VOLUME 76, NUMBER 21 PHYSICAL REVIEW LETTERS 20 MAY 1996 Universality of Flux Creep in Superconductors with Arbitrary Shape and Current-Voltage Law Ernst Helmut Brandt Max Planck Institute für Metallforschung, Institut für Physik, D-70506 Stuttgart, Germany (Received 12 January 1996) The nonlinear and nonlocal diffusion equation for the relaxing current density Jsr, td in long superconductors of arbitrary cross section in a constant perpendicular magnetic field Ba is solved exactly by separation of variables in the electric field Esr, td ­ fsrdgstd. This solution includes the limiting cases of longitudinal and transverse geometries and applies to the current-voltage laws E ~ J n ranging from Ohmic (n ­ 1) to Bean-like (n ! `) behavior. The electric field profile fsrd weakly depends on n and becomes universal for n exceeding ø5. At large times t one finds E ~ 1yt nysn21d and J ~ 1yt 1ysn21d for n . 1, and E ~ J ~ exps2tyt0 d for n ­ 1. The contour lines of the creeping Esr, td coincide with the field lines of Bsr, td in the remanent state Ba ­ 0. [S0031-9007(96)00286-4] PACS numbers: 74.60.Ge, 74.25.Ha Type-II superconductors, in particular the high-Tc superconductors, in general are not ideal conductors of electric current when put into a magnetic field Ba . Nonzero resistivity appears when the Abrikosov vortices induced by Ba depin due to a current density J exceeding a critical value Jc , or by thermal activation occurring also at J , Jc . The resulting motion of vortices generates an electric field E ­ By, where B is the flux density and y the drift velocity. A superconductor may thus be characterized by its current-voltage law EsJd, which in general is nonlinear and strongly depends on Ba and on the temperature T . This EsJd characteristic is most sensitively extracted from magnetization measurements, e.g., by slowly increasing or decreasing Ba std and then keeping it at a constant (or zero) value at times t $ 0. During such creep experiments, the magnetic moment caused by persistent currents relaxes with an approximately logarithmic time law when EsJd is strongly nonlinear, and exponentially when EsJd ­ rJ is linear (Ohmic). Recently, Gurevich and co-workers have shown that in both longitudinal [1,2] and transverse [2,3] geometries, corresponding to zero and unity demagnetizing factors, respectively, the relaxing electric field Esr, td is universal if EsJd is sufficiently nonlinear. This means that after some transient time t1 , Esr, td ­ fsrdgstd separates into a universal profile fsrd and a time dependence gstd ~ 1yst1 1 td ø 1yt. The relaxingRcurrent density 1 Jsr, td and magnetic moment mstd ­ 2 r 3 Jsr, tdd 3 r are then obtained by inserting this general electric field into the material law J ­ JsEd. This separation was found to be exact if one has ≠Ey≠J ­ EyJ1 with constant J1 , corresponding to an exponential law EsJd ­ Ec expfsJ 2 Jc dyJ1 g, and if E depends only on one spatial coordinate. This applies to slabs [1,2] or cylinders [4] in parallel field, and to thin strips or circular disks in perpendicular field [2,3]. The same universality of creep, and the existence in transverse geometry of “neutral lines” along which the flux-density Bsr, td stays constant during creep, was recently demonstrated by magneto-optic obser4030 0031-9007y96y76(21)y4030(4)$10.00 vation and by computation to occur also in thin specimens of square shape [5]. In the present Letter I show that the exact solution of the creep problem by separation of variables of Esr, td is possible for a much more general geometry including specimens of finite thickness and arbitrary cross section in a perpendicular field, and for all current-voltage laws EsJd ~ J n , or, more precisely, (1) EsJd ­ Ec jJyJc jn sgnJ , yielding JsEd ­ Jc jEyEc j1yn sgnE. This power law is observed in numerous experiments and was considered elsewhere in connection with creep [2,6] and flux penetration and ac susceptibility [4,7–10]. It corresponds to a logarithmic current dependence of the activation energy UsJd ­ Uc lnsJc yJd, which inserted into an Arrhenius law yields EsJd ­ Ec exps2UykT d ­ Ec sJyJc dn with n ­ Uc ykT ¿ 1; it contains only two parameters Ec yJcn and n; and it interpolates from Ohmic behavior (n ­ 1) over typical creep behavior (n ­ 10, . . . , 20) to “hard” superconductors with Bean-like behavior (n ! `). A power law avoids the unphysical behavior at J ­ 0 exhibited by the exponential law originally used in Refs. [1– 3] to achieve separation of variables in the creep problem. Consider the rather general geometry of a long (along z) superconductor of arbitrary cross section S in a perpendicular field Ba directed along y, e.g., a rectangular bar filling the volume jxj # a, j yj # b, jzj , `, cf. Fig. 1. The current density Jsx, yd, electric field Esx, yd, and vector potential Asx, yd then point along z and the magnetic induction Bsx, yd ­ = 3 A is in the x-y plane. Throughout this Letter I shall assume B ­ m0 H, i.e., disregard the finite value of the lower critical field Bc1 . This approximation is excellent when everywhere inside the superconductor one has B . 2Bc1 . From J ­ = 3 H ­ m21 0 = 3 s= 3 Ad one then gets for our geometry J ­ 2 2m21 0 = A, which has the solution Z d 2 r 0 Qsr, r 0 dJsr 0 d 2 xBa , Asrd ­ 2m0 S Qsr, r 0 d ­ s1y2pd lnjr 2 r 0 j . © 1996 The American Physical Society (2) VOLUME 76, NUMBER 21 PHYSICAL REVIEW LETTERS 20 MAY 1996 µ t Esr, td ­ Ec fn srd t1 1 t FIG. 1. The field lines of the induction B during penetration of perpendicular flux into long bars with side ratios bya ­ 2 (left) and bya ­ 0.4 (right) in the Bean limit (n ­ 51) for applied fields Ba ­ 0.3, 0.7 (Ba ­ 0.05, 0.1, 0.2, 0.4, in units m0 Jc a. The field of full penetration is Bp ­ 0.96 (0.87, 0.72, 0.49, 0.33) for bya ­ 4 (2, 1, 0.4, 0.2). The dashed rectangle marks the specimen boundary. The bold line (composed of the merging contour lines jJjyJc ­ 0.5, . . . , 0.3) shows the penetrating flux front inside which J ­ 0 and B ­ 0. Here and in the following r denotes sx, yd and the integration is over the specimen cross section S. The Ù ­ ≠By≠t ­ 2= 3 E in this geometry induction law B reduces to AÙ ­ 2E. Combining this with Eq. (2) and with the material law E ­ EsJd or J ­ JsEd, one obtains the equation of motion for Esr, td, Z ≠ Ù a . (3) d 2 r 0 Qsr, r 0 d JfEsr 0 , tdg 1 x B Esr, td ­ m0 ≠t S Figure 1 shows the magnetic field lines in and around a rectangular superconductor during flux penetration obtained from a similar integral equation for A. Ù a ­ 0, In creep experiments one has Ba ­ const; thus B and Eq. (3) simplifies to Z Ù 0 , td ≠J . Esr, td ­ m0 d 2 r 0 Qsr, r 0 dEsr (4) ≠E This integral equation describes the nonlinear and nonlocal diffusion of Esr, td during flux creep. For the power law EsJd (1), one has ≠Jy≠E ­ 1ys≠Ey≠Jd ­ sJc yhEd sEyEc d1yh , yielding m 0 Jc Z 2 0 Ù 0 , tdE s1ynd21 . (4a) d r Qsr, r 0 dEsr Esr, td ­ 1yn nEc Remarkably, this nonlinear integral equation can be solved exactly by the ansatz E ­ fsrdgstd, yielding ∂nysn21d . (5) If we choose t ­ m0 Jc Sy4psn 2 1dEc we obtain fh srd from 4p Z 2 0 d r Qsr, r 0 dfn sr 0 d1yn . (6) fn srd ­ 2 S This nonlinear integral equation is easily by iterR solved sm11d smd1yn ­ 2s4pySd Qfn starting ating the relation fn s0d s1d s2d with fn ­ 1. The resulting series fn , fn , . . . , converges rapidly if n . 1. For m ¿ 1 one has approxism11d smd srd ø fn srd s1 1 cynm d with c ø 1. For mately fn n ¿ 1 (practically for n $ 5) the shape fn srd of the electric field becomes a universal function which depends only on the specimen shape but not on the exponent n, 2Z 2 0 fn$5 srd ø f` srd ­ 2 d r lnjr 2 r 0 j . (7) S S In the Ohmic case n ­ 1, the ansatz (5) makes no sense since the exponent nysn 2 1d diverges. For this special case the integral Eq. (4) is linear since the factor ≠Jy≠E ­ s ­ 1yr is the constant Ohmic conductivity. This linear integral equation is solved by the ansatz Esr, td ­ E0 f0 srd exps2tyt0 d , (8) yielding the relaxation time t0 ­ m0 sSyL, where L and f0 srd are the lowest eigenvalue and eigenfunction of the linear integral equation 2L Z 2 0 f0 srd ­ 2 d r lnjr 2 r 0 jf0 sr 0 d . (9) S S From (1) and (5) the current density becomes ∂1ysn21d µ t 1yn sgnfn srd . Jsr, td ­ Jc j fn srdj t1 1 t (10) For n ¿ 1, t ¿ t1 the time factor in (10) equals 1 2 1 n21 lnstytd and one has jJj ø Jc everywhere. The magnetization along y per unit length along z is Z Mstd ­ ŷmstdyLz ­ xJsx, y, td dx dy . (11) S 1 1R In (11) the prefactor 2 of mstd ­ 2 r 3 Jsr, tdd 3 r was compensated by the contribution to m of the U-turning currents at the far away ends of the bar at z ­ 6Lz y2 ¿ a, b. The resulting factor of 2 in M was sometimes missed in previous work on slabs. These results apply to arbitrary specimen cross section S. For the realistic rectangular cross section 2a # x # a, 2b # y # b, S ­ 4ab, with Ba along y, the symmetry Jsx, yd ­ 2Js2x, yd ­ Jsx, 2yd (and same symmetry for E and A) allows one to restrict the integration to the quarter 0 # x # a, 0 # y # b by using the symmetric kernel Qsym sr, r 0 d ­ 2 d sx 2 1 y 2 d sx 2 1 y2 1 2 1 , ln 2 2 2 d sx 2 1 y 2 d 4p sx1 1 y2 1 1 (12) 4031 VOLUME 76, NUMBER 21 PHYSICAL REVIEW LETTERS 20 MAY 1996 with x6 ­ x 6 x 0 , y6 ­ y 6 y 0 . One now has in (5) (13) t ­ m0 Jc abyfpsn 2 1dEc g , Z a dx 0 Z b dy 0 sx 2 1 y 2 d sx 2 1 y 2 d 2 1 1 ln 1 fn sx, yd ­ 2 1 y 2 d sx 2 1 y 2 d a 0 b sx2 0 1 2 2 (14) 3 fn sx 0 , y 0 d1yn . Before discussing the rectangular cross section I first show that in the limits of longitudinal (b ¿ a) and transverse (b ø a) geometry the above expressions reduce to known and new results. In both limits, the functions J, E, A, Bx , and By depend only on x. One may thus put y ­ 0 writing, Rae.g., Esx, yd ø Esx, 0d ­ Esxd, and one gets M ­ 4b 0 xJsxd dx. In the transverse limit (strip with thickness 2b ø a), the reduced one-dimensional kernel is Qtrans sx, x 0 d ­ 2bQsym sx, 0, x 0 , 0d ­ sbypd lnfjx 2 x 0 jysx 1 x 0 dg. This kernel was used in calculations of creep [3,10], flux penetration [9], and nonlinear [10] and linear [11,12] ac response of superconducting strips. In the creep solution (5) one now has t (13) and the shape fn sxd is determined by Ç Ç 1 Z a 0 x 1 x0 fn sxd ­ dx ln (15) fn sx 0 d1yn . a 0 x 2 x0 For n ¿ 1 this reproduces the E of Ref. [3], µ ∂ a1x x a2 2 x 2 m0 Jc ab 1 ln 1 ln . Esx, td ­ psn 2 1d t a2x a x2 (16) In the longitudinal limit (slab Rwith b ¿ a), the reduced ` kernel is Qlong sx, x 0 d ­ 2 0 dy 0 Qsym sx, 0, x 0 , y 0 d ­ 1 0 0 0 (the min2 sjx 2 x j 2 jx 1 x jd ­ 2Minsx, x d 0 imum value of x, x ), which has the property 00 ­ dsx 2 x 0 d. One now has in (5) t from Qlong (13) and fn sxd from p Z a 0 fn sxd ­ dx Minsx, x 0 dfn sx 0 d1yn , (17) ab 0 0 # x # a, fs2xd ­ 2fsxd. For large exponents n ¿ 1 this reproduces the result of Gurevich [1,2], m0 Jc xs2a 2 jxjd Esx, td ­ . (18) n21 2t The unphysical dependence of t (13) and fn sxd (17), but not of Esx, td (18), on the specimen length 2b may be removed by redefining t and fn , multiplying the integrals in (14) and (17) by a factor 1 1 pby4a, and dividing t (13) by the same factor. This definition leaves the transverse limit unchanged but replaces the prefactor pyab in (17) by p 2 y4a2 . The integral equation (17) is equivalent to a differential equation with boundary conditions, fn s0d ­ fn0 sad ­ 0 , (19) fn00 sxd ­ 2k 2 fn sxd1yn , where k ­ py2a in our new definition of t. The solutions of (19) in the Ohmic (n ­ 1) and Bean (n ­ `) limits look very similar, f1 sxd ­ const 3 sinspxy2ad and f` sxd ­ sp 2 y8a2 dxs2a 2 jxjd, cf. Fig. 2. 4032 FIG. 2. Profiles of the electric field E ~ fn sxd and current density J ~ fn sxd1yn during creep in longitudinal (17) and transverse (15) geometries for exponents n ­ 1, 2, 5, and `. Creep profiles fn sxd obtained from (14) and (17) are depicted in Fig. 2 for exponents n ­ 1, 2, 5, and `. Notice that the fn sxd only weakly depend on n but are qualitatively different for the two geometries: In the longitudinal limit the fn sxd are maximum at the boundary x ­ a, whereas the transverse fn sxd exhibit a maximum inside the specimen, e.g., at x ­ 0.735a for n ­ 1 [11] p and x ­ ay 2 ­ 0.707a for n ! ` [3]. The contour lines of the creeping Esx, y, td inside and outside rectangular bars with aspect ratios bya ­ 2, 1, and 0.2 are depicted in Fig. 3 for the Bean limit n ¿ 1. These contour lines of E are also the field lines of the induction Bsx, y, td in the remanent state. Namely, for n ¿ 1 one gets from (2) and (12) the vector potential Z aZ b Qsym sr, r 0 ddy 0 dx 0 2 xBa , Asx, yd ø 2m0 Jc 0 0 (20) because one has J ø Jc sgnx during creep. The lines A ­ const are the field lines of B 5 = 3 sẑAd. For Ba ­ 0 these lines coincide with the contour lines of E ­ Ù since during creep the time dependence separates, 2A, Esr, td ­ fsrdgstd, Eq. (5). For nonzero applied field Ba , the lines E ­ const are still as depicted in Fig. 3. The field lines of B for Ba near the penetration field Bp look VOLUME 76, NUMBER 21 PHYSICAL REVIEW LETTERS 20 MAY 1996 and induction B ' z, during flux creep is presented for nonlinear conductors with constitutive laws E ~ J n and B ­ m0 H and with rectangular cross section 2a 3 2b in a perpedicular field Ba k y. The obtained twodimensional universal profiles of E during creep (Fig. 3) explain how the one-dimensional profiles Esx, td of the two limiting geometries b ¿ a and b ø a (Fig. 2) come about. In particular, the maximum of Esx, td in transverse geometry, corresponding to a maximum in the nearly constant J ­ Jc sEyEc d1yn ø Jc and in the energy dissipation EJ ~ E 111yn ~ J n11 , is related to the maximum of the vector potential A k z (2) caused by this current and depicted in Fig. 3. This theory is easily extended to circular disks or cylinders with finite height by modifying the kernel Qsr, r 0 d. The origin of the well known sign reversal of the perpendicular component By at the surfaces y ­ 6b near the edges x ­ 6a, occurring in the remanent state and leading to a neutral line on which B ­ Ba stays constant during creep [3,5], becomes clear from the magnetic field lines in Fig. 3, which coincide with the contour lines of E and A during creep. Interesting further effects [13] are expected at positions with small B if a more general BsHd with finite Bc1 is accounted for. Work in this direction is under way. FIG. 3. The contour lines of the electric field E ­ 2AÙ during creep in long rectangular superconductors with side ratios bya ­ 2, 1, and 0.2 (from top) for n ­ 51 and arbitrary constant applied field Ba . These lines coincide with the magnetic field lines in the fully saturated remanent state Ba ­ 0. Bottom: 3D plot of E (and of A) for bya ­ 0.2. similar as depicted in Fig. 1, bottom row; they are nearly parallel lines slightly inflated inside the specimen. All these analytical results are confirmed by computations of creep from Eq. (4): During constant ramp rate BÙ a fi 0 one has E ­ x BÙ a in the fully penetrated state. When Ba is held constant, the straight E profile starts to curve down near the edge and, after a short transition time t1 , it reaches the universal profiles depicted in Figs. 2 and 3. During creep the shapes of E, J, and B practically do not change over many decades of the creep time t, but their amplitudes decrease according to Eqs. (5) and (10). In particular, for n ¿ 1 and t ¿ t1 one has E ~ 1yt and 1 M ~ J ~ stytd1ysn21d ø 1 2 n21 lnstytd. In conclusion, the exact solution for the electric field Esx, y, td k z, and thus for the current density J k z [1] A. Gurevich and H. Küpfer, Phys. Rev. B 48, 6477 (1993). [2] A. Gurevich, Int. J. Mod. Phys. B 9, 1045 (1995). [3] A. Gurevich and E. H. Brandt, Phys. Rev. Lett. 73, 178 (1994). [4] E. H. Brandt, Rep. Prog. Phys. 58, 1465 (1995). [5] Th. Schuster, H. Kuhn, and E. H. Brandt, Phys. Rev. B 51, 697 (1995). [6] V. M. Vinokur, M. V. Feigel’man, and V. B. Geshkenbein, Phys. Rev. Lett. 67, 915 (1991). [7] J. Rhyner, Physica (Amsterdam) 212C, 292 (1993). [8] J. Gilchrist and C. J. van der Beek, Physica (Amsterdam) 231C, 147 (1994). [9] Th. Schuster et al., Phys. Rev. Lett. 73, 1424 (1994); Phys. Rev. B 50, 16 684 (1994); E. H. Brandt, Physica (Amsterdam) 235C– 240C, 2939 (1994). [10] A. Gurevich and E. H. Brandt, Phys. Rev. Lett., 70, 1723 (1996). [11] E. H. Brandt, Phys. Rev. Lett. 71, 2821 (1993); 49, 9024 (1994); Phys. Rev. B 50, 4034 (1994); 50, 13 833 (1994). [12] A. T. Dorsey, Phys. Rev. B 51, 15 329 (1995). [13] M. V. Indenbom, Th. Schuster, H. Kuhn, H. Kronmüller, T. W. Li, and A. A. Menovsky, Phys. Rev. B 51, 15 484 (1995). 4033