Palaiseau - FRANCE Spatio-Temporal Chirped Pulse Amplification for Avoiding Spectral Modifications in UltraShort Petawatt Lasers C. Radier1,2, F. Giambruno1,3, C. Simon-Boisson2, V. Moro2, G. Chériaux1 1 LOA, Chemin de la Hunière, 91761 Palaiseau Cedex, France 2 TOSA-DSL, 2 Avenue Gay Lussac, 78995 Elancourt, France 3 ILE, CNRS, Ecole Polytechnique, ENSTA, Institut d’optique, 91761 Palaiseau Cedex, France christophe.radier@fr.thalesgroup.com Context (1/2) • Generation of multi-tens of joules energy and several tens of femtoseconds duration pulses leading to petawatt peak power levels • Extremely high peak power pulses (10 PW) : => Vulcan laser 300 J / 30 fs (OPCPA) in LBO and KDP => Apollon-10P 150 J / 15 fs (CPA) in Ti:Sa • Management of the spectral energy distribution in terms of shape and bandwidth during their amplification process : => Temporal profile adapted to the high intensity interaction http://loa.ensta.fr/ UMR 7639 Context (2/2) • OPCPA configuration in LBO / BBO / KDP : Control of the spectrum (width and shape) by the angles in the non-linear crystal and by the pump (temporal profile and intensity) • CPA configuration in Ti:Sa : Amplification of temporally chirped pulses => Gain narrowing (inhomogeneous spectral gain ) 2,40 0,90 Normalized spectral gain (u.a.) Normalized spectral intensity (u.a.) 1,00 0,80 0,70 0,60 0,50 0,40 0,30 0,20 0,10 0,00 650 700 750 800 850 Wavelength (nm ) 900 950 Input : Δλ½ = 85 nm 2,20 Pass 6 : Δλ½ = 62 nm 2,00 1,80 1,60 1,40 1,20 650 700 750 800 850 900 950 Wavelength (nm ) Frantz et Nodvik model : « Gain regime : J0(t) ~ Jsat / 1000 & G = 100 » http://loa.ensta.fr/ UMR 7639 Context (2/2) • OPCPA configuration in LBO / BBO / KDP : Control of the spectrum (width and shape) by the angles in the non-linear crystal and by the pump (temporal profile and intensity) • CPA configuration in Ti:Sa : Amplification of temporally chirped pulses = Gain shifting (amplification saturation ) 0,90 Normalized spectral gain (u.a.) Normalized spectral intensity (u.a.) 1,00 0,80 0,70 0,60 0,50 0,40 0,30 0,20 0,10 0,00 650 700 750 800 850 Wavelength (nm ) 900 950 1,90 Input : λc = 794 nm 1,70 Pass 6 : λc = 808 nm 1,50 1,30 1,10 0,90 -1500 -1000 -500 0 500 1000 1500 Duration (ps) Wavelength (nm ) Frantz et Nodvik model : « Saturation regime : J0(t) ~ Jsat / G = 1,8 » http://loa.ensta.fr/ UMR 7639 Existing solutions • Different relevant active and passive solutions to overcome the gain narrowing issue (mJ-level pulses in the 10 fs regime) Acousto-optic programmable dispersive filter1 Multilayer Gain Narrowing compensators2,3,4 Negatively and Positively Chirped Pulsed Amplification5 • No solution to suppress the spectral shape modifications due to saturation effects at moderate or high level energy (> 1J). 1. 2. 3. 4. 5. F. Verluise et al., “Amplitude and phase control of ultrashort pulses by use of an acousto-optic programmable dispersive filter: pulse compression and shaping”, Opt. Lett. 25, 575–577 (2000). A. Amani Eilanlou et al., “Direct amplification of terawatt sub-10-fs pulses in a CPA system of Ti:sapphire laser,” Opt. Express 16, 13431–13438 (2008). H. Takada, et al., “High-repetition-rate 12fs pulse amplification by a Ti:sapphire regenerative amplifier system,” Opt. Lett. 31, 1145–1147 (2006). L. Antonucci, et al., “14 fs high temporal quality injector for ultra-high intensity laser,” Opt. Commun. 282, 1374–1379 (2009). M. P. Kalashnikov et al., “Suppression of gain narrowing in multi-TW lasers with negatively and positively chirped pulse amplification,” Appl. Phys. B 81, 1059 (2005). http://loa.ensta.fr/ UMR 7639 Spatio-Temporal Chirped Pulse Amplification (STCPA) (1/2) • Principle : Combination of temporal and spatial dispersion enable amplified spectra to be unaffected by saturation effect. i.e. spatially spreading spectral components to separately amplify them and thus deleting the gain competition http://loa.ensta.fr/ UMR 7639 Spatio-Temporal Chirped Pulse Amplification (STCPA) (1/2) • Principle : Combination of temporal and spatial dispersion enable amplified spectra to be unaffected by saturation effect. Ti:Sa Crystal Pump Beam IR Beam Classical CPA scheme Oscillator http://loa.ensta.fr/ Stretcher Power amplifier Compressor UMR 7639 Spatio-Temporal Chirped Pulse Amplification (STCPA) (1/2) • Principle : Combination of temporal and spatial dispersion enable amplified spectra to be unaffected by saturation effect. Ti:Sa Crystal Pump Beam IR Beam STCPA scheme Oscillator Spatial spreading Stretcher Spatial compression Power amplifier Compressor Gain zone shape adaptation http://loa.ensta.fr/ UMR 7639 Spatio-Temporal Chirped Pulse Amplification (STCPA) (2/2) • Advantages : No spectral shifting while preserving energy extraction in saturation regime i.e. saturation effect is equally distributed on all the spectral range instead of only the infrared edge. • Conditions : Input pulse has to be collimated Spatial spreading law has to be inverse of that of spatial compression Pump beam has to be matched to the oblong seeded beam • Inconvenient : Gain narrowing not avoided in this configuration http://loa.ensta.fr/ UMR 7639 Experiment Set Up Frequency doubled Nd:YVO4 3,7 W Ti:Sa Oscillator 3,8 nJ / 80 MHz http://loa.ensta.fr/ UMR 7639 Experiment Set Up Frequency doubled Nd:YVO4 3,7 W Öffner triplet Stretcher 250 ps http://loa.ensta.fr/ Ti:Sa Oscillator 3,8 nJ / 80 MHz UMR 7639 Experiment Set Up Frequency doubled Nd:YVO4 1,5 mJ 1 kHz 3,7 W Regenerative Amplifier 7,1 mJ / 1 kHz Öffner triplet Stretcher 250 ps Ti:Sa Oscillator 3,8 nJ / 80 MHz Q-switched Nd:YLF http://loa.ensta.fr/ UMR 7639 Experiment Set Up Frequency doubled Nd:YVO4 500 µJ 1 kHz + Birefringent Plate 3,7 W Regenerative Amplifier 7,1 mJ / 1 kHz Öffner triplet Stretcher 250 ps Ti:Sa Oscillator 3,8 nJ / 80 MHz Q-switched Nd:YLF http://loa.ensta.fr/ UMR 7639 Experiment Set Up Cylindric lenses 180 mJ / 10 Hz LaK8 Prisms Nd:YAG Multipass amplifier 6 passes Ti:Sa Absorption : 90% Ø = 15 mm Output 40 µJ 10 Hz Pockels Cell + Birefringent Plate 500 µJ 1 kHz Regenerative Amplifier 7,1 mJ / 1 kHz Frequency doubled Nd:YVO4 3,7 W Öffner triplet Stretcher 250 ps Ti:Sa Oscillator 3,8 nJ / 80 MHz Q-switched Nd:YLF http://loa.ensta.fr/ UMR 7639 Experiment Set Up Cylindric lenses 180 mJ / 10 Hz LaK8 Prisms Output 40 µJ 10 Hz Multipass amplifier 6 passes Ti:Sa Absorption : 90% Ø = 15 mm IR Beam Before Prisms Øx,y,FWHM = 1900 µm Nd:YAG IR Beam After Prisms Øx,FWHM = 3000 µm Øy,FWHM = 1900 µm Aspect Ratio of 1,6 http://loa.ensta.fr/ UMR 7639 Experiment Set Up Cylindric lenses 180 mJ / 10 Hz LaK8 Prisms Output 40 µJ 10 Hz Nd:YAG Multipass amplifier 6 passes Ti:Sa Absorption : 90% Ø = 15 mm IR Beam After Prisms Wavelength spreading 19 nm/mm Øx,FWHM = 3000 µm Øy,FWHM = 1900 µm http://loa.ensta.fr/ UMR 7639 Experiment Set Up Cylindric lenses 180 mJ / 10 Hz LaK8 Prisms Output 40 µJ 10 Hz Øx,FWHM = 4000 µm Øy,FWHM = 600 µm Left Side http://loa.ensta.fr/ Nd:YAG Multipass amplifier 6 passes Ti:Sa Absorption : 90% Ø = 15 mm Øx,y,FWHM = 10 mm Output Beam Pump Øx,FWHM = 4000 µm Øy,FWHM = 600 µm Right Side UMR 7639 Experiment Set Up Cylindric lenses 180 mJ / 10 Hz LaK8 Prisms Output 28 mJ ~ 1,8 J/cm² Nd:YAG Multipass amplifier 6 passes Ti:Sa Absorption : 90% Ø = 15 mm 40 µJ 10 Hz FFT Calculation 1,00E+00 0,8 0,6 0,4 0,2 Normalized Intensity (a.u.) 1,0 Normalized Intensity (a.u.) Normalized Intensity (a.u.) 1,0 0,8 0,6 0,4 0,2 0,0 745 770 795 820 845 Wavelength (nm) Simulation CPA http://loa.ensta.fr/ 870 1,00E-02 1,00E-03 1,00E-04 1,00E-05 0,0 720 1,00E-01 720 745 770 795 820 845 Wavelength (nm) Experiment STCPA 870 -100 -50 0 Duration (fs) UMR 7639 50 100 Experiment Set Up Cylindric lenses 180 mJ / 10 Hz LaK8 Prisms Output 28 mJ ~ 1,8 J/cm² Nd:YAG Multipass amplifier 6 passes 40 µJ 10 Hz Ti:Sa Absorption : 90% Ø = 15 mm Near field Far field No angular and transverse chirp http://loa.ensta.fr/ UMR 7639 Conclusion • First amplification scheme in Ti:Sa using a combination of spatial and temporal chirp • STCPA concept avoids effects of saturation / enables a control of the amplified spectrum at high energy • Using appropriate chirp tool : output beam free of angular and transverse chirp • Fully relevant technique for obtaining very intense and short laser pulses (energy in excess of 10’s of Joules) with good temporal quality http://loa.ensta.fr/ UMR 7639 Thank you ! http://loa.ensta.fr/ UMR 7639