Int. J. Environment and Pollution, Vol. 52, Nos. 3/4, 2013 Prescribed burn smoke impact in the Lake Tahoe Basin: model simulation and field verification Tom Malamakal, L-W. Antony Chen*, Xiaoliang Wang, Mark C. Green, Steven Gronstal, Judith C. Chow and John G. Watson Division of Atmospheric Sciences, Desert Research Institute, 2215 Raggio Parkway, Reno, NV 89512, USA and Atmospheric Science Program, University of Nevada, 1664 N. Virginia St., Reno, NV 89557, USA E-mail: Tom.Malamakal@dri.edu E-mail: Antony.Chen@dri.edu E-mail: Xiaoliang.Wang@dri.edu E-mail: Mark.Green@dri.edu E-mail: Steve.Gronstal@dri.edu E-mail: Judy.Chow@dri.edu E-mail: John.Watson@dri.edu *Corresponding author Abstract: Smoke dispersion modelling based on the Fire Emission Production Simulator and the Hybrid Single Particle Lagrangian Integrated Trajectory (FEPS-HYSPLIT) model was applied to prescribed burns in the Lake Tahoe Basin (LTB) during fall 2011. This, in conjunction with measurements at sources and real-time ambient PM2.5 monitoring around LTB, served to evaluate the prescribed burning impacts on air quality. For a given combustion efficiency, in-plume measurements suggest FEPS to underestimate PM2.5 emission factors by up to six-fold, though FEPS agrees relatively well with laboratory combustion of dry fuels. Prescribed burns in LTB were mostly < 100 acres; time series analysis and model prediction (with 2 km or 12 km spatial resolution) suggest generally small effects on PM2.5 exposure of local communities due to careful selection of the burn windows. In regard to a few scenarios where significant impact (≥ 2 μg/m3 hourly) is predicted, the model with 2 km resolution shows smoke arrival times more consistent with ambient observations. However, uncertainties in the model predictions should be reduced further by acquiring more accurate burn records and measuring markers specific to biomass burning at the monitoring sites. Keywords: smoke forecast; biomass burning; emission model; PM2.5 emission factor; WRF; IMPROVE network; USA. Reference to this paper should be made as follows: Malamakal, T., Chen, L-W.A., Wang, X., Green, M.C., Gronstal, S., Chow, J.C. and Watson, J.G. (2013) ‘Prescribed burn smoke impact in the Lake Tahoe Basin: model simulation and field verification’, Int. J. Environment and Pollution, Vol. 52, Nos. 3/4, pp.225–243. Copyright © 2013 Inderscience Enterprises Ltd. 225 226 T. Malamakal et al. Biographical notes: Tom Malamakal received his MS in Atmospheric Science from the University of Nevada, Reno in 2013. His research interests involve atmospheric transport of chemicals and environmental impact assessment. He is currently a research staff member at the Desert Research Institute (DRI). L-W. Antony Chen received his PhD in Chemical Physics from University of Maryland in 2002. Since 2004, he has been a Research Faculty at Desert Research Institute (DRI), Nevada System of Higher Education. His research focuses on aerosol measurement techniques, combustion aerosol characterisation, and source apportionment/modelling of air pollutants for health and climate studies. Xiaoliang Wang received his PhD in Mechanical Engineering from University of Minnesota-Twin Cities in 2006. He was a Senior Development Engineer at TSI Inc. for four years, where he invented and developed the DustTrak DRX Aerosol Monitor that was used to monitor aerosol concentrations in this study. He has been a research faculty at Desert Research Institute, Nevada System of Higher Education since 2009. His research interests include physical and chemical characterisation of aerosols, pollution source characterisation, and aerosol instrument development. Mark C. Green received his PhD in Atmospheric Sciences from the University of California at Davis in 1990. He is a Research Professor in the Division of Atmospheric Sciences at Desert Research Institute where he has been since 1990. He is also the Director of the Graduate Program in Atmospheric Sciences at the University of Nevada, Reno. His research focuses on aerosol measurement and data analysis and the relationship between meteorology and air pollution. Steven Gronstal received his MS in Physics from Creighton University in 2003. He is currently pursuing his PhD in Atmospheric Sciences at the University of Nevada, Reno, while conducting research with the Environmental Analysis Facility at the Desert Research Institute. His research focuses on aerosol measurement techniques, stack sampling methods, and CFD modelling of aerosols. Judith C. Chow is the Nazir and Mary Ansari Chair in Entrepreneurialism and Science and a Research Professor in the Division of Atmospheric Sciences at the Desert Research Institute. She received her Doctor of Science degree in Environmental Health Science and Physiology from Harvard University. She has over 38 years of experience conducting air quality studies and performing statistical data analysis. As the leader of DRI’s Environmental Analysis Facility (EAF), she develops and applies advanced analytical methods to characterise suspended atmospheric particles. John G. Watson is a Research Professor in the Division of Atmospheric Sciences at the Desert Research Institute. He received his PhD in Environmental Sciences from Oregon Graduate Institute (now Oregon Health and Science University). He has over 41 years of experience in physics, environmental sciences, air quality network design and measurement, and source/receptor modelling. He is known for formulating conceptual models as well as organising and planning large-scale, multi-year air quality studies in the USA. Prescribed burn smoke impact in the Lake Tahoe Basin 1 227 Introduction Good air quality and visibility are important assets of the Lake Tahoe Basin (LTB), located along the California (CA) and Nevada (NV) state border, as a major tourist attraction in the Sierra Nevada mountain range. The annual PM2.5 (airborne fine particulate matter with aerodynamic diameter ≤ 2.5 μm) concentrations measured at South Lake Tahoe and Bliss State Park, characteristic urban and rural environment of the basin, respectively, are 9.0 and 3.5 μg/m3 (for 2000–2004, see Green et al., 2012), well below the US National Ambient Air Quality Standard (NAAQS) of 12 μg/m3 (US EPA, 2013). Major sources of air pollutants, including PM2.5, PM10, nitric oxide (NO), nitrogen dioxide (NO2), carbon monoxide (CO), and ozone (O3), within the basin were determined to be: 1 biomass burning 2 on-road engine exhausts 3 off-road engine exhausts 4 road dust 5 natural dust (Kuhns et al., 2004; Green et al., 2012). Long-range transport of air pollution from outside the basin does not contribute significantly on average (Gertler et al., 2006). The LTB (~25 × 25 km2 in size) contains one of the visibility Class I areas, the Desolation Wilderness, which is subject to the regulation of the Clean Air Visibility Rule (CAVR, see US EPA, 2005). The rule requires the visibility in Class I areas to return to their ‘natural’ conditions by 2065. The state of CA also established an 8 hr visibility standard equating to an extinction coefficient (bext) of 70 Mm–1, roughly extinction of 7% incident light per kilometer, for LTB. Despite compliance with all NAAQS/CA standards and a generally improving visibility condition with respect to annual median bext measured at Bliss State Park, bext on the 20% worse visibility days have been increasing (visibility decreasing) since 1990. The trend was mostly attributed to an increased wildfire activity (Chen et al., 2011; Green et al., 2012). Increasing wildfire frequency and intensity have been reported across the Western US due to regional climate change (Westerling et al., 2006). On the other hand, there were episode days occurring in fall through spring with no clear evidence of wildfire impact (e.g., Chen et al., 2011). These episodes might reflect the influence of prescribed burning and/or residential wood combustion (RWC). Prescribed burning had been conducted year-around inside and outside LTB to maintain natural succession of plant communities and to reduce wildfire danger. In 2011, > 2000 acres of wildland were fire-treated within 20 km of Lake Tahoe, and roughly 20% of them belonged to broadcast/understory burns of natural vegetation (the rest being pile burns, per communications with fire agencies listed in Figure 1). Although these prescribed burns were practised under strict guidelines, they could still impact visibility and human exposure of air pollutants causing short-term, acute effects and/or long-term background change. The importance of prescribed burning contributions to air pollutants is increasing as regulations over other sources such as motor vehicles, road dust, and RWC have been implemented and shown measurable effectiveness in reducing emissions from these sources over the last two decades (Chen et al., 2011). 228 T. Malamakal et al. Figure 1 Locations of the five ambient air monitoring sites (blue balloons) during the fall 2011 study: 1) Incline Village [119°57’24.19”W; 39°15’1.49”N; 58 m above lake level (ALL)]; 2) Tahoe City (120°8’55.74”W; 39°9’57.63”N; 12 m ALL); 3) Bliss State Park (120°6’8.73”W; 38°58’33.63”N; 206 m ALL); 4) South Lake Tahoe (119°58’13.99”W; 38°56’42.26”N; 5 m ALL); 5) Cave Rock (119°56’54.83”W; 39°2’37.12”N; 1 m ALL) (see online version for colours) Notes: Also shown are the three prescribed burns (stars) measured as part of the study at Skyland (SKY), Donner Memorial State Park (DSP), and Tunnel Creek (TNC). Solid circles indicate other known prescribed fire events carried out by Lake Tahoe Basin Management Unit (red), California State Park (pink), Nevada Division of Forestry (green), and North Lake Tahoe Fire Protection Department (yellow) during September–November, 2011. Smoke transport simulation is useful to assess the impact of prescribed burns and develop control strategies, thus contributing to an integrated approach to address air quality and deposition issues in LTB (Gertler et al., 2009). The simulation could be achieved by interfacing the Fire Emission Production Simulator (FEPS) to the Hybrid Single Particle Lagrangian Integrated Trajectory (HYSPLIT) model run with high-resolution meteorological data (Goodrick et al., 2012). This paper presents the first application of FEPS-HYSPLIT modelling for prescribed burns in LTB. In-plume measurements were conducted to evaluate FEPS emission estimates, while overall model performance (with different spatial resolutions) was verified with ambient monitoring data in cases where significant smoke impacts were predicted. The potential effects of prescribed burning on LTB air quality and future research needs are discussed. 2 Technical approaches This study focuses on the fall 2011 prescribed burning season (September–November, 2011). The period featured above-average temperatures and below-average precipitation in Northern NV, leading to relatively dry fuel conditions. This, combined with the abundance of growth due to an abnormally wet spring earlier in the year and sufficient Prescribed burn smoke impact in the Lake Tahoe Basin 229 ignition sources, led to an active wildfire season (Nevada Climate Office, 2012). Based on satellite imaginary, i.e., the MOderate Resolution Imaging Spectroradiometer (MODIS) fire product (see http://modis-fire.umd.edu), large wildfires that clearly impacted LTB air quality during the study period include Idaho’s Salmon-Challis Forest Fire (9/9–9/10) and CA’s Humboldt-Toiyabe Forest (Buckeye) Fire (9/27–9/29). Moreover, Figure 1 shows locations of 60 prescribed burns conducted in 29 days during this period. 2.1 Ambient monitoring network Five monitoring stations were established around the Lake Tahoe (Figure 1) for fall 2011. The Incline Village (NV), Tahoe City (CA), and South Lake Tahoe (CA) sites were located near the centre of the respective township representing community exposure to air pollutants. The Bliss State Park site is 206 m above Lake Tahoe and has been part of the Interagency Monitoring of PRotected Visual Environments (IMPROVE) network since 1990. It represents the Desolation and Mokelumne Wilderness Class I areas according to the CAVR. Cave Rock is a pier located on the east shore of Lake Tahoe. The site is considered rural but could be influenced by emissions from boats and US-50 traffic (~50 m above it). Chen et al. (2011) described the site characteristics in greater detail. Each site was equipped with a DustTrak 8520 (TSI Inc., Shoreview, MN) to continuously measure PM2.5 concentration at 1 min time resolution. All sites except the Bliss State Park also contained two MiniVol samplers (AirMetrics, Eugene, Oregon) to collect weekly integrated PM2.5 samples. One MiniVol used a Teflon-membrane filter for gravimetric mass and elemental composition measurement. The other MiniVol used a quartz-fibre filter followed by citric acid-impregnated cellulose filter to quantify water soluble ions as well as organic carbon (OC), elemental carbon (EC), and ammonia (NH3). Detailed chemical analysis methods and quality assurance/quality control for filter samples can be found in Chow et al. (2002) and Chow and Watson (2012) while the PM2.5 chemical composition will be presented in other papers. The DustTrak data correlated well with collocated MiniVol gravimetric PM2.5 mass across all four sites (r2 = 0.91) though they generally overestimated PM2.5 concentrations by two-fold. A calibration curve was established for all DustTraks using the regression coefficients. After the correction, 24-hr average DustTrak PM2.5 concentrations at the Bliss State Park agreed well (within ±10%) with collocated measurements made independently as part of the IMPROVE network (Green et al., 2012). 2.2 Source measurement Source measurements were conducted for three prescribed burn events (Table 1 and Figure 1) out of > 50 known burns in the basin using an in-plume monitoring system (Wang et al., 2012). The in-plume system was generally located downwind just a few meters outside the fire perimeter, though it might be moved to better capture the smoke if the prevailing wind direction changed during the experiment. The sample inlet was located ~3 m above the ground. In addition to PM2.5 [quantified by a DustTrak DRX (Wang et al., 2009), TSI Inc., Shoreview, MN), carbon dioxide (CO2), CO, reactive nitrogen oxides (NOx), and black carbon (BC) concentrations were monitored in real time at 1- to 10-sec resolution by non-dispersive infrared sensor (SBA-4, PP Systems, Amesbury, MA), electrochemical detector (Model 350S, Testo Inc., Sparta, NJ), 230 T. Malamakal et al. chemiluminescence analyzer (Model 400/401, 2B Technologies Inc., Boulder, CO), and micro-aethalometer (AE51, Magee Scientific, Berkeley, CA), respectively. Background concentrations were taken before the burn and subtracted from the in-plume measurements. The DustTrak has a precision of ~±20% and ±5% for 1-sec and 1-min averaging time, respectively (Wang et al., 2012). The 1-min maximum DustTrak concentration observed was ~50 mg/m3, well below its 150 mg/m3 measurement limit. Time-integrated filter samples were acquired every hour for analysis of PM2.5 mass (gravimetry) and chemical composition. The DustTrak data were normalised to the corresponding gravimetric mass on filters, with normalisation factors of 0.3 to 0.6. Table 1 Prescribed burns measured with an in-plume air monitoring system Burn Burn location ID Date Burn type Burn area (acres) Fuel moisture Burn Ignition start time duration* (hours) (LST) Fuel load† (tons/ acre) SKY 39°01’02”N 06/11/2011 Understory/ 119°57’00”W piles 27 10 (pile)–100% 1100 3 28 DSP 39°18’29”N 10/03/2011 Understory 120°14’43”W 9 70–100% 1100 5 35.6 TNC 39°13’45”N 10/20/2011 Understory 119°53’20”W 7 90–100% 1200 4 16.3 Notes: SKY and TNC were burns conducted within the basin and DSP was located outside the basin (Figure 1). *Duration of active ignition by fire agencies. Fire continues after ignition. †Estimated from agencies’ report and Fuel Characteristic Classification System (FCCS); canopy and duff excluded. The fuel-based emission factors were calculated from carbon balance following Nelson (1982), Andreae and Merlet (2001), and Chen et al. (2007): EFi = CMF fuel × ( CMFCO 2 × ρCO2 ρi + CMFCO × ρCO (1) +CMFVOCs × ρVOCs + CMFPM × ρPM ) where • EFi: emission factor of pollutant i (e.g., g/kg) • ρi: concentration of pollutant i measured above background levels (e.g., μg/m3) • CMFfuel: carbon mass fraction of fuel • CMFi: carbon mass fraction of species i, including CO2, CO, volatile organic compounds (VOCs), and PM2.5. The combustion efficiency (CE), i.e., the fraction of carbon in the fuel ending up in CO2, would be: CE = CMFCO2 × ρCO2 CMFCO2 × ρCO2 + CMFCO × ρCO + CMFVOCs × ρVOCs + CMFPM × ρPM (2) Prescribed burn smoke impact in the Lake Tahoe Basin 231 Since the contribution of VOCs to carbon is generally minor, the VOCs term in equaitons (1) and (2) was ignored. Chen et al. (2010) suggested that CMFfuel of 0.49 is reasonable for a mixture of forest fuels in LTB, and filter analysis showed an average CMFPM of 0.58. EFi was calculated for each minute as well as the filter integrating periods. It should be noted that the in-plume system was not always in the plume, and our measurements were not always representative of the entire smoke plume. Nonetheless, the measurements contrast between field and laboratory observations and help determine the range of emission factors and combustion efficiencies that can be compared with default model parameters. 2.3 Fire Emission Production Simulator FEPS, developed by the US Forest Service (Anderson et al., 2004), is an integrated platform for modelling wild- or prescribed fire emissions. FEPS contains default values for fuel loading and fraction of fuel consumed specific to most vegetation type/moisture content combinations in the USA. Based on the fuel information and user supplied hourly burned area, FEPS calculates fuel consumption by flaming, short-term smouldering (STS), and long-term smouldering (LTS) phases. Flaming combustion with high CE produces relatively complete oxidation converting fuel carbon to CO2, while smouldering smoke contains higher fractions of partially reduced compounds such as CO, VOCs, and PM (Crutzen and Andreae, 1990). Dynamic emission factors, modulated by CE (i.e., based on the relative strength of flaming, STS, and LTS at each hour), are used to determine the hourly emission rates: ERi = CR × EFi = CR × ( ai − bi × CE ) (3) where • ERi: emission rate of pollutant i (e.g., g/hour) • EFi: emission factor of pollutant i (e.g., g/kg) • CR: fuel consumption rate (e.g., kg/hr) • ai, bi: emission factor constant and coefficient for pollutant i (default ai = 67.4 g/kg and bi = 66.8 g/kg for PM2.5). Outputs from FEPS also include hourly heat release (kJ/hr) from the fire, which is useful for calculating the plume height. Fuel loading was determined from FEPS by matching the burn area with a Fuel Characteristic Classification System (FCCS; Ottmar et al., 2007) map of 1 km × 1 km resolution for the USA, supplemented by field observation and/or report from fire agencies. The agencies’ reports were especially important for piled slash burns. They also provided information such as fire shape (e.g., rate of progress), ignition time, and fuel moisture content. Field measurements of fire emissions were made in a few burns (i.e., burns in Table 1), but however these burns did not appreciably impact any of our ambient monitoring sites based on observation and modelling of smoke transport. Even with all the available information, temporal fuel consumption could still be quite uncertain due to the dynamic nature of fire. EFPM 2.5 (i.e., PM2.5 emission per unit mass of fuel burned) 232 T. Malamakal et al. could also be biased as they were mostly based on laboratory studies (Yokelson et al., 2013). 2.4 HYSPLIT dispersion model The HYSPLIT model was developed and maintained by the NOAA Air Resource Laboratory (ARL) (Draxler and Hess, 1998; Draxler, 1999; Draxler and Rolph, 2013). The dispersion of a pollutant can be calculated by assuming either puff or particle dispersion, while a mixed mode of top-hat horizontal puff and vertical particle distribution was used in this study. This approach takes advantage of the greater accuracy of the particle mode in vertical dispersion parameterisation and an expanding number of puffs to represent the pollutant distribution as the spatial coverage of the pollutant increases over time (Draxler and Hess, 1998). A prescribed fire is simulated as a point source centred at the burn area typically of 2 to 100 acres, with hourly PM2.5 emission rates determined from FEPS. The plume rise is computed assuming an air parcel’s rise based on the buoyancy terms (Briggs, 1969; Arya, 1999) using the fire heat release also provided by the FEPS. This approach is generally compatible with the US Forest Service’s BlueSky smoke modelling framework (Larkin et al., 2009). HYSPLIT can run with multiple nested data grids of a wide range of spatial resolution. The model was adapted to meteorological fields from the North American Mesoscale (NAM) model (12 km resolution, 43 vertical levels from surface to ~100 mb) provided by ARL and Weather Research and Forecasting (WRF) model (2 km resolution, 32 vertical levels from surface to 100 mb, updated every 12 hours) provided by the California and Nevada Smoke and Air Committee (CANSAC) for the period of September–November, 2011. The WRF model is particularly suitable for modelling complex terrain in Sierra Nevada to capture complex flow and meteorological parameters critical in dispersion calculations (Lu et al., 2012). 3 Results and discussion 3.1 Diurnal variation of PM2.5 Site-specific PM2.5 diurnal patterns were determined from medians of all hourly data (Figure 2) as a guide to distinguish repetitive sources’ (e.g., motor vehicles, RWC, and cooking) contribution from potential prescribed burning impact. Individual days with diurnal profile substantially different from this pattern and/or with extreme PM2.5 concentrations (> 95 percentile) were subject to further investigation using prescribed burn records. Field observations and model simulations suggest that effect of individual controlled burns is usually inhomogeneous over the basin and varies rapidly in time (Cliff and Cahill, 2000; Cahill, 2009). Large-scale wildfires outside the basin produce more uniformly high PM2.5 concentrations. Exclusion of days influenced by known wildfires (i.e., 9/9–10/2011 and 9/27–29/2011) does not change the diurnal patterns significantly. The traffic influences are most clear at Tahoe City with distinguishable morning [0700–0800 Local Standard Time (LST)] and evening PM2.5 peaks (1600–1700 LST) corresponding to the rush hours (Figure 2). The morning rush hour is visible at the urban South Lake Tahoe site but the evening peak appears to be delayed until ~2000 LST. This likely reflects a combined effect of traffic emissions, commercial activities (e.g., Prescribed burn smoke impact in the Lake Tahoe Basin 233 restaurants, stores, etc.) as well as RWC towards winter. RWC, but not traffic, may also influence the Incline Village site. Cave Rock at the lake level and Bliss State Park ~200 m above the lake without significant sources nearby served as the low and elevated background sites, respectively. The cold lake surface develops a strong (~10°C), shallow (~30 m) inversions at all times throughout the year (Cahill, 2009). While little diurnal variation of PM2.5 was observed at Bliss, a mid-afternoon peak at Cave Rock is consistent with downward mixing by turbulence when PM2.5 concentrations aloft (e.g., 30 m) are higher than those at the surface (e.g., Grivas et al., 2008). PM2.5 levels appear relatively uniform across the basin during 1300–1700 LST, suggesting extensive horizontal mixing besides vertical mixing in the afternoon. Figure 2 Diurnal variation of PM2.5 at five ambient monitoring sites in the Lake Tahoe Basin, based on medians of hourly PM2.5 measurement (from corrected DustTrak data) during September–November, 2011 (see online version for colours) Note: All times are in LST. 3.2 Prescribed burning emission characteristics Figure 3(a) to Figure 3(b) show the time series of in-plume measurements for the TNC burn as an example. An initial flaming combustion phase was identified during the first ~15 minutes of burning, as CE generally exceeded 0.9 with the highest PM2.5 and BC concentrations measured. BC is known to be generated mostly from flaming combustion (Kuhlbusch and Crutzen, 1995; Chen et al., 2006). The EFPM 2.5 during the period was below 30 g/kg. Following the flaming phase was a transition period of ~30 minutes featuring CE of 0.8 to 0.9 and much higher EFPM 2.5 (up to 90 g/kg). BC concentrations and emission factors remained high, but there were apparently increasing influences of smouldering combustion. One hour after ignition, CE fluctuated between 0.75 and 0.85 with more variable EFPM 2.5 while EFBC decreased gradually [Figure 3(b)]. The later period would likely be dominated by smouldering emissions (i.e., STS + LTS). 234 Figure 3 T. Malamakal et al. Time series of in-plume measurements (1-min time resolution) during the Tunnel Creek burn on 10/20/2011 for (a) carbon (i.e., C) concentrations and combustion efficiency (b) PM2.5 concentrations and emission factors (see online version for colours) Notes: Total C emission includes carbon in CO2, CO, and BC. Arrows indicate the ignition time. Flaming, transition, and smouldering phases are separated empirically (see text for details). All times are in LST. Fire-integrated combustion efficiencies and emission factors are presented in Table 2. FEPS confirms the increasing importance of fuel consumption by STS and LTS and decreasing values of CE as the burns progress. Based on the default flaming, STS, and LTS CE coefficients (i.e., 0.90, 0.76, and 0.76), FEPS calculates the fire-integrated CE to be 0.87, 0.83, and 0.84 for the SKY, DSP, and TNC burns, respectively, lower than the measured values of 0.92 for SKY and 0.86 for both DSP and TNC. Providing that CE > 0.9 is observed during the prescribed burns, a higher flaming CE may need to be implemented in FEPS. Table 2 Fire integrated combustion efficiencies and emission factors (see Table 1 for burn details) Burn ID CE MCE* EFCO2 (g/kg) EFCO (g/kg) EFPM 2.5 (g/kg) SKY 0.92 0.94 1,654 61.5 21.7 DSP 0.86 0.89 1,545 124.6 26.5 TNC 0.86 0.89 1,543 117.6 32.6 Note: *MCE: modified combustion efficiency, i.e., ignoring both the VOCs and PM terms in equation (2). EFPM 2.5 is suggested to anti-correlate with CE since incomplete combustion causes higher particulate emission. The relationship should also depend on the fuel type (Janhäll et al., 2010). Our field measurements from SKY, DSP, and TNC prescribed burning events show a wide range of EFPM 2.5 for any measured CE. They can be bounded, however, between two extremes (Figure 4). The default FEPS equation, equation (3), Prescribed burn smoke impact in the Lake Tahoe Basin 235 closely describes the lower bound EFPM 2.5 . The upper bound can be parameterised by using ai and bi of 431.8 and 429.7 g/kg, respectively in equaiton (3), as derived from the highest 10th percentile data with respect to the EFPM 2.5 / (1 − CE ) ratio. Figure 4 EFPM 2.5 -CE relationship (1-min data) over three prescribed burning events (i.e., SKY, DSP, and TNC) (see online version for colours) Notes: The lower bound of distribution is the FEPS default parameterisation while the upper bound is determined from the top 10th percentile of data with respect to the EFPM 2.5 / (1 − CE ) ratio. Blue triangles and green circles indicate data from laboratory combustion of wet and dry fuels, respectively (Chen et al., 2010). The FEPS default algorithm underestimates the observed PM2.5 emissions in most cases. The bias could be up to a factor of 6. A recent laboratory combustion study using the forest fuels from LTB (Chen et al., 2010) highlights the sensitivity of EFPM 2.5 to fuel moisture content. The EFPM2.5 -CE relationship for wet fuels across several species (pines, bitterbrush, manzanita, etc.) and types (stems, leaves, duffs, etc.) in that study agrees better with the upper bound in Figure 4. For dry fuels (< 10% moisture content), however, it is closer to the lower bound and FEPS estimates. Providing that most laboratory studies focus on dried fuels (e.g., Hays et al., 2002; McMeeking et al., 2009), extrapolating the laboratory data to predict wildland fire emissions would require some positive adjustments, especially for smouldering combustion with low CE. Other factors such as wind and scale of burn could also impact the emissions of prescribed burning (Yokelson et al., 2013). For a similar range of fire-integrated CE [0.86–0.92, or modified combustion efficiency (MCE) 0.89–0.94, see Table 2], Burling et al. (2011) report EFPM 2.5 of 10 to 25 g/kg for conifer forest understory burns, slightly lower than observed in this study (22 to 33 g/kg). 236 T. Malamakal et al. 3.3 Smoke impact scenarios Although multiple agencies carried out prescribed burning in LTB (Figure 1), strict guidelines have been used for smoke management. Preferred weather conditions include an unstable boundary layer (i.e., no inversion) with moderate winds to carry smoke outside the basin. Burns usually begin in the late morning and continue through early afternoon to take advantage of the strong turbulent updraft in the afternoon. While the ignition and flaming phase stop completely in 2 to 5 hours, smouldering can continue overnight and even into the next day. Clear impact of prescribed burning smoke on ambient air quality is not often observed and/or reported. Out of 60 burns in Figure 1, the FEPS-HYSPLIT model (with WRF meteorology) noted only a few scenarios (Table 3) where smoke was transported over one or more of our ambient monitoring sites producing ≥ 2 μg/m3 impact on hourly PM2.5 concentrations. Table 3 Prescribed burns with potential impacts on air quality during the fall 2011 monitoring period Ignition start time (LST) Burn duration*† (hours) 10 (pile)–100% 0700 4 32 10 (pile)–100% 1000* 5 39°15’51”N 10/19/2011 Understory 119°58’35”W 8 90–100% 1000 7 39°08’02”N 10/18/2011 120°13’04”W 2 10% 1000* 2 Date Burn type Burn area Fuel moisture* (acres) Burn ID Burn location Angora1 38°52’21”N 10/20/2011 Understory/ 120°03’02”W piles 32 Angora2 39°52’25”N 11/02/2011 Understory/ 120°03’01”W piles North1 West1 Piles Notes: *Estimated values. †Assuming linear progression of fire. Angora Fire (6/24–7/2/2007) was the largest wildfire within LTB in the last decade, burning 3100 acres of forest south of Lake Tahoe (Safford et al., 2009). Since the Angora Fire, the Lake Tahoe Basin Management Unit (LTBMU) has been carrying out prescribed burns in the Angora area to clean out debris to reduce future fire danger. Model simulations for two of the burns on 10/20/2011 (Angora1) and 11/2/2011 (Angora2) predict smoke transport to northeast [Figure 5(a) to Figure 5(b)]. Five to eight hours after ignition the smoke starts to impact the air quality of South Lake Tahoe and Cave Rock as well as Bliss to a lesser degree. The smoke appears to move along the eastern side of the basin with horizontal transport limited by the mountain ridges. The North Lake Tahoe Fire Protection Department (NLTFPD) and Nevada Division of Forestry (NDF) have consistently conducted small-scale (< 10 acres) prescribed burns on the north shore of Lake Tahoe. Due to the proximity to the burn areas, Incline Village can sometimes experience the smoke. Figure 5(c) shows an example occurring on 10/19/2011 (i.e., North1). The smoke is transported southeast, covering Incline Village and Cave Rock in a few hours, though the impacts are not severe. Prescribed burns on the western bank had been carried out by LTBMU and CA State Park from time to time. The smoke could be transported northeast impacting Tahoe City and Incline Village, as demonstrated in Figure 5(d) (i.e., burn West1). These burns are usually very small in size (< 5 acres). Prescribed burn smoke impact in the Lake Tahoe Basin Figure 5 237 FEPS-HYSPLIT (WRF 2 km meteorological data) simulated surface PM2.5 concentrations (μg/m3, 0 to 25 m AGL average in log scale) during four prescribed burning events at (a) 1300 LST, 10/20/2011 (b) 2000 LST, 11/2/2011 (c) 1600 LST, 10/19/2011 (d) 1500 LST, 10/18/2011 (see Table 3 for details) (see online version for colours) Note: The diamond symbol indicates the prescribed burn location while the numbers mark the ambient monitoring stations as in Figure 1. 3.4 Verification of model simulation On 11/2/2011, the South Lake Tahoe site recorded a PM2.5 peak of 37.4 μg/m3 at 0700 LST, well above the typical levels defined by the 10th and 90th percentile of the diurnal data (Figure 6). A simultaneous peak was also observed at Cave Rock. These 238 T. Malamakal et al. peaks correspond well with the maximum impact of the prescribed burn by LTBMU on 11/2/2011 (Angora2), as simulated by FEPS-HYSPLIT with the WRF meteorological data. The model, however, predicts lower concentrations and does not capture a secondary peak at both sites around midnight of 11/3/2011. This is consistent with underestimation of fuel loading and/or smouldering emission factors, though certainly the unaccounted PM2.5 could result from other sources. The late afternoon PM2.5 highs on 11/3/2011 at both sites also deviate from the normal diurnal pattern. There are no prescribed burning records for that day but a continuous operation of the fire crew in adjacent plots (i.e., unrecorded burns) is possible, according to LTBMU. The model does indicate transport of smoke from the previous day’s burn over the two sites through the evening of 11/3/2011. Snowfall began ~1900 LST on 11/3/2011, which likely extinguished the combustion and removed particles from the air. Figure 6 Measured hourly PM2.5 concentrations at, (a) site 4 (South Lake Tahoe) (b) site 5 (Cave Rock), compared with FEPS-HYSPLIT predicted smoke PM2.5 concentrations at the sites originating from the 11/2 prescribed burn by LTBMU (Angora2, see Table 2) (see online version for colours) (a) (b) Notes: Models are based on WRF or NAM meteorological data. Arrows indicate the ignition time. The shaded region indicates the range of diurnal variations defined by the 10th and 90th percentile of diurnal data at the site. All times are in LST. Using NAM instead of WRF data causes a shift of modelled smoke arriving time. This is especially clear for Cave Rock [Figure 6(b)]. The mountain barrier consistently shown in Figure 5(a) to Figure 5(b) is not resolved in the simulation with NAM (12 km resolution), which predicts the plumes to extend eastward compared to the WRF simulation causing changes in the smoke forecast. The 10/20 burn (Angora1, see Figure 7) is an example where smoke impact could show up one and half days after ignition. FEPS assumes smouldering long (> 2 days) after the active ignition period. The late night PM2.5 peak on 10/22/2011 at South Lake Tahoe is consistent with the model predicted strong impact from the 10/20 burn in the Angora area [Figure 7(a)]. However, the PM2.5 highs are within the typical range of diurnal pattern, and no such effect is predicted with the NAM data. Less confidence could be placed on asserting the influence of this burn. The model also predicts small impact on the other sites relative to the site-specific diurnal variations [e.g., Figure 7(b)]. Prescribed burn smoke impact in the Lake Tahoe Basin Figure 7 239 Measured hourly PM2.5 concentrations at, (a) site 4 (South Lake Tahoe) (b) site 3 (Bliss State Park), compared with FEPS-HYSPLIT predicted smoke PM2.5 concentrations at the sites originating from the 10/20 prescribed burn by LTBMU (Angora1, see Table 2) (see online version for colours) (a) (b) Notes: Models are based on WRF or NAM meteorological data. Arrows indicate the ignition time. The shaded region indicates the range of diurnal variations defined by the 10th and 90th percentile of diurnal data at the site. All times are in LST. Figure 8 Measured hourly PM2.5 concentrations at, (a) site 1 (Incline Village) (b) site 2 (Tahoe City), compared with FEPS-HYSPLIT predicted smoke PM2.5 concentrations at the sites originating from (a) 10/19 prescribed burn by NLTFPD and (b) 10/18 prescribed burn by LTBMU (North1 and West1, respectively, see Table 2) (see online version for colours) (a) (b) Notes: Models are based on WRF or NAM meteorological data. Arrows indicate the ignition time. The shaded region indicates the range of diurnal variations defined by the 10th and 90th percentile of diurnal data at the site. All times are in LST. Figure 8(a) and Figure 8(b) show the smoke impact at Incline Village (10/19 burn, i.e., North1) and Tahoe City (10/18 burn, i.e., West1). The burning contribution to PM2.5 is generally minor, according to the simulations. It would have been larger if higher emission factors, as suggested by Figure 4, were used in FEPS. Estimating the contribution of the 10/19 burn to Incline Village is challenging since the distance between the burn plot and monitoring site is close to the model grid size and because of difficulties to model boundary layer movement (Pournazeri et al., 2012). Nonetheless, smoke impact is expected when westerly or northwesterly winds prevail, which happened during the first five hours of this prescribed burning and after midnight of 10/21/2011. There is an unusually high afternoon PM2.5 peak at Tahoe City on 10/18/2011 240 T. Malamakal et al. [Figure 8(b)], consistent in time with the transport of smoke from the burn area to the monitoring site. The predicted smoke peak, however, appears to be off by a few to several hours. 4 Conclusions A smoke dispersion model such as HYSPLIT can be a simple yet effective tool to predict/evaluate the influence of prescribed burning in sensitive environmental zones such as Lake Tahoe. In this approach, particles (i.e., PM2.5) are treated as inert tracer without chemical interaction with other atmospheric constituents. The model grid resolution should be adequate to reflect the topography while incurring manageable computation times. Burns could be modelled individually with the effects being accumulated. The emission information was found to be the most challenging part of the study. Prescribed burns were not always recorded with complete information such as fuel load, moisture content, ignition time, rate of progress, and burn duration that are required by the FEPS to calculate temporally-resolved (e.g., hourly) PM2.5 and heat release. Some known burns are completely missing in the records. Since field observations could not be made for each of the burns, inaccurate burning information leads to uncertainties in evaluating smoke transport and the overall effect of prescribed burning on air quality. Measurements at three prescribed burn events show increasing fractions of smouldering combustion and decreasing CE as the burn progress. EFPM 2.5 generally increases with the decreasing CE, but with a wide range of EFPM2.5 / (1 − CE ) ratio. FEPS, in its default setting, often reports lower CE than measured values. It also underestimates the PM2.5 emission factors for a given CE by up to a factor of 6. The high-end emission factors measured in this study are consistent with those from laboratory combustion of relatively moist fuels. Since most laboratory studies focus on dry fuels, emission models based on laboratory data may need to be positively adjusted for real-world burns. During our three-month observing period in fall 2011, serious and obvious impact from a known prescribed burn on air quality (e.g., causing short-term PM2.5 concentrations several times the three-month averages or exceeding the 24-hr PM2.5 standard) at one or more of the ambient monitoring sites around Lake Tahoe was rare. This should be the case if the prescribed burning guidelines are strictly followed by all the agencies. A few scenarios with potential impacts were identified by the FEPS-HYSPLIT model. Model predicted smoke contributions were consistent with elevated ambient PM2.5 concentrations in two cases, and a higher model resolution generally produce more accurate smoke arrival times. In other cases, the model performance was difficult to evaluate due to low predicted smoke contributions relative to the typical ambient PM2.5 level. Future studies may include hourly measurement of more specific biomass burning markers, such as water soluble potassium and/or levoglucosan, at the ambient monitoring sites to reduce the ambiguity in model evaluation and facilitate development of optimal modelling parameters. Prescribed burn smoke impact in the Lake Tahoe Basin 241 Acknowledgements This project was funded by the USDA Forest Service through the Southern Nevada Public Land Management Act (SNPLMA Round 11). The authors thank John Washington from LTBMU and Roland Shaw from NDF for their assistance in the field and providing the burn information. The authors also appreciate Tim Brown for providing WRF data, Keith Szelagowski for organising the database, and Steve Kohl for laboratory analysis. The reviewers’ comments are greatly appreciated. The conclusions are those of the authors and do not necessarily reflect the views of the sponsoring agencies. References Anderson, G., Sandberg, D. and Norheim, R. 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