Continued improvements of air quality forecasting through emission adjustments using surface and satellite data & Estimating fire emissions: satellite vs. bottom-up Talat Odman, Yongtao Hu and Ted Russell School of Civil & Environmental Engineering, Georgia Institute of Technology With thanks to Pius Lee and the NOAA ARL Forecasting Team AQAST Meeting, January 15th, 2014 Georgia Institute of Technology Objective Improve air quality forecasting accuracy using earth science products through dynamic adjustments of emissions inventories and simulation of wildland fire impacts – Air quality forecasting is an integral part of air quality management. – Current forecasting accuracy calls for improvement. – Forecasting with 3-D models relies on accuracy of emissions. – Emission inventories are typically at least 4 years behind and “growth factors” are outdated. – Wildland fires are becoming an increasingly important contributor to PM and ozone. – Fire is one of the most uncertain emission categories as multi-year averages of past fires do not represent future fires. Georgia Institute of Technology Hi-Res Forecasting System Hi-Res Modeling Domains 4-km (123x123) 12-km (123x138) 36-km (148x112) • Based on SMOKE, WRF and CMAQ models • Forecasting ozone and PM2.5 since 2006 • 48-hour forecast at 4-km resolution for Georgia and 12-km for most of Eastern US • Used by GA EPD assisting their AQI forecasts for Atlanta, Columbus and Macon • Potentially useful for other states Georgia Institute of Technology Hi-Res performance during 2006-2013 ozone seasons for Metro Atlanta Ozone PM2.5 150 70.0 165 0 0 4-km 4-km 185 75 35.0 1068 60 749 52 0 0.0 75 0 150 70 35 0 Obs. Obs. MNB 20% MNB -10% MNE 25% MNE 32% Georgia Institute of Technology Inverse Modeling Approach for Adjusting Emissions An emissions and air quality auto-correction system utilizing near real-time satellite and surface observations • Minimizes the differences between forecasted and observed concentrations (or AOD) • With minimum adjustment to source emissions • Using contributions of emission sources calculated by CMAQ-DDM-3D – Source contributions can be used for dynamic air quality management.(e.g., fires) Georgia Institute of Technology Inverse Model Formulation • Solve for Rj that minimizes 2 DDM-3D calculated sensitivity of concentration i to source j emissions J obs sim ci ci Si , j ( R j 1) N total number of obs j 1 2 2 i 1 Ciobs total number of sources uncertainties Georgia Institute of Technology 2 weigh for the amount of change in source strengths J (ln R ) 2 j 2 j 1 ln R j emission adjustment ratio Off-line tests using “real-time” PM2.5 observations • Surface PM2.5 data from six sites in Atlanta – Direct use of satellite data (AOD) was problematic because of much larger uncertainties compared to surface data. – AOD will be “fused” to PM2.5 concentration fields to provide “real-time” spatial patterns. Kennesaw Gwinnet NE Atlanta Yorkville Atlanta West Atlanta Confederate Ave Douglasville South DeKalb Atlanta Conyers Fayetteville Newnan Georgia Institute of Technology Walton McDonough Peachtree City SLAMS O3 SLAMS PM2.5 NWS Met DDM-3D sensitivities calculated for week1: Dec. 1-7, 2013 Shown for select day Dec. 2, 2013 Obtained emissions adjustments ratios (Rj) Source Area On-road Non-road Dec. 1-7,2013 0.17Georgia Institute 0.83 of Technology 0.85 Point 0.97 PM2.5 Forecasting Performance for week 2: Dec. 08-14, 2013 with emissions adjustments Dec.11, 2013 PM2.5 Concentration without emissions adjustments Dec. 11, 2013 PM2.5 Concentration Obs (ug/m3) Sim (ug/m3) NFE NFB 8.57 16.57 65% 65% Emis adjusted 8.45 24% 2% Dec. 8-14, 2013 4.64 10.04 86% 85% Emis adjusted 5.62 54% 39% Dec. 11, 2013 Georgia Institute of Technology Comparison of Fire Emission Estimates: Satellite vs. Bottom-up • Both have roles in improving accuracy of fire impact forecasts: Satellite for wildfires and bottom-up for prescribed burns. • Global Biomass Burning Emissions Product (GBBEP) is currently using Fire Radiative Power from GOES • Buttom-up estimates use fuel-loads, consumption and emission factors. • GBBEP and buttom-up emissions compared for Williams fire, a 200 acre chaparrel fire in California on November 11, 2009 Akagi et al., ACP, 2012 Georgia Institute of Technology Comparison of Emission Estimates: Williams Fire • Buttom-up PM2.5 emission estimates are ~50% larger than GBBEP emissions • Aircraft measured aerosol light scattering, converted to PM2.5 and compared to modeled PM2.5 concentrations Georgia Institute of Technology Comparison of Modeled PM2.5 to Aircraft Measurements • Uncertainties in dispersion modeling (WS, WD, plume height, etc.) must be reduced to better evaluate emission estimates. Georgia Institute of Technology Conclusions • Dynamic emissions inventory adjustment dramatically improving PM forecast accuracy in offline testing. On-line testing and implementation underway – Large bias in dust emissions in winter corrected – Improved approach to assimilating AOD and PM measurements underway • Bottom-up and satellite-based fire emission estimates being improved with airborne smoke measurements – Fire emission contribution forecasts underway for dynamic prescribed-burn management Georgia Institute of Technology Poster • Davis et al., Nitrogen Deposition (Tiger Team Project) Acknowledgements • • • • NASA Georgia EPD Georgia Forestry Commission US Forest Service – Scott Goodrick, Yongqiang Liu, Gary Achtemeier • Strategic Environmental Research and Development Program • Joint Fire Science Program (JFSP) • Environmental Protection Agency (EPA) Georgia Institute of Technology Georgia Emission Totals (tons/yr) Georgia Totals (2013 Hi-Res) VOC NOx CO SO2 PM10 PM25 NH3 area-dust 241150 39240 area-others 366497 41790 118093 64613 32450 26965 80896 egu 1439 174136 11689 648564 11863 5977 5 non-egu 32843 49791 76059 60353 15059 10909 3613 non-road 69803 101653 786873 9403 9685 9242 49 on-road (NEI2011) 101360 241964 1084877 1133 10943 8144 4382 Georgia Institute of Technology DDM-3D sensitivities calculated for week1: Jul. 6-12, 2011 Shown for Jul. 11, 2011 Emission adjustments ratios (Rj) Source Area On-road Non-road Jul. 6-12,2011 Institute of Technology 3.34 Georgia 1.09 1.46 Point 1.10 PM2.5 Forecasting Performance of week2: Jul. 13-19, 2011 with emissions adjustments Jul.15, 2011 PM2.5 Concentration without emissions adjustments Jul. 15, 2011 PM2.5 Concentration Jul. 15, 2011 Obs (ug/m3) Sim (ug/m3) NFE NFB 11.35 3.85 94% -94% 7.23 50% -40% 8.67 54% -44% 14.92 44% 7% Emis adjusted Jul. 13-19, 2011 Emis adjusted 14.39 Georgia Institute of Technology