09.03.2007 PARTNER SEARCH FOR FP7 PROJECT ENV.2007.1.2.1.1. Contact person dr Nataša Todorović e-mail: zikic@im.ns.ac.yu The Nuclear Physics Laboratory, member of Department of Physics, Faculty of Sciences, University of Novi Sad Serbia, have a long-term experience of indoor radon measurements. The Laboratory is the national focal point for European radon mapping by the European Commission Joint Research Centre (http://radonmapping.jrc.it). The list of present equipment for radon measurements is given below: 1. Alpha-ray spectrometer dedicated to the measurement of low levels of radon, and other alpha-ray emitting isotopes, in different gaseous and liquid media. Canisters with charcoal for passive adsorption of radon from the air, the gamma-ray spectroscopy of which, providing proper calibration, yields the concentration of radon in the air. 2. Two hyper pure HPGe germanium spectrometers of nominal efficiencies of 36% shielded by 12 cm thick lead shield with the Canberra four input Multiport data acquisition system. 3. The big low-background iron chamber of a useful volume of 1 m3, with 25 cm thick walls, made out of pre-WWII iron (free of 60Co). The chamber accommodates another HPGe detector actively shielded with a large (9”x9”) NaI(Tl) annulus acting also as a Compton suppressor. 4. Shallow underground laboratory. It is situated at the depth equivalent to 30 meters of water, what reduces the cosmic-ray muon flux 4.5 times as compared to the flux at the surface. It has an active area of about 60m2 and is completely lined with aluminum foil 1 mm thick, which is hermetically sealed against the penetration of radon from the surrounding soil and concrete used for construction. The laboratory is continuously ventilated with fresh air which is filtered through the battery of coarse and fine charcoal active filters in such a way that an overpressure of some 2 mbar is maintained over the atmospheric pressure. This is aimed at keeping the radon from eventually leaking into the laboratory. The levels of radon lower than 10 Bq/m3 are routinely achieved. The pressure-buffer corridor with double air-tight doors keeps the laboratory space radio pure. Sampling strategy: Indoor radon activity concentration in air has been measured at the whole area of the province Vojvodina. Special attention has been paid to rural regions of 45 municipalities and type of dwellings, characteristic for Vojvodina region. The main aim of the present study was to exploit the critical group for radon exposure. Thus the mean values obtained for the whole region should be most probably considered as upper limits at the evaluation of the radon doses. The Southern area of the country is geologically very different from the Danube Basin and probably will be faced with the quite different radon build-up problems. Measurement technique Detector type Track-etch detectors (CR-39) Measurements time (days) 90 Season Winter Measurement location Living room Measurement time (units in days) Detector type Mean Std. Dev. Min. Max. Track-etch detectors 90 NA NA NA Statistics of the measurements 3 Measurements statistics (units in Bq/m ) Measurements Mean Geo. Mean Std. Dev. Min. Max. 968 144 104.6 120 2 893 Estimated mean annual radon levels in dwellings of the Province of Vojvodina 3 Mean % of dwellings above 200 Bq/m and % of dwellings above 3 (Bq/m ) 144 below 400 Bq/m 18 3 3 400 Bq/m 4 Maps: Indoor radon activity concentration in air has been measured at the whole area of the province Vojvodina (on 1000 locations) by plastic track detectors CR-39. On the base of the obtained results, the average indoor activity concentrations of 222Rn for individual municipalities and for the whole province of Vojvodina were estimated. In Vojvodina the average indoor radon activity concentration yields 144 Bq/m3 . Distribution of indoor radon activity concentrations measured by CR-39 during the period December 2002 – March 2003 Radon map of Vojvodina. Numbers given along the names of municipalities indicate geometric mean radon concentration in Bqm-3. The method of the adsorption on activated charcoal canister was applied in some measurements of radon activity concentrations. The canister gamma activity (the activity of 214Bi and 214Pb radon daughters) was measured by means of high resolution germanium and NaI(Tl) scintillation spectrometers. The efficiency of the detectors was determined using the EPA 226Ra Reference source. The canisters were exposed for two days. The typical time between the end of the exposion and the beginning of the measurement was about two hours. Gamma spectrometric measurements were performed with high resolution HPGe gamma spectrometer with nominal efficiency 22%, was placed in another schielding chamber with iron walls 25 cm thick. In order to achieve 5% statistical accuracy at 100 Bq/m3 the time of measurement was usually 1 hour. In our measuring chamber the radon levels are very low (less than 5Bq/m3) so radon fluctuations could not affect the results of most measurements. On Fig. results of measurements of indoor radon concentrations in Novi Sad flats by charcoal cannisters are presented. The results of the statistical analysis of about 180 measurements are listed in Table. Frequency distribution of radon activity concentrations in Novi Sad flats during period 1992-2003 Maximum (Amax), minimum (Amin) and average indoor radon activity concentration Aav A in Novi Sad flats radionuclide 222 Rn Amax [Bq/m3] 391 Amin [Bq/m3] 2 Aav [Bq/m3] 50 A [Bq/m3] 69 The mean value of indoor radon activity concentration obtained by charcoal canisters is (50 ± 69) Bq/m3. Only 5 % of the results exceed the 200 Bq/m3 value accepted as an intervention level in Serbia. The highest results are obtained for flats on ground level. The owners of this flats and houses were advised how to solve the radon build-up problem. The lognormal distribution obtained proves the random nature of the radon build-up in the flats investigated. The results are above the expectations for the low-land districts and show that dominant sampling in new city flats can seriously underestimate the radon buildup problem. Selected References: S. Forkapić, I. Bikit, J. Slivka, Lj. Čonkic, M. Vesković, N. Todorović, E. Varga, D. Mrđa and E. Hulber (2006) INDOOR RADON IN RURAL DWELLINGS OF THESOUTH-PANNONIAN REGION, Radiation Protection Dosimetry (2006), 1 of 6 doi:10.1093/rpd/ncl156 Curcic, S., I. Bikit, Lj. Conkic, M. Veskovic, J. Slivka, E. Varga, N. Todorovic, D. th Mrdja (2004). The first radon map of Vojvodina. In: Proceedings of the 11 International Congress of the International Radiation Protection Association, 23-28 May 2004, Madrid, Spain (paper 6a11 published on CD). • Curcic S.M., I. Bikit, J. Slivka, M.J. Veskovic, Lj. U. Conkic, E. Varga (2003). Radioecological problems in home building in the city of Novi Sad. In: Proceedings th of the 6 International Symposium &Exhibition on Environmental Contamination in Central and Eastern Europe and the Commonwealth of Independent States, 1-4 September 2003, Prague, Czech Republic (Book of Abstracts p.138, published on CD). • Curcic, S., I. Bikit, J. Slivka, Lj. Conkic, M. Veskovic, E. Varga, N. Zikic-Todorovic, D. Mrdja (2003). The first radon map of Vojvodina. In: Proceedings of the XXII Symposium of Yugoslav Radiation Protection Association, Petrovac, Serbia and Montenegro, pp. 195-198. Biography of the key personnel and the staff Key personnel: Dr. Istvan Bikit is a Professor of nuclear physics at the Faculty of Sciences in Novi Sad. He obtained his PhD form the University of Novi Sad in 1976. His international experiences includes visiting positions at Sussex University (Brighton, UK), ICTP (Trieste, Italy), Laue-Langevin Institute (Grenoble, France), NIST (Geithersburg, US), and Institute of Surface Chemistry and Isotopes (Budapest, Hungary). He has led national and international projects in fundamental and applied nuclear physics research in continuity from 1981 onwards, including the bilateral project with US “Improvements on the determination of low-levels of gamma radioactivity” (JF-847 NIST, 1988-90). He was the Dean of the Faculty of Sciences and is the Director of the Department of Physics, University of Novi Sad. His research fields of interest are: nuclear structure, low background gamma spectroscopy, physics of rare nuclear events and radioecology. Dr. Miroslav Veskovic is Professor of nuclear, particle and medical physics at the Faculty of Sciences in Novi Sad. He received his PhD degree at the University of Novi Sad in 1989. He was a research fellow at the Sussex University in 1986-87, Oak Ridge National Laboratory in 1989, CERN in 1991-92, and a visiting professor at Oxford University for two years, from 1994 to 1996. Within the Faculty of Sciences in Novi Sad he has served as the Head of the Nuclear Physics Group (1996-2000) and the Head of the Department of Physics (2000-2002). He served as the vice-Rector of the University of Novi Sad in charge of research and development, and currently serves as the Dean of the Faculty of Sciences. His research interests are low temperature nuclear orientations, nuclear structure, nuclear spectroscopy, physics of rare nuclear events, low background gamma spectroscopy, environmental protection, radioecology, and medical physics. Dr. Ivan Aničin is a Professor of nuclear physics at the Faculty of Physics of the University of Belgrade. His PHD degree he obtained in 1973, from the University of Belgrade. His scientific interests are concentrated mainly in the field of different branches of nuclear spectroscopy, pure and applied. In particular, he specialized in angular correlations of nuclear radiations, and later on in low-background studies of rare nuclear and particle processes. He also participates in the CMS collaboration at CERN, Geneva. He has spent two years in England, France and Germany, collaborating with different researchers in the field of nuclear physics. Dr. Jaroslav Slivka is a Professor of nuclear physics at the Faculty of Sciences in Novi Sad. He obtained his PhD form at the University of Novi Sad in 1986. He was a research fellow at the Institute of Physics in Zurich University in 1982-1984 working in the field of Moessbauer spectroscopy. His recent research interests are nuclear structure, physics of rare nuclear events, low background gamma spectroscopy and radioecology. Dr. Miodrag Krmar is a Professor of nuclear physics at the Faculty of Sciences in Novi Sad. He obtained his PhD form at the University of Novi Sad in 1996. As a research fellow he joint two times the JINR Dubna (Moscow) working on nuclear structure problems by means of nuclear orientation techniques. His research interests are nuclear structure, physics of rare nuclear events, low background gamma spectroscopy, radioecology and medicine physics. He is a member of American Society of Physicist in Medicine. Dr Nataša Todorović Dr Tijana Prodanović Mr Dušan Mrđa Mr Sofija Forkapić