Recent Advances in Optically Pumped Semiconductor Lasers Juan Chilla, Qi-Ze Shu, Hailong Zhou, Eli Weiss, Murray Reed & Luis Spinelli Coherent Inc. 5100 Patrick Henry Dr. Santa Clara, CA 95054 ABSTRACT Optically pumped semiconductor lasers offer significant advantages with respect to all traditional diode-pumped solid state lasers (including fiber lasers) in regards to wavelength flexibility, broad pump tolerance, efficient spectral and spatial brightness conversion and high power scaling. In this talk we will describe our recent progress in the lab and applying this technology to commercial systems. Results include diversified wavelengths from 460 to 570nm, power scaling to >60W of CW 532nm, and the launch of a low cost 5W CW visible source for forensic applications. 1. INTRODUCTION Semiconductors are in many ways ideal laser materials. They are suitable for both optical pumping and direct electrical pumping, they are able to produce high optical gain and their quantum efficiency is high. Their emission is not limited to discrete lines set by atomic levels but can instead be chosen by design. Similarly multi-layered structures with varying index of refraction can be fabricated with great precision. The same physical processes that are responsible for such advantages impose limitations on the kind of devices that can be realized. In order to achieve optical gain in semiconductor, the active material cannot have arbitrary shape: one of the dimensions must be small (a few microns in the case of optical pumping, around one micron or less for electrical pumping), thus defining a plane that dictates the geometry of the laser devices. To date, the typical (and enormously successful) implementation of the semiconductor laser is what is commonly known as a “laser diode”, variations of which can be found everywhere. Low power devices are used in your CD drives and carry phone conversations and data through optical communication lines, high power diodes pump solid state laser materials and are used in material processing applications. Laser diodes are electrically pumped monolithic devices, contained within a “chip” of semiconductor material with typical dimensions around one millimeter. In spite of its many applications, this particular implementation of the semiconductor laser severely limits the performance of semiconductors as laser materials. If laser emission is in a direction contained in the plane, the most common case known as “edge emitters”, the laser is optically just a waveguide with gain, the modal characteristics of the laser defined by the waveguide. In order to obtain single mode operation the mode size has to be small (typically 1 × 3 μm) and the output power is limited by optical damage at the facets. High power can be obtained of course, but at the expense of brightness. Even single mode edge emitters are astigmatic and highly divergent, in order to obtain round beams with lower divergence the active region can be placed between two highly reflective mirrors, commonly made out of semiconductor materials. In that case the light is emitted perpendicular to the plane of the device. The resonator Fresnel number for this configuration (known as VCSEL, i.e. Vertical Cavity Surface Emitting Laser) is very high, and again there is a severe limitation to the power generated in a single mode. Contrary to the case for edge emitters, VCSELs cannot be practically scaled to high power by increasing the emission area. To bring the pump current to the center of the active region highly doped, or very thick layers would be needed right in the optical path, where they would cause unacceptable absorption loss. 2. OPTICALLY PUMPED SEMICONDUCTOR LASERS In order to take full advantage of semiconductors materials, our approach is to use them as we would any other solidstate laser material, pumping it optically and building it into a conventional laser cavity (Fig. 1). By using optical pumping we avoid the optical losses associated with doped materials, and we gain the ability to deliver the energy precisely where it is needed, while at the same time the fabrication process is simplified. By not restricting ourselves to a monolithic implementation we can use discrete optical components and free space propagation to obtain the desired characteristics of the output beam. The ability to access the intracavity radiation allows us to include a frequency doubling crystal and expose it to high circulating power1. Pump Diode Output Coupler Pump Delivery Optics OPS chip on Heatsink Optical Cavity Fig. 1. Schematic representation of an optically pumped semiconductor laser The OPS chip (Fig. 2) consists of two sections, both semiconductor alloys grown by MBE or MOCVD epitaxy. The top section is the gain medium and the bottom section is a high reflecting mirror that constitutes one of the ends of the cavity. The gain at the laser wavelength is provided by narrow layers of InGaAs (quantum wells), the composition of the spacer layers is chosen such as to make them transparent to the laser wavelength, and strongly absorbent to the pump wavelength (around 800 nm) 2. With this arrangement, all of the volume of the gain section is available for pump absorption, and the carriers that are generated decay rapidly to the lower energy levels available at the quantum wells, where population inversion is achieved. The quantum wells are located at the antinodes of the standing wave pattern of the linear resonator. This periodic gain structure makes optimum use of the available gain and eliminates any possibility of spatial hole burning, making it ideal for single longitudinal mode operation. Laser Out Pump Confinement Layer Quantum Wells Pump Absorption Layers HR Mirror Heat Sink Fig. 2. The OPS chip (optically pumped semiconductor). The different layers and their functions are indicated. Optical pumping of semiconductors had long been used as one of the early steps in the development of new semiconductor lasers, but usually as a research tool, not with the objective of creating a practical device but as a means of learning about material properties, i.e. as a step towards the ultimate goal of creating a monolithic, electrically driven device, a laser diode. Only recently there has been increased academic interest on the technology as a means to producing unique practical devices, a review of the theory of operation and recent activity can be found in ref. 3. 3. SEMICONDUCTORS AS SOLID STATE LASER MATERIALS In our description so far we have concentrated on the advantages of using semiconductors in the OPSL configuration instead of the more traditional laser diode configurations, in this section we will discuss what are their differences and advantages respect to traditional solid state laser materials. 3.1 Wavelength Flexibility In traditional solid state laser materials the energy levels involved in the laser transitions are those of a dopant or impurity in a crystal or glass. The levels in play are essentially atomic levels, with some limited modification caused by the solid matrix that surrounds these atoms. As atomic levels are discrete, so are the available transitions. Many applications for lasers were developed using bulky inefficient gas lasers, or gas laser pumped dye lasers. For some of those applications the exact wavelength used is not important, and can thus be served by solid state lasers, one example of such application is pumping of Ti:Sapphire ultrashort pulse lasers, initially carried out with Ar ion lasers at 488 and 514 nm, now almost exclusively done with frequency doubled Nd lasers at 532 nm. Other applications require a particular wavelength, for reasons related to the chemistry of the application. An example of these applications is ophthalmology, that has switched to 532 nm due to the advantages of solid state lasers, but is much better served at 577 nm, initially achieved with dye lasers. For semiconductors on the other hand, the laser transitions are the bands of the solid material itself. Traditional diode laser technology is based on epitaxial growth of material on top of crystalline substrates. Two III-V compounds have been developed significantly and there are established processes for their manufacture and use as substrates for epitaxial growth, they are GaAs, used for near IR and visible lasers, and InP, used in long wavelength communication devices. The wavelength flexibility of semiconductors comes from the possibility of growing alloys, i.e. mixtures of two or more III-V compounds. The ones most commonly used are GaAs, InP, AlAs, InAs and GaP. When these material alloys are grown in crystalline form many of the physical properties of the resulting material are simply weighted averages of the properties of the constituting compounds. One of those physical properties is the bandgap energy, i.e. the emission wavelength for a semiconductor laser. This is usually represented in the following diagram, that also shows the lattice constant of the different materials. Epitaxial growth is only possible when the free standing lattice constant of the desired alloy is very close to that of the substrate. 2.5 AlP GaP AlAs Bandgap Energy (eV) 2 AlSb 1.5 GaAs InP 1 GaSb 0.5 InAs InSb 0 5.4 5.6 5.8 6 6.2 Lattice Constant (A) 6.4 6.6 Fig. 3. Representation of possible III-V alloys, the shaded areas roughly represent the alloys that can be grown epitaxially on GaAs and InP, widely available substrates. Our interest in the OPS technology was initially sparked by the possibility of creating solid state lasers emitting at 488 nm. In 2001, the first commercial lasers based on the OPSL technology were introduced. The low power Sapphire™ platform was launched with two versions available: 20 mW at 488 nm and 10 mW at 460 nm. Since then, Sapphire™ has proven its extraordinary reliability and superior performance compared to the air-cooled argon ion laser. In Fall 2002 the family was expanded with the 200 mW version: Sapphire™ 488-200. Versions available today range between 10 mW and 500 mW. We have concentrated on frequency doubled configurations based on chips grown in the InGaAs material system, we have demonstrated a variety of wavelengths as listed in the table below. Doubled Wavelength (nm) Demonstrated Power (W) Application 460 479 488 505 532 570 7 7 15 8 64 9 Display Pump Ar Ion Ar Ion Many Ophtalmic Table 1. Frequency doubled wavelength of different OPS designs and maximum demonstrated power. OPS structures in the InGaAs material system can be grown to emit in any wavelength roughly within the range spanned by the table, the particular wavelengths we explored were chosen because of potential commercial application, and typically have been previously produced with other laser technologies. The limit on the short wavelength side is the reduced confinement and consequent loss of efficiency due to low indium concentration, on the long wavelength side the limit is the ability to grow highly strained material and the incorporation of high indium concentration. We have yet to convince ourselves that we have reached that limit. The powers listed in the table are only partially related to the inherent efficiency of each design, there is only a small increase in efficiency as wavelength gets longer, but due to mostly historic reasons our attempts to push the envelope and achieve new records are usually conducted on 980 nm material, the most mature, or on 1060 nm material, slightly more efficient. 3.2 High Power Scaling The ability to use a laser material to generate high powers is to a great extent dictated by the ability to remove excess heat. This is certainly true for solid state laser materials, for which their highest power expressions are obtained by using geometries that allow for easy removal of the excess heat, i.e. one dimension extremely longer than the other two, as in fiber lasers, or one dimension much shorter than the other two, as in disk lasers or slabs. Similar to the case of VCSELs, when pump power is increased in OPS lasers, we observe a roll over effect, i.e. output power increases up to a maximum and then falls with increasing pump power. Again the same as VCSELs, this experiment can be repeated several times with identical results, indicating that the limitation in output power is the effect of temperature on laser efficiency and not optical damage. Fig. 4. Some recent single chip high power results on different OPS designs The OPSL architecture lends itself to a natural way of scaling in power by simply increasing the beam size and pumped area on the OPS chip. By increasing the area in which heat is generated, we increase the amount of power needed to reach temperatures that have a detrimental effect on laser efficiency. Here the similarities with VCSELs end, as the external cavity can be redesigned to match the new spot size, the OPSL can be scaled up in power without sacrifice in optical performance. This procedure was successfully followed in going from the 20 mW product to the 200 mW product. The same OPS chip is used in both lasers, but cavity design and pump laser are different. In addition, the materials and techniques employed in mounting the OPS chip can be optimized for heat extraction efficiency. This approach was employed to obtain the results presented herein. The OPS structure is grown inverted, with the DBR as the topmost layer. After processing the wafer is cut into individual chips, which are then soldered on CVD diamond heat-spreaders. The DBR and solder layer are only a few microns thick, thus ensuring the heat only travels a short distance through high thermal impedance materials before entering the diamond that has very good thermal conductivity. The heat spreader in turn is soldered to a copper submount for handling of the device. Figure 4 summarizes some of our higher power results out of single OPS chips. In all cases the heat is ultimately removed by means of a water cooling system, but that is a matter of convenience more than strict need. The chips are pumped by fiber coupled arrays of diodes (FAP), in some cases more than one of them is arranged to illuminate a single chip. An effect that must be taken into account when designing an end-pumped high power solid state laser is thermal lensing. The excess heat is generated in the same volume that is occupied by the laser beam, the surrounding areas are colder. This difference induces in turn a difference in index of refraction (higher in the center) producing a considerable focusing effect. The power of the thermal lens depends on the amount of power being dissipated, and as a consequence solid state lasers typically operate in optimum configuration only for a narrow range of pump power. In contrast, the thermal lens is a minor effect for an OPSL because of the small optical thickness of the structure, furthermore, due to the area scaling procedure it becomes less of a problem as we increase the power level. Higher power requires larger area, that in turn results in smaller temperature gradients. We performed experiments to verify this. 980 nm SM Laser Wedge Pump Beam HR mirror Laser cavity OPS Chip Wedge CCD Camera Fig. 5. Setup employed to measure thermal lensing on OPS chips The experiment was conducted on 980 nm chips, but the results apply equally well to the other designs. A chip was used as one of the mirrors of a Mach-Zehnder interferometer, the chip could be pumped and used within a laser cavity as usual. The interferometer was illuminated with a single mode 980 nm laser (a 500 mW OPSL), in order to detect any phase disturbance caused by the chip relative to a reference flat mirror. The reflection of the beam on the chip happens in the DBR after going through the active region, in that way the interferometer detects not only changes in shape but also dephasing due to change in index of refraction. The setup is able to resolve changes of the order of 20 nm. 5´10 - 8 200 -0 8 ´10 - 7 150 -5 -1 ´10 2 ´10 --77 1´10 0 -1 ´10 - 7 50 100 50 100 50 150 100 200 150 100 50 150 Fig. 6. Measured phase disturbance normalized to surface height (in meters). Left: Laboratory Aluminum mirror pumped with 0.69W on 420 μm diameter spot. Right: OPS chip pumped with 70 W on 900 μm diameter spot. The experimental setup was carefully characterized; we verified its calibration by using it to measure a known surface, previously measured by using a commercial interferometric optical profiler. We also made sure it was able to detect thermally induced deformation by replacing the chip with a conventional aluminum coated laboratory mirror on glass substrate. The aluminum coating absorbs part of the incident pump power, and the poor thermal conductivity of the glass assures the presence of a hot spot at the center of the beam. Non uniform thermal expansion then induces a phase disturbance that shows as a clearly resolved hump in the pumped spot. When the chip was pumped with up to 70 W on a spot 900 μm in diameter we clearly saw the fringes move due to overall thermal expansion of the copper submount and supporting hardware, but the shape of the interferogram did not change, we were unable to detect any lensing effect. In further efforts pumping tighter with 9 W on a 420 μm diameter spot we were able to detect lensing at the edge of our resolution, a negligible effect of the order of λ/40. The fact that thermal lensing is negligible for high power OPS lasers opens an additional avenue for further scaling of the output power. Scaling up the power without radical changes to the chip structure does not improve the efficiency, so more output power implies proportionally higher excess heat that has to be removed from the chip. If we continue to pump harder and harder on a chip, we have large amounts of excess heat that have to be removed from a very small volume. From purely thermal considerations it would make more sense to separate the heat sources, instead of doubling (or tripling) the pump power to a chip, use two (or three!) chips. With conventional solid state laser materials thermal lensing makes the idea of multiple gain elements in a cavity a harder proposition, specially if good mode quality is required, in the case of OPS it is relatively simple. 60 70 3 chips 60 50 50 Power (W) Power (W) 40 30 2 chips 40 30 20 20 10 0 10 0 50 100 150 Pump Power (W) 200 250 0 0 50 100 150 Pump Power (W) 200 250 Fig. 7. Green (532 nm) output from multi-chip OPS lasers. Left: TEM00 (M2<1.3). Right: Multimode with 3 chips 300 Figure 7 shows the results of some of our multi-chip experiments, we are able to deliver close to 100 W of pump power in 900 μm diameter spot on each of the chips. Multiple chips are added as folding mirrors, the cavity design includes curved mirrors to create a waist on each of the chips. On one end of the cavity a 5 mm long LBO crystal is placed in a tighter waist within the cavity and provides the frequency doubled output. As seen in the left plot, the increase in power can be achieved without sacrifice of beam quality, when the mirror distances within the cavity are properly chosen the laser emits in a single transverse mode, and roll-over powers of 40 and 55 W are obtained with two and three chips respectively, always with M2 of less than 1.3. The lack of thermal lensing is evident from the smooth shape of these curves, the cavity operates the same way at all power levels. As it is also the case for single chip cavity, our multi-chip laser is capable of providing higher green power with slightly worse beam quality. The plot on the right shows the green output power off the three chip laser when aligned for maximum green output and operating slightly multimode. More than 60 W of power are obtained. We did not measure the M2 in this configuration, but the increase in power is consistent with what is observed in single chip lasers where the maximum green power is obtained at M2 around 4. 3.3 Relaxed Pump Requirements One of the key advantages of OPS respect to traditional solid state laser materials is the relaxed requirements it imposes on the pump diodes. First, the absorption spectrum of the semiconductor materials is much broader than traditional solid state laser materials, essentially any wavelength shorter than the bandgap can be absorbed and used for pump purposes. There is not, as for traditional laser crystals, the need to accurately control the temperature of the diode to keep the emission within a narrow absorption line. X view 2 0 -2 0 5 10 15 20 25 30 35 40 Y view 10 5 0 -5 -10 0 5 10 15 Fig. 8. Layout and ray tracing simulation of the pump optics 20 25 30 35 40 Not only there is great freedom to choose pump wavelength, but also the spatial requirement on the pump beam quality are significantly reduced. This is an advantage even respect to fiber lasers, that require high brightness pumps, typically achieved by aggregating several fiber coupled single emitters. The pump radiation is absorbed in just a few microns of material, therefore the pump beam needs practically no depth of focus, i.e. the acceptance angle is almost unlimited. The significance of this is that for OPS there is no need to go through the extra step of coupling the pump into a fiber, with the associated loss of efficiency and increased complexity. Figure 8 shows a design for pump optics used in our concept demonstration of lasers for rear projection TV4. As with other aspects of that prototype we limited ourselves to “off the shelf” optics, because of that it was necessary to use a total of four lenses to achieve the desired pump spot characteristics. We have explored the design space and believe the same performance can be achieved using just two simple custom lenses, making the design simpler and hence more suitable for mass production. 4. APPLICATIONS OF HIGH POWER OPS LASERS So far we have discussed experiments and laboratory demonstrations of the advantages of OPS lasers. As a commercial enterprise, Coherent manufactures laser systems, and is now introducing the first products in the high power OPS line. These laser designs represent an evolution from the design used for the concept TV demonstration, and are targeted at applications where the advantages of OPS bring value to the user, we will briefly discuss two of those applications. One of the tools employed in crime scene investigation is the fluorescence of trace evidence. Fingerprints, bodily fluids and fibers fluoresce under blue-green illumination, either naturally or when sprayed with a dye solution. Lasers have long been recognized as the preferred source of light for this application, in work pioneered using ion lasers from Coherent, but the cost, bulk and power requirements of lasers have until now prevented their use outside the laboratory. Investigators have used portable lamps to take to the field, the evidence found was bagged and photographed in the lab typically using a laser. Fig. 9 TracER, battery operated portable laser system for forensic applications. Coherent recently released the TracER ™ laser system that includes an OPS laser emitting in the green. The system was designed specifically for forensic application both in the lab and in the field. The laser is fiber delivered to a wand that provides the user with a variable zoom and the ability to remotely control the laser with up to 5 W out of the hand-piece. The most unique feature of this system is that it is battery powered. When plugged in, it can simultaneously operate and charge the batteries, off the electric grid it can run for over 90 minutes before needing a charge. This is made possible by the high efficiency of the OPS laser. As can be expected that a device used in the field will be subjected to severe treatment, the system was designed with ruggedness in mind and was subjected to extensive testing. As part of that testing the OPS laser head survived shocks over 500 G! Another example where the wavelength flexibility of OPS is a valuable advantage is ophthalmic applications. Studies conducted by using dye lasers showed that the preferred radiation for the treatment was yellow light, 577 nm in wavelength. There have been some attempts to address this application with Nd:YAG doubled to 561 nm, but the difficulties associated with operating the laser material outside of the most efficient green line make it not very practical. With OPS we can simply dial in the design to produce the desired wavelength. Fig. 10. Prototype yellow (577 nm) laser for ophthalmic applications REFERENCES 1. 2. 3. 4. A. Caprara et al, US Patent No. 6167068, US Patent No. 5991318 M. Kuznetsov et al, IEEE Photonics Technology Letters, vol. 9 (1997), p. 1063. A. C. Tropper & S. Hoogland, Prog. Quantum Electronics 30 (2006), p. 1 J. Chilla et al, Proc. SPIE Vol. 5740 p. 41-47, Projection Displays XI (2005)