DRAFT IMECE '02 ASME International Mechanical Engineering Congress & Exposition November 17–22, 2002, New Orleans, Louisiana Proceedings of IMECE'02 ASME International Mechanical Engineering Congress & Exposition 2002 November 17-22, 2002, New Orleans, Louisiana, November 17-22, 2002 IMECE2002-xxxxx IMECE 2002 33918 T U R B U L E N C E - R A D I A T I O N INTERACTIONS IN FLAMES: A C H A O T I C - M A P BASED FORMULATION Ying Xu 1 J. M. McDonough 2 M. Pinar MengSc: 3 Department of Mechanical Engineering University of Kentucky Lexington, KY 40506-0108 Department of Mechanical Engineering University of Kentucky Lexington, KY 40506-0108 Department of Mechanical Engineering University of Kentucky Lexington, KY 40506-0208 ABSTRACT Pe qR R Re ~' Sc T u U v In this paper we report initial efforts in developing largeeddy simulation (LES) subgrid-scale (SGS) models capable of treating turbulence-radiation interactions in sufficient detail to permit calculation of radiation intensity fluctuations on small scales. These models are constructed with a fluctuating component consisting of a discrete dynamical system (chaotic map) and are thus completely deterministic. We present an outline of the development of this formulation and then employ experimental data to generate large-scale behavior permitting what might be viewed as part of an a priori test of the SGS model. We display spatially extensive instantaneous fluctuating temperatures produced by the model as well as time series of fluctuating intensity calculated from the radiative transfer equation at several heights in a pool fire. We conclude that such results are physically realistic (and very efficiently computed) and warrant continued investigations, but we have at this time not yet completely validated the approach due to lack of detailed laboratory data. a fl # ~, p r NOMENCLATURE CB Di FB Gr I~, k L p specific heat binary diffusion coefficient body force Grashof number spectral intensity thermal conductivity length scale pressure P~clet number thermal radiation specific gas constant Reynolds number radiation propagation direction chemical source temperature u velocity component referenced velocity magnitude v velocity component mass fractions of species i thermal diffusivity thermal volumetric expansion coefficient anisotropy correction dimensionless temperature absorptivity dynamic viscosity kinematic viscosity density time scale INTRODUCTION Most industrial scale flames are strongly radiating and turbulent in nature; they can be viewed as time dependent dynamical systems. Turbulence-radiation interactions (TRI) need to be accounted for thoroughly in such flames in order to include the underlying physical mechanisms. Numerical modeling of turbulent diffusion flames requires at least qualitatively accurate simulation of small-scale fluctuations of velocity, temperature, and concentration fields, in addition to the corresponding large-scale values. Most 1Ph.D Student 2Professor; jmmcd@uky.edu 3Professor; mengucQengr.uky.edu 1 Copyright (~) 2002 by ASME of the time-dependent information is lost if flow field simulations are not carried out in detail. Even though some modern techniques such as the direct numerical simulation (DNS) are mathematically rigorous and do yield a high level of accuracy, they are not computationally feasible for application to complex practical systems. Instead, it is preferable to "model" the small-scale fluctuations and solve for the large-scale parameters accurately. This strategy (largeeddy simulation, LES) allows us to save significant amounts of CPU time, and brings us to the realm of simulating turbulent flames of practical importance. The first attempt to include effects of radiation on flow and temperature fields in a turbulent environment was made by Townsend [1]. Later studies included those by Cox [2], Tamanini [3], Kabashnikov and Myasnikova [4], Grosshandler and Joulain [5], Fischer et al. [6], Fischer and Grosshandler [7], as well as Faeth and his students (see Gore et al. [8] [9], and Faeth et al. [10] for an overview). One of the earliest accounts of TRI in the heat transfer literature is that by Song and Viskanta [11] who investigated a turbulent premixed flame inside a two-dimensional furnace. More recently, Gore et al. [12] and Hartick et al. [13] solved the problem for diffusion flames using a k-a model. They discussed a closure for the governing equations and correlated gas radiative properties using probability density function (PDF) of mixture fraction and total enthalpy. Mazumder and Modest [14] used a velocitycomposition PDF method to investigate TRI; the so-called P D F / M o n t e Carlo method they developed was accurate, yet computationally demanding. Li and Modest [15] used a similar approach; they assumed the species concentrations and temperature/enthalpy are the random variables and applied this to a methane-air diffusion flame. It is now widely believed that turbulence in a flow field is not random, but deterministically chaotic in light of the seminal work of Ruelle and Takens [16]. Moreover, it is possible to model the turbulent fluctuations via numerical time series calculated from a linear combination of chaotic maps, with different parameters and weights (see, e.g., McDonough et al. [17]) with the maps derived from the governing equations (see McDonough and Huang [18], and Yang et al. [19]). Here, we will present an analysis that investigates TRI using a system of chaotic maps. Fluctuations of absorption coefficient will be calculated as a function of temperature modeled in terms of these maps, and the emission from flames will be quantified in terms of parameters of the chaotic maps. The concept of chaotic-map based TRI has been discussed before by Mengfi~ and McDonough [20], McDonough et al. [21], Mengfi~ and McDonough [22], and details of the chaotic map formulation were reported elsewhere (Mukerji et al. [231; Hylin and McDonough [24]). Our focus in this paper is on the effect of chaotic map induced fluctuations on radiation emission at various locations in a flame, which can be measured experimentally. We follow this introduction with a fairly detailed section containing the mathematical formulation of the governing equations, an overview of typical treatments of turbulenceradiation interactions, and the formalism based on chaotic maps (discrete dynamical systems, DDSs) that we will employ. We then present and discuss results of applying DDSs in the context of a pool fire flame studied by Weckman and Strong [25]. Conclusions drawn from this initial study are then presented, the main one being that the use of chaotic maps as subgrid-scale (SGS) models provides a rational approach to efficiently introducing physically-realistic behavior on subgrid scales, but considerable research is still needed to develop this into a predictive tool. FORMULATION AND ANALYSIS We begin this section with introduction of the system of governing equations needed for the complete discription of combustion physics. Then we provide a brief treatment of past approaches to accounting for turbulence-radiation interactions, indicating their shortcomings. Following this we state and justify the assumptions to be employed for the present study and present the chaotic map formalism. Governing Equations The equations governing most combustion processes consist of the Navier-Stokes (N.-S.) equations in a form appropriate for non-constant density (but low-Mach number) flows, a thermal energy equation and species concentration equations, along with an equation of state. These can be expressed as p, + v . ( p u ) = 0, (la) D(pU) Dt-- - V p + # A U + FB, (lb) DT p C p - ~ - = k A T + V "qR + So, (lc) D(pYi) D--T- - V . Di~7(pYi) + &i, i = 1,..., Ns. (ld) In these equations U K (u, V) T is the two-dimensional velocity vector; p, p, T are, respectively pressure, density and temperature related through an equation of state, say p = p R T , with R being the specific gas constant. Tile Yi are mass fractions of species i, and cbi are corresponding 2 Copyright (~) 2002 by ASME species production terms. FB, Sc and qR are, respectively body force, chemical source and thermal radiation contributions to momentum and thermal energy, and #, k, D~ and Cp are transport and thermodynamic properties: (dynamic) viscosity, thermal conductivity, binary diffusion coefficient and specific heat, respectively. Finally, the differential operators D~, V and A are the usual substantial derivative, gradient and Laplacian, respectively, in a chosen coordinate system. Further details can be found in, e.g., Libby and Williams [26]. the chemical source term in Eq. (lc), but report that their approach is not computationally feasible for anything but the simplest kinetic models. Hence, no details of effects of species concentration can be deduced, although more global effects of TRI are produced. It is important to recognize, however, that there is no true instant-to-instant interaction between the velocity field and the temperature field, and thus no detailed turbulence-radiation interaction. Such details cannot be produced when the governing equations are averaged (RANS) or filtered (usual LES), and then closed with statistical models representing phenomena on precisely the scales at which the interactions must occur. Treatments for TRI At present the main alternatives available for analysis of radiating turbulent flows are DNS, RANS and LES, with the latter two often coupled with PDF methods, specifically to treat chemistry and/or radiation (see, e.g., [27]). It is not hard to check that DNS is not possible for simulation of large-scale practical problems due to the O(Re 3) arithmetic operation scaling for fluid flow alone. Formally, LES and RANS are similar, although the details of LES are more rigorous. Furthermore, the ~ O ( R e 2) arithmetic required by LES will be feasible on the next generation of parallel supercomputers, and probably LINUX clusters, up to Re at least 106 . The starting point for treatment of radiation is the radiation transfer equation (RTE) consisting of the radiant energy balance for a non-scattering, absorbing-emitting gas confined to a solid angle d~t within a spectral interval [I, 1 + d l ] : (K" V)Ix = ~X[/bx(T) -/~], Chaotic Map Subgrid-Scale Models The principal difficulty in all approaches to turbulence (except DNS) is dealing with the "closure problem." What seems not to have been recognized is that the most difficult (and least sound from a pure mathematical viewpoint) aspects of this problem would never have occurred had we not averaged (or, in the LES case, filtered) the governing equations. This process results in a need for statistical models that inherently suffer from a basic mathematical inconsistency: the mapping from physics to statistics is many-to-one, implying that it is noninvertible. Yet, it is precisely an attempt to invert this mapping that is embodied in every RANS approach, and in most (but not all) LES techniques; namely, attempt to use statistics (velocity correlations, velocity-temperature correlations, etc.) to deduce physics (velocity, temperature and composition fields). Thus, the context into which we will introduce chaotic map models is a modification of LES based on the following key ideas: i) filter solutions rather than equations; ii) model physical variables instead of their statistical correlations; iii) directly use model results to enhance the (deliberately) under-resolved large-scale solutions of LES, rather than discarding these results. Within this context we can still employ the usual LES decomposition: (2) where ~is the radiation propagation direction; ~x is absorptivity at wavelength I, and Ix is the corresponding spectral intensity. The formal solution to Eq. (2) is (Viskanta and Mengfi~ [28]; Modest [29]) Ix(s, t) = Ioe- fo~~(s',t)ds'+ Q(x,t)=q(x,t)+q*(x,t), ~0 8 (8', t)Ibx (T(< t)) el.'s ' (3) x E F ~ ~, d = 2 , 3 (4) with q representing large (computed) scales, and q* denoting the small scales that must be modeled, of any dependent variable vector Q = (Q1,Q2,"" ,QN,) T, where Nv is the number of variables. In earlier work (e.g., McDonough and Bywater [30] [31]) components of q* were obtained as solutions to low-dimensional systems of ordinary differential equations (ODEs) corresponding to high-wavenumber Fourier modes arising from a Galerkin procedure applied to the small-scale system of additively split partial differential equations (PDEs). But beginning with McDonough et al. where I0x is radiation intensity incident at the boundary (s'= 0) of the medium. It should also be noted that ~x depends on temperature and species concentrations in a nontrivial way, so Eq. (3) is considerably more complicated than is explicitly apparent. In turn, this shows that application of Reynolds averaging to Eq. (2) leaves the entire right-hand side unclosed. Li and Modest [15] describe the use of a PDF formalism to treat both the radiation source term and 3 Copyright (~) 2002 by ASME 1 [32] the solution ansatz q* = A ( M , ut + uuz + vu u = ~ e A u , (6a) 1 Gr vt + uv~ + vv u = ~eAV - ~e20, (6b) Ot + uO~ + vOu = ~--~eAO. (6c) (5) was introduced. Here, A is an amplitude factor computed via Kolmogorov scaling (see, e.g., Frisch [33]; ~ is an anisotropy correction obtained from scale similarity, as employed in the dynamic SGS models of Germano et al. [34]; the factor M is analogous to Kolmogorov's stochastic variable, but in the present context is a deterministic discrete dynamical system. These ideas are implicitly contained in [32], and much of the theory required for modeling subgrid-scale physical variables is presented in [24]. Furthermore, many of these ideas were applied specifically to the TRI problem in [22]. In these earlier studies, chaotic maps having no particular connection to the appropriate physics were employed (to some extent successfully) as subgrid-scale models. More recently, McDonough and Huang [18] [35] have devised a method whereby discrete dynamical systems (i.e., chaotic maps) can be derived directly from the governing PDEs of essentially any physical system. To date these have been studied in a comparison of free and forced convection (McDonough and Joyce [36]) and in association with three different H2-O2 and H2-air kinetic mechanisms (McDonough and Zhang [37] [38]; Zhang et al., [39]). But in all of these studies emphasis has been placed on the time series of SGS behavior at a single spatial location; moreover, the bifurcation parameters needed to evaluate the DDSs were chosen somewhat arbitrarily. In the present study we employ experimental data from a spatially extended set of measurements for a pool fire to automatically set required bifurcation parameters over the entire physical domain of the experiments. To keep the problem at a relatively simple level we will not model Eq. (ld) for the species mass fractions. Hence, the chemical source term in Eq. (lc) will be ignored (but see the above cited references for treatments of this). Furthermore, because the pool fire of the Weckman and Strong [25] data is burning methanol, and soot formation will be at a relatively low level, we also ignore the radiation source term in Eq. (lc) - - despite its general importance. This permits us to focus on the effects of fluctuating temperature in producing radiation intensity fluctuations without needing to separate the feedback from thermal radiation via the radiation source term in Eq. (lc). Thus, as in [36] we employ the following system of 2-D equations, utilizing the Boussinesq approximation to obtain the form of the body force term in Eq. (lb) and Leray projection [40] to remove the pressure gradient from this equation. This produces the following system written in dimensionless form: Here G r is the Grashof number, R e the Reynolds number and P e the P~clet number: G r _= I~g6TL 3 u~~ , R e =- UL , Pe ~ V UL , (7) C~ where a is thermal diffusivity, /3 is thermal volumetric expansion coefficient, and u is kinematic viscosity. The velocity components (u, v) have been scaled with a reference velocity magnitude U, and distances are scaled by a fixed length scale L. The dimensionless temperature is defined as T-To 0 =- Ti- ~ 0 ' (8) where To and T1 are reference temperatures, and ~T = T1 To. The subscripts x, y, t denote partial differentiation with respect to the spatial coordinates (x,y) and time t respectively, and A is the Laplacian. We apply the Galerkin procedure to this system and represent all dependent variables by Fourier series as (9a) u(x, y, t) = E ak (t)~ok (X, y), k (9b) v(x, y, t) = E b} (t)~k (X, y), k O(x, y, t) = E (9C) ck(t)cpk(X, y). k Application of the Galerkin procedure consists of substituting Eqs. (9) into Eqs. (6), and then computing inner products with each of the countably infinite (pks. The result of this (see [36]) is reduced to /~+ A(1)a 2 + A ( 2 ) a b - + B(1)b2 + B(2)ab _ C[k[2 b _ d 4- C(1)ac 4- C(2)bc 4 Clkl 2 R e a, Re Gr ~ 7c' Clkl~ ~e c, (10a) (10b) (10c) Copyright @ 2002 by ASME by retaining only a single Fourier mode. Eqs. (10a, b) have been treated in detail in [18] without the buoyancy term on the right-hand side of (10b). The process introduced in [36] consists of a forward Euler numerical integration of the ODEs (10a,b), with backward Euler applied to (10c), leading to a (~+1) = 81a (n) ( 1 - a (n)) -'Tla(n)b (n), (lla) b(~+1) : 82b (~) ( 1 - b (~)) - 7 2 a ( n ) b (n) +aTC(n), (llb) It should be noted that Eq. (11c) is linear in c, implying that unless a reference level is prescribed, the DDS will either approach zero or infinity after sufficiently long time. This is remedied with the term Co, which is set by the high-pass filtered resolved-scale solution in the context of a complete LES implementation. In the present study, it is assigned a fixed value. Choosing Parameter values In the preceding subsection, we introduced numerous bifurcation parameters. Here, we describe the assignment of their values• Since natural convection is important in a pool fire, aT is assigned the value 0.06 rather than 0 used in the case of forced convection. In addition, co = 0.1 and ~T : 0.5 are chosen• The relation of 81 and 82 to the Reynolds number gives us the rationale to choose 8 = 81 = 82 such that 8 increases in radial and axial directions. Values of '71, '72, ~uT and ")'vT are related to rescaled Uy, vx, Ty and Tx, respectively• T h e absorption coefficient n is determined by using Planck-mean absorption coefficients of CO2 and H20 (see [29])• The ranges of absorption coefficients for C02 and H20 in the current temperature field are 0.146--0.324cm -1 and 0.031--0.078cm -1 respectively. Hence, we estimated n = O.lcm -1 as the large-scale absorption coefficient of mixture. We also assume the absorption coefficient is a function only of temperature, so the small-scale absorption coefficient can be determined by fluctuating temperature. Therefore, radiation intensity is computed by directly integrating Eq. (2). c (n+l) : (1-- ~uTa(n) -- ~vT b(n)) / ( 1 + S T ) +CO- ( l l c ) We remark that Eqs. (11) can be viewed as the simplest possible shell model (see Bohr et al. [41]); it consists of a single Fourier mode for each original P D E (similar to the well-known Lorenz equations [42]). But in contrast to those, the single mode is arbitrary, with the mode number embedded in the bifurcation parameters. One might question the accuracy, even validity, of a single mode representation, but we emphasize that these representations are local. Hence, one should expect that at most a few modes would be needed to capture the local physics. Indirect evidence of this can be seen in [23] and more recently, and more directly, in Yang et al. [19] in which Eqs. ( l l a , b) are directly fit to high-pass filtered (hence, analogous to subgrid scales) experimental data for two velocity components measured via LDV. Considering the physical meaning of the various 8s and 7s in Eqs. (11), it is shown in [18] that both ~l and 82 are related to the Reynolds number via ~=4 1 Re ]' RESULTS AND DISCUSSION Our main overall objective in this research program is to devise a high-fidelity model for the small-scale behavior of radiating turbulent flames. Such a model will allow us to predict the fundamental physical and chemical phenomena that take place in a flame, and availability of such a model is likely to allow us to control such flames more effectively. To this end, we propose to represent the small-scale fluctuations with chaotic maps, as discussed above. Here, we will present a series of results that model temperature and radiation intensity fluctuations as observed outside the flame• We will discuss the affect of chaotic map parameters on these results and comment on the robustness of the approach. Below, we will present fluctuating temperature contours for two different amplitude factors (see Eq. 5). Physically, these factors are simply the magnitude of the energy contained in the unresolved scales, local in space and time. Using these factors, we obtain the temperature fluctuations within the entire domain. After that, we calculate the radi- i=1,2, and since we have based our derivations on a single wavevector k it is natural to set j31 = j32. By comparing Eqs. (10) and (11) one sees that 8T = TCIkl 2 Pe ' also, aT vGr Re 2 In these equations, C is a normalization constant (set to unity in the present case), and 7 is a time scale. The various 7s all correspond to gradients of the velocity vector and the temperature• These are obtained from the Galerkin triple products that produce the coefficients A (i), A (2), etc., appearing in Eqs. (10) in combination with numerical time step parameters to produce 71, 72, 7~T, %T of Eqs. (11). 5 Copyright (~) 2002 by ASME ~o ation intensity time series that can be measured at different flame heights. The intensity fluctuations are a direct manifestation of radiation-turbulence interactions. In a typical turbulent flow field simulation, small-scale calculations are the most time consuming and usually the least accurate. If these calculations can be replaced with reasonably accurate ones that can be obtained faster and more reliably, more accurate flow field simulations can be realized. This requirement is particularly important for chemically reacting flows, where radiation, turbulence and chemical kinetics interactions need to be accounted for. In order to perform the chaotic map based calculations in lieu of more detailed differential equation based smallscale simulations, we need to have spatially extended resolved scale velocity and temperature fields. These can be obtained from any available computational or experimental source, e.g., resolved-scale LES results. In this study, we chose to use data from Ref. [25]. Time-averaged axial and radial velocity data reported in [25] were read directly from the figures and then interpolated. Readings from the experimental data plots were obtained on a 17 × 10 grid; then via (linear) interpolation the grid resolution was increased to 33 × 19. The corresponding velocity profiles are depicted in Fig. 1. The same approach was carried out for the mean temperature profile, and plotted in Fig. 2a. By obtaining the entire velocity and temperature fields, we are able to estimate the velocity and temperature gradients at every location in the flame. These gradients are directly used to calculate the bifurcation parameters, ~ , '~2, ~uT, ~vT at every point of the computational grid as indicated in the previous section. Results for the instantaneous fluctuating temperature are displayed in Figs. 2b and 2c. This is the first time these maps (see Eqs. 11) have been used in a spatially extended simulation. In the past, time series were constructed only at single points. This provides a proof of concept of the overall discrete dynamical systems approach to subgrid-scale modeling, and the results presented here can be viewed as a first step in what is often termed a priori testing of SGS models. Here, however, we have employed experimental data rather than DNS results. Noting that the Reynolds number, defined based on unit height, is increasing along the flame axis, we choose a value of/313(=/31= / 7 2 ) , and then (linearly) increase it along the flame. Figure 3 depicts fluctuating intensity time series as computed at different heights in the flame. Four different cases are plotted, corresponding to different ranges of the bifurcation parameter/3. Fig. 3a shows that for low/3 values, (i.e., low Re) changing from 2.7 at the base to 2.9 at the flame tip produces no fluctuations in intensity at any flame height. Fig. 3b has a higher range, which varies from 3.0 at the flame base to 3.2 at the flame tip. The corresponding ~8 ~6 E N ~o 8 e 4 2 -le -12 ~ ~ 0 Radius, r 4 ~ 12 4 e 12 [cml 18 16 E 12 ~1o e 6 4 2 -16 -~2 -a -4 o Radius, r le [cm] Figure 1. RECONSTRUCTED AXIAL AND RADIAL MEAN VELOCITY CONTOURS FROM EXPERIMENTAL DATA OF WECKMAN AND STRONG [25]: (a) AXIALVELOCITYCOMPONENT;(b) RADIALVELOCITY COMPONENT time series for intensity display a periodic behavior throughout the flame. If the range of/3 is increased further from 3.4 (base) to 3.6 (tip), quasiperiodic intensity fluctuations are observed, as seen in Fig. 3c. Finally, if the/3 range is from 3.6 (base) to 3.8 (tip), the behavior is chaotic (see Fig. 3d). This change in qualitative behavior corresponds to the well-known Ruelle and Takens [16] bifurcation sequence. In Figs. 3, the level of fluctuations in radiation intensity is higher at the base than at the tip of the flame. The reason is that the width across which intensity is measured, is greater at the base. In these figures, we also show the mean radiation intensity (in red) based on the mean temperature and absorption coefficient values. Note that, if turbulence-radiation interactions are accounted for, the resulting intensities are larger. This result is expected and consistent with those published earlier (see e.g., [10], [11], [15]). It should be understood, however, that the exact effect of TRI on mean radiation intensity is a function of flame conditions considered, and may vary from one flame to another. Another parameter that affects the extent of TRI is the magnitude of small-scale fluctuations in the turbulent flow field, which is a function of the actual flow conditions. Here, however, we investigate the affect of fluctuations by simply 6 Copyright (~) 2002 by ASME 80QO ~o, h= 3cnn m' 70QO m~ __ h=11crn 600O la' h=14cm 5000 h=19cxn 4~ (a) 400O -~ -8 4 0 4 8 12 16 | 80OO ~K ! ! h=3cm Radius, r [can] 2oJ 7000 • h=11orn `zA~AAAaA&AA~AAAA|~LkAAAAAAkAAaAAAAkAAAAA~ahaA~AkAAA~AAa"AaAAAAA~AAa~AA~AAAuAAka~AAAAAAAk" 6O0O h=14cm |•••|•|•|•A••A••••|A•••••A••••AA•A••A•••AAA•A•••A•••••••A•AA•A•A•••A/•A•|A•A•u|••••••A•A••A••••AAi rf~T~y~|~;~TT~T~|~v~T~T~T~T~T~|~Tf~T~v~T~v~|~ 500O _ _ . - - _ . - : -.- =- - - - : . . . . . . . . . --:-:--.- =lgcm - - - - : - - : : - : - :h -: - -:.--: -. - .:--::- -: - -- -...::.:.:.... 400O | 8O0O 4: .......... _ .-:: (b) e, ! ! h= =* 3cm o) -~2 -e -4 o 4 e 12 1~ 7000 h=11cm I~zdlus, • [cxnt ~ 6O00 ~ i ~ n n ~ T ~ ~ 1 h=14crn 500O , r~ h = l 9c,m 4000 (c) i ! ! 80OO , -" " 'lq"W "'v V " "y v v v ~ ' ' w l T ' T ' "'~ ,iv vvy,'v , 7O00 -ul, -12 ~ -,4 0 4 8 12 1£ aa(l~*, r [cm] ~v~,~ . . . . . 600O p|- V ' qYN" 'Y' - Figure 2. TEMPERATURE CONTOURS; (a) RECONSTRUCTED FROM T H E EXPERIMENTAL DATA OF REF. [25]; (b) FROM CHAOTIC MAPS, A M P L I T U D E FACTOR 0.36; (c) FROM CHAOTIC MAPS, A M P L I T U D E FACTOR 0.75. "~ vv r , , , - r ~/ q , , w h=14cm 5OOO r-,' 400O Vv ~"~" ! v-y-V,v-Trvvv,, v"yv,'"Q{y,'v,y", ....... "v , (o) m • 0.380 0,385 • 0.395 0.390 ,Scaled Time adjusting the amplitude factor A given in Eq. (5). Figure 4 provides a comparison of intensity of fluctuations for two different values of the amplitude factor A in Eq. (5). We note that in a complete LES this factor would be set automatically utilizing the approach described by McDonough [43] in conjunction with the scale similarity hypothesis employed in dynamic SGS models (see [34]). But here we employ experimental data, so the amplitude has been set somewhat arbitrarily simply to allow assessment of effects on intensity fluctuations when it is changed. Part (a) of Fig. 4 displays results at four locations through the flame with an amplitude of 36% of the mean applied to temperature fluctuations. This is a repeat of Fig. 3(d). Fig. 4(b) presents results for only two locations (because amplitudes are significantly higher, and plotted curves overlap excessively if all four are displayed), calculated exactly as | (Arbitrary 0.400 Units) Figure 3. TIME SERIES OF RADIATION INTENSITY ALONG FLAME AXIS; (a) FOR ,8 RANGE OF 2.7 (AT FLAME BASE) TO 2.9 (AT FLAME TIP); (b) ~ RANGE 3.0--3.2; (c) ,/3 RANGE 3.4--3.6; (d) /~ RANGE 3.6-3.8. for part (a) except the amplitude is set at 75%. These time series are taken from detailed results as shown in Figs. 2(b) and (c) for a single instant of time. Also shown in Figs. 4 are the mean intensities (shown in red) calculated from data corresponding to Fig. 2(a), i.e., with no turbulent fluctuations. It is clear from the figures that although the temperature fluctuates about its mean (not shown), the intensities fluctuate about a different (higher) mean value. This is a consequence of the nonlinear 7 Copyright (~) 2002 by ASME F ,e F ficult to provide a complete a priori test. Nevertheless, the results displayed herein show significant promise for this DDS approach to provide high-fidelity models, not only for LES (and possibly RANS), but also for use in real-time control strategies where very high-speed computations are necessary. We remark that run times for results presented herein for the complete 33 × 19 grid were a fraction of a second on a workstation with only a 260 MHz clock. This approach can be used easily, and in a computationally-economical way, to determine the effect of local turbulence-radiation interactions in chemically reacting flames, and will allow more detailed studies of turbulence-radiation-chemical kinetics interactions. Extension of this methodology will yield prediction of soot formation variations in industrial flames based on the input flame structure properties. Such a computational tool is very much required for the development of smart adaptivecontrol modalities. 8DQO~ h=14cm gOOD 8000! 6OO@ h=lgcm 4OQO REFERENCES 0.3~ 0.38,5 0.390 0.395 0.400 [1] Townsend, A. A., 1958, "The effects of radiative transfer on turbulent flow of a stratified fluid," J. Fluid Mech., 4, pp. 361-375. Scaled Time (Arbitranj Units) Figure 4. TIME SERIESFOR RADIATION INTENSITY CORRESPONDING TO TWO DIFFERENT AMPLITUDE FACTORS: (a) 0.36 (SEE FIG. 2B); (b) 0.75 (SEE FIG. 2C). [2] Cox, G., 1977, "On radiant heat transfer from turbulent flames," Combust. Sci. and Tech., 17, pp. 75-78. interactions implied by Eq. (3), and is a significant effect reported earlier in [21] and [22] in the context of a more detailed (and less efficient) modeling approach. [3] Tamanini, F., 1977, "Reaction rates, air entrainment and radiation in turbulent fire plumes," Combust. Flame, 30, pp. 85-101. [4] Kabashnikov, V. P. and Myasnikova, G. I., 1985, "Thermal radiation in turbulent flows-temperature and concentration fluctuations," Heat Trans]er-Soviet Research., 17, pp. 116-125. CONCLUSIONS In this paper we have presented a new approach to SGS modeling of turbulence-radiation interactions in the context of large-eddy simulation. We outlined the derivation of model equations and then conducted what can be viewed as (a portion of) an a priori test of this new discrete dynamical system technique. Computed temperature and radiation intensity fluctuations were provided to characterize behavior of the model as bifurcation parameters of the DDS were varied. These simulations represent the first application of this approach over a spatially-extended region, and furthermore the first direct use of large-scale results (experimental in the present case) to automatically set bifurcation parameters of the DDS. The results produced by the model are physically reasonable and self consistent; however, the nature and quantity of extant experimental data, and absence of detailed DNS data for turbulence-radiation interactions, make it dif- [5] Grosshandler, W. L. and Joulain, P., 1986, Prog. Astro. and Aero., 105, Part II, AIAA, Washington, pp. 123-152. [6] Fischer, S. J., Hardouin-Duparc, B. and Grosshandler, W. L., 1987, "The structure and radiation of an ethanol pool fire," Combust. Flame, T0, pp. 291-306. [7] Fischer, S. J. and Grosshandler, W. L., 1988, "Radiance, soot, and temperature interactions in turbulent alcohol fires," Twenty Second Symposium (International) on Combustion, pp. 1241-1249, The Combustion Institute, Pittsburgh, PA. [8] Gore, J. P., Jeng, S. M. and Faeth, G. M., 1987, "Spec8 Copyright (~) 2002 by ASME tral and total radiation properties of turbulent hydrogen/air diffusion flames," ASME J. Heat Transfer., 109, No. 1, pp. 165-171. [19] Yang, T., McDonough, J. M. and Jacob, J. D., 2001, "2-D 'poor man's Navier-Stokes equations' model of turbulent flows," Submitted to AIAA J. [9] Gore, J. P. and Faeth G. M., 1988, "Structure and radiation properties of luminous turbulent acetylene/air diffusion flames," ASME J. Heat Transfer., 110, No. 1, pp. 173-181. [20] Mengfi~, M. P. and McDonough, J. M., 1994, "Regime maps for radiation-turbulence interactions," presented in the poster session, 25th International Symposium on Combustion, Irvine, CA, August 1994. [10] Faeth, G. M., Gore, J. P., Chuech, S. G. and Jeng, S. M., 1989, "Radiation from turbulent diffusion flames," Ann. Rev. Numerical Fluid Mech. and Heat Transfer, C. L. Tien and T. C. Chawla, eds. Hemisphere, New York, pp. 1-38. [21] McDonough, J. M., Wang, D. and Mengfiq, M. P., 1996, "Radiation-turbulence interaction in flames using additive turbulent decomposition," Radiative Transfer--I: Proceedings of the First International Symposium on Radiative Transfer, Begell House, New York, 1996. [11] Song, T. H. and Viskanta, R., 1987, "Interaction of turbulence with radiation: application to combustion systems," AIAA J. Thermophysics and Heat Transfer, 1, pp. 56-62. [22] Mengii~, M. P. and McDonough, J. M., 1998, "Chaotic radiation-turbulence interactions in flames," EUR O T H E R M Seminar 56, Delphi, Greece, April 3, 1998. [23] Mukerji, S., McDonough, J. M., Mengfi~, M. P., Manickavasagam S. and Chung, S., 1998, "Chaotic map models of soot fluctuations in turbulent diffusion flames," Int. J. Heat Mass Transfer, 41, pp. 4095-4112. [12] Gore, J. P., Ip, U. S. and Sivathanu, Y. R., 1992. "Coupled structure and radiation analysis of acetylene/air flames," ASME J. Heat Transfer, 114, pp. 487-493. [13] Hartick, J. W., Tacke, M. T., Fruchtel, G., Hassel, E. P. and Janicka, J., 1996, "Interaction of radiation and turbulence in confined diffusion flames," Proceedings of the Twenty Sixth Symposium (International) on Combustion, Combustion Institute, Pittsburgh, PA, pp. 75-82. [24] Hylin, E. C. and McDonough, J. M., 1999. "Chaotic small-scale velocity fields as prospective models for unresolved turbulence in an additive decomposition of the Navier-Stokes equations," Int. J. Fluid Mech. Res., 26, pp. 539-567. [14] Mazumder, S. and Modest, M. F., 1999, "A probability density function approach to modeling turbulenceradiation interactions in nonluminous flames," Int. J. Heat Mass Transfer, 40, 1999, pp. 971-991. [25] Weckman, E. J. and Strong, A. B., 1996, "Experimental investigation of the turbulence structure of medium-scale methanol pool fires," Combust. Flame, 105, pp. 245-266. [15] Li, G. and Modest, M. F., 2002, "Application of Composition PDF methods in the investigation of turbulenceradiation interactions," J. of Quantitative Spectroscopy and Radiative Transfer, pp. 461-472. [26] Libby, P. A. and Williams, F. A., 1994, Turbulent Reacting Flows, Academic Press, San Diego, CA. [27]Peters, N., 2000, Turbulent Combustion, Cambridge University Press, Cambridge. [16] Ruelle, D. and Takens, F., 1971, "On the nature of turbulence," Commun. Math. Phys., 20, pp. 167-192. [28] Viskanta, R. and Mengfi~, M. P., 1987, "Radiation heat transfer in combustion systems," Prog. Energy Combust. Sci., 13, pp. 97-160. [17] McDonough, J. M., Mukerji, S. and Chung, S., 1998, "A data-fitting procedure for chaotic time series," Appl. Math Comput., 95, pp. 219-243. [29] Modest, M. F., 1993, Radiative Heat Transfer, McGraw-Hill, Inc., New York. [18] McDonough, J. M. and Huang, M. T., 2001, "A 'poor man's Navier-Stokes equation': derivation and numerical experiments--the 2-D case," Univ. of Kentucky Mech. Engr. Report CFD-03-01, 2001. (submitted to Int. J. Numer. Meth. Fluids, 2001) [30] McDonough, J. M. and Bywater, R. J., 1986, "Largescale effects on local small-scale chaotic solutions to Burgers' equations," AIAA J., 24, pp. 1924-1930. [31] McDonough, J. M. and Bywater, R. J., 1989, "Turbu9 Copyright (D 2002 by ASME lent solutions from an unaveraged additive decomposition of Burgers' equation," In Turbulent Flows-1989, ASME FED 76, pp. 7-12. bridge University Press, Cambridge, UK. [42] Lorenz, E. N., 1963, "Deterministic nonperiodic flow," J. Atmos. Sci., 20, pp. 130-141. [32] McDonough, J. M., Yang, Y. and Hylin, E. C., 1995, "Modeling time-dependent turbulent flow over a backward-facing step via additive turbulent decomposition and chaotic maps," In Proceedings of First Asian Computational Fluid Dynamics Conference, Hui, Kwok and Chasnov (eds), Hong Kong University of Science and Technology, Hong Kong, pp. 747-752. [43] McDonough, J. M., 2002, "A 'synthetic scalar' subgridscale model for large-eddy simulation of turbulent combustion," presented at Spring Tech. Mtg. Central States Sea Combust. Inst., Knoxville, TN, April 7-9, 2002. [33] Frisch, U., 1995, TURBULENCE The Legacy of A. N. Kolmogorov, Cambridge University Press, Cambridge. [34] Germano, M., Piomelli, U., Moin, P. and Cabot, W. H., 1991. "A dynamic subgrid scale eddy viscosity model," Phys. Fluids, A3, pp. 1760-1765. [35] McDonough, J. M. and Huang, M. T., 2000, "A lowdimensional model of turbulence-chemical kinetics interactions," Proc. 3rd Int. Symp. Scale Modeling, Nagoya, Japan. [36] McDonough, J. M. and Joyce, D. L., 2002, "A discrete dynamical system subgrid-scale model of turbulent convection," AIAA Paper 2002-3209, presented at 8th AIAA/ASME joint Thermophysics and Heat Transfer Conf., St. Louis, MO., June 24-27, 2002. [37] McDonough, J. M. and Zhang, S., 2002, "LES subgridscale models of turbulence-chemical kinetics interactions based on discrete dynamical systems," AIAA Paper 20023172, presented at 32nd AIAA Fluid Dynamics Conf., St. Louis, MO., June 24-27, 2002. [38] McDonough, J. M. and Zhang, S., 2002, "Discrete dynamical system model of turbulence-chemical kinetics interactions," presented at 37th International Energy Conversion Engineering Conf., Washington DC, July 28-Aug 1, 2002. [39] Zhang, S., Slade, J. D. and McDonough, J. M., 2002, "A low-order discrete dynamical system model of turbulent fluctuations in a reduced mechanism for H2-O2 combustion," presented at Spring Tech. Mtg. Central States Sec. Combust. Inst., Knoxville, TN, April 7-9, 2002. [40] Leray, J., 1934, "Essai sur le mouvement d'um liquide visquex emplissat l'espace," Acta. Math., 63, pp. 193-248. [41] Bohr, T., Jensen, M. H., Paladin, G., and Vulpiani, A., 1998, Dynamical Systems Approach to Turbulence, Cam10 Copyright (~) 2002 by ASME