Spatially nonreciprocal Bragg gratings based on surface plasmons: Supplementary Online Material In this appendix we study a generic Bragg grating using coupled mode theory and elucidate the conditions required for nonreciprocal operation. Fig. S1 shows a sketch of a periodic dielectric slab grating. Fig. S1: Contra-directional coupling in a Bragg grating. The complex permittivity varies periodically along z with period of Λ. Assuming coupling between the two identical counter-propagating modes, the net electric field in the grating is expressed as E(x,y,z)=U(x,y)[A(z) e-jβBz +B(z) e+jβBz], where U(x,y) is the normalized transverse mode distribution, A(z) and B(z) are respectively the amplitudes of the forward and backward propagating modes, and βB=π/Λ is the Bragg constant. The coupled mode equation for the Bragg grating is given as: (A1) dA j l B j A dz dB j l A j B dz where δ=β-βB is the detuning parameter. κ±l is the coupling coefficient which is defined as: k 2 l ( x, y ) U ( x, y ) dxdy l 0 2 2 U ( x, y ) dxdy 2 (A2) where k0=2π/λ0 is the free space propagation constant, β=2π/λ is the propagation constant in the grating and Δε±l is the ±lth Fourier component of the periodic permittivity, Ref[1]. The transmission matrix for the coupling due to the ±lth Fourier component is derived from the coupled equations in Eq.A1. cosh( L) j sinh( L) j l sinh( L) A( L ) A(0) T T l B ( L) B(0) j sinh( L) cosh( L) j sinh( L) (A3) Where σ2=κlκ-l-δ2. Using the transmission matrix given above, the reflectance and transmittance from the right and left sides are obtained as: T Rr 21 T11 Rl Tr 2 T12 T11 1 T11 (A4) 2 2 T T T T Tl 11 22 12 21 T11 2 It can be shown that T11T22-T12T21=1, thus Tr=Tl or the transmittance is always reciprocal. However only if T21=T12 will the reflectance be reciprocal. It is obvious from the transmission matrix in Eq.A3 that we need κl=κ-l* in order to have T21=T12 Fourier analysis shows that the coupling coefficients for a Bragg grating with modulation of only the real permittivity always satisfy κl=κ-l*. Therefore reflectance will always be reciprocal for these gratings. However if there is significant modulation of imaginary permittivity (gain/loss) then the coupling coefficient will not be symmetric and nonreciprocal reflectance will occur. Ideal non-reciprocity occurs when κl≠0 and κ-l=0 (or vice versa). This requires that the refractive index of the grating have a form similar to Eq.1, which implies that the modulation of the real and imaginary components of refractive index must be equal (Δn= Δk), and that there must be an exact 90˚ phase difference between them. Using the Hamiltonian operator, we demonstrate that the realization of these 2 conditions corresponds to the breaking threshold of PT symmetry. The Hamiltonian of a Bragg grating is defined using the coupled equations in Eq.A1 as: j A d A H H dz B B j l j l j (A5) The eigenvalues of the Hamiltonian are obtained as λ = ±σ = ± (κl κ-l - δ2)1/2. We will explore the eigenvalues at the Bragg wavelength where δ=0 and eigenvalues simplify to λ = ± (κl κ-l*)1/2 If κl=κ-l* (i.e. for a grating with a real modulation of refractive index only), the eigenvalues of the Hamiltonian will be real 𝜆 = ±|𝜅𝑙 |. This state corresponds to unbroken PT symmetry. If one of κl or κ-l is zero, then the eigenvalues coalesce to λ=0 which corresponds to the threshold for PT symmetry breaking. This state is also referred to as a PT symmetry phase transition or exceptional point. At this state ideal non-reciprocity is attainable. If κl≠κ-l* the eigenvalues form a complex conjugate pair which corresponds to a PT symmetry broken state. The coupling coefficient will not be symmetric, which in turn causes asymmetric reflectance, but it is not ideal non-reciprocity which occurs precisely at the breaking threshold. References: [1]. L. A. Coldren, Scott. W. Corzine, “Diode lasers and Photonic Integrated Circuits”, (John Wiley and Sons, Inc, 1995).