. Note Note Effects of control rods and boron described above show that thermal utilization factor is one of factors that an operator can manipulate to control keff in an operating nuclear reactor. Fuel Temperature Increasing Fast fission factor — no effect. Non-leakage factors — no effect. Resonance escape probability — the resonance escape probability varies with changes in fuel temperature. In water-moderated, low uranium-235 enrichment reactors, raising the temperature of the fuel will increase the resonance absorption in uranium-238 due to the Doppler Effect, broadening the normally narrow resonance absorption peaks due to thermal motion of nuclei. The increase in resonance absorption decreases the resonance escape probability. Figure: Resonance Escape Probability Change With Fuel Temperature 44 Rev 1 Thermal utilization — no effect. Reproduction factor — no effect. keff — decreases from the decrease in resonance escape probability. Pressure Increasing PWRs operate in a tightly controlled pressure band. Water is an incompressible fluid as well. Therefore, any moderator density changes are negligible as would be changes to the terms in the six-factor formula. A one (1) degree temperature change is equivalent to 100 pounds per square inch (psi) pressure change. Poison (Fission Products) Increase Poisons have the same effect on keff as boron and control rods because they are all reactivity poisons. Fast fission factor — no effect. Non-leakage factors — no effect. Resonance escape probability — no effect. Thermal utilization — concentration of non-fuel neutron absorbing materials increases, thermal utilization decreases. Reproduction factor — no effect. keff — decreases from thermal utilization decreases. Fuel Enrichment Increase Fuel enrichment is a design issue, something over which the operator has no direct control. Fuel enrichment is included here for comparison with operating parameter changes. Fast fission factor — a higher concentration of uranium-235 atoms results in a very slightly higher fast fission factor. Non-leakage factors — no effect Resonance escape probability — increasing the concentration of uranium235 atoms in the core results in a minor increase in resonance escape probability due to the corresponding decrease in uranium-238 concentration. This results in fewer neutrons being resonance captured by uranium-238 nuclei. Thermal utilization — concentration of fuel neutron absorbing materials increases, thermal utilization increases. Rev 1 45 Reproduction factor – increases with uranium-235 enrichment increases because of less uranium-238 in the reactor making it more likely that a neutron absorbed in the fuel will be absorbed by uranium-235 and cause fission. Refer to the equation below. π= π π−235 ππ π−235 π£ π−235 ππ−235 ππ π−235 + ππ−238 ππ π−238 keff — increases from ρ f π. Knowledge Check In an under moderated reactor, if the temperature of the moderator is increased, f will ________ and p will _________. A. increase; decrease B. increase; remain the same C. decrease; increase D. decrease; remain the same TLO 4 Summary During this lesson, you learned about neutron life cycle and reactor control: terms associated with the neutron life cycle, describing the terms in the sixfactor formula, how the physical design of the reactor core affects each term in the six-factor formula, and how a change to plant parameters affects each part of the six-factor formula. The listing below provides a summary of sections in this TLO. 1. Define the following terms associated with the neutron life cycle: ο· ο· ο· ο· 46 Infinite multiplication factor (k∞) ratio of number of neutrons produced by fission in one generation to the number of neutrons lost through absorption in the preceding generation. Infinitely sized reactor, no neutron leakage considered. Effective multiplication factor, keff, ratio of number of neutrons produced by fission in one generation to the number of neutrons lost through absorption and leakage in the preceding generation. Finite sized reactor. Critical is the condition where the neutron chain reaction is selfsustaining and the neutron population is neither increasing nor decreasing. keff = 1. Subcritical is the condition in which the neutron population is decreasing each generation. keff < 1. Rev 1 ο· Supercritical is the condition in which the neutron population is increasing each generation. keff > 1. 2. Describe each term in the six-factor formula: ο· ππππ = ππΏπ ππΏπ‘β ππ. Each of the six factors is defined below. ππ’ππππ ππ πππ π‘ πππ’π‘ππππ πππππ’πππ ππ¦ πππ πππ π ππππ ο· π = ππ’ππππ ππ πππ π‘ πππ’π‘ππππ πππππ’πππ ππ¦ π‘βπππππ πππ π ππππ ο· πΏπ = ο· π = ππ’ππππ ππ πππ π‘ πππ’π‘ππππ π‘βππ‘ π π‘πππ‘ π‘π π πππ€ πππ€π ο· ππ’ππππ ππ πππ π‘ πππ’π‘ππππ π‘βππ‘ ππ πππ‘ ππππ ππππ πππππ‘ππ ππ’ππππ ππ πππ π‘ πππ’π‘ππππ πππππ’πππ ππ¦ πππ πππ π ππππ ππ’ππππ ππ πππ’π‘ππππ π‘βππ‘ ππππβ π‘βπππππ ππππππ¦ πΏπ‘β = ο· π= ο· π= ππ’ππππ ππ π‘βπππππ πππ’π‘ππππ π‘βππ‘ ππ πππ‘ ππππ ππππ πππππ‘ππ ππ’ππππ ππ πππ’π‘ππππ π‘βππ‘ ππππβ π‘βπππππ ππππππππ ππ’ππππ ππ π‘βπππππ πππ’π‘ππππ πππ πππππ ππ π‘βπ ππ’ππ ππ’ππππ ππ π‘βπππππ πππ’π‘ππππ πππ πππππ ππ πππ πππππ‘ππ πππ‘ππππππ ππ’ππππ ππ πππ π‘ πππ’π‘ππππ πππππ’πππ ππ¦ π‘βπππππ πππ π πππ ππ’ππππ ππ π‘βπππππ πππ’π‘ππππ πππ πππππ ππ π‘βπ ππ’ππ 3. Explain how the physical design of the reactor core affects each of the terms in the six-factor formula. ο· Design factors affecting the value of the fast fission factor include the following: — Fuel atomic density — Fuel pellet diameter — Moderator — Enrichment ο· Design factors affecting resonance escape probability include the following: — Moderator-to-fuel ratio — Fuel temperature — Fuel enrichment ο· Design factors affecting thermal utilization factor (f) — Moderator-to-fuel ratio — Uranium-235 Enrichment ο· Design factors affecting reproduction factor (η) — Enrichment ο· Design factors affecting fast non-leaking probability (Lf) ο· Design factors affecting thermal non-leaking probability (Lth) 4. Physical core changes most directly from the operator produce the following changes to the Six-Factor Formula: Rev 1 47 Figure: Core Operating Changes and the Six-Factor Formula ο· ο· ο· ο· Fast fission factor and reproduction factor are primarily determined by reactor design and remain essentially constant in the temperature range of an operating nuclear reactor. Moderator-to-fuel ratio has the largest impact on the values of the resonance escape probability and thermal utilization factor in an operating nuclear reactor. — Nuclear reactor operator can control reactor moderator temperature, affecting density and the moderator-fuel ratio. This affects the non-leakage terms, the thermal utilization factor, and the resonance escape probability. In or with an under-moderated reactor (what we want), as moderator temperature increases and density decreases, moderator-to-fuel ratio decreases with an accompanying insertion of negative reactivity. This provides some inherent stability for controlling reactor power. In or with an over-moderated reactor, positive reactivity is inserted as the temperature increases, which is not a desirable condition for power control in a PWR. Now that you have completed this lesson, you should be able to do the following: 1. Define the following terms associated with the neutron life cycle: a. Infinite multiplication factor (k∞) b. Effective multiplication factor (keff) c. Subcritical d. Critical e. Supercritical 2. Describe each term in the six-factor formula using the ratio of the number of neutrons present at different points in the neutron life cycle. 3. Explain how the physical design of the reactor core affects each of the terms in the six-factor formula. 48 Rev 1 4. Explain how a change to plant operating parameters affects each of the factors of the six-factor formula. Neutron Life Cycle Summary This module presented the neutron life cycle because nuclear fission generates or is controlled by the way atoms splits from neutrons combined with the neutrons respective thermalization by things such as moderators in the reactor to reduce the energy level of a neutron from its birth energy to the energy level of the surrounding atoms. The addition of chemical elements such as Uranium-235 or Plutonium-239 to neutrons and the respective results of each, including prompt and delayed neutrons and their effects. When nuclear fission occurs slowly, the energy is used to produce electricity. TLO 1 presented how thermalization works with a moderator to reduce the velocity of the fission neutrons, average logarithmic energy decrement, and macroscopic slowing down power and moderating ratio. TLO 2 presented prompt and delayed neutrons, their origin and production, the approximate fraction of neutrons born delayed from the fission of Uranium-235 and Plutonium-239, the lifetime and generation times of both prompt and delayed neutrons, and the effects of delayed neutrons on reactor control. TLO 3 presented neutron flux, the average energy that produces prompt neutrons, the shape of the neutron energy spectrum in a thermal reactor, and the reason for the neutron energy spectrum’s shape for a thermal reactor, including variable(s) that have the most effect on thermal neutron velocity TLO 4 presented neutron life cycle and reactor control: terms associated with the neutron life cycle, describing the terms in the six- factor formula, how the physical design of the reactor core affects each term in the sixfactor formula, and how a change to plant parameters affects each part of the six-factor formula. Summary Now that you have completed this module, you should be able to demonstrate mastery of this topic by passing a written exam with a grade of 80 percent or higher on the following TLOs: 1. Describe the process of neutron moderation in a nuclear reactor and the characteristics of desirable moderators. 2. Describe the production of prompt and delayed neutrons from fission, and how these neutrons affect nuclear reactor control. 3. Describe the neutron flux spectrum in thermal reactors. 4. Describe the neutron life cycle throughout the lifetime of a thermal reactor and how it is affected by core design and variations in operating parameters. Rev 1 49