10 fs laser chain based on optical parametric chirped pulse amplification Lourdes Patricia Ramirez Equipe Lasers Solides et Applications Laboratoire Charles Fabry de l’Institut d’Optique (LCFIO), Palaiseau, France Frédéric Druon Directeur de thèse Journées Scientifiques de l’EDOM March 8, 2011 1 Outline • Motivation: Front end of the Apollon laser • Optical parametric chirped pulse amplification (OPCPA) • Seed source for OPCPA Ultrashort approach Direct XPW approach • Summary and future work Journées Scientifiques de l’EDOM March 8, 2011 2 Front end of the Apollon 10 PW laser Ultrashort seed source @ 800 nm High contrast, CEP stable, sub-10 fs, >100 µJ, 1 kHz Noncollinear Optical Parametric Chirped Pulse Amplification stages NOPCPA (BBO or LBO) Optical synchronization <10 fs, 100 mJ, @800 nm, 10-100 Hz 10 TW! HEC-DPSSL pumped high rep-rate amplifiers (Yb:KGW, YAG, CaF2) 2 J @ 1030 nm, 10-100 Hz SHG: ps-ns 1 J @ 515 nm 10-100 Hz Pump source @ 515 nm Applications: high harmonic generation, attosecond physics, particle acceleration, plasma physics, high energy physics experiments Journées Scientifiques de l’EDOM March 8, 2011 3 Optical parametric amplification (OPA) Generation pump Nonlinear Crystal X(2) p s i Amplification pump signal Nonlinear Crystal X(2) • Extremely broad amplification bandwidth signal • High gain per single pass • High quantum efficiency idler • Low thermal effects • Reduced amplified spontaneous emission – high energy and intensity contrast ratio residual pump pulses • Scalability to high amplified signal energies idler Journées Scientifiques de l’EDOM March 8, 2011 4 Chirped pulse amplification (CPA) Journées Scientifiques de l’EDOM March 8, 2011 5 OPA + CPA = OPCPA Replace with nonlinear crystals e.g. BBO, LBO, KDP Journées Scientifiques de l’EDOM March 8, 2011 6 Front end of the Apollon 10 PW laser Ultrashort seed source @ 800 nm High contrast, CEP stable, sub-10 fs, >100 µJ, 1 kHz Noncollinear Optical Parametric Chirped Pulse Amplification stages NOPCPA (BBO or LBO) Optical synchronization <10 fs, 100 mJ, @800 nm, 10-100 Hz 10 TW! HEC-DPSSL pumped high rep-rate amplifiers (Yb:KGW, YAG, CaF2) 2 J @ 1030 nm, 10-100 Hz SHG: ps-ns 1 J @ 515 nm 10-100 Hz Pump source @ 515 nm Journées Scientifiques de l’EDOM March 8, 2011 7 Ultrashort seed source • Sub-10 fs , >100 µJ, 1 kHz, CEP stable, high contrast ratio at 800 nm • 2 approaches: Commercial ultrashort Ti:Sa system 25 fs, 1.5 mJ, 1 kHz, CEP stable, CR ~ 108 Ultrashort approach: 5 fs Hollow core fiber (HCF) pulse compression Cross polarized wave generation (XPW) 5 fs, 100 µJ, CEP preserving, CR ~ 1010 Main disadvantages: low efficiency - Compression in between two stages Journées Scientifiques de l’EDOM March 8, 2011 Direct XPW: Sub-10 fs approach Spectral broadening and contrast enhancement via cross polarized wave generation only < 10 fs, 200-300 µJ, CEP preserving, CR ~ 1010 Advantages: higher efficiency - Single stage for broadening and contrast enhancement - Simple and compact setup 8 Ultrashort approach: hollow fiber compression 1.4mJ, 25fs >850 µJ >750 µJ Pulse compression: 25 fs to 4.4 fs Spectral broadening in the HCF: 60 nm to 250 nm 25 1.0 1.0 HCF 250µm diam, 1m long, 1.3bar Ne: ----Ein=1.3 mJ (~48nm) ----Eout=0.8mJ (~250nm) 0.8 60nm 250 nm 0.4 20 0.6 0.4 15 0.2 0.2 0.0 0.0 500 Phase (rad) 0.6 Laser HCF Intensity (a.u.) Intensity (a.u.) 0.8 10 600 700 800 Wavelength (nm) Journées Scientifiques de l’EDOM March 8, 2011 900 1000 -30 -20 -10 0 10 20 30 Time (fs) 9 Cross polarized wave generation (XPW) XPW is based on a degenerated four-wave mixing process governed by the anisotropy of the real part of a crystal’s third-order nonlinearity tensor. I XPW (t ) I L (t ) 3 χ(3) Glan 1 BaF2 Glan 2 Main features: - Contrast enhancement: depends on the polarizer exctinction ratio (105) t 3 - Temporal pulse shortening: - Spectral cleaning and broadening 3 Journées Scientifiques de l’EDOM March 8, 2011 10 Ultrashort approach: HCF + XPW ~550μJ, 5fs ~80 μJ, 5fs ~100μJ Energy/Spectrum FROG 3ω/f-2f Spectral cleaning with XPW: 250 nm to 200 nm Compression: 5 fs 60 1.0 50 0.8 XPW HCF 30 0.4 20 0.2 10 -20 -10 0 Time (fs) Journées Scientifiques de l’EDOM March 8, 2011 Main result: HCF + XPW 5 fs, 100 μJ 0 0.0 -30 Phase (rad) Intensity (a.u.) 40 0.6 10 20 30 11 Direct XPW Filtered spatial profile of laser beam Actual spatial profile of laser beam 1.5 mJ 25 fs f = 1.5 m f Spatial profile of XPW beam 25-41 cm 300 μJ f XPW 20-cm hollow core waveguide Spectral broadening with XPW: 60 nm to 140 nm 2.5-mm BaF2 Polarizer Pulse compression with XPW: 25 fs to 9.6 fs Main result: Direct XPW 9.6 fs, 300 μJ! Journées Scientifiques de l’EDOM March 8, 2011 12 Summary and future work • Implemented two seed sources for an OPCPA based laser chain. - Hollow core fiber compression and cross polarized wave generation: 5 fs, 100 µJ, 10-10 contrast ratio - Direct cross polarized wave generation: 9.6 fs, 300 µJ, 10-10 contrast ratio • Improving the stability and reliability of the direct XPW seed source • Developing a stretcher for the seed source • Perform OPCPA Journées Scientifiques de l’EDOM March 8, 2011 13 Merci pour votre attention! Journées Scientifiques de l’EDOM March 8, 2011 14 Ultrashort approach: contrast HCF XPW - Pre-pulses are removed. - Contrast ratio is estimated to be 10-10. Journées Scientifiques de l’EDOM March 8, 2011 15