1 Impacts of ENSO events on cloud radiative effects in 2 preindustrial conditions: Changes in cloud fraction and 3 their dependence on interactive aerosol emissions, 4 deposition and transport 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 Yang Yang1, Lynn M. Russell1, Li Xu1, Sijia Lou1, Maryam A. Lamjiri1, Richard C. J. Somerville1, Arthur J. Miller1, Daniel R. Cayan1, Michael J. DeFlorio1, Steven J. Ghan2, Ying Liu2, Balwinder Singh2, Hailong Wang2, Jin-Ho Yoon2, and Philip J. Rasch2 1 Scripps Institution of Oceanography, University of California, San Diego, La Jolla, California, USA 2 Atmospheric Science and Global Change Division, Pacific Northwest National Laboratory, Richland, Washington, USA 20 21 22 23 24 25 26 27 28 29 Key points: • Interannual variability in cloud radiative effects is driven by mid-level and high clouds. • Wind-related feedbacks on natural aerosol emissions enhance this variability by 3– 4%. • Wet scavenging dampens interannual variability by 4-6% over the tropics. 30 31 32 33 34 35 36 37 38 39 40 41 42 43 44 45 46 47 48 49 50 51 52 53 54 55 56 57 Abstract We use three 150-year pre-industrial simulations of the Community Earth System Model (CESM) to quantify the impacts of El Niño–Southern Oscillation (ENSO) events on shortwave and longwave cloud radiative effects (CRESW and CRELW). Compared to recent observations from the Clouds and the Earth’s Radiant Energy System dataset, the model simulation successfully reproduced larger variations of CRESW and CRELW over the tropics. The ENSO cycle is found to dominate interannual variations of cloud radiative effects. Simulated cooling (warming) effects from CRESW (CRELW) are strongest over the tropical western and central Pacific Ocean during warm ENSO events, with the largest difference exceeding 40 Wm–2 (30 Wm–2), with weaker effects of 10–30 Wm–2 over Indonesian regions and the subtropical Pacific Ocean. Sensitivity tests show that variations of cloud radiative effects are mainly driven by ENSO-related changes in cloud fraction. The variations in mid-level and high cloud fractions each account for approximately 20–50% of the interannual variations of CRESW over the tropics and almost all of the variations of CRELW between 60°S and 60°N. The variation of low cloud fraction contributes to most of the variations of CRESW over the mid-latitude oceans. Variations in natural aerosol concentrations explained 10–30% of the variations of both CRESW and CRELW over the tropical Pacific, Indonesian regions and the tropical Indian Ocean. Changes in wet scavenging of natural aerosols dampen more than 4–6% of the variations of cloud radiative effects averaged over the tropics. In contrast, changes in sea spray emissions enhance the variations by 3–4%. 58 59 60 61 62 63 64 65 66 67 68 69 70 71 72 73 74 75 76 77 78 79 80 81 82 83 84 85 86 87 88 89 90 91 92 93 94 95 96 97 98 99 1. Introduction Clouds strongly influence the Earth’s radiation balance. They reflect incoming solar radiation back to space (shortwave albedo effect), which enhances the reflected solar flux by 47.5±3 Wm–2 globally, and absorb outgoing infrared radiation (longwave greenhouse effect), which reduces the outgoing longwave flux relative to clear sky by approximately 26.4±4 Wm–2. Overall, clouds exert a net cooling effect of about –21.1±5 Wm–2 at the top of atmosphere (TOA) (Stephens et al., 2012), which is 6 times larger than that from doubling CO2 concentration (Ramanathan et al. 1989; Loeb et al. 2009). Any changes in cloud properties such as cloud fraction, cloud top height, and microphysical features would perturb cloud radiative forcing and greatly modulate the radiative balance of the Earth system (Slingo, 1990; Wielicki et al. 1998; Curry et al. 2000; Stephens, 2005). The Intergovernmental Panel on Climate Change (IPCC) reported that simulations of clouds and their radiative feedbacks are still one of the largest uncertainties in the fifth-generation climate models (Boucher et al., 2013). On interannual time scales, many regional changes in the global climate system are associated with the El Niño–Southern Oscillation (ENSO) phenomena. ENSO is characterized by anomalous sea surface temperatures (SST) in the equatorial Pacific and has far reaching impacts on global and regional temperature, precipitation, and circulation. Using cloud data from the Extended Edited Cloud Reports Archive (EECRA) from year 1954 to recent years, Park and Leovy (2004) and Eastman et al. (2011) both showed that interannual variations of cloud cover in the tropics have strong correlations to the ENSO index. For example, warmer central and eastern tropical Pacific SST (warm ENSO phase, i.e. El Niño) is associated with increased cloud cover in the tropical central Pacific Ocean and reduced cloud cover over the Indonesian and eastern Pacific regions, and vice versa for cool ENSO phase (La Niña) events. ENSO’s influence on cloud fraction typically varies with height. Zhu et al. (2007) showed that thick low cloud fraction decreased more than 20% in the tropical eastern Pacific during the 1997–1998 El Niño event, which was associated with an upward large-scale motion and a weak atmospheric stability. However, thin high cloud fraction was found to increase over the tropical Pacific and decrease over Indonesian regions during El Niño events compared to those during La Niña events (Norris, 2005; Marchand, 2013). The mean vertical distribution of clouds is also sensitive to ENSO events. Zelinka and Hartmann (2011) and Lelli et al. (2014) reported that during warm ENSO events, the vertical distribution of tropical clouds shifts upward. Due to anomalous tropical atmospheric conditions during ENSO events, cloud radiative effects exhibit year-to-year differences. Moore and Vonder Haar (2001) examined the interannual variability of net cloud radiative effects 100 101 102 103 104 105 106 107 108 109 110 111 112 113 114 115 116 117 118 119 120 121 122 123 124 125 126 127 128 129 130 131 132 133 134 135 136 137 138 139 140 141 from 1984 to 1990 using radiative flux data from the Earth Radiation Budget Experiment (ERBE). They found that during the El Niño season of 1986/87, Pacific basin and global net cloud cooling effects were reduced by 0.90 Wm–2 and 1.29 Wm–2, respectively, compared to those during the La Niña season of 1988/89. Kato (2009) examined the interannual variation of the global radiation budget using the Clouds and the Earth’s Radiant Energy System (CERES) dataset from 2000 to 2004. He found that large anomalies in TOA shortwave and longwave fluxes over the tropical western and central Pacific were associated with changes in ENSO phase, and that clouds are mostly responsible for the observed year-to-year variations. Loeb et al. (2007) also reported that most of the variability in CERES TOA flux is driven by variations in global cloud fraction, as observed using coincident CERES and the Moderate Resolution Imaging Spectrometer (MODIS) data between 2000 and 2005. With CERES data from 2000 to 2010, Dessler (2010) showed that the short-term shortwave and longwave cloud feedback are 0.12 ± 0.78 and 0.43 ± 0.45Wm–2K–1, respectively. The TOA radiation balance is sensitive to cloud heights, since low clouds exert cooling effects on the TOA, while high clouds exert warming effects. However, previous studies have not evaluated the contributions of clouds at different heights to interannual variations of cloud radiative effects. Aerosols are another component of the atmosphere that substantially perturbs the Earth’s radiative balance. Aerosol particles affect the climate system directly by scattering and absorbing solar radiation and indirectly by altering cloud microphysical properties (Twomey 1977; Albrecht 1989; Lohmann and Feichter 2005). Climate variability, such as changes in ENSO phase, can influence the concentrations and distribution of aerosols and trace gases through changing their emissions, deposition and transport (Chandra et al., 1998, 2009; Prospero and Lamb, 2003; Ziemke and Chandra, 2003; Logan et al., 2008; Mitchell et al., 2010; Li et al., 2011; Hsu et al., 2012; Wu et al., 2013; Yang et al., 2014, 2015; DeFlorio et al., 2015; Lou et al., 2015; Xu et al., 2015). Using Sea-viewing Wide Field-of-view Sensor (SeaWiFS) measurements from 1997 to 2010, Hsu et al. (2012) found a high correlation between ENSO Index and monthly AOD anomalies over the Indonesian regions. With MODIS and Global Precipitation Climatology Project (GPCP) data from 2000–2010, Wu et al. (2013) reported that warm ENSO events are associated with aerosol increases over the Indonesian regions resulting from suppressed precipitation, which reduces the wet scavenging of aerosols and promotes dry conditions favorable for fire burning. The influence of ENSO on aerosols is not confined to local tropical Pacific regions. Prospero and Lamb (2003) suggested that increased remote concentrations of Barbados summer dust might be related to warm ENSO events in the previous winter, which promote remote zonal teleconnection 142 143 144 145 146 147 148 149 150 151 152 153 154 155 156 157 158 159 160 161 162 163 164 165 166 167 168 169 170 171 172 173 174 175 176 177 178 179 180 181 182 patterns in atmospheric circulation and precipitation over Africa which favor increased dust emission and subsequent westward transport. Mitchell et al. (2010) also found that Australian dust emission may be enhanced by El Niño-induced dry conditions. Li et al. (2011) retrieved the column-average Ångström exponent from MODIS, the Multiangle Imaging Spectroradiometer (MISR) and SeaWiFS for the period 2000–2011. The Ångström exponent is often used as a qualitative indicator of aerosol particle size. They showed that increases in Ångström exponent over the tropical western Pacific during El Niño events resulted from reductions of sea salt emissions and aerosol transport associated with surface wind anomalies. van der Werf et al. [2006] and Logan et al. [2008] showed that a significant increase in biomass burning emissions occurred because of the enhanced fires in Indonesia during El Niño events. These ENSO-related variations of natural aerosol emissions and concentrations also have potential impacts on the interannual variations of cloud radiative effects. However, few previous studies have considered the role of variations in natural aerosols when investigating interannual variations of cloud radiative effects. Studies which have addressed interannual variations of cloud radiative effects have been constrained by relatively short 10-year satellite data observations, which only contain a few cycles of interannual variability. Consequently, the conclusions drawn from using these datasets are subject to sampling error. Extensive model simulations with realistic ENSO physics can be used to estimating the interannual variations of cloud radiative effects. In addition, the roles of ENSO-related variations in cloud fraction at different heights and variations in natural aerosols due to interactive emissions, deposition and transport can be explored, and can potentially provide a better understanding of climate variability and contribute to improved predictions of tropical climate. We present here a systematic investigation of the interannual variations of cloud radiative effects based on a set of three 150-year simulations in preindustrial conditions using the Community Earth System Model (CESM). We quantify: (1) the observed and simulated interannual variations of cloud radiative effects; (2) their relationship with ENSO events; and (3) the contributions of natural aerosol variability and cloud fraction at various vertical levels to interannual variations in cloud radiative effects. The CESM model and numerical experiments are described in Section 2. Section 3 provides an overview of the simulated interannual variations of cloud radiative effects and comparisons to observations. Section 4 investigates ENSO-related interannual variations of cloud radiative effects by comparing simulations with and without interactive emissions and concentrations of natural aerosols. Section 5 shows the contributions of cloud fractions and 183 184 185 186 187 188 189 190 191 192 193 194 195 196 197 198 199 200 201 202 203 204 205 206 207 208 209 210 211 212 213 214 215 216 217 218 219 220 221 222 223 224 natural aerosols to the interannual variations of cloud radiative effects. Section 6 summarizes these results. 2. Model description and experimental design Simulations in preindustrial conditions were performed using CESM, which includes components from the Earth’s atmosphere, ocean, land, land-ice, and sea-ice (Hurrell et al., 2013). The atmospheric model resolution is 1.9° latitude by 2.5° longitude with 30 vertical layers ranging from the surface to 3.6 hPa. The CESM treats the properties and processes of major aerosol species (sea salt, mineral dust, sulfate, black carbon, primary organic matter and secondary organic aerosol) in the modal aerosol module (MAM3) (Liu et al., 2012). Aerosol size distributions are represented by three lognormal modes: Aitken, accumulation and coarse modes. Mass mixing ratios of different aerosol species and the number mixing ratio are predicted for each mode. Aerosol optical properties are parameterized according to Ghan and Zaveri (2007). The model physically treats the aerosol effects on stratiform cloud microphysics using an up-to-date prognostic method, through droplet activation parameterized in terms of sub-grid updraft velocity, size distribution and volume-mean hygroscopicity of aerosol modes (Abdul-Razzak and Ghan, 2000). The simulated droplet number concentration affects conversion of cloud water to rain through the dependence of the droplet collision and coalescence process on droplet number (Khairoutdinov and Kogan, 2000). A more detailed description of the model aerosol representation can be found in Liu et al. (2012). CESM simulations which include aerosol indirect effects more accurately reproduce the observed time evolution of globally averaged surface air temperatures (Meehl et al., 2013). Stratiform cloud microphysics predicts number and mass mixing ratios of droplets and ice crystals and diagnoses number and mass mixing ratios of rain and snow as described by Liu et al. (2007), Morrison and Gettelman (2008), and Gettelman et al. (2010). The treatment of deep and shallow convective cloud parameterizations is described in Zhang and McFarlane (1995) and Park and Bretherton (2009), respectively. These parameterization schemes convert condensate to precipitation as a function of the local convective mass flux and temperature, without explicit aerosol effects. Cloud macrophysical processes are represented according to Park et al. (2014). To identify the relative roles of variations in cloud fractions and interactive natural aerosol emissions, deposition and transport in interannual variations of cloud radiative effects, the following 150-year simulations are performed: 1. IRUN: the standard simulation of preindustrial conditions using interactive (“I”) emissions, deposition and transport. Emissions, deposition and transport of natural aerosols are allowed to interact with 225 226 227 228 229 230 231 232 233 234 235 236 237 238 239 240 241 242 243 244 245 246 247 248 249 250 251 252 253 254 255 256 257 258 259 260 261 262 263 264 265 266 meteorological fields. 2. ERUN: the sensitivity simulation of preindustrial conditions using prescribed emissions (“E”) of natural aerosols. The emissions of sea salt aerosol used in the simulation are interpolated in time between the 12 monthly mean values derived from the 150-year IRUN simulation, and they are not changed by the actual yearly values of wind and temperature. Hence, this simulation contains no interannual variability of sea salt emissions. However, the emissions of dust aerosol are interactive in this simulation. The model setup conditions are otherwise the same as those in IRUN. 3. CRUN: the sensitivity simulation of preindustrial conditions using prescribed aerosol concentrations. The concentrations of all aerosol components are interpolated in time between the 12 monthly mean values derived from the 150-year IRUN simulation, and they are not changed by interactive processes such as emission, deposition or transport. Hence, this simulation contains no interannual variability of aerosol concentration for all aerosol species. The model setup conditions are otherwise the same as those in IRUN. In this work, we focus on the interannual variations of cloud radiative effects in preindustrial conditions (for the year 1850 emissions), because much of the uncertainty in aerosol indirect forcing arises from uncertainties in natural aerosols (Carslaw et al., 2013). The fire emissions have no interannual variations in any of the simulations. Only regions between 60°S–60°N are analyzed in this study because the cloud radiative effects over the polar regions are highly affected by sea ice and snow (Kato, 2009; Dong et al., 2010). The cloud radiative effect (CRE) is defined as the difference of net downward radiative flux between all sky and clear sky at the TOA, with positive (negative) cloud radiative effect indicating that the cloud warms (cools) the underlying atmosphere and surface (Ramanathan et al. 1989). 3. Simulated interannual variations of cloud radiative effects The observed and simulated annual shortwave and longwave cloud radiative effects (CRESW and CRELW) are shown in Fig. 1. CESM successfully reproduces the observed maximum value of annual CRESW and CRELW over the tropics, as well as large CRESW over the mid-latitude oceans and the subtropical eastern Pacific Ocean. The simulated global climatological mean CRESW and CRELW from IRUN is –51.1 and 24.1 Wm–2, respectively. These values are in agreement with satellite observations (–47.1 and 26.5 Wm–2 from CERES Energy Balanced and Filled (CERES-EBAF; Loeb et al. 2009) and – 54.2 and 30.4 Wm–2 from ERBE (Harrison et al. 1990) for CRESW and CRELW respectively) and multi-model mean values (–51.4 and 26.0 Wm–2 from The 267 268 269 270 271 272 273 274 275 276 277 278 279 280 281 282 283 284 285 286 287 288 289 290 291 292 293 294 295 296 297 298 299 300 301 302 303 304 305 306 307 308 Coupled Model Intercomparison Project Phase 5; Dolinar et al., 2015). For the ERUN and CRUN sensitivity simulations, the spatial distribution and magnitudes of CRESW and CRELW are almost the same as those in the IRUN simulation, with global mean CRESW (CRELW) of –51.5 (24.1) and –50.6 (24.1) Wm–2 from ERUN and CRUN, respectively (Fig. S1). Detailed evaluation of simulated cloud radiative effects from CESM can be found in Park et al. (2014). Standard deviations of observed CRESW and CRELW from CERES-EBAF satellite observations for years 2001–2014 as well as those from model simulations are plotted in Fig. 2. In this work, the standard deviation is used to represent the magnitude of variation, which is calculated with monthly anomalies of CRESW and CRELW for each grid over the 150-yr model record. The standard deviation of simulated CRESW is largest over the tropical western and central Pacific Ocean, the eastern Pacific Ocean, the tropical Indian Ocean, and parts of Europe, eastern Asia, Africa, Australia, North and South America (Fig. 2c), which is consistent with observations (Fig. 2a), with maximum variations exceeding 18 Wm–2. The global (60°S–60°N, hereafter) area-weighted mean value of the simulated CRESW standard deviation computed from monthly anomalies over each grid is 13.2 Wm–2 for preindustrial conditions in IRUN, which is larger than 10.5 Wm–2 from present-day observation. For simulated CRELW, large standard deviation values are located mainly within the tropics, with maximum values over the tropical western and central Pacific and the tropical Indian Ocean (Fig. 2d), which also have a positive bias over the tropics compared to observations (Fig. 2a). The global area-weighted mean value of the simulated CRELW standard deviation in IRUN is 8.4 Wm–2, larger than observed value of 6.8 Wm–2. Overall, the model realistically captures the spatial distribution of observed interannual variations of CRESW and CRELW, with global spatial pattern correlation coefficients of 0.76 and 0.84, respectively. However, the model overestimates the observed variations both in CRESW and CRELW by 23–36% globally. For fixed emissions of sea salt, the global area-weighted mean of standard deviation is reduced by 2–3% for ERUN (Fig. 2e and f) relative to those in IRUN. With fixed aerosol concentrations, the model produces more variations of cloud radiative effects over the tropics, with global area-weighted mean values of simulated standard deviations for CRESW and CRELW of 13.6 and 8.6 Wm–2 (Fig. 2g and h). In order to examine the interannual variations of cloud radiative effects from both observations and simulations for different latitudinal bands, the zonal mean of the standard deviation of simulated and observed CRESW and CRELW are presented in Fig. 3. The model reproduces the observed spatial variability of CRESW and CRELW, with the largest standard deviation over the tropics and decreasing values as the latitude increases. However, the model 309 310 311 312 313 314 315 316 317 318 319 320 321 322 323 324 325 326 327 328 329 330 331 332 333 334 335 336 337 338 339 340 341 342 343 344 345 346 347 348 349 overestimates the observed variations in all simulations, especially over the tropics. The largest variations of simulated CRESW are in the range of 16–17 Wm–2 in IRUN and ERUN and about 19 Wm–2 in CRUN, larger than the observed value of 13–14 Wm–2 from CERES-EBAF. The maximum simulated CRELW variability ranges from 14 to 16 Wm–2, also larger than observed values of 9–10 Wm–2. Notably, the standard deviations of CRESW and CRELW over the tropics from IRUN are reduced compared to CRUN, and the standard deviation simulated from IRUN is more realistic than CRUN, suggesting that variations of natural aerosols play an important role in modulating interannual variations of CRESW and CRELW. Averaged over the tropics (23°S–23°N), the mean standard deviation of CRESW (CRELW) are 15.2 (11.5), 14.8 (11.1), and 16.1 (12.0) Wm–2 in IRUN, ERUN, and CRUN, respectively. With interactive sea salt emissions, the model simulated 3–4% higher variations over the tropics, whereas deposition- and transport-related feedbacks decreased variations of cloud radiative effects by 4–6% relative to the IRUN simulation. 4. ENSO-related interannual variations of cloud radiative effects To explore the interannual variations of cloud radiative effects, we calculated empirical orthogonal functions (EOFs) of yearly anomalies of the simulated CRESW and CRELW. The leading EOF of yearly CRESW and CRELW anomalies for the 150-year IRUN simulation are shown in Fig. 4. The leading EOFs explain 22.5% and 31.4% of the interannual variations of simulated CRESW and CRELW, respectively. The variability is generally largest over regions in the 30°S to 30°N latitudinal band for both CRESW and CRELW. In this region, most of the observed climate variability is associated with ENSO phenomena. The EOF of CRESW shows a negative pattern over the tropical western and central Pacific Ocean, whereas it displays a positive pattern over the Indonesian regions, the eastern Indian Ocean, the tropical eastern Pacific Ocean, the subtropical Pacific Ocean, and the subtropical west coast of North America. The EOF of CRELW shows a similar pattern with opposite sign as that of CRESW. The leading principal components (PCs) that correspond to the leading EOF mode of CRESW and CRELW (shown in Fig. 4) and the time series of the Niño 3.4 Index calculated from the simulated SST are shown in Figure 5a. The Niño 3.4 Index is the averaged SST anomaly over Niño 3.4 region (5°S–5°N, 170–120°W), which is one of several ENSO indicators and is used to characterize the intensity of an ENSO event. The leading PCs are strongly correlated with the Niño 3.4 Index, with correlation coefficients of 0.89 (0.93), which are statistically significant at the 95th percentile. These strong correlations demonstrate that the ENSO cycle has strong impacts on interannual variations of cloud radiative effects. 350 351 352 353 354 355 356 357 358 359 360 361 362 363 364 365 366 367 368 369 370 371 372 373 374 375 376 377 378 379 380 381 382 383 384 385 386 387 388 389 390 391 To further investigate the relationship between the ENSO cycle and interannual variations of cloud radiative effects, we show the power spectrum of the modeled Niño 3.4 Index as well as the leading PCs of yearly CRESW and CRELW anomalies in Fig. 5b. The Niño 3.4 Index shows a significant peak at a frequency of 0.23 cycles per year, suggesting that the simulated ENSO occurs on a time scale of about 4.3 years. It is in the range of the observed ENSO period, which ranges from 2 to 7 years with an average value of approximately 4 years (MacMynowski and Tziperman, 2008). The PCs of the leading EOF of CRESW and CRELW display the same peak of 0.23 cycles per year with the Niño 3.4 Index. This similarity in the cycle frequency indicates that ENSO has a strong effect on the interannual variations of cloud radiative effects between 60°S and 60°N. Spatial patterns of the correlation coefficients between monthly anomalies of CRESW (CRELW) and the Niño 3.4 index are almost the same as the patterns of the EOF, with statistically significant values mainly between 30°S and 30°N, as shown in Fig. 6. Spatial patterns of the correlation coefficients between the PCs of the leading EOF mode of CRESW (CRELW) and SST monthly anomaly also show significant ENSO signal (Fig. S2). These further imply a close relationship between the ENSO cycle and the interannual variations of cloud radiative effects. To quantify the impacts of ENSO events on cloud radiative effects, we show the composite differences in observed and simulated CRESW and CRELW between El Niño events and La Niña events in Fig. 7, in addition to the changes in CRESW and CRELW caused by variations of natural aerosol emissions and concentrations. An El Niño (La Niña) event is characterized by a three month running mean of the monthly Niño 3.4 Index that is above (below) the threshold of +0.4°C (–0.4°C) (Trenberth, 1997). Based on this method, 506 (720) of the 1800 months from the IRUN simulation and 35 (37) of the 168 months from CERES-EREB observations are identified as occurring El Niño (La Niña) events. Relative to those during La Niña events, simulated cooling (warming) effects from CRESW (CRELW) during El Niño events from IRUN are stronger over the tropical western and central Pacific Ocean, with the largest difference exceeding 40 Wm–2 (30 Wm–2) (Fig. 7c and d). Simulated CRESW (CRELW) during El Niño events have weaker cooling (warming) effects than those during La Niña events by 10–30 Wm–2 over the Indonesian regions and the subtropical Pacific Ocean. The pattern of the composite differences in cloud radiative effects agrees with the leading EOF mode pattern (Fig. 4). Compared to the composite differences in observed CRESW and CRELW between El Niño and La Niña events from the CERES-EBAF satellite data (Fig. 7a and b), the model realistically simulates the observed spatial distribution of these differences, although some values over the tropics are over-predicted. Variations in sea salt emissions between El Niño and La Niña 392 393 394 395 396 397 398 399 400 401 402 403 404 405 406 407 408 409 410 411 412 413 414 415 416 417 418 419 420 421 422 423 424 425 426 427 428 429 430 431 432 433 events slightly enhance the cooling (warming) effect of CRESW (CRELW) over the tropical Pacific Ocean and weaken this effect over the Indonesian regions, with magnitudes less than 10 Wm–2 (Fig. 7e and f). The changes of CRESW and CRELW resulting from variations in natural aerosol concentrations (IRUN– CRUN, considering interactive emissions, deposition and transport processes) (Fig. 7g and h) are larger than those due to variations in emissions (IRUN– ERUN). Over eastern Indonesian regions and the tropical western Pacific Ocean, changes in natural aerosol concentrations increase the cooling (warming) effect of CRESW (CRELW) by 10–30 (0–20) Wm–2, whereas the CRESW (CRELW) effect is weaker over the tropical central Pacific Ocean. Observed and simulated composite differences of CRESW and CRELW averaged over the Indonesian regions (90–150°E, 20°S–20°N) and the tropical western and central Pacific Ocean (150°E –120°W, 20°S–20°N) are presented in Fig. 8. Over the Indonesian regions, the composite difference of simulated CRESW (CRELW) between El Niño and La Niña events in IRUN is 7.1 (–7.4) Wm–2. With fixed sea salt emissions, the magnitude of this difference decreases to 4.3 (–5.2) Wm–2 in ERUN. With fixed natural aerosol concentrations, this difference increases to 11.2 (–8.9) Wm–2 in CRUN. Over the western and central Pacific Ocean, the composite difference of simulated CRESW (CRELW) is –6.0 (5.6) Wm–2 in IRUN. The magnitude of this difference also decreases in ERUN and increases in CRUN. These results indicate that variability in natural aerosol emissions is associated with larger differences in cloud radiative effects over the tropics between El Niño and La Niña events, and variations in natural aerosol concentrations dampen these differences. 5. Contributions of ENSO-related cloud fractions and natural aerosols Variations in cloud radiative effects are largely affected by variations in cloud fraction (Loeb et al., 2007; Kato, 2009), which correlate strongly with ENSO patterns in the tropics (Park and Leovy, 2004; Eastman et al., 2011; Zelinka and Hartmann, 2011). The composite differences in observed total cloud fraction between El Niño and La Niña events from MODIS for years 2001–2014, as well as simulated values from the IRUN simulation are shown in Fig. 9a and b. The model realistically reproduces the pattern of larger cloud fraction over the tropical western and central Pacific Ocean and lower cloud fraction over the Indonesian regions during El Niño events relative to those during La Niña events. Over the tropics, a positive ENSO event is associated with larger values of cloud fraction in the tropical western and central Pacific Ocean, likely resulting from the stronger and deeper convection during El Niño events driven by warmer SST. Reduced cloud fraction is found over the Indonesian regions and the tropical eastern Indian Ocean because of increased subsidence likely caused by the shifting of convection to the central Pacific. We also find that the cloud cover over the tropical eastern Pacific 434 435 436 437 438 439 440 441 442 443 444 445 446 447 448 449 450 451 452 453 454 455 456 457 458 459 460 461 462 463 464 465 466 467 468 469 470 471 472 473 474 475 Ocean decreases slightly, which is driven by changes in low stratiform clouds associated with an upward large-scale motion and a weak atmospheric stability (Zhu et al., 2007; Eastman et al., 2011). During a positive ENSO event, total cloud fraction decreases over the southwest coast of North America between 10°N and 30°N, because the warmer sea surface can cause a reduction in marine stratiform clouds (Norris and Leovy 1994; Wyant et al. 1997; Clement et al. 2009). Over the southern Pacific Ocean, the cloud fraction also decreases, possibly as a result of weakened convection associated with decreasing SST over this region. Composite differences between El Niño and La Niña events from the IRUN simulation in simulated low, mid-level, and high cloud fractions, respectively, are presented in Fig. 9c, d, and e. Relative to those in La Niña events, the low cloud fraction during El Niño events decreases over the tropical eastern and central Pacific Ocean, whereas mid-level and high cloud fractions increase over this region, consistent with observations (Norris, 2005; Zhu et al., 2007; Marchand, 2013). Differences in mid-level and high cloud fractions between El Niño and La Niña events are largest between 30°S and 30°N and are similar to differences in total cloud fraction. This suggests that changes in mid-level and high cloud fractions, which dominate the variation of total cloud fraction, have large influences on the interannual variations of cloud radiative effects between 30°S and 30°N (see Section 6). Differences in total, low, mid-level and high cloud fractions between El Niño and La Niña events from the ERUN simulation are similar to those from the IRUN simulation in both spatial distribution and magnitudes (Fig. S3). However, variations in mid-level and high cloud fractions are smaller in CRUN than those in IRUN. This result indicates that although changes in cloud fraction are driven by changes in meteorology, changes in natural aerosol emissions and concentrations also influence cloud fraction and can further perturb cloud radiative effects. Previous findings have identified changes in aerosols as the main drivers of global dimming and brightening (Streets et al., 2009; Ruckstuhl et al., 2008; Cermak et al., 2010). After evaluating the role of changes in SST on variations of marine cloud, Eastman et al. (2011) suggested that changes in aerosol concentrations in the atmosphere could also be a factor influencing cloud fraction. Composite differences of observed and simulated wind fields at 850 hPa between El Niño and La Niña events from the NCEP/NCAR (National Centers for Environmental Prediction/National Center for Atmospheric Research) reanalysis data for years 2001–2014 (Kalnay et al., 1996) and the IRUN simulation are plotted in Fig. 10a and c. During El Niño events, easterly winds are reduced over the tropical Pacific. The sea salt emissions show a similar pattern and decrease over the tropical central Pacific Ocean and increase over the subtropical Pacific Ocean (Fig. 10e), similar to the findings of Xu et al. (2015). Reduced sea salt emissions also cause increased SST 476 477 478 479 480 481 482 483 484 485 486 487 488 489 490 491 492 493 494 495 496 497 498 499 500 501 502 503 504 505 506 507 508 509 510 511 512 513 514 515 516 through the reduction in scattered light (Fig. 10g), which in turn decreases zonal wind (Martensson et al., 2003). The changes in SST further result in the corresponding changes in the cloud fraction (Fig. 10i) and cloud radiative effects (Fig. 7e and f). In addition to emissions, changes in natural aerosol concentrations are primarily driven by wet scavenging and transport processes, which are manifested in the precipitation and wind fields, respectively. The spatial distribution of correlation coefficients between monthly anomalies of sea salt concentrations and monthly anomalies of precipitation rate and zonal winds from the ERUN simulation are compared in Fig. 11. There are significant negative correlations over most ocean regions between sea salt concentrations and precipitation, whereas weaker correlations are found between sea salt concentrations and zonal winds. This difference in correlations could indicate that wet scavenging has a stronger effect on sea salt concentrations than transport. Although dry deposition also plays an important role in determining sea salt aerosol concentrations (Liu et al., 2012), the changes between El Niño and La Niña events in sea salt dry deposition are much smaller than those of wet deposition (Fig. S4). The composite differences in observed and simulated precipitation rate between El Niño and La Niña events from the CMAP (CPC Merged Analysis of Precipitation) dataset for years 2001–2014 (Xie and Arkin, 1997) and the IRUN simulation are shown in Fig. 10b and d. The model adeptly reproduces the observed pattern of increasing precipitation over the tropical Pacific Ocean, with the largest difference of 6-8 mm day-1 over the tropical western Pacific Ocean and decreasing precipitation over the Indonesian regions. These changes in precipitation lead to increases in wet scavenging of sea salt aerosols over the tropical Pacific Ocean and decreases over the Indonesian regions between El Niño and La Niña events (Fig. 10f). Changes in aerosol concentrations associated with wet scavenging process also increase SST through the reduction of scattered light and increased cloud fraction over the tropical western Pacific Ocean, as well as decreased SST and cloud fraction over the Indonesian regions (Fig. 10h and j). These effects result in increases and decreases, respectively, of cloud radiative effects over the tropical Pacific Ocean and over the Indonesian regions (Fig. 7g and h). To estimate the contribution of ENSO-related variations in cloud fractions and natural aerosols to the interannual variations of cloud radiative effects, we used a multivariate regression for both CRESW and CRELW in the IRUN simulation, similar to the approach of Xu et al. (2015). The variations in low, mid-level and high cloud fractions illustrate the contributions of clouds at different heights to cloud radiative effects. The variations in sea salt concentrations are chosen as a proxy for variations in natural aerosols due to 517 518 519 520 521 522 523 524 525 526 527 528 529 530 531 532 533 534 535 536 537 538 539 540 541 542 543 544 545 546 547 548 549 550 551 552 553 554 555 their large role as CCN over the oceans in preindustrial conditions. A general model relating these quantities can be framed in the following form. ( )( ) = + ( )+ ( )+ ( ) ( )+ + where CRESW(t), CRELW(t), CLDLOW(t), CLDMED(t), CLDHGH(t), and SSLT(t) are the annual anomalies of shortwave and longwave cloud radiative effects, low, mid-level and high cloud fractions, and column burden concentration of sea salt. is an error term. The regression coefficients , , , ..., are determined by a least squares fit. The total variance explained by the regressions (R2) are presented in Fig. S5. The regressions account for 80% and 82% of CRESW and CRELW variability, respectively, averaged over regions between 60°S and 60°N, as well as 90% and 86% averaged between 30°S and 30°N. One sensitivity test of the regression model using total cloud fraction instead of low, mid-level and high cloud fractions shows large decreases in R2 from 80% and 82% to 63% and 56% for CRESW and CRELW, respectively. This suggests that the interannual variations of cloud radiative effects depend not only on cloud fraction, but also on cloud height, especially in the longwave bands. Although the changes in liquid water path can also influence the variations of cloud radiative effects (Stanfield et al., 2015), the liquid water path is a function of cloud fraction in the model and it is also perturbed by aerosols. When we included the liquid water path term in the regression model, R2 values are almost the same as those without the liquid water path term. Therefore, we only consider the low, mid-level, and high cloud fractions and the sea salt concentration in the linear regression model. In order to evaluate the contributions of predictors in linear models, we applied the LMG (Lindeman, Merenda and Gold) method (Lindeman et al., 1980; Grömping, 2006). This method provides a decomposition of the model explained variance into non-negative contributions. The estimated fraction of annual variance in CRESW and CRELW explained by the low, mid-level, and high cloud fractions, as well as sea salt concentration using the LMG method, are shown in Fig. 12. Over the tropics, the variations in mid-level and high cloud fraction each account for about 20–50% of the interannual variations of CRESW (Fig. 12c and e). This results from large variations in mid-level and high cloud fractions during ENSO events. In the mid-latitude oceans, the interannual variations of CRESW are primarily driven by low cloud fraction variability (Fig. 12a) due to the important role of marine stratocumulus over these regions. For CRELW, almost all variations between 60°S and 60°N are contributed by the mid-level and high cloud fraction variability (Fig. 12d and f), whereas the low cloud fraction variability exerts little effect (Fig. 12b) since CRELW are primarily driven by mid-level and high clouds. The variation in sea 556 557 558 559 560 561 562 563 564 565 566 567 568 569 570 571 572 573 574 575 576 577 578 579 580 581 582 583 584 585 586 587 588 589 590 591 592 593 594 595 596 597 salt concentration (including interactive emissions, deposition and transport processes) explains 10–30% of the interannual variations of both CRESW and CRELW over the tropical Pacific Ocean, the Indonesian regions, and the tropical Indian Ocean (Fig. 12g and h). Although wet scavenging of natural aerosols dampens interannual variations in cloud radiative effects, simulated variations are larger than those from the present-day observations, especially over the tropics (Fig. 3). He et al. (2015) found CESM overestimated observed precipitation over 30°S–30°N compared to the data from GPCP, possibly leading to under-prediction of natural aerosols over the tropics. By comparing to MODIS-derived CCN data, Gantt et al. (2014) also found CESM under-predicted 66.7% of column CCN globally. Due to this underestimation of aerosol concentrations, the dampening role of variations in natural aerosols may be underestimated as well, which might explain why the model overestimates the variations of cloud radiative effects over the tropics. On the other hand, it is worth noting that observations are at the present-day conditions for only 14 years from 2001 to 2014, which is a constraint on studying interannual atmospheric variations in a robust way. Furthermore, present-day observations may not fully represent the variability in cloud radiative effects at preindustrial conditions. 6. Conclusions 150-year simulations in preindustrial conditions with the CESM model showed interannual variations of cloud radiative effects with features that are characteristic of the El Niño–Southern Oscillation (ENSO) events. The interannual variations of shortwave and longwave cloud radiative effects at the top of atmosphere (CRESW and CRELW) are quantified using standard deviation values. The model produces large variations in CRESW over the tropical western and central Pacific, the eastern Pacific, the tropical Indian Ocean, as well as parts of Europe, eastern Asia, Africa, Australia, North and South America, similar to what is observed in CERES observations, with maximum variations exceeding 18 Wm–2. The large variations of CRELW are located mainly within the tropics. The global area-weighted mean standard deviations of CRESW and CRELW are 13.2 and 8.4 Wm–2, respectively. Both of these values are larger than the observed values of 10.5 and 6.8 Wm–2 in present-day conditions. Using EOF analysis, the leading PCs of simulated CRESW (CRELW) are strongly correlated with the ENSO index. Correlation coefficients between the Niño 3.4 Index and the leading PCs of CRESW (CRELW) are 0.89 (0.93). Using spectral analysis, the power spectrum of the leading PCs of CRESW (CRELW) showed the same peak with the Niño 3.4 Index at the frequency of 0.23 cycles per year, about 4.3 years per cycle. These results demonstrate that the ENSO is the only detectable cycle in the interannual variations of cloud radiative 598 599 600 601 602 603 604 605 606 607 608 609 610 611 612 613 614 615 616 617 618 619 620 621 622 623 624 625 626 627 628 629 630 631 632 633 634 635 636 637 638 639 effects in the preindustrial atmosphere simulated by CESM. Relative to those during La Niña events, simulated cooling (warming) effects from CRESW (CRELW) during El Niño events are stronger over the tropical western and central Pacific Ocean, with the largest difference exceeding 40 Wm–2 (30 Wm– 2 ). In contrast, the cooling (warming) effects are weaker by 10–30 Wm–2 over the Indonesian regions and the subtropical Pacific Ocean. The changes in cloud fraction are found to be mainly responsible for the variations of cloud radiative effects between El Niño and La Niña events. In a positive ENSO event (El Niño), the cloud fraction increases in the tropical western and central Pacific Ocean and decreases over the Indonesian regions, the tropical eastern Indian Ocean, the eastern Pacific Ocean, the southwest coast of North America and the southern Pacific Ocean. Relative to those in La Niña events, the low cloud fraction during El Niño events decreases over the tropical eastern and central Pacific Ocean, whereas mid-level and high cloud fraction increases over this region, consistent with observations. Wind-related changes in sea salt emissions, transport and precipitation-related changes in wet scavenging are found to contribute to the variations in sea surface temperature and cloud fraction. Variations in sea salt emissions between El Niño and La Niña events slightly enhance the cooling (warming) effect of CRESW (CRELW) over the tropical Pacific Ocean and weaken this effect over the Indonesian regions, with magnitudes less than 10 Wm–2. The cooling (warming) effects of CRESW (CRELW) are also enhanced by 10–30 (0–20) Wm–2 over the eastern Indonesian regions and the tropical western Pacific Ocean, whereas the CRESW (CRELW) are weaker over the tropical central Pacific Ocean, mainly resulting from variations in wet scavenging of natural aerosols. These indicate that the variations in natural aerosol emissions enhance 3–4% of variations in cloud radiative effects over the tropics, and the variations in natural aerosol concentrations resulting from wet scavenging process dampen these variations of CRESW (CRELW) by 4– 6%. The LMG method for the linear model used here suggests that the variability in mid-level and high cloud fractions each account for about 20–50% of the interannual variations of CRESW over the tropics and almost all of the interannual variations of CRELW between 60°S and 60°N. In the mid-latitude oceans, the interannual variations of CRESW are primarily driven by low cloud fraction variability. The variations in sea salt concentrations caused by interactive emissions, deposition and transport processes explain 10–30% of the interannual variations of both CRESW and CRELW over the tropical Pacific Ocean, the Indonesian regions, and the tropical Indian Ocean. The combination of simulations with fully interactive aerosol, climatological mean emissions, and climatological mean concentrations could also be used 640 641 642 643 644 645 646 647 648 649 650 651 652 653 654 655 656 to investigate the role of feedbacks of other aerosol sources with climate variability, such as dust, dimethyl sulfide and carbonaceous aerosol from wild fires. Acknowledgments. This research was supported by NSF AGS1048995 and by DOE DE-SC0006679 as part of the U.S. Department of Energy, Office of Science, Biological and Environmental Research, Decadal and Regional Climate Prediction using Earth System Models (EaSM) program. 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Global area-weighted mean values of cloud radiative effects are presented at upper right corner of each panel. Figure 2. Standard deviation of observed (a) shortwave and (b) longwave cloud radiative effects from Clouds and the Earth’s Radiant Energy System Energy Balanced and Filled dataset (CERES-EBAF) for years 2001–2014, and standard deviation of simulated (c, e, g) shortwave and (d, f, h) longwave cloud radiative effects from IRUN, ERUN and CRUN using CESM model. Global (60°S–60°N) area-weighted mean of standard deviations computed from monthly anomalies for each grid boxes are given at the upper right corner of each panel. Figure 3. Observed and simulated zonal mean of standard deviation of (a) shortwave and (b) longwave cloud radiative effects. Black line represents values from CERES-EBAF observations. Red, green and blue lines represent values from IRUN, ERUN and CRUN of CESM model simulations. Figure 4. The leading EOF mode of simulated yearly (a) CRESW and (b) CRELW from IRUN simulation. The variance explained by the leading mode EOF is given at the upper right corner of each panel. Figure 5. (a) The time series of principal components (PCs) of leading mode EOF (corresponding to EOF in figure 3) of simulated CRESW (blue line) and CRELW (green line) and Niño 3.4 Index (red line). (b) The power spectrum of PCs of EOF of simulated CRESW and CRELW and power spectrum of Niño 3.4 Index. Correlation coefficient between Niño 3.4 Index and PCs of EOF of CRESW/CRELW is shown in the top-right corner of the each left panel. The corresponding dashed lines in the right panel indicate the 95% significance levels. CRESW, CRELW and Niño 3.4 Index are computed from IRUN simulation. Figure 6. Spatial distribution of the correlation coefficients between month anomalies of (a) shortwave and (b) longwave cloud radiative effects and monthly Niño 3.4 Index. Cloud radiative effects and Niño 3.4 Index are computed from IRUN simulation. The dotted areas indicate statistical significance with 95% confidence from a two-tailed Student’s t test. Figure 7. Composite differences in (a, b) observed and (c, d) simulated CRESW (left column) and CRELW (right column) from CERES-EBAF satellite data and IRUN simulation, as well as the effects of changes of these differences due to changes in (e, f) natural aerosol emissions (IRUN–ERUN) and (g, h) concentrations (IRUN–CRUN) on CRESW and CRELW between El Niño and La Niña events. Observed monthly Niño 3.4 Index are calculated using surface air temperature from NCEP/NCAR (National Centers for Environmental Prediction/National Center for Atmospheric Research) reanalysis data. The location boxed (90–150°E, 20°S–20°N and 150°E – 120°W, 20°S–20°N) selected to capture the features of changes in CRESW and CRELW in Indonesian Regions and the tropical eastern and central Pacific between El Niño and La Niña events from different simulations is also shown in (a). Figure 8. Composite differences in simulated CRESW (top) and CRELW (bottom) over Indonesian region (IR, 90–150°E, 20°S–20°N) and the tropical eastern and central Pacific (TP, 150°E –120°W, 20°S–20°N) between El Niño and La Niña events from CERES-EBAF dataset, and IRUN, ERUN, and CRUN simulations. Figure 9. Composite differences in (a) observed and (b) simulated total cloud fraction and simulated (c) low (d) mid-level and (e) high cloud fraction between El Niño and La Niña events. Low, mid-level and high cloud are cloud in pressure range of 1200–700, 700–400 and 400–50 hPa, respectively. Observed cloud fraction are from the Moderate Resolution Imaging Spectrometer (MODIS) for years 2001 to 2014. Simulated cloud fraction are from 150-year IRUN simulation. Figure 10. Composite differences in wind field at 850 hPa from (a) NCEP/NACR reanalysis dataset and (c) IRUN simulation, as well as differences in (b) observed and (d) simulated precipitation rate from CMAP data and IRUN simulation between El Niño and La Niña events. The corresponding composite differences in sea salt (e) emissions and (f) wet scavenging between El Niño and La Niña events in IRUN, and the associated changes in changes in (g, h) sea surface temperature (SST) and (i, j) total cloud fraction (CLDTOT) caused by changes in emissions and concentrations between El Niño and La Niña events. CMAP and NCEP/NACR data are used for years 2001–2014. Figure 11. Correlation coefficients between monthly anomalies of sea salt concentrations and (a) monthly anomalies of precipitation rate and (b) zonal winds from ERUN simulation. The dotted areas indicate statistical significance with 95% confidence from a two-tailed Student’s t test. Figure 12. The LMG method for estimated fraction of annual variance in CRESW (left column) and CRELW (right column) explained by (a, b) low, (c, d) mid-level, and (e, f) high cloud fraction, and (g, h) sea salt concentrations from IRUN simulation.