A STUDY OF TRACER TRANSPORTS BY PLANETARY SCALE WAVES IN THE MIT STRATOSPHERIC GENERAL CIRCULATION MODEL by GARY EDWARD MOORE B.S., Walla Walla College (1973) SUBMITTED IN PARTIAL FULFILLMENT OF THE REQUIREMENTS FOR THE DEGREE OF MASTER OF SCIENCE at the MASSACHUSETTS INSTITUTE OF TECHNOLOGY (AUGUST, 1977) Signature of Author [,.11- epartment of Meteorology, August 29, 1977 Certified by Thesis Supervisor Accepted by............................................................. Chairman, Department Committee WIT Ial A Study of Tracer Transports by Planetary Scale Waves in the MIT Stratospheric General Circulation Model by Gary Edward Moore Submitted to the Department of Meteorology on August 29, 1977, in partial fulfillment of the requirements for the degree of Master of Science. ABSTRACT The quasi-geostrophic global stratospheric model at MIT developed by D. Cunnold, F. Alyea, N. Phillips, and R. Prinn is used to study the zonal and time-averaged transport of potential temperature and ozone by the planetary zonal wavenumbers 1-6. Several types of covariances between the winds, geopotential, and the tracers are calculated in order to evaluate the directions and strength of the fluxes and the winds causing the fluxes. The eddy covariances show that, in the lower stratosphere, ozone and potential temperature b6th move polewards and downwards in longitudes of low geopotential, in agreement with observations. In the upper stratosphere and lower mesosphereozone and potential temperature are negatively correlated. In the midlatitudes of this region the eddy flux of potential temperature horizontally diverges; with downwards eddy fluxes occuring in low latitudes and upwards fluxes occurring in high latitudes. The meridional eddy flux of ozone is found to be only 1-3% efficient since the meridional wind and ozone waves are nearly 900 out of phase. Another contributing factor to the inefficiency of the eddy transport is the tendency for the transient eddy flux to nearly cancel the standing eddy flux in the lowest layers of the stratosphere. The total flux of ozone is further diminished in some regions of the atmosphere by the opposition of the eddy fluxes to the mean circulation flux. In the final chapters, some of the calculated covariances are applied in an attempt to calculate the eddy diffusivities. Because of the unsuitability of the mathematical form of the equation used to define the eddy diffusivity, Kyy, and the uncertainties in the averaged covariances; Kyy could not be estimated in a straightforward manner with any accuracy. The eddy diffusivity Kyy is then assumed to be the product of the meridional EKE and the timescale typical of the mixing processes taking place. The timescale was calculated two ways. One used the LaGrangian integral timescale of Taylor's dispersion theorem. The other was an attempt to find the timescale typical of the advective processes by using a mean length scale and the mean zonal wind. Both results showed reasonable agreement of the timescale with previously observed timescales in the atmosphere. Thesis Supervisor: Ronald Prinn Title: Associate Professor TABLE OF CONTENTS Page INTRODUCTION 1. The stratosphere: 2. Representation of the eddy fluxes 3. A consistent model of tracer transport in the stratosphere 4. Introduction to the MIT stratospheric GCM 5. A comparison of selected model covariances with observation 6. The behavior of the meridional and vertical eddy wind a descriptive review of its behavior velocities 7. A survey of the eddy fluxes of ozone and potential temperature in the model 8. A survey of the phase difference between the winds and the tracers 9. Introduction to the mixing length hypothesis 10. A first attempt at obtaining eddy diffusivities 11. The use of Taylor's dispersion theorem in determining eddy diffusivities 12. Conclusions and summary ACKNOWLEDGMENTS APPENDIX REFERENCES TABLE I FIGURE CAPTIONS FIGURES -1Introducion A large numerical general circulation model(GCM) such as the stratospheric model developed by Cunnold et al. (1975) allows a study of the simulated atmosphere to an extent not achieved by observation. Physical transport processes associated with certain mathematical terms can easily be switched on and off for the purposes of study. Furthermore, the predicted variables are easily analyzed without having to be modified as observations like radiosonde data are. A diagnostic study of the eddy transport of tracers such as potential temperature and ozone in the MIT Stratospheric GCM should be helpful in determining whether the simulations of the atmosphere bear a resemblance to observations. Secondly;'the diagnostic study should be helpful in both the interpretation and as a guide for future observations such as improved remote sensing by satellite. The average transport by the eddies of such tracers as momentum, heat and certain chemical species presently remains one of the least understood of the processes occurring in the general circulation. The actual eddy transport of a tracer is the result of the little understood complex interactions occurring between the zonal waves which shears, stretches, and deforms parcels of air. The wave interactions are reflected in the behavior of the tracer and wind variation's amplitude, and in the variation of the phase angle between the two. By making a diagnostic study of the behavior of the wind and tracer amplitudes and their phase differences, as a function of zonal wavenumber, one might possibly find a simple means of roughly describing the tracer transport done by the long planetary waves. -21. The Stratosphere: A Descriptive Review of its Behavior A great body of observational studies of the stratosphere have been done by members of the Planetary Circulations Project at MIT. Historically, some of the first statistically significant studies were conducted on the IGY (1957-1958) data collected in the region 10-100 mb. The result of these investigations are detailed quite thoroughly in Barnes' (1962) report. Further data for the region 2-200 mb have been summed up quite neatly in a report given by Newell et al. (1974). Newell has also organized and summar- ized the observations of tracer transports in the lower stratosphere in an earlier paper (Newell, 1963). The mean temperature field shows a surprising feature in that the 10200 mb layer generally has warm poles and a cold equator, despite radiational cooling at high and midlatitudes, and warming in low latitudes. The stratospheric profile exhibits its greatest complexity during the winter. Above 100 mb during this period, the pole becomes cooler than midlatitudes. Consequently one finds a CWC pattern on traveling from the pole to the equator. The observed zonal wind field is dominated by a winter polar jet which increases at 40* from a minimum near 50 mb to what appears to be a maximum at about .2 mb. During the summer, easterlies extend upwards from around 30 mb at the midlatitudes to a broad core which Murgatroyd (1969a) shows to close at .2 mb. The zonal averaged meridional circulation was once a source of controversy until the eddy heat flux observations presented by Newell et al. (1974) were used by Louis (1974) to deduce the circulation from the thermodynamic equation. The circulation shows a winter Hadley cell which extends into -3the lower stratosphere. the stratosphere. The Ferrel cells of both hemispheres also penetrate Thus a two-cell circulation operates in the stratosphere with a direct cell in low and midlatitudes, and an indirect cell at high and midlatitudes. As one compares a 50 mb geopotential map with a 500 mb map, it becomes evident that there is a qualitative difference between the stratospheric and tropospheric eddies. The smaller eddies of the troposphere disappear, leaving only planetary scale waves 1-3 to dominate at 50 mb. Sawyer (1965), in an address to the Royal Meteorological Society, mentioned some work done by G. R. Benwell that showed a phase relationship between 50 and 500 mb, but there was no apparent correlation of the amplitudes of the waves between the two levels. White (1954) was the first to note that the horizontal heat flux in the lower stratosphere was counter gradient. Peng (1963) and Newell (1965,1972) firmly established that the eddy heat flux is northwards in the lower stratosphere right up to high latitudes where a minor southward flux occurs. A counter- gradient heat transport by the eddies directly implies that EAPE is being converted to ZAPE which maintains the positive zonally averaged temperature gradient. Unfortunately the vertical transient eddy heat flux cannot be directly measured. However, Oort and Rasmussen (1971) found that the stand- ing eddies in the lower stratosphere transport heat downwards towards the tropopause. In the lower stratosphere the diabatic heating is sufficiently small to allow the calculation of adiabatic vertical velocities from the thermodynamic equation. Jensen (1961) made a pilot study and found a downward motion of less dense (warm) parcels and an upward motion of denser (cooler) parcels. Oort (1964) also found a convergence of the vertical transport of -4geopotential. Such a convergence means that pressure forces are doing work on the stratospheric air mass. One might draw the tentative conclusion that the stratosphere appears to be driven from the tropospheric motions in a fashion that Newell calls a "refrigerator" mode. Loisel and Molla (1962) found that by using adiabatic vertical velocities the vertical and northward wind components of the transient eddies are negatively correlated in the lower stratosphere, but positively correlated in the troposphere. Further work by Newell et al. (1974) found that negative values of the standing eddy covariance between V and W occur up to 10 mb. Dickipson (1962) discussed the momentum budget of the IGY wind data. The data show a horizontal convergence of angular momentum into the regions of maximum zonal flow by the eddies. Newell (1972) used five years of wind data to study the northward eddy transport of angular momentum. He also found a maximum of northward eddy momentum flux just south of the polar night jet which fluctuated as a function of the jet velocity. The counter- gradient flux-of momentum indicates that a conversion of EKE to ZKE is taking place. Of all the tracers measured, the distribution of ozone in the lower stratosphere has probably been studied the most. It was once surmised that ozone was in photochemical equilibrium; but the ozonesonde network observations show that the maximum total columnar amounts of ozone are found in high latitudes during the spring. Such observations are in direct contra- diction to the photochemical equalibrium theory which implies an equatorial maximum of ozone during the summer. Martin (1956) found from observations of the horizontal eddy ozone fluxes that ozone must be removed from the low latitude and moved northwards. Newell (1963) used IGY data to find that the meridional flux by the transient -5and standing eddies is predominantly polewards in midlatitudes. The spread of radioactive tungsten 185 from equatorial nuclear tests has been studies by Stebbins (1960), Feeley and Spar (1960), and Newell (1963). Feely and Spar (1960) used a Gaussian model to simulate the spread of the debris in the lower stratosphere. They found eddy diffusivities in the horizontal of 1-106 m2 sec-1 and in the vertical of the magnitude 1-40 m2 sec~ . Newell (1963) published meridional-vertical distributions of tungsten 185 which showed the northward and downward spread of the center of gravity of the radioactive debris cloud in the lower stratosphere. -6- 2. Representation of the Eddy Fluxes In the atmosphere there are four types of wave motion. Waves are classified as to whether they are standing or traveling waves or steady or transient waves. Standing waves are geostationary and are distinctly rela- ted to forcing features of topography and heating at the ground. Traveling waves are generally will-o'-the-wisps since their source of energy fluctuates as a function of longitude and time. It is impossible to separate transient standing wave amplitudes from steady traveling wave amplitudes; thus only steady stationary waves can be separated from the total eddy quantity. The model of Cunnold et al. (1975) that is used in this study specifies the wave components as spherical harmonics at a given level. The eddy amplitudes at a given latitude, level, and instant of time can be written as a zonal Fourier series, i.e., In this study six zonal wavenumbers plus the zonal mean are used to represent a variable in the model. The averaging scheme of Starr and White (1951) will be applied in describing the covariances of variables. denoted by brackets, <( )>. a star, ( )*. The zonal averaging operator is The zonal deviation from the mean is shown by The time operator shall appear an an overbar, ( ), time deviation is represented by a prime, ( )'. while the The order of applying the averaging operators results in different kinds of eddy products. If the time operator is applied first, the product of two variables A and B is written following Starr and White (1951) as: -7- ) 3) (2.2) Term 1 of (2.2) is simple the product of the time-zonal means. The second term represents the eddy product due to standing steady waves. The third term represents the contribution due to the transient standing waves and both. the transient and steady traveling waves. If the zonal-averaging operator is used before the time-averaging operator, the two-variable product, AB, becomes: <AI3> =-<A> <0e> + <A><1'> '(1 +,Af~t Q) (2.3) (3) The first term of (2.3) is the product of the zonal-time averaged terms and it does not equal the first term in (2.2). The second term is the pro- duct resulting from correlations between transients in the zonally averaged variables. The last term contains the amplitude contributions from all four types of waves. The second term of (2.2) is calculated by taking time averages of the B and C coefficients of (2.1). Since the longitudinally dependent terms of the Fourier series are orthogonal, the zonally-averaged product of two variables, P and Q, can be written as: (pf > 6 s Z ( 60 %89Ph c-Qc) nh (2.4) The third term of (2.2) is calculated as a residual by subtracting the first two terms on the right-hand side of (2.2) from the total covariance. -8The amplitude of a given zonal wavenumber is given by the relation: W~I = -S BQ ,+ IN ) 16,(2.5) % (2.5) The phase angle of a given zonal wavenumber is found from the relation: 0 V,1 rt (2.6) gIC1 The amplitude and phase angle contain all of the information to be known about the waves. The cpvariance of two quantities A and B can also be found directly by going from a spherical harmonic representation to a Gaussian-weighted grid Once on the grid, the multiplication space via a Fourier transformation. of the two variables can be carried out. An exponential filter is used to smooth the grid field so that the truncation of the product will not result The exponential filter has the added in significant negative overshoot. advantage of no phase shift and the conservation horizontally averaged AB value. After filtering,the reverse Fourier transformation is used to trans- form back to spherical harmonics. The transformation automatically truncates the product and eliminates aliasing. The zeroth order harmonic becomes the zonal average of AB that is desired. The spectral-grid-spectral method (SPS) has the advantage of not specifying more information in the meridional direction than the spherical harmonics allow, as is sometimes the case with the zonal Fourier series technique (ZFS). -9A Consistent Model of Tracer Transport in the Stratosphere 3. After reviewing previous observations, Newell (1964) proposed a logi* cally consistent model based on the phase relations between T * , * V , W and , * 03 Newell spoke of the tracer transports in the lower stratosphere as . arising naturally from the motions and temperature patterns of the troposphere. In a midlatitude amplifying disturbance the temperature wave lags the geopotential wave by 0-ff radians. The lag results in perturbation potential energy generation and a westward slope of the lines of constant phase with height. The disturbance amplifies due to cold advection beneath the upper tropospheric trough, and warm advection under the upper tropospheric ridge. The vertical motions must be downwards in the air behind the midtropospheric trough and upwards ahead of the trough so that the divergent motions can make the necessary geostrophic vorticity change in the upper troposphere. * The results pattern of winds imply positive correlations between V * and T . * , W Geopotential and meridional velocity are negatively correlated, while the vertical velocity is positively correlated with geopotential. Figure 1 shows the typical phase relations of a geostrophic disturbance in the troposphere. * ratio ozone, X , Note that in mid-troposphere the perturbation mixing is generally positively correlated with temperature, so that its eddy flux is generally polewards and upwards. In the lower stratosphere the vertically propagating waves phase -still slopes westwards with height. Temperature, ozone, and the meridional winds of the disturbance are still positively correlated. The crucial difference, shown * in Figure 1, is that the lines of constant phase for W do not slope west- * wards at the same slope the V lines do. As a result, in the lower -10stratosphere the vertical velocity advances in phase relative to V * T , * * and X so that all of the correlations are negative. The phase relation between the geopotential and the winds remains of the same sign as in the upper troposphere. "refrigerator". Newell (1963) likened the lower stratosphere to a In this region warm parcels are further adiabatically warmed as they are forced to descend down the temperature gradient into the upper troposphere, thus warming it. Cooler upper tropospheric parcels are forced up the temperature gradient, adiabatically cooling as they go, to where they end up cooling the lower stratosphere. An interesting question is: why does the vertical velocity's phase change relative to the cool trough as one goes from the troposphere to the stratosphere? It would seem that the air motions are trying to occur in such a manner as to decrease the stability of the lower stratosphere. The decrease of stability implies an increase in potential energy due to the tropospheric waves. should result. w equation. Thus an upwards eddy geopotential flux, <W 4> >0, Sawyer (1965) addressed this question with a comment on the If diffusion is neglected, and there is to be a small merid- ional circulation, then the differential vorticity advection term in the w equation has to oppose the thickness heating term in order for the equation to be balanced. For such an opposition to occur in a cooling layer, there must be a negative correlation between vorticity and vertical velocity. Thus rising motion occurs above the geopotential maxima and sinking motion above the minima. The result, again shown in Figure 1, is consistent for a mechanically cooled lower stratosphere. In the case at hand it is of interest to discover whether geostrophic disturbances of limited zonal wavenumber can explain the observations presented. Although the phase model proposed seems, by observation, to -11physically hang together, it has by no means been proven to be the only consistent scheme. A GCM might uncover different relationships. The limited set of physics in the GCM make is possible to deduce a physical mechanism whereby a batter parameterization can be deduced. The GCM can also produce those correlations that are the "missing links" in the observations. An example would be the direct calculation of all covariances that contain the vertical velocity. The GCM has a final obvious advantage in that it can be extended to regions that are not easily observed. -124. Introduction to the MIT Stratospheric GCM The data used in this study come from various runs of the quasi-geostrophic model of Cunnold et al. (1975). The reader is referred to the referenced cited for a more detailed explanation of the dynamical and chemical formulations in the model. At best only a simple physical descrip- tion of the model will be given in this section. The model has 25 prediction levels in the vertical axis which is in increments of log pressure. The lowest level is the ground and the highest level is centered at 71 km. The model uses a global spectral technique and represents each variable at a level with 79 spherical harmonics. The longitudinal truncation only allows zonal waves of up to wavenumber six. The set of dynamical equations used are the energetically consistent balance equation set described by Lorenz (1960). The model does not pre- dict the globally-averaged temperature, but rather it is externally specified. Another simplification is that the horizontal advection due to the nondivergent wind is neglected. Vertical transport of ozone and momentum by the subspectral scale eddies is simulated with a specified vertical eddy diffusivity. Frictional stress, topography, and all types of thermal forcing are included as terms in the vorticity and thermodynamic equations. The ozone mixing ratio is predicted from two equations which separately predict the globally-averaged ozone mixing ratio and its deviation from the global mean. The coupling between both prediction equations comes only through a single term in the global average prediction equation. This term is the vertical divergence of the globally-averaged flux due to the product of the deviations of ozone mixing ratio and the vertical wind from the global mean. -13The photochemistry in the model includes reactions of odd nitrogen and water vapor with odd oxygen. The photochemistry and the dynamics are coupled through both the temperature dependent reaction rates and the diabatic heating due to solar radiation absorption by ozone. -145. A Comparison of Selected Model Covariances with Observation * * Of crucial importance to the phase model is the <V W > covariance * which sums up the phase relation between V eddies. * and W for all classes of Because of equatorial symmetry, only the winter and spring northern hemispheric seasonal averages are presented in Figures 2 and 3 respectively. * A positive average correlation exists between V the summer and winter months in the troposphere. * and W during both The positive correlation indicates that upward and poleward motions are taking place in the model as they do in the observed atmosphere. The winter hemisphere has correspond* ingly larger covariances due to the increased magnitudes of the V winds. * , W The region of 200-30 mb possesses a negative average correlation * between V * and W for both summer and winter seasons. The observed adia- batic vertical wind correlations are in a sense justified since it seems that long planetary waves with geostrophic winds can have velocity components that result in the negative correlations. In the winter season a maximum covariance of one-half the magnitude of the upper troposphere occurs at about 90 mb at 40-50*. In the summer the maximum still lies at 90 mb, but it is shifted much closer to the equator, having a peak near 20-30*. While the lower stratospheric maximum is about the same magnitude as the peak in the winter, it is almost five times larger than the upper tropospheric covariances. This fact indicates that the lower stratosphere has much less seasonal variability of the mixing slopes than the troposphere. Above 30 mb the covariance patterns again change. The winter season * undergoes a shift back to positive average covariances between V * and W The positive covariances are about as large as those in the lower stratosphere up at about .5 mb. It is not apparent at this point whether the -15vertical velocity's phase has slipped back to that of the troposphere, or whether it has advanced in phase half a vertical wavelength. The summer ** hemisphere maintains the negative V ,W at high to midlatitudes. correlation through the stratosphere At equatorial latitudes a slight positive corre- lation eixsts up to .5 mb. Above .5 mb, the low latitude winter season correlations again become negative. In the summer season the positive correlation in the equatorial regions also go negative. * * After this once over of the V ,W average covariances, one sees several unique regions in the vertical, namely 1000-200 mb, 200-30 mb, 30-.5 mb, and above and fall. ,.5 mb., The regions are quite distinct especially in the spring These two seasons have nearly symmetric covariances that are almost identical to one another. In the upper stratosphere there appears to be two distinct latitudinal regions. The regions in the vertical are represented by dominantly positive (1000-200 mb), negative (200-30 mb), and positive (30-.5 mb) covariances. The +,-,+,-, pattern looks suspiciously as if it might have its roots in vertically periodic motions. * * The vertical flux of geopotential by the eddies, <W $ >, indicates the upwards or downwards export of potential energy. A vertical conver- gence of this covariance indicates that a source of energy within the layer exports eddy pressure work to other regions. Figures 4 and 5 show the vertical eddy flux of geopotential. During the winter season, eddy potential energy propagates vertically upwards at high to midlatitudes clear to the top of the model. the eddy covariance occurs in the troposphere. Vertical divergence of This result is hardly sur- prising in view of the present knowledge of the energy cycle of the troposphere. Convergence occurs from 200 mb to about 25 mb. Such a finding -16reinforces Oort's (1964) analysis which found the lower stratosphere to be driven by the troposphere and not by internal energy sources. occurs above 25 mb up to about 2 mb at 300 and .3 mb at 70*. occurs above the region of divergence. Divergence Convergence One would expect to find conver- gence near the upper boundary as pressure forces propagating from below do work on the layer adjacent to the rigid lid. The most peculiar feature in the winter hemisphere is the strong region of divergence in the low latitude region .1-.5 mb. In the lower mesosphere the mean temperature has a maximum at midlatitudes and minima at the poles and equator. Although the eddy heat fluxes are directed along slopes going northwards and downwards, the eddy heat flux at low latitudes is downgradient like the stratosphere. An examination of the mean temperature and zonal wind gradients in both the vertical and horizontal did not seem to reveal any favorable conditions for baroclinic instability as a source for the downwards propagating eddy potential energy flux below this region. How- ever a growing disturbance might occur if the ozone radiative-dynamical coupling described by Leovy (1964) occurs. If significant coupling occurs, EKE is generated when parcels carry excess ozone on the downward side of their trajectory and undergo a net heating due to solar absorption. Some- times the EKE generation outstrips the radiational damping of the wave motions. Barotropic instability cannot be ruled out either. Since the region of the presumed instability occurs southwards of the polar night jet where large positive horizontal shears can make a change of sign in the potential vorticity gradient. The question can be settled only by looking at more covariances and their divergences. The summer season looks much like the winter season and high to midlatitudes; the only difference is that the magnitudes of the convergences and -17- divergences are much smaller than in the winter. The low latitudes of the summer season lack the odd feature of the winter season in the upper stratosphere and lower mesosphere. During the spring and fall seasons there is still an upwards eddy flux of geopotential in midlatitudes. Also there is still convergence in the lower stratosphere, divergence from 20 mb to the stratopause, and convergence above that. At high latitudes there are downward eddy fluxes of geopotential for both hemispheric seasons. It is of interest to check on the sign of the average producE of the vertical and horizontal eddy fluxes in order to determine the direction of the slope 'along which the eddies are moving ozone. * * * Figures 6 and 7 show the * seasonally-averaged eddy covariance, <V W 03 03 >. During the winter season ozone is generally transported downwards and equatorwards in the troposphere. In the lower stratosphere at midlatitudes, ozone is transported downwards and polewards in the region up to 30 mb. maximum covariance occurs near 100 mb at 50*. The Thus it is quite possible for large amounts of ozone to be brought into the troposphere during the formation of an upper tropospheric thermally-indirect front. Danielson (1968) found from analyzed observations that ozone-rich air is brought down into the troposphere during a frontal occurrence. Above 30 mb, the midlatitude winter season shows a tendency to have ozone brought upwards and polewards with a slope sign like that of the troposphere. In the low to midlatitude mesosphere, the slope of the ozone fluxes appears to be directed downwards and polewards. Ozone convergence is taking place in this region. In the summer hemisphere the tropospheric and lower stratospheric covariances are smaller; however, the direction of the slope remains unchanged. --18The only significant difference is that the polewards and downwards slopes extend to the top of the model throughout almost all the hemisphere. During the spring and fall seasons there are still polewards and upwards directed flux slopes in the troposphere, and poleward-downwards slopes in the lower stratosphere. In the region 1-20 mb, a polewards and upwards slope occurs in midlatitudes for both the spring and fall seasons. The sign of the average product of the horizontal and vertical eddy fluxes of temperature are also calculated in order to note the thermal behavior of certain regions. of <V W T T >. * the <W Figures 8 and 9 show the seasonal averages A connection can be drawn between these covariances and * # > dovariance by remembering that Eliassen and Palm (1960 * * Equation 10.12) showed that positive <W $ > directly implies a poleward heat flux for quasi-geostrophic waves. The winter season shows the eddies in the troposphere to be dominated by mainly polewards and upwards slopes along which heat is transferred. In the upper troposphere near the tropopause gap the direction of the flux slopes changes from polewards and upwards to polewards and downwards. change in the direction of the slope is lower than in The the case of ozone. The lower stratosphere up to about 30 mb has a polewards and downwards slope along which the eddies move heat. This result is consistent with Newell's (1964) concept of the behavior of the lower stratosphere. Since the horizontal eddy flux direction is counter to the average temperature gradient the region sppears to be destroying EAPE and converting it to ZAPE. At the same time the vertical eddy flux is downgradient which indicates a conversion of EKE to EAPE. At very high latitudes the polewards and downwards slope, along which sensible heat is moved, persists up into the mesosphere. The covariance -19increases steadily with height from about 50 mb on up. Above 20 mb in the high to midlatitudes, the direction of the potential temperature fluxes tends upwards and polewards. In the low to midlatitudes an upwards and equatorwards direction of the heat flux is evident. A large heat source is implied at midlatitudes to balance the divergence of heat. The most interesting feature of the winter hemisphere is the strong region of an equatorwards and downwards flux of heat centered near 3 mb and 200. This feature appears to be connected with the <W * * # > feature during the winter season. The summer season shows the polewards and upwards flux of temperature in the mid to lower troposphere. While the stratosphere and the mesosphere have the expected polewards and downwards flux slopes that are opposed to those in the troposphere, the covariances in the stratosphere are miniscule compared to the winter season as the observations dempnstate. The spring and fall seasons present a confusing situation in regard to the direction of the heat fluxes. The lower stratosphere up to 30 mb of both spring and fall have polewards and downwards eddy flux slopes. Above 30 mb both seasons possess a polewards and downwards flux slope at low and high latitudes which continues on up into the mesosphere. The midlatitudes for both seasons have a polewards and upwards flux slope above 30 mb. This behavior is similar to that in the troposphere. It is interesting to see how the two tracers correlate. A positive correlation is expected in the lower stratosphere due to the similarities of the source regions. The covariance of ozone to potential temperature is shown in Figures 10 and 11. -20The winter season shows ozone to be dominantly positively correlated to temperature below 3 mb. Above 3 mb the only positive correlation that extends into the mesosphere occurs only at very high latitudes. The only remaining region where a negative correlation exists is in the lower tropical troposphere where ozone is quite scarce since there is no significant local source, while the temperatures are quite large. In the summer season the positive correlation extends up to 5 mb)and above 5 mb a negative correlation exists. It should be noted that for both winter and summer seasons the changeover in the sign of the correlation occurs at about 10 mb near the equator. The spring season has a predominantly negative ozone-temperature corelation in the lower to midtroposphere. tion exists up to about 5 mb. Above 300 mb a positive correla- Above 5 mb the correlation becomes negative. The fall season has a negative ozone-temperature correlation only in the low latitude troposphere. The region of positive correlation extends up to 5 mb. The region above 5 mb and equatorwards of 600 has a negative ozone- temperature correlation. The negative correlation above 5 mb is probably due to the fact that the rate constants for the production and destruction of ozone are dependent on the exponential of the inverse temperature. As temperature decreases, the production rate increases slightly, while the destruction rate due to NO,0 decreases. In the region below 5 mb the bulk of the ozone is produced near the tropics; however, dynamical motions move ozone into warmer regions, thus making the correlation positive in the stratosphere. -21- 6. The Behavior of the Meridional and Vertical Eddy Wind Velocities A study of the eddy winds themselves is of prime importance since the winds make up one-half of the amplitude factor of a flux. phase lag between a tracer, For a given * Q , and the wind, the strength of the meridion- al wind of the eddies determines in part the size of the poleward flux which is of primary importance in this study. Another reason for the interest in the eddy winds stems from the need to compare the modeled eddy winds with the observations in order to see if the winds in the model are of sufficient accuracy so as to result in the proper eddy fluxes. A final reason for investigating the meridional wind amplitudes is that the decay and growth rates of the amplitudes of zonally propagating waves can be related to eddy diffusivities in a crude fashion as Green (1970) has pointed out. The model makes use- of only the horizontally nondivergent wind, V$, for the horizontal advection of heat or ozone. Thus the advection by the eddies will be considered to be done entirely by the nondivergent wind. Under these circumstances the nondivergent meridional wind relations of the form: (6.1) can be written. Figures 12, 13, and 14 show the area weighted variances <V2 > <(V 2 >9 and <(V')2> 22 respectively for the months of June and December of Run 26. The <V and <(V') 2 > are the steady standing wave, and residual transient eddy components respectively. -22The total meridional EKE, <V >, has a winter maximum at 200-500 mb and 500 which is about three times greater than the summer maximum at 500. The observed winter maximum according to Oort and Rasmussen (1971) is about 2 2 2 2 320 m /sec compared with the model's 700 m /sec2. The summer maximum is 2 2 2 2 observed to be 195 m /sec compared to the model's 263 m /sec2. One dis- tinct difference between the model's tropospheric meridional wind variances and the observed variances occurs in the equatorial regions. At the equator the observed total variance <V2> equals about 65 m2/sec2 compared with the model's huge value of 250 m 2/sec2 The difference in the variance can be ascribed to the fact that the model is a quasi-geostraphic model. Near the equator, the assumptions in- volved in the quasi-geostrophic approximation do not hold. The Rossby number near the equator becomes of order 1 or greater, therefore making it impossible to balance the Coriolis term with the pressure gradient term. The balance should occur between the pressure gradient term and the inertial term. By using the Coriolis force, the wind in the waves is strongly over- estimated. These spuriously large amplitude eddies make it quite difficult to calculate the interhemispheric tropospheric transport. The lower stratosphere of the model exhibits a strong dropoff in the EKE as one progresses from the troposphere to the lower stratosphere. At 650 and 50 mb, the winter observations show a variance of 210 m 2/sec 2, but 2 2 the model gives a value of only 150 m /sec2. height during the summer is even greater. The dropoff of EKE with Summer observations at 55* and 2 2 2 2 50 mb show values of 26 m /sec while the model has a value of 50 m /sec . The highest analyzed observations by Newell (1972) show the total winter meridional wind variance to be 225 m 2/sec2 at 10 mb and 600 while the model has a value of 240 m 2/sec2 at this location. Thus in the winter -23hemisphere the tropospheric eddies are two times too strong; while in the lower stratosphere they are too weak. By about the altitude of 10 mb the eddies appear to be about the right strength. The equatorial regions suffer from quasi-geostrophic theory breakdown; but despite the fact that the tropospheric meridional EKE is five times too strong, the variance at 10 mb of 10 m 2/sec2 agrees quite well with the values found by Newell (1972). On the average the summer hemisphere shows a tendency for the modeled meridional EKE to be one to two times greater than the observations. By studying the analysis of observations made by Oort and Rasmussen (1971), one finds that in the region 200-500 mb the ratio of the transient wave EKE to the steady standing wave EKE is about six during the winter, and it increases to about 25 during the summer. The midlatitude ratio ob- served in the model is slightly more erratic but it is generally in the range of four to ten during the winter and increases in the summer midlatitude regions to about 25 to 35. The tropospheric ratio of the standing EKE to the transient EKE seems to agree with observations in a satisfactory manner at midlatitudes. In the summer hemisphere, at 50 mb, the midlatitude steady standing wave EKE is greater by an order of magnitude than what is observed. The transient EKE appears to be twice the observed value as was the case in the lower troposphere. Above 50 mb both types of eddy variances fall off rapidly and settle down to a transient to standing wave ratio of five to ten. In the winter hemisphere the standing waves appear to be attenuated much too rapidly in the high to midlatitudes. At 50 mb and 600 the observa- tions show an EKE of 50 m 2/sec2 while the model has an EKE of 60 m 2/sec2 yet the standing EKE in the troposphere is two times too large. It seems -24- that the standing waves are sufficiently trapped so as to allow only the amount of variance that is observed. The transient waves are strongly trapped so that at 50 mb only the amount of variance comparable to the observations exists; despite the fact that in the troposphere the transient variance is two times too large. Above 50 mb the transient wave to standing wave amplitude ratio is about five to ten in midlatitudes. The standing wave spectra are plotted in Figures 15, 16, and 17 as a function of zonal wavenumber. Each spectrum has been plotted so that the summation over the zonal wavenumbers of all the amplitudes equals one. what is plotted is the fractional contribution to the total variance. 132, 40, 12, Thus The 1, pnd .089 mb levels are of particular interest since the levels each occur in a distinctly differently behaving section of the atmosphere. The horizontal resolution is limited to the equatorial region and the midlatitudes at 40*. The winter hemisphere standing wave spectrum exhibits a spectral gap at wavenumber 4 in the lower stratosphere. wavenumbers 3 and 5. In this region, maxima occur at In the upper stratosphere the gap disappears and wave- number 5 strongly dominates. As one progresses up into the mesosphere the peak moves to wavenumber 3 at 1 mb and finally to wavenumber 1 at .089. The shift to dominant lower wavenumbers is both observed and expected from theory. At the equator a spectral gap still appears at wavenumber 4 in the lower stratosphere. The maxima occur at wavenumbers 2 and 5, with wavenum- ber 2 being very dominant by 40 mb. It is not clear why a spectral gap should appear at the stationary wavenumber 4 since sources for the forcing of wavenumber 4 should be about the same as wavenumber 5. There is a possi- bility that wave energy is being reflected from the truncation at zonal -25- wavenumber 6, which makes wavenumbers 5 and 6 too large. The summer hemisphere exhibits maxima at wavenumbers 2 and 4 in the midlatitude lower stratosphere. In the upper stratosphere the maxima shifts to wavenumbers 1 and 3. At the altitude of 1 mb wavenumber 3 is very dominant. Upon progressing upwards to .089 mb an even more unusual spectrum exists where wavenumbers 1 and 6 dominate. The seeming dominance of wavenumber 6 may again be due to the spectral truncation. Figure 18 shows the energy-weighted zonal wavenumber contours. The weighted wavenumber is defined through the relation: L~~Yvxv*>''/ I (6.2) A comparison of Figure 18 with Figures 15, 16 and 17 shows that the addition of the transient wave variance weights the zonal wavenumber center of moment towards a higher wavenumber. In figure 18 one can see the Eulerian spec- trum characteristic baroclinic peak near zonal wavenumber 5. The shift of the spectrum towards lower zonal wavenumber shows up quite strongly at high latitudes and altitudes. The trapping of wavenumbers greater than 2 appears to be stronger during summer than winter. This fact is probably due to the easterlies and the zero line in the zonal wind field. The average phase change of the standing waves as a function of height is also of interest. Van Loon et al. (1973) show that the zonal wavenumbers 1 and 2 vary roughly as ffand n/2 radians per 30 km respectively. At mid- latitudes the observed phase of wavenumber 1 varies linearly with height. Wavenumber 2 at midlatitudes shows a larger rate of phase variation near the ground. -26Figures 19, 20, and 21 show the phase in radians as a function of height for wavenumbers 1, 2, and 3 respectively during the winter. At lati- tude 40 during winter, wavenumber 1 appears to vary 27r radians in 30 km. Furthermore its phase becomes constant with height above 1 mb. This con- stancy of the phase with height could be due to a standing wave pattern caused by upward propagating waves reflecting off the regions of large <U> and the lid. Possibly the Newtonian cooling is not large enough to prevent the wave reflection off the jet. Simmons (1974) found that the <U> and the presence of Newtonian cooling are critical in avoiding the reflecting wave. In winter, stationary wavenumber 2 calculated by the model also exhibits abouta 2n radians shift per 30 km and a constancy of phase above 5 mb. During the summer, the phase shift is only ffradians per 30 km at midlatitudes, but reflection is still apparent above 5 mb. Notice that in both wavenumbers 1 and 2 the further polewards one goes, the lower the level drops at which the constancy of phase appears. This effect could be the result of either ducting or the change in the resulting damping rate of the wave. Wavenumber 3 has again a winter midlatitude 2ff radian phase shift per 30 km and again it exhibits a changeover to constant phase at 5 mb. In the summer hemisphere the phase shift is only ffradians per 30 km. Matsuno (1970) used a quasi-geostrophic model in spherical coordinates and found that the standing waves are attenuated much too strongly. Second- ly, he found that his model gave phase shifts of ffradians and nearly 1.5ff radians per 30 km for wavenumbers 1 and 2 respectively. Matsuno also found very little southward tilt of the isophases which indicated little or no ducting of waves towards to equatorial zero line. This result could stem from the fact he was using a hemispheric, not a global model. -27The excessive phase tilt in the lower 30 km of the model in this study can be due to either an excessive southward phase shift or too much vorticity advection which, when balanced by vortex stretching, leads to a reduced vertical wavelength for the waves. In the equatorial regions all wavenumbers show that most of the phase shift takes place above 50 mb where the zero line for <U> reaches the equator. This fact suggests that ducting of the wave phase from different lati- tudes could be responsible for this apparent shift. Figure 22 shows the total vertical velocity variance due to the eddies. There is not much to say about the variance except that it has a very strong similarity, to the <V 2>. One other note of interest is that in the upper atmosphere, the maximum in the variance occurs equatorward of the polar night jet. The summer hemispheric atmosphere above 30 mb has little or no vertical eddy velocities to speak of. The only way to get at what the transient eddies are doing is to plot and study the time histories of the phase and the amplitude of the wave. A preliminary study was made by making a time history for the month of December at the 12 mb level and at latitude 40 for wavenumbers 1, 3, and 5. These histories are shown in Figures 23, 24, and 25. The purpose of such a plot was merely to look at the typical behavior * of the amplitude and phase of V as a function of time. From such a plot the velocity of the wave with respect to a fixed point can be found. Second- ly, it was unknown whether or not discontinuities would occur in the wave history due to the daily sampling. The failure to sample often enough has been thought to be a problem for the higher wave numbers in particular. Wavenumber 1 seems well-behaved in both amplitude and phase. 30-day decay in the trend of the wave amplitude shows up. A definite The phase exhibits -28- a general westward motion with no great discontinuities. The average phase velocity is about -9 m/sec with respect to the ground. Wavenumber 3 appears to hesitate between going from a decaying mode to a growing mode near days 2-4. in the wavenumber 1 case. respect to the ground. The variations in amplitude are greater than The phase shifts very quickly westward with It moves at an average velocity of about -30 m/sec. From the Rossby wave dispersion relation, the latitudinal scale of this wave must be quite large in order to produce the large retrogression. Wavenumber 5 has very large amplitude changes with a period of roughly 7 days. Note that near day 6 the sampling of the wave seems to catch a wave in the.act of switching from a decaying to a growing mode, which causes The phase motion of the wave is east- a spurious "bump" in the amplitude. wards with an average phase speed of about 4 m/sec. A calculation was made of the average mixing slope defined by Reed and Unfortunately the mixing slope covariance shows German (1965) as <W /V >. a large amount of point-to-point variation. The problems appears to be too short an averaging interval, and an improper grid and spectral representa* tion which allowed small values of V to dominate the covariance. Another less "noisy", but possibly less legitimate estimate of the mixing slope can be formed by taking the ratio <VW>/<VV>. assumes that Kyy = T<V2> * relation and Kyz = T<VW> This approximation instead of Reed and German's * L(Y) = L(Z)(W /V ). T is a time scale that is not necessarily velocity independent, but is characteristic of the exchange of parcels. A more developed discussion of this matter will be given in a later chapter. Figure 26. Shows the mixing slope defined by <VW>/<VV>. The dominant feature below 20 mb is the downwards-polewards slopes in the lower stratosphere and the upwards-polewards slopes in the troposphere. The typical -29stratospheric slope is 2-4.E-04 radians, slopes of the same magnitude. Reed and German (1965) found In the troposphere, Hantel and Baader (1976) found slope maxima of 1.OE-3 radians which are also reproduced in Figure 26. In the summer hemisphere, the rest of the atmosphere above 20 mb has a downwards-polewards slope that has a maximum near midlatitudes and minima at the poles and the equator as one would expect. The winter hemisphere shows downwards-equatorwards slopes in the upper stratosphere and lower mesosphere of the same sign as the troposphere. The maximum slope is cen- * * tered near the region where the <W $ > anomaly exists in the mesosphere. Above 1 mb, in the low to midlatitudes the downwards-polewards slopes again dominate. -30- 7. A Survey of the Eddy Fluxes of Ozone and Potential Temperature in the Model The poleward fluxes of ozone are of particular interest in this study. These fluxes are responsible for the ozone number density maximum which appear in the lower stratospheric high latitudes. maxima in Figure 27 where <03> is shown. One can observe these The ozone number densities simu- lated by the model appear to agree reasonably well with the observations analyzed by Wilcox et al. (1977). The total meridional ozone flux due to the eddies is shown in Figure 28. All fluxesthat are presented are area-weighted to give an idea of their true contribution to the global flux budget. The winter hemisphere shows an equatorward flux of ozone at high to midlatitudes in the lowest part of the mesosphere near 1 mb. This flux is downgradient according to Figure 27. Everywhere else in the winter hemisphere, down to the 30 mb level, a poleward flux exists which comes to a maximum between 10 to 20 mb and 400. Below 30 mb a confusing region occurs. Here the eddies act to cause alternating signs in the flux in going from level to level. At midlatitudes the vertical average of the fluxes between 50 and 150 mb in midlatitudes are actually of the same size as those near 20 mb. Proof of this is shown in Figure 29 where the average flux of the 50-150 mb layer is shown. that large interhemispheric transports appear to be occurring. Notice The direc- tion of the flux is towards the winter hemisphere, and this kind of export is expected due to the exchange of stratospheric air with the troposphere at midlatitudes. Below 150 mb, the eddy ozone flux decreases, but it re- mains polewards at high to midlatitudes. In the equatorial troposphere the eddy flux is directed equatorwards, which implies downgradient transport -31into the tropical ozone-poor air shown in Figure 27. In the summer hemisphere, the mesospheric horizontal ozone eddy flux is generally directed equatorwards. tains its poleward flux. The midlatitude upper stratosphere main- The lower summer stratosphere in the 50 to 150 mb region has poleward fluxes north of 500, and net equatorwards fluxes south of 50*. It will be shown later that the vertical transient eddy flux is responsible for the change of direction of the flux from one season to another since it changes the mixing surface's slope from horizontally upgradient to downgradient fluxes. The upper troposphere has poleward fluxes of ozone, but the lower troposphere has equatorward directed fluxes. This behavior is reflected in the changeover of the horizontal ozone gradient shown in Figure 27. A further breakdown of the eddy ozone flux was made. The steady stand- ing wave flux and the residual transient wave flux are shown in Figures 30 and 31 respectively. In winter the region from 30 mb up to the stratopause has a transient eddy flux that dominates over the standing eddy flux by factors of five to ten. Both the eddy flux components are directed polewards. Below 50 mb in winter, the two eddy components are much larger than the total eddy flux. However, at many places they nearly cancel each other and leave only a small residual. This behavior is quite puzzling. Somehow the transient eddies are tied to the standing eddies in such a manner that causes them to oDnose one another systematically over a large number of points. The interhemispheric flux in the 50 to 150 mb region seems control- led by the transient eddies which win out in the tug-of-war going on between the standing and the transient eddies. In the summer hemisphere the opposition of the flux components occurs from the troposphere clear up to 30 mb. At high latitudes the cancellation -32effect continues up to the stratopause. At midlatitudes in the upper stratosphere and lower mesosphere, the transient eddy flux dominates over the standing eddies by at least a factor of two. The total vertical flux of ozone, including the mean circulation, is shown in Figure 32. The winter hemisphere shows a strong downwards flux of ozone throughout the whole vertical extent of the atmosphere from 10-50*. The maximum in the flux occurs near the tropopause. This result agrees with the flux directions given by the tropopause gap mechanism of Danielsen (1968) and the downward Hadley-Ferrel cell branches of the mean circulation. At very high latitudes ozone is moved upwards at all levels. The summer lemisphere troposphere has a downwards total flux of ozone in the 20-40* belt, and an upwards flux in the 50-60* belt. Upon comparing the total flux in Figure 32 with the standing and transient fluxes in Figures 33 and 34, one finds that the mean circulation transport of ozone tends to oppose the transient eddy fluxes, and actually dominates the vertical fluxes in some regions. Mahlman (1973) showed that this opposition of the mean circulation and transient eddy fluxes also occurs in a primitive equation model. In summer, the total vertical flux of ozone in the midlatitude lower stratosphere is directed upwards. The upwards flux is due to the action of the eddies, mainly the transient eddies and not the mean circulation. This direction of eddy flux is completely opposite to the winter hemisphere and its cause is not clearly understood at the present. At low latitudes in the summer mid-stratosphere the total vertical flux is directed upwards. However in this case the eddies have a combined downwards flux, but the Hadley circulation opposes and wins out over the eddies. Higher up, near 5 mb, the summer season midlatitude transient eddies are upwards and -33- dominate the eddy flux budget over the standing eddies by as much as a factor of ten. downward. In the low and high latitude regions the eddy ozone flux is The domination of the vertical eddy flux by the transient eddies is probably due to the fact that tropospheric-forced steady stationary waves are trapped by the easterlies and the zero wind line. Again, when looking at the zonally-averaged streamfunction of Cunnold et al. (1975) above 5 mb, one sees that the eddy flux is in opposition to the mean circulation flux. In the winter hemisphere for the low to midlatitudes, the 5 to 20 mb layer has upwards transient eddy fluxes. show downward flpxes. The high latitudes of this layer In winter, the 50 to 200 mb region shows downwards transient eddy fluxes at most latitudes. In the troposphere the transient eddy fluxes can best be described as everywhere opposing the mean circulation transport. The standing eddies in the winter hemisphere compete with the transient eddies up to the 1 mb level where they abruptly taper off due to the fact that the lines of constant phase become vertical at this level. The 5 to 30 mb region at midlatitudes exhibits an upwards eddy flux which generally acts to aid the transient eddies in opposing the mean circulation. In the tropical lower stratosphere a curious standing eddy flux pattern appears. A downwards flux of ozone due to the standing waves appear in the summer hemisphere, and an upwards flux appears in the winter hemisphere. The horizontal flux of potential temperature due to all the eddies is shown in Figure 35. The flux of temperature is polewards clear to the top of the model in the winter hemisphere throughout the high and midlatitudes. This type of flux is expected if the wave disturbances are to propagate vertically. -34In the mid-troposphere, there occurs a convergence of heat into the equator coupled to a divergence at the tropopause. This feature also appeared in Manabe and Mahlman's (1976) primitive equation model. They suggested that the flux was due to the gravity-Rossby wave modes. The quasi-geostrophic model can roughly simulate such modes at the equator, and if they are forced by the applied heating they could be responsible for the feature. The most exciting feature by far is the equatorward flux of heat near .5 mb in the low latitude winter hemisphere. This flux appears to be rela* * ted to the strong low latitude divergence of <W $ >. bits a strpng divergence of heat. The 20-40* belt exhi- Solar heating by ozone appears to be the only significant source of heat for this region. The equatorwards flux of heat according to Eliassen and Palm (1960) would cause a downwards eddy geopotential flux. The vertical flux of potential temperature by all the eddies is shown in Figure 36. The vertical potential temperature flux is directed upwards in most of the troposphere for both summer and winter as Oort and Rasmussen (1971) show. Above 10 mb, the high to midlatitude winter upper stratosphere and mesosphere exhibit an upwards eddy flux of potential temperature. In the low latitudes, the winter upper stratosphere and mesosphere exhibit a downwards eddy flux of potential temperature. The lower stratosphere at high to midlatitudes of both seasons shows a downgradient downward flux of potential temperature. The negative correla- tion between potential temperature and vertical wind velocity comes from the tendency for the vertical motions to respond to the diabatic cooling in a manner that causes downward motions to occur in cyclonic regions. -35The tropical tropopause region shows an eddy upwards flux of potential temperature in the summer hemisphere and a downwards flux in the winter hemisphere. These features appear to be related to the strong horizontal convergence of heat by the eddies into this region. In order to determine which wavenumbers are doing most of the transport, the total eddy fluxes of ozone were broken down by wavenumber for the levels 132, 40, 12 and 1 mb for the latitudes 80*N, 40*N, 0*, 40*S, and 80*S. The fraction of the total covariance as a function of wavenumber is plotted in Figures 37 and 38. At 80* both December and June show that the flux is extremely dominated by wavenumbers 1 and 2 at all levels. During the winter the eddy ftux at 40* in the lower stratosphere is divided fairly evenly between wavenumbers 1, 5, and 6. During the winter, wavenumbers 5 and 6 contribute significantly to the eddy flux up to 12 mb. In the lower meso- sphere, however, only wavenumber 1 makes a significant contribution. At the equator there appears to be a tendency for all the wavenumbers to contribute a flux in the same direction. This is in contrast to mid- latitudes where various wavenumbers of significant contribution tend to oppose one another. The lower equatorial mesosphere curiously enough has a strong contribution to the total flux made by wavenumber 4. This contri- bution probably comes from the mixed mode Rossby wave. During the summer, the midlatitude fluxes are either dominated by or strongly influenced by a strong wavenumber 4 component at all levels. The contribution to the flux by wavenumber 4 is in the same direction at all levels. Wavenumbers 1 and 2 become significant only above 12 mb. In all the months the midlatitudes do not show a dominant wavenumber that would be useful in aiding a parameterization of the flux. Only at high latitudes and mesospheric altitudes would such a scheme work. The only -36hope for a useful parameterization in terms of phase would occur only if all the wavenumbers had nearly the same phase difference between ozone and the wind. However, this hope is also destroyed as one sees that there is significant opposition in the fluxes as a function of wavenumber. One apparently cannot restrict the parameterization scheme to one zonal wavenumber. -378. A Survey of the Phase Difference Between the'Winds and the Tracers The particular eddy flux of interest in this study is the poleward flux of ozone. Consequently the study of the phase lags for the time being * will be limited to V * and 03. In order to ascertain the gross "efficiency" of the eddies in transporting ozone, the average phase angle defined by was calculated. This phase angle contains not only average size of the phase difference between V the information and 03 on the but also the corre- lation between the amplitude size and the phase difference. The expression is unsuitable in trying to get an idea of the phase difference. Neverthe- less it does give one an idea of the average "efficiency" at which the eddies transport ozone. The phase difference, y, is shown in Figure 39. the eddies are very poor transporters of ozone. It can be seen that Only about 1-3% of the total possible transport is realized since the phase angle is nearly always near 7r/2 radians on the average. inefficient. The 50 to 200 mb region is notoriously This result is to be expected since the net flux in this region is about the flux one finds for a layer one-third the thickness near 20 mb. The most efficient regions of transport can muster only about a 5% efficiency. The average phase difference between 03 * * and V for the standing waves at levels 132, 12, 1 and .089 mb are plotted as a function of zonal wavenumber in Figures 40 and 41. The most obvious fact is that the standing eddies have a phase difference much greater than the gross phase difference. -38This result should be expected since the standing eddy wind variance is much smaller than that of the transient eddies, yet the standing eddy fluxes are nearly able to cancel the transient eddy fluxes in some places. This kind of behavior then implies that the phase difference should be * fairly large. The phase difference between V * and 03 is quite random in the sense that the phase difference randomly fluctuates back and forth across the 900 line as a function of wavenumber. There doesn't appear to be any particular "spectrum" of phase differences that can easily be fitted by a simple relation. * Phase histories of V * and 03 for the first three zonal wavenumbers at 12 mb and latitude 40 are shown in Figures 42, 43 and 44. The time period for the histories is set in the winter month of December. Zonal wavenumber 1 shows a fairly constant leading of the ozone wave which on the average has a phase difference of 1.86 radians. Wavenumber 2 shows ozone still to be leading, however the phase difference shows a larger amount of variance. ans. On the average the phase difference is about 1.71 radi- Wavenumber 3 retrogrades rapidly with a westward motion, but the ozone wave still leads the wind. The variance of the phase difference grows still larger, and it is found that this trend continues out to wavenumber 6. The average phase difference for wavenumber 3 is about 1.81 radians. In summary one can see that the transient eddies have phase differences which are very close to 1.57 radians on the average. The meridional wind and the ozone in these eddies appear to be almost completely out of phase. The standing waves on the other hand exhibit larger phase differences, but in many cases the different wavenumbers show a tendency to cancel one another. The transient waves show a fair amount of constancy in the phase difference as a function of zonal wavenumber, while the stationary waves do not. At -39- this point it is not exactly clear what the transient wave phase difference depends on so that one can write these phase differences in terms of averaged quantities. -40- 9. Introduction to the Mixing Length Hypothesis The gradient law approximation to the mixing length hypothesis has been reviewed elsewhere, i.e., see Corrsin (1969). For any question about the historical development and the validity of usage of the mixing length hypothesis one is referred to the previous reference cited and to Launder (1974). The mixing length hypothesis is at best a physically meaningless analog to molecular diffusion. One of the main drawbacks in parameterizing the fluxes by eddy diffusion is a lack of physical guidance in calculating the eddy-diffusion coefficients K(I,J) = <L(I) V"(J)>. Stone (1973) found functional expressions for Kyy in terms of the mean state variables. However this case is misleading since the eddy diffusivi- ties really result from the explicit expressions for the heat fluxes, with the fluxes, who needs the eddy diffusivities? The first is There are two approaches to getting eddy diffusivities. to simply fit or "tune" the eddy diffusivities to the observed fluxes. The second way is to use statistical methods like Kao (1965) to deduce the mean behavior of an ensemble of parcels. Reed and German (1965) were the first to discuss relations between the different elements of the two-dimensional eddy diffusivity tensor. the two-dimensional case, a perturbation in the tracer field, can be written to first order terms as: In Q" = Q - <Q>, -41Reed and German assumed that the turbulence to be approximately isotropic so that V"L = W"L . This assumption allowed the definition of a mixing slope as being the wind ratio of the form: S=P(9.2) By multiplying (9.1) by V" and both zonally and time averaging one can arrive at the relation: (9.3) where % , and where e equals the density. The triple covariance in (9.3) can be expanded if V"L single variable. and <V"Ly>, where is treated as a By ignoring the correlations between variations in <o> the resulting form of (9.3) can be written as: Kyy = <V"LY>. The same kind of manipulation can be done for the vertical flux corre- lation with the result: Reed and German (1965) were the first to use a direct method of determining two-dimensional eddy diffusivities from the wind and tracer statistics. The method in reality is just a direct way of tuning the eddy diffusivities as opposed to tuning them in a model by trial and error. -42The eddy diffusivity of the midlatitude mid-tropospheric disturbances was found by using Eady's (1949) approximation that for heat, mixing tends to occur along slopes one-half that of the mean isentropes. This approxi- mation plus the observed eddy heat flux allows the direct calculation of Kyy at that point. The eddy diffusivity, Kyy, is extrapolated to other regions by the use of Prandtl's (1945) improved assumption that the eddy diffusivities are proportional to the variance of the wind. By using observed horizontal eddy heat fluxes, Reed and German were able to calculate <a>. They also assumed <a> to vanish at the equator so that the ratio Kzz/Kyy equals <a'a'> which is then held constant everywhere. Unfortunately Gudiksen et al. (1968) found that the eddy diffusivities were much too large and had to be reduced by factors to 5 to 10 so that the modeled distribution of tungsten 185 would fit the observations. By using five years of data on the heat fluxes and wind variances, Luther (1973) made a set of eddy diffusivities. Luther extrapolated the values of Kyy above the region of observation by assuming that the upward propagating wave motions have a constant energy density so that the wind variances increase by the inverse square root of the density. Later)Louis (1974) used a meridional circulation that he deduced and the observed ozone distribution to get improved estimates for Kyy. -4310. A First Attempt at Obtaining Eddy Diffusivities The model of Cunnold et al. (1975) can be facilitated to calculate all of the variables in (9.4) except Kyy for the cases of ozone and potential temperature. If one substitutes < > = -3<Q>/Y/3<Q>/DZ, and makes some mathematical arrangements, Equation (9.4) can be solved by Kyy by the expression: 4KI> 4 V (10.1) Equatiqn (10.1) presents some problems mathematically since it becomes singular as <a> = <f> . In the case that the tracer is potential tempera- ture the possibility of a singularity becomes inevitable. sphere <at> < < > nature. In the tropo- since the disturbances are generally of a baroclinic <O> > <> While in the stratosphere a "refrigerator" and EKE is changed to EAPE. troposphere and the lower stratosphere <a> since the motions behave like Somewhere in between the mid- = . In the equatorial regions <a> and <f> become quite small and they tend to equal one another. The smallest amount of error in either <ct> or <6> can cause a large spurious Kyy. Several calculations using both the ozone mixing ratio and potential temperature showed singularity problems in both these regions, and also at high latitudes in the stratosphere. The vertical eddy flux relation (9.5) also has the same problem of singularities when <a><I > . Computations again showed the same problem in approximately the same regions. The uncertainty in the average values tend to make it impossible to exclude even the pseudo-singularities from occurring in (10.1). -44Another, more basic complication in the direct computation stems from the uncertainty in the average values. One cannot time-average over an infinite number of winter seasons to get a true winter average. age value has a finite level of uncertainty. Each aver- The standard error gives a measure of the random "noise" that the average is buried in. The standard error is not really a true measure of the amount of variation which takes place about the mean since the spectrum of the winds is not a constant as a function of frequency. A better indicator of the uncertainty might come from using a high order Markov process instead of a random process. However, it is a line of analysis that would be complicated, and for the effort the estimate of the uncertainty is provided well enough by a random model. The standard error is given by a//N, where a is the standard deviation of the uncertain variable and N is the number of independent samples of the variable. Averaging over a season instead of a month decreases the error only by a factor of .58, while averaging over a year reduces it by a factor of .29. The standard error strongly reflects the effect of beginning and ending If one averages over 30 days and the devia- in a small averaging interval. tions from the average are on the average 30 times larger than the average, then if there are one or two more positive deviations than negative ones, due to the point of beginning and ending, large errors are possible because the standard error is of the order of the average value. Confidence limits can be established by using the T statistic defined A confidence level of 95% can be set by using a T statistic by <(>/a/Ar. of two which is simply twice the standard error. * * were set for <V 03 >, *f* <V V >, The 95% confidence limits - <ca>, and <03>. The appropriate monthly -45values and their uncertainties are shown in Table 1 for selected levels and latitudes. * * From looking at Table 1, one can note that for the covariance <V 03 > even the sign cannot be accurately ascertained in many cases. The uncer- tainties in the covariance are particularly large at level 21 and at high and low latitudes. An even worse case is the mixing surface slopes, <a>. Sometimes the uncertainties are nearly a factor of two larger than the average value. Variances and single variables fared much better. Note that for * * <V V > the uncertainty is at least a factor of three less than the average value, while for<0 3> at high altitudes, the uncertainty is one-tenth the average. In the case of <0 3> one can see the distinct increase of the uncer- tainty to average ratio as one progresses from level 15 to 21. The increase in the uncertainty is probably due to the increased importance of the divergence of the eddy fluxes in determining the mean value. From the uncertainties in the mixing slopes and the fluxes, it looks as though only monthly averages taken from nine years of data will significantly reduce the uncertainties anywhere near to the fractional level of un* * certainty in <V V > and <03> . per experiment. Unfortunately only three years are simulated The first year is generally evolutionary towards the steady yearly oscillation. Run 26, which appears to be the most successful to date, has only two years of simulation, thus only one month at a time can be simulated. Nevertheless one can at least make a preliminary study from the small amount of data at hand. As an example to illustrate what sort of problem uncertainty is in the calculation of Kyy from (10.1), a specific calculation of the Kyy uncertainty was made for Level 15 and 400 S. The uncertainty relation for Kyy is -46derived in Appendix 1. Substituting in the values from Table 1 along with Kyy = 2.45E+6 ± 6.63E+6. the ozone gradients gives the result: The uncer- tainty can be seen to be so large as to make it difficult to determine even the sign of Kyy. In the past, the assumption that Kyy is proportional to -*2 <(V ) >) has been used quite often. L<(V') 2 > + It is of interest to find out what the size of the constant of proportionality is: whether it is 1 minute, 1 day, or 1 week. <(V) Secondly, one might ask if perhaps a different power of 2> + <(V ) 2> might work better. A test was conducted to see what the variance-gradient produce relation * * was to the, fluxes. V* e > and X was set equal to . A scatter plot of X versus Y was made and shown in [7 Figure 45. 30-60*S Y was set equal to -<V The region chosen included the levels 15-19 and the latitudes for the northern hemispheric month of June. A polynomial regression was made of X on Y. The largest reduction of variance was only .15 which indicated a large amount of random scatter. The result when the Y intercept was zeroed indicated that the reduction of variance was accomplished mainly by a linear fit with the slope of 1.lE+5 sec. The large uncertainties in the Y's are the cause of the scatter and the negative X values which tend to detract from the validity of the plot, however not much can be done about it. In the troposphere, Schneider and Dickinson (1976) interpreted the <(V) 2> + <(V )2> to be roughly the in- verse of the growth rate of the most unstable wave. The growth rate goes proportionality factor in Kyy approximately as f/v/R'I, where f is the Coriolis parameter and RI is the Richardson number. For the midlatitude troposphere the inverse of the growth rate is roughly three days. In comparing this result with the lower -47stratosphere the proportionality coefficient does not seem to differ much despite the different dynamics of the two regions. since if the slope had been on the order of 10 6 This is encouraging, sec, the proportionality argument would be much less credible. One could find the proportionality coefficient by using Reed and German's (1965) technique, however it would be better if the coefficient could be calculated directly. There are two ways of doing this. One way is to make use of Taylor's dispersion theory which is discussed in the next section. The other way is to try to formalize the physical mechanism which controls the proportionality coefficient of interest. By taking a,cue from the growth of a tropospheric growing baroclinic eddy, one can obtain some physical insight as to what the proportionality time constant means. perature advection. The growth of the eddy basically comes from the temThe advection must in a sense be "localized" so that the advective processes will preserve the scale of the disturbance and not * try to distort it beyond recognition. If the phase difference between V * is close to 7r/2 radians, the advective scale can be thought to be and T of the order of one-half the wavelength. If the phase relation holds for most wavenumbers, then the distance would be about one-half the meridional EKE weighted wavelength. The rate at which parcels are brought into a disturbance and taken out, in an average sense is roughly determined by the absolute value of the average zonal wind. The coefficient of proportionality, which shall be henceforth called T, is regulated directly by the advective scale, and inversely by the zonal wind. The idea is simply that the larger the wind, the shorter the time it takes for a parcel to move the advective length scale. The coefficient T can be tentatively written as -48- (10.2) pd The constant C II| is simply a small constant to avoid singularities near = 0. T tends to remain constant in the vertical. As one goes to higher levels in the stratosphere, the zonal wind velocity increases, but the meridional EKE weighted zonal wavelength also increases. As one goes from the equator to the pole the zonal wind velocity reaches a maximum near 50*. The weighted zonal wavenumber on the other hand tends to remain constant. One expects -some,latitudinal variation with T reaching a minimum at midlatitudes as Murgatroyd (1969) found. Several experiemtns were conducted with this formula. One experiment was conducted on Run 17 data with the intent of getting well-behaved Kyy eddy diffusivities. In this experiment the advection length was not calcu- lated explicitly, but rather was artificially fixed by specifying the Kyy value at 50*. The value chosen was Kyy = 2.6E+5 m2/sec and spring northern hemispheric seasons. for both winter The Kyy eddy diffusivities calcu- lated arehown in Figures 46 and 47 respectively for the case C = 5 m/sec. * Run 17 variances of V were found to be roughly four times larger than observation due to the lack of significant subspectral diffusion. Secondly, a large computational two-level oscillation showed up. Compared with those of Gudiksen et al. (1968), the Kyy's show a much wider range of values. While the Gudiksen et al. set show only variations of a factor of five in the troposphere, the values in Figure 46 show the tropospheric variation to be about a factor of ten. several features are common to both sets. In the troposphere These are the tropospheric -49inimum at 20-30*N and the maxima near the jet core and at the equator. Also appearing in both sets is the minimum in the lower troposphere of the equatorial regions. The Gudiksen et al. Kyy's decrease slightly in midlatitude from the tropopause maximum to a minimum near 25 km of about 4.OE+5 m 2/sec. The model Kyy's also exhibit a minimum in this region of about the same size, but the decrease is about a factor of ten. In going upwards from 50 mb, the Gudiksen et al. values of Kyy increase much more rapidly at high latitudes than the model Kyy's do. The equatorial regions exhibit a rapid decrease in Kyy in the lower stratosphere for both sets. However, the minimum of the model Kyy's is about 3.OE+5 while the Gudiksen et al. value is more than three times smaller. For a further comparison one is referred to the CIAP Monograph Vol. 1 (1975) for other sets of Kyy eddy diffusivities. Another experiment was run using the meridional EKE weighted zonal wavenumber found from (6.1). The northern hemispheric month of June from Run 26 was used in order to calculate T. The factor C The result is shown in Figure 48. was arbitrarily set to 2 m/sec. T does not seem so constant as was anticipated. order of magnitude at most. T varies about an Fortunately the only sharp gradients in T occur near the equator, and in the lower troposphere. Upon looking at the pattern of T one finds a strong inverse proportionality of T with (<V'V'> + <V V >). Minima occur in T where maxima occur in the variance. One might be led to redefine the formula for Kyy as: k= C1 (V v.> + < (10.3) where n falls in the range .5 to 1.0 and C2 is a true constant, say the space-averaged T. -50- 11. The Use of Taylor's Dispersion Theorem in Determining Eddy Diffusivities Taylor (1921) demonstrated the relation of the distance dispersion, <fi2>, to22the velocity variance, coefficient, R(T). If <. V 2and the velocity autocorrelation 2> is the square of the distance the particles have diffused in a time period T, the dispersion rate can be expressed by the now well-known Taylor relation: < < V> >y-Z , S C)/e3 z (1.1 As t,goes to infinity, the integral in (11.1) becomes what is known as the LaGrangian integral time scale (LIT). Generally the time period t is taken as an averaging time period much greater than the lifetime of the individual eddies so that in most cases the integral in (11.1) closely approximates the LIT. The most important eddy diffusivity component Kyy can be expressed as r:.v9(11.2) where T is now used to denote the LIT. The LaGrangian frame of reference has been used in the discussion. In many cases the LaGrangian variables are computationally awkward since one must work with moving particle trajectories, rather than the handy instantaneous point sampling of radiosondes. In order to make use of the Euler- ian variables, Hay and Pasquill (1959) proposed the following EulerianLaGrangian transformation: -51- =4(1)(11.3) Lpe) R where RL AND RE are the LaGrangian and Eulerian autocorrelation coefficients. The parameter S is a scale dependent parameter linking the integral timescales by the relation L = E' Kao (1965) proposed a relation for the waves. associated with Rossby The relation takes into account the Doppler shifting effect of the zonal wasterly wind which tends to move the energy spectrum peak towards lower frequencies. The average S which is independent over wave- number cap .be expressed by the relation: p~ lxc~ 2/~ic9) -ai (11.4) where LW2 is the square of the meridional EKE weighted mean zonal wavenumber of the turbulence. A plot of of June. 3 is shown in Figure 49 for the northern hemispheric month At midlatitudes 3 appears to be about 0.5. This value agrees quite well with the set of 1 made by Murgatroyd (1969b). 1 as a whole tends to have an inverse proportionality with the zonal wind profile, with strong westerlies appearing as low lies show 0.5. 1 to be one or larger. The jets appear as minima. 1 regions, and the strong easter- In the troposphere 1 is generally about While at high latitudes the cos$3 term becomes quite small; giving values of unity or greater. The summer hemi- sphere stratosphere exhibits an almost uniform region of 1 of 1-2 equatorwards of 60*. of the range -52In order to calculate T , the Eulerian integral timescale TE is calculated by taking the sum over all time lags of the autocorrelation coefficient Rvv(t). Unfortunately the accuracy of the estimate of the * Rvv(t) is limited by the length of the time record of V scale of the dominant eddies. , and the time- The length of the record must be at least five times longer than the dominant eddy timescales. be careful of how the longest time lag is ended. Secondly, one must Otherwise the ending of the record on a large Rvv(t) will prevent accurate estimate of the LIT. Figure 50 shows the autocorrelation coefficient at 12 mb and 40* for the month of December. The form of the autocorrelation coefficient * * as a function of time is somewhat like R (t) = exp(-P t)cos(Q t). vv Murgatroyd (1969b) used this form for Rvv(t) in his study. for R vv (t) is simply the Fourier transformation of a spectrum with a peak. Q are P and This relation tral peak. parameters that adjust the frequency and strength of the specIn the autocorrelation coefficient case at hand, the dominant period seems to be about 12 to 14 days. The meridional winds that went to make up the autocorrelation coefficients were preprocessed to remove any linear trend that would bias the autocorrelation coefficient. The 32-day time period seems to be insuffi- cient in many regions for estimating the LaGrangina integral timesacle. At 12 mb the autocorrelation shows a dominant period of about 12 days. Obviously a 32-day sample cannot represent this frequency well. Secondly, at the 3 1 st day lag, the autocorrelation coefficient is still quite large. This indicates that a very long period is biasing the total area under the Rvv(t) curve. This problem is compounded by the fact that TL is quite small compared with any given Rvv(t) that goes into making the sum for T . -53The LaGrangian timescale was plotted for those regions in which it was felt that there was some significance in the TL obtained. The LIT, The timescale is meant for the northern hemi- TL, is shown in Figure 51. spheric month of June. The timescale seems to have a maximum near 80 mb and a minimum in the mid-troposphere. file. Murgatroyd (1969a) also found the same kind of pro- Murgatroyd's values for TL are about one-half the values calculated from the model data. The variation in TL calculated range by a factor of three between 400 and 50 mb. The comparison of the calculated TL with the T shown in Figure 48 shows a rough smilarity. In both cases there is a mid-tropospheric minimum, a 50 mb maximum, and a maximum in the lowest part of the troposphere. -5412. Conclusions and Summary One of the basic purposes of this diagnostic study on the data from the MIT stratospheric GCM was to compare the observations of the eddy fluxes of ozone and potential temperature with the model simulation. Another pur- pose was to present findings from the model in regions where observations have not yet been made so that the results can act as a guide to future observations. The study conducted on Runs 17 and 26 of the model has several significant conclusions which can be made. An attempt shall be made to present the more important points of the study by type of analysis and by region of the atmosphere. In themidlatitude troposphere the surfaces along which ozone and potential temperature mix are directed polewards and upwards. The slopes of the mixing surfaces are of the same size (5.OE-4 radians) as those observed in the troposphere. In the troposphere the mean circulation fluxes tend to oppose the eddy fluxes of ozone and heat. In the troposphere the ratio of the meridional transient EKE to that of the standing eddies is about that observed by Oort and Rasmussen (1971). The midlatitude meridional EKE for both the transient and the standing eddies is about twice that observed. In the mid-troposphere the equatorial region behaves quite differently from midlatitudes in that it exhibits an equatorward eddy flux of heat converging into the euqator, while ozone appears to be diverging. The merid- ional EKE is spuriously large at the equator also. The stratosphere in the 10 to 150 mb region has some similarities and some differences from the troposphere. In the midlatitudes, the stratospheric temperature flux remains polewards, and the vertical flux of geopotential is -55positive like the upper troposphere. The convergence of the vertical eddy flux of geopotential, along with the downwards vertical eddy flux of temperature agrees with Oort's (1964) analysis which found the stratosphere was forced by the pressure forces from the troposphere, and that the EKE of the wave motions is being converted to EAPE. Both ozone and potential temperature in the lower midlatitude winter stratosphere have polewards and downwards fluxes that tend to occur in longitudes of low geopotential. The slopes of the mixing surfaces are about the right size (4.OE-4 radians) and exhibit a maximum at midlatitudes as previous estimates by Reed and German (1965) have shown. The horizontal steady stationary wave fluxes of ozone tend to cancel the transient eddy ozone fluxes in the lower stratosphere. ponent is much larger than the total eddy flux. Each flux com- In the 50 to 150 mb region the large variability makes the total eddy flux of ozone undergo changes from polewards to equator-wards directed fluxes from level to level, although the total eddy flux in this region is directed polewards during the winter. The vertical eddy fluxes ofozone also show a tendency to oppose the mean circulation fluxes. The meridional EKE for both the stationary and transient waves decreases to about the observed values at 30 mb for most latitudes. The only excep- tion occurs at high latitudes where the steady stationary wave variances decrease instead of increase as the observations show to be the case. The vertical scale of the nondivergent meridional standing wave wind seems to be roughly twice as small as it should be in the lower stratosphere. This standing wave also exhibits a constant phase with height above 10 mb. As one goes polewards and upwards, both the transient and standing wave motions show a spectral shift towards lower wavenumber. The fluxes of ozone -56also exhibit this spectral shift. The only true exception is near the equator where wavenumber 4, due possibly to the mixed-mode Rossby wave, dominates the transient eddy fluxes. The waves as a whole show ozone and the meridional wind to be nearly 900 out of phase so that only 1-3% of the total potential flux of ozone is realized. The traveling wave fluxes of ozone seem to have better behaved phase differences between ozone and the meridional wind than the steady stationary eddy fluxes. The region from .5 to 10 mb shows some interesting behavior in the winter hemisphere. The mixing slopes change sign with respect to the rest of the stratosphere, and possess a sign simialr to that of the troposphere. In the lowest part of the mesosphere the potential temperature fluxes are mainly equatorwards on the low latitude side of 400 and polewards on the high latitude side. Heat diverges out of the region about 40*. The verti- cal fluxes of potential temperature equatorwards of 40* are downwards, while those polewards of 40* are upwards. The winter transient vertical eddy fluxes of ozone equatorwards of 40* are upwards, while those polewards of 40* are downwards. The horizontal eddy fluxes of ozone show a convergence into the midlatitudes. The convergence is even strong enough to produce equatorward eddy fluxes of ozone near 1 mb in midlatitudes. Because of the tropospherically similar mean temperature gradients in the vertical and horizontal, the high latitude mesospheric regions could quite possibly be baroclinically unstable. The downwards directed eddy geopotential flux in the low latitudes is quite interesting, for in this region one cannot rule out barotropic instabilities due to the large horizontal zonal wind shears on the low latitude side of the polar night jet. -57Of course, further studies on the energetics of both regions would have to be done in order to show conclusively the energy conversions going on. However, the general directions of the mean gradients of wind, temperature, and the eddy fluxes suggest the possibilities for instability to the extent that such further study is highly encouraged. The region above .5 mb seems to behave much like the 20 to 150 mb region. The mixing slopes tilt so that the eddy fluxes of potential tem- perature are directed downwards and polewards. The only significant dif- ference between the two regions is that ozone and temperature are negatively correlated. The later part of the study which was directed towards obtaining eddy diffusivities demonstrated several points. The first one is that one can- not use the eddy flux equation to get the eddy diffusivities without running into serious difficulties with singularities. Secondly, the daily varia- tion of the fluxes is so large that one needs at least 300 samples in a particular timespan of averaging in order to reduce the uncertainty of an average to an acceptable level. The uncertainty has a tendency to mask any relation between Kyy and the meridional EKE. Several approaches of finding the time scale relating the meridional EKE and Kyy were tried. The first method involved the finding of the typical advective timescale due to all the waves. The second method used Taylor's dispersion theorem to calculate the LaGrangian integral timescale. The model's Eulerian variables were transformed to LaGrangian ones via a Hays and Pasquill (1959) type transformation specifically derived for Rossby waves. The first method gave Kyy eddy diffusivities that compared favorably -58- with the Gudiksen et al. (1968) values. The timescales found from both methods compared favorably with those of Murgatroyd (1969b). A longer averaging period is needed in order to make a good estimate of the Lagrangian integral timescale for the whole atmosphere. By using the <a>, <a2 >, the <v2 > and the T from the model it seems quite possible for one to calculate meaningful eddy diffusivities. -59ACKNOWLEDGEMENTS The author would like to acknowledge the helpful discussions that he had with Derek Cunnold and Fred Alyea. He would also like to acknow- ledge the patient and helpful editing of this thesis by his advisor, Professor Ron Prinn. A special acknowledgement should go to the author's wife, Layla, who put up with the long sessions he spent with the computer. supported by a research assistantship under Grant No. rQ The author was 4 ASA -60- APPENDIX Equation (10.1) can be expressed in the form k b - - A (1 -ic (A. 1) where AY <V'*> C'C CC(AL- ( V M The uncertainty of (A.1) can be expressed by taking logarithms of (A.1) and then differentiating, leaving = _ The uncertainty, 6(B + CD), 6B and 6CD. t CD) (A.2) can further be simplified if broken up onto The two uncertainties are simply additive. 6CD can be written as 6CD = CD(6C/C + 6D/D). The uncertainty By combining these results and substituting into (A.2) one arrives at the result I Sk~ (Ct~~Zf(t~t ii (A.3) -61- The uncertainty of the derivatives are calculated by assuming a centered finite difference approximation that makes the uncertainty 6( ) = 2-6<Q>/DN, where DN = DPHI, DZ, etc. Given A, B, C, D and the uncertainties of the type in Table 1, the uncertainty 6Kyy can be calculated. -62References Barnes, A. A., Jr., 1962: Kinetic and potential energy between 100 mb and 10 mb during the first six months of the IGY. Final Report, Department of Meteorology, Massachusetts Institute of Technology, 8-131. ClAP Monograph 1, 1974: The natural stratosphere of 1974. Transportation final report, DOT-TST-75-51. Department of Corrsin, S., 1974: Limitations of gradient transport models in random walks and in turbulence. Advances in Geophysics, 18a, 25-60. Cunnold, D., F. Alyea, N. Phillips, and R. Prinn, 1975: A three-dimensional dynamical-chemical model of atmospheric ozone. 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White, 1951: A hemispherical study of the atmospheric angular momentum balance. Quart. J. Roy. Met. Soc., 77, 215-225. -65- S'tebbins, A. K., III, 1960: Progress report on the high altitude sampling program. DASA 532B, H.Q. Defence Atomic Support Agency. Stone, P. H., 1973: The effect of large-scale eddies on climatic change, J. Atmos. Sci., 30, 521-529. Taylor, G. I., 1921: Diffusion by continuous movements. Math. Soc., 20, 196. Proc. London White, R. M., 1954: The countergradient flux of sensible heat in the lower stratosphere. Tellus, 6, 177-179. Wilcox, R. W., G. D. Nastrom, and A. D. Belmont, 1977: Periodic variation of total ozone and its vertical distribution. J. Appl. Met., 7, 290-298. Van Loon, H., R. L. Jenne, and K. Labitzke, 1973: The zonal harmonic standing waves. J. Geophys. Res., 78, 4463-4471. T A B L 80*N V03 40*N 00 1.44E6±7.18E6 -8.29E7±4.86E7 -6.78E7±7.9.1E7 -2.71E7±2.23E8 -1.97E9±8.34E8 -1.03E9±1.07E9 400S -5.53E7±5.6E7 80*S -1.17E7±9.66E7 2.0E10±1.13E10 3.65E9±3.37E9 5.68E10±1.45E10 5.24E10±2.22E10 -1.21Ell±3.7E10 -2.85E11±1.04E11 3.91E9±3.19E10 -6.16E11±7.15Ell 3.74E12±8.36E12 -2.67E12±8.8E12 -3.43E12±8.60E12 -2.02E12±5.61E11 Vv 9.38±1.43 28.5±6.90 253±7.07 202±48. 7 60.6±20.4 4.37±.66 5.30±1.13 32.3±8.38 132±26.1 13.0±1.79 3.23±. 65 5. 96±.65 10.2±1.30 98. 8±17.0 35.3±5.33 11.9±2.11 221±29. 7 170±32.0 414±85.0 14.0±3.18 1.03E9±1.17E8 1.22E9±6.60E7 1.21E9±2.02E7 7.53E8±1.14E8 4.25E9±2.24E9 6.4E10±3.73E8 7.61E10±3.30E8 8.38E10±3.32E8 1.12E11±2.55E9 2.19E11±1.03E10 1.95E12±4.42E10 2.88E12±2.16E10 2.75E12 2.21E10 1.41E12±2.03E10 1.30E12±5.18E10 2.4E12±9.41E11 1.04E12±4.57E11 1.OE11±3.59Ell 1.41E12±3.15E11 4.18E12±1.28E12 03 -1.3E-4±1.2E-4 -6.2E-5±6.7E-5 -3.OE-6±4.6E-5 1.6E-4±1.6E-4 -8.9E-5±8.5E-5 -1.2E-4±1.3E-4 -1.2E-5±1.4E-4 1.1E-4±3.1E-4 1.lE-4±3.5E-4 -1.5E-4±1.8E-4 -7.7E-5±1.6E-4 -2.6E-5±1.lE-4 -5.8E-5±1.OE-4 -2.lE-5±3.9E-5 -4.8E-5±1.7E-4 -1.5E-4±2.7E-4 -6.6E-5±1.7E-4 1.OE-4±5.6E-5 -2.9E-5±1.lE-4 7.9E-4±1.7E-3 -67- Figure Captions 1. The phase relations as implied by observations. 2. The <V W > covariance from run 17 for the northern hemispheric winter. * * Units are 10 -2 2 -2 . m sec * * 3. The <V W > covariance from run 17 for the northern hemispheric spring. Units are 10 * * 4. # The <W -2 2 -2 m sec . > covariance from run 17 for the northern hemispheric winter. 3 -3 Units are m sec . * * 5. The <W $ > covariance from run 17 for the northern hemispheric spring. 3 3 Units are m sec . * * 6.. winter. * 22 2 2 -6 -2 m molecules cm sec . * 0 > covariance from run 17 for the norther hemispheric Units are 10 222 2 -6 -2 m molecules cm sec The <W V T T > covariance from run 17 for the northern hemispheric 1 2 2 -2 Units are 10 m K sec winter. * 9. * The <W V 0 spring. 8. * Units are 10 * 7. * The <W V 03 03 > covariance from run 17 for the northern hemispheric * * * The <W V T T > covariance from run 17 for the northern hemispheric -2 1l2 2 Units are 10 m *K sec . spring. * * 10. The <03 e > covariance from run 17 for the northern hemispheric winter. Units are 10 13molecules cm- 3K. * * 11. The <03 0 > covariance from run 17 for the northern hemispheric spring. Units are 101molecules cm K. 12. The area-weighted <VV> covariance from run 26 for the northern hemispheric month of June. 2 -2 Units are m sec 13. The area-weighted <V V > covariance from run 26 for the northern hemispheric month of June. 2 -2. Units are m sec -6814. The area-weighted <V'V'> covariance from run 26 for the northern hemispheric 2 -2 month of June; units are m -sec 15. The normalized variance spectrum of <V*V*> from run 26 at 40*S for the northern hemispheric month of June 16. The normalized variance spectrum of <V*V*> from run 26 at the equator for the northern hemispheric month of June 17. The normalized variance spectrum of <V*V*> from run 26 at 40*N the northern hemispheric month of June 18. The <V*V*> weighted zonal wavenumber from run 26 for the northern hemispheric month of June. 19. The phaseof the steady stationary zonal wavenumber 1 V* amplitude from run 26 for the northern hemispheric month of June 20. The same as 19 for zonal wavenumber 2 21. The same as 19 for zonal wavenumber 3 22. The area-weighted <W*W*> covariance form run 26 for the northern hemisphric month of June; units are 10 23. -6 2 -2 m sec The amplitude and phase history for days 450-480 of run 26 for the zonal wavenumber 1 meridional wind V* at 40*S and 12 mb. 24. The same as 23 for zonal wavenumber 3 25. The same as 23 for zonal wavenumber 5 26. The mixing slope <VW>/<VV> from run 26 for the northern hemispheric month of June; units are 10 4radians 27. The number density of ozone <0 3> from run 26 for the northern hemispheric month of June; units are 1011 molecules cm-3 28. The area-weighted <VO 3 > covariance from run 26 for the northern hemispheric month 29. of June; units are 10 11 m-molecules-cm-3sec-1 The total area weighted horizontal eddy flux of ozone for the 50-150 mb layer from run 26 for the northern hemispheric month of June; units are -6910 30. 11 -3sec -1 m-molecules-cm The area-weighted <V'O'> 3 covariance from run 26 for the northern hemispheric 11 month of June; units are 10 31. The area-weighted <V'0 3'> 11 34. 8 m molecules cm -3 sec -1 The area-weighted <W'0 3'> covariance from run 26 for the northern hemispheric month of June; units are 10 8 m molecules cm-3sec -1 The area-weighted <W*0 3*> covariance from run 26 for the northern hemispheric month of June; units are 10 35. -3 -l m molecules cm sec The area-weighted <WO 3> covariance from run 26 for the northern hemispheric month of June; units are 10 33. -3 -1 sec covariance from run 26 for the northern hemispheric month of June; units are 10 32. m-molecules-cm 8 m molecule cm -3 -1 sec The area-weighted <V*0*> covariance from run 26 for the northern hemispheric month of June; units are 101 m *K sec~1 36. The area-weighted <W*®*> covariance from run 26 for the northern hemispheric month of June; units are 10-2 m *K sec~1 37. The fractional contribution of each zonal wavenumber to the total meridional eddy ozone flux <V*0 3*> as a function of zonal wavenumber. The covariznce <V*0 3*> is from run 26 for the northern hemispheric month of June 38. Same as 37 39. The phase angle, y from run 26 for the northern hemispheric month of June, the units are 10-2 radians. 40. The phase difference in degrees between ozone and the meridional wind for the standing waves as a function of zonal wavenumber. The phase angles are from run 26 for the northern hemispheric month of June 41. Same as 40 42. The phase angles of IV*I and 103*1 for wavenumber 1 at 400 S and 12 mb -70- during the days 450-480 from run 26 for the northern hemispheric month of June; units are degrees 43. The same for wavenumber 2 44. The same for wavenumber 3 45. A plot of -<V*O*> versus <V*V*> [3<>/aD# + <a>3<0>/3z] 46. from The eddy diffusivity K yy -l 2 .4 units are 10 m sec 47. The eddy diffusivity K run 17 for the northern hemispheric winter; from run 17 for the northern hemispheric spring; 42 -l units are 10 m sec 48. The timescale T with C1 =2 m/sec from run 26 for the northern hemispheric month of June; units are 10 49. 4 sec the Eulerian-Langrangian conversion factor from run 26 for the northern hemispheric month of June, units-none. 50. The auto correlation coefficient R (t) vv for days 450-480 from run 26 at 400 S and 12 mb for the northern hemispheric month of June. 51. The Lagrangian integral time scale from run 26 for the northern hemispheric month of June; units are 101days. +1 50MB -STRATOSPHERE -1 P +1 500 MB -TROPOSPHERE -I WEST EAST PHASE ANGLE T i.-ure (RADIANS) ,. . 80N WINTER 40N 60N 20N 0 20S SUMMER 60S 40S 80S 0.05 70 0.1 60 0.2 0.5 50 1.0 E E 2 .0 40 5.0 10 30 20 50 20 100 200 I0 500 000 80N 60N 40N 20N 20S 0 LATITUDE figure 2. 40S 60S 80S SPRING 60N 40N 80N 0.05- ' 20N 0 i FA LL 40S 60S 20S I I I - I I I 80S I 70 -10 0.10.2- 60 0.550 1.02.0 E -40- L 5.0- n U 30 20- bJ 50- 20 100200-10 5001000 u 80N - -- 1.... 0 / 60N 40N ~0 - -\ 20S 20N LATITUDE f i;ure 3. ~ 40S 60S 80S 0 80N 0.05 1 WINTER 40N 60N 1 20S 0 20N SUMMER 60S 40S 80S -70 I- 0.1-60 0.2 0.5- -50 -5 E 2.0 0 -- 40 U5.0-0 -30 ( n10w a_, t 20-CLU 5U0- 2 500 1000 0I 80N i 60N 40N 1 -J - 1 20N 1 0 LATITUDE f ure 4. 20S 40S 60S 80S 0 80N SPRING 60N 40N 20N 0 20S FALL 40S 60S 0.05 80S -70 0.1 0.2 -60 0.5 -50 1.0. E 2.0 40 5.0 10 -30 20 50 20 100 20010 5001000 80N 60N 40N 20N 0 20S LATITUDE figure . 40S 60S 80S 0 WINTER 80N 60N I SUMMER 40N I , 20N 0 20S 40S 60S -70 -60 -50 E 0 0J 0 20S LATITUDE figure r . 80N 0.05 - SPRING 60N 40N FALL 20N 0 20S 40S 60S 80S -70 Q 0.1- 0.2 60 - 00 05 0 0 1.0 E 2.0 - -40 u 5.0 cl) 30 J20- 0 50 0 -- uJ 20 dI 100 2000 010 5001000 80N 60N 40N 20N - 0 20S LATITUDE f i t:u re 7. 40S i 60S 80S 0 80N WINTER 60N 40N 20N 20S SUMMER 60S 40S 0.05- -70 110 0.1- ( 0.2- 0.51.0- 80S -00 100 5 5 -10 ~60 -50 1 In5 E E 2.040 i 5.0r --30 S20- a: L 50~ 20 100200-10 500~ Is,- 0 I 1000 80N 60N 40N ~~~ 20N ~ 0 20 S LATITUDE f i gure . 1- ) 40S 60 S 80S 0 8ON SPRING 40N 60N 20S 0 20N FALL 60S 40S 80S 0.05- -70 \Y t o5 -5 0.I-1 0.2- 100 0 5 50 -60 0.51.0- 50 E 2.0-- -10 -. 0 5.0 50 5 - E 0 0 40- -5) cr-I 5 ~-- 10O 0 Cf) 120 82 AI0T0 50- 20 100- 00 200-0-1 500- 0iiI 8ON 60N 40N 20N 20S 0 LATITUDE f i u re '. 40S 60S 8S 0 WINTER 60N 40N 80N I 0.05- I I I. SUMMER 20N 40S 20S 60S 80S I I I -70 0.10.2- -60 0.5-50 1.0E2.0-. E -40 5.0- 0 10- 30F 2050- -20 100- 2005001000 - 10 ~ -0-. I 80N 2- <Z2 ____I I I 60N 40N I 0 0 ~ I 20N I 1 I~ I 0 20S LATITUDE I I 40S I I 60S I IL 80S 0 SPRING 60N 40N 80N 0.05- I I I I 20N FALL 40S 60S 20S I I I I I I I I 80S I I 70 0.10.2- -60 0 0.5-50 1.0E 2 .00 5.0 - 40 0 Dio-30 J 2050- -20 100- 7-044 *- c 20010 0 500- 1'~ ___ -~ 1000 -- I 80N I I 60N I I 40N I I 20N I I I I 0 20S LATITUDE figure 11. I I 40S J~ 60S 80S 0 ' O SOP S09 SO8 0o T ajnl--,!- 0 SO2 NO2 N09 NOV NO8 oo 00001 -009 01 ooog c oot,00 001 001 09 001 0 F,00_-02 ofU / 00 ~02-c -01m ~0 t 3 0, Z 3-O S 09- 0900 09- * -Foo~ 0 z SOB SO9 S OP SO2 0 NO2 NOp NO9 NO8 , SO8 I- - S O7 S09 I I I T S oz I I o jn c. - 0 I I NOt' NO2 I I NO9 I NOB I I0001 -009 01-OO -001 -09 -OZ m U) 02- OtP Ocn -01 m: - -0*l9 09-9'0 09-1'O I SO8 I I SO9 I I I SOt' I I SO2 I 0 I I I I * NO2 NOt? _ _ -90-0 I NO9 NO8 I 0.05- 80N 80N 60N 60N I UI I 40N 40N I Ii 20N 20N 20S 203 40S 40S 60S 60S 80S SOS -70 0.10.2- 60 10 0.5I 1.0- s- 10 -5 0 2.0 -L -40 0 Ll 5.0- D I0U -I30 - 20- LI L 50- -20 10020010 5001000 w o 80N 60N -I 40N 50I I 20N 0 LATITUDE figure 14. 20S 40S I I 60S I I 80S 0 40* De -6. .089mb .4 -mb 40 mb 132mb .2 S2 3 Zonol 4 Wavenumber figure 15 5 2 3 Zonal Wavenumber figure 1b. 4 5 .6- I mb .4- 13 12mb 2 - 40mb 2 3 Zonal 4 Wavenumber figure 17. u~j 80N 60N 40N 20N JUNE 0 20S 40S 60S 80S :D -70 z uJ -60 z 0 -50 Lu E 40 30 20 10 8ON 60N 40N 20N 0 20S LATITUDE figure 1.. 40S 60S 80S 0 PHASE OF V* ZONAL WAVENUMBER I. N.H.JUNE .06 :1 .2 40N :' *%% 8 0N EQ N. P(MB) 5 -. \ 40S 40N 40I..........0S.... 200N 200- \1 EQ .- 40 N -3 -2 -0 O RADIANS f ii.ure 12. PHASE OF V ZONAL WAVENUMBER 2. N.H. JUNE .06 .2 40N 40S P (MB) 80S 5 80N \EQ* 40 k N 40N 40S 8SS EQ 200 k \ -. B8N 40N -3 -2 -1 figure 20. 0 RADIANS I 2 3 PHASE OF V* ZONAL WAVENUMBER .06 3. N.H. JUNE 40N 64 - - I - .2 EQ 80N 80S 40S- P(MB) 5 4 N % 0N EQ 80.S 40 H 80N 404oS 40N 200 80N II. -3 -2 -I figure 21. 0 RADIANS 1 2 3 308e 309 St7 sO, U 0 NO0 N 0 t7 ",09 NU 000 1 009 01 -0 -001 009 -09 OZm (I) (n 02- 001~ 0909- o l'O 90*0 SO8 SO9 SOP SO2 0 NO2 NOV NO9 NOB 40* Winter Wavenumber I 5- -400* 4- <v I v-> m/sec 300 34 --- 2-200* %%- -00 Doys f i g-u re * 40* Winter Wavenumber 3 400* 8- 6- P \-300* <I V*l > m/sec 4 -200* <2- -L1000 I 5 lO 15 Days figure 24. 20 25 30 400 Winter 'Wawenumber 5 10 8 <1 V*I> m/sec 6 4 2 5 15 Days 0 fii Li re 20 25 30 80N 60N 40N 20N 20S 40S 60S 80S 0.05 .70 0.| 0.2 -60 0.5 .50 |.0 E E 2.0 40 5.0 10 30 20 50 20 100 200 I0 500 1000 8ON 60N 40N 20S 20 N I I ;ure ~ 40 S 60 S 80S 0 209 209 S20P O u 0 N0OF NOt& N09 NU9 0001 009 0z of 001 09 009 m 00 -Z m 0*9 0* 1 09g 09- £09 £09 0 £0 ? s OV N0Z NOV' N09 N08 80N 80N 0.05- 40N 40N 60N GON 20N 20N I 20S 20S I I I 40S 40S I 60S 60S 80S 805 70 0 .- 0.20.5- -60 ~/2 0 50 1.00 2.0 -{_ E 40 5.01I0-' 30 200-22 50- 20 0 100200- 55 - 0 5001000 I 80N I I 60N I I 40N I ~ I I I I 20N 20 S LATITUDE fi ure . I I 40S I I 60S I 80S 0 1.0 IV03) M-MOL CM SEC' 40S 40N EQ 0 -5- -1.0- f iure 2J. 0.05- 80N 80N I I 60N 60N I I 40N 40N 20N 20N I I I 20S 203 I I 40S 403 I a 60S 603 I I 80S 803 I 70 0.160 0.20.5- 50 1.0- 'O . 0 E 2.0-L 0 -40 5.01 0- -30 2050- -20 100200500000 10 -~-~0 N a 80N I I 60N 40N 20S 20N LATITUDE fir-ure 3 . I 40S I I 60S I I~ 80S 0 80N 60N 40N 20N 20S 0 40S 60S 80S 0.0 5- -7 0 0.1- 60 0.2 0.5-0 -50 1.0 E 2 .0 N -- 40 E 5.0 D1 0 - -3 0 2n 50 20- - 2 a-- 500-C 100000 80N 60N 40N 20N 20S 0 LATITUDE f i ure 1. 40S 60S 80S 0 C 80N 60N 40N 20N 0 20S 40S 60S 80S 70 0.05- 0.10.2- 0 0 60 0.5050 1.0- E E 2.0 -40 -5 5.0-.5 1 0IO 'O-0 3QD 30 cn. W20- wi -10 0 50- -20 100- 10 200- 1000 - 20 5 80N 60N 55 40N 20N 0 20S LATITUDE f i. ure 3 . 40S 60S 80S 0 60N 80N 40N 20N 0 20S 40S 80S 60S 0.05- -70 0.160 0.20.5 - -50 1.0E 2.0-_- -40 w 5.0D1 cn - 0 3 5 -30 0 ct 20 50 00 20000 0 5001000 80N 60N 40N 20S 0 20N LATITUDE i ure 33. I 40S I I 60S 0 I_ 80S E 80N 40N 60N 20N 40S 20S 60S 80S 0.05 70 0.1 0.2 \ _-----o 60 0,- 0.5 0 50 1.0 E p2.0 40 -0 10 30 ui 20 o~~~ 0 100 200 10 --------- 0 500 1000 0 80N 60N 40N 20N 20S 0 LATITUDE f igu re 314. 40S 60S 80S 0 S09 S OP I I 0 I I NOZ I I NOtp I i N09 I I NO8 I 0001 -009 01.. / -001 /i -09 -OZ m -Qc() -' OP m - -0* 1 09-9'0 09-rlO . SOB I SO9 I I ,I SOV SO 0 NOV NO2 I NO9 I NO9 SOB SO9 SO S0 SO17 *r i S ni fi ~z 0 N0Z S NOP I N09 I NOB I 0001 -~. -009 0 -001 -09 -OZ -01 m: O9v- -O'9m 09-90 091O - II I I I I a I I I II II II I N O2 Oo SO SO SO9 SOB . N Ot? I I I I -90,0 I I NO8 NO9 No09 NoOt' L'I ~rK~i4 ALTI 03 sol?- qwot ~II- , Jyi .5 soot, NoOt7 No08 s 0 08 qwZ21 N0 08 i~' c Jn2I 1' sIOotp 03 N0 017 S0 0 8 qwI TEFII -r No08 TTFT soot, No Ot' sooe qw - I 38 SO SO9 S ot s 0 02 NO& N9 NO 000 C 009 01 -O9z ~02- 00 cI 00 -A C-., 0*1-Z 09 ~ OL- .. SOB , SO9 S Otp SO2 NO2 0 NOV NO9 NO9 132 mb 80S 1 6 0 1 1 6 100'- 100- 100- 100- 8 ON 40N EQ. 40S IL I1 6 6 ulil 1 6 40 mb 8 0S EQ. 40S 80 I 40N 100- 1 6 1 6 1 6 fi:;u r~ 1 4r~~* 6 1 6 Tt ~JflKI4 IE -(9'01T .0 -~juT T 1 NO 1 0 8 lei q Lu 9 ti O 1 .1 Setn NO ti sod *qwJ T t~m 12 mb. 40' winter wavenumber 1 301- V ia1 Days f i gUre 42. 15 20 25 12 mib. 40'winter wavenumber 2 300 V 200-- 100 Days figure 43. 12 ib. 40' winter wavenumber 3 300- 200 - V 10 063 I I I | 5 10 15 20 Da ys figuro 44. 01 >i 1 9?3-Vl oIxg- oixg t7- 0I-' 0393G-N~ 09 02 £09 £09 sO ot 0sO ari GJi 0 NO0 N OP N09 N08 00 00 001 009 01 O0 i ~ -0 ~~001 cos- 099 099 (N? of____ - SOB SO9 S Op SO2 0 NO2 N OV NO9 NOB s09 £09 sO £t Oz 0 NQ0 N Ot? J N 08 oI 009 001 01 - 0 001 00 oo 001 ()0 09 01 F 0I -01 ......... 12 o .......... - 09 n. 001 -0*1 09 0001 01 SOe S O, SO9 SO2 0 N02 N OV NO9 NOB SO9 S09 i SO17 - 3l?1in'' 0 SOe I I sI NO2 I NOV I I N09 I I N08 I 0001 I I -009 0 1- 00Z 001 -09 -OZ c C/) -0-9 m OP cr -OI -9'0 09190 OIL - S08 SOe sot, £09 SO9 SO ot 0 SO~ SO2 O N09 NO9 NOP N OV NO~ N O2 N08 NO9 £09 £09 sot £OZ -G;oji nr i 0 NO0 N Ot N3D9 0 N0O CG, 1 -009 /1009 01 - 01c 7, -- O Bn n -01 /E02 090L / ( 09\~9P- 09SOB 0*0 0£ OP z0* 0ONP 9 SO9 O SO2 S 017 NO2 NOV N0 NO9 NO9 a 1.0 . . I1 -. Iu re 0 ~C)R £09 I sO t selO TC ir!l i~ GfiI-,-v7 N0 0 I I I I I I N OP I T N09 I - I I N09 I 0001 I I I -009 01 - -ooZ -001 -09 -O' m C/) -01ic x OP, - 0* 099*0 09'O OL - I SO9 SOe I I I I I I I I I 0 SOF, SO t I I I -90*0 I I NO9 NO9 N Ot? NO2