Journal of Atmospheric and Solar-Terrestrial Physics 81–82 (2012) 76–85 Contents lists available at SciVerse ScienceDirect Journal of Atmospheric and Solar-Terrestrial Physics journal homepage: www.elsevier.com/locate/jastp Cloud microphysical properties over Indian monsoon regions during CAIPEEX-2009 Savita B. Morwal n, R.S. Maheskumar, B. Padma Kumari, J.R. Kulkarni, B.N. Goswami Indian Institute of Tropical Meteorology, Pashan, Pune 411 008, India a r t i c l e i n f o a b s t r a c t Article history: Received 2 August 2011 Received in revised form 4 April 2012 Accepted 24 April 2012 Available online 6 May 2012 Cloud microphysical data collected from an instrumented aircraft in the Cloud Aerosol Interaction and Precipitation Enhancement Experiment (CAIPEEX-2009) during May–September 2009 have been used to examine the nature of cloud drop size distributions (DSD), cloud drop effective radius (RE) and their height variations at different locations during tropical Indian monsoons. Single mode drop size distributions were observed over Pathankot, Hyderabad and Bengaluru regions and bimodal DSD were recorded often over Guwahati and Bareilly regions. DSD spectral width showed height variation, being narrow at lower heights and broadening with increasing height. DSD spectra were narrow even at higher levels over Pathankot during pre-monsoon season and were very broad at Bareilly and Guwahati during the active phase of monsoon. The total concentrations of cloud droplets and percentage contribution of cloud droplet of radiir10 mm (small) and 410 mm (large) showed interesting height variations and were different over different regions. The RE showed nearly linear increases with height over all the regions. However, the droplet growth rate is observed to be different over different regions, being less over north (Bareilly and Pathankot: 1.3–1.46 mm/km), intermediate over central (Hyderabad: 1.74 mm/km) and highest over northeast (Guwahati: 1.92 mm/km) and south (Bengaluru: 1.99 mm/km) India. For the first time an attempt has been made to collect and explore cloud microphysical characteristics using in-situ aircraft observations during Indian monsoon conditions. & 2012 Elsevier Ltd. All rights reserved. Keywords: Atmospheric processes Microphysics of clouds Cloud droplet distributions CAIPEEX 1. Introduction Clouds play a vital role in the dynamics and thermodynamics of the atmosphere. Cloud-scale processes are considered sub grid scale as far as cloud dynamics and cloud microphysics is considered. Hence, representation of these processes in large-scale weather and climate models is a challenge. Cloud microphysics includes the small scale properties of clouds such as material state (i.e., solid or liquid) of the cloud particles, their size and concentration. Clouds form in the atmosphere when the air becomes supersaturated so that water vapor condenses on particles to form droplets. During cloud formation the concentration of cloud droplets depends on the concentration of certain particles present in the air mass. Therefore, preexisting particles determine cloud properties such as droplet concentration and size. Increases in particle (i.e., CCN) concentrations due to anthropogenic sources leads to higher concentrations of smaller cloud droplets. Cloud drop size distributions also depend on the development stages n Corresponding author. Tel.: þ91 020 25904262; fax: þ 91 020 25893825. E-mail addresses: morwal@tropmet.res.in (S.B. Morwal), mahesh@tropmet.res.in (R.S. Maheskumar), padma@tropmet.res.in (B. Padma Kumari), jrksup@tropmet.res.in (J.R. Kulkarni), goswami@tropmet.res.in (B.N. Goswami). 1364-6826/$ - see front matter & 2012 Elsevier Ltd. All rights reserved. http://dx.doi.org/10.1016/j.jastp.2012.04.010 i.e., an early developing stage with precipitation associated with numerous small cloud drops to mature stage and dissipating stage and precipitation with larger drops. The cloud drop size spectrum has been studied by many workers (Zaitsev, 1950; Weickmann and Aufm Kampe, 1953; Squires, 1958a, 1958b; Warner, 1969a, 1969b, 1973; Twomey and Warner, 1967; Hudson and Yum, 1997; Yum and Hudson, 2005; Hudson et al., 2009; Gerber, 1996). Cloud droplet number concentrations vary with height and cloud type (Martinsson et al., 2000). Further, it has been observed that normally the concentrations have been found to be less than a few hundreds cm 3 and rarely above 1000 cm 3 in stratiform clouds (Hudson et al., 2010; Anderson et al., 1994; Garrett and Hobbs, 1995; Gillani et al., 1995; Leaitch et al., 1986, 1996; Martin et al., 1994; Twohy et al., 1995) although a very high concentration was observed by Martinsson et al. (2000). Fair weather continental cumulus clouds with no precipitation have relatively narrow drop size spectra while continental cumulus clouds which have reached more mature stages of cumulus congetus show much broader cloud drop spectra (Hobbs et al., 1980). Further, they showed that cumulus clouds embedded in a stratus layer have even broader spectra. Maritime clouds have broader drop size spectra compared to continental clouds (Hudson and Yum, 1997; Pinsky and Khain, 2003; Wang et al., 2009; Battan and Reitan, 1957). S.B. Morwal et al. / Journal of Atmospheric and Solar-Terrestrial Physics 81–82 (2012) 76–85 Increases in aerosol concentrations result in decreased drop sizes (Breon et al., 2002; Rosenfeld et al., 2008a) which may suppress precipitation (Albrecht, 1989; Rosenfeld, 2000; Hudson and Yum, 2001; Hudson et al., 2009;). An appropriate measure of the mean drop size is the effective radius (RE), which is the ratio between the third and the second moment of the cloud droplet size distribution (Stephens, 1978). This is indicative of the threshold size of cloud drops below which precipitation seldom forms. Cloud drops at the threshold size rapidly grow to raindrops (Houze, 1993). The RE has been studied by many workers (Rosenfeld et al., 2008b; Martins et al., 2007), which is related to the spectral width of the cloud droplet spectrum (Pontikis and Hicks, 1992; and Martin et al., 1994). In order to understand the interaction between clouds and aerosols and also to understand the microphysical properties of clouds over the tropical Indian region, a national experiment called ‘Cloud Aerosol Interaction and Precipitation Enhancement Experiment (CAIPEEX)’ was launched during 2009 and completed successfully by making observations of cloud microphysical parameters and aerosols from 17 May to 30 September 2009 over various geographical regions of India by the Indian Institute of Tropical Meteorology, Pune. The observations of aerosols and cloud microphysical and dynamical parameters were collected onboard aircraft over various Indian regions including some close to the coast. The following Section gives some details of the observations and meteorological conditions that prevailed over the different base stations during the observation periods. We attempt to examine the characteristic features of cloud droplet spectra over various regions with different geography and meteorology. 2. Data and instruments The national scientific program CAIPEEX launched on 17th May 2009 from Pune base station was envisaged to have three phases. The main objective of Phase I was collection of good spatio-temporally resolved data of aerosols and cloud microphysical parameters from May to September 2009 over various regions of India. The specific objectives of Phase I were: (i) to measure background concentrations of aerosols and CCN during the monsoon season, (ii) observations of hydrometeors in clouds, (iii) observations of space-time variability (during the monsoon season) of trace gases over India and (iv) selection of sites for the phase II experiments. An instrumented Piper Cheyenne aircraft was used to collect in-situ observations of aerosols and cloud microphysical parameters viz. Liquid Water Content (LWC), total water content, concentrations of Cloud Condensation Nuclei (CCN) and number concentration of cloud droplets of different sizes, temperature, humidity, etc. The different aircraft instruments include AIMMS Probe, Cloud Droplet Probe (CDP), Cloud Imaging Probe (CIP), CCN counter, Gas Analyzer, LWC probe, etc. The program was conducted in missions and IOP (Intensive Observation Periods) mode. The mission consist of observations during the transit of the aircraft from one base to the other. The IOP consists of aircraft observations and other routine ground-based observations over the selected base station regions. The IOP base stations included Pune (18.521N, 73.851E), Pathankot (32.261N, 75.651E), Bareilly (28.351N, 79.411E), Bengaluru (12.971N, 77.591E), Hyderabad (17.381N, 78.481E) and Guwahati (26.181N, 91.751E) (Fig. 1). Pathankot and Bareilly are located in northern India, Hyderabad is in the Central region, Pune and Bengaluru are in southern India and Guwahati is in the northeast. Based on the analysis of synoptic and thermodynamic conditions a work area was chosen with high potential for development of cumulus clouds. On a particular day the observations were collected preferably in the isolated growing cumulus clouds by profiling the clouds so that we would have a succession of growing towers until we reached the maximum cloud top. Sometimes clouds at different 77 heights were also chosen. All data are 1 s averages. If observed LWC is40.0 and total cloud droplet concentration is420 cm 3 of a minimum 3 s, it is considered as cloud. All the observations satisfying this condition in the updraft regions have been chosen for analysis. A Cloud Droplet Probe (CDP) from Droplet Measurement Technologies (DMT), USA was mounted externally below the right wing of the aircraft. CDP sized and counted cloud droplets in the size range from 2 to 50 mm in 30 size bins at the sampling frequencyof 1 Hz. By using the sample area at a known velocity, particle concentrations were calculated. Other parameters that can be computed include the average drop diameter, mass weighted diameter, mode distributed diameter, standard deviation and liquid water content (LWC). Cloud drop size distributions, cloud drop effective radii and their height variations over different regions are presented and discussed. For convenience data of one day for each of the IOP regions is presented: 28 May 2009 (Pathankot), 15 June 2009 (Hyderabad), 1 July 2009 (Bengaluru), 24 August 2009 (Bareilly) and 4 September 2009 (Guwahati). Liquid Water Content (LWC, g/m3) was measured onboard the instrumented aircraft by a Johnson Williams (JW) Hotwire probe, which was mounted externally in the nose. LWC was also derived from measurements of CDP cloud droplet size distributions. The CDP was size calibrated from time to time in the field with known bead sizes. Baumgardner (1983) made an analysis to estimate measurement accuracies of the water droplet measuring probes and JW Hotwire probe. In order to validate the LWC data computed from CDP observations, correlation between the LWC values directly measured from JW Hotwire probe and CDP derived LWC is examined for all the days considered in this study. There was a high correlation (40.85) between the two probes. For the measurement of precloud aerosol a Passive Cavity Aerosol Spectrometer Probe (PCASP-100X) was mounted below the left wing of the aircraft. The PCASP counts and sizes the fine and accumulation mode size particles (such as soot, organic carbon and smaller mineral dust) of diameters in the range 0.1–3 mm in 30 size bins (Padma Kumari et al., 2011; Liu et al., 2009). The PCASP is factory calibrated using known size latex spheres (Johnson et al., 2008) and is also calibrated from time to time in the field. Data was collected at an interval of 1 s (or 100 m) by all the above mentioned instruments. 3. Results and discussion The height variation of cloud droplet concentrations of different sizes over different IOP base stations during May–September 2009 has been studied by using the number concentration spectra of cloud droplets with radius between 1 mm and 25 mm. These drop size spectra are available at various altitudes between 0.6 km and 8 km. Here, the observations associated only with updrafts are considered. Average cloud droplet spectra at 1 km intervals have been computed for each km up to 8 km for all the days. Cloud Droplet size Spectra (DSD) in different layers, percentage concentration (normalized to total number of cloud droplets in the size range 1–25 mm) of droplets in the size ranger10 mm (small) and 410 mm (large) and effective radius in each layer for the five base stations as mentioned above, is shown in Fig. 2. SMOKE-LBA campaign observations suggest that when RE is close to 12 mm, the efficiency of coalescence increases (Andreae et al., 2004). The study carried out by Rangno and Hobbs (2005) to determine the microphysical structures and precipitation-producing mechanisms in cumulus and small cumulonimbus clouds over the warm pool of the tropical Pacific Ocean showed that cloud effective radius of 12–14 mm is required for the onset of an effective collisioncoalescence process. Hence, in order to examine the increase in coalescence efficiency/initiation of the warm rain process, the cloud 78 S.B. Morwal et al. / Journal of Atmospheric and Solar-Terrestrial Physics 81–82 (2012) 76–85 Pathankot Bareilly Guwahati Patna Pune Hyderabad Bengaluru Fig. 1. Map of India showing the location and name of the different IOP (Intensive Observation Periods) base stations during CAIPEEX 2009. droplets with radius 12 mm and greater are separated. The dark vertical line in the DSD in Fig. 2a indicates the value of the cloud drop radius for the initiation of the coalescence/warm rain processes (i.e., 12 mm). 3.1. Height variation of cloud droplet spectra Cloud droplet spectra have been studied extensively (e.g., Yum and Hudson, 2001, 2002; Derksen et al., 2009; Miles et al., 2000; Warner, 1969a; Paul, 2000; Cooper, 1989; Pawlowska et al., 2006). In this sub section in-situ aircraft measurements of cloud droplet spectra collected using the CDP during CAIPEEX 2009 over various regions at various levels are explored and shown in Fig. 2a. May 28, 2009 was a normal pre-monsoon dry day over north India, with surface temperatures of 40 1C and no clouds over Pathankot except over the Himalayan mountain to the north of Pathankot. To the north of Pathankot the observed cloud base of 4545 m was the top of a haze layer at 3 to 4 km. From the radiosonde ascent at the base station, the lifting condensation level was approximately 3.7 km and the freezing level was 4.5 km. From DSD spectra in different vertical layers for Pathankot, it is evident that the droplet radius ranges from 1.25 mm to 13.75 mm. In all the layers the droplet spectra are very narrow and associated with a single mode. However, the spectra showed broadening with increasing altitude (Paul, 2000; Warner, 1969a) with simultaneous increase of modal radius except in the 5–6 km layer. The concentrations are more or less the same for sizes below the modal value (but modal values are different in different layers) in all the layers except in the 4–5 km layer, which is associated with very high concentrations of small droplets. Above the modal value the concentrations are less in the lowermost layer (4–5 km) and showed continuous increase with height except in the 5–6 km layer where it was lower. It is clearly evident from DSD spectra that the modal radius, in all the vertical layers is well below 12 mm which indicates that there is little possibility of initiation of the warm rain (Rangno and Hobbs, 2005). Suppressed convection was observed over the Pathankot IOP region where convection was usually observed only during afternoon hours. Also, a polluted haze layer extended up to 4 km (black line in Fig. 3. The aerosol concentration was very high up to 4 km and decreased above this altitude.). The observed DSD spectra, narrow and single mode with high number concentrations, represents typical super-continental types of clouds. On 15 June 2009 over the Hyderabad region weather conditions were partly cloudy with the possibility of development of deep convection within radial distances of 100 nautical miles NE and SW of Hyderabad. However, due to military restrictions, observations on this day were made only in the region east of Hyderabad. In the observational area, clouds with base heights above 2.7 km were encountered. Fig. 2a shows the cloud droplet size (DSD) spectra in the layers 2–3 km to 6–7 km. The droplet size spectra are narrow in the lower layers (2–3 and 3–4 km) and broaden with height and the maximum size range reaches up to 18.5 mm. According to Pawlowska et al. (2006) the broadening of the spectra/ spectral width affects the radiative properties of clouds (Liu and Daum, 2000) and development of drizzle and rain (Seifert and Beheng, 2001). All the spectra showed a single mode in droplet size distributions. The maximum concentration of different cloud droplets was 50 cm 3/mm which is very less as compared to that over Pathankot. The modal radius showed a gradual increase with height. However, the modal radius (o 9 mm) was still below the value of 12 mm at all the altitudes indicating the S.B. Morwal et al. / Journal of Atmospheric and Solar-Terrestrial Physics 81–82 (2012) 76–85 79 Fig. 2. Variation, in different layers over Pathankot, Hyderabad, Bengaluru, Bareilly and Guwahati during CAIPEEX 2009, of (a) Number concentration spectra of cloud droplets, (b) total concentration (black solid line with open triangle) and percentage contribution of clouds drops of radius r 10 mm (solid line with solid circles in black) and410 mm (solid line with solid circles in red) and (c) effective radius (RE). Note that the different distances in (b) are above cloud base (mentioned below the title) and distances are above mean sea level in (a) and (c). (For interpretation of the references to colour in this figure legend, the reader is referred to the web version of this article.) 80 S.B. Morwal et al. / Journal of Atmospheric and Solar-Terrestrial Physics 81–82 (2012) 76–85 6000 Pathankot Hyderabad Bengaluru Bareilly Guwahati Altitude (m) 5000 4000 3000 2000 1000 0 0 500 1000 1500 2000 2500 Aerosol Concentration (cm-3) 3000 Fig. 3. Vertical variation of cloud free aerosol concentration from PCASP-100X at different stations viz. Pathankot (Black), Hyderabad (Red), Bengaluru (Green), Bareilly (Blue) and Guwahati (Magenta). Very high aerosol concentration is observed over Pathankot. The pollution is high in the lower layers over Bareilly (below 2 km) and Guwahati (below 1 km). (For interpretation of the references to colour in this figure legend, the reader is referred to the web version of this article.) inefficiency of the collision-coalescence processes (Pawlowska et al., 2006). The observed DSD spectra with a single mode represent continental type of clouds which are influenced by the prevailing weather conditions, i.e., subdued convective activity. Number concentration spectra on 1 July 2009 at IOP base Bengaluru, in different layers from 1–2 km to 6–7 km are shown in Fig. 2a. The cloud base is around 1.8 km. All the spectra show a single mode and are associated with gradual increase in modal radius with altitude. The maximum droplet number concentration at the modal radius in different layers vary from 22–63 cm 3/mm. The droplet size range is higher ( 420 mm) than that observed over Pathankot and Hyderabad. The droplet spectra in the 1–2 and 2–3 km layers are narrow (radius rangeo10 mm) and showed broadening in the layers above this (range 415 mm). The broadening of the spectra may be due to the growth of the size of the cloud droplets with increasing altitude (Pawlowska et al., 2006 and Seifert and Beheng, 2001). Also, it can be attributed to the incursion of moisture in the higher altitudes under the large scale influence of the monsoon circulation (confirmed from vertical profiles of temperature and mixing ratio using radiosonde data over the region, not shown). As seen from Fig. 2a, the modal radius at all the altitudes is much less than the vertical line of 12 mm ( 10 mm). Thus, over this region, the DSD spectra were broad and associated with a single mode. The north–south shift of the monsoon trough has an important bearing on the rainfall distribution over India (Rao, 1976). Under the normal monsoon conditions, the axis of the monsoon trough extends from Ganganagar (in Rajasthan, westward end) to Kolkata with its eastward end over the Head Bay. When the axis of the monsoon trough moves north and lies close to the Himalaya, a break in rainfall is observed over most parts of India (Rajkumar and Narasimha, 1997; Parasnis et al., 1991; Rao, 1976). The normal position of the monsoon trough is usually associated with enhanced monsoon activity over India (Rao, 1976; Sikka and Narasimha, 1995). Bareilly is at the meeting point between the surface SW winds and the easterlies at the north of a west moving tropical depression to the south. Over the IOP region Bareilly, on 24th August 2009 the monsoon was very active due to the presence of the monsoon trough over this region. The observed cloud base was at 0.7 km. The cloud base was extremely warm (25.3 1C) and the atmosphere was extremely polluted (high concentration of aerosols below 2 km as shown with the blue line in Fig. 3) and moist. The depth of the cloud was more than 5 km. Fig. 2a shows the number concentration spectra of cloud droplets in different layers starting from 0–1 km to 7–8 km at Bareilly. Over this base the spectra are very broad starting from the lowermost layer (radius range 413.5 mm) and broadening continued with increase in height and reached up to radius of 25 mm. Some of the droplets are bigger than 12 mm even in the lowest layer (0–1 km), suggesting the effect of giant CCN. The spectra have single mode in the lower layers up to 2–3 km layer with modal radius of 6–7 mm. Above this layer, all the spectra are bimodal with increase in modal radius and the second mode reaching up to 12 mm. Even though the modal radius was above 12 mm in all the layers above 3 km warm rain was not observed, this may be due to the high pollution over this region (as seen from Fig. 3. The concentration of aerosols was high in the layers below 2 km indicating polluted air masses in the boundary layer). Thus, this particular day indicated that pollution was able to prevent warm rain from forming in growing convective towers up to 5.5 km, which was associated with negative temperature.. Thus, the observations collected on 24 August 2009 at Bareilly demonstrate that heavy air pollution can suppress warm rain from clouds below the freezing level even in very moist tropical conditions, with the thickest cloud depth between base and freezing level (Rosenfeld, 2000). Aerosols serve as a source of both cloud condensation nuclei (CCN) and ice nuclei (IN) and affect microphysical properties of clouds. Clouds forming in a more polluted atmosphere, as observed here, contain a larger number of smaller drops and assumed to retard the cloud droplet coalescence thereby decreasing precipitation. Also, according to Rosenfeld et al. (2002) the polluted clouds over land need to grow beyond 6 km in height to start precipitating. On 4th September 2009 a weak southerly flow from the head Bay to the north-east Indian region (Assam) was observed. The observations were conducted over the Meghalaya region, which is south west of IOP region Guwahati and west of Bangladesh. Over this region, isolated thunderstorms were predicted to occur in the afternoon. The cloud base varied from less than 1 km to 1.5 km at different locations in Guwahati. Fig. 2a shows the cloud droplet concentration (with base at 1.8 km) in the different vertical layers from 1–2 km to 6–7 km. The droplet spectrum is narrow in the 1–2 km layer and shows continuous broadening with successive increase in altitudes. The range of the spectra reaches 25 mm. The droplet spectrum is single mode in the lowest layer with gradual increase of the modal diameter with increasing altitude. The spectra are bimodal in the layers above lowest layer as observed by Warner (1969a). The second modal diameter crosses the value of 12 mm in the layers at and above 3–4 km. Thus, the initiation of the warm rain processes may take place above this height as mentioned by Pawlowska et al. (2006). As per flight scientists’ day-to-day reports rainfall was noticed at altitudes above 4.5 km. All the clouds are well grown clouds and associated with rain as reported in the flight report. All the spectra are very broad with modal radii above 12 mm. The characteristic of all the spectra are: (i) droplet spectra at the top of a good growing cloud in the 3–4 km layer (at an altitude of 3.8 km, not shown in Fig. 2a) was of single mode at radius 12.5 mm. (ii) droplet spectra in the 4–5 km layer at the top of freshly formed cloud (at an altitude of 4.54 km) was single modal with mode radius of 13.5 mm and (iv) the spectra in the layer 5–6 km at the top of a strongly growing tower (at altitudes of 5.44 km, 5.8 km) and in the layer 6–7 km (at altitude of 6.36 km) showed bimodal distribution where secondary mode was above 15 mm radius. Thus all the growing clouds are associated with broad spectra and greater number of larger cloud droplets as compared to small droplets. According to the basic microphysical process in warm tropical clouds, the particle growth by condensation begins below cloud base and continues in clouds under supersaturated conditions, giving rise to droplet formation (Khain et al., 2000). The process of condensation growth of particles includes nucleation as well as S.B. Morwal et al. / Journal of Atmospheric and Solar-Terrestrial Physics 81–82 (2012) 76–85 diffusional growth of droplets. From cloud model simulations Pinsky and Khain (2002) found that droplet spectral formation is affected by three stages of in-cloud droplet nucleation which lead to formation of primary and secondary modes, i.e., mono-modal and bi-modal drop size distributions. They have also shown that the secondary mode in the droplet spectrum contributes significantly to raindrop formation. Two main mechanisms have been suggested in the literature for the formation of secondary small droplet mode in droplet spectra. (i) Entrainment mechanism: mixing of clouds with environmental air accompanied by partial evaporation of cloud droplets in subsaturated zones, as well as by fresh droplet nucleation of CCN penetrating the clouds through the lateral cloud boundaries (Warner, 1973; Brenguier and Grabowski, 1993; Lasher-Trapp et al., 2005; Su et al., 1998) (ii) In-cloud nucleation mechanism: this enables in-cloud nucleation of new droplets on CCN penetrating the cloud base and ascending together with cloud droplets formed at low levels (Khain et al., 2000; Pinsky and Khain, 2002; Segal et al., 2003). Such in-cloud nucleation takes place when supersaturation within an ascending cloud parcel exceeds its local maximum near the cloud base (Ludlam, 1980; Pinsky and Khain, 2002; Segal et al., 2003). In the present study the bimodal drop size distribution has been observed over Bareilly and Guwahati. Over Bareilly, the atmosphere was moist, extremely polluted and hazy (shown in Fig. 3). The cloud base was very warm and at very low levels ( o1 km). The bimodal droplet spectra might have been produced by entrainment of polluted environmental air through the lateral cloud boundaries. 3.2. Total concentration and effective radius (RE) of cloud droplets It is expected that cloud droplet concentrations of different sizes change with height depending on the microphysical processes in the cloud. To examine this, height variation of the percentage (normalized by respective layer total concentration) of cloud droplets of radius r10 mm (black line, small droplets) and410 mm (red line, large droplets), for all the days over each IOP base stations in each layer is shown in Fig. 2b. In this figure, solid line with open triangles indicates the total concentration in each layer. The bar diagrams for effective radius in all the vertical layers are shown in Fig. 2c. From Fig. 2b, it is seen that the total concentration over Pathankot is high (390–650 cm 3) in all layers except the 5–6 km layer (154 cm 3). The percentage contribution of small droplets is very high (498%) throughout. This indicates the existence of super continental clouds. This could be due to low LWC (as shown in Fig. 5 first row) or entrainment of polluted air masses (as shown in Fig. 3). The percentage of large drops is negligible in all the layers. The effective radius increases from the lowermost layer to the highest layer as observed by others (Pawlowska et al., 2006; Martin et al., 1994; Miles et al., 2000; Wood, 2000). However, the magnitude of RE is (below 6.4 mm) very much less than 10–12 mm at which the warm rain process initiates according to Rangno and Hobbs (2005). Thus, during the pre-monsoon season, the possibility of precipitation initiation from the observed clouds is inhibited due to the presence of high concentrations of small droplets. Over the Hyderabad region the total concentration of cloud droplets (Fig. 2b) is more or less the same in each layer and is in the range of 210–280 cm 3. The total concentration of cloud drops is less at all levels compared to Pathankot. The percentage of small drops is very high up to the 4 km layer (499%) and thereafter decreases with height. The percentage contribution of large drops increases monotonically above 4 km to the 6–7 km layer and it is 24% in the highest layer. The RE showed continuous increase from lower layers to higher layers (3.8 to 9.5 mm). However, the RE is still below the value required for the initiation of warm rain at all levels. 81 Thus, the cloud microphysical features as seen on 15 June 2009 over the Hyderabad region clearly indicates the inhibition of natural initiation of the warm rain processes under prevailing weather conditions. At Bengaluru, the total concentration of cloud drops showed less variation with height (171–308 cm 3) compared to that over Pathankot and attains a maximum in the 3–4 km layer (530 cm 3). This region is under the influence of widespread monsoon activity and there was an incursion of moisture in the mid levels (3–5 km) as seen from the radiosonde profiles (not shown here). The percentage of small droplets is very high ( 499%) in the lower layers up to 3 km and thereafter it decreases continuously with height. Also, the percentage of large drops increases with height and to 33% in the highest layer. This may be due to the (i)conversion of small cloud drops to bigger drops in the higher layers and (ii) intrusion of moisture at higher levels due to the prevailing large scale monsoon conditions as observed from vertical profiles of temperature and moisture obtained from radiosonde data. The effective radius increases continuously with height and it is slightly more than 10 mm in the 6–7 km layer. The cloud base at Bareilly was observed at very low level and the environment was polluted with the existence of a haze layer (Fig. 3 shows the high concentration of aerosols up to 2 km indicating polluted air masses). The monsoon was very active over this region. Total concentration varied between 70–395 cm 3 in the various vertical layers. The percentage concentration of the smaller drops is very high (496%) below 2 km and it decreases with height. The percentage of large cloud drops increases with height and it exceeds the small cloud drops above 4 km. The effective radii showed an increasing trend with height up to more than 12 mm in the layers above 4–5 km. This supports the rain observed above 5 km as stated in the sub Section 3.1 and the criteria for the initiation of warm rain. Over Guwahati, where the monsoon was active on 4th September 2009, the total concentration of cloud droplets decreased with height. The percentage contribution of small drops showed a very sharp decrease with height up to 5 km and thereafter a slight increase. The percentage contribution of large drops increases with height and it becomes more than the smaller drop concentration just below 3 km. There are many drops with radius412 mm above this height. The effective radius showed a gradual increase in the layers from 1–2 km to 4–5 km. RE is more than 12 mm above the 3–4 km layer and it is more or less the same in these layers. Thus, the existence of bigger cloud drops which in turn initiate the warm rain process supports the observed rain over this region. Fig. 3 shows the concentration of particles of 0.1–3 mm diameters as measured by PCASP averaged over 200 m layers in the vertical in the cloud free regions over all the base stations. The aerosol concentration in the lower layers (below 4 km) is highest over Pathankot (4 1500 cm 3) as observations were taken during the pre-monsoon conditions and least over Bengaluru (o500 cm 3) as this observation period is associated with moist active monsoon conditions. Even though over Bareilly the observations were conducted during the very active moist monsoon conditions under the influence of a monsoon trough, particle concentrations were high below 2 km (4500 cm 3) which are responsible for the formation of haze. Same features were observed over Guwahati below 1 km. The concentration of particles showed a decreasing trend in the higher levels over all the stations. Cloud droplet spectral broadening is an important problem in warm rain processes as it is responsible for the initiation of coalescence. Theoretically condensational growth predicts narrowing of droplet spectra under adiabatic conditions (Rogers and Yau, 1989). Contrary to this theory, in real clouds the standard deviation of the droplet diameters often leads to broadening of droplet spectra (Yum and Hudson, 2005; Yum and Hudson, 2001; 82 S.B. Morwal et al. / Journal of Atmospheric and Solar-Terrestrial Physics 81–82 (2012) 76–85 Politovich, 1993; Martin et al., 1994; Hudson and Yum, 1997). Many attempts have been made to explain the discrepancy between theory and observations (Derksen et al., 2009; Feingold and Chung, 2002; Chaumat and Brenguier, 2001; Brenguier and Chaumat, 2001; Vaillancourt et al., 1998; Shaw et al., 1998; Khain and Pinsky, 1997; Pinsky and Khain, 1997; Beard and Ochs, 1993). Standard deviation (s) and mean radius of the cloud droplet spectra considered in Section 3.1 for different vertical layers over various base stations have been computed. Fig. 4 shows the standard deviation against mean radius, altitude above cloud base and cloud droplet concentration (bottom row, column 1, 2 and 3). It is evident from the bottom row plots that increase in mean radius and cloud depth (i.e., altitude above cloud base) and decrease in cloud droplet concentration is associated with increase in s over all the regions (Yum and Hudson, 2005, 2001; Hudson and Yum, 1997). The cloud droplet spectra broadened with increase in mean radius and cloud depth and became narrow with increasing cloud droplet concentrations. This relationship between s and altitude above cloud base was also observed and reported by Hudson and Svensson (1995), Martin et al. (1994), Politovich (1993), and Nicholls and Leighton (1986). The droplet spectra are very broad over Guwahati in all layers and narrow over Pathankot. Thus, over Guwahati, which was associated with minimum pollution (Fig. 3) and active moist monsoon conditions, cloud droplets were bigger with lower concentrations compared to other stations. Also, over Bareilly, under the influence of the monsoon trough, the cloud droplets were big and growing with altitude but due to the high pollution in the lower layers (blue line in Fig. 3) the concentration of cloud droplets was greater compared to Guwahati at all levels. Over Pathankot due to the presence of very high air pollution (as seen from Fig. 3, the concentration of particles below the cloud base was very high) there are numerous small cloud droplets with narrow cloud droplet spectra at all altitudes (Yum and Hudson, 2001, 2005). The concentrations of small cloud droplets (mean radius 2– 4 mm) was very high just above cloud base over Pathankot (Fig. 4 middle row) compared to that over other stations. In general, the droplet concentration showed decreasing trend with increasing mean radius and cloud depth (middle row column 1 and 2 of Fig. 4). Also the mean radius showed increasing trend with increase in cloud depth over all the base stations (top row in Fig. 4) and is supported by the findings of Yum and Hudson (2001, 2005) and Hudson and Yum (1997). In the lower portion of the cloud mean radius showed maximum increasing trend over Bengaluru, next is Guwahati and minimum is over Pathankot. The vertical variation of cloud droplet effective radius is an important cloud property that manifests both condensation and coalescence growth (Chen et al., 2008). Height variation of RE of cloud droplets over all the five regions is shown in Fig. 5. The solid lines show the regressions. The vertical dotted line represents the RE threshold associated with the initiation of the warm rain process. The height at which the linear fit line intersects the dotted line represents the height of initiation of warm rain Altitude above Cloud base (m) 7000 Pathankot (4545) Hyderabad (2815) Bengaluru (1755) Bareilly (735) Guwahati (1980) 6000 5000 4000 3000 2000 1000 0 Cloud Droplet Concentration (cm -3) 0 2 4 6 8 10 12 14 700 700 600 600 500 500 400 400 300 300 200 200 100 100 0 0 Standard Deviation (µm) 0 2 4 6 8 10 12 0 14 1000 2000 3000 4000 5000 6000 7000 6 6 6 5 5 5 4 4 4 3 3 3 2 2 2 1 1 1 0 0 0 2 4 6 8 10 Mean Radius ( µm) 12 14 0 0 1000 2000 3000 4000 5000 6000 7000 Altitude above cloud base (m) 0 100 200 300 400 500 600 700 -3 Cloud Droplet Concentration (cm ) Fig. 4. Top Row: variation of altitude above cloud base with mean radius (column 1), Middle Row: variation of cloud droplet concentration with mean radius (column 1) and altitude above cloud base (column 2) and Bottom Row: variation of standard deviation (of cloud droplet radius) with mean radius (column 1), altitude above cloud base (column 2) and cloud droplet concentration (column 3) at Pathankot (Black), Hyderabad (Red), Bengaluru (Green), Bareilly (blue) and Guwahati (magenta) during CAIPEEX-2009. The numbers within the bracket after name of the base station indicate cloud base height. (For interpretation of the references to colour in this figure legend, the reader is referred to the web version of this article.) S.B. Morwal et al. / Journal of Atmospheric and Solar-Terrestrial Physics 81–82 (2012) 76–85 processes in these clouds (rain height). Measured RE varied from 1.8 mm to 14.5 mm above all the stations. As the cloud droplets ascend inside the cloud, they grow by condensation but they can also coalesce into larger droplets, both of which will increase RE. The aircraft data presented here shows that RE increases with height inside clouds over all the regions. However, the rate of this increase in droplet size is not the same at all the locations, which is evident from the slope of the linear fit lines. These values are shown in Table 1. From this table it is clearly evident that the growth rate (mm/km) of the RE of cloud droplets with height is less at Bareilly (1.30 mm/km) and Pathankot (1.46 mm/km), intermediate at Hyderabad (1.74 mm/km) and high over Bengaluru (1.99 mm/km) and Guwahati (1.92 mm/km). Even though the growth rate is highest over the Bengaluru region, the effective radius at the cloud base is very much less (1.78 mm). Hence, the 8000 7000 Altitude (m) 6000 5000 4000 Pathankot Hyderabad Bengaluru Bareilly Guwahati 3000 2000 1000 0 0 2 4 8 10 12 14 6 Effective Radius (µm) 16 18 20 83 linear fit line intersects the 12 mm line above 6 km altitude which is above the freezing level. The rain height is 10.4 km, 7.4 km and 6.45 km for Pathankot, Hyderabad and Bengaluru, respectively. For Bareilly and Guwahati it is at 5.5 km and 4.2 km, respectively. This implies that over these stations, above these heights, there is a possibility of initiation of efficient warm rain processes. This level is at very low altitude over Guwahati and at very high altitude for Hyderabad and Pathankot. Therefore, under the then prevailing synoptic/meteorological conditions there seems to be no possibility of initiation of rain over these regions by warm rain processes. The LWC is the mass of the water in a cloud in a specified amount of dry air and is measured per volume of air (g/m3) or mass of air (g/kg) (Bohren and Albrecht, 1998). This variable is important in classification of clouds and is strongly linked to cloud microphysical variables viz. cloud droplet effective radius (RE), cloud droplet concentration (N), and cloud droplet size distribution (Wallace and Hobbs, 2006). Gerber (1996) and Liu and Hallett (1997) showed that for an assumed cloud droplet size distribution, effective radius is proportional to (LWC/N)1/3. Thus, effective radius is directly proportional to cube root of LWC and inversely proportional to cube root of cloud droplet concentration (N). Fig. 5 (bottom) shows the LWC in different layers over various base stations. Over Pathankot LWC is less as RE is less and droplet concentration is more. There is a one to one relationship between RE and LWC over all the stations. For Bengaluru due to the incursion of moisture in the middle levels the RE and LWC both showed increases in the corresponding levels. Thus the aircraft observations described above give insight into the microphysical processes, especially the cloud droplet size distributions over different environments in the Indian tropical region during the southwest monsoon season of 2009. Altitude (m) 8000 7000 4. Summary and conclusions 6000 Aircraft observations of cloud droplet size distributions (DSD), total and percentage contribution of small (radiusr10 mm) and large (radius410 mm) cloud droplets and effective radius (RE) and their height variations over different regions in the tropical Indian monsoon region during May–September 2009 showed the following: Single mode drop size distributions were observed over Pathankot, Hyderabad and Bengaluru regions. DSD spectra showed bimodal distributions over Bareilly and Guwahati regions. DSD spectral width showed height variation, being narrow at lower altitudes (radiuso15 mm) and broadening with increasing height. However, spectra were narrow even at higher levels over Pathankot during the pre monsoon conditions. DSD spectra were very broad at Guwahati and Bareilly under the influence of active monsoon conditions. The increase in width of the spectra can be associated with the existing weather conditions, prevailing pollution and the origin of the air mass (continental/marine). During the pre monsoon conditions (Pathankot) the temperatures were very warm, the cloud base was above 4 km, air was very polluted and the origin of the air mass was 5000 4000 Pathankot (4545 m) Hyderabad (2815 m) Bengaluru (1755 m) Bareilly (735 m) Guwahati (1980 m) 3000 2000 1000 0 0.0 0.5 1.0 1.5 2.0 HW-LWC (g m-3) Fig. 5. Vertical variation of effective radius (RE) (top) and Liquid water content (bottom) over different regions shown with different colors Viz. Pathankot: black, Hyderabad: red, Bengaluru: green, Bareilly: blue and Guwahati: magenta. In the top figure the continuous line with corresponding color represents the linear fit for each region. (For interpretation of the references to colour in this figure legend, the reader is referred to the web version of this article.) Table 1 The number of clouds samples in the updraft regions, cloud base, the effective radius at cloud base, Growth rate of cloud droplets and the height where the linear fit line crosses the 12 mm radius for different stations is given in the table. Base station Date No of samples Cloud base (m) RE at Cloud base (lm) Growth Rate of Cloud drops with height (lm/km) Height where RE 412 mm(km) Pathankot Hyderabad Bengaluru Bareilly Guwahati 28 May 15 June 1 July 24 August 4 September 43 30 45 28 8 4545 2815 1755 735 1980 3.77 4.01 1.78 3.55 7.14 1.46 1.74 1.99 1.30 1.92 10.42 7.42 6.45 5.51 4.26 84 S.B. Morwal et al. / Journal of Atmospheric and Solar-Terrestrial Physics 81–82 (2012) 76–85 super continental (cloud drop radiuso15 mm). Hyderabad associated with subdued monsoon activity also showed narrow and single mode DSD spectra. Over, Bengaluru, though there was incursion of moisture above 700 hPa levels, the DSD spectra showed little widening (cloud drop radius reached up to 20 mm). The clouds were continental in nature at both the locations. The marine originated clouds moved over Bareilly along the monsoon trough which were responsible for widening of the DSD spectra. However, due to heavy air pollution, these clouds did not precipitate below 5.5 km. The DSD spectra were very broad and bimodal over the Guwahati region and this may be due to the prevailing active monsoon conditions and the influence of the cyclonic circulation in the head of the Bay of Bengal (clouding as seen from satellite pictures). The total concentrations of cloud droplets were highest at Pathankot, the possible causes include: (i) this observation period was during the pre-monsoon season, (ii) high pollution and lack of cloud scavenging during the pre-monsoon season. The observed total concentrations were lowest over the Guwahati region. The percentage of small cloud drops is very high up to 7–8 km over Pathankot and minimum over Guwahati. Thus, over Pathankot the nature of the cloud drops showed the influence of continental air masses (negligible contribution of the bigger size drops) and that over Guwahati the influence of marine originated air masses was clearly evident (major contribution of bigger size drops). Over Hyderabad, Bengaluru and Bareilly the percentage contribution of the larger drops increased with height and at some level it became more than the contribution of the small drops, except for Hyderabad. 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