Quaternary Science Reviews 28 (2009) 1825–1830 Contents lists available at ScienceDirect Quaternary Science Reviews journal homepage: www.elsevier.com/locate/quascirev Rapid Communication The characterization and significance of a MIS 5a distal tephra on mainland Australia Sarah E. Coulter a, *, Chris S.M. Turney b, Peter Kershaw c, Susan Rule c a School of Geography, Archaeology and Palaeoecology, Queen’s University Belfast, 42 Fitzwillian Street, Belfast, UK School of Geography, Archaeology and Earth Resources, The University of Exeter, Exeter, UK c Department of Geography and Environmental Science, Monash University, VIC 3800, Australia b a r t i c l e i n f o a b s t r a c t Article history: Received 6 November 2008 Received in revised form 17 April 2009 Accepted 22 April 2009 Lynch’s Crater provides the main reference section for late Quaternary environmental change in northeast Australia. We have identified a cryptotephra horizon within late Marine Isotope Stage-5 (MIS-5) lake sediments obtained from the site. The major element geochemistry of this tephra has been compared with data from southwest Pacific sources, and our results indicate that the cryptotephra is most likely to be of Papuan origin. This is the first discovery of an aerially derived tephra in Australia that originated from outside the mainland. The Lynch’s Crater tephra is potentially an important marker horizon which could be used to connect disparate palaeoarchives at a time of significant climatic and environmental change. Ó 2009 Elsevier Ltd. All rights reserved. 1. Introduction The correlation and chronological control of widespread palaeoenvironmental records has been significantly advanced through the application of tephrochronology (Turney and Lowe, 2001). Distal sites may be linked by cryptotephras, layers of tephra generally consisting of particles of small size and/or low in concentration which are invisible to the naked eye (Lowe and Hunt, 2001; Gehrels et al., 2006). These layers (also known as microtephra horizons) may be identified thousands of kilometres from their source and can be used to precisely link disparate palaeoarchives. Tephrostratigraphies have been developed for many parts of the world (e.g. Davies et al., 2002; Newnham et al., 2003; Turney et al., 2004; Aoki and Machida, 2006; Shane et al., 2006) but detailed studies have not yet been developed for the Australian continent, in spite of experiencing a long history of volcanism (Johnson, 1989). Importantly, Australia’s eastern and northern margins are fringed by multiple island and continental arc systems that may also be a source of volcanic ash. The identification of both distal and local tephras could prove invaluable for linking scarce and discontinuous palaeoarchives in Australia and further afield. * Corresponding author. Tel.: þ44 02890975153; fax: þ44 028 9097 3897. E-mail addresses: sarah.coulter@qub.ac.uk (S.E. Coulter), c.turney@exeter.ac.uk (C.S.M. Turney), peter.kershaw@arts.monash.edu.au (S. Rule). 0277-3791/$ – see front matter Ó 2009 Elsevier Ltd. All rights reserved. doi:10.1016/j.quascirev.2009.04.018 The Atherton Tableland, northeast Queensland, is one region in Australia known to have been volcanically active during the late Quaternary. The Tableland lies towards the northern end of a long chain of igneous provinces which run approximately north–south over w4400 km, stretching from the Torres Strait to Tasmania (Finn et al., 2005). At a general level, it belongs to the ‘lava fields’ volcanic group first categorised by Wellman and McDougall (1974) as an extensive basaltic area associated with lava and scoria cones, maars and shield volcanoes (Fig. 1a). In north Queensland, Atherton is the only province in which maar volcanism has occurred, most probably facilitated by high precipitation and groundwater levels (Stephenson, 1989). Maar formation and subsequent infilling has provided an opportunity to develop a series of high-resolution palaeoenvironmental and climatic reconstructions for the late Quaternary (e.g. Kershaw et al., 1991; Kershaw, 1994; Hope et al., 2004; Haberle, 2005). Lynch’s Crater is a volcanic maar situated in the southeastern sector of the Atherton Tableland (Fig. 1b). Continuous accumulation of lake and swamp sediments at this site since its formation c. 230,000 years ago, provides an opportunity to place tephra layers within the main reference section for late Quaternary environmental change in northeastern Australia (Kershaw et al., 2007). The uppermost 20 m of the sequence (representing approximately the last 100,000 years) were recovered in 2003 before extraction of the full record in 2004. These 20 m were investigated for the presence of tephra and the findings from this study are reported here (Coulter, 2007). 1826 S.E. Coulter et al. / Quaternary Science Reviews 28 (2009) 1825–1830 Fig. 1. (a) Northeast Queensland Lava Field provinces, from Stephenson et al. (1980) reproduced with permission of the Geological Society of Australia, Queensland Division; (b) the location of Lynch’s Crater on the Atherton Tableland, Australia. 2. Lynch’s Crater and the regional setting Lynch’s Crater (17 370 S, 145 700 E) is located in the wet tropics of Australia at an altitude of 760 m above sea level (Fig. 1b) and experiences a rainfall of about 2500 mm/a and a mean annual temperature of w20.4 C (Busby, 1991). It is approximately circular in shape with a maximum width of w850 m. The region lies at the southern limit of summer monsoon penetration across northern Australia, experiencing both northwesterly and southeast trade winds (Kershaw, 1994). North–south trending mountain ranges border the western and eastern margins of the Atherton Tableland which is situated on a steep precipitation gradient; rainfall varies from 4000 mm/a at the coast to 1500 mm/a between 20 and 60 km inland (Kershaw et al., 1993). The region is drained by the Baron, Mulgrave and Russell rivers, which discharge into the Coral Sea (Kershaw et al., 1993). In 2004, funding from The National Geographic allowed drilling of the complete sedimentary sequence, providing the opportunity to undertake a comprehensive multi-proxy analysis. A full pollen record is now available for this 64 m long archive (Kershaw et al., 2007) and has been placed within an age model constructed through correlation to the SPECMAP marine isotope stratigraphy (Martinson et al., 1987) and ODP site-820 from the adjacent Coral Sea (Peerdeman et al., 1993; Moss and Kershaw, 2000). then prepared for geochemical analysis using the acid digestion method described by Dugmore et al. (1995) followed by flotation and alkali treatment using 10% KOH (Rose et al., 1996). Tephra-rich samples were embedded in araldite, course-ground and polished using 12 mm aluminium oxide powder and 1 mm diamond paste, respectively. Tephra major element concentrations were analysed on the Cameca SX-100 electron microprobe at the Tephrochronology Analytical Unit, University of Edinburgh. Two operating conditions were applied during wavelength dispersive analysis: (1) 15 kV, 5 nA, 5 mm beam diameter; and (2) 10 kV, 10 nA and 5 mm beam diameter. Due to the scarcity of glass shards recovered, their size and vesicle-rich nature, analyses with totals >94% were accepted. 4. Results and discussion Few shards were recorded through most of the sequence but significant quantities of tephra were found at 1877 cm (w60 shards per cm3 of wet sediment) and 1899 cm (w53 shards per cm3 of wet sediment). The tephra horizon at 1877 cm (henceforth described as LY 1877) consisted of small (40–60 mm), clear-pink tephra shards with exceptionally thin walls and prominent vesicles. Unfortunately, there were insufficient shards within the 1899 cm horizon for geochemical characterization. 3. Materials and methods 4.1. LY 1877 tephra age determination A truck-mounted drill rig was used to extract a 20 m core from a central location within Lynch’s Crater in 2003. The following treatments were used to concentrate tephra contained within the cored sediments for optical identification: loss-on-ignition, 10% HCl digestion and sieving. The residues were placed on a glass slide and analysed under an optical microscope at 400 magnification. Glass shards were found within the older sediments at 1876–1880 cm and 1899–1903 cm. Flotation, using sodium polytungstate with a density of 2.25 g/cm3 (Eden et al., 1992; Turney, 1998; Blockley et al., 2005), was used to remove high concentrations of biogenic silica in the flot and help to isolate the shards in these sections. Samples of peak concentration within a single centimetre were An approximate age for the LY 1877 tephra was estimated through comparison with the age model developed by Kershaw et al. (2007) for the complete sequence (Fig. 2). Loss-on-ignition profiles for both records were found to be identical. The tephra is located just below the transition between MIS-5 and -4, marked by a decrease in precipitation inferred from the dryland pollen signature and sediment stratigraphy, which shows a shift from lake sediments to swamp conditions (Kershaw et al., 2007). Lake levels appear to have fallen at this time and swamp conditions became reestablished; the inwash of inorganic sediment into the lake centre was significantly reduced. This transition is found at w17.4 m in the S.E. Coulter et al. / Quaternary Science Reviews 28 (2009) 1825–1830 1827 Fig. 2. (a) Stratigraphy and Loss-on-Ignition for the Lynch’s Crater 20 m core; (b) Loss-on-Ignition and age model for the 64 m core (Kershaw et al., 2007). 20 m core and at w23 m in the 64 m core (Fig. 2). A tentative correlation between the two records suggests an age of between 75,000 and 90,000 years for the LY 1877 tephra (Coulter, 2007). A MIS-5a age is demonstrated for pollen samples within this part of the sequence by a distinctive assemblage that includes high values for rainforest taxa such as Oraniopsis and Dacrydium in combination with low sclerophyll representation. Together these indicate rainfall as high as that in the present interglacial but temperatures that were several degrees lower than today. 4.2. Geochemistry and source of the Lynch’s Crater tephra Geochemical analyses on single glass shards from LY 1877 are presented in Table 1. This tephra has a rhyolitic composition and Table 1 Major element compositional data (un-normalized) expressed as weight % for (a) twelve analyses on eight individual glass shards within sample LY 1877. Standard analyses are reported in Appendix 1. (b) tephra bed 311.2 from the New Ireland basin (Horz et al., 2004). Total iron is calculated as FeO. (c) Cameca SX-100 electron microprobe conditions used during analysis of LY 1877 single glass shards. a LY 1877 SiO2 Al2O3 TiO2 FeO MnO MgO CaO Na2O K2O P2O5 Total A B C D E F G H I J K L Mean 73.92 73.55 74.21 74.21 74.42 74.66 73.60 74.41 74.04 75.03 74.49 76.35 74.41 0.74 11.49 11.60 11.16 11.30 11.18 11.10 11.49 11.61 12.34 12.03 12.21 11.54 11.59 0.41 0.23 0.25 0.27 0.26 0.25 0.29 0.29 0.19 0.23 0.27 0.24 0.25 0.25 0.03 1.34 1.49 1.57 1.49 1.48 1.47 1.59 1.81 1.79 1.96 1.96 1.42 1.61 0.21 0.02 0.10 0.03 0.10 0.10 0.02 0.09 0.06 0.07 0.12 0.12 0.03 0.06 0.05 0.34 0.35 0.31 0.32 0.34 0.34 0.34 0.34 0.47 0.46 0.45 0.31 0.36 0.06 2.01 2.01 1.92 1.98 1.82 1.98 1.92 2.02 2.37 2.23 2.43 1.83 2.04 0.20 3.92 3.81 3.99 3.96 3.67 4.05 3.61 3.39 2.44 2.03 1.94 1.76 3.21 0.90 1.39 1.43 1.34 1.36 1.39 1.28 1.50 1.48 1.15 1.15 1.13 1.18 1.31 0.14 0.06 0.05 0.00 0.05 0.06 0.06 0.05 0.00 0.08 0.07 0.11 0.05 0.05 0.03 94.70 94.64 94.80 95.02 94.69 95.23 94.48 95.31 95.00 95.35 95.05 94.72 94.91 0.28 75.97 0.89 11.72 0.14 0.25 0.02 1.59 0.05 0.08 0.02 0.33 0.02 1.91 0.18 3.82 0.13 1.37 0.04 0.09 0.02 97.13 0.97 s b 311.2 tephra (n ¼ 22) Mean s c Tephra shards A–G H–L Electron microprobe operating conditions 5 mm beam, 10 nA, 10 kV 5 mm beam, 5 nA, 15 kV 1828 S.E. Coulter et al. / Quaternary Science Reviews 28 (2009) 1825–1830 Fig. 3. Biplots of (a) CaO, K2O; (b) SiO2, Al2O3; (c) Na2O, MgO; (d) FeO, TiO2; and (e) Na2O þ K2O, SiO2 (%) for the Lynch’s Crater tephra and southwest Pacific source rocks and tephras. Important source locations are shown in (f). Bulk sample XRF and ICP-AES compositional data for southwest Pacific volcanics from: Lowder and Carmichael (1970), Smith (1976), Johnson and Chappell (1979), Wood et al. (1995), Polvé et al. (1997), Turner et al. (1997), Elburg and Foden (1998), Honthaas et al. (1999), Abdullah et al. (2000), Smith et al. (2003), Paulick et al. (2004), Reubi and Nicholls (2004). Glass electron microprobe analyses from: Whitford et al. (1977), each point represents an average of multiple electron microprobe analyses: Lowe (1988), Shane et al. (1995), Eden and Froggatt (1996), Newnham et al. (1998), Lowe et al. (1999), Pattan et al. (1999), Shane (2000), Alloway et al. (2004), Horz et al. (2004). S.E. Coulter et al. / Quaternary Science Reviews 28 (2009) 1825–1830 shards did not contain visible crystal inclusions. The major oxide values have been normalized, with SiO2 values averaging 78.4%, with low FeO (w 1.7%) and Al2O3 (w12.2%). The combination of low CaO (1.9–2.6%) and K2O (1.2–1.6%) concentrations is a particularly unusual feature. The high silica content of this tephra is not consistent with locally derived material; bulk rock major and trace element analyses indicate that volcanic constituents in the northern Queensland volcanic provinces are generally of mafic composition (Stephenson et al., 1980; Stephenson and Chappell, 1989; O’Reilly and Zhang, 1995; Zhang et al., 2001). Four analyses (reported as I–L; Table 1) displayed notably low concentrations of Na2O. This is unlikely to be the result of analytical variation as the beam current (which if too high can lead to alkali mobilization) was set 5 nA lower during these analyses than the other shards analysed (Table 1c). No physical signs of weathering were detected under the light microscope. The shards, however, are exceptionally small and thin walled which would leave them vulnerable to chemical attack. It is therefore considered likely that these shards have been subject to minor chemical alteration rather than that they represent a different phase of the eruption. Many of the island arc systems that lie off the east coast of Australia are dominated by basaltic, basaltic–andesite, and dacitic volcanism; only late Holocene activity is known for the silicicproducing centres of Fiji and Vanuatu (Robin et al., 1994; Cronin et al., 2004). Alternative silica rich sources include: Indonesia, New Zealand, Papua New Guinea and the northern Kermadecs. Comparison of the geochemical data obtained from the Lynch’s Crater tephra with that published from these regions is displayed in Fig. 3a–e. In many areas, except New Zealand and parts of Indonesia, a lack of precise tephra characterization means that comparison between these source regions must be based on whole-rock XRF analyses rather than single shard geochemical analyses. It is clear that there is some overlap between the geochemistry of the New Zealand, Papua New Guinea, Indonesian tephra and LY 1877 (Fig. 3a–e). Only the Papua New Guinea data, however, is found to consistently overlap with the Lynch’s Crater tephra across all 8 major elements, including the distinctive K2O and CaO ratios (Fig. 3a). Correlation appears strongest between the Lynch’s Crater tephra and volcanic constituents of Rabaul (Wood et al., 1995), Sulu Range (Woodhead et al., 1998) and the submerged volcanic system PACMANUS (Paulick et al., 2004), as shown in Fig. 3f. Importantly, a tephra layer known as 311.2, one of several glass-rich layers identified within marine sediments in the New Ireland basin (Papua New Guinea), has been identified and described by Horz et al. (2004) (Core 17682, Fig. 3f), and is most closely matched with the LY 1877 tephra (Fig. 3a–e). The 311.2 tephra has been marine d18O dated to w70.4 ka (Bassinot et al., 1994; Horz et al., 2004). A Papua New Guinea source seems most likely for the Lynch’s Crater tephra (Fig. 3f). Although easterly winds generally dominate the Papuan region, northerly airflow predominates during the Australian Summer monsoon. Changes in the pervasive wind direction has previously been shown to significantly influence the concentration of tephra within the western Pacific e.g. Machida et al. (1996) in northern New Britain. If the above correlation is correct, this seems a likely scenario for the distribution of the LY 1877 tephra. We consider it highly likely that strengthened summer monsoon conditions are likely to have aided the deposition of tephra glass shards in northern Queensland. 5. Conclusions and wider significance The occurrence of an aerially derived tephra on the Australian mainland demonstrates that rhyolitic tephras in the western Pacific can be transported over several hundreds of kilometres and be preserved in tropical environments, providing a critical time- 1829 parallel marker horizon beyond the range of radiocarbon dating at a time of considerable environmental change in the latter part of MIS-5. A tephra with similar geochemical composition in the New Ireland basin implies that a large eruption (possibly of Papuan origin) may be responsible for this widespread deposit and could prove to be an important marker horizon across the west Pacific. Acknowledgements This research was carried out during a DEL-funded PhD studentship. The authors are grateful to the Research School of Earth Sciences, Australian National University, for the provision of the drilling-rig, and to Bill Anderson, Jonathan Brown, Heather Builth, Joanne Muller, Raphael Wust, Weiming Wang, and particularly the driller, Damien Kelleher, who helped with extraction of the sediment core used in this study. CSMT and PK gratefully acknowledge funding by The National Geographic for their support of this work. SEC thanks Phil Shane for useful discussions about southwestern Pacific tephras. Many thanks are due to David Steele, Peter Hill and Anthony Newton for their assistance with the use of the electron microprobe facility at the Tephrochronology Analytical Unit, University of Edinburgh. We are grateful to NERC for supporting access to this facility. Appendix 1. Supplementary information Supplementary data associated with this article can be found, in the online version, at doi:10.1016/j.quascirev.2009.04.018. 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